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At least 1,603 records · Page 89

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DOE OSTI2021

Promoting the Selectivity of Pt/m-ZrO 2 Ethanol Steam Reforming Catalysts with K and Rb Dopants

The ethanol steam reforming reaction (ESR) was investigated on unpromoted and potassium- and rubidium-promoted monoclinic zirconia-supported platinum (Pt/m-ZrO 2 ) catalysts. Evidence from in situ diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) characterization indicates that ethanol dissociates to ethoxy species, which undergo oxidative dehydrogenation to acetate followed by acetate decomposition. The acetate decomposition pathway depends on catalyst composition. The decarboxylation pathway tends to produce higher overall hydrogen selectivity and is the most favored route at high alkali loading (2.55 wt.% K and higher or 4.25 wt.% Rb and higher). On the other hand, decarbonylation is a significant route for the undoped catalyst or when a low alkali loading (e.g., 0.85% K or 0.93% Rb) is used, thus lowering the overall H 2 selectivity of the process. Results of in situ DRIFTS and the temperature-programmed reaction of ESR show that alkali doping promotes forward acetate decomposition while exposed metallic sites tend to facilitate decarbonylation. In previous work, 1.8 wt.% Na was found to hinder decarbonylation completely. Due to the fact that 1.8 wt.% Na is atomically equivalent to 3.1 wt.% K and 6.7 wt.% Rb, the results show that less K (2.55% K) or Rb (4.25% Rb) is needed to suppress decarbonylation; that is, more basic cations are more efficient promoters for improving the overall hydrogen selectivity of the ESR process.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2016

Sulfate Separation by Selective Crystallization with a Bis-iminoguanidinium Ligand

One simple and effective method for selective sulfate separation from aqueous solutions by crystallization with a bis-guanidinium ligand, 1,4-benzene-bis(iminoguanidinium) (BBIG), is demonstrated. The ligand is synthesized as the chloride salt (BBIG-Cl) by in situ imine condensation of terephthalaldehyde with aminoguanidinium chloride in water, followed by crystallization as the sulfate salt (BBIG-SO4). Alternatively, BBIG-Cl is synthesized ex situ in larger scale from ethanol. Furthermore, the sulfate separation ability of the BBIG ligand is demonstrated by selective and quantitative crystallization of sulfate from seawater. These ligands can then be recycled by neutralization of BBIG-SO4 with aqueous NaOH and crystallization of the neutral bis-iminoguanidine, which can be converted back into BBIG-Cl with aqueous HCl and reused in another separation cycle. Finally, 35S-labeled sulfate and β liquid scintillation counting are employed for monitoring the sulfate concentration in solution. Overall, this protocol will instruct the user in the necessary skills to synthesize a ligand, employ it in the selective crystallization of sulfate from aqueous solutions, and quantify the separation efficiency.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2016

MOTION VERIFIED RED STARS (MoVeRS): A CATALOG OF PROPER MOTION SELECTED LOW-MASS STARS FROM WISE, SDSS, AND 2MASS

We present a photometric catalog of 8,735,004 proper motion selected low-mass stars (KML-spectral types) within the Sloan Digital Sky Survey (SDSS) footprint, from the combined SDSS Data Release 10 (DR10), Two Micron All-Sky Survey (2MASS) point-source catalog (PSC), and Wide-field Infrared Survey Explorer (WISE) AllWISE catalog. Stars were selected using r − i, i − z, r − z, z − J, and z − W1 colors, and SDSS, WISE, and 2MASS astrometry was combined to compute proper motions. The resulting 3,518,150 stars were augmented with proper motions for 5,216,854 earlier type stars from the combined SDSS and United States Naval Observatory B1.0 catalog (USNO-B). We used SDSS+USNO-B proper motions to determine the best criteria for selecting a clean sample of stars. Only stars whose proper motions were greater than their 2σ uncertainty were included. Our Motion Verified Red Stars catalog is available through SDSS CasJobs and VizieR.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2016

