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At least 163 records · Page 9
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Reaction Rate Ratios for Recent Fast Metal Experiments with Large Plutonium Masses

Reaction rate ratios are integral responses that are used within the criticality experiments field because they contain spectral information. While these types of measurements have been utilized for nuclear data validation with historic experiments, few experiments of this type have been utilized for recent experiments, as few exist. This work focuses on measured reaction rate ratios for two nearly bare plutonium critical assemblies with different geometries: one that is cube like (with a Pu mass of 40 kg) and one that is slab like (with a Pu mass of 109 kg). Irradiations were performed with both configurations in which foils were placed near the center of the assembly. Plutonium, highly enriched uranium, depleted uranium, and Au foils were included in the irradiation and counted via high-purity germanium detectors. From these measurements, reaction rate ratios were calculated. Measured and simulated values and uncertainties are presented for the reaction rate ratios. Ratios utilizing the following reactions are given in this work: 197 Au(n, γ), 197 Au(n,2n), 235 U(n,fission), 238 U(n, fission), 238 U(n,2n), 238 U(n,γ), and 239 Pu(n,fission). Uncertainties for the measured reaction rate ratios ranged from 4% to 7%, and the contribution of various parameters to this uncertainty was investigated. The results are compared to historical experiments and should be used for nuclear data validation for future nuclear data library releases. These measurements are part of the EUCLID (Experiments Underpinned by Computational Learning for Improvements in Nuclear Data) project, which utilizes measurement responses in addition to k eff (such as these reaction rate ratios) to help reduce uncertainties in 239 Pu nuclear data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Design Report on the MiniFuel Instrumented Test Apparatus for Understanding Radiation Effects

Most nuclear fuels irradiations at Oak Ridge National Laboratory (ORNL) over the past decade have been conducted using MiniFuel—a static capsule design employing subscale fuel specimens to collect separate-effects irradiated fuel performance data. Irradiation conditions for MiniFuel experiments are predicted pre-test using reactor physics, and thermal models are verified post-irradiation via SiC dilatometry and various spectrometry methods. Relevant fuel performance parameters are also observed post-irradiation in a hot cell, thereby providing a single data point for each parameter representing the cumulative effects of the irradiation conditions. Substantially more data can be harvested from a single test and within a shorter duration by instrumenting irradiation vehicles and measuring desired quantities in situ. This report presents the design and analysis of the MiniFuel INstrumented Irradiation Test Apparatus for Understanding Radiation Effects (MINITAURE)—an instrumented test rig based on the separate-effects MiniFuel concept that aims to capture fission gas release (FGR) and thermal conductivity degradation of fuel specimens during irradiation in the High Flux Isotope Reactor (HFIR). MINITAURE will be integrated with the Materials Irradiation Facility (MIF) located in the HFIR building outside the reactor containment. The MIF will act as the instrumentation and control center for the experiment, enabling real-time feedback from in situ sensors and control of irradiation temperatures via a gas delivery system. Two unique capsule designs were developed to capture each phenomenon: the thermal conductivity capsule, which uses a thermopile method to estimate fuel specimen thermal conductivity, and the fission gas release capsule, which will have continuous flowing gas communication to high-purity germanium detectors that are housed in the MIF for monitoring FGR. This report details the reactor physics and heat transfer modeling activities that were used to inform the experiment design and predict capsule performance. It also describes out-of-pile activities conducted to stand up this new capability and verify the measurement techniques. Modeling efforts to date have demonstrated the feasibility of the in situ measurement techniques and supported the development of the MINITAURE assembly configuration. Out-of-pile testing of the thermal conductivity measurement shows promise in capturing relative changes in thermal conductivity. However, significant errors exist in the measured absolute value, posing a need for further refinement.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2025

