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THE PHYSICS OF THE 'HEARTBEAT' STATE OF GRS 1915+105

We present the first detailed phase-resolved spectral analysis of a joint Chandra High-Energy Transmission Grating Spectrometer and Rossi X-ray Timing Explorer observation of the {rho} variability class in the microquasar GRS 1915+105. The {rho} cycle displays a high-amplitude, double-peaked flare that recurs roughly every 50 s and is sometimes referred to as the 'heartbeat' oscillation. The spectral and timing properties of the oscillation are consistent with the radiation pressure instability and the evolution of a local Eddington limit in the inner disk. We exploit strong variations in the X-ray continuum, iron emission lines, and the accretion disk wind to probe the accretion geometry over nearly six orders of magnitude in distance from the black hole. At small scales (1-10 R{sub g}), we detect a burst of bremsstrahlung emission that appears to occur when a portion of the inner accretion disk evaporates due to radiation pressure. Jet activity, as inferred from the appearance of a short X-ray hard state, seems to be limited to times near minimum luminosity, with a duty cycle of {approx}10%. On larger scales (10{sup 5}-10{sup 6} R{sub g}), we use detailed photoionization arguments to track the relationship between the fast X-ray variability and the accretion disk wind. For the first time, we are able to show that changes in the broadband X-ray spectrum produce changes in the structure and density of the accretion disk wind on timescales as short as 5 s. These results clearly establish a causal link between the X-ray oscillations and the disk wind and therefore support the existence of a disk-jet-wind connection. Furthermore, our analysis shows that the mass-loss rate in the wind may be sufficient to cause long-term oscillations in the accretion rate, leading to state transitions in GRS 1915+105.

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PHOTOELECTRIC CHARGING OF DUST GRAINS IN THE ENVIRONMENT OF YOUNG STELLAR OBJECTS

The evolution of disks around young stellar objects (YSOs) is deeply affected by the YSOs' ultraviolet (UV) radiation field especially in the 500-1100 A spectral range. The two dominant processes are: the photodissociation of H{sub 2} molecules in the Werner and Lyman bands, and the emission of photoelectrons from dust grains when high energy photons are absorbed. Photoelectrons are an important source of gas heating. In this paper, dust grain charging when exposed to various possible UV fields in the YSOs' environment is investigated. Numerical simulations of the evolution of photoelectrons in the electric field created by the charged dust grains are carried out to obtain the charging profile of dust grains. From the simulations it appears that the different spectra produce significant quantitative and qualitative differences in the charging processes. Both the UV background and the Ae-Herbig star radiation field produce a relatively slow charging of dust grains due to the low fraction of sufficiently energetic photons. The radiation field of T Tauri stars (TTSs) is harder due to the release of magnetic energy in the dense magnetospheric environment. These numerical results have been used to propose a new simple analytical model for grain charging in the atmosphere of protostellar disks around TTSs susceptible to be used in any disk modeling. It has been found that the yield decreases exponentially with the dust charge and that two populations of photoelectrons are produced: a low energy population with mean kinetic energy E = 2.5 eV and a high energy population with E = 5.5-6 eV; the energy dispersion within the populations is {approx}1.3 eV (T {approx} 1.5 x 10{sup 4} K). The high energy population is susceptible of dissociating the H{sub 2} and ionizing some low ionization potential species, such as the Mg. These results add an additional role to dust on the chemistry of the layers just below the H{sub 2} photoionization front. This photoelectic yield has been applied to a simple evaluation of the dust charge in the atmospheres of accretion disks ({alpha}-disks).

