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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,585 records · Page 88
All sourcesNASA NTRSDOE OSTI
DOE OSTI2019

Unraveling the Interfacial Structure–Performance Correlation of Flexible Metal–Organic Framework Membranes on Polymeric Substrates

Pure metal–organic framework (MOF) layers deposited on porous supports are important candidates for molecular sieving membranes, but their performance usually deviates from theoretical estimations. Here, we combine stepwise scanning electron microscopy imaging, time-resolved synchrotron X-ray scattering, terahertz infrared spectroscopy, and density functional theory calculation to investigate the ZIF-8 membrane formation on two types (polydopamine and TiO2) of functionalized porous supports. Though molecular sieving of ZIF-8 membranes for smaller gases (He, H 2 , and CO 2 ) can be achieved with both types of functionalized supports, we unravel that the strong interaction between MOF and polydopamine can disrupt the formation of “perfect” MOF crystals at the interface, leading to a “contracted” MOF structure with partially uncoordinated imidazolate ligands. This further affects the low-frequency dynamical parameters of the framework and inhibits the effective seeded growth. Eventually, it leads to an unexpected loss of selectivity for the bulkier gases (N 2 and CH 4 ) for ZIF-8 on polydopamine-functionalized supports. This work links the dynamical aspects of MOFs with their gas transport behavior and highlights the importance of regulating the interfacial weak forces to preserve the ideal molecular sieving efficiency of MOF membranes, which a

36 MATERIALS SCIENCE↗
DOE OSTI2025

Breakdown of the Static Dielectric Screening Approximation of Coulomb Interactions in Atomically Thin Semiconductors

Coulomb interactions in atomically thin materials are remarkably sensitive to variations in the dielectric screening of the environment, which can be used to control exotic quantum many-body phases and engineer exciton potential landscapes. For decades, static or frequency-independent approximations of the dielectric response, where increased dielectric screening is predicted to cause an energy redshift of the exciton resonance, have been sufficient. These approximations were first applied to quantum wells and were more recently extended with initial success to layered transition metal dichalcogenides (TMDs). Here, we use charge-tunable exciton resonances to investigate screening effects in TMD monolayers embedded in materials with low-frequency dielectric constants ranging from 4 to more than 1000, a range of 2 orders of magnitude larger than in previous studies. In contrast to the redshift predicted by static models, we observe a blueshift of the exciton resonance exceeding 30 meV in higher dielectric constant environments. We explain our observations by introducing a dynamical screening model based on a solution to the Bethe-Salpeter equation (BSE). When dynamical effects are strong, we find that the exciton binding energy remains mostly controlled by the low-frequency dielectric response, while the exciton self-energy is dominated by the high-frequency one. Our results supplant the understanding of screening in layered materials and their heterostructures, introduce a knob to tune selected many-body effects, and reshape the framework for detecting and controlling correlated quantum many-body states and designing optoelectronic and quantum devices.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

Acoustic scattering by elastic cylinders of elliptical cross-section and splitting up of resonances

The scattering of a plane acoustic wave by an infinite elastic cylinder of elliptical cross section is studied from a modal formalism by emphasizing the role of the symmetries. More precisely, as the symmetry is broken in the transition from the infinite circular cylinder to the elliptical one, the splitting up of resonances is observed both theoretically and experimentally. This phenomenon can be interpreted using group theory. The main difficulty stands in the application of this theory within the framework of the vectorial formalism in elastodynamics. This method significantly simplifies the numerical treatment of the problem, provides a full classification of the resonances, and gives a physical interpretation of the splitting up in terms of symmetry breaking. An experimental part based on ultrasonic spectroscopy complements the theoretical study. A series of tank experiments is carried out in the case of aluminium elliptical cylinders immersed in water, in the frequency range 0 ≤ kr ≤ 50, where kr is the reduced wave number in the fluid. The symmetry is broken by selecting various cylinders of increasing eccentricity. More precisely, the greater the eccentricity, the higher the splitting up of resonances is accentuated. The experimental results provide a very good agreement with the theoretical ones, the splitting up is observed on experimental form functions, and the split resonant modes are identified on angular diagrams.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Electromagnetic resonant modes of dielectric sphere bilayers

