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Aerosol Sampling Experiment on the International Space Station

The International Space Station (ISS) is a unique indoor environment which serves as both home and workplace to the astronaut crew. There is currently no particulate monitoring, although particulate matter requirements exist. An experiment to collect particles in the ISS cabin was conducted recently. Two different aerosol samplers were used for redundancy and to collect particles in two size ranges spanning from 10 nm to hundreds of micrometers. The Active Sampler is a battery operated thermophoretic sampler with an internal pump which draws in air and collects particles directly on a transmission electron microscope grid. This commercial-off-the-shelf device was modified for operation in low gravity. The Passive Sampler has five sampling surfaces which were exposed to air for different durations in order to collect at least one sample with an optimal quantity of particles for microscopy. These samples were returned to Earth for analysis with a variety of techniques to obtain long-term average concentrations and identify particle emission sources. Results are compared with the inventory of ISS aerosols which was created based on sparse data and the literature. The goal of the experiment is to obtain data on indoor aerosols on ISS for future particulate monitor design and development.

Aerosol

The Relationship Between MAIAC Smoke Plume Heights and Surface PM

Biomass burning is a source of fine particulate matter (PM2.5) air pollution, which adversely impacts human health. However, quantifying the health effects from biomass burning PM2.5 is difficult. Monitoring networks generally lack the spatial density needed to capture the heterogeneity of biomass burning smoke. Satellite aerosol optical depth (AOD) can be used to fill spatial gaps but does not distinguish surface‐level aerosols. Plume height (PH) observations may provide constraints on the vertical distribution of smoke and its impact on surface concentrations. We assessed PH characteristics from Multi‐Angle Implementation of Atmospheric Correction (MAIAC) and evaluated its correlation with colocated PM2.5 and AOD measurements. PH is generally highest over the western United States. The ratio PM2.5:AOD generally decreases with increasing PH:PBLH (planetary boundary layer height), showing that PH has the potential to refine surface PM2.5 estimates for collections of smoke events.

satellite retrieved smoke plume heights

Toward the Next Generation of Air Quality Monitoring Indicators

This paper introduces an initiative to bridge the state of scientific knowledge on air pollution with the needs of policymakers and stakeholders to design the "next generation" of air quality indicators. As a first step this initiative assesses current monitoring and modeling associated with a number of important pollutants with an eye toward identifying knowledge gaps and scientific needs that are a barrier to reducing air pollution impacts on human and ecosystem health across the globe. Four outdoor air pollutants were considered e particulate matter, ozone, mercury, and Persistent Organic Pollutants (POPs) e because of their clear adverse impacts on human and ecosystem health and because of the availability of baseline data for assessment for each. While other papers appearing in this issue will address each pollutant separately, this paper serves as a summary of the initiative and presents recommendations for needed investments to provide improved measurement, monitoring, and modeling data for policyrelevant indicators. The ultimate goal of this effort is to enable enhanced public policy responses to air pollution by linking improved data and measurement methods to decision-making through the development of indicators that can allow policymakers to better understand the impacts of air pollution and, along with source attribution based on modeling and measurements, facilitate improved policies to solve it. The development of indicators represents a crucial next step in this process.

Particulate matter

Life Cycle Emissions and Health Cost Impacts of Producing Ethanol and Electricity from Willow and Switchgrass in the Riparian Buffers of Mid-Atlantic United States

The United States (US Mid-Atlantic Region (MAR) has the potential to grow a variety of perennial feedstocks such as switchgrass and shrub willow to increase domestic energy production. These cellulosic feedstocks have also shown improved ecosystem services, such as soil carbon sequestration, nitrate leaching reduction, and flood mitigation along rivers and streams as partially harvested riparian buffers. To examine the effects on greenhouse gases (GHGs) and criteria air pollutants (CAPs) from using these feedstocks to produce ethanol or electricity, we conducted a comprehensive life cycle assessment (LCA) and estimated the impact on human health costs when land use is changed from corn production for ethanol. Results indicate up to 54% reduced GHG per hectare from using willow and switchgrass feedstock sources to produce ethanol instead of corn. However, there was a trade-off in terms of CAP emission, as grass-based energy emitted more NO x and SO x compared to the corn ethanol pathway, except for SO X emissions from willow-based electricity. Electricity from cellulosic biomass had higher particulate matter (PM) emission compared to that from corn ethanol. Estimates for health cost to society ranged from $2498 ha –1 for electricity from switchgrass to a net benefit of $448 ha –1 for ethanol production from willow, depending on varying biomass yield under different market scenarios. Although using cellulosic feedstocks to produce bioenergy has great potential to reduce GHG emissions, CAP control measures are needed to manage CAP-induced health costs.

