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Operation of the Planetary Plasma Interactions Node of the Planetary Data System

Five years ago NASA selected the Planetary Plasma Interactions (PPI) Node at UCLA to help the scientific community locate, access and preserve particles and fields data from planetary missions. We propose to continue to serve for 5 more years. During the first five years we have served the scientific community by providing them with high quality data products. We worked with missions and individual scientists to secure the highest quality data possible and to thoroughly document it. We validated the data, placed it on long lasting media and made sure it was properly archived for future use. So far we have prepared and archived over 10(exp 11) bytes of data from 26 instruments on 4 spacecraft. We have produced 106 CD-ROMs with peer reviewed data. In so doing, we have developed an efficient system to prepare and archive the data and thereby have been able to steadily increase the rate at which the data are produced. Although we produced a substantial archive during the initial five years, we have an even larger amount of work in progress. This includes preparing CD-ROM data sets with all of the Voyager, Pioneer and Ulysses data at Jupiter and Saturn. We will have the Jupiter data ready for the Galileo encounter in December, 1995. We are also completing the Pioneer Venus data restoration. The Galileo Venus archive and radio science data from Magellan will be prepared early in the next period. We are assisting the Small Bodies Node of PDS in the preparation of comet data and will be archiving the asteroid data from Galileo. We will be moving in several new directions as well. We will archive the PPI Node's first Earth based data with data from the International Jupiter Watch and Hubble data taken in support of Ulysses particles and field observations. We will work with the Cassini mission in archive planning efforts. For the inner planets we will begin an archive of Mars data starting with Phobos data and will support the US and Russian Mars missions in the late 1990's. We will restore the Mercury data from Mariner 10 and prepare the lunar data from Clementine in time for the lunar data analysis program in 1995. We will work with the Discovery mission teams to plan their archive and have already started with one, NEAR. Finally we will begin archiving our first heliospheric data from Voyager, Galileo, and Mars observers. We will continue to serve the science community by providing access to the data products. During the past 19 months we have filled nearly 6000 requests for on-line and CD-ROM data. The data delivered directly by the PPI Node has been - 5 x 10(exp 11) bytes. In addition to providing the data, we have provided users with software tools to manage and read the data which are computer, operating system and format independent. We have developed scalable systems so that the same software we use to manage and access the data for the entire PPI Node can be used by individual investigators to manage the data on a single CD-ROM, thereby greatly reducing the software development effort for both the PPI Node and users. We deliver this software with the disks. Recent technical advances have made it possible for us to serve a broader community than before. In the next five year period we plan to extend our outreach to the general public and in particular to increase our support for education. Since planetary plasma data are varied and require expertise in many areas the PPI Node will continue to be distributed. In addition to the primary node at UCLA, the PPI Node has three subnodes with an Outer Planets Subnode at the University of Iowa, an Inner Planets Subnode at UCLA, and a Radio Science Subnode at Stanford University. During the first two years of the renewal period there will be a Radio Astronomy Data Node at GSFC. These organizations will provide scientific expertise on the data, participate in node data selection activities and help with data restoration and mission activities.

Walker, Raymond J.↗

Development and Characterization of a Small Spacecraft Electro-Optic Scanner for Free-Space Laser Communications

Emergent data-intensive missions coupled with dramatic reductions in spacecraft size plus an increasing number of space-based missions necessitates new high performance, compact and low cost communications technology. Free space optical communications offer advantages including orders of magnitude increase for data rate performance, increased security, immunity to jamming and lack of frequency allocation requirements when compared with conventional radio frequency (RF) means. The spatial coherence and low divergence associated with the optical frequencies of laser communications lends themselves to superior performance, but this increased directionality also creates one of the primary technical challenges in establishing a laser communications link by repeatedly and reliably pointing the beam onto the receive aperture. Several solutions have emerged from wide angle (slow) mechanical articulation systems, fine (fast) steering mirrors and rotating prisms, inertial compensation gyros and vibration isolation cancellation systems, but each requires moving components and imparts a measured amount of burden on the host platform. The complexity, cost and size of current mechanically scanned solutions limits their platform applicability, and restricts the feasibility of deploying optical communications payloads on very compact spacecraft employing critical systems. A high speed, wide angle, non-mechanical solution is therefore desirable. The purpose of this work is to share the development, testing, and demonstration of a breadboard prototype electro-optic (EO) scanned laser-communication link (see Figure 1). This demonstration is a step toward realizing ultra-low Size, Weight and Power (SWaP) SmallSat/MicroSat EO non-mechanical laser beam steering modules for high bandwidth ( greater than Gbps) free-space data links operating in the 1550 nm wavelength bands. The elimination of all moving parts will dramatically reduce SWaP and cost, increase component lifetime and reliability, and simplify the system design of laser communication modules. This paper describes the target mission architectures and requirements (few cubic centimeters of volume, 10's of grams of weight with milliwatts of power) and design of the beam steering module. Laboratory metrology is used to determine the component performance including horizontal and vertical resolution (20urad) as a function of control voltage (see Figure 2), transition time (0.1-1ms), pointing repeatability and optic insertion loss. A test bed system demonstration, including a full laser communications link, is conducted. The capabilities of this new EO beam steerer provide an opportunity to dramatically improve space communications through increased utilization of laser technology on smaller platforms than were previously attainable.