Sphere bilayers have been proposed as promising structures for electromagnetic management in photonic crystal devices. These arrangements are made of two intertwined subsets of spheres of different size and refractive index, one subset filling the interstitial sites of the other. We present a systematic study of the electromagnetic resonant modes of the bilayers, in comparison with those of the constituent subsets of spheres. Three samples were built with glass and Teflon spheres and their transmission spectra measured in the microwave range (10–25 GHz). Simulations with finite integration time-domain method are in good agreement with experiments. Results show that the bilayer presents the same resonances as one of the subsets but modified by the presence of the other in its resonant frequencies and in the electric field distributions. As this distortion is not very large, the number of resonances in a selected spectral region is determined by the dominant subset. The degree of freedom that offers the bilayer could be useful to fine tune the resonances of the structure for different applications. A map of modes useful to guide this design is also presented. Scale invariance of Maxwell equations allows the translation of these results in the microwave range to the visible region; hence, some possible applications are discussed in this framework.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Piezo-optomechanical cantilever modulators for VLSI visible photonics

Visible-wavelength very large-scale integration photonic circuits have a potential to play important roles in quantum information and sensing technologies. The realization of scalable, high-speed, and low-loss photonic mesh circuits depends on reliable and well-engineered visible photonic components. Here, we report a low-voltage optical phase shifter based on piezo-actuated mechanical cantilevers, fabricated on a CMOS compatible, 200 mm wafer-based visible photonics platform. We show linear phase and amplitude modulation with 6 V π cm in differential operation, −1.5 to −2 dB insertion loss, and up to 40 dB contrast in the 700–780 nm range. By adjusting selected cantilever parameters, we demonstrate a low-displacement and a high-displacement device, both exhibiting a nearly flat frequency response from DC to a peak mechanical resonance at 23 and 6.8 MHz respectively, which, through resonant enhancement of Q ∼ 40, further decreases the operating voltage down to 0.15 V π cm.

Dong, Mark↗
DOE OSTI2014

Optical spectroscopic observations of γ-ray blazar candidates. I. Preliminary results

A significant fraction (∼30%) of the γ-ray sources listed in the second Fermi/LAT (2FGL) catalog is still of unknown origin, being not yet associated with counterparts at lower energies. Using the available information at lower energies and optical spectroscopy on the selected counterparts of these γ-ray objects, we can pinpoint their exact nature. Here, we present a pilot project pointing to assess the effectiveness of the several classification methods developed to select γ-ray blazar candidates. To this end, we report optical spectroscopic observations of a sample of five γ-ray blazar candidates selected on the basis of their infrared Wide-field Infrared Survey Explorer (WISE) colors or of their low-frequency radio properties. Blazars come in two main classes, BL Lac objects and FSRQs, showing similar optical spectra except for the stronger emission lines of the latter. For three of our sources, the almost featureless optical spectra obtained confirm their BL Lac nature, while for the source WISEJ022051.24+250927.6 we observe emission lines with equivalent width EW ∼ 31 Å, identifying it as a FSRQ with z = 0.48. The source WISEJ064459.38+603131.7, although not featuring a clear radio counterpart, shows a blazar-like spectrum with weak emission lines with EW ∼ 7 Å, yielding a redshift estimate of z = 0.36. In addition, we report optical spectroscopic observations of four WISE sources associated with known γ-ray blazars without a firm classification or redshift estimate. For the latter sources, we confirm a BL Lac classification, with a tentative redshift estimate for the source WISEJ100800.81+062121.2 of z = 0.65.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Radiological HEPA Filter 10-year Lifetime Evaluation in Research Facilities

