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At least 163 records · Page 9

HFIR SiC Bowing Test Ready to Insert

This report describes the successful assembly of a High Flux Isotope Reactor (HFIR) irradiation experiment designed to assess radiation-induced lateral bowing of silicon carbide fiber–reinforced, silicon carbide matrix composite (SiC/SiC) components under a radial fast neutron flux gradient. Excessive bowing of a SiC/SiC channel box in a boiling water reactor could potentially interfere with control blade movements. Similar concerns exist for SiC/SiC fuel cladding in light water reactors. The experiment described herein will provide experimental validation of the structural response of a miniature SiC/SiC channel box and tube specimens with pressurized water reactor diameters during irradiation. The significant radial fast neutron flux gradients that exist in the permanent reflector of HFIR were characterized using detailed three-dimensional neutronic calculations. The three-dimensional displacement damage dose rate profile and the resulting volumetric swelling in SiC were used as inputs to structural analyses that predicted the deformation and stresses in the channel box specimen. The specimens were thoroughly characterized prior to irradiation using traditional dimensional inspection and surface profilometry so that these measurements can later be compared with similar measurements that will be made post-irradiation to determine radiation-induced deformations. Furthermore, fine engraving markers were inscribed along all outer surfaces of the specimen and mapped using a digital microscope and a three-dimensional stage. This technique allowed for accurate measurements of the marker spacings, which can be compared with similar measurements that will be made post-irradiation to provide local radiation-induced strain mapping. The experiment was successfully assembled and is scheduled for insertion during HFIR cycle 492, which is currently scheduled to run from May 25, 2021 to June 18, 2021.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Smaller, Lower-Power Fast-Neutron Scintillation Detectors

Scintillation-based fast-neutron detectors that are smaller and less power-hungry than mainstream scintillation-based fast-neutron detectors are undergoing development. There are numerous applications for such detectors in monitoring fast-neutron fluxes from nuclear reactors, nuclear materials, and natural sources, both on Earth and in outer space. A particularly important terrestrial application for small, low-power, portable fast-neutron detectors lies in the requirement to scan for nuclear materials in cargo and baggage arriving at international transportation facilities. The present development of miniature, low-power scintillation-based fast-neutron detectors exploits recent advances in the fabrication of avalanche photodiodes (APDs). Basically, such a detector includes a plastic scintillator, typically between 300 and 400 m thick with very thin silver mirror coating on all its faces except the one bonded to an APD. All photons generated from scintillation are thus internally reflected and eventually directed to the APD. This design affords not only compactness but also tight optical coupling for utilization of a relatively large proportion of the scintillation light. The combination of this tight coupling and the avalanche-multiplication gain (typically between 750 and 1,000) of the APD is expected to have enough sensitivity to enable monitoring of a fast-neutron flux as small as 1,000 cm(exp -2)s(exp -1). Moreover, pulse-height analysis can be expected to provide information on the kinetic energies of incident neutrons. It has been estimated that a complete, fully developed fast-neutron detector of this type, would be characterized by linear dimensions of the order of 10 cm or less, a mass of no more than about 0.5 kg, and a power demand of no more than a few watts.

Patel, Jagdish↗

Monte Carlo Simulations of the Water Draining Experiment of Giacint Critical Assembly

The MCNP6 computer program has been successfully extended to simulate reactor dynamics problems with moving parts of the geometries. Different from the dynamic method developed in other Monte Carlo codes, a movement scheme has been developed to account for the geometrical parts motion during the particle random walk. The MCNP6 computer program has been used to simulate two transient experiments of the Giacint critical assembly. The MCNP6 calculated total neutron flux was compared with that from the Serpent simulation. An excellent agreement was obtained between the results of the two Monte Caro computer programs. The MCNP6 calculated total neutron flux was also compared with the two measured transients. The MCNP6 results predicted a faster transient than the experimental data. The MCNP6 transient simulation was improved with an adjusted geometrical model which shifts the fuel rods slightly to match the measured reactivity worth due to the drained water. (c) 2021 Elsevier Ltd. All rights reserved.

