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At least 163 records · Page 9

Tilted spin current generated by the collinear antiferromagnet ruthenium dioxide

Symmetry plays a central role in determining the polarization of spin currents induced by electric fields. It also influences how these spin currents generate spin-transfer torques in magnetic devices. Here, we show that an out-of-plane damping-like torque can be generated in ruthenium oxide (RuO 2 )/permalloy devices when the Néel vector of the collinear antiferromagnet RuO 2 is canted relative to the sample plane. By measuring characteristic changes in all three components of the electric-field-induced torque vector as a function of the angle of the electric field relative to the crystal axes, we find that the RuO 2 generates a spin current with a well-defined tilted spin orientation that is approximately parallel to the Néel vector. A maximum out-of-plane damping-like spin torque efficiency per unit electric field of 7±1 × 10 3 Ω -1 m -1 is measured at room temperature. Here, the observed angular dependence indicates that this is an antiferromagnetic spin Hall effect with symmetries that are distinct from other mechanisms of spin-current generation reported in antiferromagnetic and ferromagnetic materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Switchable electronic and enhanced magnetic properties of CrI 3 edges

Owing to its novel electronic and magnetic properties, two-dimensional CrI 3 has great potential in the application of spintronic devices. However, as an inevitable line defect, the properties of the edges of CrI 3 remain elusive. Here, via first-principles calculations with spin–orbit coupling, we investigated the thermodynamic stabilities, electronic and magnetic properties of thirteen CrI 3 edges with different structures. We showed that zigzag edges are more stable than armchair edges, and a CrI 3 nanoribbon can be either metallic or insulating depending on its chemical growth conditions. Here, the edge stability and associated electronic properties can be understood in terms of the octahedron ligand field and electron counting model. In most cases, both the magnetic moment and Curie temperature can be enhanced by edges, which are in startle contrast to the surfaces of three-dimensional ferromagnetic materials, where a magnetic dead layer is often observed.

36 MATERIALS SCIENCE↗

Giant magnetostriction in Tb-doped Fe{sub 83}Ga{sub 17} melt-spun ribbons

Giant magnetostriction is achieved in lightly Tb-doped Fe{sub 83}Ga{sub 17} melt-spun ribbons. The average perpendicular magnetostriction λ{sub ⊥} is −886 ppm along the melt-spun ribbon direction in the Fe{sub 82.89}Ga{sub 16.88}Tb{sub 0.23} alloy and the calculated parallel magnetostriction λ{sub ‖‖} is 1772 ppm. These values are more than four times as large as those found in binary Fe{sub 83}Ga{sub 17}. The enhanced magnetostriction is attributed to a small amount of Tb entering solution in the A2 matrix phase during rapid solidification. The strong localized magnetocrystalline anisotropy of terbium is thought to cause the giant magnetostriction.

36 MATERIALS SCIENCE↗

Neutron diffraction study of MnNiGa{sub 2}—Structural and magnetic behaviour

MnNiGa{sub 2} crystallizes in the L21 (Heusler) structure and has a ferromagnetic ordering temperature T{sub C} ∼ 192 K. Rietveld refinement of the neutron diffraction patterns indicates that the Ga atoms occupy the equivalent 8c position, while Mn and Ni share the 4a (0, 0, 0) and 4b (0.5, 0.5, 0.5) sites with a mixed occupancy of Mn and Ni atoms. It is found that that ∼83% of Mn and ∼17% Ni are located at the 4a site while ∼83% of Ni and ∼17% Mn occupy the 4b site. There is no evidence of a magneto-volume effect around T{sub C}. In agreement with this finding, our detailed critical exponent analyses of isothermal magnetization curves and the related Arrott plots confirm that the magnetic phase transition at T{sub C} is second order.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Structural and magnetic properties of irradiated SiC

We present a comprehensive structural characterization of ferromagnetic SiC single crystals induced by Ne ion irradiation. The ferromagnetism has been confirmed by electron spin resonance, and possible transition metal impurities can be excluded to be the origin of the observed ferromagnetism. Using X-ray diffraction and Rutherford backscattering/channeling spectroscopy, we estimate the damage to the crystallinity of SiC, which mutually influences the ferromagnetism in SiC.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Dynamics of skyrmions in chiral magnets: Dynamic phase transitions and equation of motion

We study the dynamics of skyrmions in a metallic chiral magnet. First, we show that skyrmions can be created dynamically by destabilizing the ferromagnetic background state through a spin polarized current. We then treat skyrmions as rigid particles and derive the corresponding equation of motion. The dynamics of skyrmions is dominated by the Magnus force, which accounts for the weak pinning of skyrmions observed in experiments. Finally, we discuss the quantum motion of skyrmions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Perfect spin-valley filter controlled by electric field in ferromagnetic silicene