High-efficiency particulate air (HEPA) filters are widely employed by nuclear facilities to remove radiological particulate matter from their effluent exhaust streams. The purpose of this study is to evaluate the relationships between the 10-year HEPA filter lifetime deployment and its other performance indicators. This 10-year-long endeavor to collect and analyze data regarding the service life of HEPA filters at the Pacific Northwest National Laboratory began in 2010. A set of HEPA filters were selected and have been surveyed and analyzed at least annually to verify compliance with permit conditions. The study suggests the frequency of filter replacement should be based on the actual operational requirements, such as fume hood face velocity and/or efficiency test results, instead of on the prescribed filter “age limit” of 10 years from the date of manufacture (e.g., birth date) when operating under dry conditions. The study has now been completed, and over the past decade all the HEPA filters have been replaced, due to either technical issues as listed in this report or the previously recommended filter “age limit” of 10 years as prescribed by the oversight bodies. Experimentally determined failure rates are also determined from the data set and can be used to estimate the chances of HEPA filters surviving 15, 20, or even 30 years.

61 RADIATION PROTECTION AND DOSIMETRY↗
DOE OSTI2025

Terahertz stimulated parametric downconversion of a magnon mode in an antiferromagnet

Parametric amplification, where one signal is enhanced by the action of another, offers both practical utility for boosting weak signals and fundamental insights into the nonlinear coupling between degrees of freedom. In condensed matter systems, interactions between collective modes offer avenues for nonlinear coherent manipulation of coupled excitations and quantum phases. Antiferromagnets, with inherently coupled magnon modes, provide a promising platform for nonlinear control of spin waves and magnetization. However, nonlinear magnon-magnon interactions have been only partially elaborated, leaving key gaps in the prospects for potential ultrahigh-bandwidth magnonic signal processing. Here, we excite two distinct coherent magnon modes in an antiferromagnet and find that the magnon mode with a lower frequency undergoes amplification when the higher-frequency mode is driven. We unveil the nonlinear excitation pathways of this stimulated parametric downconversion process by using polarization-selective two-dimensional terahertz spectroscopy. Our work provides fundamental insights into nonlinear magnonics in antiferromagnets, laying the groundwork for forthcoming spintronic and magnonic devices.

Science & Technology - Other Topics↗
DOE OSTI2019

The Nature of Anomalous Red Luminescence in K{sub 2}Al{sub 2}B{sub 2}O{sub 7} : Fe Nonlinear Optical Crystals

Spectra of anomalously intense luminescence at 1.675 eV (740 nm, FWHM = 0.173 eV) have been experimentally recorded for the first time in wide-band (180–3600 nm) K{sub 2}Al{sub 2}B{sub 2}O{sub 7} nonlinear optical crystals upon excitation in the spectral region of 4–5 harmonics of the fundamental frequency of Nd{sup 3+} radiation. It is shown by low-temperature (7–80 K) luminescence–optical spectroscopy under selective excitation by synchrotron radiation that red luminescence arises at the intracenter {sup 4}T{sub 1}({sup 4}G) → {sup 6}A{sub 1}({sup 6}S) transitions in Fe{sup 3+} impurity ions with a concentration below 2 ppm. The high excitation efficiency in the exciton region is due to partial overlap of the fundamental absorption edge of the crystal, where mobile excitons are excited, and wide O–Fe charge-transfer absorption band peaking at 6.5 eV. The luminescence spectrum and temperature dependence are caused by the superposition of the luminescence centers of two types (activation energies 9 and 20 meV) based on Fe{sup 3+} impurity ions located at regular Al{sup 3+} sites of two nonequivalent Al{sub 2}O{sub 7} clusters.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

All-dielectric multi-resonant bullseye antennas

Integrated devices that generate multiple optical resonances in the same volume can enhance on-chip nonlinear frequency generation, nonlinear spectroscopy, and quantum sensing. Here, we demonstrate circular Bragg antennas that exhibit multiple spatially overlapping, polarization-selective optical resonances. Using templated atomic layer deposition of TiO 2 , these devices can be fabricated on arbitrary substrates, making them compatible with a wide range of nonlinear materials and sensing targets, and couple efficiently to underlying films. In this work, we detail the design, simulation, and fabrication of all-dielectric multi-resonant bullseye antennas and characterize their performance using polarized broadband reflection spectroscopy.