MCNP, Moving Geometries, Monte Carlo Reactor Trans↗

Energy spectrum and flux of fast neutrons in the atmosphere

The neutron energy spectrum and flux in the atmosphere at the Pfotzer maximum (about 100 g per cm squared) were measured at geomagnetic latitude 42 deg N, using a system capable of detecting a small flux of fast (5 to 20 MeV) neutrons in a much larger background flux of gamma rays and charged particles. The detector consisted of a cylindrical cell of organic liquid scintillator coupled to a high-resolution two-parameter multiparticle pulse shape discriminator with a two-parameter logarithmic pulse-height analyzer. The spectral parameter for the differential neutron energy spectrum was found to decrease from 4.4 plus or minus 0.8 between 3.5 and 6.0 MeV to 1.5 plus or minus 1.0 in the interval 11 to 20 MeV; a value of 0.36 plus or minus 0.10 neutrons per cm squared was calculated for neutron flux between 3.5 and 10 MeV. The importance of these results for evaluating the role of albedo neutron leakage as a source of the energetic proton flux in the radiation belts is also considered.

Saint Onge, R. N.↗

Sensor Reduction for Diversion Detection in a Realistic Heat Pipe Microreactor Using Supervised Machine Learning

Microreactors are designed as a smaller, cheaper, and safer alternative to traditional nuclear power plants. Their non-traditional characteristics and prospect of mass production and deployment will likely require new approaches to nuclear safeguards. The primary proliferation concern with microreactors is the diversion of fuel material. Such diversion may produce measurable defects in key physical attributes like neutron flux, which may in turn be detectable using machine learning models. Preliminary work has demonstrated this ability for modeled nominal and diversion scenarios using large quantities of energy integrated neutron flux data. In practice, the number of available sensors for such measurements will be limited and energy integrated flux information will not be available. This work explores the ability of tree-based gradient boosted ensemble models to classify a given microreactor core is nominal or diversion, and determine the number of fuel pins diverted in the case of diversion with reduced numbers of sensors and more realistic detector responses. Classification accuracy of greater than 98% and regression errors as low as 5% of the total number of fuel pins were achieved with as few as 15 sensors, compared to 99% and 4.1% with a maximum of 240 sensors.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Neutron fluences and energy spectra in the Cosmos-2044 biosatellite orbit

Joint Soviet-American measurements of the neutron component of space radiation (SR) were carried out during the flight of the Soviet biosatellite Cosmos-2044. Neutron flux densities and differential energy spectra were measured inside and on the external surface of the spacecraft. Three energy intervals were employed: thermal (En < or = 0.2 eV), resonance (0.2 eV < En < 1.0 MeV) and fast (En > or = 1.0 MeV) neutrons. The first two groups were measured with U.S. 6LiF detectors, while fast neutrons were recorded both by U.S. fission foils and Soviet nuclear emulsions. Estimations were made of the contributions to absorbed and equivalent doses from each neutron energy interval and a correlation was presented between fast neutron fluxes, measured outside the satellite, and the phase of solar activity (SA). Average dose equivalent rates of 0.018 and 0.14 mrem d-1 were measured for thermal and resonance neutrons, respectively, outside the spacecraft. The corresponding values for fast neutrons were 3.3 (U.S.) and 1.8 (U.S.S.R.) mrem d-1. Inside the spacecraft, a value of 3.5 mrem d-1 was found.

NASA Discipline Number 00-00↗

Comprehensive Analysis of Streaming and Shutdown Dose Rate Experiments at JET with ORNL Fusion Neutronics Workflows