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A VIEW OF THE NARROW-LINE REGION IN THE INFRARED: ACTIVE GALACTIC NUCLEI WITH RESOLVED FINE-STRUCTURE LINES IN THE SPITZER ARCHIVE

We queried the Spitzer archive for high-resolution observations with the Infrared Spectrograph of optically selected active galactic nuclei (AGNs) for the purpose of identifying sources with resolved fine-structure lines that would enable studies of the narrow-line region (NLR) at mid-infrared wavelengths. By combining 298 Spitzer spectra with 6 Infrared Space Observatory spectra, we present kinematic information of the NLR for 81, z {approx}< 0.3 AGNs. We used the [Ne V], [O IV], [Ne III], and [S IV] lines, whose fluxes correlate well with each other, to probe gas photoionized by the AGN. We found that the widths of the lines are, on average, increasing with the ionization potential of the species that emit them. No correlation of the line width with the critical density of the corresponding transition was found. The velocity dispersion of the gas, {sigma}, is systematically higher than that of the stars, {sigma}{sub *}, in the AGN host galaxy, and it scales with the mass of the central black hole, M{sub BH}. Further correlations between the line widths and luminosities L, and between L and M{sub BH}, are suggestive of a three-dimensional plane connecting log(M{sub BH}) to a linear combination of log ({sigma}) and log (L). Such a plane can be understood within the context of gas motions that are driven by AGN feedback mechanisms, or virialized gas motions with a power-law dependence of the NLR radius on the AGN luminosity. The M{sub BH} estimates obtained for 35 type 2 AGNs from this plane are consistent with those obtained from the M{sub BH{sup -{sigma}}} relation.

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DEEP VERY LARGE ARRAY RADIO CONTINUUM SURVEYS OF GLIMPSE EXTENDED GREEN OBJECTS (EGOs)

We present the results of deep, high angular resolution Very Large Array surveys for radio continuum emission toward a sample of 14 GLIMPSE Extended Green Objects (EGOs). Identified as massive young stellar object (MYSO) outflow candidates based on their extended 4.5 {mu}m emission in Spitzer images, the EGOs in our survey sample are also associated with 6.7 GHz Class II and/or 44 GHz Class I CH{sub 3}OH masers. No continuum is detected at 3.6 or 1.3 cm toward the majority (57%) of our targets (median rms {approx}0.03 and 0.25 mJy beam{sup -1}). Only two EGOs are associated with optically thin emission consistent with ultracompact/compact H II regions. Both of these sources exhibit cm-{lambda} multiplicity, with evidence that one of the less-evolved members may be driving the 4.5 {mu}m outflow. Most of the other cm-{lambda} EGO counterparts are weak ({approx}<1 mJy), unresolved, undetected at 1.3 cm, and characterized by intermediate spectral indices consistent with hypercompact (HC) H II regions or ionized winds or jets. One EGO centimeter (cm) counterpart, likely an optically thick HC H II region, is detected only at 1.3 cm and is associated with hot core line emission and H{sub 2}O and 6.7 GHz CH{sub 3}OH masers. The results of our exceptionally sensitive survey indicate that EGOs signify an early stage of massive star formation, before photoionizing feedback from the central MYSO significantly influences the (proto)cluster environment. Actively driving outflows (and so, presumably, actively accreting), the surveyed EGOs are associated with significant clump-scale gas reservoirs, providing sufficient material for sustained, rapid accretion.