The spin-valley currents in silicene-based normal/sublattice-dependent ferromagnetic/normal junction are investigated. Unlike that in graphene, the pseudo Dirac mass in silicene is generated by spin-orbit interaction and tunable by applying electric or exchange fields into it. This is due to silicon-based honeycomb lattice having buckled structure. As a result, it is found that the junction leads to currents perfectly split into four groups, spin up (down) in k- and k{sup ′}-valleys, when applying different values of the electric field, considered as a perfect spin-valley polarization (PSVP) for electronic application. The PSVP is due to the interplay of spin-valley-dependent Dirac mass and chemical potential in the barrier. The PSVP also occurs only for the energy comparable to the spin-orbit energy gap. This work reveals potential of silicene for spinvalleytronics applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Enhanced magnetic anisotropy in cobalt-carbide nanoparticles

An outstanding problem in nano-magnetism is to stabilize the magnetic order in nanoparticles at room temperatures. For ordinary ferromagnetic materials, reduction in size leads to a decrease in the magnetic anisotropy resulting in superparamagnetic relaxations at nanoscopic sizes. In this work, we demonstrate that using wet chemical synthesis, it is possible to stabilize cobalt carbide nanoparticles which have blocking temperatures exceeding 570 K even for particles with magnetic domains of 8 nm. First principles theoretical investigations show that the observed behavior is rooted in the giant magnetocrystalline anisotropies due to controlled mixing between C p- and Co d-states. (C) 2014 AIP Publishing LLC.

El-Gendy, AA↗

Ultrafast reduction of the total magnetization in iron

Surprisingly, if a ferromagnet is exposed to an ultrafast laser pulse, its apparent magnetization is reduced within less than a picosecond. Up to now, the total magnetization, i.e., the average spin polarization of the whole valence band, was not detectable on a sub-picosecond time scale. Here, we present experimental data, confirming the ultrafast reduction of the total magnetization. Soft x-ray pulses from the free electron laser in Hamburg (FLASH) extract polarized cascade photoelectrons from an iron layer excited by a femtosecond laser pulse. The spin polarization of the emitted electrons is detected by a Mott spin polarimeter.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Multi-state magnetoresistance in ferromagnet/organic-ferromagnet/ferromagnet junctions

Spin-dependent transport through a ferromagnetic metal/organic-ferromagnet/ferromagnet metal junction is investigated theoretically. It is demonstrated that the current through the device strongly depends on the alignment of the magnetization orientations of the electrodes and interlayer. The spin-related electron tunnelling between the ferromagnetic electrodes suffers a further spin selection induced by the spin-polarized states of the central organic ferromagnet. This work indicates an intriguing prospect of organic ferromagnets in spintronic devices, such as four-state magnetoresistance manipulated by a magnetic field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Resonant spin and valley polarization in ferromagnetic silicene quantum well

We propose a silicene-based lateral resonant tunneling device by placing silicene under the modulation of top nonmagnetic/ferromagnetic/nonmagnetic sandwich nanogates. Following the electric-tunable bandgap of silicene, lateral double-barrier structure is formed by imposing the flexible electrostatic modulation on top gates. By aligning the spin and valley-resolved confined states in magnetic well, remarkable spin/valley polarization can be accessed through spinor-relying resonant tunneling mechanism. Under the electrostatic, magnetic, and size manipulation, the confined well state can be efficiently engineered, and the observed spin and valley polarization can be further flexibly tuned, offering some helpful strategies to construct spinor-electronic logic atomically.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Micromagnetic simulations of spin-wave normal modes and the spin-transfer-torque driven magnetization dynamics of a ferromagnetic cross

We studied spin-transfer-torque (STT) switching of a cross-shaped magnetic tunnel junction in a recent report [Roy et al., J. Appl. Phys. 113, 223904 (2013)]. In that structure, the free layer is designed to have four stable energy states using the shape anisotropy of a cross. STT switching showed different regions with increasing current density. Here, we employ the micromagnetic spectral mapping technique in an attempt to understand how the asymmetry of cross dimensions and spin polarization direction of the injected current affect the magnetization dynamics. We compute spatially averaged frequency-domain spectrum of the time-domain magnetization dynamics in the presence of the current-induced STT term. At low currents, the asymmetry of polarization direction and that of the arms are observed to cause a splitting of the excited frequency modes. Higher harmonics are also observed, presumably due to spin-wave wells caused by the regions of spatially non-uniform effective magnetic field. The results could be used towards designing a multi-bit-per-cell STT-based random access memory with an improved storage density.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Spin wave based parallel logic operations for binary data coded with domain walls