Bioenergy

CROCUS Air Quality Data at University of Illinois - Chicago Tower

The AQT (Vaisala AQT530) instrument provides observations on meteorological conditions, including particulate matter (PM2.5, PM10), gas species concentrations (NO, NO2, O3, CO), and environment temperature and moisture. These measurements are critical for understanding air quality. These measurements are useful for understanding changes in aerosol properties, air quality research, and comparing to model experiments especially in urban environments. These measurements are collected at the University of Illinois in Chicago, Illinois, on the meteorological tower near the greenhouse on campus. Data is available in the netCDF data format, we encourage data users review documentation through Project Pythia to understand how to work with netCDF data https://foundations.projectpythia.org/core/data-formats/netcdf-cf.html. Each file contains one day's worth of data (24 hours, starting at 0000 UTC). File naming convention includes the project (CROCUS), location (UIC), data level (raw, a1), date (year, month, day), and hour (0000).

54 ENVIRONMENTAL SCIENCES

A Network of Field-Calibrated Low-Cost Sensor Measurements of PM2.5 in Lomé, Togo, Over One to Two Years

Air pollution is a leading cause of global premature mortality and is especially prevalent in many low- and middle-income countries (LMICs). In sub-Saharan Africa, preliminary monitoring networks, satellite retrievals of air-quality-relevant species, and air quality models show ambient fine particulate matter (PM 2.5 ) concentrations that far exceed the World Health Organization guidelines, yet many areas remain largely unmonitored and understudied. Deploying a network of five low-cost PurpleAir PM 2.5 monitors over 2 years (2019–2021), we present the first multiyear ambient air pollution monitoring data results from Lomé, Togo, a major West African coastal city with a population of about 1.4 million people. The full-study time period network-wide mean measured daily PM 2.5 concentration is 23.5 μ g m –3 m –3 . The strong regional influence of the dry and dusty Harmattan wind increases the local average PM 2.5 concentration by up to 58% during December through February, but the diurnal and weekly trends in PM 2.5 are largely controlled by local influences. At all sites, more than 87% of measured days exceeded the new WHO Daily PM 2.5 guidelines; these first measurements highlight the need for air quality improvement in a rapidly growing urban metropolis.

air pollution

CROCUS Low Cost All-in-One Weather Station AMB-001 Data Argonne National Laboratory Prairie Site

The Ambient Weather WS-2902D (AMB) is a low cost weather station that has become very useful for filling data gaps in harder to deploy locations. These low cost weather stations collect 13 second data, which is averaged to a five minute data output available to users through an API key. The data files contain measurements for precipitation, temperature, wind chill/heat index, relative humidity, dew point, UV index, solar radiation, wind speed, wind direction, wind gust, and with an external particulate matter 2.5 (PM 2.5) sensor. Having all of these measurements in one condense system allows for fast deploying and dense network capabilities. Three of the AMB weather stations were deployed at the Argonne Testbed for Multiscale Observational Science (ATMOS), a 20-acre prairie site at Argonne National Laboratory in Lemont, Illinois. The instruments are denoted by their three digit identifier (CMS-AMB-xxx) format. The data is presented as daily NetCDF (.nc) files, each containing approximately 24 hours of observations. Files follow the naming convention of: the project (CROCUS), location (atmos), instrument name (CMS-AMB-001), data level (raw, a1), and date (year, month, day). The NetCDF format can be accessed using common scientific software such as Python using xarray, netCDF4 or ACT-DOE.

