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Temperature-Dependent Spin-Lattice Relaxation of the Nitrogen-Vacancy Spin Triplet in Diamond
Spin-lattice relaxation within the nitrogen-vacancy (NV) center’s electronic ground-state spin triplet limits its coherence times, and thereby impacts its performance in quantum applications. We report measurements of the relaxation rates on the NV center’s $|m_s = 0 \rangle ↔ |m_s = ± 1 \rangle$ and $|m_s = -1 \rangle ↔ |m_s = + 1\rangle$ transitions as a function of temperature from 9 to 474 K in high-purity samples. We show that the temperature dependencies of the rates are reproduced by an ab initio theory of Raman scattering due to second-order spin-phonon interactions, and we discuss the applicability of the theory to other spin systems. Using a novel analytical model based on these results, we suggest that the high-temperature behavior of NV spin-lattice relaxation is dominated by interactions with two groups of quasilocalized phonons centered at 68.2(17) and 167(12) meV.
Guiding diamond spin qubit growth with computational methods
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Proposal for the search for new spin interactions at the micrometer scale using diamond quantum sensors
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Precision Electron-Beam Polarimetry at 1 GeV Using Diamond Microstrip Detectors
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Antiferromagnetic and Orbital Ordering on a Diamond Lattice Near Quantum Criticality
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Hyperfine Spectroscopy of Isotopically Engineered Group-IV Color Centers in Diamond
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Detecting Spin-Bath Polarization with Quantum Quench Phase Shifts of Single Spins in Diamond
Single-qubit sensing protocols can be used to measure qubit-bath coupling parameters. However, for sufficiently large coupling, the sensing protocol itself perturbs the bath, which is predicted to result in a characteristic response in the sensing measurements. Here, we observe this bath perturbation, also known as a quantum quench, by preparing the nuclear spin bath of a nitrogen-vacancy (NV) center in polarized initial states and performing phase-resolved spin-echo measurements on the NV electron spin. These measurements reveal a time-dependent phase determined by the initial state of the bath. We derive the relationship between the sensor phase and the Gaussian spin-bath polarization and apply it to reconstruct both the axial and transverse polarization components. Using this insight, we optimize the transfer efficiency of our dynamic nuclear polarization sequence. This technique for directly measuring bath polarization may assist in preparing high-fidelity quantum memory states, improving nanoscale NMR methods, and investigating non-Gaussian quantum baths.
Deducing density and strength of nanocrystalline Ta and diamond under extreme conditions from X-ray diffraction
Abstract not provided
Diamond Sampling for Approximate Maximum All-pairs Dot-product (MAD) Search.
Abstract not provided.
Dynamic Response to Electro-Optical Control of Diamond Based Non-Volatile Photo-Switch
Not provided.
Argonne Discovery Yields Self-Healing Diamond-Like Carbon
We report that large-scale reactive molecular dynamics simulations carried out on the US Department of Energy’s IBM Blue Gene/Q Mira supercomputer at the Argonne Leadership Computing Facility, along with experiments conducted by researchers in Argonne’s Energy Systems Division, enabled the design of a “self-healing” anti-wear coating that drastically reduces friction and related degradation in engines and moving machinery. Now, the computational work advanced for this purpose is being used to identify the friction-fighting potential of other catalysts.
Characterizing Damage on Si Wafer Surfaces Cut by Slurry and Diamond Wire Sawing
Abstract not provided
Demonstration and Analysis of Ultrahigh Forward Current Density Diamond Diodes
Not provided.