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THE STRUCTURE OF THE STAR-FORMING CLUSTER RCW 38

We present a study of the structure of the high-mass star-forming region RCW 38 and the spatial distribution of its young stellar population. Spitzer Infrared Array Camera (IRAC) photometry (3-8 {mu}m) is combined with Two Micron All Sky Survey near-IR data to identify young stellar objects (YSOs) by IR-excess emission from their circumstellar material. Chandra X-ray data are used to identify class III pre-main-sequence stars lacking circumstellar material. We identify 624 YSOs: 23 class 0/I and 90 flat spectrum protostars, 437 class II stars, and 74 class III stars. We also identify 29 (27 new) O star candidates over the IRAC field. Seventy-two stars exhibit IR-variability, including 7 class 0/I and 12 flat spectrum YSOs. A further 177 tentative candidates are identified by their location in the IRAC [3.6] versus [3.6]-[5.8] color-magnitude diagram. We find strong evidence of subclustering in the region. Three subclusters were identified surrounding the central cluster, with massive and variable stars in each subcluster. The central region shows evidence of distinct spatial distributions of the protostars and pre-main-sequence stars. A previously detected IR cluster, DB2001{sub O}bj36, has been established as a subcluster of RCW 38. This suggests that star formation in RCW 38 occurs over a more extended area than previously thought. The gas-to-dust ratio is examined using the X-ray derived hydrogen column density, N{sub H} and the K-band extinction, and found to be consistent with the diffuse interstellar medium, in contrast with Serpens and NGC 1333. We posit that the high photoionizing flux of massive stars in RCW 38 affects the agglomeration of the dust grains.

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THE COSMOLOGICAL IMPACT OF LUMINOUS TeV BLAZARS. III. IMPLICATIONS FOR GALAXY CLUSTERS AND THE FORMATION OF DWARF GALAXIES

A subset of blazars are powerful TeV emitters, dominating the extragalactic component of the very high energy gamma-ray universe (E {approx}> 100 GeV). These TeV gamma rays generate ultrarelativistic electron-positron pairs via pair production with the extragalactic background light. While it has generally been assumed that the kinetic energy of these pairs cascades to GeV gamma rays via inverse Compton scattering, we have argued in Broderick et al. (Paper I in this series) that plasma beam instabilities are capable of dissipating the pairs' energy locally on timescales short in comparison to the inverse Compton cooling time, heating the intergalactic medium (IGM) with a rate that is independent of density. This dramatically increases the entropy of the IGM after redshift z {approx} 2, with a number of important implications for structure formation: (1) this suggests a scenario for the origin of the cool core (CC)/non-cool core (NCC) bimodality in galaxy clusters and groups. Early-forming galaxy groups are unaffected because they can efficiently radiate the additional entropy, developing a CC. However, late-forming groups do not have sufficient time to cool before the entropy is gravitationally reprocessed through successive mergers-counteracting cooling and potentially raising the core entropy further. This may result in a population of X-ray dim groups/clusters, consistent with X-ray stacking analyses of optically selected samples. Hence, blazar heating works differently than feedback by active galactic nuclei, which we show can balance radiative cooling but is unable to transform CC into NCC clusters on the buoyancy timescale due to the weak coupling between the mechanical energy to the cluster gas. (2) We predict a suppression of the Sunyaev-Zel'dovich (SZ) power spectrum template on angular scales smaller than 5' due to the globally reduced central pressure of groups and clusters forming after z {approx} 1. This allows for a larger rms amplitude of the density power spectrum, {sigma}{sub 8}, and may reconcile SZ-inferred values with those by other cosmological probes even after allowing for a contribution due to patchy reionization. (3) Our redshift-dependent entropy floor increases the characteristic halo mass below which dwarf galaxies cannot form by a factor of approximately 10 (50) at mean density (in voids) over that found in models that include photoionization alone. This prevents the formation of late-forming dwarf galaxies (z {approx}< 2) with masses ranging from 10{sup 10} to 10{sup 11} M{sub Sun} for redshifts z {approx} 2 to 0, respectively. This may help resolve the 'missing satellite problem' in the Milky Way of the low observed abundances of dwarf satellites compared to cold dark matter simulations and may bring the observed early star formation histories into agreement with galaxy formation models. At the same time, it explains the 'void phenomenon' by suppressing the formation of galaxies within existing dwarf halos of masses <3 Multiplication-Sign 10{sup 10} M{sub Sun} with a maximum circular velocity <60 km s{sup -1} for z {approx}< 2, hence reconciling the number of dwarfs in low-density regions in simulations and the paucity of those in observations.