54 ENVIRONMENTAL SCIENCES

CROCUS Low Cost All-in-One Weather Station AMB-004 Data Argonne National Laboratory Prairie Site

The Ambient Weather WS-2902D (AMB) is a low cost weather station that has become very useful for filling data gaps in harder to deploy locations. These low cost weather stations collect 13 second data, which is averaged to a five minute data output available to users through an Application Programming Interface (API) key. The data files contain measurements for precipitation, temperature, wind chill/heat index, relative humidity, dew point, UV index, solar radiation, wind speed, wind direction, wind gust, and with an external particulate matter 2.5 (PM 2.5) sensor. Having all of these measurements in one condense system allows for fast deploying and dense network capabilities. Three of the AMB weather stations were deployed at the Argonne Testbed for Multiscale Observational Science (ATMOS), a 20-acre prairie site at Argonne National Laboratory in Lemont, Illinois. The instruments are denoted by their three digit identifier (CMS-AMB-xxx) format. The data is presented as daily NetCDF (.nc) files, each containing approximately 24 hours of observations. Files follow the naming convention of: the project (CROCUS), location (atmos), instrument name (CMS-AMB-004), data level (raw, a1), and date (year, month, day). The NetCDF format can be accessed using common scientific software such as Python using xarray, netCDF4 or ACT-DOE.

EARTH SCIENCE > ATMOSPHERE > AEROSOLS > PARTICULAT

Two decades of aerosol trends over India: seasonal characteristics and urban-rural dynamics

Abstract India faces significant air quality challenges, with one of the highest air pollution levels of any country in the world. Here, we examine two decades (2001–2019) of both particulate matter (PM 2.5 ) concentration and aerosol optical depth (AOD) over the country. Increases are seen between the two decadal averages, for 2001–2010 and 2011–2019, in western India, particularly in the Indo-Gangetic Plain (IGP). IGP region, including Bihar, West Bengal, Jharkhand, and Uttar Pradesh, shows the highest increases in AOD (+0.03, 13%) and PM 2.5, s (+8 µ g m −3 ). Seasonal AOD patterns fluctuate, with the IGP experiencing the highest wintertime increase, especially in Bihar (+0.07). In summer, there are increases in AOD along the southern and eastern coastal areas. Monsoons cause a slight rise in AOD, except in Rajasthan. In the post-monsoon season, the IGP experiences a notable increase in AOD (+0.057, 25%), potentially driven by biomass burning in Bihar (+0.11) and Uttar Pradesh (+0.075). Dividing our study area into urban and peri-urban clusters ( n = 2791), AOD is found to be similar, possibly due to advective mixing. However, the differences between urban and rural areas become more noticeable, especially in the second decade. Correlations between AOD and PM 2.5, g vary across locations, with the highest found in Kanpur ( R 2 = 0.61) and weaker in Delhi ( R 2 = 0.42), highlighting the need for more ground monitoring. However, it suggests that satellite-derived AOD can generally be used to examine trends in PM 2.5 over longer time frames.

54 ENVIRONMENTAL SCIENCES

Assessment of the Impact of Discontinuity in Satellite Instruments and Retrievals on Global PM2.5

Exposure to fine particulate matter (PM2.5) is the leading environmental risk factor for mortality globally. Satellite-derived estimates of surface PM2.5 developed from a combination of satellites, simulations, and ground monitor data are relied upon for health impact studies. The ability to develop satellite-derived PM2.5 estimates requires the continued availability of aerosol optical depth (AOD) sources. This work examines the impact of the addition or loss of satellite AOD data sources on global PM2.5 estimation and the impact of continuing the longterm record with AOD from the Visible Infrared Imaging Radiometer Suite (VIIRS) on the Suomi-National Polar orbiting Partnership (S-NPP) satellite after the loss of the MODIS (MODerate resolution Imaging Spectroradiometer) and MISR (Multi-angle Imaging Spectroradiometer) instruments on board the Terra and Aqua satellites. We find that the addition of VIIRS S-NPP AOD products to geophysical PM2.5 estimates from satellites and simulations causes regional differences that correspond to differences in the VIIRS and MODIS Deep Blue AOD algorithms and sampling. Changes in long-term trends and timeseries due to the addition or loss of AOD data sources are generally within their uncertainties. Statistical fusion with ground monitor data partially corrects for changes due to sampling differences when introducing the VIIRS AOD products, but uncertainty remains over desert regions where ground monitor coverage is sparse. This work provides promise for the sustained development of global satellite-derived PM2.5 estimates, despite discontinuities in instruments and retrieval methods.