Variance Preserving Spectral Subsampling

Generating statistically faithful short-duration gamma-ray spectra from a single long measurement is essential in nuclear safeguards, supporting tasks such as algorithm development and machine-learning applications, especially when list-mode data are unavailable. Existing subsampling methods often distort the statistical characteristics of genuine short-duration measurements, leading to biased or unreliable analytical outcomes and thereby undermining downstream tasks. In this work, we compare five subsampling approaches using a benchmark set of 156 genuine replicate spectra collected with a high-purity germanium detector. We evaluate each method with respect to run-to-run variance, channel-to-channel variance, and preservation of total counts (losslessness). Across a wide range of subsampling ratios, only binomial subsampling without replacement consistently reproduces the statistical properties of genuine short-duration spectra, maintaining proper dispersion even in sparse spectral regions and perfectly preserving total counts. These results provide a mathematically principled and practically validated framework for generating synthetically shortened spectra when true short-duration measurements are unavailable.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗
NASA NTRS1973

Feasibility of an on-line fission-gas-leak detection system

Calculations were made to determine if a cladding failure could be detected in a 100-kW zirconium hydride reactor primary system by monitoring the highly radioactive NaK coolant for the presence of I-131. The system is to be completely sealed. A leak of 0.01 percent from a single fuel pin was postulated. The 0.364-MeV gamma of I-131 could be monitored on an almost continuous basis, while its presence could be varified by using a longer counting time for the 0.638-MeV gamma. A lithium-drifted germanium detector would eliminate radioactive corrosion product interference that could occur with a sodium iodide scintillation detector.

Lustig, P. H.↗
NASA NTRS1976

Development of doped-germanium photoconductors for astronomical observations at wavelengths from 30 to 120 micrometers

Technology was developed for production of doped-germanium detectors which have optimized performance in the 30- to 120-micrometer wavelength range and are capable of achieving the objectives of the Infrared Astronomy Satellite space mission. The work of this phase was divided into the following major tasks: (1) growth of Ge:Ga crystals from high-purity starting material with Ga concentrations different from that previously produced, and development of a zone leveling method to produce a uniform Ga doping concentration; (2) growth of uncompensated Ge:Be crystals from high-purity starting material with a range of Be concentrations between 10 to the 14th power and 10 to the 16th power atoms/cubic cm; (3) evaluation of crystals by means of Hall effect and resistance measurements as a function of temperature; (4) fabrication and test of detectors made from both Ge:Be and Ge:Ga crystals to determine the relative performance between different crystals. Correlation of detector test data with material evaluation data and analysis of how to further optimize detector performance.

Bratt, P. R.↗
NASA NTRS1978

Continued development of doped-germanium photoconductors for astronomical observations at wavelengths from 30 to 120 micrometers

The development of doped-germanium detectors which have optimized performance in the 30- to 120-mu m wavelength range and are capable of achieving the objectives of the infrared astronomical satellite (IRAS) space mission is discussed. Topics covered include the growth and evaluation of Ge:Ga and Ge:Be crystals, procedures for the fabrication and testing of detectors, irradiance calculations, detector responsivity, and resistance measurements through MOSFET. Test data are presented in graphs and charts.

Bratt, P. R.↗
NASA NTRS1978

Detection of 511 keV positron annihilation radiation from the galactic center direction

A balloon-borne gamma ray telescope with an approximately 130 cu cm high purity germanium detector was flown over Australia to detect sharp spectral features from the galactic center direction. A 511 keV positron annihilation line was observed at a flux level of (1.21 plus or minus 0.22) x (10/cu cm) photons/sec/sp cm. Suggestive evidence for the detection of the three-photon positronium continuum is presented. The possible origin of the positrons is discussed.

Leventhal, M.↗
NASA NTRS1981

Spectroscopy from 2 to 200 keV

The astrophysical processes responsible for line and continuum emission in the spectra range 2 keV to 200 keV are examined from the viewpoint of designing a spectrometer which would operate in this regime. Phenomena considered include fluorescent line radiation in X-ray binaries, magnetically shifted iron lines and cyclotron emission from neutron star surfaces, line emission from cosmically abundant elements in thermal plasmas, and nuclear deexcitation lines in fresh nucleosynthetically produced matter. An instrument consisting of a approximately 10 sq cm array of planar germanium detectors surrounded by a large sodium-iodide anticoincidence shield is described and projected background rates and sensitivities are considered. A sample observing program for a two-day shuttle-based mission is included as an example of the wide range of scientific questions which could be addressed by such an instrument.

