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At least 1,603 records · Page 89
All sourcesNASA NTRSDOE OSTI
NASA NTRS1977

Laser induced photoluminiscence studies of primary photochemical production processes of cometary radicals

A tunable vacuum ultraviolet flash lamp was constructed. This unique flash lamp was coupled with a tunable dye laser detector and permits the experimenter to measure the production rates of ground state radicals as a function of wavelength. A new technique for producing fluorescent radicals was discovered. This technique called multiphoton ultraviolet photodissociation is currently being applied to several problems of both cometary and stratospheric interest. It was demonstrated that NO2 will dissociate to produce an excited fragment and the radiation can possibly be used for remote detection of this species.

Jackson, W. M.↗
NASA NTRS1977

Atmospheric lidar research applying to H2O, O2 and aerosols

Experimental research on a near infrared tunable dye laser was reported, and theoretical simulations were presented for various lidar configurations. The visible and nearinfrared wavelengths considered were suitable for observations of aerosols, water vapor, molecular oxygen pressure and temperature in the troposphere and above. The first phase of development work was described on a ruby pumped, tunable dye laser for the wavelength region 715 to 740 nanometers. Lidar simulations were summarized for measurements of H2O and for two color lidar observations of aerosols in the atmosphere.

Mcilrath, T. J.↗
NASA NTRS1977

Double resonance spectroscopy of multiple-photon excited molecules

Multiple infrared photon absorption is a quite general process which molecules can undergo when placed in a high flux of infrared energy, such as the focussed beam of a CO2 laser. In order to understand how this process works, one must be able to follow the evolution of the molecules through their internal states, populated by photon absorption. Double-resonance spectroscopy is the method of a choice for getting at this information. A system pumped by CO2 laser radiation can be examined with a tunable laser probe beam, such as that from a lead-salt diode laser. From such an experiment, one can directly observe Rabi modulation of the absorption lines, determine elementary state-to-state relaxation pathways, and locate higher excited vibrational states. Systems currently under investigation include SF6 and vinyl chloride. In suitable cases, the probe beam can be a tunable visible or UV source, such as a dye laser. Fluorescence spectroscopy can then be used to monitor the transient absorptions produced by multiple-photon excitation. Among the systems which can be examined are biacetyl and glyoxal.

Steinfeld, J. I.↗
NASA NTRS1980

Studies of laser and laser devices

The generation of tunable, infrared, and ultraviolet light, and the control of this light by mode-locking and modulation techniques are discussed. Particular emphasis is given to energy storage and extraction using atomic levels, the development of a tunable narrowband vacuum ultraviolet light source, and to the generation and applications of ultrashort optical pulses.

Harris, S. E.↗
NASA NTRS1980

Atmospheric solar absorption measurements in the 9-11 micron region using a diode laser heterodyne spectrometer

A tunable diode laser heterodyne radiometer was developed for ground based measurements of atmospheric solar absorption spectra in the 9 to 12 micron spectral range. The performance and operating characteristics of this tunable infrared heterodyne radiometer (TIHR) is discussed along with recently measured heterodyne solar absorption spectra in the 10 to 11 micron spectral region.

Harward, C. N.↗
NASA NTRS1980

RF spectrometers for heterodyne receivers

Several types of spectrometers developed for radio astronomy receivers which utilize RF filters, multiple oscillators and mixers, digital autocorrelators and acoustic/optic devices are considered. The RF spectrometer developed at GSFC to provide wide bandwidths (greater than 1 GHz) as well as high resolution (5MHz) is described. The 128 channel filter bank is divided into high and low resolution sections. The high resolution section is tunable by providing a second mixer ahead of the filter bank. This is necessary because infrared receivers which use gas lasers as local oscillators are only tunable to specific laser frequencies. To compensate for astronomical Doppler shifts and molecule frequency differences a second local oscillator and mixer is needed. A diagram of the RF section of the filter bank is shown. The RF spectrometer is shown to be the best means of achieving ultra-wide bandwidths for infrared heterodyne receivers. For high resolution with a large number of channels, the acousto/optical spectrometer is the principle instrument, particularly for balloon or space flight applications.

Buhl, D.↗
NASA NTRS1980

Submillimeter local oscillators for heterodyne spectroscopy

The major technological innovations in continuous wave (CW) submillimeter sources which are specifically suitable for application as local oscillators in heterodyne systems are reviewed. A description of the various sources is given which underscores the general principles and operating features for each type of device. Particular emphasis is placed on CW optically pumped lasers, which have had a dramatic impact as widely available sources of narrow linewidth coherent radiation. The state-of-the-art is summarized for these lasers and performance data are presented for several local oscillator packages. Optically pumped lasers are then compared and contrasted with other competing sources such as backward wave oscillators, IMPATT diodes, and Josephson junctions. By comparing their advantages and limitations for use as local oscillators, the potential applications of these different sources are projected. The prospects for increased tunability, reliability, and scalability are briefly considered, and several novel techniques for generating partially tunable radiation using Schottky diode mixers or CW Raman lasers are highlighted.