Remote sensing

Quantifying air quality co-benefits to industrial decarbonization: the local Air Emissions Tracking Atlas

Many decarbonization technologies have the added co-benefit of reducing short-lived climate pollutants, such as particulate matter (PM), nitrogen oxides (NO x ), and sulfur dioxide (SO 2 ), creating a unique opportunity for identifying strategies that promote both climate change solutions and opportunities for air quality improvement. However, stakeholders and decision-makers may struggle to quantify how these co-benefits will impact public health for the communities most affected by industrial air pollution. To address this problem, the LOCal Air Emissions Tracking Atlas (LOCAETA) fills a data availability and analysis gap by providing estimated air quality benefits from industrial decarbonization options, such as carbon capture and storage (CCS). These co-benefits are calculated using an algorithm that connects disparate datasets that separately report greenhouse gas emissions and other pollutants at U.S. industrial facilities. Version 1.0 of LOCAETA displays the estimated primary PM 2.5 emission reduction co-benefits from additional pretreatment equipment for CCS on industrial and power facilities across the state of Louisiana, as well as the potential for VOC and NH 3 generation. The emission reductions are presented in the tool alongside facility pollutant emissions information and relevant air quality, environmental, demographic, and public health datasets, such as air toxics cancer risk, satellite and in situ pollutant measurements, and population vulnerability metrics. LOCAETA enables regulators, policymakers, environmental justice communities, and industrial and commercial users to compare and contrast quantifiable public health benefits due to air quality impacts from various climate change mitigation strategies using a free and publicly-available tool. Additional pollutant reductions can be calculated using the same methodology and will be available in future versions of the tool.

29 ENERGY PLANNING, POLICY, AND ECONOMY

Global Premature Mortality Due to Anthropogenic Outdoor Air Pollution and the Contribution of Past Climate Change

Increased concentrations of ozone and fine particulate matter (PM2.5) since preindustrial times reflect increased emissions, but also contributions of past climate change. Here we use modeled concentrations from an ensemble of chemistry–climate models to estimate the global burden of anthropogenic outdoor air pollution on present-day premature human mortality, and the component of that burden attributable to past climate change. Using simulated concentrations for 2000 and 1850 and concentration–response functions (CRFs), we estimate that, at present, 470 000 (95% confidence interval, 140 000 to 900 000) premature respiratory deaths are associated globally and annually with anthropogenic ozone, and 2.1 (1.3 to 3.0) million deaths with anthropogenic PM2.5-related cardiopulmonary diseases (93%) and lung cancer (7%). These estimates are smaller than ones from previous studies because we use modeled 1850 air pollution rather than a counterfactual low concentration, and because of different emissions. Uncertainty in CRFs contributes more to overall uncertainty than the spread of model results. Mortality attributed to the effects of past climate change on air quality is considerably smaller than the global burden: 1500 (−20 000 to 27 000) deaths yr (exp -1) due to ozone and 2200 (−350 000 to 140 000) due to PM2.5. The small multi-model means are coincidental, as there are larger ranges of results for individual models, reflected in the large uncertainties, with some models suggesting that past climate change has reduced air pollution mortality.

human health

Impacts of Improved Process Representation of Particle Dry Deposition on PM Pollution in a Global Chemistry-Climate Model: Differences Across Regions, Seasons, and PM Sizes