Laser Optical Communications↗

rHealth One Demonstration Aboard ISS: A Microfluidic Bioanalyzer Based on Sheath/Hydrodynamic Focusing Flow Cytometry

The Exploration Medical Capability (ExMC) element aims to provide astronauts with the means for their own health monitoring, diagnosis, and treatment during exploration missions. As space flight ventures further from earth, the need for autonomous medical care increases under greater constraints on size, mass, and resources. One pillar for diagnosis that crew would be separated from is laboratory analysis. Even now on ISS, blood samples must be collected and returned to earth for testing. In response, ExMC is assessing how assays for hematology, bone health, radiation exposure etc. could be addressed through commercial-off-the-shelf (COTS) and Small Business Innovation Research (SBIR) funded bioanalyzers that are miniaturizing lab technology. Since missions will reach distances where there are no timely replacements, validation on the International Space Station (ISS) is a necessary part of that assessment. In partnership with NASA Johnson Space Center (JSC) Immunology Lab and the Research Operations and Integration (ROI) element, ExMC conducted a technology demonstration on ISS of the rHEALTH ONE, a flow cytometry based bioanalyzer, to assess future devices based on this design. In flow cytometry, there are predominantly three ways to focus the cells (or particles) into a single file stream: hydrodynamic focusing, microcapillary, and acoustic focusing. The rHEALTH ONE utilizes the commercial standard, sheath-based hydrodynamic focusing. rHEALTH itself represents both a company and a suite of medical tools NASA has funded through SBIR grants towards the development of a promising diagnosis instrument for exploration missions. rHEALTH ONE is the interim version of the technology, functional as a benchtop analyzer and test bed for the next generation of rHEALTH in development. Several modifications were made to the rHEALTH ONE analyzer for operation in microgravity. For function, fluid management was key. A sheath-based analyzer uses sheath fluid to flow the sample, cleaning fluid to prevent biological contamination, and a reservoir to collect the liquid waste. The rHEALTH ONE analyzer uses bottles dependent on gravity to separate the air and liquid pathways and keep the liquids contained. It uses only 1 psig of air pressure to directly push the liquid through the device, requiring little-to-no resistance at inlet and outlet. A microtubing assembly with self-sealing luer connectors was designed – featuring 0.014 mm thick durable medical balloons to hold water inside the supply bottles – to create safe containment and easy access for the crew while maintaining the analyzer’s function. For safety, copper tape was added to the interior of the plastic housing to reduce electromagnetic interference, fluid and electrical connections were secured against vibration and leaks, and gaps were further sealed to ensure containment of the optical block and lasers. Water as the sheath and cleaning fluid and TOX 0 samples were used to reduce the biohazard risk to the crew. In May 2022, European Space Agency astronaut Samantha Cristoforetti demonstrated the rHEALTH ONE aboard ISS for its sample loading, flow cytometry, and data collection capability in microgravity. The JSC Immunology Lab provided flow cytometry expertise, designed the sample test protocol, and manufactured and benchmarked the flight samples on a ‘gold-standard’ flow cytometer. The analyzer was primed with water, purged of air, and four calibration solutions of polystyrene microparticles were tested to characterize its performance. Tightly controlled procedures and excellent execution prevented air bubble interference during air/water separation, fluid transfer, sample mixing and loading. Data showed a slight increase in signal noise on 3 of 5 channels and an anomaly of fluorophores migrating in one sample (confirmed by JSC post-flight). Flight results correctly detected the change in sample, matched the analyzer’s ground performance, and were consistent with the gold-standard’s ground results. Although areas were noted for improvement, these outcomes signified complete mission success.

R. S. Miller↗

Stove Solutions: Improving Health, Safety, and the Environment in Darfur with Fuel-Efficient Cookstoves

Nearly three billion people across the globe cook every day using open, three-stone fires, or rudimentary stoves that burn biomass such as wood, agricultural waste, animal dung, and charcoal. Cooking with these traditional cookstoves is inefficient and grossly polluting, harming health and the environment, and contributing to global warming. In many places worldwide, women must walk for hours to collect firewood, risking their safety and sacrificing energy and time that could be used to earn a living. While often overlooked as a major contributor to the global burden of disease, cooking over open fires indoors is the largest environmental health risk in developing countries, and exposes women (and the young children near them) to amounts of smoke equivalent to burning 1,000 cigarettes inside the home. In Darfur, Sudan, where about 2.7 million people have been displaced from their homes by conflict, the situation is particularly dire. Each day, Darfuri women face the difficult choice between risking sexual assault during treks to collect firewood or selling a portion of their family’s meager food rations for cash to purchase wood. Here, the Berkeley-Darfur Stove, developed by scientists at the Lawrence Berkeley National Laboratory (LBNL) and volunteers from UC Berkeley and Engineers Without Borders, is a metal stove that reduces the need for firewood by more than half, owing to its improved combustion and heat transfer efficiencies. LBNL has partnered with a nonprofit organization, Potential Energy, and a number of aid organizations to disseminate more than 22,000 Berkeley-Darfur Stoves to Darfuri women. Several hundred thousand more are needed.

