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DOE OSTI2016

Verification of antiferromagnetic exchange coupling at room temperature using polar magneto-optic Kerr effect in thin EuS/Co multilayers with perpendicular magnetic anisotropy

We report on magneto-optic Kerr measurements in polar geometry carried out on a series of thin Co/EuS multilayers on suitable Co/Pd-multilayer substrates. Thin Co/EuS multilayers of a few nanometers individual layer thickness usually have their magnetization in plane. Co/Pd multilayers introduce a perpendicular magnetic anisotropy in the Co/EuS layers deposited on top, thus making it possible to measure magneto-optic signals in the polar geometry in remanence in order to study exchange coupling. Magneto-optic Kerr-effect spectra and hysteresis loops were recorded in the visible and ultraviolet photon-energy range at room temperature. The EuS contribution to the magneto-optic signal is extracted at 4.1 eV by combining hysteresis loops measured at different photon energies with polar magneto-optic Kerr-effect spectra recorded in remanence and in an applied magnetic field of 2.2 T. The extracted EuS signal shows clear signs of antiferromagnetic coupling of the Eu magnetic moments to the Co layers. This implies that the ordering temperature of at least a fraction of the EuS layers is above room temperature proving that magneto-optic Kerr-effect spectroscopy can be used here as a quasi-element-specific method.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2016

Strain effects on the optical conductivity of gapped graphene in the presence of Holstein phonons beyond the Dirac cone approximation

In this paper we study the optical conductivity and density of states (DOS) of doped gapped graphene beyond the Dirac cone approximation in the presence of electron-phonon (e-ph) interaction under strain, i.e., within the framework of a full π-band Holstein model, by using the Kubo linear response formalism that is established upon the retarded self-energy. A new peak in the optical conductivity for a large enough e-ph interaction strength is found which is associated to transitions between the midgap states and the Van Hove singularities of the main π-band. Optical conductivity decreases with strain and at large strains, the system has a zero optical conductivity at low energies due to optically inter-band excitations through the limit of zero doping. As a result, the Drude weight changes with e-ph interaction, temperature and strain. Consequently, DOS and optical conductivity remains stable with temperature at low e-ph coupling strengths.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

DOE OSTI2024

Multiparameter optical fiber sensing for energy infrastructure through nanoscale light–matter interactions: From hardware to software, science to commercial opportunities

Monitoring of energy infrastructure through robust yet economical sensing platforms is becoming an area of increased importance, with ubiquitous applications including the electrical grid, natural gas and oil transportation pipelines, H2 infrastructure (storage and transportation), carbon storage, power generation, and subsurface environments. Plasmonic and functional nanomaterial enabled fiber optic sensors show excellent promise for a wide range of sensing applications due to their versatility to be engineered for specific analytes of interest while retaining inherent advantages of the optical fiber sensor platform. Through the design of novel sensing layers, the optical transduction mechanism and wavelength dependence can also be tailored for ease of integration with low-cost interrogation systems enabling an inexpensive yet highly functional optical fiber sensing platform. In addition, recent advances in artificial intelligence and machine learning theoretical methods have been leveraged to simultaneously extract multiple parameters through multi-wavelength interrogation such that unique wavelengths can also serve as unique sensing elements, analogous to electronic nose sensor technologies. The concept of an optical fiber based “photonic nose” via multiple interrogation wavelengths and/or sensor nodes offers a compelling platform technology to realize multiparameter speciation of chemical analytes within complex gas mixtures. In this Perspective, we further generalize the notion of multiparameter sensing through the novel “photonic nervous system” concept based upon low-cost, functionalized optical fiber sensor probes monitoring a variety of distinct analyte classes (physical, chemical, electromagnetic, etc.) simultaneously to provide broad situational awareness via integrated sensors.