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WINDS, CLUMPS, AND INTERACTING COSMIC RAYS IN M82

We construct a family of models for the evolution of energetic particles in the starburst galaxy M82 and compare them to observations to test the calorimeter assumption that all cosmic ray energy is radiated in the starburst region. Assuming constant cosmic ray acceleration efficiency with Milky Way parameters, we calculate the cosmic-ray proton and primary and secondary electron/positron populations as a function of energy. Cosmic rays are injected with Galactic energy distributions and electron-to-proton ratio via Type II supernovae at the observed rate of 0.07 yr{sup -1}. From the cosmic ray spectra, we predict the radio synchrotron and {gamma}-ray spectra. To more accurately model the radio spectrum, we incorporate a multiphase interstellar medium in the starburst region of M82. Our model interstellar medium is highly fragmented with compact dense molecular clouds and dense photoionized gas, both embedded in a hot, low density medium in overall pressure equilibrium. The spectra predicted by this one-zone model are compared to the observed radio and {gamma}-ray spectra of M82. {chi}{sup 2} tests are used with radio and {gamma}-ray observations and a range of model predictions to find the best-fit parameters. The best-fit model yields constraints on key parameters in the starburst zone of M82, including a magnetic field strength of {approx}250 {mu}G and a wind advection speed in the range of 300-700 km s{sup -1}. We find that M82 is a good electron calorimeter but not an ideal cosmic-ray proton calorimeter and discuss the implications of our results for the astrophysics of the far-infrared-radio correlation in starburst galaxies.

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HUBBLE SPACE TELESCOPE IMAGING OF THE BINARY NUCLEUS OF THE PLANETARY NEBULA EGB 6

EGB 6 is an ancient, low-surface-brightness planetary nebula. The central star, also cataloged as PG 0950+139, is a very hot DAOZ white dwarf (WD) with an apparent M dwarf companion, unresolved from the ground but detected initially through excesses in the JHK bands. Its kinematics indicates membership in the Galactic disk population. Inside of EGB 6 is an extremely dense emission knot-completely unexpected since significant mass loss from the WD should have ceased {approx}10{sup 5} yr ago. The electron density of the compact nebula is very high (2.2 Multiplication-Sign 10{sup 6} cm{sup -3}), as indicated by collisional de-excitation of forbidden emission lines. Hubble Space Telescope imaging and grism spectroscopy are reported here. These resolve the WD and apparent dM companion-at a separation of 0.''166, or a projected 96{sub -45}{sup +204} AU at the estimated distance of 576{sub -271}{sup +1224} pc (using the V magnitude). Much to our surprise, we found that the compact emission nebula is superposed on the dM companion, far from the photoionizing radiation of the WD. Moreover, a striking mid-infrared excess has recently been reported in the Spitzer/IRAC and MIPS bands, best fit with two dust shells. The derived ratio L{sub IR}/L{sub WD} = 2.7 Multiplication-Sign 10{sup -4} is the largest yet found for any WD or planetary nucleus. The compact nebula has maintained its high density for over three decades. We discuss two possible explanations for the origin and confinement of the compact nebula, neither of which is completely satisfactory. This leaves the genesis and confinement of the compact nebula an astrophysical puzzle, yet similar examples appear in the literature.

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ABSOLUTE INTEGRAL CROSS SECTIONS AND PRODUCT BRANCHING RATIOS FOR THE VIBRATIONALLY SELECTED ION-MOLECULE REACTIONS: N{sub 2}{sup +}(X {sup 2}{Sigma}{sub g}{sup +}; v {sup +} = 0-2) + CH{sub 4}

