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At least 1,585 records · Page 88

Applicability of post-ionization theory to laser-assisted field evaporation of magnetite

Analysis of the mean Fe ion charge state from laser-assisted field evaporation of magnetite (Fe3O4) reveals unexpected trends as a function of laser pulse energy that break from conventional post-ionization theory for metals. For Fe ions evaporated from magnetite, the effects of post-ionization are partially offset by the increased prevalence of direct evaporation into higher charge states with increasing laser pulse energy. Therefore the final charge state is related to both the field strength and the laser pulse energy, despite those variables themselves being intertwined when analyzing at a constant detection rate. Comparison of data collected at different base temperatures also show that the increased prevalence of Fe2+ at higher laser energies is possibly not a direct thermal effect. Conversely, the ratio of 16O+:16O2+ is well-correlated with field strength and unaffected by laser pulse energy on its own, making it a better overall indicator of the field evaporation conditions than the mean Fe charge state. Plotting the normalized field strength versus laser pulse energy also elucidates a non-linear dependence, in agreement with previous observations on semiconductors, that suggests a field-dependent laser absorption efficiency. Together these observations demonstrate that the field evaporation process for laser-pulsed oxides exhibits fundamental differences from metallic specimens that cannot be completely explained by post-ionization theory. Further theoretical studies, combined with detailed analytical observations, are required to understand fully the field evaporation process of non-metallic samples.

Environmental Molecular Sciences Laboratory↗

Investigation of UV, ns-laser damage resistance of hafnia films produced by electron beam evaporation and ion beam sputtering deposition methods

Laser-induced damage in coating materials with a high index of refraction, such as hafnia, limits the performance of high power and high energy laser systems. Understanding the underlying physics responsible for laser damage holds the key for developing damage-resistant optical films. Previous studies have reported a substantial difference in laser damage onset for hafnia films produced by different deposition methods, yet the underlying mechanisms for the observed difference remain elusive. We combined laser damage testing with analytical characterizations and theoretical simulations to investigate the response of hafnia films produced by electron (e-) beam evaporation vs ion beam sputtering (IBS) methods upon UV ns-laser exposure. We found that e-beam produced hafnia films were overall more damage resistant; in addition, we observed a polarization anisotropy associated with the onset of damage in the e-beam films, while this effect was absent in the latter films. The observed differences can be attributed to the stark contrast in the pressure inside the pores inherent in both films. The high pressure inside the IBS-induced nanobubbles has been shown to reduce the threshold for laser-induced plasma breakdown leading to film damage. The polarization effects in the e-beam coatings can be related to the asymmetric electric field intensification induced by the columnar void structure. Our findings provide a fundamental basis for developing strategies to produce laser damage-resistant coatings for UV pulsed laser applications.

36 MATERIALS SCIENCE↗

Path to a single-stage, 100-GeV electron beam via a flying-focus-driven laser-plasma accelerator

Dephasingless laser wakefield acceleration (DLWFA), a novel laser wakefield acceleration concept based on the recently demonstrated “flying focus” technology, offers a new paradigm in laser-plasma acceleration that could advance the progress toward a TeV linear accelerator using a single-stage system without guiding structures. The recently proposed NSF OPAL laser facility could be the transformative technology that enables this grand challenge in laser-plasma acceleration. We review the viable parameter space for DLWFA based on the scaling of its performance with laser and plasma parameters, and we compare that performance to traditional laser wakefield acceleration. These scalings indicate the necessity for ultrashort, high-energy laser architectures such as NSF OPAL to achieve groundbreaking electron energies using DLWFA. Initial results from MTW-OPAL, the platform for the 6-J DLWFA demonstration experiment, show a tight, round focal spot over a distance of 3.7 mm. New particle-in-cell simulations of that platform indicate that using hydrogen for DLWFA reduces the amount of laser light that is distorted due to refraction at ionization fronts. An experimental path, and the computational and technical design work along that path, from the current status of the field to a single-stage, 100-GeV electron beam via DLWFA on NSF OPAL is outlined. Progress along that path is presented.