Su, Yang-Duan (ORCID:0000000214820902)↗

DOE OSTI2012

OPTICAL AND NEAR-INFRARED MONITORING OF THE BLACK HOLE X-RAY BINARY GX 339-4 DURING 2002-2010

We present the optical/infrared (O/IR) light curve of the black hole X-ray binary GX 339-4 collected at the SMARTS 1.3 m telescope from 2002 to 2010. During this time the source has undergone numerous state transitions including hard-to-soft state transitions when we see large changes in the near-IR flux accompanied by modest changes in optical flux, and three rebrightening events in 2003, 2005, and 2007 after GX 339-4 transitioned from the soft state to the hard. All but one outburst show similar behavior in the X-ray hardness-intensity diagram. We show that the O/IR colors follow two distinct tracks that reflect either the hard or soft X-ray state of the source. Thus, either of these two X-ray states can be inferred from O/IR observations alone. From these correlations we have constructed spectral energy distributions of the soft and hard states. During the hard state, the near-IR data have the same spectral slope as simultaneous radio data when GX 339-4 was in a bright optical state, implying that the near-IR is dominated by a non-thermal source, most likely originating from jets. Non-thermal emission dominates the near-IR bands during the hard state at all but the faintest optical states, and the fraction of non-thermal emission increases with increasing optical brightness. The spectral slope of the optical bands indicate that a heated thermal source is present during both the soft and hard X-ray states, even when GX 339-4 is at its faintest optical state. We have conducted a timing analysis of the light curve for the hard and soft states and find no evidence of a characteristic timescale within the range of 4-230 days.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2012

INVESTIGATING THE OPTICAL COUNTERPART CANDIDATES OF FOUR INTEGRAL SOURCES LOCALIZED WITH CHANDRA

We report on the optical spectroscopic follow-up observations of the candidate counterparts to four INTEGRAL sources: IGR J04069+5042, IGR J06552-1146, IGR J21188+4901, and IGR J22014+6034. The candidate counterparts were determined with Chandra, and the optical observations were performed with 1.5 m RTT-150 telescope (TUeBITAK National Observatory, Antalya, Turkey) and 2.4 m Hiltner Telescope (MDM Observatory, Kitt Peak, Arizona). Our spectroscopic results show that one of the two candidates of IGR J04069+5042 and the one observed for IGR J06552-1146 could be active late-type stars in RS CVn systems. However, according to the likelihood analysis based on Chandra and INTEGRAL, two optically weaker sources in the INTEGRAL error circle of IGR J06552-1146 have higher probabilities to be the actual counterpart. The candidate counterparts of IGR J21188+4901 are classified as an active M-type star and a late-type star. Among the optical spectra of four candidates of IGR J22014+6034, two show H{alpha} emission lines, one is a late-type star, and the other is an M type. The likelihood analysis favors a candidate with no distinguishing features in the optical spectrum. Two of the candidates classified as M-type dwarfs, are similar to some IGR candidates claimed to be symbiotic stars. However, some of the prominent features of symbiotic systems are missing in our spectra, and their NIR colors are not consistent with those expected for giants. We consider the IR colors of all IGR candidates claimed to be symbiotic systems and find that low-resolution optical spectrum may not be enough for conclusive identification.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2013

THE RADIO AND OPTICAL LUMINOSITY EVOLUTION OF QUASARS. II. THE SDSS SAMPLE

We determine the radio and optical luminosity evolutions and the true distribution of the radio-loudness parameter R, defined as the ratio of the radio to optical luminosity, for a set of more than 5000 quasars combining Sloan Digital Sky Survey optical and Faint Images of the Radio Sky at Twenty cm (FIRST) radio data. We apply the method of Efron and Petrosian to access the intrinsic distribution parameters, taking into account the truncations and correlations inherent in the data. We find that the population exhibits strong positive evolution with redshift in both wavebands, with somewhat greater radio evolution than optical. With the luminosity evolutions accounted for, we determine the density evolutions and local radio and optical luminosity functions. The intrinsic distribution of the radio-loudness parameter R is found to be quite different from the observed one and is smooth with no evidence of a bimodality in radio loudness for log R {>=} -1. The results we find are in general agreement with the previous analysis of Singal et al., which used POSS-I optical and FIRST radio data.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2013