54 ENVIRONMENTAL SCIENCES↗

Impact histories inferred from exogenic boulders on asteroids Ryugu and Bennu

Rubble-pile asteroids, such as (162173) Ryugu and (101955) Bennu, are formed as a result of catastrophic disruption of a parent body and re-accumulation of the fragments by self-gravity. Therefore, reaccumulated rubble piles could include mixtures of materials from both the parent body and its catastrophic impactor, as they did in the case of 2008 TC3 and the Almahata Sitta meteorites (Jenniskens et al. 2009). Indeed, six unusually bright, basaltic, meter-scale boulders were recently identified on Bennu’s dark surface (DellaGiustina et al. 2021), and their close spectral matches to the Howardite-Eucrite-Diogenite (HED) meteorites and Vesta family members indicate that they originated from asteroid (4) Vesta. In parallel, bright exogenic anhydrous-silicate–rich materials were found on Ryugu (Tatsumi et al. 2021). The bright boulders on Ryugu are consistent with ordinary chondrite meteorites, based on their albedo and weak or even absent absorption band at 2 µm. These exogenous materials on the surfaces of rubble-pile asteroids could be a key to constraining their specific impact conditions and collisional evolution. In this study, we report further study of the visible spectrophotometry and morphology of exogenic boulders on Ryugu and Bennu using two multi-band cameras: the telescopic Optical Navigation Camera (ONC-T) onboard the Hayabusa2 spacecraft, and MapCam onboard the Origins, Spectral Interpretation, Resource Identification, and Security–Regolith Explorer (OSIRIS-REx) spacecraft, respectively. For Ryugu, we first detected objects with peak reflectance brighter by a factor of >1.5 than the surrounding area. Tatsumi et al. (2021) found two spectral groups among the bright boulders: S-type with an absorption near 1 µm and C/X-type with a flat spectrum. That study found 6 S-types and 15 C/X-types, and in this work we additionally find one S-type and ~70 C/X-types. We found that S-type bright boulders follow two parallel trends consistent with space weathering of ordinary chondrites. Fragments from projectiles suggest that Ryugu may not have formed directly from the original parent body, i.e., it is from a second or higher generation of collisional descendants (Sugimoto et al. in revision). For Bennu, we directly surveyed absorption near 1 µm, which is indicative of anhydrous silicates. We propose 77 objects of exogenic origin including 6 boulders previously reported by DellaGiustina et al. (2021). We find that proposed exogenic objects follow two mixing trends with respect to the average spectrum of Bennu (Tatsumi and Popescu et al. submitted). One trend can be explained by mixing with HED as discussed in DellaGiustina et al. (2021), and the other trend can be explained by mixing with another, olivine-rich composition. Near-infrared spectra also support the possibility of multiple compositions among exogenic objects on Bennu. Thus, similar to Ryugu, Bennu could represent a second or higher generation. Using high-resolution images, we found that more than half of the exogenic objects that we identified on Bennu have breccia-like or inclusion-like morphologies. We do not observe a correlation between morphology and spectral shape. Direct comparison of reflectance spectra of exogenic object spectra between Ryugu and Bennu suggests a compositional difference. Furthermore, the number density of exogenic objects > 0.5 m on Bennu is ~40 times that on Ryugu (Tatsumi and Popescu et al. submitted). Bennu exhibits much more contamination from exogenic materials than Ryugu, which likely reflects differences in impact conditions, such as impact velocity and impactor size.

E. Tatsumi↗

Improving Cyber Situational Understanding

Effective cybersecurity operations require the ability to analyze large amounts of information to assess security risks and formulate defensive strategies against adversaries. This has become more complex in recent years as the sprawl and interconnectivity of devices grows through implementation of virtualization, cloud computing, and Internet of Things (IoT). The amount of data and analysis required for effective cybersecurity command and control decisions far exceeds humans’ capacity to perform manually. We characterize the analysis problem as cyber situational understanding. The research presented to improve cyber situational understanding focuses on vulnerability analysis and threat intelligence. Regarding vulnerabilities, entities must analyze and plan work for between thousands and tens of thousands of software vulnerabilities annually. Entities heavily use network firewalls to limit vulnerability exposure. As a result, some of these vulnerabilities permit exposure to adversarial exploitation, whereas others are inaccessible and therefore present negligible risk of exploitation. Distinguishing between high and low risk software vulnerabilities requires a deep understanding of the vulnerability, network firewall protection, and characteristics of the targeted device. This problem is solved by extracting network service features from vulnerability data features using both machine-learning and natural language processing. Then, the network firewall topology is parsed to determine which vulnerabilities are reachable by adversaries. Ultimately, a state-based safety analysis ascertains which vulnerabilities are unsafe. A related vulnerability analysis problem occurs in cybersecurity operations when associating an entity’s hardware and software assets to public vulnerability databases. Assets often reveal hardware and software through installation artifacts and network service identification, and entities store these artifacts in inventory databases. However, software and hardware vendors apply a standard Common Platform Enumeration (CPE) naming convention when publicly reporting vulnerabilities. Associating these two datasets often requires many hours to days of manual inspection. The proposed solution automates the mapping approach of human analysts using fuzzy matching techniques, natural language processing, and, ultimately, machine learning to present a small set of recommendations for mapping the two datasets. The result significantly reduces human analysis time and reduces the occurrence of false positives in vulnerability notifications. Finally, cyber threat intelligence (CTI) requires associating cyber observable artifacts, such as IP addresses, URIs, and file hashes, with cyber threat tactics, techniques, and procedures. Unfortunately, most CTI data is compartmentalized across multiple organizations and cannot be shared due to the legal and reputational risk with cyber threat being associated with the entity. The approach to solving this problem inovlves using a distributed ledger with anonymous token spending and authentication. This allows a consortium of semi-trusted entities to share the workload of curating CTI for a threat sharing community’s cooperative benefit.

