October 2022 NS&T Highlights
These are the highlights from Nuclear Science and Technology for the month of October.
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
SEARCH · Engineering Papers
Results for “Nuclear science”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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October 2023 NS&T Highlights
An achievement report for the month of October 2023 for the Nuclear Science & Technology directorate.
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September NS&T Highlights
These are the highlights from the Nuclear Science and Technology organizations for the month of September.
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December 2023 NS&T Highlights
A presentation of recent achievements and activities from the Nuclear Science and Technology directorate for the month of December 2023.
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The Early History of the Quark-Gluon Plasma
We present the historical antecedents to the field of relativistic heavy ion physics, beginning with early attempts to model the strong interaction and ending with the endorsement of a relativistic heavy ion collider in the 1983 U.S. Long-Range Plan for Nuclear Science. Particular attention is paid to two major themes: 1) A program to study high density states of nuclear matter emerging from the 1974 Bear Mountain conference and 2) Efforts to understand the predictions of QCD for matter at high densities and/or temperatures.
73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
Applications of Nuclear Thermal Propulsion Systems for Deep Space Science Missions
Nuclear thermal propulsion (NTP) systems occupy a unique area in the space propulsion technology landscape, due to their ability to combine moderate-to-high thrust systems normally seen in chemical propulsion systems with specific impulses that are higher than those of more traditional chemical propulsion systems. Thus, NTP systems have the potential to greatly expand our access to deep space and can enable or enhance capabilities for a variety of missions that achieve science goals as outlined in NASA’s decadal surveys. This paper leverages previous work performed on applying NTP systems for multiple science missions. It also expands the mission portfolio to additional NTP-powered science mission profiles, evaluating the system performance benefits delivered by this propulsion option. This paper will also outline efforts to improve the fidelity of the existing NTP design concepts and vehicles that are utilized, leveraging previous work on nuclear propulsion systems for human-Mars missions to enhance the fidelity of results obtained from previous science mission concept studies – specifically Triton lander, solar polar orbiter, and the interstellar medium probe missions. The work outlined in this paper will also examine additional missions that have been highlighted in the recent decadal surveys, which may include robotic missions to the ice giant Uranus, robotic missions to Venus, and missions to various Kuiper belt objects (KBOs).
K A Polzin↗
A Decade of GRETINA Science
High-resolution γ-ray detector arrays have driven many scientific advances and discoveries in nuclear physics. Today, they provide a powerful and essential tool for a broad class of measurements in the study of nuclear structure and reactions, nuclear astrophysics, and applied nuclear science. In this article, we present an overview of the scientific program that has been enabled by the γ-ray tracking array GRETINA [Pas13]. This program is being carried out at both stable and radioactive ion beam facilities, employs a wide range of beam energies and reactions (from the Coulomb barrier to more than 30% the speed of light), and reflects the varied application of a γ-ray tracking array.
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Engagement opportunities in OECD NEA benchmark development
A myriad of opportunities is available to collaborate via international benchmark exercises and experimental data preservation activities. Many such opportunities abound under the auspices of the Nuclear Science Committee of the Organisation for Economic Co-operation and Development Nuclear Energy Agency (NEA). Key projects and activities of relevance to the development of advanced reactors design include the International Criticality Safety Benchmark Evaluation Project (ICSBEP), the International Reactor Physics Experiment Evaluation Project (IRPhEP), the International Assay Data of Spent Nuclear Fuel Database (SFCOMPO), the Shielding Integral Benchmark and Archive Database (SINBAD), and The International Experimental Thermal HYdraulicS Database (TIETHYS), and various cooperative benchmark exercises. Interested participants are encouraged to contact the leadership and secretariat of the various Technical Working Groups and Working Parties to become more engaged. This paper provides a summary of the current benchmark exercises and experimental databases available for international participation.
