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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
NASA NTRSDate not supplied

SHERLOC: Results of the first 350 sols of operations

On February 18th 2021, the Perseverance rover landed in Jezero crater, Mars. This site was chosen because orbiter data analysis provides evidence that the crater hosted a stream-fed lake during the Martian Noachian period. The Octavia Butler landing site is located ~1.9 km east of the remnants of a river delta. Deltaic and lacustrine sediments can preserve biosignatures, making Jezero crater a prime target for Mars sample return science. One of the seven instruments on Perseverance’s science payload is SHERLOC –Scanning Habitable Environments with Raman and Luminescence for Organics and Chemicals. SHERLOC combines fluorescence and Raman spectroscopy with microscopic imaging to analyze surface material to better understand the history of the aqueous environments recorded in the rocks of Jezero crater and to search for potential biosignatures. SHERLOC imaging obtains high spatial resolution images of geological targets to identify grain-scale structure and texture. SHERLOC spectroscopy enables high-sensitivity detection, characterization, and spatially resolved correlation of trace organic materials. Native fluorescence emissions from aromatic organic species allow for detection and classification of aromatic organic molecules, whereas Raman scattered photons from molecules allow identification of functional groups of organics, chemicals, and minerals. In the first 300 sols, SHERLOC has analyzed 3 natural surfaces, and 5 abraded rock patches created during the Crater Floor Campaign within Jezero crater. SHERLOC has been able to identify phosphates, amorphous/microcrystalline silicate (AMS), olivine, sulfates, and carbonates in abraded patches in the green zone campaign within Jezero Crater Máaz and Séítah formations. Within these detections we have begun to tell the story of what this crater was like when it was full of liquid water over 3 billion years ago. In each of these samples we have identified fluorescence features that are likely aromatic organics native to the rock interiors. We have identified multiple unique fluorescence signatures, within each of the abraded patches. The organic signatures have either been widely distributed over an extended area, which is probably due to planetary wide dust, or have spatially resolved locations that are collocated with different mineral signatures. Note: Additional information available on attachment.

L. W. Beegle↗
NASA NTRS2023

Optimizing the Resolution of Hydrodynamic Simulations for MCRaT Radiative Transfer Calculations

Despite their discovery about half a century ago, the Gamma-ray burst (GRB) prompt emission mechanism is still not well understood. Theoretical modeling of the prompt emission has advanced considerably due to new computational tools and techniques. One such tool is the PLUTO hydro dynamics code, which is used to numerically simulate GRB outflows. PLUTO uses Adaptive Mesh Refinement to focus computational efforts on the portion of the grid that contains the simulated jet. Another tool is the Monte Carlo Radiation Transfer (MCRaT) code, which predicts electromagnetic signatures of GRBs by conducting photon scatterings within a jet using PLUTO. The effects of the underlying resolution of a PLUTO simulation with respect to MCRaT post-processing radiative transfer results have not yet been quantified. We analyze an analytic spherical outflow and a hydrodynamically simulated GRB jet with MCRaT at varying spatial and temporal resolutions and quantify how decreasing both resolutions affect the resulting mock observations. We find that changing the spatial resolution changes the hydrodynamic properties of the jet, which directly affect the MCRaT mock observable peak energies. We also find that decreasing the temporal resolution artificially decreases the high energy slope of the mock observed spectrum, which increases both the spectral peak energy and the luminosity. We show that the effects are additive when both spatial and temporal resolutions are modified. Our results allow us to understand how decreased hydrodynamic temporal and spatial resolutions affect the results of post-processing radiative transfer calculations, allowing for the optimization of hydrodynamic simulations for radiative transfer codes.