Huff, Philip↗

Introduction to Special Issue on the Early History of Nuclear Fusion

This introductory paper to the special issue of Fusion Science and Technology commemorates early research on fusion conducted at Los Alamos (the singular entity denoted Los Alamos Laboratory/Los Alamos Scientific Laboratory/Los Alamos National Laboratory at different times is designated “Los Alamos” in this paper) in support of the eventual H-bomb program. We survey the historical origins of the thermonuclear program, what was known of fusion reactions at the outbreak of the war, and the remarkable breakthroughs involving particularly the prospect of deuterium-tritium (DT) reactions conducted during the war, and we summarize the papers in this volume. Much of the nuclear fusion technical history presented herein has not been previously reported. Papers describe aspects of fusion science during these days, on shock hydrodynamics and on electron-radiation coupling, and on nuclear physics including the discoveries of resonances in both the DT cross section and in the lithium tritium-breeding cross section. Three papers follow our colleague Mark Paris’s finding Arthur Ruhlig’s 1938 paper on the first observation of DT fusion: one on how it influenced subsequent Manhattan Project research, another on a modern calculation of that historic experiment, and a third that has repeated the experiment using modern experimental capabilities. Other papers discuss how the first H-bomb test, Ivy Mike, led to the discovery of the new elements einsteinium and fermium and how the DT fusion processes played a key role in our universe’s development after the Big Bang. We also present a paper that analyzes the pioneering Cambridge University 1934 experiment by Marcus Oliphant, Paul Harteck, and Ernest Rutherford where deuterium-deuterium fusion was first observed and that describes how Ernest Lawrence missed identifying fusion in 1933. Finally, we present a summary of early concepts for controlled fusion energy that grew out of wartime discussions at Los Alamos. The papers show how J. Robert Oppenheimer played a leading technical role in the early developments of the H-bomb, before his later opposition—our first paper in this issue addresses the U.S. Department of Energy’s 2022 vacation of the earlier 1954 decision to revoke his security clearance.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗

Phyllosilicate Decomposition on Bennu Due to Prolonged Surface Exposure

The Origins, Spectral Interpretation, Resource Identification, and Security–Regolith Explorer (OSIRIS-REx) mission to carbonaceous asteroid (101955) Bennu performed detailed mapping with a suite of instruments to characterize the composition and geology of its surface. Here we use data from the OSIRIS-REx Thermal Emission Spectrometer (OTES) instrument to investigate the relationship of OTES-derived spectral indices to other derived data products from OTES, the OSIRIS-REx Camera Suite (OCAMS), and the OSIRIS-REx Visible and InfraRed Spectrometer (OVIRS) at global and local scales. We quantitatively confirm that high values of the OTES silicate stretching slope (from ∼10 to ∼12 μm) in midday spectra that are indicative of thin and/or patchy dust cover are strongly associated with low thermal inertia (high porosity), low albedo boulders on Bennu. These high porosity boulders have brecciated textures with embedded clasts that likely originated on Bennu's parent body or during its disruption. The high porosity of these boulders is a key factor in the local production of the dust or its entrapment, as some large, brecciated boulders with a lower porosity have little evidence of dust. A second OTES spectral parameter, the silicate bending band depth near 22.7 μm applied to early evening spectra, is not correlated to thermal inertia, but is weakly to strongly correlated to albedo, OVIRS-derived 1.05 μm and 2.74 μm band depths, OVIRS-derived hydrogen abundance, and modeled nanophase troilite abundance. In several regions on Bennu there is a strong spatial relationship between these parameters, whereby areas with shallower silicate bending bands also have shallower 1.05 μm and 2.74 μm bands and lower albedo with higher nanophase troilite abundances. These correlations, combined with analysis of the silicate bending band in laboratory experiments of space weathered and mildly heated carbonaceous chondrites, suggests that decreased silicate bending band depths signify decomposition of phyllosilicates, likely Fe-bearing, due to space weathering or mild heating (<600 °C) via solar radiation during Bennu's time in near-Earth space. There is a strong association of larger silicate bending band depths in areas dominated by small rocks and unresolved material and in areas with small (≤ 25 m) craters identified as the spectrally reddest on Bennu, suggesting that this material has been more recently exposed due to impact and/or mass wasting processes. The shallowest silicate bending depths are associated with larger rocks and boulders that appear to have the longest surface exposure history, although there is band depth variation among them suggesting either initial composition variation that resulted in different responses to space weathering or heating, or varied exposure history of individual boulders themselves. We predict that any grains returned from Bennu with a significant surface exposure history will be characterized by shallower 22.7 μm, 1.05 μm and 2.7 μm band depths and increased sulfide (troilite) abundance, as well as textural and chemical evidence for phyllosilicate dehydration.

Asteroids, surfaces↗

Fully Distributed Acoustic and Magnetic Field Monitoring Via a Single Fiber Line for Optimized Production of Unconventional Resource Plays