96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗
Applications of Nuclear Thermal Propulsion Systems for Deep Space Science Missions
Nuclear thermal propulsion (NTP) systems occupy a unique area in the space propulsion technology landscape due to their ability to combine moderate-to-high thrust systems normally seen in chemical propulsion systems with specific impulses that are closer to those observed in some electric propulsion systems. Consequently, NTP systems have the potential to greatly expand access to deep space and can enable a variety of missions that achieve the science goals outlined in NASA’s decadal surveys. This paper leverages previous analysis performed to show the applicability of NTP systems for notional science missions, expanding the analyzed portfolio to encompass additional science mission profiles and demonstrating how the use of NTP affects various mission parameters, such as trip time and delivered mass. This paper also outlines efforts to improve the fidelity of the existing NTP design concepts and vehicles that are utilized by leveraging previous work on nuclear propulsion systems for human-Mars missions. The fidelity of the analysis in this work is improved over previous studies, permitting commensurate improvements in the analyses of previous mission concept studies –the Triton lander, the solar polar orbiter, and the interstellar medium probe missions.
Nuclear thermal propulsion↗
NuScale Physics ECAR and Hardware Pictures
NuScale is requesting information on their Consolidated Innovative Nuclear Research (CINR) experiment. The CINR was awarded through the Nuclear Science User Facilities. Photos include the NuScale basket, insert, and instrumentation holder.
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Probing the hydrolytic degradation of UF 4 in humid air
This manuscript describes the chemical transformations that occur during hydrolysis of uranium tetrafluoride (UF 4 ) due to its storage in humid air (85% and 50% relative humidity) at ambient temperatures. This hydrolysis was previously reported to proceed slowly or not at all (depending on the percent relative humidity); however, previous reports relied primarily on X-ray diffraction methods to probe uranium speciation. Here, we employ a battery of physiochemical probing techniques to explore potential hydrolysis, including Raman spectroscopy, powder X-ray diffraction, 19 F nuclear magnetic resonance spectroscopy, scanning electron microscopy, and focused ion beam microscopy with energy-dispersive X-ray spectroscopy. Of these, only Raman spectroscopy proved to be particularly useful at observing chemical changes to UF 4 . It was found that anhydrous UF 4 slightly oxidizes over the course of thirteen days to Schoepite-like uranium complexes and possibly UO 3 . In contrast, UF 4 exposed to 50% relative humidity slightly decomposes into UO 2 F 2 , Schoepite-like uranium complexes, and possibly a high order uranium oxide that eluded chemical assignment (U x O y ). Despite the rich chemical speciation observed in our Raman spectroscopy measurements, X-ray diffraction and 19 F NMR measurements on the same material showed no changes. Microscopy measurements suggest that the observed reactions between UF 4 and water occur primarily on the surface of UF 4 particulates via a method that is visually similar to surface corrosion of metals. Therefore, we postulate that NMR spectroscopy and X-ray diffraction, which are well-suited for bulk analysis, are less suited than Raman spectroscopy to observe the surface-based reactions that occur to UF 4 when exposed to humid air. Considering the importance of UF 4 in the production of nuclear fuel and weapons, the results presented herein are widely applicable to numerous nuclear science fields where uranium detection and speciation in humid environments is of value, including nuclear nonproliferation and nuclear forensics.
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
Production of High Specific Activity 155 Tb, 161 Tb and 203 Pb for Research and Clinical Applications: Effective Target Design, Target Material Recycling and Radioisotope Separation (Final Technical Report)
The overall objectives of this project were (1) to develop methods for the production and separation of a diagnostic and therapeutic or “theranostic” pair of radioisotopes, terbium-155 ( 155 Tb) and terbium-161 ( 161 Tb) and (2) to train graduate students and postdoctoral fellows in technologies and methods used in radionuclide production. Radionuclides can be incorporated into drugs called radiopharmaceuticals that target a specific disease (e.g., cancer). The need for theranostic radionuclides is escalating with the clinical translation of radiopharmaceuticals due to their implementation in personalized medicine, which has demonstrated enhanced patient treatments. High purity and high specific activity radionuclides are critical for theranostic agent development, for example to maintain diagnostic image quality, to minimize radiation dose to the patient, and to increase uptake in the targeted tissue (e.g., tumor), especially in the case of receptor- and antigen-targeted agents. The 155 Tb (diagnostic) and 161 Tb (therapeutic) radioisotopes that were generated through this project are a theranostic pair with demonstrated potential for the development and translation into individualized, targeted, and dosimetry-driven radiotherapies. However, the development of such radiotherapies has been hindered by the lack of a routine and reliable supply of these isotopes in the United States. Methods for the production, separation, and supply of 155 Tb and 161 Tb were investigated and developed in this project. Further, the strong emphasis throughout the project on the training of graduate students and postdoctoral fellows has helped to ensure and enhance the nuclear science workforce through the training of the next generation of highly qualified scientists in nuclear and radiochemistry. This grant also continued a collaboration between scientists at the University of Washington (UW), the University of Missouri (MU) and Brookhaven National Laboratory (BNL). All three institutions were involved in the project, but to different degrees on the various tasks through which the overall objectives were met.