HeCS-SZ: The hectospec survey of Sunyaev–Zeldovich-selected clusters

We estimate cluster masses and velocity dispersions for 123 clusters from optical spectroscopy to compare the Sunyaev–Zeldovich (SZ) mass proxy and dynamical masses. Our new survey, HeCS-SZ (Hectospec Cluster Survey of SZ-selected clusters), includes 7721 new or remeasured redshifts from MMT/Hectospec observations of 21 SZ-selected clusters at redshifts z = 0.05–0.20. We supplement the Hectospec data with spectra from the Sloan Digital Sky Survey (SDSS) and cluster data from the Cluster Infall Regions in SDSS project and the Hectospec Cluster Survey, our Hectospec survey of clusters selected by X-ray flux. We measure the scaling relation between velocity dispersion and SZ mass estimates from the integrated Compton parameter for an SZ-complete sample of 83 clusters. The observed relation agrees very well with a simple virial scaling from mass (based on SZ) to velocity dispersion. The SZ mass estimates (calibrated with hydrostatic X-ray mass estimates) are not significantly biased compared to dynamical mass estimates under the assumption of small velocity bias of galaxies compared to dark matter particles. Significant mass bias in SZ mass estimates could relieve tension between cosmological results from Planck SZ cluster counts and Planck CMB data. In principle, SZ mass bias and velocity bias of galaxies could conspire to yield good agreement, but the required velocity bias is σ{sub galaxy}≈0.77σ{sub DM}, outside the range of recent models of velocity bias in the literature. More likely, SZ mass bias and velocity bias are both small, and the tension between SZ cluster counts and CMB data requires another explanation.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2016

Absolute integral cross sections for the state-selected ion–molecule reaction N{sub 2}{sup +}(X{sup 2}Σ{sub g}{sup +}; v{sup +} = 0–2) + C{sub 2}H{sub 2} in the collision energy range of 0.03–10.00 eV

Using the vacuum ultraviolet laser pulsed field ionization-photoion source, together with the double-quadrupole–double-octopole mass spectrometer developed in our laboratory, we have investigated the state-selected ion–molecule reaction N{sub 2}{sup +}(X{sup 2}Σ{sub g}{sup +}; v {sup +} = 0–2, N{sup +} = 0–9) + C{sub 2}H{sub 2}, achieving high internal-state selectivity and high kinetic energy resolution for reactant N{sub 2}{sup +} ions. The charge transfer (CT) and hydrogen-atom transfer (HT) channels, which lead to the respective formation of product C{sub 2}H{sub 2}{sup +} and N{sub 2}H{sup +} ions, are observed. The vibrationally selected absolute integral cross sections for the CT [σ {sub CT}(v {sup +})] and HT [[σ {sub HT}(v {sup +})] channels obtained in the center-of-mass collision energy (E {sub cm}) range of 0.03–10.00 eV reveal opposite E {sub cm} dependences. The σ {sub CT}(v {sup +}) is found to increase as E {sub cm} is decreased, and is consistent with the long-range exothermic CT mechanism, whereas the E {sub cm} enhancement observed for the σ {sub HT}(v {sup +}) suggests effective coupling of kinetic energy to internal energy, enhancing the formation of N{sub 2}H{sup +}. The σ {sub HT}(v {sup +}) curve exhibits a step at E {sub cm} = 0.70–1.00 eV, suggesting the involvement of the excited C{sub 2}H{sub 2}{sup +}(A{sup 2}Σ{sub g}{sup +}) state in the HT reaction. Contrary to the strong E {sub cm} dependences for σ {sub CT}(v {sup +}) and σ {sub HT}(v {sup +}), the effect of vibrational excitation of N{sub 2}{sup +} on both the CT and HT channels is marginal. The branching ratios and cross sections for the CT and HT channels determined in the present study are useful for modeling the atmospheric compositions of Saturn's largest moon, Titan. These cross sections and branching ratios are also valuable for benchmarking theoretical calculations on chemical dynamics of the titled reaction.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2018

Deep CFHT Y-band Imaging of VVDS-F22 Field. II. Quasar Selection and Quasar Luminosity Function