47 OTHER INSTRUMENTATION↗
DOE OSTI2021

PIP-II 800 MeV Proton Linac Beam Pattern Generator

The PIP2 IT Beam Pattern Generator is the system that synchronizes beam injection and the RF systems between the PIP2 LINAC to the Booster. The RF frequencies of these two accelerator systems are not harmonically related. Synchronization is accomplished by controlling two MEBT Beam Choppers, which select 162.5MHz beam bunches from the LEBT and RFQ to produce an appropriate reduced beam bunch pattern that enables bucket-to-bucket transfer to the Booster RF at 46.46MHz (84th harmonic). This chopping pattern also reduces the beam current to an average of 2mA over the Booster injection, matching the Linac nominal beam current. The BPG also generates the RF frequency/phase reference which the Booster will phase lock to during injection. The BPG is fully programmable, allowing for arbitrary beam patterns with adjustable timing parameters, having a fine adjustment resolution of 38ps. The latter is accomplished using digital signal processing techniques. This paper discusses the design of the BPG, its construction, test results, and operational experience after being integrated into the PIP2 IT test accelerator and concludes with a discussion of the system’s performance and future plans.

43 PARTICLE ACCELERATORS↗
DOE OSTI2019

Interim Status of HEPA Filter 10-Year Lifetime Evaluation

High-efficiency particulate air (HEPA) filters are widely employed by nuclear facilities to remove radiological particulate matter from their effluent exhaust streams. The purpose of this study is to evaluate the relationships between the 10-year HEPA filter lifespan and its other performance indicators. The 10-year-long endeavor to collect and analyze data regarding the lifetime of HEPA filters at the Pacific Northwest National Laboratory began in 2019. Forty-nine HEPA filters were selected and have been surveyed and analyzed at least annually to verify compliance with permit conditions. The study suggests the frequency of filter replacement should be based on the actual operational requirements, such as fume hood face velocity and/or efficiency test results, instead of on the prescribed filter “age limit” of 10 years from the date of manufacture (e.g., birth date) when operating under dry conditions. Over the past nine years, only four HEPA filters have been replaced for technical issues.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Final Status of HEPA Filter 10-Year Lifetime Evaluation

High-efficiency particulate air (HEPA) filters are widely employed by nuclear facilities to remove radiological particulate matter from their effluent exhaust streams. The purpose of this study is to evaluate the relationships between the 10-year HEPA filter lifespan and its other performance indicators. The 10-year-long endeavor to collect and analyze data regarding the lifetime of HEPA filters at the Pacific Northwest National Laboratory began in 2010. Forty-nine HEPA filters were selected and have been surveyed and analyzed at least annually to verify compliance with permit conditions. The study suggests the frequency of filter replacement should be based on the actual operational requirements, such as fume hood face velocity and/or efficiency test results, instead of on the prescribed filter “age limit” of 10 years from the date of manufacture (e.g., birth date) when operating under dry conditions. Over the past decade, the study has now been completed, and all forty-nine HEPA filters have been replaced, due to either technical issues listed in this report, or the previously recommended filter “age limit” of 10 years.