Helfand, D. J.↗
NASA NTRS1981

Hard X-ray astrophysics

Past hard X-ray and lower energy satellite instruments are reviewed and it is shown that observation above 20 keV and up to hundreds of keV can provide much valuable information on the astrophysics of cosmic sources. To calculate possible sensitivities of future arrays, the efficiencies of a one-atmosphere inch gas counter (the HEAO-1 A-2 xenon filled HED3) and a 3 mm phoswich scintillator (the HEAO-1 A-4 Na1 LED1) were compared. Above 15 keV, the scintillator was more efficient. In a similar comparison, the sensitivity of germanium detectors did not differ much from that of the scintillators, except at high energies where the sensitivity would remain flat and not rise with loss of efficiency. Questions to be addressed concerning the physics of active galaxies and the diffuse radiation background, black holes, radio pulsars, X-ray pulsars, and galactic clusters are examined.

Rothschild, R. E.↗
NASA NTRS1981

HEAO 3 measurements of the atmospheric positron annihilation line

The atmospheric positron annihilation line at 511 keV was the first gamma-ray line observed which originates from processes of astrophysical importance. Measurements of the properties of a positron annihilation line make it possible to determine many of the physical conditions present at the source of emission. An investigation was conducted of the 511-keV line measured with the HEAO C-1 experiment. The HEAO C-1 experiment consisted of a cluster of four, large, high-purity germanium detectors surrounded by an active anticoincidence CsI shield. A strong atmospheric line was measured at 511.07 + or - 0.10 keV. The net atmospheric emission has been accurately determined as a function of geomagnetic latitude and varies from 0.01 photons/sq cm-sec-sr near the magnetic equator to 0.035 photons/sq cm-sec-sr at a latitude of 55 deg.

Mahoney, W. A.↗
NASA NTRS1982

A high-resolution measurement of the 2.223 MeV neutron capture line in a solar flare

An intense solar flare lasting 40 s was observed by the HEAO 3 gamma-ray spectrometer on November 9, 1979, at 3:05 UT. The flare was observed in four high-resolution germanium detectors as well as in five CsI shield detectors over an energy range of 100 keV to above 5 MeV. Of particular interest is a line feature at 2.2248 + or - 0.0010 MeV. The precise energy measurement provides unambiguous evidence that this is the (H-1)(n, gamma)(H-2) line resulting from neutron capture on hydrogen. An upper limit of 5 keV is found for the natural line width. The time dependence of the neutron capture line is discussed as well as the overall characteristics of the November 9 flare.

Prince, T. A.↗
NASA NTRS1982

The HEAO-3 high resolution gamma-ray spectrometer

Features and results produced by the HEAO 3 spacecraft gamma ray spectrometer are outlined. The instrument had high resolution germanium detectors, each 55 mm diam and 45 mm long, surrounded by a cesium iodide anticoincidence shield with four quadrants of well-crystal and a collimayor crystal. The crystals had a total effective area of 70 sq cm at 100 keV and 26.4 sq cm at .511 MeV with a spectral resolution at launch of .23 percent at 1.33 MeV. The spacecraft travels a circular orbit of 500 km altitude with an inclination of 43.6 deg. Solid methane and ammonia cryogenic fluids refrigerated the crystals for 8.5 mos, after which the shield crystals functioned as isotropic detectors for solar flare events and gamma ray bursts until mission termination in May 1981. A total of 37 solar flare type events were observed, with gamma ray events occurring with flares of class X1 or stronger.

Jacobson, A. S.↗
NASA NTRS1982

Gamma-ray and optical observations of the 1979 November 8 solar flare

The solar flare on 1979 November 8 11h 21m 28s UT was observed by the Tel Aviv telescope of the Big Bear Solar Observatory and the High Resolution Gamma-Ray Spectrometer on the High Energy Astronomy Observatory HEAO 3. Photographs in alpha hydrogen show the development of the flare and a subsequent Moreton wave. Although the flare was not detected with the high spectral resolution germanium detectors, the HEAO C-1 CsI shield detected a statistically significant signal above 80 keV, from 420 to 585 keV, and above 3.8 MeV. The temporal structure of microwave, optical, X-ray, and gamma-ray emission is consistent to within about 1 s with a simultaneous flare response at all energies. There is no evidence for either second-stage acceleration of charged particles (Bai and Ramaty, 1979) or a delay between gamma-ray and X-ray continuum emission due to energy-dependent electron energy loss times (Bai and Ramaty).