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February 2023 NS&T Highlights
Monthly highlights for February for the Nuclear Science & Technology directorate
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Report on Capability Expansion towards the Development of an Accelerated Creep Test Scheme at ANL
This report reports the expansion of creep testing capabilities at ANL through the installation of 9 new creep frames in the Nuclear Science and Engineering Division. Data from the commissioning tests is presented.
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NACS 2022 FRIB Investment Strategy
The Facility for Rare Isotope Beams (FRIB) that will begin operations later this year will vastly increase the number of unstable isotopes available for experiments that, together with new theoretical developments will expand our understanding of nuclear structure and nuclear reactions that produce the elements of the periodic table and power the cosmos. The knowledge and understanding gained from FRIB will benefit a variety of applications including stockpile science, nuclear forensics, nonproliferation, nuclear energy, and nuclear medicine. LLNL is actively involved in a variety of basic and applied science activities related to FRIB. These activities are listed below and documented in the following sections: 1. FRIB Decay Station, 2. Isotope Harvesting, 3. Direct Reactions, 4. Surrogate Reactions, 5. Nuclear Structure and Collectivity, 6. Nuclear Fission, and 7. Nuclear Theory.
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January 2023 NS&T Highlights
Highlights for the Nuclear Science and Technology Directorate
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Passive Temperature Sensors for Nuclear Applications
In April 2007, the Department of Energy (DOE) designated the Advanced Test Reactor (ATR) a National Scientific User Facility (NSUF) to advance US leadership in nuclear science and technology. By attracting new users from universities, laboratories, and industry, this program supports basic and applied nuclear research to help address the nation's energy security needs. In support of this program, the Idaho National Laboratory (INL) established in-house capabilities to develop, fabricate, test, and qualify new and enhanced temperature sensors for irradiation testing. This effort is continuing today through the DOE?s Advanced Sensors and Instrumentation (ASI) program. Although most efforts emphasize sensors capable of providing real-time data, selected tasks have been completed to enhance passive sensors for irradiations where instrumentation leads cannot be included. These sensors include silicon carbide (SiC) monitors, melt wires and the sublime temperature monitor. SiC monitors are available to detect peak irradiation temperatures between 200°C and 800°C in reactor locations where instrumentation leads cannot be used. SiC monitors may be evaluated using specialized equipment installed at INL?s Measurement Sciences Laboratory (MSL). A melt wire inventory is also maintained at MSL. This inventory contains wires for specific use in irradiation experiments ranging in temperatures from 30°C to 1500°C. Melt wires and SiC monitors have had decades of research and application. Recent research has produced a passive monitor known as the sublime temperature monitor. This passive sensor has the capability of recording temperature gradients. This paper will discuss passive temperature sensors currently being researched and implemented under the ASI program.
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Department of Energy: Office of Scientific and Technical Information
The international acquisitions functions and activities of the Office of Scientific and Technical Information (OSTI) are described. There are four mechanisms for obtaining foreign information related to energy and nuclear science: The Energy Technology Data Exchange consisting of 14 member countries and 2 associate members; the International Nuclear Information System consisting of 86 countries and 17 international organizations; the Nuclear Energy Agency's 19 member countries provide reports for departmental scientists' use; bilateral agreements with countries such as Germany, the Nordic Consortium, and Australia result in records of foreign research in progress.
Grissom, Catherine↗