Jose Arita-Escalante↗
DOE OSTI2026

Improvements to In-Canal Assay of High Specific Activity 60Co at the ATR

Improvements to the quality of measurements in the assaying of High Specific Activity (HSA) cobalt 60 produced at the Advanced Test Reactor at the Idaho National Laboratory are presented. Such assays are conducted regularly between cycles at the ATR, and due to the radiological safety concerns, they are performed within the ATR canal. A standard ion chamber detector was placed in a collimated assay tube within the canal. Another tube, parallel to the detector, was used to position various cobalt 60 standards and targets. The collimated port between these tubes allows for the targets to be pulled across via a winch system. Previous measurements were performed at discrete 1.5-inch steps using a hand-cranked winch system. Charge was collected and integrated for 10 seconds at each discrete step during a scan. Two substantial improvements to the assay include an electronically controlled, motor-driven winch system and a software controlled continuous charge collection. Combined, these changes improved the quality of measurements as well as streamline the assay process. Further examination of these charge profiles indicated a reasonable amount of photon scattering, or shine, before a line-of-sight is established. This created inaccuracies in the reported activity of the cobalt targets. A series of MCNP-6.3 calculations were performed in an effort to quantify and correct for this shine effect. The results of the calculations and how they were employed to a create shine correction factor for the in-canal cobalt assay at the ATR are presented. The overall bias showed an overestimation of the HSA cobalt 60 activity by around 7-8%.

07 - ISOTOPES AND RADIATION SOURCES↗
NASA NTRS1982

Rayleigh, Raman and particulate scattering

Analysis of the visible and near infrared spectra of planetary atmospheres and the multiple scattering of photons within the atmosphere are discussed. Photons detected within the spectral region are solar photons which were scattered by the gas and particles in the planetary atmosphere. An example is given for the incident and emitted fluxes for a hypothetical planet with an effective temperature of 100 K. The absorption spectrum of the planetary atmosphere is discussed in terms of the various scattering processes photons undergo within the atmosphere. Three different physical processes are considered. Rayleigh scattering and Raman scattering by the gas molecules, and scattering by any cloud or dust aerosol particles in the atmosphere. The physics of each of these processes is examined.

Cochran, W. D.↗
NASA NTRS1986

Photon-deficient Compton scattering by nonthermal electrons - Comparison with gamma-ray burst spectra

The model of gamma-ray-burst spectra proposed by Zdziarski and Lamb (1986, 1987) is reviewed and compared with observed spectra. In the model, the spectrum arises from multiple Compton scatterings in a nonthermal source with a deficit of soft photons. The steady-state electron distribution in such a source is a nonthermal power law that joins at low energies onto a thermal distribution that may be either optically thick or thin. Both cases lead naturally to a two-component spectrum with a photon-energy index in the X-ray spectrum which is much less than one and a photon-energy index in the gamma-ray spectrum which is larger than the X-ray photon-energy index. Fits to the observed gamma-ray-burst spectra (where data exist for both X-ray and gamma-ray energies) show good agreement with the model.

Zdziarski, Andrzej A.↗
DOE OSTI2024

Open-Source Data Analysis Tool for Spectral Small-Angle X-ray Scattering Using Spectroscopic Photon-Counting Detector

Spectral small-angle X-ray scattering (sSAXS) is a powerful technique for material characterization from thicker samples by capturing elastic X-ray scattering data in angle- and energy-dispersive modes at small angles. This approach is enabled by the use of a 2D spectroscopic photon-counting detector that provides energy and position information of scattered photons when a sample is irradiated by a polychromatic X-ray beam. Here, we describe an open-source tool with a graphical interface for analyzing sSAXS data obtained from a 2D spectroscopic photon-counting detector with a large number of energy bins. The tool takes system geometry parameters and raw detector data to output 1D scattering patterns and a 2D spatially-resolved scattering map in the energy range of interest. We validated these features using data from samples of caffeine powder with well-known scattering peaks. This open-source tool will facilitate sSAXS data analysis for various material characterization applications.

Chemistry↗
DOE OSTI2021

Inelastic Scattering of a Photon by a Quantum Phase Slip

Spontaneous decay of a single photon is a notoriously inefficient process in nature irrespective of the frequency range. We report that a quantum phase-slip fluctuation in high-impedance superconducting waveguides can split a single incident microwave photon into a large number of lower-energy photons with a near unit probability. The underlying inelastic photon-photon interaction has no analogs in non-linear optics. Instead, the measured decay rates are explained without adjustable parameters in the framework of a new model of a quantum impurity in a Luttinger liquid. Our result connects circuit quantum electrodynamics to critical phenomena in two-dimensional boundary quantum field theories, important in the physics of strongly-correlated systems. Here, the photon lifetime data represents a rare example of verified and useful quantum many-body simulation.