Absolute vibrationally selected integral cross sections ({sigma}{sub v+}'s) for the ion-molecule reaction N{sub 2}{sup +}(X {sup 2}{Sigma}{sub g}{sup +}; v {sup +} = 0-2) + CH{sub 4} have been measured by using the newly developed vacuum ultraviolet (VUV) laser pulsed field ionization-photoion (PFI-PI) double-quadrupole-double-octopole ion guide apparatus. By employing a novel electric field pulsing scheme to the VUV laser PFI-PI source, we have been able to prepare reactant N{sub 2}{sup +} ions in single-vibrational quantum states with not only high intensity and high purity but also high kinetic energy resolution, allowing integral cross section measurements to be conducted in the center-of-mass kinetic energies (E{sub cm}'s) from 0.05 to 10.00 eV. Three primary product channels corresponding to the formations of CH{sub 3}{sup +}, CH{sub 2}{sup +}, and N{sub 2}H{sup +} were identified. After correcting for the secondary reactions involving CH{sub 3}{sup +} and CH{sub 2}{sup +}, we have determined the {sigma}{sub v+} values of the formation of these primary product ions, {sigma}{sub v+}(CH{sub 3}{sup +}), {sigma}{sub v+}(CH{sub 2}{sup +}), and {sigma}{sub v+}(N{sub 2}H{sup +}), and their branching ratios, [{sigma}{sub v+}(CH{sub 3}{sup +}): {sigma}{sub v+}(CH{sub 2}{sup +}): {sigma}{sub v+}(N{sub 2}H{sup +})]/{sigma}{sub v+}(CH{sub 3}{sup +} + CH{sub 2}{sup +} + N{sub 2}H{sup +}), v {sup +} = 0-2, in the E{sub cm} range of 0.05-10.00 eV, where {sigma}{sub v+}(CH{sub 3}{sup +} + CH{sub 2}{sup +} + N{sub 2}H{sup +}) = {sigma}{sub v+}(CH{sub 3}{sup +}) + {sigma}{sub v+}(CH{sub 2}{sup +}) + {sigma}{sub v+}(N{sub 2}H{sup +}). The branching ratios are found to be nearly independent of the v {sup +} state and E{sub cm}. Complex v {sup +}-state and E{sub cm} dependences for {sigma}{sub v+}(CH{sub 3}{sup +}), {sigma}{sub v+}(CH{sub 2}{sup +}), and {sigma}{sub v+}(N{sub 2}H{sup +}) along with vibrational inhibition for the formation of these product ions are observed. The vibrational effects on the {sigma}{sub v+} values are sufficiently large to warrant the inclusion of the vibrationally excited reactions N{sub 2}{sup +}(X {sup 2}{Sigma}{sub g}{sup +}; v {sup +} {>=} 1) + CH{sub 4} for a more realistic modeling of the ion and neutral densities observed in the atmosphere of Titan. The cross-sectional data obtained in the present study are also useful for benchmarking theoretical calculations on ion-neutral collision dynamics.

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Constraints on two active galactic nuclei in the merger remnant cosmos J100043.15+020637.2

COSMOS J100043.15+020637.2 is a merger remnant at z = 0.36 with two optical nuclei, NW and SE, offset by 500 mas (2.5 kpc). Prior studies suggest two competing scenarios for these nuclei: (1) SE is an active galactic nucleus (AGN) lost from NW due to a gravitational-wave recoil. (2) NW and SE each contain an AGN, signaling a gravitational-slingshot recoil or inspiralling AGNs. We present new images from the Very Large Array (VLA) at a frequency ν = 9.0 GHz and a FWHM resolution θ = 320 mas (1.6 kpc), and the Very Long Baseline Array (VLBA) at ν = 1.52 GHz and θ = 15 mas (75 pc). The VLA imaging is sensitive to emission driven by AGNs and/or star formation, while the VLBA imaging is sensitive only to AGN-driven emission. No radio emission is detected at these frequencies. Folding in prior results, we find: (a) The properties of SE and its adjacent X-ray feature resemble those of the Type 1 AGN in NGC 4151, albeit with a much higher narrow emission-line luminosity. (b) The properties of NW are consistent with it hosting a Compton-thick AGN that warms ambient dust, photoionizes narrow emission-line gas, and is free-free absorbed by that gas. Finding (a) is consistent with scenarios (a) and (b). Finding (b) weakens the case for scenario (a) and strengthens the case for scenario (b). Follow-up observations are suggested.