THE TURBULENCE POWER SPECTRUM IN OPTICALLY THICK INTERSTELLAR CLOUDS

The Fourier power spectrum is one of the most widely used statistical tools to analyze the nature of magnetohydrodynamic (MHD) turbulence in the interstellar medium. Lazarian and Pogosyan predicted that the spectral slope should saturate to -3 for an optically thick medium and many observations exist in support of their prediction. However, there have not been any numerical studies to date for testing these results. We analyze the spatial power spectrum of MHD simulations with a wide range of sonic and Alfvenic Mach numbers, which include radiative transfer effects of the {sup 13}CO transition. We numerically confirm the predictions of Lazarian and Pogosyan that the spectral slope of line intensity maps of an optically thick medium saturates to -3. Furthermore, for very optically thin supersonic CO gas, where the density or CO abundance values are too low to excite emission in all but the densest shock compressed gas, we find that the spectral slope is shallower than expected from the column density. Finally, we find that mixed optically thin/thick CO gas, which has average optical depths on the order of unity, shows mixed behavior: for super-Alfvenic turbulence, the integrated intensity power spectral slopes generally follow the same trend with sonic Mach number as the true column density power spectrum slopes. However, for sub-Alfvenic turbulence the spectral slopes are steeper with values near -3 which are similar to the very optically thick regime.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2013

The microlensing event rate and optical depth toward the galactic bulge from MOA-II

We present measurements of the microlensing optical depth and event rate toward the Galactic Bulge (GB) based on two years of the MOA-II survey. This sample contains ∼1000 microlensing events, with an Einstein radius crossing time of t {sub E} ≤ 200 days in 22 bulge fields covering ∼42 deg{sup 2} between –5° < l < 10° and –7° < b < –1°. Our event rate and optical depth analysis uses 474 events with well-defined microlensing parameters. In the central fields with |l| < 5°, we find an event rate of Γ = [2.39 ± 1.1]e {sup [0.60±0.05](3–|b|)} × 10{sup –5} star{sup –1} yr{sup –1} and an optical depth (for events with t {sub E} ≤ 200 days) of τ{sub 200} = [2.35 ± 0.18]e {sup [0.51±0.07](3–|b|)} × 10{sup –6} for the 427 events, using all sources brighter than I{sub s} ≤ 20 mag. The distribution of observed fields is centered at (l, b) = (0.°38, –3.°72). We find that the event rate is maximized at low latitudes and a longitude of l ≈ 1°. For the 111 events in 3.2 deg{sup 2} of the central GB at |b| ≤ 3.°0 and 0.°0 ≤ l ≤ 2.°0, centered at (l, b) = (0.°97, –2.°26), we find Γ=4.57{sub −0.46}{sup +0.51}×10{sup −5} star{sup –1} yr{sup –1} and τ{sub 200}=3.64{sub −0.45}{sup +0.51}×10{sup −6}. We also consider a red clump giant (RCG) star sample with I{sub s} < 17.5, and we find that the event rate for the RCG sample is slightly lower than but consistent with the all-source event rate. The main difference is the lack of long duration events in the RCG sample due to a known selection effect. Our results are consistent with previous optical depth measurements, but they are somewhat lower than previous all-source measurements, and slightly higher than previous RCG optical depth measurements. This suggests that the previously observed difference in optical depth measurements between all-source and RCG samples may largely be due to statistical fluctuations. These event rate measurements toward the central GB are necessary to predict the microlensing event rate and to optimize the survey fields in future space missions such as Wide Field Infrared Space Telescope.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2013

A unified lense-thirring precession model for optical and X-ray quasi-periodic oscillations in black hole binaries

Recent observations of accreting black holes reveal the presence of quasi-periodic oscillations (QPO) in the optical power density spectra. The corresponding oscillation periods match those found in X-rays, implying a common origin. Among the numerous suggested X-ray QPO mechanisms, some may also work in the optical. However, their relevance to the broadband—optical through X-ray—spectral properties have not been investigated. For the first time, we discuss the QPO mechanism in the context of the self-consistent spectral model. We propose that the QPOs are produced by Lense-Thirring precession of the hot accretion flow, whose outer parts radiate in optical wavelengths. At the same time, its innermost parts are emitting X-rays, which explains the observed connection of QPO periods. We predict that the X-ray and optical QPOs should be either in phase or shifted by half a period, depending on the observer position. We investigate the QPO harmonic content and find that the variability amplitudes at the fundamental frequency are larger in the optical, while the X-rays are expected to have strong harmonics. We then discuss the QPO spectral dependence and compare the expectations to the existing data.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2013