Danielewicz, E. J., Jr.↗
NASA NTRS1980

Atmospheric solar absorption measurements in the 9 to 11 mu m region using a diode laser heterodyne spectrometer

A tunable diode laser heterodyne radiometer was developed for ground-based measurements of atmospheric solar absorption spectra in the 8 to 12 microns spectral range. The performance and operating characteristics of this Tunable Infrared Heterodyne Radiometer (TIHR) are discussed along with atmospheric solar absorption spectra of HNO3, O3, CO2, and H2O in the 9 to 11 microns spectral region.

Harward, C. N.↗
NASA NTRS1980

A 10 micron heterodyne receiver for ultra high resolution astronomical spectroscopy

An improved CO2 laser heterodyne spectrometer is examined. The present system uses reflective optics to eliminate refocusing at different wavelengths, and the local oscillator is a line-center-stabilized isotopic CO2 laser. A tunable diffraction grating makes possible easy and rapid selection of over 50 transitions per isotope of CO2. The IF (0 to 1.6 GHz) from the HgCdTe photomizer is analyzed by a 128-channel filter bank, consisting of 64 tunable 5-MHz filters and 64 fixed 25-MHz RF filters. These filters provide resolving powers of about 1,000,000 to 10,000,000 and velocity resolution of 50 to 250 m/sec; their output is synchronously detected, integrated, multiplexed and stored in a buffer memory for the desired integration period. Kitt Peak observations show the wide spectral coverage, wide mixer and electronics bandwidth, and high sensitivity of the system.

Buhl, D.↗
NASA NTRS1981

Development of a diode laser heterodyne spectrometer and observations of silicon monoxide in sunspots

A state of the art, tunable diode laser infrared heterodyne spectrometer was designed and constructed for ground based observations throughout the 8 to 12 micron atmospheric window. The instrument was optimized for use with presently available tunable diode lasers, and was designed as a flexible field system for use with large reflecting telescopes. The instrument was aligned and calibrated using laboratory and astronomical sources. Observations of SiO fundamental (v = 1-0) and hot band (v = 2-1) absorption features were made in sunspots near 8 microns using the spectrometer. The data permit an unambiguous determination of the temperature pressure relation in the upper layers of the umbral atmosphere, and support the sunspot model suggested by Stellmacher and Wiehr.

Glenar, D. A.↗
NASA NTRS1982

High resolution atmospheric spectroscopy using a diode laser heterodyne spectrometer

Ultrahigh resolution (0.007 per cm) atmospheric solar absorption spectra that have been obtained from a tunable infrared heterodyne radiometer are discussed. The radiometer was developed for ground based observations in the 8-12 micron region, and tunability is achieved through the use of Pb-salt semiconductor laser local oscillators. Spectra have been obtained in a piecewise fashion from 9.1 to 11.1 microns using laser emission modes that exhibit characteristics suitable for local-oscillator operation. Spectra showing absorption features of HNO3, O3, CO2, and H2O are presented along with comparisons of experimental and synthetic spectra calculated using a line-by-line atmospheric transmission model.

Hoell, J. M., Jr.↗
NASA NTRS1981

Imaging spectroscopy; Proceedings of the Seminar, Los Angeles, CA, February 10, 11, 1981

The seminar concentrated on the science applications of spectral imaging, multispectral imaging sensors, and spectral filtering. Papers are presented on spectroscopic remote sensing for geological applications, spectral mapping of Jupiter, system design of an interferometer imaging sounder and a common module imaging spectral radiometer. Other topics discussed include the performance and application of an intensified linear self-scanned array instrument, tunable optical filtering using an interferometer for selective modulation, design studies for a spectrally agile staring sensor system, and acousto-optic tunable filters for high-resolution spectral analysis.

Norris, D. D.↗
NASA NTRS1981

Meteorological lidar developments

A research program on remote optical measurements of humidity and temperature is summarized, and new results are given of such measurements as well as new data on the near IR absorption spectrum of H2O. The basic atmospheric technique is differential absorption lidar (DIAL) using narrow band, tunable dye lasers. Approximate wavelengths are 720, 820, 940 nm (H2O) and 690, 760 nm (O2; temperature). The requisite absorption line strengths and widths are measured in a controlled environment by means of grating spectroscopy and tunable lasers. Prospects for routine lidar meteorology, even from airplane and satellite platforms, appear excellent in several important applications; the conditions and the optical properties of the atmosphere can be obtained remotely by these means.