Current experimental fusion systems and conceptual designs of fusion pilot plants (FPPs) are growing in complexity and size. Several radiation metrics are crucial to the safe operation of fusion machines, including neutron flux streaming through openings and the shutdown dose rate (SDDR). Most current designs of advanced experimental fusion systems—and the most probable candidates for FPPs—are based on the tokamak concept, which is prone to neutron streaming through the myriad openings needed for diagnostic and support systems. SDDR is caused by decay gamma rays from radionuclides that become activated by neutrons during the operation of a fusion system that use deuterium-deuterium (DD), tritium-tritium, or deuterium-tritium plasma. Because computational tools have become essential for determining these radiation metrics, they must be validated against reliable and applicable experimental data. Experiments at the Joint European Torus (JET) provide a unique source of experimental data for validating computational tools and nuclear data used to determine SDDR and neutron fluxes in streaming-dominated geometries. Here, this paper presents the comprehensive analysis of the high-performance DD JET SDDR, and streaming experiments performed using Oak Ridge National Laboratory (ORNL) fusion workflows. The computational results were compared with experimental results that consist of online SDDR measurements with ionization chambers and neutron fluence streaming measurements using thermoluminescent detectors. The ratio of calculated-to-experimental SDDR values ranges from 0.6 to 2.5, and the streaming results range from 0.5 to 8.0. Future work will include analyzing the JET 2021 DTE2 campaign alongside the integration of the Shift Monte Carlo transport code into all ORNL fusion neutronics workflows.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Martian volatiles determined using the Mars observer gamma ray spectrometer

The relative abundances of H2O and CO2 and their latitude, longitude, and depth profiles on Mars sensitively reflect, as well as help control, past and present Martian climate patterns. Seasonal variations of their distributions at high latitudes also reflect and help control global weather patterns and erosion through surface weathering. A combined analysis of gamma ray line and neutron flux maps constructed from data measured using the Mars Observer Gamma Ray Spectrometer (MOGRS) should allow a determination of seasonal changes in both the horizontal and vertical structure of CO2 ice that covers the north polar cap during winter and the south polar cap throughout the year and both the horizontal and vertical structure of residual H2O ice within the top meter of the surface that was predicted from Viking observations to exist primarily at high latitudes. Particularly important in this regard will be maps of thermal and epithermal neutron fluxes measured using the MOGRS anticoincidence shield, the intensity of the hydrogen, neutron capture gamma ray line at 2.223 MeV, the intensity of a capture gamma ray line as 1.725 MeV from iron, and the intensity of an inelastic scatter gamma ray line as 1.779 MeV from silicon.

Feldman, W. C.↗

(U) Updated Godiva-IV Benchmark Preview

A note of errata prepended to the Godiva-IV delayed-critical benchmark (HEU-METFAST-086) identifies two corrections that need to be made to the model: The glory hole in the spindle should be made larger, and the height of the safety block should be made smaller (and therefore its density made larger). In addition, the safety block at its full-in position is closer to the inner subassembly plate than was modeled in the benchmark. These changes have been made to HEU-METFAST-086 Case 4 in order to estimate the effect on k eff and on the neutron flux spectrum. Using smaller separation, a smaller safety block, and a larger glory hole caused k eff to increase by 453 ± 1 pcm from the benchmark. The latest nuclear data, ENDF-B/VIII.0, have also been used; this caused k eff to increase another 37 ± 1 pcm. Flux spectra were compared in a modeled fission foil and at three external point detectors. Within the fission foil, using ENDF/B-VIII.0 for Godiva-IV induced changes in the flux spectrum similar in size to the changes due to using smaller separation, a smaller safety block, and a larger glory hole. At the point detectors, using ENDF/B-VIII.0 induced changes in the flux spectrum much larger than those due to changing the model. In other words, the corrections to the benchmark model cause a large increase in k eff , but the changes to the neutron flux spectrum are small compared to those caused by using the latest nuclear data. This study presents a preview of results expected during the reevaluation of the Godiva IV benchmark, but it is not a substitute for the full reevaluation

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Novae, supernovae, and neutron sources

The evolution of thermonuclear runaways is examined in two models of white dwarfs with extreme enhancements of C-12 in their envelopes to test the predictions of Hoyle and Clayton (1974) that novae will result from such stars and a large neutron flux will be produced. In agreement with these predictions, it is assumed that the large amount of C-12 is due to the accretion of hydrogen-rich material from a disk surrounding a carbon-oxygen white dwarf. The evolution of the two models is described in detail, and the results suggest that accretion of hydrogen-rich material will always result in a thermonuclear runaway, although mass ejection will not occur unless CNO nuclei are enhanced. It is noted that one model produces a substantial neutron flux for a short time which is sufficient to drive an intermediate neutron-capture process.