This is the final technical report for the Virginia Tech Center for Photonics Technology (VT-CPT) research project entitled “Fully Distributed Acoustic and Magnetic Field Monitoring Via a Single Fiber Line for Optimized Production of Unconventional Resource Plays”. In the the four-year effort, VT-CPT collaborated with the Departments of Mathmatics at VT and Sentek Instrument, LLC (Sentek) to develop a fiber-optic sensing system capable of real-time simultaneous distributed measurement of multiple subsurface, drilling, and production parameters. The ultra-sensitive fiber optic distributed acoustic sensing technology, picoDAS, developed by Sentek was integrated with a novel multi-material optical sensing fiber fabricated by CPT-VT to obtain distributed acoustic and magnetic field measurements with ultrahigh sensitivity and high spatial resolution. The sensing technology successfully developed and demonstrated under this research program is truly unique has application beyond subsurface imaging to include carbon storage and electrical grid monitoring, as well as healthcare and nuclear fusion. The project, sponsored by the Advanced Technology Program, began in 2019 and had the original goal of developing the next generation of harsh environment sensing systems. Exhaustive theoretical modeling was performed to optimize the multi-material optical fiber design. VT developed the processing techniques employed to successfully fabricate single mode fibers with metal cladding wires. Sensing fibers with nickel and Metglas cladding wires were fully characterized, inscribed with sensors, and fully integrated with the picoDAS system. Laboratory scale testing was performed to demonstrate performance upon exposure to lateral and transverse magnetic fields. Preliminary field trials were performed for prototype magnetic and acoustic sensing systems upon near surface deployment at VT. The distributed acoustic and magnetic field sensing system was advanced from a (Technology Readiness Level) TRL=2 to a TRL=5 via laboratory scale system validation in relevant environments. The truly one-of-its kind distributed magnetic and acoustic sensing system is expected to find immediate applications that require subsurface monitoring, to include carbon storage site monitoring, and has the potential to be a distributive technology in healthcare and electric grid markets. The technologies developed by Virginia Tech’s Center for Photonics Technology will support the mission of the National Energy Technology Laboratory (NETL) to drive innovation and deliver solutions for an environmentally sustainable and prosperous energy future by ensuring affordable, abundant, and reliable energy that drives a robust economy and national security. Technical accomplishments during the program are summarized briefly here and described in detail in the remainder of the report.

02 PETROLEUM↗

Generative large language models for predictive maintenance planning

Maintenance planning and the generation of necessary components for tasks can prove time-consuming and complex. Automating the creation of recurring or similar tasks by leveraging previous planning packages and data, while uncovering insights to automate planning package generation, presents an opportunity to conserve valuable time and resources. This work aims to harness the textual and probabilistic capabilities of large language models (LLMs) to automate the generation of planning packages. Utilizing diverse data sources ranging from raw data to handwritten text, both singular and collaborative LLMs are trained and tested. Results demonstrate their capability to generate essential planning package components, effectively replicating the statistical patterns in the data. This demonstrates the use of these tools inside a digital asset for automated planning. This work outlines a methodology for constructing datasets, a training suite, and evaluation methods for LLM-based textual and conversational planning tools utilized in an asset digital twin. Results indicate that the fine-tuned models generate estimated planning information within the statistical ranges observed in real maintenance data. The models achieve high accuracy (>90%) in document question-answering and instruction generation tasks. Furthermore, the conversational retrieval-augmented generation (RAG) assistant system achieves 100% document retrieval accuracy, while conversational information capture exceeds 98% across the majority of work-package assistant modules.

97 MATHEMATICS AND COMPUTING↗

Sensitive Resources Assessment and Forest Analysis for the Proposed Versatile Test Reactor, Oak Ridge, Tennessee

The US Department of Energy’s (DOE’s) Oak Ridge National Laboratory (ORNL) is a leading institution in advanced materials, supercomputing, neutrons, and nuclear science. As a research laboratory managed by UT-Battelle, LLC for DOE, ORNL has national priorities in energy, security, and scientific discovery that necessitate facility improvements and expansions. DOE is also committed to environmental stewardship. The laboratory is located on the ~32,000-acre (~13,000-ha) Oak Ridge Reservation (ORR), much of which is categorized as a National Environmental Research Park (NERP) and a state Wildlife Management Area. DOE works with the Tennessee Wildlife Resources Agency (TWRA), Tennessee Department of Environment and Conservation (TDEC), US Fish and Wildlife Service (USFWS), US Department of Agriculture, and other agencies to serve as an effective steward of the ORR. Accordingly, project managers must conform to environmental regulations, agreements, and policies at the federal, state, and institutional levels. Per 40 CFR (Code of Federal Regulations) 1508.14, potential effects on research and science education also represent potential effects of federal actions on the NERP, and impacts on, e.g., deer harvest, must be considered on the Oak Ridge Wildlife Management Area when other aspects of the human environment are affected. The United States currently has no fast neutron testing capability to support advanced nuclear research and development. The proposed Versatile Test Reactor (VTR) will take advantage of current investments by the US government and private industry in nuclear reactors to expedite the design and construction process, using proven technology to create a world-class scientific infrastructure. The VTR will take advantage of fast neutrons provided by this proven technology, along with a capability to rapidly insert, conduct, and remove state-of-the-art experiments. An advantage of the VTR is that it can support future innovations in experimental capabilities without modifying the facility. The VTR will support progress in a variety of science and technology areas, including testing and qualification of advanced reactor fuels; testing and qualification of innovative structural materials; testing of innovative components and instruments; validation of advanced modeling and simulation tools; and versatility for future technical missions. Through proven technology, the VTR can take advantage of existing reactor designs and operating experience to reduce the risk, cost, and time for design and construction. The top available resources of DOE laboratories, industry, and universities will be used to expedite reactor design and construction toward developing the scientific infrastructure that affords a strong testing capability that can be sustained over many years. This report summarizes current knowledge of natural and cultural resources primarily within the VTR construction area. At the time of this report, the proposed VTR site design includes a construction area of ~150.4 acres (~69.9 ha), which contains an ~51.3-acre (~20.8-ha) operations area, located within forested natural areas of the ORR. The primary goal of the work presented here was to evaluate potential effects on sensitive resources that might result from development and construction activities associated with VTR. In addition to on-the-ground surveys during spring and summer 2020 by the ORNL Natural Resources Management Program and Aquatic Ecology Group staff, this report makes use of historical (pre-1995) and contemporary (1995 to present) data from additional confirmed sources (e.g., TDEC). Likewise, forest conditions were compiled from a 2011 forest inventory and supplemented with limited ground observations in 2020. The individuals who obtained and compiled the data presented here are familiar with and routinely assess sensitive resources on the ORR. Anyone who references this report must consider that the timing of surveys did not permit a complete delineation of the resources that will be affected. If the VTR project proceeds, additional surveys will be required to account for the seasonal patterns of various threatened and endangered species. Data deficiencies and potential resources that likely went undetected are indicated where possible. Accordingly, this report should facilitate more environmentally sound decisions during planning and 2 development of the VTR site, provide a foundation for further assessment of sensitive and cultural resources, and help project managers better address regulatory guidance and DOE policies on sustainable development in compliance with, for example, the US Endangered Species Act (ESA), Migratory Bird Treaty Act (MBTA), Tennessee Rare Plant Protection and Conservation Act of 1985, Tennessee Nongame and Endangered or Threatened Wildlife Species Conservation Act of 1974, several federal and state regulations regarding aquatic resource protection, and site-specific policies as outlined in various ORR management plans developed by ORNL and TWRA for DOE.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Godiva IV Simulated Radiation Field Characterization and Variance Reduction