Dry deposition (DD) is a primary removal pathway of particulate matter (PM). The aerosol DD schemes in most global models do not reflect current mechanistic understanding gleaned from observations. The NASA GISS global chemistry-climate model has a new and more dynamic DD scheme that largely captures observed changes in deposition velocities with particle size. We quantify the response of simulated PM to changes in the DD scheme for the Northeast US, Central Europe, North China Plain, and Punjab. Relative to the widely used old scheme, the new scheme shows higher annual PM2.5 for all regions (up to +14%) except C. Europe where there are very small decreases. For PM1, annual increases occur over all regions (up to +20%). For PM10, there are decreases in C. Europe (-8%) and very small decreases in the NE US yet increases (up to +12%) in Punjab and N. China Plain. While there are always increases across seasons for Punjab and N. China Plain, there are both seasonal increases and decreases for the NE US and C. Europe. Given incomplete understanding of observed variations in deposition velocities for a given particle size, we perform sensitivity simulations that perturb the magnitude of the deposition velocities simulated by the new scheme. The annual PM response to increasing DD is similar in magnitude to decreasing DD, implying linearity in the PM sensitivity to DD. The relative annual response to perturbing the DD magnitude is weaker over Punjab and sometimes N. China Plain than the NE US and C. Europe. Higher PM over Punjab and N. China Plain implies a stronger sensitivity to DD when aerosol abundances are low. More mechanistic representation of aerosol DD can sometimes improve or worsen existing model PM biases, which suggests that PM biases due to other processes can be confounded or compounded by biases in DD. Further improvements to DD parameterizations require not only more observational constraints on aerosol deposition velocities but also an advanced understanding of the processes controlling observed variability.

Environmental pollution

Evaluation of CMIP6 Model Simulations of PM 2.5 and its Components Over China

Earth system models (ESMs) participating in the latest Coupled Model Intercomparison Project Phase 6 (CMIP6) simulate various components of fine particulate matter (PM 2.5 ) as major climate forcers. Yet the model performance for PM 2.5 components remains little evaluated due in part to a lack of observational data. Here, we evaluate near-surface concentrations of PM 2.5 and its five main components over China as simulated by 14 CMIP6 models, including organic carbon (OC; available in 14 models), black carbon (BC; 14 models), sulfate (14 models), nitrate (4 models), and ammonium (5 models). For this purpose, we collect observational data between 2000 and 2014 from a satellite-based dataset for total PM2.5 and from 2469 measurement records in the literature for PM 2.5 components. Seven models output total PM 2.5 concentrations, and they all underestimate the observed total PM 2.5 over eastern China, with GFDL-ESM4 (−1.5 %) and MPI-ESM-1-2-HAM (−1.1 %) exhibiting the smallest biases averaged over the whole country. The other seven models, for which we recalculate total PM 2.5 from the available component output, underestimate the total PM 2.5 concentrations partly because of the missing model representations of nitrate and ammonium. Concentrations of the five individual components are underestimated in almost all models, except that sulfate is overestimated in MPI-ESM-1-2-HAM by 12.6 % and in MRI-ESM2-0 by 24.5 %. The underestimation is the largest for OC (by −71.2 % to −37.8 % across the 14 models) and the smallest for BC (−47.9 % to −12.1 %). The multi-model mean (MMM) reproduces the observed spatial pattern for OC (R = 0.51), sulfate (R = 0.57), nitrate (R = 0.70) and ammonium (R = 0.74) fairly well, yet the agreement is poorer for BC (R = 0.39). The varying performances of ESMs on total PM 2.5 and its components have important implications for the modeled magnitude and spatial pattern of aerosol radiative forcing.