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Protoplanetary disk masses in the young NGC 2024 cluster

We present the results from a Submillimeter Array survey of the 887 μm continuum emission from the protoplanetary disks around 95 young stars in the young cluster NGC 2024. Emission was detected from 22 infrared sources, with flux densities from ∼5 to 330 mJy; upper limits (at 3σ) for the other 73 sources range from 3 to 24 mJy. For standard assumptions, the corresponding disk masses range from ∼0.003 to 0.2 M{sub ⊙}, with upper limits at 0.002–0.01 M{sub ⊙}. The NGC 2024 sample has a slightly more populated tail at the high end of its disk mass distribution compared to other clusters, but without more information on the nature of the sample hosts it remains unclear if this difference is statistically significant or a superficial selection effect. Unlike in the Orion Trapezium, there is no evidence for a disk mass dependence on the (projected) separation from the massive star IRS 2b in the NGC 2024 cluster. We suggest that this is due to either the cluster youth or a comparatively weaker photoionizing radiation field.

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ON THE IMF IN A TRIGGERED STAR FORMATION CONTEXT

The origin of the stellar initial mass function (IMF) is a fundamental issue in the theory of star formation. It is generally fit with a composite power law. Some clues on the progenitors can be found in dense starless cores that have a core mass function (CMF) with a similar shape. In the low-mass end, these mass functions increase with mass, albeit the sample may be somewhat incomplete; in the high-mass end, the mass functions decrease with mass. There is an offset in the turn-over mass between the two mass distributions. The stellar mass for the IMF peak is lower than the corresponding core mass for the CMF peak in the Pipe Nebula by about a factor of three. Smaller offsets are found between the IMF and the CMFs in other nebulae. We suggest that the offset is likely induced during a starburst episode of global star formation which is triggered by the formation of a few O/B stars in the multi-phase media, which naturally emerged through the onset of thermal instability in the cloud-core formation process. We consider the scenario that the ignition of a few massive stars photoionizes the warm medium between the cores, increases the external pressure, reduces their Bonnor–Ebert mass, and triggers the collapse of some previously stable cores. We quantitatively reproduce the IMF in the low-mass end with the assumption of additional rotational fragmentation.

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The Los Alamos suite of relativistic atomic physics codes

The Los Alamos SuitE of Relativistic (LASER) atomic physics codes is a robust, mature platform that has been used to model highly charged ions in a variety of ways. The suite includes capabilities for calculating data related to fundamental atomic structure, as well as the processes of photoexcitation, electron-impact excitation and ionization, photoionization and autoionization within a consistent framework. These data can be of a basic nature, such as cross sections and collision strengths, which are useful in making predictions that can be compared with experiments to test fundamental theories of highly charged ions, such as quantum electrodynamics. The suite can also be used to generate detailed models of energy levels and rate coefficients, and to apply them in the collisional-radiative modeling of plasmas over a wide range of conditions. Such modeling is useful, for example, in the interpretation of spectra generated by a variety of plasmas. In this work, we provide a brief overview of the capabilities within the Los Alamos relativistic suite along with some examples of its application to the modeling of highly charged ions.

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Resonant ionization spectroscopy of autoionizing Rydberg states in cobalt and redetermination of its ionization potential

We obtained multi-step resonance ionization spectroscopy of cobalt using a hot-cavity laser ion source and three Ti:Sapphire lasers. Furthermore, the photoionization spectra revealed members of five new autoionizing Rydberg series that originate from three different lower levels of 3d 7 4s5s h 4 F 9/2 , 3d 7 4s4d f 4 G 11/2 , and 3d 7 4s4d f 4 H 13/2 and converge to the first four excited states of singly ionized Co. Our analyses of the Rydberg series yield 63564.689 0.036 cm -1 as the first ionization potential of Co, which is an order of magnitude more accurate than the previous estimation. Using a three-step resonance ionization scheme that employs an autoinizing Rydberg state in the last transition, we obtained an overall ionization efficiency of about 18% for Co.