Periodic optical variability of radio-detected ultracool dwarfs

A fraction of very low mass stars and brown dwarfs are known to be radio active, in some cases producing periodic pulses. Extensive studies of two such objects have also revealed optical periodic variability, and the nature of this variability remains unclear. Here, we report on multi-epoch optical photometric monitoring of six radio-detected dwarfs, spanning the ∼M8-L3.5 spectral range, conducted to investigate the ubiquity of periodic optical variability in radio-detected ultracool dwarfs. This survey is the most sensitive ground-based study carried out to date in search of periodic optical variability from late-type dwarfs, where we obtained 250 hr of monitoring, delivering photometric precision as low as ∼0.15%. Five of the six targets exhibit clear periodicity, in all cases likely associated with the rotation period of the dwarf, with a marginal detection found for the sixth. Our data points to a likely association between radio and optical periodic variability in late-M/early-L dwarfs, although the underlying physical cause of this correlation remains unclear. In one case, we have multiple epochs of monitoring of the archetype of pulsing radio dwarfs, the M9 TVLM 513–46546, spanning a period of 5 yr, which is sufficiently stable in phase to allow us to establish a period of 1.95958 ± 0.00005 hr. This phase stability may be associated with a large-scale stable magnetic field, further strengthening the correlation between radio activity and periodic optical variability. Finally, we find a tentative spin-orbit alignment of one component of the very low mass binary, LP 349–25.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2014

Comprehensive monitoring of gamma-ray bright blazars. I. Statistical study of optical, X-ray, and gamma-ray spectral slopes

We present γ-ray, X-ray, ultraviolet, optical, and near-infrared light curves of 33 γ-ray bright blazars over 4 years that we have been monitoring since 2008 August with multiple optical, ground-based telescopes and the Swift satellite, and augmented by data from the Fermi Gamma-ray Space Telescope and other publicly available data from Swift. The sample consists of 21 flat-spectrum radio quasars (FSRQs) and 12 BL Lac objects (BL Lacs). We identify quiescent and active states of the sources based on their γ-ray behavior. We derive γ-ray, X-ray, and optical spectral indices, α{sub γ}, α{sub X}, and α{sub o}, respectively (F{sub ν}∝ν{sup α}), and construct spectral energy distributions during quiescent and active states. We analyze the relationships between different spectral indices, blazar classes, and activity states. We find (1) significantly steeper γ-ray spectra of FSRQs than for BL Lacs during quiescent states, but a flattening of the spectra for FSRQs during active states while the BL Lacs show no significant change; (2) a small difference of α{sub X} within each class between states, with BL Lac X-ray spectra significantly steeper than in FSRQs; (3) a highly peaked distribution of X-ray spectral slopes of FSRQs at ∼ –0.60, but a very broad distribution of α{sub X} of BL Lacs during active states; (4) flattening of the optical spectra of FSRQs during quiescent states, but no statistically significant change of α{sub o} of BL Lacs between states; and (5) a positive correlation between optical and γ-ray spectral slopes of BL Lacs, with similar values of the slopes. We discuss the findings with respect to the relative prominence of different components of high-energy and optical emission as the flux state changes.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

D-Egg: a dual PMT optical module for IceCube

The D-Egg, an acronym for "Dual optical sensors in an Ellipsoid Glass for Gen2," is one of the optical modules designed for future extensions of the IceCube experiment at the South Pole. The D-Egg has an elongated-sphere shape to maximize the photon-sensitive effective area while maintaining a narrow diameter to reduce the cost and the time needed for drilling of the deployment holes in the glacial ice for the optical modules at depths up to 2700 m. The D-Egg design is utilized for the IceCube Upgrade, the next stage of the IceCube project also known as IceCube-Gen2 Phase 1, where nearly half of the optical sensors to be deployed are D-Eggs. With two 8-inch high-quantum efficiency photomultiplier tubes (PMTs) per module, D-Eggs offer an increased effective area while retaining the successful design of the IceCube digital optical module (DOM). The convolution of the wavelength-dependent effective area and the Cherenkov emission spectrum provides an effective photodetection sensitivity that is 2.8 times larger than that of IceCube DOMs. The signal of each of the two PMTs is digitized using ultra-low-power 14-bit analog-to-digital converters with a sampling frequency of 240 MSPS, enabling a flexible event triggering, as well as seamless and lossless event recording of single-photon signals to multi-photons exceeding 200 photoelectrons within 10 ns. Mass production of D-Eggs has been completed, with 277 out of the 310 D-Eggs produced to be used in the IceCube Upgrade. In this paper, we report the design of the D-Eggs, as well as the sensitivity and the single to multi-photon detection performance of mass-produced D-Eggs measured in a laboratory using the built-in data acquisition system in each D-Egg optical sensor module.