Shaw, J. L. [University of Rochester, NY (United S↗

SU-D-BRE-05: Feasibility and Limitations of Laser-Driven Proton Therapy: A Treatment Planning Study

Purpose: Laser-acceleration of particles may offer a cost- and spaceefficient alternative for future radiation therapy with particles. Laser-driven particle beams are pulsed with very short bunch times, and a high number of particles is delivered within one laser shot which cannot be portioned or modulated during irradiation. The goal of this study was to examine whether good treatment plans can be produced for laser-driven proton beams and to investigate the feasibility of a laser-driven treatment unit. Methods: An exponentially decaying proton spectrum was tracked through a gantry and energy selection beam line design to produce multiple proton spectra with different energy widths centered on various nominal energies. These spectra were fed into a treatment planning system to calculate spot scanning proton plans using different lateral widths of the beam and different numbers of protons contained in the initial spectrum. The clinical feasibility of the resulting plans was analyzed in terms of dosimetric quality and the required number of laser shots as an estimation of the overall treatment time. Results: We were able to produce treatment plans with plan qualities of clinical relevance for a maximum initial proton number per laser shot of 6*10{sup 8}. However, the associated minimum number of laser shots was in the order of 10{sup 4}, indicating a long delivery time in the order of at least 15 minutes, when assuming an optimistic repetition rate of the laser system of 10 Hz. Conclusion: With the simulated beam line and the assumed shape of the proton spectrum it was impossible to produce clinically acceptable treatment plans that can be delivered in a reasonable time. The situation can be improved by a method or a device in the beam line which can modulate the number of protons from shot to shot. Supported by DFG Cluster of Excellence: Munich-Centre for Advanced Photonics.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Fundamental Physical Mechanisms of Mitigation Approaches to Laser-Induced Damage on Ultraviolet Optics (FY08 LDRD Final Report)

The objective was to explore and further develop the concept that laser–induced damage on surfaces of an optic can be mitigated to extend its lifetime in high-fluence laser systems. The project scope explored mitigation processes utilizing laser, micro-machining, and chemical techniques including laser-induced damage testing of the mitigated site, and characterization of the size and shapes of the mitigation site with respect to downstream intensification of the high energy laser beam. Advanced materials processing and characterization tools, and computational tools were developed to investigate physical properties of the mitigated regions. The material focus of the mitigation effort was fused silica and potassium di-hydrogen phosphate (KDP) crystal optics. and to develop a fundamental understanding of the physical mechanisms of the mitigation processes is sought in order to extend their applicability to larger and deeper damage sites and to larger laser fluences. When successful, these mitigation processes will significantly extend the useful lifetime of the optic and drastically reduce the associated operating costs. For silica optics, mitigation processes utilizing mid-infrared (4.6 μm) and far infrared (10.6 μm) laser radiation from carbon dioxide lasers was used to ablate, evaporate, melt and anneal the damaged silica surface. By varying the laser parameters (power, pulse rate, spot size, etc.) these investigations evaluated the almost 100x difference in the optical absorption depth between these wavelengths in the efficacy in arresting damage growth, and controlling the end-state of the material in terms of shape morphology, residual stress and process by-products (vapor and re-condensed material). For crystal optics, micro-diamond tool machining and micro re-crystallization of KDP were investigated. A precision three-axis micro machine tool was developed, tested and shown capable of treating damage sites to 1 mm in size that were robust against re-initiation of damage and exhibited acceptable downstream intensification. Micro re-crystallization of KDP was accomplished through Gibbs-Thompson condensation at the tip of an Atomic Force Microscope stylus. By controlling the humidity at the tip and raster scanning of the stylus over damaged crystal surfaces, filling of scratched surfaces with re-crystallized material was demonstrated.

42 ENGINEERING↗

Collaborative Research: Instability and transport of laser beam in plasma

Our goal was to determine the onset of laser light scattering due to plasma wave instabilities. Such scatter is usually regarded as deleterious since laser beam strength is thereby diminished. While this kind of laser-plasma-instability (LPI) has long been understood for the case of coherent laser light, the theory of LPI onset for a laser beam with degraded coherence is recent. Such a laser beam fills plasma with a mottled intensity distribution, which has large fluctuations. The key question is: do the exceptionally large fluctuations control LPI onset or is it controlled by the relatively quiescent background laser intensity? We have answered this question. This is significant because LPI onset power in the former case is typically small compared to that of the latter. In addition, if large laser intensity fluctuations control LPI onset, then nonlinear effects become significant for less powerful laser beams than otherwise estimated.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Precision Laser Annealing of Focal Plane Arrays