Riegler, G. R.↗
NASA NTRS1983

A balloon-borne instrument for high-resolution astrophysical spectroscopy in the 20-8000 keV energy range

The Low Energy Gamma ray Spectrometer (LEGS) is designed to perform fine energy resolution measurements of astrophysical sources. The instrument is configured for a particular balloon flight with either of two sets of high purity germanium detectors. In one configuration, the instrument uses an array of three coaxial detectors (effective volume equal to or approximately 230 cubic cm) inside an NaI (T1) shield and collimator (field of view equal to or approximately 16 deg FWHM) and operates in the 80 to 8000 keV energy range. In the other configuration, three planar detectors (effective area equal to or approximately square cm) surrounded by a combination of passive Fe and active NaI for shielding and collimation (field of view equal to or approximately 5 deg x 10 deg FWHM) are optimized for the 20 to 200 keV energy range. In a typical one day balloon flight, LEGS sensitivity limit (3 sigma) for narrow line features is less than or approximately .0008 ph/cm/s square (coaxial array: 80 to 2000 keV) and less than or approximately .0003 ph/square cm/s (planar array: 50 to 150 keV).

Paciesas, W. S.↗
NASA NTRS1982

Gamma-ray burst observations by the HEAO-3 high-resolution gamma-ray spectrometer

Special attention is given to two bursts occurring on November 16, 1979. Because of the close temporal coincidence of the two events, the possibility that both originated from a single celestial source is considered, as is the possibility that the scanning motion of HEAO-3 (nominal spin period, 20 min) was such as to exclude the first from the (approximately 30 deg FWHM) field of view of the germanium detectors and include the second. Directional data from the relative response of the shield pieces and earth occultation constraint are found to be consistent with this interpretation, and high-resolution spectral data from the second burst are discussed in this light. It is noted that recent unpublished analyses of long-baseline timing data from interplanetary spacecraft reveal that the response in the HEAO high-resolution detectors is probably earth albedo scattering. This, it is noted, can be an important systematic effect in low-earth orbit.

Wheaton, W. A.↗
NASA NTRS1984

High resolution X- and gamma-ray spectroscopy of solar flares

A balloon-borne X- and gamma-ray instrument was developed, fabricated, and flown. This instrument has the highest energy resolution of any instrument flown to date for measurements of solar and cosmic X-ray and gamma-ray emission in the 13 to 600 keV energy range. The purpose of the solar measurements was to study electron acceleration and solar flare energy release processes. The cosmic observations were to search for cyclotron line features from neutron stars and for low energy gamma-ray lines from nucleosynthesis. The instrument consists of four 4 cm diameter, 1.3 cm thick, planar intrinsic germanium detectors cooled by liquid nitrogen and surrounded by CsI and NaI anti-coincidence scintillation crystals. A graded z collimator limited the field of view to 3 deg x 6 deg and a gondola pointing system provided 0.3 deg pointing accuracy. A total of four flights were made with this instrument. Additional funding was obtained from NSF for the last three flights, which had primarily solar objectives. A detailed instrument description is given. The main scientific results and the data analysis are discussed. Current work and indications for future work are summarized. A bibliography of publications resulting from this work is given.

Lin, R. P.↗
NASA NTRS1984

Twilight Intensity Variation of the Infrared Hydroxyl Airglow

The vibration rotation bands of the hydroxyl radical are the strongest features in the night airglow and are exceeded in intensity in the dayglow only by the infrared atmospheric bands of oxygen. The variation of intensity during evening twilight is discussed. Using a ground-based Fourier Transform Spectrometer (FTS), hydroxyl intensity measurements as early as 3 deg solar depression were made. Models of the twilight behavior show that this should be sufficient to provide measurement of the main portion of the twilight intensity change. The instrument was equipped with a liquid nitrogen-cooled germanium detector whose high sensitivity combined with the efficiency of the FTS technique permits spectra of the region 1.1 to 1.6 microns at high signal-to-noise to be obtained in two minutes. The use of a polarizer at the entrance aperture of the instrument reduces the intensity of scattered sunlight by a factor of at least ten for zenith observations.

Lowe, R. P.↗