1-dimensional systems↗
NASA NTRS2016

Cyclotron Resonant Scattering Feature Simulations I. Thermally Averaged Cyclotron Scattering Cross Sections, Mean Free Photon-Path Tables, and Electron Momentum Sampling

Electron cyclotron resonant scattering features (CRSFs) are observed as absorption-like lines in the spectra of X-ray pulsars. A significant fraction of the computing time for Monte Carlo simulations of these quantum mechanical features is spent on the calculation of the mean free path for each individual photon before scattering, since it involves a complex numerical integration over the scattering cross section and the (thermal) velocity distribution of the scattering electrons. We aim to numerically calculate interpolation tables which can be used in CRSF simulations to sample the mean free path of the scattering photon and the momentum of the scattering electron. The tables also contain all the information required for sampling the scattering electron's final spin. The tables were calculated using an adaptive Simpson integration scheme. The energy and angle grids were refined until a prescribed accuracy is reached. The tables are used by our simulation code to produce artificial CRSF spectra. The electron momenta sampled during these simulations were analyzed and justified using theoretically determined boundaries. We present a complete set of tables suited for mean free path calculations of Monte Carlo simulations of the cyclotron scattering process for conditions expected in typical X-ray pulsar accretion columns (0.01 B/B(sub crit) is less than or equal to 0.12, where B(sub crit) = 4.413 x 1013 G, and 3 keV kBT 15 keV). The sampling of the tables is chosen such that the results have an estimated relative error of at most 1/15 for all points in the grid. The tables are available online (see link in footnote, page 1).

Schwarm, F.-W.↗
DOE OSTI2023

Search for an axion-like particle with forward proton scattering in association with photon pairs at ATLAS

A search for forward proton scattering in association with light-by-light scattering mediated by an axion-like particle is presented, using the ATLAS Forward Proton spectrometer to detect scattered protons and the central ATLAS detector to detect pairs of outgoing photons. Proton-proton collision data recorded in 2017 at a centre-of-mass energy of $\sqrt{s}$ = 13 TeV were analysed, corresponding to an integrated luminosity of 14.6 fb –1 . A total of 441 candidate events were selected. A search was made for a narrow resonance in the diphoton mass distribution, corresponding to an axion-like particle (ALP) with mass in the range 150–1600 GeV. No excess is observed above a smooth background. Upper limits on the production cross section of a narrow resonance are set as a function of the mass, and are interpreted as upper limits on the ALP production coupling constant, assuming 100% decay branching ratio into a photon pair. The inferred upper limit on the coupling constant is in the range 0.04–0.09 TeV –1 at 95% confidence level.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS2012

Radiative Transfer Through Clouds and Its Applications in Support of the Ice, Cloud, and Land Elevation Satellite-2 (ICESat-2) Mission

