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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

A Finite-Time Ensemble Method for Mixed Layer Model Comparison

Here, this work evaluates the fidelity of various upper-ocean turbulence parameterizations subject to realistic monsoon forcing and presents a finite-time ensemble vector (EV) method to better manage the design and numerical principles of these parameterizations. The EV method emphasizes the dynamics of a turbulence closure multimodel ensemble and is applied to evaluate 10 different ocean surface boundary layer (OSBL) parameterizations within a single-column (SC) model against two boundary layer large-eddy simulations (LES). Both LES include realistic surface forcing, but one includes wind-driven shear turbulence only, while the other includes additional Stokes forcing through the wave-average equations that generate Langmuir turbulence. The finite-time EV framework focuses on what constitutes the local behavior of the mixed layer dynamical system and isolates the forcing and ocean state conditions where turbulence parameterizations most disagree. Identifying disagreement provides the potential to evaluate SC models comparatively against the LES. Observations collected during the 2018 monsoon onset in the Bay of Bengal provide a case study to evaluate models under realistic and variable forcing conditions. The case study results highlight two regimes where models disagree 1) during wind-driven deepening of the mixed layer and 2) under strong diurnal forcing.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Site Disorder as a Predictor for Compositionally Complex 5RE 2 Zr 2 O 7 Ceramic Phase Stability

Here, phase formation and stability of five component compositionally complex rare earth zirconates (5RE 2 Zr 2 O 7 ) were investigated by X-ray diffraction and electron microprobe analysis. Zirconates with different rare earth compositions (LaNdSmEuDy, LaNdSmEuYb, LaNdEuErYb, LaNdDyErYb, SmEuDyYHo, LaYHoErYb, and DyYHoErYb) were synthesized at 1700°C and 2000°C by the solid-state method to investigate the effect of A-site site disorder (δ A ) on phase stability. Increased site disorder results from mixed cation occupancy with localized crystallographic strain and bond disorder. Compositions LaNdSmEuDy (δ A = 4.6) and LaNdSmEuYb (δ A = 6.0) produced a single pyrochlore phase and compositions SmDyYHoErYb (δ A = 2.8), LaYHoErYb (δ A = 6.2), and DyYHoErYb (δ A = 1.7) produced a single fluorite phase. High δ A compositions LaNdEuErYb (δ A = 6.9) and LaNdDyErYb (δ A = 7.2) produced a pyrochlore and fluorite phase mixture at 1700°C. Single phase was obtained for the latter composition at 2000°C. Of the single phase compositions calcined at 1700°C, LaNdSmEuYb and LaYHoErYb (both with largest δ A ) showed decomposition to mixed fluorite and pyrochlore phases during lower temperature anneals, indicating entropic stabilization. Comparison with prior work shows a temperature dependence of the critical δ A for phase stability, and compositions near it are expected to be entropy stabilized.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Cooling Mixed A-Site Halide Perovskites: Impact of Temperature on Optical and Structural Properties

The widespread utilization of perovskite-based photovoltaics requires probing both the structural and optical properties under extreme operating conditions to gain a holistic understanding of the material behavior under stressors. Here, in this study, we investigate the temperature-dependent behavior of mixed A-site cation lead triiodide perovskite thin films (85% methylammonium and 15% formamidinium) in the range from 300 to 20 K. Through a combination of optical and structural techniques, we find that the tetragonal-to-orthorhombic phase transition occurs at similar to 110 K for this perovskite composition, as indicated by the change in the diffraction pattern. With decreasing temperature, the quantum yield increases with a concurrent elongation of the carrier lifetimes, indicating suppression of nonradiative recombination pathways. Interestingly, in contrast to single A-site cation perovskites, an additional optical transition appears in the absorption spectrum when the phase transition is approached, which is also reflected in the emission spectrum. We propose that the splitting of the optical absorption and emission is due to local segregation of the mixed cation perovskite during the phase transition.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Quantifying the Diversity of an Atmospheric Aerosol Population in an Arctic Oil Field on a Single‐Particle Level