47 OTHER INSTRUMENTATION↗

DOE OSTI2014

LINKING Lyα AND LOW-IONIZATION TRANSITIONS AT LOW OPTICAL DEPTH

We suggest that low optical depth in the Lyman continuum (LyC) may relate the Lyα emission, C II and Si II absorption, and C II* and Si II* emission seen in high-redshift galaxies. We base this analysis on Hubble Space Telescope Cosmic Origins Spectrograph spectra of four Green Pea (GP) galaxies, which may be analogs of z > 2 Lyα emitters (LAEs). In the two GPs with the strongest Lyα emission, the Lyα line profiles show reduced signs of resonant scattering. Instead, the Lyα profiles resemble the Hα line profiles of evolved star ejecta, suggesting that the Lyα emission originates from a low column density and similar outflow geometry. The weak C II absorption and presence of non-resonant C II* emission in these GPs support this interpretation and imply a low LyC optical depth along the line of sight. In two additional GPs, weak Lyα emission and strong C II absorption suggest a higher optical depth. These two GPs differ in their Lyα profile shapes and C II* emission strengths, however, indicating different inclinations of the outflows to our line of sight. With these four GPs as examples, we explain the observed trends linking Lyα, C II, and C II* in stacked LAE spectra, in the context of optical depth and geometric effects. Specifically, in some galaxies with strong Lyα emission, a low LyC optical depth may allow Lyα to escape with reduced scattering. Furthermore, C II absorption, C II* emission, and Lyα profile shape can reveal the optical depth, constrain the orientation of neutral outflows in LAEs, and identify candidate LyC emitters.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Dark Energy Survey Identification of A Low-Mass Active Galactic Nucleus at Redshift 0.823 from Optical Variability

We report the identification of a low-mass active galactic nucleus (AGN), DES J0218−0430, in a redshift z = 0.823 galaxy in the Dark Energy Survey (DES) Supernova field. We select DES J0218−0430 as an AGN candidate by characterizing its long-term optical variability alone based on DES optical broad-band light curves spanning over 6 yr. An archival optical spectrum from the fourth phase of the Sloan Digital Sky Survey shows both broad Mg ii and broad H β lines, confirming its nature as a broad-line AGN. Archival XMM–Newton X-ray observations suggest an intrinsic hard X-ray luminosity of |$L_{{\rm 2-12\, keV}}\approx 7.6\pm 0.4\times 10^{43}$| erg s^−1, which exceeds those of the most X-ray luminous starburst galaxies, in support of an AGN driving the optical variability. Based on the broad H β from SDSS spectrum, we estimate a virial black hole (BH) mass of M_• ≈ 10^6.43–10^6.72 M_⊙ (with the error denoting the systematic uncertainty from different calibrations), consistent with the estimation from OzDES, making it the lowest mass AGN with redshift > 0.4 detected in optical. We estimate the host galaxy stellar mass to be M_* ≈ 10^10.5 ± 0.3 M_⊙ based on modelling the multiwavelength spectral energy distribution. DES J0218−0430 extends the M_•–M_* relation observed in luminous AGNs at z ∼ 1 to masses lower than being probed by previous work. Our work demonstrates the feasibility of using optical variability to identify low-mass AGNs at higher redshift in deeper synoptic surveys with direct implications for the upcoming Legacy Survey of Space and Time at Vera C. Rubin Observatory.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2025

Contemporaneous optical-radio observations of a fast radio burst in a close galaxy pair