The Greenland and Antarctic ice sheets, which contain enough ice to raise sea level by about 7 and 60 m, respectively, are losing mass at an increasing rate. To acquire continuous information of the cryosphere, after the Ice, Cloud, and land Elevation Satellite (ICESat) (2003-2010), NASA is actively planning for the ICESat-2 mission. Both ICESat and ICESat-2 are space-borne lidar altimetry systems. The systems measure the time of flight of the arriving photons that are reflected by the surface to deduce the elevation of the underlying terrain. As one of NASA's top priority missions, ICESat-2 is scheduled to launch in 2016. One of the major science goals of ICESat-2 is to quantify the ice sheet mass balance to determine its contributions to the sea level change and its impacts on ocean circulation (Abdalati et al. 2010). Compared to ICESat, which operates at 40 Hz and records the reflected laser energy as a waveform, the significantly improved ICESat-2 lidar employs a 532 nm micro-pulse photon counting system that operates at a high frequency of 10kHz with single photon detectability (Yang et al. 2012). To achieve its science goals, ICESat-2 requires the ability of detecting the elevation change with an accuracy of 0.2 cm/year over the entire ice sheet. Since every photon emitted by the lidar system will travel through the atmosphere, clouds can certainly affect the flight time of the arriving photons. Forward scattering by cloud particles increases the photon path length, thus resulting in biases in ice sheet elevation measurements known as atmospheric path delay (Duta et al. 2001, Yang et al. 2010, 2011). To ensure the accuracy of ICESat-2 surface elevation measurements, it is critical to understand how clouds would affect the travel time of arriving photons. In this talk, we will first present a framework that simulates the behavior of a space-borne 532 mn micro-pulse photon counting lidar in cloudy and clear atmospheres. To investigate the process of laser propagation through clouds, a 3-D Monte Carlo radiative transfer model is used to simulate the photon path distribution and the Poisson distribution is adopted for the number of photon returns. Since the photon counting system only registers the time of the first arriving photon within the detector "dead time", the retrieved average surface elevation tends to bias towards higher values. This is known as the first photon bias. With the scenarios simulated here, the first photon bias for clear sky is about 6.5 cm. Clouds affect surface altimetry in two ways: (1) cloud attenuation lowers the average number of arriving photons and hence reduces the first photon bias; (2) cloud forward scattering increases the photon path length and makes the surface appear further away from the satellite. Compared to clear sky, the average surface elevation detected by the photon counting system for cloudy sky with optical depth 1.0 is 4.0 to 6.0 cm lower for the simulations conducted. The effect of surface roughness on the accuracy of elevation retrievals will also discussed.

Yang, Yuekui↗
DOE OSTI2021

Quantum kinetics of anomalous and nonlinear Hall effects in topological semimetals

Highlights: • Linear and photogalvanic anomalous Hall responses are systematically derived. • Extrinsic mechanisms of AHE include Gaussian, diffractive, hybrid skew scattering. • Diagrammatic calculations are matched to semiclassical picture of AHE. • The Pancharatnam phase of multifold fermions determines the skew scattering amplitude. • Photon-induced interband scattering are accompanied by coordinate shifts. We present a systematic microscopic derivation of the semiclassical Boltzmann equation for band structures with the finite Berry curvature based on Keldysh technique of nonequilibrium systems. In the analysis, an AC electrical driving field is kept up to quadratic order, and both cases of small and large frequencies corresponding to intra- and interband transitions are considered. In particular, this formulation is suitable for the study of nonlinear Hall effect and photogalvanic phenomena. The role of impurity scattering is carefully addressed. Specifically, in addition to previously studied side-jump and skew-scattering processes, quantum interference diffractive contributions are now explicitly incorporated within the developed framework. This theory is applied to multifold fermions in topological semimetals, for which the generic formula for the skew scattering rate from the Pancharatnam phase is obtained along with the corresponding anomalous Hall conductivity.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Target normal single-spin asymmetry in inclusive electron-nucleon scattering with two-photon exchange: Analysis using 1/$N_c$ expansion

We calculate the target normal single-spin asymmetry caused by two-photon exchange in inclusive electron-nucleon scattering in the resonance region. Our analysis uses the 1/$N_c$ expansion of low-energy QCD and combines $\textit{N}$ and Δ intermediate and final states using the contracted $\textit{SU}$(4) spin-flavor symmetry. The normal spin asymmetry obtained in leading-order accuracy in 1/$N_c$ has magnitude ~10 -2 and different sign in $\textit{ep}$ and $\textit{en}$ scattering. It can be measured in electron scattering at lab energies ~0.5-1.5 GeV and provides a clean probe of two-photon exchange dynamics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS2002

Monte Carlo Radiative Transfer Modeling of Lightning Observed in Galileo Images of Jupiter