Godiva IV is a system comprised of highly enriched uranium alloyed with molybdenum in the form of fuel plate rings. The reactor, along with its predecessors, was designed with the unique ability to satisfy interests in the super-prompt-critical reactor operation space. Originally, the reactor was part of the Los Alamos Critical Experiments Facility (LACEF) at Technical Area-18 (TA-18). The radiation field around Godiva at this facility was well characterized and understood. As a fast neutron system, the neutron spectrum in and around Godiva was close to a Watt Fission spectrum. The Kiva where Godiva IV was located at LACEF was made of thin, sheet metal walls which did not contribute significantly to the neutron spectrum. Following the transition of LACEF to the National Critical Experiments and Research Center (NCERC) in Nevada, Godiva-IV was moved from TA-18 to the Device Assembly Facility (DAF) at the Nevada National Security Site (NNSS). Part of this move brought renewed interest in radiation field characterization. The new facility introduced significant changes to the environment surrounding Godiva, and preliminary foil irradiation results suggested that the room contribution to the neutron spectrum was significant. Unlike at TA-18, a large thermal neutron signature was added to the fast spectrum from Godiva due to significant room return. A primary goal due to the additional complexity that the room return adds to the Godiva IV radiation emission spectrum was the development of an efficient Monte Carlo N-Particle (MCNP) calculation capable of characterizing the neutron spectrum anywhere in the room around Godiva. A campaign of activation foil irradiations and analysis were completed to support the validation of the MCNP model. The modeling of these foils in MCNP can be easily done with a standard volumetric neutron flux tally. However, given the multitude of locations and reaction rates to be modeled, further steps must be taken to increase the efficiency of these calculations in MCNP. During this study, a benchmark model currently under development for Godiva IV was used. A qualitative assessment of the thermal neutron contributors was performed using spatial neutron distribution plots. Additional detail was added to the model based on the qualitative results showing the thermal spectrum’s large sensitivity to hydrogenous material. Neutron energy spectra was evaluated at discrete locations in the room around Godiva to quantify the relative contribution of various components. It was discovered that the concrete walls are the largest contributor to the thermal signature, with minor contributions from plastic components surrounding Godiva. Following these results, two different variance reduction techniques were implemented to improve the problem efficiency in these calculations. In the first approach, an F5 point detector tally was implemented in the standard Godiva IV criticality problem. The second approach involved a weight-window generator implementation with an F5 point detector tally in a fixed source problem. The weight window implementation reduced the runtime from 42739.55 minutes to 1803.34 minutes (computer time), compared to the F5 KCODE implementation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Tooling Techniques Enhance Medical Imaging

They can release as much energy as tens of billions of hydrogen bombs exploding at the same time. They send protons and electrons rocketing at near the speed of light. They heat gas in the Sun s atmosphere to tens of millions of degrees Celsius. They send a blast of gas and particles toward Earth, posing a danger to spacecraft and astronauts outside the planet s magnetosphere, in rare cases even knocking out radio communications and power grids on the ground. They are so-called solar eruptive events, made up of solar flares and the often associated coronal mass ejections. Because of the scientific mystery of how these solar eruptions are produced on the Sun with such scale and force, and also the major role they play in space weather that can impact life on Earth, NASA researchers have innovated new methods of gathering information about these violent events. One NASA mission, the Reuven Ramaty High Energy Solar Spectroscopic Imager (RHESSI) has significantly advanced understanding of solar flares since its launch in 2002. RHESSI scientists use the spacecraft s imaging spectrometer to piece together pictures of solar flares from the high-energy X-ray and gamma-ray radiation they emit. While there is still much to be learned, data gathered by RHESSI has revealed how magnetic fields in the vast expanse of the solar atmosphere may be the force that drives the immense explosions. The instrument has imaged around 50,000 flares to date, providing information that may explain not only the workings of solar flares but also of much more massive energy releases from distant objects like black holes and quasars. We have been able to make images from X-rays with much finer resolution and greater sensitivity than have ever been made before, says Brian Dennis, RHESSI Mission Scientist and astrophysicist in the Solar Physics Laboratory at Goddard Space Flight Center. The key to RHESSI s unprecedented capabilities lie in a set of essential components a NASA partner created for the mission. The manufacturing techniques developed to create the components have yielded innovations advancing medical imaging, transportation security, and even energy efficiency.