As the Arctic rapidly warms, sea ice extent is decreasing and oil and gas extraction activities are expanding. Local combustion emissions affect the Arctic atmospheric aerosol chemical mixing state (the distribution of chemical species across the aerosol population), which impacts climate-relevant properties. Bulk and single-particle measurements of submicron aerosols were conducted at Oliktok Point, Alaska within the North Slope of Alaska oil fields. In this work, we quantify aerosol diversity using online single-particle mass spectrometry data (32,880 individual particles), offline single-particle microscopy data (20,912 individual particles), and online bulk aerosol mass spectrometry and aethalometer data. This method was used to derive individual particle mass fractions for both refractory and non-refractory material within distinct particle types. Single-particle, average single-particle, and bulk population diversities (D i , D α , D γ , respectively) and mixing state indices (χ) were calculated for the data set. Calculated D i values were generally low (2.2 ± 0.6), as individual particle masses were dominated by a few chemical species of interest. Aged aerosol particles (those internally mixed with nitrate and/or sulfate) exhibited higher D i values (>3) compared to recently emitted (fresh) aerosol particles. During oil field plume periods, D α values approached three due to the abundance of diesel combustion particles, which were rich in sulfate, black carbon, and organic aerosol. Overall, the submicron aerosol population within the Arctic oil fields was found to be relatively externally mixed (χ < 50%), due to the constant local emissions within oil fields combining with background aerosol and locally emitted sea spray aerosol at the coastal site.

Wu, J.↗
DOE OSTI2020

Ionization wave propagation in a He plasma jet in a controlled gas environment

Characterizing ionization wave propagation in low temperature plasma jets is critical to predicting production of reactive species and plasma–surface interactions for biomedical applications and surface functionalization. In this work, results from optical emission and laser induced fluorescence measurements of the ionization wave in a He plasma jet operating in a controlled gas environment are discussed and used for comparison with numerical modeling. Additionally, the ionization wave was observed using ICCD (Intensified Charge Coupled Device) imaging and characterized by time and spatially resolved electron density measurements using laser-collision-induced fluorescence. The plasma jet was initially characterized using pure He (nominally at 200 Torr), while varying pressure and voltage. When operating in pure He, the ionization wave broadly expands exiting the plasma tube. Increasing the operating pressure reduces the speed and isotropic expansion of the ionization wave. Furthermore, the jet operated with a humid He shroud was also studied. The humid He shroud results in the electron density increasing and having an annular profile due to the lower ionization potential of H2O compared to He and localized photoionization in the mixing region. Numerical modeling highlighted the importance of resonance radiation emitted by excited states of He, photoelectron emission from the quartz tube, and the kinetic behavior of the electrons produced by photoionization ahead of the ionization front.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Imaging quantum melting in a disordered 2D Wigner solid

Two-dimensional strongly interacting electrons crystalize into a solid phase known as the Wigner crystal at low densities and form a Fermi liquid at high densities. At intermediate densities, the two-dimensional solid evolves into a strongly correlated liquid phase around a critical density. We observed this quantum melting of a disordered Wigner solid in bilayer molybdenum diselenide (MoSe2) using a noninvasive scanning tunneling microscopy imaging technique. At low densities, the Wigner solid forms nanocrystalline domains pinned by local disorder. It exhibits a quantum densification behavior with increased densities in the solid phase. Above a threshold density, the Wigner solid melts locally and enters a mixed phase in which solid and liquid regions coexist. The liquid regions expand and form a percolation network at even higher densities.