We present results from laser annealing experiments in Si using a passively Q-switched Nd:YAG microlaser. Exposure with laser at fluence values above the damage threshold of commercially available photodiodes results in electrical damage (as measured by an increase in photodiode dark current). We show that increasing the laser fluence to values in excess of the damage threshold can result in annealing of a damage site and a reduction in detector dark current by as much as 100x in some cases. A still further increase in fluence results in irreparable damage. Thus we demonstrate the presence of a laser annealing window over which performance of damaged detectors can be at least partially reconstituted. Moreover dark current reduction is observed over the entire operating range of the diode indicating that device performance has been improved for all values of reverse bias voltage. Additionally, we will present results of laser annealing in Si waveguides. By exposing a small (<10 um) length of a Si waveguide to an annealing laser pulse, the longitudinal phase of light acquired in propagating through the waveguide can be modified with high precision, <15 milliradian per laser pulse. Phase tuning by 180 degrees is exhibited with multiple exposures to one arm of a Mach-Zehnder interferometer at fluence values below the morphological damage threshold of an etched Si waveguide. No reduction in optical transmission at 1550 nm was found after 220 annealing laser shots. Modeling results for laser annealing in Si are also presented.

42 ENGINEERING↗

FIBER LASER CONSTRUCTION AND THEORY INCLUDING FIBER BRAGG GRATINGS Photonic Crystal Fibers (PCFs) and applications of gas filled PCFs

The principles used in fiber lasers have been around for a while but it is only within the past few years that fiber lasers have become commercially available and used in high power laser applications. This paper will focus on the basic design principles of fiber lasers, including fiber Bragg gratings, principles of operation, and forms of non-linear effects. It will describe the type and associated doping of the fiber used and difficult designs used to guide energy from the pump to the active medium. Topics covered include fiber laser design, fiber Bragg gratings, materials used, differences in quantum energy loss, thermo-optical effects, stimulated Raman scattering, Brillouin scattering, photonic crystal fibers and applications of gas filled Photonic Crystal Fibers (PCFs). Thanks to fiber lasers, the energy required to produce high power lasers has greatly dropped and as such we can now produce kW power using a standard 120V 15A circuit. High power laser applications are always requiring more power. The fiber laser can now deliver the greater power that these applications demand. Future applications requiring more power than can be combined using standard materials or configurations will need to be developed to overcome the high energy density and high non-linear optical scattering effects present during high power operations.

47 OTHER INSTRUMENTATION↗

Time Dependent Analysis of Laser Heating of Metal Parts in Contact with HE

We consider the time dependent heat transfer of laser energy impinging on metal parts that are in contact with high explosives (HE). The predecessor to this calculation was TN-J4-17-2109, “Heat Transfer Analysis from Laser Energy on Metal Parts in Contact with HE”, which considered the time independent heat transfer and compared to experimental results. The intent here is to extend those results to the time dependent case. The steady-state results were developed because they were the “worst case” from a safety perspective: the steady state represents the highest possible temperature excursion. However, we found that the temperatures achieved were well above the safety limits established by the DOE High Explosives Safety Manual. Moreover, they were well above the safety limit published by the LANL / Weapons Facilities Operations (WFO) in WFO-OS-ES-48, which establishes an upper temperature limit of 70°C for metal in contact with High Explosive (HE). The J-4 response to the original results was to design, build, and deploy an interlock system for DARHT that would ensure no laser energy on the firing point when both personnel and HE were present. This system was tested and proved effective, refer TP-DARHT-1150, (12/19/2016). It was reviewed and approved by the LANL Explosives Instrumentation Review Committee, refer PRES-J4-16-2140, “DARHT Laser Diagnostics Interlock System: Presentation to the EIRC”, (2016). Although the interlock system prevented personnel from being on the firing point under conditions where the diagnostic lasers would heat metal above the WFO limit, the WFO limit was still exceeded during the Multiplexed Photonic Doppler Velocimetry (MPDV) tuning process. The only practical solution is to limit the amount of time that the MPDV lasers are engaged at full power. The diagnostics interlock system was implemented with laser shutters that can fully interrupt the beams, and these shutters can be used to limit the amount of time that the lasers will impinge on the hydrotest assembly. It is the purpose of this paper to provide quantitative guidance on what length of time can be permitted during this tuning process. Therefore, we will solve the time-dependent heat transfer equation to determine the temperature increase as a function of time. This function can be inverted to determine the maximum allowable time for energizing the lasers based on the maximum allowable temperature at the metal to HE interface.

