Sensitivity of Assimilated Tropical Tropospheric Ozone to the Meteorological Analyses
Tropical tropospheric ozone fields from two different experiments performed with an off-line ozone assimilation system developed in NASA's Data Assimilation Office (DAO) are examined. Assimilated ozone fields from the two experiments are compared with the collocated ozone profiles from the Southern Hemispheric Additional Ozonesondes (SHADOZ) network. Results are presented for 1998. The ozone assimilation system includes a chemistry-transport model, which uses analyzed winds from the Goddard Earth Observing System (GEOS) Data Assimilation System (DAS). The two experiments use wind fields from different versions of GEOS DAS: an operational version of the GEOS-2 system and a prototype of the GEOS-4 system. While both versions of the DAS utilize the Physical-space Statistical Analysis System and use comparable observations, they use entirely different general circulation models and data insertion techniques. The shape of the annual-mean vertical profile of the assimilated ozone fields is sensitive to the meteorological analyses, with the GEOS-4-based ozone being closest to the observations. This indicates that the resolved transport in GEOS-4 is more realistic than in GEOS-2. Remaining uncertainties include quantification of the representation of sub-grid-scale processes in the transport calculations, which plays an important role in the locations and seasons where convection dominates the transport.