Xiang, Ziyu↗
DOE OSTI2024

Historical Subsurface Cooling in the Tropical Pacific and Its Dynamics

Abstract Understanding how the tropical Pacific responds to rising greenhouse gases in recent decades is of paramount importance given its central role in global climate systems. Extensive research has explored the long-term trends of tropical Pacific sea surface temperatures (SSTs) and the overlying atmosphere, yet the historical change in the upper ocean has received far less attention. Here, we present compelling evidence of a prominent subsurface cooling pattern along the thermocline in the central-to-eastern tropical Pacific since 1958. This subsurface cooling has been argued to be contributing to the observed cooling or lack of warming of the equatorial cold tongue SST. We further demonstrate that different mechanisms are responsible for different parts of the subsurface cooling. In the central-to-eastern equatorial Pacific and the southeastern off-equatorial Pacific, where zonal wind stress strengthens, a pronounced subsurface cooling trend emerges just above the thermocline that is closely tied to increased Ekman pumping. In the eastern equatorial Pacific where zonal wind stress weakens, the westward surface current and eastward Equatorial Undercurrent weaken as well, resulting in reduced vertical current shear and increased ocean stability, which suppresses vertical mixing and leads to local cooling. We conclude that the historical subsurface cooling is primarily linked to dynamical adjustments of ocean currents to tropical surface wind stress changes.

Jiang, Feng↗
DOE OSTI2025

American WAKE Experiment (AWAKEN) Field Campaign Report

The American WAKE experimeNt (AWAKEN) was a large-scale, international collaborative field campaign funded primarily by the U.S. Department of Energy (DOE) Wind Energy Technologies Office. Its main purpose was to gather detailed observations of wind farm-atmosphere interactions to improve understanding of wind farm physics, validate and improve simulation tools, lower uncertainties in wind farm modeling, understand environmental impacts, and ultimately reduce the cost and increase the reliability of wind energy systems. The campaign specifically focused on seven testable hypotheses that include characterizing wind turbine and wind farm wake effects, wind farm blockage, turbulent mixing, structural loading impacts, local environmental impacts, and testing wind farm control technologies. AWAKEN was a highly collaborative effort involving numerous agencies, including: DOE, through the Wind Energy Technologies Office and the Office of Science Atmospheric Radiation Measurement (ARM) User Facility, the U.S. Department of Commerce through the National Oceanic and Atmospheric Administration, many American universities, and internationally funded collaborators from Germany and Brazil.

17 WIND ENERGY↗
NASA NTRS1975

Integrated investigation of the mixed origin of lunar sample 72161,11

The comminution-agglutination model and the solar-wind implantation-retention model are used to postulate the origins of the particulate components of lunar sample (72161,11), a submillimeter fraction of a surface sample for the dark mantle regolith at LRV-3. Grain-size analysis was performed by wet sieving with liquid argon, and analyses for CO2, CO, CH4, and H2 were carried out by stepwise pyrolysis in a helium atmosphere. The results indicate that the present sample is from a mature regolith, but the agglutinate content is only 30% in the particle-size range between 90 and 177 microns, indicating an apparent departure from steady state. Analyses of the carbon, methane, and hydrogen concentrations in size fractions larger than 149 microns show that the volume-correlated component of these species increases with increased grain size. It is suggested that the observed increase can be explained in terms of mixing of a dominant local population of coarser agglutinates having high carbon and hydrogen concentrations with an imported population of finer agglutinates relatively poor in carbon and hydrogen.

Basu, A.↗
NASA NTRS1979

Complex igneous processes and the formation of the primitive lunar crustal rocks

Crystallization of a magma ocean with initial chondritic Ca/Al and REE ratios such as proposed by Taylor and Bence (TB, 1975), is capable of producing the suite of primitive crustal rocks if the magma ocean underwent locally extensive assimilation and mixing in its upper layers as preliminary steps in formation of an anorthositic crust. Lunar anorthosites were the earliest permanent crustal rocks to form the result of multiple cycles of suspension and assimilation of plagioclase in liquids fractionating olivine and pyroxene. There may be two series of Mg-rich cumulate rocks: one which developed as a result of the equilibration of anorthositic crust with the magma ocean; the other which formed in the later stages of the magma ocean during an epoch of magma mixing and ilmenite crystallization. This second series may be related to KREEP genesis. It is noted that crystallization of the magma ocean had two components: a low pressure component which produced a highly fractionated and heterogeneous crust growing downward and a high pressure component which filled in the ocean from the bottom up, mostly with olivine and low-Ca pyroxene.