CMIP6

Global Air Quality and Health Co-benefits of Mitigating Near-term Climate Change Through Methane and Black Carbon Emission Controls

Tropospheric ozone and black carbon (BC), a component of fine particulate matter (PM < or = 2.5 microns in aerodynamic diameter; PM2.5), are associated with premature mortality and they disrupt global and regional climate. Objectives: We examined the air quality and health benefits of 14 specific emission control measures targeting BC and methane, an ozone precursor, that were selected because of their potential to reduce the rate of climate change over the next 20-40 years. Methods: We simulated the impacts of mitigation measures on outdoor concentrations of PM2.5 and ozone using two composition-climate models, and calculated associated changes in premature PM2.5‑ and ozone-related deaths using epidemiologically derived concentration-response functions. Results: We estimated that, for PM2.5 and ozone, respectively, fully implementing these measures could reduce global population-weighted average surface concentrations by 23-34% and 7-17% and avoid 0.6-4.4 and 0.04-0.52 million annual premature deaths globally in 2030. More than 80% of the health benefits are estimated to occur in Asia. We estimated that BC mitigation measures would achieve approximately 98% of the deaths that would be avoided if all BC and methane mitigation measures were implemented, due to reduced BC and associated reductions of nonmethane ozone precursor and organic carbon emissions as well as stronger mortality relationships for PM2.5 relative to ozone. Although subject to large uncertainty, these estimates and conclusions are not strongly dependent on assumptions for the concentration-response function. Conclusions: In addition to climate benefits, our findings indicate that the methane and BC emission control measures would have substantial co-benefits for air quality and public health worldwide, potentially reversing trends of increasing air pollution concentrations and mortality in Africa and South, West, and Central Asia. These projected benefits are independent of carbon dioxide mitigation measures. Benefits of BC measures are underestimated because we did not account for benefits from reduced indoor exposures and because outdoor exposure estimates were limited by model spatial resolution.

air quality

Satellite-Based View of the Aerosol Spatial and Temporal Variability in the Cordoba Region (Argentina) Using over Ten Years of High-Resolution Data

Space-based observations offer a unique opportunity to investigate the atmosphere and its changes over decadal time scales, particularly in regions lacking in situ and/or ground based observations. In this study, we investigate temporal and spatial variability of atmospheric particulate matter (aerosol) over the urban area of Córdoba (central Argentina) using over ten years (2003–2015) of high-resolution (1 km) satellite-based retrievals of aerosol optical depth (AOD). This fine resolution is achieved exploiting the capabilities of a recently developed inversion algorithm (Multiangle implementation of atmospheric correction, MAIAC) applied to the MODIS sensor datasets of the NASA-Terra and -Aqua platforms. Results of this investigation show a clear seasonality of AOD over the investigated area. This is found to be shaped by an intricate superposition of aerosol sources, acting over different spatial scales and affecting the region with different yearly cycles. During late winter and spring (August-October), local as well as near- and long-range transported biomass burning (BB) aerosols enhance the Córdoba aerosol load, and AOD levels reach their maximum values (>0.35 at 0.47 µm). The fine AOD spatial resolution allowed to disclose that, in this period, AOD maxima are found in the rural/agricultural area around the city, reaching up to the city boundaries pinpointing that fires of local and near-range origin play a major role in the AOD enhancement. A reverse spatial AOD gradient is found from December to March, the urban area showing AODs 40–80% higher than in the city surroundings. In fact, during summer, the columnar aerosol load over the Córdoba region is dominated by local (urban and industrial) sources, likely coupled to secondary processes driven by enhanced radiation and mixing effects within a deeper planetary boundary layer (PBL). With the support of modelled AOD data from the Modern-Era Retrospective Analysis for Research and Application (MERRA), we further investigated into the chemical nature of AOD. The results suggest that mineral dust is also an important aerosol component in Córdoba, with maximum impact from November to February. The use of a long-term dataset finally allowed a preliminary assessment of AOD trends over the Córdoba region. For those months in which local sources and secondary processes were found to dominate the AOD (December to March), we found a positive AOD trend in the Córdoba outskirts, mainly in the areas with maximum urbanization/population growth over the investigated decade. Conversely, a negative AOD trend (up to −0.1 per decade) is observed all over the rural area of Córdoba during the BB season, this being attributed to a decrease of fires both at the local and the continental scale.

aerosols

Low-Cost Sensor Performance Intercomparison, Correction Factor Development, and 2+ Years of Ambient PM2.5 Monitoring in Accra, Ghana