We report the results of a faint quasar survey in a one-square-degree field. The aim is to test the Y−K/g−z and J−K/i−Y color selection criteria for quasars at faint magnitudes to obtain a complete sample of quasars based on deep optical and near-infrared color–color selection and to measure the faint end of the quasar luminosity function (QLF) over a wide redshift range. We carried out a quasar survey based on the Y−K/g−z and J−K/i−Y quasar selection criteria, using the deep Y-band data obtained from our CFHT/WIRCam Y-band images in a two-degree field within the F22 field of the VIMOS VLT deep survey, optical co-added data from Sloan Digital Sky Survey Stripe 82 and deep near-infrared data from the UKIDSS Deep Extragalactic Survey in the same field. We discovered 25 new quasars at 0.5 2.5.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

The Target-selection Pipeline for the Dark Energy Spectroscopic Instrument

Abstract In 2021 May, the Dark Energy Spectroscopic Instrument (DESI) began a 5 yr survey of approximately 50 million total extragalactic and Galactic targets. The primary DESI dark-time targets are emission line galaxies, luminous red galaxies, and quasars. In bright time, DESI will focus on two surveys known as the Bright Galaxy Survey and the Milky Way Survey. DESI also observes a selection of “secondary” targets for bespoke science goals. This paper gives an overview of the publicly available pipeline ( desitarget ) used to process targets for DESI observations. Highlights include details of the different DESI survey targeting phases, the targeting ID ( TARGETID ) used to define unique targets, the bitmasks used to indicate a particular type of target, the data model and structure of DESI targeting files, and examples of how to access and use the desitarget code base. This paper will also describe “supporting” DESI target classes, such as standard stars, sky locations, and random catalogs that mimic the angular selection function of DESI targets. The DESI target-selection pipeline is complex and sizable; this paper attempts to summarize the most salient information required to understand and work with DESI targeting data.

47 OTHER INSTRUMENTATION↗

DOE OSTI2026

Highly Efficient Selection of High-redshift Emission-line Galaxies for Future DESI-like Surveys with Deep Multiband Imaging

Emission-line galaxies (ELGs) are an important tracer of baryon acoustic oscillations (BAOs) and large-scale structure at z > 1. In this work, we investigate the feasibility of using deep wide-area multiband imaging (e.g., from the Rubin Observatory) to efficiently select high-redshift ELGs. Using Hyper Suprime-Cam grizy photometry and COSMOS2020 many-band photometric redshifts, we design simple color cuts guided by a probabilistic random forest classifier to select galaxies at z = 1.1–1.6. We then empirically test and refine these color cuts using two samples of galaxies with deep spectroscopy and broad color coverage obtained with the Dark Energy Spectroscopic Instrument (DESI). Compared to DESI ELGs at z = 1.1–1.6, we achieve a higher redshift-measurement success rate (89% versus 69%), a much higher correct redshift-range success rate (84% versus 34%), and a far higher net surface density yield (1372 deg −2 versus 660 deg −2 ). Combining our sample with current DESI ELGs would increase the net ELG number density by a factor of ∼2.5, moving it out of the shot-noise limited regime and reducing the uncertainties on the BAO scale parameter at z = 1.1–1.6 by a factor of ∼2 at the highest redshifts. We also test selections using shallower photometry and obtain qualitatively similar results.

Salcedo Hernandez, Yoquelbin [University of Pittsb↗

DOE OSTI2017

The Lyman Continuum Escape Fraction of Emission Line-selected z ∼ 2.5 Galaxies Is Less Than 15%

Recent work suggests that strong emission line, star-forming galaxies (SFGs) may be significant Lyman continuum leakers. We combine archival Hubble Space Telescope broadband ultraviolet and optical imaging (F275W and F606W, respectively) with emission line catalogs derived from WFC3 IR G141 grism spectroscopy to search for escaping Lyman continuum (LyC) emission from homogeneously selected z ∼ 2.5 SFGs. We detect no escaping Lyman continuum from SFGs selected on [O ii] nebular emission ( N = 208) and, within a narrow redshift range, on [O iii]/[O ii]. We measure 1 σ upper limits to the LyC escape fraction relative to the non-ionizing UV continuum from [O ii] emitters, f {sub esc} ≲ 5.6%, and strong [O iii]/[O ii] > 5 ELGs, f {sub esc} ≲ 14.0%. Our observations are not deep enough to detect f {sub esc} ∼ 10% typical of low-redshift Lyman continuum emitters. However, we find that this population represents a small fraction of the star-forming galaxy population at z ∼ 2. Thus, unless the number of extreme emission line galaxies grows substantially to z ≳ 6, such galaxies may be insufficient for reionization. Deeper survey data in the rest-frame ionizing UV will be necessary to determine whether strong line ratios could be useful for pre-selecting LyC leakers at high redshift.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Preliminary Target Selection for the DESI Bright Galaxy Survey (BGS)