42 ENGINEERING↗

Investigating Laser Preheat and Applied Magnetic Fields Relevant to the MagLIF Fusion Scheme

The MAGnetized Liner Inertial Fusion (MagLIF) scheme has achieved thermonuclear fusion yields on the Z Facility by imploding a cylindrical liner filled with D 2 fuel that is preheated with a multi-kJ laser and pre-magnetized with an axial Bz=10 T magnetic field. Preheating (T e = 100-200 eV) and pre-magnetizing (10-30 T) the fuel serves to reduce the implosion velocity required to achieve multi-keV fusion-relevant temperatures at stagnation with a modest radial convergence. The challenge of fuel preheat in MagLIF is to deposit multiple-kJ of energy into the underdense (n e /n c <0.1) fuel over ~10 mm target length efficiently and without introducing contaminants. Once the fuel is heated the applied axial magnetic field (ω ce τ e ~ 10) needs to suppress electron thermal conduction sufficiently to prevent unacceptable heat losses to the liner walls. In this LDRD we investigated laser energy deposition at two facilities: The OMEGA-EP laser at the Laboratory for Laser Energetics and the Z-beamlet laser at Sandia National Labs utilizing the PECOS chamber. Multiple experiments were carried out investigating laser transmission through LEH foils, laser heating of underdense gasses and the effects of magnetization on laser preheat. The studies find that magneto-hydrodynamic simulations are able to reproduce energy deposition at MagLIF-like conditions but that at the intensities currently used to preheat MagLIF significant laser plasma instabilities (LPI) occur which partly explain the inability of codes to reproduce previous MagLIF preheat studies. The experiments find that reducing the intensity and smoothing the beam dramatically reduces the amount of stimulated Brillouin backscatter and produces deposition profiles more similar to those produced in simulations. The experiments have provided a large and varied dataset that can be compared to simulations. As part of the LDRD new experimental capabilities have also been developed that will be used to design future MagLIF integrated experiments and investigate fuel magnetization.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Laser aircraft

The concept of a laser-powered aircraft is discussed. Laser flight would be completely compatible with existing airports and air-traffic control, with the airplane using kerosene only power, up to a cruising altitude of 9 km where the laser satellite would lock on and beam laser energy to it. Two major components make up the laser turbofan, a heat exchanger for converting laser radiation into thermal energy, and conventional turbomachinery. The laser power satellite would put out 42 Mw using a solar-powered thermal engine to generate electrical power for the closed-cycle supersonic electric discharge CO laser, whose radiators, heat exchangers, supersonic diffuser, and ducting will amount to 85% of the total subsystem mass. Relay satellites will be used to intercept the beam from the laser satellite, correct outgoing beam aberrations, and direct the beam to the next target. A 300-airplane fleet with transcontinental range is projected to save enough kerosene to equal the energy content of the entire system, including power and relay satellites, in one year.

Hertzberg, A.↗

Ultraviolet lasers. Citations from the International Aerospace Abstracts data base

Reports cited from the international literature describe various aspects of ultraviolet lasers including laser output, far ultraviolet radiation, electron pumping, optical pumping, and laser materials. Gas lasers, pulsed lasers, dye lasers, CO2 lasers, xenon fluoride lasers, and transversely excited atmospheric (TEA) lasers are considered. This updated bibliography contains 283 citations, 66 of which are new additions to the previous edition.

Mauk, S. C.↗

Tunable diode lasers for 3-30 micron infrared operation

The tunable diode laser is now widely used in high resolution infrared spectroscopy studies, taking into account laboratory and industrial applications. The present investigation is concerned with advances related to laser performance and reliability. The advances are the result of improvements in materials and device technologies. Reliability data for broad-area Pb(1-x)Sn(x)Se lasers are considered along with performance improvements in stripe-geometry lasers, laser performance at wavelengths above 25 microns, and laser performance at wavelengths below 4 microns. Attention is given to tunable Pb-salt infrared diode lasers, mesa-stripe geometry lasers of Pb(1-x)Sn(x)Se and PbS(1-x)Se(x), and long wavelength diode laser emission observed in both Pb(1-x)Sn(x)Te and Pb(1-x)Sn(x)Se.

