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At least 163 records · Page 9

Method for computationally efficient design of dielectric laser accelerator structures

Here, dielectric microstructures have generated much interest in recent years as a means of accelerating charged particles when powered by solid state lasers. The acceleration gradient (or particle energy gain per unit length) is an important figure of merit. To design structures with high acceleration gradients, we explore the adjoint variable method, a highly efficient technique used to compute the sensitivity of an objective with respect to a large number of parameters. With this formalism, the sensitivity of the acceleration gradient of a dielectric structure with respect to its entire spatial permittivity distribution is calculated by the use of only two full-field electromagnetic simulations, the original and ‘adjoint’. The adjoint simulation corresponds physically to the reciprocal situation of a point charge moving through the accelerator gap and radiating. Using this formalism, we perform numerical optimizations aimed at maximizing acceleration gradients, which generate fabricable structures of greatly improved performance in comparison to previously examined geometries.

43 PARTICLE ACCELERATORS↗

Emergent Phenomena at Oxide Interfaces

Transition metal oxides (TMOs) are an ideal arena for the study of electronic correlations because the s -electrons of the transition metal ions are removed and transferred to oxygen ions, and hence the strongly correlated d -electrons determine their physical properties such as electrical transport, magnetism, optical response, thermal conductivity, and superconductivity. These electron correlations prohibit the double occupancy of metal sites and induce a local entanglement of charge, spin, and orbital degrees of freedom. This gives rise to a variety of phenomena, e.g., Mott insulators, various charge/spin/orbital orderings, metal-insulator transitions, multiferroics, and superconductivity. In recent years, there has been a burst of activity to manipulate these phenomena, as well as create new ones, using oxide heterostructures.

74 ATOMIC AND MOLECULAR PHYSICS↗

Subband structure of a two-dimensional electron gas formed at the polar surface of the strong spin-orbit perovskite KTaO 3

We demonstrate the formation of a two-dimensional electron gas (2DEG) at the (100) surface of the 5d transition-metal oxide KTaO 3 . From angle-resolved photoemission, we find that quantum confinement lifts the orbital degeneracy of the bulk band structure and leads to a 2DEG composed of ladders of subband states of both light and heavy carriers. Despite the strong spin-orbit coupling, we find no experimental signatures of a Rashba spin splitting, which has important implications for the interpretation of transport measurements in both KTaO 3 - and SrTiO 3 -based 2DEGs. The polar nature of the KTaO 3 (100) surface appears to help mediate formation of the 2DEG as compared to non-polar SrTiO 3 (100).

36 MATERIALS SCIENCE↗

LDRD FY2013 Annual Report

The Department of Energy (DOE) and the SLAC National Accelerator Laboratory (SLAC) encourage innovation, creativity, originality and quality to maintain the Laboratory’s research activities and staff at the forefront of science and technology. To further advance the Laboratory’s scientific research capabilities, the Laboratory allocates a portion of its funds for the Laboratory Directed Research and Development (LDRD) program. With DOE guidance, the LDRD program enables SLAC scientists to make rapid and significant contributions to seeding new strategies for solving important national science and technology problems. The LDRD program is conducted using existing research facilities.

ACCPHY↗

SLAC Laboratory Directed Research and Development Program: FY2014 Annual Report

The Department of Energy (DOE) and the SLAC National Accelerator Laboratory (SLAC) encourage innovation, creativity, originality and quality to maintain the Laboratory’s research activities and staff at the forefront of science and technology. To further advance the Laboratory’s scientific research capabilities, the Laboratory allocates a portion of its funds for the Laboratory Directed Research and Development (LDRD) program. With DOE guidance, the LDRD program enables SLAC scientists to make rapid and significant contributions to seeding new strategies for solving important national science and technology problems. The LDRD program is conducted using existing research facilities. The project proposals can be characterized as: Small-scale research and development activities or pilot projects; Bench-scale research projects; and Information gathering, computer modeling, conceptual design and feasibility studies. In addition to building new core competencies that support the DOE missions, the LDRD project proposals may also conduct scientific research and development that support the missions of other federal agencies and/or non-federal sponsors. In FY2014, SLAC continued to see some of the previously funded LDRD programs transition to follow on funding with the Office of Science, (including an Early Career Award), EERE and other agencies such as DARPA and NIH. This external validation shows that the projects selected were important to continuing forefront science and use-inspired applications with mission relevance and demonstrates they were delivering significant results. Annual reports for the FY14 project activities are included in this report.