The Dark Energy Spectroscopic Instrument (DESI) will execute a nearly magnitude-limited survey of low redshift galaxies (0.05 ≤ z ≤ 0.4, median z ≈ 0.2). Clustering analyses of this Bright Galaxy Survey (BGS) will yield the most precise measurements to date of baryon acoustic oscillations and redshift-space distortions at low redshift. DESI BGS will comprise two target classes: (i) BRIGHT (r < 19.5 mag), and (ii) FAINT (19.5 < r < 20 mag). Here we present a summary of the star-galaxy separation, and different photometric and geometrical masks, used in BGS to reduce the number of spurious targets. The selection results in a total density of ~800 objects deg -2 for the BRIGHT and ~600 objects deg -2 for the FAINT selections. A full characterization of the BGS selection can be found in Ruiz-Macias et al.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

Selection of high-redshift Lyman-Break Galaxies from broadband and wide photometric surveys

In this paper, we investigate the possibility of selecting high-redshift Lyman-Break Galaxies (LBG) using current and future broadband wide photometric surveys, such as the Ultraviolet Near Infrared Optical Northern Survey (UNIONS) or the Vera C. Rubin Legacy Survey of Space and Time (LSST), using a Random Forest algorithm. This work is conducted in the context of future large-scale structure spectroscopic surveys like DESI-II, the next phase of the Dark Energy Spectroscopic Instrument (DESI), which will start around 2029.We use deep imaging data from the Hyper Suprime Camera (HSC) and the Canada-France-Hawaii Telescope Large Area U-band Deep Survey (CLAUDS) on the COSMOS and XMM-LSS fields. To predict the selection performance of LBGs with image quality similar to UNIONS, we degrade the u,g,r,i and z bands to UNIONS depth.The Random Forest algorithm is trained with the u,g,r,i and z bands to classify LBGs in the 2.5 < z < 3.5 range.We find that fixing a target density budget of 1,100 deg$^{-2}$, the Random Forest approach gives a density of z > 2 targets of 873 deg$^{-2}$, and a density of 493 deg$^{-2}$ of confirmed LBGs after spectroscopic confirmation with DESI. This UNIONS-like selection was tested in a dedicated spectroscopic observation campaign of 1,000 targets with DESI on the COSMOS field, providing a safe spectroscopic sample with a mean redshift of 3. This sample is used to derive forecasts for DESI-II, assuming a sky coverage of 5,000 deg$^{2}$. We predict uncertainties on Alcock-Paczynski parameters α$_{⊥}$ and α$_{∥}$ to be 0.7% and 1% for 2.6 < z < 3.2, resulting in a potential 2% measurement of the dark energy fraction at high redshift. Additionally, we estimate the uncertainty in local non-Gaussianity and predict σ$_{fNL}$ ≈ 7, which would be comparable to the current best precision achieved by Planck. The latter forecast suggests that achieving the precision required to place stringent constraints on inflationary models (σ$_{fNL}$ ≈ 1) using spectroscopic galaxy surveys necessitates the development of a next-generation (Stage V) spectroscopic survey.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2022

IM3 SELECT Urbanization Data

IM3 SELECT Urbanization Data Urban fraction is provided in TIF files projected on the WGS84 datum at coarse (1/8 degree) and downscaled (1km) resolutions across the globe for each of three Shared Socioeconomic Pathway (SSP) scenarios corresponding to SSP2, SSP3, and SSP5; and each of two population scenarios corresponding to the default population scenario and an updated population scenario with more detailed projections for the United States. The population projections are provided as CSV files. Folder structure: default_population population urban_fraction coarse SSP2 SSP3 SSP5 downscaled SSP2 SSP3 SSP5united_states_updated_population population urban_fraction coarse SSP2 SSP3 SSP5 downscaled SSP2 SSP3 SSP5 Urban fraction data was produced using the SELECT model v1.0.0 (Gao, J. & O'Neill, B.C. 2019). Default population data derived from Gao, J. & O'Neill, B.C. 2020. Original model outputs produced using the default population data are available from Gao, J. 2020. Updated United States population data derived from Zoraghein, H. & O'Neill, B.C. 2020. Other SELECT input files available at Gao, J. & O'Neill, B.C. 2022.