Starrfield, S.↗

Editorial: Using high energy density plasmas for nuclear experiments relevant to nuclear astrophysics

Thermonuclear reaction rates and nuclear processes have traditionally been explored by means of accelerator experiments, which are difficult to execute at conditions relevant to nucleosynthesis. High energy density (HED) plasmas generated using lasers, such as the inertial confinement fusion (ICF) platform, more closely mimic astrophysical environments in several ways, including with thermal distributions of reacting ions as opposed to mono-energetic ions impinging on a cold target; stellar-relevant plasma temperatures and densities; and neutron flux densities not found anywhere else on earth. The most extreme conditions can currently be achieved at the National Ignition Facility (NIF) laser in the US, where densities of 10 3 g/cm 3 and neutron fluxes up to 5∙10 27 neutrons/cm/s have been demonstrated over a time period of a few tens of picoseconds. The HED platform is emerging as an interesting complement to accelerator experiments.

charged-particle-induced reactions↗

Thermomechanics coupling to Monte Carlo particle transport on unstructured mesh geometries using Cardinal

Geometry deformation due to thermal expansion influences neutron transport in many systems. Studying this phenomenon involves coupling models for neutronics, thermal hydraulics, and solid mechanics. To enable high fidelity modeling of these coupled physics, new capabilities were introduced in Cardinal, coupling OpenMC Monte Carlo particle transport models with MOOSE thermomechanical physics on unstructured moving-mesh geometries. In this work, we present a fully open-source capability leveraging on-the-fly mesh skinning to automatically regenerate OpenMC geometry, which allows multiphysics feedback from temperature, density, and geometry changes. The new capability is verified using an analytic benchmark slab problem, which couples S 2 neutron transport with thermal conduction, convective boundary conditions, Doppler-broadened cross sections, and nonlinear thermal expansion effects along the heated slab. Cardinal reproduces the analytic solutions for the neutron flux, heating, k eff , and temperature with demonstrated convergence in various error terms including mesh resolution and cross section temperature library spacing. For the nominal benchmark conditions and with a fine mesh, maximum relative errors for neutron flux, temperature, and heating are lower than 1%, while errors in integral quantities such as k eff and slab length are within 1 pcm and 48 µm, respectively. This work (i) presents a new numerical approach to thermomechanics coupling with OpenMC models, (ii) is the first (to our knowledge) to utilize a mechanical partial differential equation (PDE) solution to solve the (Griesheimer and Kooreman, 2022) analytic benchmark, and (iii) develops this verified capability within an open-source package.

97 - MATHEMATICS AND COMPUTING↗

Innovative control mechanism for research and test reactors using mandrel-shaped control rods

Research and test reactors have historically played a pivotal role in supporting the initial development of nuclear reactors. They continue to provide essential data for enhancing fuel designs and material knowledge. However, with many such reactors aging and the growing demand for data to bolster advanced reactor development, it is more necessary to research potential design attributes of the next generation of research and test reactors. For test reactors dedicated to fuel and material testing, the design of control mechanisms significantly influences the stabilization of neutron flux levels in irradiation positions while sustaining criticality. This study presents an innovative control mechanism for potential research and test reactor designs. It employs small absorber rods that move in opposite axial directions to maintain axial symmetry of power and neutron flux during burnup cycles. These rods maximize reactivity worth while also offering flexibility to flatten the radial power distribution. An axial translation of the control mechanisms’ absorbers, as compared to the rotational movement of absorbers in control cylinders, also provides a benefit to available excess reactivity and cycle length. Additionally, this work utilizes a simplified core model of the Advanced Test Reactor to assess the performance of this control mechanism. Compared to the current control system based on rotating control cylinders, the new control mechanism has the potential to enhance, or at least maintain, neutronic performance parameters in this reactor design.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

High Flux Isotope Reactor (HFIR)

Oak Ridge National Laboratory’s High Flux Isotope Reactor (HFIR) is the highest-flux reactor-based neutron source in the United States. HFIR’s intense neutron flux and state-of-the-art facilities result in world-class capabilities, including neutron scattering, radioisotope production, materials irradiation, and neutron activation analysis. HFIR’s multimission capabilities are attributed to its versatile high-power-density core design consisting of a series of concentric regions, including a flux trap target region, an inner fuel element, an outer fuel element, a control element region, and a beryllium reflector. The pressurized, light-water-cooled research reactor operates at 85 MW and is fueled by 9.4 kg 235U.