Longhi, J.↗
NASA NTRS1981

Polarization characteristics of hydromagnetic waves at low geomagnetic latitudes

A field campaign, using three magnetometer stations spaced in latitude around the equatorial magnetic field distance L approximately 1.9, was conducted in early 1979 to investigate the polarization characteristics of hydromagnetic waves at low geomagnetic latitudes. The magnetic pulsations are observed to have periods in the range approximately 20-25 s and to occur primarily in the local morning hours. Statistically, the polarizations at all three stations were predominantly left handed in the local morning hours and right handed in the local afternoon. At the highest-latitude station (L approximately 2) the orientation of the major axis of the polarization ellipse changed from a predominantly NW-SE direction in the local morning to a mixed NW-SE/NE-SW direction in the afternoon. These two statistical results are consistent with the excitation of the waves by the Kelvin-Helmholtz instability at the magnetopause. However, frequent changes in phase are often observed in the magnetic variations, which result in polarization variations on the time scale of minutes, a situation not readily reconcilable with the Kelvin-Helmholtz instability. The existence of the waves at very low latitudes, furthermore, places constraints on the damping rate of externally excited surface waves inside the magnetosphere. We conclude that present theories for hydromagnetic waves in the geomagnetosphere cannot readily incorporate all of these low-latitude results.

Lanzerotti, L. J.↗
NASA NTRS1982

The Reiner Gamma Formation - Composition and origin as derived from remote sensing observations

In order to investigate the composition and origin of Reiner Gamma, near-infrared spectra and vidicon images were obtained and interpreted. The 0.40/0.56 micron ratio image shows that the high albedo portion of Reiner Gamma is surrounded by a 'red halo' and the 0.95/0.56 micron image indicates that Reiner Gamma exhibits a strong pyroxene absorption band. Analysis of the near-infrared spectra of various portions of the formation indicated the presence of major amounts of fresh mare basalt. Spectral mixing models demonstrate that the Reiner Gamma spectra can be reproduced by mixing major amounts of local fresh mare material (Reiner K crater) with small amounts of fresh highlands material (Oelbers A crater). No evidence was found for the presence of 'exotic' components (i.e., magnetite, free iron, cometary material). Together with photogeologic considerations, these results suggest that Reiner Gamma is quite young and is composed of a mixture of fresh highland materials with much larger quantities of local mare basalt.

Bell, J. F.↗
NASA NTRS1982

The lunar regolith - Chemistry, mineralogy, and petrology

The data base on the lunar regolith is surveyed to form a synthesis of the lunar regolith chemistry, mineralogy, and petrology. The data were derived from samples collected by the Apollo missions 11-17 and the Luna 16, 20, and 24 probes. The missions were sent to sample formations and areas which typified the common observed features of the lunar surface. Drive tubes were used to extract samples from beneath the surface in order to study the relationship between the regolith and the bedrock, as well as to identify the processes that formed the regolith, which is regarded as the prime source of raw materials for early lunar industrial activities. Regolith origins are now understood to be destructive processes of comminution and constructional processes of agglutinate formation. Mixing occurs on the local scale, although lateral transport is inefficient on the moon. The usual contents of the fraction of regolith less than 10 microns in diameter are Al2O3, CaO, Na2O, K2O, light REE, and Th.

Papike, J. J.↗
NASA NTRS1988

Efficiency of shear induced entrainment in convectively mixed layers

Lidar data of mixed layer height are used to compare the model of process partitioning to that of Eulerian partitioning. It is found that the Eulerian partitioning model more closely follows the data and that the process partitioning model underpredicts the mixed layer depth. The results suggest that shear production and consumption of turbulent kinetic energy at the mixed layer top are local processes.