McManamay, Ryan↗

NASA NTRS1972

Automatic computer subprogram selection from application program libraries

The program ALTLIB (ALTernate LIBrary) which allows a user access to an alternate subprogram library with a minimum effort is discussed. The ALTLIB program selects subprograms from an alternate library file and merges them with the user's program load file. Only subprograms that are called for (directly or indirectly) by the user's programs and that are available on the alternate library file will be selected. ALTLIB eliminates the need for elaborate control-card manipulations to add subprograms from a subprogram file. ALTLIB returns to the user his binary file and the selected subprograms in correct order for a call to the loader. The user supplies the alternate library file. Subprogram requests which are not satisfied from the alternate library file will be satisfied at load time from the system library.

Drozdowski, J. M.↗

NASA NTRS1971

Solid propellant selection and characterization

The techniques of propellant selection and characterization and the compromises that may be forced on the designer by the change of a propellant parameter are discussed. Rules for the selection of a general propellant type are presented. The characterization of various propellant properties is then approached parameter by parameter. Tailoring pitfalls and compromises are identified whenever possible, and appropriate cross references are used. Related design criteria monographs frequently are cited for a more detailed treatment of the topic under discussion. A list of source references is provided. These references, coupled with established texts in the field, should give the depth of knowledge necessary to the designer to aid in the selection of the most nearly optimum propellant for the design application.

Source record↗

NASA NTRS1972

Engine selection for transport and combat aircraft

The procedures that are used to select engines for transport and combat aircraft are discussed. In general, the problem is to select the engine parameters including engine size in such a way that all constraints are satisfied and airplane performance is maximized. This is done for four different classes of aircraft: (1) a long haul conventional takeoff and landing (CTOL) transport, (2) a short haul vertical takeoff and landing (VTOL) transport, (3) a long range supersonic transport (SST), and (4) a fighter aircraft. For the commercial airplanes the critical constraints have to do with noise while for the fighter, maneuverability requirements define the engine. Generally, the resultant airplane performance (range or payload) is far less than that achievable without these constraints and would suffer more if nonoptimum engines were selected.

Dugan, J. F., Jr.↗

NASA NTRS1972

Program management aid for redundancy selection and operational guidelines

Although this criterion was developed specifically for use on the shuttle program, it has application to many other multi-missions programs (i.e. aircraft or mechanisms). The methodology employed is directly applicable even if the tools (nomographs and equations) are for mission peculiar cases. The redundancy selection criterion was developed to insure that both the design and operational cost impacts (life cycle costs) were considered in the selection of the quantity of operational redundancy. These tools were developed as aids in expediting the decision process and not intended as the automatic decision maker. This approach to redundancy selection is unique in that it enables a pseudo systems analysis to be performed on an equipment basis without waiting for all designs to be hardened.

Hodge, P. W.↗

NASA NTRS1971

Reflectance and transmittance characteristics of several selected green and blue-green unialgae.

Obtained reflectance properties of green and blue-green unialgae are evaluated for determining the feasibility of using selected wavelengths in differentiating between green and blue-green algae. The attempt is made to establish selected wavelengths and ratios that would delineate relative concentrations of the algal suspensions. The results should prove helpful in the selection of spectral bands usable in conjunction with multispectrum scanners for qualitative and quantitative studies of algae in bodies of water.

Gramms, L. C.↗

NASA NTRS1972

Path selection system simulation and evaluation for a Martian roving vehicle

The simulation and evaluation of proposed path selection systems for an autonomous Martian roving vehicle was developed. The package incorporates a number of realistic features, such as the simulation of random effects due to vehicle bounce and sensor-reading uncertainty, to increase the reliability of the results. Qualitative and quantitative evaluation criteria were established. The performance of three different path selection systems was evaluated to determine the effectiveness of the simulation package, and to form some preliminary conclusions regarding the tradeoffs involved in a path selection system design.

Boheim, S. L.↗