Wilkerson, T. D.↗
NASA NTRS1983

Dye laser traveling wave amplifier

A flash lamp pumped dye laser suitable for use as an amplifier stage was developed. The desired output laser pulses are of nanosecond duration, tunable in center frequency, and of good optical quality. Its usefulness as a laser oscillator is emphasized, because it constitutes a compact, relatively efficient source of tunable dye laser light.

Davidson, F.↗
NASA NTRS1983

Balloon-borne diode-laser absorption spectrometer for measurements of stratospheric trace species

An instrument has been designed for the measurement of stratospheric trace species which utilizes tunable infrared diode lasers as sources for sensitive in situ absorption spectroscopy in selected wavelength regions. This instrument, the Balloon-Borne Laser In Situ Sensor (BLISS), is a high-resolution absorption spectrometer designed to provide measurements of the concentrations of stratospheric species and their diurnal variations. The instrument employs second-harmonic detection of the absorption of tunable diode laser (TDL) radiation (3-30 microns) in a 1 km path length defined by a retroreflector lowered 0.5 km below the BLISS gondola. Retroreflector tracking under microprocessor control is obtained using a He-Ne laser and coaligned TV camera with CID imaging. Simultaneous measurements of molecular species in the 20-40 km altitude range will be performed using four TDLs, with the predicted minimum-detectable mixing ratio at 30 km being typically less than or equal to 0.1 ppbv.

Menzies, R. T.↗
NASA NTRS1983

High-resolution lidar system for measuring the spatial and temporal structure of the mesospheric sodium layer

The design of a high-resolution tunable-dye laser-based lidar system for the study of the mesospheric sodium layer is presented and results of sodium measurements are indicated. The lidar system comprises a tunable flashlamp-pumped dye laser operating at the sodium D2 resonance line at 589.0 nm with a pulse width of 2 microsec FWHM and pulse frequency of 10 Hz and a telescope with a 1.22=m diameter Fresnel lens. Sodium profiles are obtained from the integration of 100 to 250 laser shots, with spatial and temporal resolution enhanced by two-dimensional filtering techniques. Measurements obtained over a 9-hour nighttime period illustrate the highly dynamic nature of the sodium layer, which was observed with a spatial resolution of 2 km and temporal resolution of 30 min. Observations made with a steerable apparatus have confirmed a presunrise enhancement of over 100 percent in sodium column abundance.

Gardner, C. S.↗
NASA NTRS1983

Development of compact excimer lasers for remote sensing

The capabilities of excimer lasers for remote sensing applications are illustrated in a discussion of the development of a compact tunable XeCl excimer laser for the detection of atmospheric OH radicals. Following a brief review of the operating principles and advantages of excimer lasers, measurements of the wavelength dependence of the net small signal gain coefficient of a discharge excited XeCl laser are presented which demonstrate the overlap of several absorption lines of the A-X(0,0) transition of OH near 308 nm with the wavelengths of the XeCl laser. A range of continuous narrow bandwidth tunability of from 307.6 to 308.4 nm with only a 30 percent variation in output is reported for an XeCl laser used as a double-pass amplifier for a frequency-doubled dye laser, and measurements demonstrating the detection of laser-induced fluorescence from OH in a methane-oxygen flame are also noted. The design of an oscillator-amplifier excimer system comprising a corona-preionized, transverse-discharge oscillator and amplifier is then presented. Output energies of 12-15 mJ have been achieved in the regions where injection locking was established, with energies of 8-10 mJ elsewhere.

Laudenslager, J. B.↗
NASA NTRS1984

A measurement of the vibrational band strength for the v3 band of the HO2 radical

Laboratory measurements of the v(3) band strength of HO2 using a tunable diode laser to measure the absorption strength of a vibration-rotation line in the P branch near 1080/cm are reported. The HO2 is generated in a discharge-flow system by reaction of fluorine atoms with excess H2O2: F + H2O2 - HO2 + HF. The HO2 concentration is determined from measurements of F-atom concentrations using both chemical titration with Cl2 and tunable diode laser absorption by the F-atom spin-orbit transition near 404/cm. The experimental data are consistent with a value of k(3) = (1.6 + or - 0.3) x 10 to the 12th cu cm/s and a ratio k(4)/k(1) = 1.0 + or - 0.4. The line strength for the 6(15) - 7(16)F(1) transition is 2.9 x 10 to the -21 sq cm/molecule/cm, which corresponds to a v(3) band strength of 35 + or - 9/sq cm/(STP atm). This value is a factor of 1.6 to 6 lower than previous ab initio calculations.

Zahniser, M. S.↗