Source record↗

Airborne hyperspectral imaging of nitrogen deficiency on crop traits and yield of maize by machine learning and radiative transfer modeling

Nitrogen is an essential nutrient that directly affects plant photosynthesis, crop yield, and biomass production for bioenergy crops, but excessive application of nitrogen fertilizers can cause environmental degradation. To achieve sustainable nitrogen fertilizer management for precision agriculture, there is an urgent need for nondestructive and high spatial resolution monitoring of crop nitrogen and its allocation to photosynthetic proteins as that changes over time. Here, we used visible to shortwave infrared (400–2400 nm) airborne hyperspectral imaging with high spatial (0.5 m) and spectral (3–5 nm) resolutions to accurately estimate critical crop traits, i.e., nitrogen, chlorophyll, and photosynthetic capacity (CO 2 -saturated photosynthesis rate, V max,27 ), at leaf and canopy scales, and to assess nitrogen deficiency on crop yield. We conducted three airborne campaigns over a maize (Zea mays L.) field during the growing season of 2019. Physically based soil-canopy Radiative Transfer Modeling (RTM) and data-driven approaches i.e. Partial-Least Squares Regression (PLSR) were used to retrieve crop traits from hyperspectral reflectance, with ground truth of leaf nitrogen, chlorophyll, V max,27 , Leaf Area Index (LAI), and harvested grain yield. To improve computational efficiency of RTMs, Random Forest (RF) was used to mimic RTM simulations to generate machine learning surrogate models RTM-RF. The results show that prior knowledge of soil background and leaf angle distribution can significantly reduce the ill-posed RTM retrieval. RTM-RF achieved a high accuracy to predict leaf chlorophyll content (R 2 = 0.73) and LAI (R 2 = 0.75). Meanwhile, PLSR exhibited better accuracy to predict leaf chlorophyll content (R 2 = 0.79), nitrogen concentration (R 2 = 0.83), nitrogen content (R 2 = 0.77), and V max,27 (R 2 = 0.69) but required measured traits for model training. We also found that canopy structure signals can enhance the use of spectral data to predict nitrogen related photosynthetic traits, as combining RTM-RF LAI and PLSR leaf traits well predicted canopy-level traits (leaf traits × LAI) including canopy chlorophyll (R 2 = 0.80), nitrogen (R 2 = 0.85) and V max,27 (R 2 = 0.82). Compared to leaf traits, we further found that canopy-level photosynthetic traits, particularly canopy V max,27 , have higher correlation with maize grain yield. This study highlights the potential for synergistic use of process-based and data-driven approaches of hyperspectral imaging to quantify crop traits that facilitate precision agricultural management to secure food and bioenergy production.

54 ENVIRONMENTAL SCIENCES↗

Total absorption spectroscopy of two isomers in 70 Cu influencing nucleosynthesis signatures

Isomers have long been known to be important for astrophysical nucleosynthesis processes, yet they are often neglected in network calculations due to computational limitations or lack of data. "Astromers" are astrophysically metastable nuclear states that can greatly impact nucleosynthesis pathways. In this work we show that astromers further impact the time-dependent electromagnetic signal during heavy element nucleosynthesis. In an experiment performed at the National Superconducting Cyclotron Laboratory, three 𝛽-decaying states of 70 Cu (6 − ground state, and two isomeric states: 3 − and 1 + ) were produced. 𝛽-feeding values were extracted from experimental spectra and compared to shell-model and QRPA+PVC calculations. Here, average 𝛾-ray energies from the 𝛽-decay events were incorporated into simulations of heavy element nucleosynthesis and were found to exhibit different energy release profiles over time, which may impact, in aggregate, time-dependent observable signals.

59 ≤ A ≤ 89↗

Nevada National Security Site 2019 Waste Management Monitoring Report Area 3 and Area 5 Radioactive Waste Management Sites

Environmental monitoring data are collected at and around the Area 3 and Area 5 Radioactive Waste Management Sites (RWMSs) within the Nevada National Security Site (NNSS). This report summarizes the 2019 environmental data to provide an overall evaluation of RWMS performance and to support environmental compliance and performance assessment (PA) activities. Some of these data (e.g., radiation exposure, air, and groundwater) are presented in other reports (Mission Support and Test Services, LLC 2019, 2020a, 2020b). Direct radiation monitoring data indicate exposure levels at the Area 3 and Area 5 RWMSs are within the range of background levels measured at the NNSS. Slightly elevated exposure levels outside the Area 3 RWMS are attributed to nearby historical aboveground nuclear weapons tests. Air monitoring data at the Area 3 and Area 5 RWMSs show that tritium concentrations in water vapor and americium and plutonium concentrations in air particles are below Derived Concentration Standards for these radionuclides. Groundwater monitoring data indicate the groundwater in the uppermost aquifer beneath the Area 5 RWMS is not impacted by RWMS operations. Results of groundwater analysis from wells around the Area 5 RWMS are below established investigation levels. Leachate samples collected from the leachate collection systems at the Area 5 mixed low-level waste disposal unit are below established contaminant regulatory limits. During 2019, precipitation at the Area 3 RWMS was 77 percent above average, and precipitation at the Area 5 RWMS was 69 percent above average. Water balance measurements indicate that evapotranspiration from the vegetated weighing lysimeter at the Area 5 RWMS dries the soil and prevents downward percolation of precipitation more effectively than evaporation as measured from the bare-soil weighing lysimeter. Vadose zone monitoring in the Area 3 and Area 5 RWMS soil covers shows no evidence of precipitation percolating through the covers to the waste. Moisture from precipitation did not percolate below 120 centimeters (3.9 feet [ft]) in the vegetated final cover on the U-3ax/bl disposal unit at the Area 3 RWMS during 2019. There was no drainage through 2.4 meters (8 ft) of soil as indicated from the Area 3 drainage lysimeters that received only natural precipitation. At the Area 3 RWMS, which received three times the natural precipitation, 57 percent of the applied precipitation and irrigation drained from the bare-soil drainage lysimeter. All 2019 monitoring data indicate that the Area 3 and Area 5 RWMSs are performing within expectations of the model and parameter assumptions for the facilities’ PAs.