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Roadmap of ultrafast x-ray atomic and molecular physics

X-ray free-electron lasers (XFELs) and table-top sources of x-rays based upon high harmonic generation (HHG) have revolutionized the field of ultrafast x-ray atomic and molecular physics, largely due to an explosive growth in capabilities in the past decade. XFELs now provide unprecedented intensity (10 20 W cm -2 ) of x-rays at wavelengths down to ~1 Ångstrom, and HHG provides unprecedented time resolution (~50 attoseconds) and a correspondingly large coherent bandwidth at longer wavelengths. For context, timescales can be referenced to the Bohr orbital period in hydrogen atom of 150 attoseconds and the hydrogen-molecule vibrational period of 8 femtoseconds; wavelength scales can be referenced to the chemically significant carbon K-edge at a photon energy of ~280 eV (44 Ångstroms) and the bond length in methane of ~1 Ångstrom. With these modern x-ray sources one now has the ability to focus on individual atoms, even when embedded in a complex molecule, and view electronic and nuclear motion on their intrinsic scales (attoseconds and Ångstroms). These sources have enabled coherent diffractive imaging, where one can image non-crystalline objects in three dimensions on ultrafast timescales, potentially with atomic resolution. The unprecedented intensity available with XFELs has opened new fields of multiphoton and nonlinear x-ray physics where behavior of matter under extreme conditions can be explored. The unprecedented time resolution and pulse synchronization provided by HHG sources has kindled fundamental investigations of time delays in photoionization, charge migration in molecules, and dynamics near conical intersections that are foundational to AMO physics and chemistry. This roadmap coincides with the year when three new XFEL facilities, operating at Ångstrom wavelengths, opened for users (European XFEL, Swiss-FEL and PAL-FEL in Korea) almost doubling the present worldwide number of XFELs, and documents the remarkable progress in HHG capabilities since its discovery roughly 30 years ago, showcasing experiments in AMO physics and other applications. Here in this paper, we capture the perspectives of 17 leading groups and organize the contributions into four categories: ultrafast molecular dynamics, multidimensional x-ray spectroscopies; high-intensity x-ray phenomena; attosecond x-ray science.

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Radiation damage free ghost diffraction with atomic resolution

The x-ray free electron lasers can enable diffractive structural determination of protein nanocrystals and single molecules that are too small and radiation-sensitive for conventional x-ray diffraction. However the electronic form factor may be modified during the ultrashort x-ray pulse due to photoionization and electron cascade caused by the intense x-ray pulse. For general x-ray imaging techniques, the minimization of the effects of radiation damage is of major concern to ensure reliable reconstruction of molecular structure. Here in this paper, we show that radiation damage free diffraction can be achieved with atomic spatial resolution by using x-ray parametric down-conversion and ghost diffraction with entangled photons of x-ray and optical frequencies. We show that the formation of the diffraction patterns satisfies a condition analogous to the Bragg equation, with a resolution that can be as fine as the crystal lattice length scale of several Ångstrom. Since the samples are illuminated by low energy optical photons, they can be free of radiation damage.

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LCLS in—photon out: fluorescence measurement of neon using soft x-rays

Here, we measured the fluorescence photon yield of neon upon soft x-ray ionization (~1200 eV) from the x-ray free-electron laser at Linac Coherent Light Source, and demonstrated the usage of a grazing incidence spectrometer with a variable line spacing grating to perform x-ray fluorescence spectroscopy on a gas phase system. Our measurements also allowed us to estimate the focal size of the beam from the theoretical description developed, in terms of the rate equation approximation accounting for photoionization shake off of neutral neon and double auger decay of single core holes.

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