We study lightning on Jupiter and the clouds illuminated by the lightning using images taken by the Galileo orbiter. The Galileo images have a resolution of 25 km/pixel and axe able to resolve the shape of the single lightning spots in the images, which have full widths at half the maximum intensity in the range of 90-160 km. We compare the measured lightning flash images with simulated images produced by our ED Monte Carlo light-scattering model. The model calculates Monte Carlo scattering of photons in a ED opacity distribution. During each scattering event, light is partially absorbed. The new direction of the photon after scattering is chosen according to a Henyey-Greenstein phase function. An image from each direction is produced by accumulating photons emerging from the cloud in a small range (bins) of emission angles. Lightning bolts are modeled either as points or vertical lines. Our results suggest that some of the observed scattering patterns axe produced in a 3-D cloud rather than in a plane-parallel cloud layer. Lightning is estimated to occur at least as deep as the bottom of the expected water cloud. For the six cases studied, we find that the clouds above the lightning are optically thick (tau > 5). Jovian flashes are more regular and circular than the largest terrestrial flashes observed from space. On Jupiter there is nothing equivalent to the 30-40-km horizontal flashes which axe seen on Earth.

Dyudine, U. A.↗
DOE OSTI2021

Simulating dust grain-radiation coupling on a moving mesh

ABSTRACT We present a model for the interaction between dust and radiation fields in the radiation hydrodynamic code arepo-rt, which solves the moment-based radiative transfer equations on an unstructured moving mesh. Dust is directly treated using live simulation particles, each of which represent a population of grains that are coupled to hydrodynamic motion through a drag force. We introduce methods to calculate radiation pressure on and photon absorption by dust grains. By including a direct treatment of dust, we are able to calculate dust opacities and update radiation fields self-consistently based on the local dust distribution. This hybrid scheme coupling dust particles to an unstructured mesh for radiation is validated using several test problems with known analytic solutions, including dust driven via spherically symmetric flux from a constant luminosity source and photon absorption from radiation incident on a thin layer of dust. Our methods are compatible with the multifrequency scheme in arepo-rt, which treats UV, optical photons as single scattered and IR photons as multi scattered. At IR wavelengths, we model heating of and thermal emission from dust. Dust and gas are not assumed to be in local thermodynamic equilibrium but transfer energy through collisional exchange. We estimate dust temperatures by balancing these dust-radiation and dust-gas energy exchange rates. This framework for coupling dust and radiation can be applied in future radiation hydrodynamic simulations of galaxy formation.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Harnessing emergent multiple scattering resonances in a photonic glass structure for photoelectrochemical energy conversion

Light trapping nanostructures are often necessary to improve carrier collection yields in semiconductor photoelectrodes with intrinsically poor electron transport. Photonic crystal templates can generate tailorable light trapping via periodic and precise nanostructure, though this is not a scalable strategy for photoelectrochemical (PEC) applications. It is therefore critical to identify alternative mechanisms for light trapping that tolerate disorder. Light trapping in disordered media is generated by the diffusive transport caused by multiple scattering. In some cases, multiple scattering can generate resonances that resemble those observed in photonic crystals. While resonant multiple scattering is a disorder tolerant light trapping mechanism, it is unclear if the effect is sufficiently adaptable, or even useful, for PEC applications. Here, we describe a photonic omission glass, a nanostructure that can controllably induce resonances in multiple scattering transport. We characterized the emergence of these resonances after coating a disordered SiO 2 colloidal structure with a layer of TiO 2 , which functions both as dielectric contrast and as a light absorbing semiconductor. We show in finite element simulations and spectroscopic characterization that the resonant multiple scattering effect improves light trapping near the interface between the structure and the bulk electrolyte. This effect, coupled with the increased electrochemically active surface area, results in a hierarchically structured TiO 2 photoanode with orders of magnitude higher photocurrents compared to an equivalent planar photoanode for PEC reactions such as alkaline water oxidation. We show that controlling this resonant multiple scattering effect can be advantageous for improving PEC energy conversion in disordered photoelectrodes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1988

Scattering of sodium D photons by neutral gas in the planetary nebula BD +30 deg 3639

Observations of the planetary nebula BD +30 deg 3639 are presented. It is shown that the Na DS photons emitted by the central star of the nebula are scattered by a neutral circumnebular envelope. These observations demonstrate the utility of optical absorption lines as tracers of the neutral material associated with planetary nebulae.

Dinerstein, Harriet L.↗