2019↗

Counterrotating-Shoulder Mechanism for Friction Stir Welding

A counterrotating-shoulder mechanism has been proposed as an alternative to the mechanism and fixtures used in conventional friction stir welding. The mechanism would internally react most or all of the forces and torques exerted on the workpiece, making it unnecessary to react the forces and torques through massive external fixtures. In conventional friction stir welding, a rotating pin tool is inserted into, and moved along, a weld seam. As the pin tool moves, it stirs together material from the opposite sides of the seam to form the weld. A large axial plunge force must be exerted upon the workpiece through and by the pin tool and a shoulder attached above the pin tool in order to maintain the pressure necessary for the process. The workpiece is secured on top of an anvil, which supports the workpiece against the axial plunge force and against the torque exerted by the pin tool and shoulder. The anvil and associated fixtures must be made heavy (and, therefore, are expensive) to keep the workpiece stationary. In addition, workpiece geometries must be limited to those that can be accommodated by the fixtures. The predecessor of the proposed counterrotating-shoulder mechanism is a second-generation, self-reacting tool, resembling a bobbin, that makes it possible to dispense with the heavy anvil. This tool consists essentially of a rotating pin tool with opposing shoulders. Although the opposing shoulders maintain the necessary pressure without need to externally apply or react a large plunge force, the torque exerted on the workpiece remains unreacted in the absence of a substantial external fixture. Depending on the RPM and the thickness of the workpiece, the torque can be large. The proposed mechanism (see figure) would include a spindle attached to a pin tool with a lower shoulder. The spindle would be coupled via splines to the upper one of three bevel gears in a differential drive. The middle bevel gear would be the power-input gear and would be coupled to the upper and lower bevel gears. The lower bevel gear would be attached to the upper shoulder and would slide and rotate freely over the spindle. The spindle would be fastened by its threaded upper end to an external submechanism that would exert axial tension on the spindle to load the workpiece in compression between the shoulders. By reducing or eliminating (relative to the use of a self reacting tool) the torque that must be reacted externally, the use of the proposed tool would reduce the tendency toward distortion or slippage of the workpiece. To begin a weld, the spindle would be inserted through a hole in the workpiece or run-on tab at the beginning of the seam and fastened to the loading submechanism. Rotation and axial loading would be increased gradually from zero and, after a time to be determined by trial and error, translation along the weld seam would be increased gradually from zero to a steady weld speed. The weld would be ended by running the mechanism off the workpiece or, if the lower shoulder were detachable, by detaching the lower shoulder from the spindle and pulling the pin tool out.

Nunes, Arthur C., Jr.↗

The TRANSCEND University Consortium: Theme 4: Nuclear Materials - 20431

The safe and secure management of Pu is a matter of international concern, with ∼250 t of separated Pu currently stockpiled worldwide. The UK's civil inventory of nuclear materials contains significant stocks of separated Pu from the reprocessing of Magnox and AGR spent fuels. The preferred option for the 138.5 tonnes of Pu is re-use as mixed oxide (MOx) fuel, although 5% is not suitable for re-use and is recommended for direct disposal. However, it will take more than 15 years to implement re-use, requiring that the Pu be kept in interim storage in its current state for that period, i.e. as PuO{sub 2} powder within inert steel storage cans at Sellafield. The focus of the work presented here is thus plutonium storage and the direct disposal of plutonium. The Research and Development needs of both are now pressing: in the case of storage due to it being the current default; in the case of immobilization and disposal because of a comparative lack of Research and Development on Pu conditioning and packaging due to policy uncertainty as to whether it would be disposed of in a Geologic Disposal Facility (GDF). Addressing these needs is complicated by Pu's high radioactivity, decay heat and radiotoxicity, criticality, nuclear safeguard requirements and, for some UK Pu contaminated materials targeted for disposal, poor inventory. Thus, there is also a critical requirement for underpinning research on Pu bearing materials in these two contexts. In response to these needs, the TRANSCEND Consortium (Transformative Science and Engineering for Nuclear Decommissioning, a multi-disciplinary collaboration of 11 universities and 8 key industry partners from across the UK's civil nuclear sector) is seeking to provide technical underpinning to ongoing option development for the UK's civil Pu stockpile. Whilst understanding the behaviour of plutonium during its re-use as MOx is beyond the scope of the TRANSCEND Consortium work plan, the main objectives of the work are: (1) For interim storage: to understand how the surface structure and properties of pristine and radiation damaged PuO{sub 2} change with time in the absence and presence of water; and (2) For immobilization and disposal: to understand the mechanisms of incorporation of Pu into ceramic and glass-ceramic waste-forms, as well as the effect on these of self-induced radiation damage. Each objective is being addressed through separate work packages, the details of which are discussed in this paper. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