Chandler, David↗

Neutron influences and energy spectra in the Cosmos-2044 biosatellite orbit

Joint Soviet-American measurements of the neutron component of space radiation (SR) were carried out during the flight of the Soviet biosatellite Cosmos-2044. Neutron flux densities and differential energy spectra were measured inside and on the external surface of the spacecraft. Three energy intervals were employed: thermal (E(sub n) less than or equal to 0.2 eV), resonance (0.2 eV less than E(sub n) less than 1.0 MeV) and fast (E(sub n) greater than or equal to 1.0 MeV) neutrons. The first two groups were measured with U.S. (6)LiF detectors, while fast neutrons were recorded both by U.S. fission foils and Soviet nuclear emulsions. Estimations were made of the contributions to absorbed and equivalent doses from each neutron energy interval and a correlation was presented between fast neutron fluxes, measured outside the satellite, and the phase of solar activity (SA). Average dose equivalent rates of 0.018 and 0.14 mrem d(exp -1) were measured for thermal and resonance neutrons, respectively, outside the spacecraft. The corresponding values for fast neutrons were 3.3 (U.S.) and 1.8 (U.S.S.R.) mrem d(exp -1). Inside the spacecraft, a value of 3.5 mrem d(exp -1) was found.

Dudkin, V. E.↗

Spectra from nuclear-excited plasmas

The paper discusses the spectra taken from He-3(n,p)H-3 nuclear-induced plasmas under high thermal neutron flux, lasing conditions. Also, initial spectra are presented for U-235F6 generated plasmas. From an evaluation of these spectra, important atomic and molecular processes that occur in the plasma can be inferred. The spectra presented are the first to be generated by He-3 and U-235F6 nuclear reactions under high neutron flux, lasing conditions. The U-235(n,ff)FF reaction, which liberates 165 MeV of fission-fragment kinetic energy, creates plasmas that are of great interest, since at sufficiently high densities of U-235F6 the gas becomes self-critical; thus, there is no need for an external driving reactor (source of neutrons). The spectra from mixtures of He-3 and Ar, Xe, Kr, Ne, Cl2, F2 and N2 indicate little difference between high-pressure nuclear-induced plasmas and high-pressure electrically pulsed afterglow plasmas for noble-gas systems

De Young, R. J.↗

The electron Boltzmann equation in a plasma generated by fission fragments

A Boltzmann equation formulation is presented for the determination of the electron distribution function in a plasma generated by fission fragments. The formulation takes into consideration ambipolar diffusion, elastic and inelastic collisions, recombination and ionization, and allows for the fact that the primary electrons are not monoenergetic. Calculations for He in a tube coated with fissionable material show that, over a wide pressure and neutron flux range, the distribution function is non-Maxwellian, but the electrons are essentially thermal. Moreover, about a third of the energy of the primary electrons is transferred into the inelastic levels of He. This fraction of energy transfer is almost independent of pressure and neutron flux but increases sharply in the presence of a sustainer electric field.

Hassan, H. A.↗

Electron distribution function in a plasma generated by fission fragments

A Boltzmann equation formulation is presented for the determination of the electron distribution function in a plasma generated by fission fragments. The formulation takes into consideration ambipolar diffusion, elastic and inelastic collisions, recombination and ionization, and allows for the fact that the primary electrons are not monoenergetic. Calculations for He in a tube coated with fissionable material shows that, over a wide pressure and neutron flux range, the distribution function is non-Maxwellian, but the electrons are essentially thermal. Moreover, about a third of the energy of the primary electrons is transferred into the inelastic levels of He. This fraction of energy transfer is almost independent of pressure and neutron flux.

Hassan, H. A.↗