Linden, K. J.↗

Laser production and heating of plasma for MHD application

Experiments have been made on the production and heating of plasmas by the absorption of laser radiation. These experiments were performed to ascertain the feasibility of using laser-produced or laser-heated plasmas as the input for a magnetohydrodynamic (MHD) generator. Such a system would have a broad application as a laser-to-electricity energy converter for space power transmission. Experiments with a 100-J-pulsed CO2 laser were conducted to investigate the breakdown of argon gas by a high-intensity laser beam, the parameters (electron density and temperature) of the plasma produced, and the formation and propagation of laser-supported detonation (LSD) waves. Experiments were also carried out using a 1-J-pulsed CO2 laser to heat the plasma produced in a shock tube. The shock-tube hydrogen plasma reached electron densities of approximately 10 to the 17th/cu cm and electron temperatures of approximately 1 eV. Absorption of the CO2 laser beam by the plasma was measured, and up to approximately 100 percent absorption was observed. Measurements with a small MHD generator showed that the energy extraction efficiency could be very large with values up to 56 percent being measured.

Jalufka, N. W.↗

Comparison of electrically driven lasers for space power transmission

High-power lasers in space could provide power for a variety of future missions such as spacecraft electric power requirements and laser propulsion. This study investigates four electrically pumped laser systems, all scaled to 1-MW laser output, that could provide power to spacecraft. The four laser systems are krypton fluoride, copper vapor, laser diode array, and carbon dioxide. Each system was powered by a large solar photovoltaic array which, in turn, provided power for the appropriate laser power conditioning subsystem. Each system was block-diagrammed, and the power and efficiency were found for each subsystem block component. The copper vapor system had the lowest system efficiency (6 percent). The CO2 laser was found to be the most readily scalable but has the disadvantage of long laser wavelength.

Deyoung, R. J.↗

Magnetically switched power supply system for lasers

A laser power supply system is described in which separate pulses are utilized to avalanche ionize the gas within the laser and then produce a sustained discharge to cause the gas to emit light energy. A pulsed voltage source is used to charge a storage device such as a distributed capacitance. A transmission line or other suitable electrical conductor connects the storage device to the laser. A saturable inductor switch is coupled in the transmission line for containing the energy within the storage device until the voltage level across the storage device reaches a predetermined level, which level is less than that required to avalanche ionize the gas. An avalanche ionization pulse generating circuit is coupled to the laser for generating a high voltage pulse of sufficient amplitude to avalanche ionize the laser gas. Once the laser gas is avalanche ionized, the energy within the storage device is discharged through the saturable inductor switch into the laser to provide the sustained discharge. The avalanche ionization generating circuit may include a separate voltage source which is connected across the laser or may be in the form of a voltage multiplier circuit connected between the storage device and the laser.

Pacala, Thomas J.↗

Development in tunable solid state lasers with high spectral purity, high efficiency and long lifetime for differential absorption lidar

The paper presents a review of tunable vibronic solid state lasers for DIAL measurements and provides new experimental results for tunable Ti:sapphire lasers, materials development, and spectral bandwidth narrowing through injection control. Pulsed injection control of a Ti:sapphire laser with a 2.5-pm narrow band pulsed dye laser and with another Ti:sapphire laser is demonstrated with nearly complete energy extraction, indicating homogeneous line broadening. The status of tunable solid state lasers in the 1.6-2.3 micron range for DIAL measurements of trace gases, and development trends for lasers with reduced cryogenic cooling needs, are included. The effects of laser gain on optical damage, energy extraction, and amplified spontaneous emission are indicated for several tunable lasers.

Hess, R. V.↗

Direct solar-pumped iodine laser amplifier

The optimum conditions of a solar pumped iodine laser are found in this research for the case of a continuous wave operation and a pulsed operation. The optimum product of the pressure(p) inside the laser tube and the tube diameter(d) was pd=40 approx. 50 torr-cm on the contrary to the case of a high intensity flashlamp pumped iodine laser where the optimum value of the product is known to be pd=150 torr-cm. The pressure-diameter product is less than 1/3 of that of the high power iodine laser. During the research period, various laser materials were also studied for solar pumping. Among the laser materials, Nd:YAG is found to have the lowest laser threshold pumping intensity of about 200 solar constant. The Rhodamine 6G was also tested as the solar pumped laser material. The threshold pumping power was measured to be about 20,000 solar constant. The amplification experiment for a continuously pumped iodine laser amplifier was performed using Vortek solar simulator and the amplification factors were measured for single pass amplification and triple pass amplification of the 15 cm long amplifier tube. The amplification of 5 was obtained for the triple pass amplification.

Han, Kwang S.↗