61 RADIATION PROTECTION AND DOSIMETRY↗
DOE OSTI2019

A Study of the Impact of Reduced Inertia in Power Systems

Inertia in power systems plays an important role in maintaining the stability and reliability of the system by counteracting changes in frequency. However, the traditional sources of synchronous generation are being displaced by renewable resources, which often have no inherent inertia. This paper investigates the impact of reduced system inertia on several aspects of the dynamic stability of power systems, such as angular stability, primary frequency response, and oscillatory modes. This study is performed on a large-scale 2000 bus synthetic Texas model by selectively replacing synchronous generators with inverter-based generation resources. This paper also compares the analysis results obtained by the above-mentioned inertia-reduction approach of renewable integration with another approach in which the inertia constant of all synchronous generators is decreased. This paper demonstrates that only reducing the inertia of all synchronous generators in a system does not provide an accurate analysis of the challenges associated with the reduced system inertia caused by renewable integration.

System Inertia, Angular stability, System Inertial↗
DOE OSTI2026

A Search for Millimeter-bright Blazars as Astrophysical Neutrino Sources

The powerful jets of blazars have been historically considered as likely sites of high-energy cosmic-ray acceleration. However, the particulars of the launched jet and the locations of leptonic and hadronic jet loading remain unclear. In the case when leptonic and hadronic particle injection occur jointly, a temporal correlation between synchrotron radiation and neutrino production is expected. We use a first catalog of millimeter wavelength (95–225 GHz) blazar light curves from the Atacama Cosmology Telescope for a time-dependent correlation with 12 yr of muon neutrino events from the IceCube South Pole Neutrino Observatory. Such millimeter emission traces activity of the bright jet base, which is often self-absorbed at lower frequencies and potentially gamma-ray opaque. We perform an analysis of the population, as well as analyses of individual, selected sources. We do not observe a significant signal from the stacked population. TXS 0506+056 is found as the most significant, individual source, though this detection is not globally significant in our analysis of selected active galactic nuclei. Our results suggest that the majority of millimeter-bright blazars are neutrino dim. In general, it is possible that many blazars have lighter, leptonic jets, or that only selected blazars provide exceptional conditions for neutrino production.

Abbasi, R. [Loyola University, Chicago, IL (United↗
NASA NTRS1973

The Pioneer 9 electric field experiment. III - Radial gradients and storm observations.

We present a detailed analysis of the Pioneer 9 VLF electric field observations for 20 selected storm periods covering a heliocentric range extending from 0.754 AU to 0.99 AU. Although data from only two low frequency channels are available, the results of the present study tend to confirm the preliminary speculation by Scarf and Siscoe (1971) that the turbulent E-field spectrum in the disturbed solar wind has a significant radial gradient.

Scarf, F. L.↗
NASA NTRS1979

Description of a 2.3 kW power transformer for space applications

The principle features and special testing of a high voltage high power transformer designed and developed for space application are described. The transformer is operated in a series resonant inverter supplying beam power to a 30 cm mercury ion thruster. Electrical requirements include operation of 2.3 kW continuous power output, primary currents to 35 amps rms, and frequencies up to 20 kHz. High efficiency was obtained through detailed considerations of the tradeoffs available in core materials, wire selection, coil configurations and thermal control. A number of novel heat removal techniques are discussed which control the winding temperature using only the available conductive cooling.

Hansen, I.↗
NASA NTRS1982

Observation of additional low-degree 5-min modes of solar oscillation

High-order solar oscillations with degrees l=3, 4, and 5 could be detected. The observations were made by measuring the difference between the shifts in the Fe 5,124 spectrum line from light integrated from a central circular portion of the solar disk and from an annular portion exterior to it. The frequencies of the octupole modes agree well with the values obtained from whole-disk measurements at the South Pole. A least-squares fit of the observed frequencies to values interpolated between and extrapolated from the predictions of a sequence of solar models with different chemical compositions selects two models. One, a helium-rich solution, agrees with that of similar analyses of whole-disk data. The extrapolated solution has a relatively deep convection zone, and is thus consistent with analyses of 5-min oscillations of high degree.

Scherrer, P. H.↗