Particulate matter air pollution is a leading cause of global mortality, particularly in Asia and Africa. Addressing the high and wide-ranging air pollution levels requires ambient monitoring, but many low- and middle-income countries (LMICs) remain scarcely monitored. To address these data gaps, recent studies have utilized low-cost sensors. These sensors have varied performance, and little literature exists about sensor intercomparison in Africa. By colocating 2 QuantAQ Modulair-PM, 2 PurpleAir PA-II SD, and 16 Clarity Node-S Generation II monitors with a reference-grade Teledyne monitor in Accra, Ghana, we present the first intercomparisons of different brands of low-cost sensors in Africa, demonstrating that each type of low-cost sensor PM2.5 is strongly correlated with reference PM2.5, but biased high for ambient mixture of sources found in Accra. When compared to a reference monitor, the QuantAQ Modulair-PM has the lowest mean absolute error at 3.04 μg/m3, followed by PurpleAir PA-II (4.54 μg/m3) and Clarity Node-S (13.68 μg/m3). We also compare the usage of 4 statistical or machine learning models (Multiple Linear Regression, Random Forest, Gaussian Mixture Regression, and XGBoost) to correct low-cost sensors data, and find that XGBoost performs the best in testing (R2: 0.97, 0.94, 0.96; mean absolute error: 0.56, 0.80, and 0.68 μg/m3 for PurpleAir PA-II, Clarity Node-S, and Modulair-PM, respectively), but tree-based models do not perform well when correcting data outside the range of the colocation training. Therefore, we used Gaussian Mixture Regression to correct data from the network of 17 Clarity Node-S monitors deployed around Accra, Ghana, from 2018 to 2021. We find that the network daily average PM2.5 concentration in Accra is 23.4 μg/m3, which is 1.6 times the World Health Organization Daily PM2.5 guideline of 15 μg/m3. While this level is lower than those seen in some larger African cities (such as Kinshasa, Democratic Republic of the Congo), mitigation strategies should be developed soon to prevent further impairment to air quality as Accra, and Ghana as a whole, rapidly grow.

Humidity

Independent and interactive effects of wet bulb globe temperature and air pollution exposures on suicide mortality

Background: Individual components of the ambient environment, such as temperature and air pollution, exist as part of a complex mixture and have been associated with suicide; however, their interactive effects remain poorly understood. This study examined the independent and interactive effects of wet bulb globe temperature (WBGT), nitrogen dioxide (NO 2 ), and fine particulate matter (PM 2.5 ) on suicide mortality. Methods: We identified 7,551 suicide cases in Utah, USA, from 2000 to 2016 and assigned exposure to daily maximum WBGT (sourced from the European Center for Medium-Range Weather Forecasts) and PM 2.5 and NO 2 concentrations (sourced from a national spatiotemporal ensemble model) using decedent’s residential address at the time of death. A case-crossover design with conditional logistic regression was used to estimate the independent and interactive effects of WBGT max , PM 2.5 , and NO 2 on suicide. For exposure windows, we considered single days preceding suicide (lag 0 to 6) and their averages across preceding days (lag 0–1, 0–3, and 0–6). Analyses were stratified by season. Results: We identified a significant association between WBGT max and suicide across all seasons (odds ratio [OR] = 1.05, 95% confidence interval [CI]: 1.01, 1.10; per 5 °C increase on lag 0–3 days). The associations were stronger in the warm season (March 22 to September 21), with ORs and 95% CIs ranging from 1.08 (1.02, 1.15) to 1.20 (1.10, 1.30) per 5 °C increase depending on the lag periods. We observed synergistic interactions between WBGT max and PM 2.5 and NO 2 in the warm season, associated with higher odds of suicide. The associations of WBGT max with suicide were most pronounced at high NO 2 levels. Conclusions: We found evidence of synergistic interactions between WBGT max and PM 2.5 and NO 2 on suicide in the warm season, emphasizing the need for considering the combined effects of heat stress and air pollution in suicide prevention strategies.

Fine particulate matter