We numerically investigate the feasibility of spin wave (SW) based parallel logic operations, where the phase of SW packet (SWP) is exploited as a state variable and the phase shift caused by the interaction with domain wall (DW) is utilized as a logic inversion functionality. A designed functional element consists of parallel ferromagnetic nanowires (6 nm-thick, 36 nm-width, 5120 nm-length, and 200 nm separation) with the perpendicular magnetization and sub-μm scale overlaid conductors. The logic outputs for binary data, coded with the existence (“1”) or absence (“0”) of the DW, are inductively read out from interferometric aspect of the superposed SWPs, one of them propagating through the stored data area. A practical exclusive-or operation, based on 2π periodicity in the phase logic, is demonstrated for the individual nanowire with an order of different output voltage V{sub out}, depending on the logic output for the stored data. The inductive output from the two nanowires exhibits well defined three different signal levels, corresponding to the information distance (Hamming distance) between 2-bit data stored in the multiple nanowires.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Giant enhancement of spin pumping in the out-of-phase precession mode

We theoretically study the spin pumping from the two ferromagnetic layers embedded in a normal metal and investigate the spin current and spin accumulation generated by the precessing magnetizations, focusing on their dependence on the relative precessional motion and the layer separation. We demonstrate a giant enhancement of spin pumping induced in the out-of-phase precession mode of the magnetizations in which the pumped spin current and spin accumulation are greatly enhanced compared to those in the in-phase precession mode. The giant enhancement of spin pumping is discussed in relation to an enhanced Gilbert damping.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Spin-orbit torque opposing the Oersted torque in ultrathin Co/Pt bilayers

Current-induced torques in ultrathin Co/Pt bilayers were investigated using an electrically driven ferromagnetic resonance technique. The angle dependence of the resonances, detected by a rectification effect as a voltage, was analysed to determine the symmetries and relative magnitudes of the spin-orbit torques. Both anti-damping (Slonczewski) and field-like torques were observed. As the ferromagnet thickness was reduced from 3 to 1 nm, the sign of the sum of the field-like torque and Oersted torque reversed. This observation is consistent with the emergence of a Rashba spin orbit torque in ultra-thin bilayers.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Optical demagnetization in defect-mediated ferromagnetic ZnO:Cu films

Optical demagnetization effect has been observed in a defect-rich ZnO:Cu film. Phenomenally, UV illumination can effectively quench dual-donor oxygen vacancy (V{sub O}) and interstitial zinc (Zn{sub i}) mediated magnetic ordering (90% loss) with carrier recapture in ionized Zn{sub i} (Zn{sub i}{sup 2+} rather than Zn{sub i}{sup +}) traps. The involvement of carriers by means of metal Zn vapor annealing provides a bound carrier related magnetic scenario, stressing a more significant place of bound carrier rather than free carrier. Using light correlated electron spin resonance and magnetic measurements, the magnetic “on” and “off” state can be continuously manipulated via UV light, which is explained by the reversible process of [Cu{sub s}{sup +}/Cu{sub s}{sup 2+}] + Zn{sub i}{sup 2+} ↔ [Cu{sub s}{sup +}, h] + Zn{sub i}{sup +} (s and h denote the substitutional Cu ions on Zn sites in ZnO lattice and hole carrier, respectively). A slow charge-transfer process (∼15 μs) from Zn{sub i}{sup +} bound carriers to [Cu{sub s}{sup +}, h] states determines the unexpected optical demagnetization, well corresponding to control experiments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Impact of interplay between magnetic field, transformation strain, and coarsening on variant selection in L1{sub 0}-type FePd

Variant selection of L1{sub 0}-type ferromagnetic alloys has been numerically investigated using the phase-field modeling, to clarify the phenomena at greater temporal and spatial resolution and to reveal the underlying mechanism. The duration for which the external magnetic field is effective is found to be very short, and variant selection is significantly affected by not only direct response to the external magnetic field but also their interplay between the field, intrinsic transformation strain, and various thermodynamic energy components involved in the course of microstructure evolution. The detailed mechanism of the interplay was quantitatively analyzed in terms of the driving force for the variant selection, by partitioning it into the various energy components. Careful examination of the variant selection at the very early stage revealed that the slight difference in size and configuration of variants during disorder-to-order transition realized by the interplay between transformation strain and external field is essentially needed before proceeding to the latter stage of the variant selection driven by interface energy.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

The adsorption of h-BN monolayer on the Ni(111) surface studied by density functional theory calculations with a semiempirical long-range dispersion correction

The geometric and spin-resolved electronic structure of a h-BN adsorbed Ni(111) surface has been investigated by density functional theory calculations. Two energy minima (physisorption and chemisorption) are obtained when the dispersive van der Waals correction is included. The geometry of N atom on top site and B atom on fcc site is the most energetically favorable. Strong hybridization with the ferromagnetic Ni substrate induces considerable gap states in the h-BN monolayer. The induced π* states are spin-polarized.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