25 ENERGY STORAGE↗

Resolving electrical conductivities from collisionally damped plasmons in isochorically heated warm dense aluminum

We measure the highly-resolved inelastic x-ray scattering spectrum of isochorically ultrafast heated aluminum. In the x-ray forward scattering spectra the electron temperature could be measured from the down- and upshifted plasmon, where the electron density of ne = 1:8 1023 cm 3 is known a priori. We have studied the plasmon damping by applying electron-particle collision models beyond the Born approximation determining the electrical conductivity of warm dense aluminum.

36 MATERIALS SCIENCE↗

Laboratory Directed Research and Development Program: FY 2015 Annual Report

The Department of Energy (DOE) and the SLAC National Accelerator Laboratory (SLAC) encourage innovation, creativity, originality and quality to maintain the Laboratory’s research activities and staff at the forefront of science and technology. To further advance its scientific research capabilities, the Laboratory allocates a portion of its funds for the Laboratory Directed Research and Development (LDRD) program. With DOE guidance, the LDRD program enables SLAC scientists to make rapid and significant contributions that seed new strategies for solving important national science and technology problems. The LDRD program is conducted using existing research facilities.

99 GENERAL AND MISCELLANEOUS↗

Synthesis of Freestanding Single-crystal Perovskite Films and Heterostructures by Etching of Sacrificial Water-soluble Layers

The ability to create and manipulate materials in two-dimensional (2D) form has repeatedly had transformative impact on science and technology. In parallel with the exfoliation and stacking of intrinsically layered crystals, atomic-scale thin film growth of complex materials has enabled the creation of artificial 2D heterostructures with novel functionality and emergent phenomena, as seen in perovskite heterostructures. However, separation of these layers from the growth substrate has proven challenging, limiting the manipulation capabilities of these heterostructures with respect to exfoliated materials. Here we present a general method to create freestanding perovskite membranes. The key is the epitaxial growth of water-soluble Sr 3 Al 2 O 6 on perovskite substrates, followed by in situ growth of films and heterostructures. Millimetre-size single-crystalline membranes are produced by etching the Sr 3 Al 2 O 6 layer in water, providing the opportunity to transfer them to arbitrary substrates and integrate them with heterostructures of semiconductors and layered compounds.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Pairing state with a time-reversal symmetry breaking in FeAs-based superconductors

We investigate the competition between the extended s{+-} wave and dx2-y2 -wave pairing order parameters in the iron-based superconductors. Because of the frustrating pairing interactions among the electron and the hole fermi pockets, a time-reversal symmetry breaking s + id pairing state could be favored. We analyze this pairing state within the Ginzburg-Landau theory, and explore the experimental consequences. In such a state, spatial inhomogeneity induces supercurrent near a non-magnetic impurity and the corners of a square sample. The resonance mode between the s{+-} and dx2?y2 -wave order parameters can be detected through the B1g-Raman spectroscopy.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Quantum spin Hall effect in a transition metal oxide Na2IrO3

We study theoretically the electronic states in a 5d transition metal oxide Na{sub 2}I{sub r}O{sub 3}, in which both the spin-orbit interaction and the electron correlation play crucial roles. Tight-binding model analysis together with the fisrt-principles band structure calculation predicts that this material is a layered quantum spin Hall system. Due to the electron correlation, an antiferromagnetic order first develops at the edge, and later inside the bulk at low temperatures.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Resource Letter on Stimulated Inelastic X-ray Scattering at an XFEL

At sufficient X-ray intensity, stimulated effects in inelastic scattering will become important. These coherent, non-linear optical phenomena may be used to impulsively produce a high degree of collective excitation in, for example, correlated electron materials, suitable for performing ultrafast time-resolved spectroscopy. This Resource Letter collects information on fundamental aspects of stimulated X-ray scattering and evaluates the prospect for successful experiments at a present or future X-ray free electron laser (XFEL) facility.