ABSTRACT We present the MeerKAT discovery and MeerLICHT contemporaneous optical observations of the fast radio burst (FRB) 20230808F, which was found to have a dispersion measure of $\mathrm{DM}=653.2\pm 0.4\mathrm{\, pc\, cm^{-3}}$. FRB 20230808F has a scattering time-scale $\tau _{s}=3.1\pm 0.1\, \mathrm{ms}$ at 1563.6 MHz, a rotation measure $\mathrm{RM}=169.4\pm 0.2\, \mathrm{rad\, m^{-2}}$, and a radio fluence $F_{\mathrm{radio}}=1.72\pm 0.01\, \mathrm{Jy\, ms}$. We find no optical counterpart in the time immediately after the FRB, nor in the 3 months after the FRB during which we continued to monitor the field of the FRB. We set an optical upper flux limit in MeerLICHT’s q-band of $11.7\, \mathrm{\mu Jy}$ for a 60 s exposure which started ${\sim}3.4$ s after the burst, which corresponds to an optical fluence, $F_{\mathrm{opt}}$, of $0.039\, \mathrm{Jy\, ms}$ on a time-scale of ${\sim}3.4$ s. We obtain an estimate for the $q-$band luminosity limit of $vL_{v}\sim 1.3\times 10^{43}\, \mathrm{erg\, s^{-1}}$. We localize the burst to a close galaxy pair at a redshift of $z_{\mathrm{spec}}=0.3472\pm 0.0002$. Our time delay of ${\sim}3.4$ s between the FRB arrival time and the start of our optical exposure is the shortest ever for an as yet non-repeating FRB, and hence the closest to simultaneous optical follow-up that exists for such an FRB.

Hanmer, K. Y. (ORCID:0000000234757752)↗

DOE OSTI2024

Light-induced microwave noise in superconducting microwave-optical transducers

Microwave-to-optical transducers are integral to the future of superconducting quantum computing, as they would enable scaling and long-distance communication of superconducting quantum processors through optical-fiber links. However, optically induced microwave noise poses a significant challenge in achieving quantum transduction between microwave and optical frequencies. In this work, we study light-induced microwave noise in an integrated electro-optical transducer harnessing the Pockels effect of thin-film lithium niobate. We reveal three sources of added noise with distinctive time constants ranging from sub-100 ns to milliseconds. Furthermore, our results provide insights into the mechanisms and corresponding mitigation strategies for light-induced microwave noise in superconducting microwave-optical transducers and pave the way toward realizing the ultimate goal of quantum transduction.

42 ENGINEERING↗

DOE OSTI2019

Effect of optically induced potential on the energy of trapped exciton polaritons below the condensation threshold

Exciton-polaritons (polaritons herein) offer a unique nonlinear platform for studies of collective macroscopic quantum phenomena in a solid-state system. Shaping of polariton flow and polariton confinement via potential landscapes created by nonresonant optical pumping has gained considerable attention due to the flexibility and control enabled by optically induced potentials. Recently, large density-dependent energy shifts (blueshifts) exhibited by optically trapped polaritons at low densities, below the bosonic condensation threshold, were interpreted as an evidence of strong polariton-polariton interactions [Y. Sun et al., Nat. Phys. 13, 870 (2017)]. In this work, we further investigate the origins of these blueshifts in optically induced circular traps and present evidence of significant blueshifts of the polariton energy due to reshaping of the optically induced potential with laser pump power. Our work demonstrates the strong influence of the effective potential formed by an optically injected excitonic reservoir on the energy blueshifts observed below and up to the polariton condensation threshold and suggests that the observed blueshifts arise due to interaction of polaritons with the excitonic reservoir, rather than due to polariton-polariton interaction.

36 MATERIALS SCIENCE↗

DOE OSTI2018

Optical Time Reversal from Time-Dependent Epsilon-Near-Zero Media

Materials with a spatially uniform but temporally varying optical response have applications ranging from magnetic field-free optical isolators to fundamental studies of quantum field theories. However, these effects typically become relevant only for time variations oscillating at optical frequencies, thus presenting a significant hurdle that severely limits the realization of such conditions. Here we present a thin-film material with a permittivity that pulsates (uniformly in space) at optical frequencies and realizes a time-reversing medium of the form originally proposed by Pendry [Science 322, 71 (2008)]. We use an optically pumped, 500 nm thick film of epsilon-near-zero (ENZ) material based on Al-doped zinc oxide. An incident probe beam is both negatively refracted and time reversed through a reflected phase-conjugated beam. As a result of the high nonlinearity and the refractive index that is close to zero, the ENZ film leads to time reversed beams (simultaneous negative refraction and phase conjugation) with near-unit efficiency and greater-than-unit internal conversion efficiency. The ENZ platform therefore presents the time-reversal features required, e.g., for efficient subwavelength imaging, all-optical isolators and fundamental quantum field theory studies.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