Boers, Reinout↗
NASA NTRS2004

Counting Magnetic Bipoles on the Sun by Polarity Inversion

This paper presents a simple and efficient algorithm for deriving images of polarity inversion from NSO/Kitt Peak magnetograms without use of contouring routines and shows by example how these maps depend upon the spatial scale for filtering the raw data. Smaller filtering scales produce many localized closed contours in mixed polarity regions while supergranular and larger filtering scales produce more global patterns. The apparent continuity of an inversion line depends on how the spatial filtering is accomplished, but its shape depends only on scale. The total length of the magnetic polarity inversion contours varies as a power law of the filter scale with fractal dimension of order 1.9. The amplitude but nut the exponent of this power-law relation varies with solar activity. The results are compared to similar analyses of areal distributions of bipolar magnetic regions.

Jones, Harrison P.↗
NASA NTRS2003

Turbulence in Supercritical O2/H2 and C7H16/N2 Mixing Layers

This report presents a study of numerical simulations of mixing layers developing between opposing flows of paired fluids under supercritical conditions, the purpose of the study being to elucidate chemical-species-specific aspects of turbulence. The simulations were performed for two different fluid pairs O2/H2 and C7H16/N2 at similar reduced initial pressures (reduced pressure is defined as pressure divided by critical pressure). Thermodynamically, O2/H2 behaves more nearly like an ideal mixture and has greater solubility, relative to C7H16/N2, which departs strongly from ideality. Because of a specified smaller initial density stratification, the C7H16/N2 layers exhibited greater levels of growth, global molecular mixing, and turbulence. However, smaller density gradients at the transitional state for the O2/H2 system were interpreted as indicating that locally, this system exhibits enhanced mixing as a consequence of its greater solubility and closer approach to ideality. These thermodynamic features were shown to affect entropy dissipation, which was found to be larger for O2/H2 and concentrated in high-density-gradient-magnitude regions that are distortions of the initial density-stratification boundary. In C7H16/N2, the regions of largest dissipation were found to lie in high-density-gradient-magnitude regions that result from mixing of the two fluids.

Bellan, Josette↗
NASA NTRS2016

Secondary Crater-Initiated Debris Flow on the Moon

In recent work, radar circular polarization echo properties have been used to identify "secondary" craters without distinctive secondary morphologies. Because of the potential for this method to improve our knowledge of secondary crater population-in particular the effect of secondary populations on crater- derived ages based on small craters-it is important to understand the origin of radar polarization signatures associated with secondary impacts. In this paper, we utilize Lunar Reconnaissance Orbiter Camera photographs to examine the geomorphology of secondary craters with radar circular polarization ratio enhancements. Our investigation reveals evidence of dry debris flow with an impact melt component at such secondary craters. We hypothesize that these debris flows were initiated by the secondary impacts themselves, and that they have entrained blocky material ejected from the secondaries. By transporting this blocky material downrange, we propose that these debris flows (rather than solely ballistic emplacement) are responsible for the tail-like geometries of enhanced radar circular polarization ratio associated with the secondary craters investigated in this work. Evidence of debris flow was observed at both clustered and isolated secondary craters, suggesting that such flow may be a widespread occurrence, with important implications for the mixing of primary and local material in crater rays.

Martin-Wells, K. S.↗
NASA NTRS2017

Chemical, Mineralogical, and Physical Properties of Martian Dust and Soil

Global and regional dust storms on Mars have been observed from Earth-based telescopes, Mars orbiters, and surface rovers and landers. Dust storms can be global and regional. Dust is material that is suspended into the atmosphere by winds and has a particle size of 1-3 micrometer. Planetary scientist refer to loose unconsolidated materials at the surface as "soil." The term ''soil'' is used here to denote any loose, unconsolidated material that can be distinguished from rocks, bedrock, or strongly cohesive sediments. No implication for the presence or absence of organic materials or living matter is intended. Soil contains local and regional materials mixed with the globally distributed dust by aeolian processes. Loose, unconsolidated surface materials (dust and soil) may pose challenges for human exploration on Mars. Dust will no doubt adhere to spacesuits, vehicles, habitats, and other surface systems. What will be the impacts on human activity? The objective of this paper is to review the chemical, mineralogical, and physical properties of the martian dust and soil.

Ming, D. W.↗