INST, MATSCI, PHYS, SYNCHRAD, XFEL↗

Fermi Surface and Van Hove Singularities in the Itinerant Metamagnet Sr(3)Ru(2)O(7)

The low-energy electronic structure of the itinerant metamagnet Sr{sub 3}Ru{sub 2}O{sub 7} is investigated by angle resolved photoemission and density functional calculations. We find well-defined quasiparticle bands with resolution limited line widths and Fermi velocities up to an order of magnitude lower than in single layer Sr{sub 2}RuO{sub 4}. The complete topography, the cyclotron masses and the orbital character of the Fermi surface are determined, in agreement with bulk sensitive de Haas - van Alphen measurements. An analysis of the dxy band dispersion reveals a complex density of states with van Hove singularities (vHs) near the Fermi level; a situation which is favorable for magnetic instabilities.

43 PARTICLE ACCELERATORS↗

Effects of Out-of-Plane Disorder on the Nodal Quasiparticle and Superconducting Gap in Single-Layer Bi_2Sr_1.6Ln_0.4CuO_6 delta (Ln = La, Nd, Gd)

How out-of-plane disorder affects the electronic structure has been investigated for the single-layer cuprates Bi{sub 2}Sr{sub 1.6}Ln{sub 0.4}CuO{sub 6+{delta}} (Ln = La, Nd, Gd) by angle-resolved photoemission spectroscopy. We have observed that, with increasing disorder, while the Fermi surface shape and band dispersions are not affected, the quasi-particle width increases, the anti-nodal gap is enhanced and the superconducting gap in the nodal region is depressed. The results indicate that the superconductivity is significantly depressed by out-of-plane disorder through the enhancement of the anti-nodal gap and the depression of the superconducting gap in the nodal region.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Unraveling the nature of charge excitations in La2CuO4 with momentum-resolved Cu K-edge resonant inelastic X-ray scattering

Results of model calculations using exact diagonalization reveal the orbital character of states associated with different Raman loss peaks in Cu K-edge resonant inelastic X-ray scattering (RIXS) from La{sub 2}CuO{sub 4}. The model includes electronic orbitals necessary to highlight non-local Zhang-Rice singlet, charge transfer and d-d excitations, as well as states with apical oxygen 2p{sub z} character. The dispersion of these excitations is discussed with prospects for resonant final state wave-function mapping. A good agreement with experiments emphasizes the substantial multi-orbital character of RIXS profiles in the energy transfer range 1-6 eV.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Imaging Nonequilibrium Atomic Vibrations with X-ray Diffuse Scattering

We use picosecond x-ray diffuse scattering to image the nonequilibrium vibrations of the lattice following ultrafast laser excitation. We present images of nonequilibrium phonons in InP and InSb throughout the Brillouin-zone which remain out of equilibrium up to nanoseconds. The results are analyzed using a Born model that helps identify the phonon branches contributing to the observed features in the time-resolved diffuse scattering. In InP this analysis shows a delayed increase in the transverse acoustic (TA) phonon population along high-symmetry directions accompanied by a decrease in the longitudinal acoustic (LA) phonons. In InSb the increase in TA phonon population is less directional.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Experimental Determination of Damage Threshold Characteristics of IR Compatible Optical Materials

The accelerating gradient in a laser-driven dielectric accelerating structure is often limited by the laser damage threshold of the structure. For a given laser-driven dielectric accelerator design, we can maximize the accelerating gradient by choosing the best combination of the accelerator's constituent material and operating wavelength. We present here a model of the damage mechanism from ultrafast infrared pulses and compare that model with experimental measurements of the damage threshold of bulk silicon. Additionally, we present experimental measurements of a variety of candidate materials, thin films, and nanofabricated accelerating structures.

36 MATERIALS SCIENCE↗

Massive Dirac Fermion on the Surface of a Magnetically Doped Topological Insulator

Topological insulators are characterized by a massless Dirac surface state and a bulk energy gap. An insulating massive Dirac fermion state is predicted to occur if the breaking of the time reversal symmetry opens an energy gap at the Dirac point, provided that the Fermi-energy resides inside both the surface and bulk gaps. By introducing magnetic dopants into the three dimensional topological insulator Bi{sub 2}Se{sub 3} to break the time reversal symmetry, we observed the formation of a massive Dirac fermion on the surface; simultaneous magnetic and charge doping furthermore positioned the Fermi-energy inside the Dirac gap. The insulating massive Dirac Fermion state thus obtained may provide a tool for studying a range of topological phenomena relevant to both condensed matter and particle physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