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NASA NTRS1985

UV lidar measurements of the stratospheric aerosol layer and comparison with other optical data

After the violent volcanic eruptions of El Chichon in Mexico (17.33 deg. N, 93.20 deg. W) in late March and early April 1982, enhanced stratospheric aerosols have been monitored by ruby (lasing wavelength lambda=694.3 nm) or Nd:YAG lidars (lambda=1064 or 532 nm). By these lidars, visible or near-infrared optical informations of stratospheric aerosols and their space-time variations can be obtained. It is usually difficult to measure the background level of stratospheric aerosols by an ultraviolet (UV) lidar, since Rayleigh scattering prevails over Mie scattering in the stratosphere. However, after the large volcanic eruptions, UV lidar measurements of stratospheric aerosols are possible. In order to obtain UV optical properties of stratospheric aerosols, measurements have been made at Fukuoka (33.65 deg. N, 130.35 deg. E) by a p-terphenyl dye laser at a wavelength of 340.5 nm. Observational results during October 1982, through May 1983, are shown and are compared with the results obtained by a ruby lidar at Tsukuba (36.05 deg. N, 140.13 deg. E).

Uchino, O.↗
NASA NTRS1985

Variations in stratospheric aerosol optical depth during northern warmings

In this paper, the properties of the stratospheric aerosol optical depth (above 50 mbar) have been studied by using aerosol extinction profiles (at 1 micron) derived from the Stratospheric Aerosol Measurement and Stratospheric Aerosol and Gas Experiment (SAGE) during warming periods in the Northern Hemisphere. It is shown that, during the disturbed periods in winter, low values of aerosol optical depth (less than 0.0002) are found within the low-pressure system(s) (at the 30-mbar pressure surface), while high values are found outside. Similar characteristics are found to exist for the simultaneously observed SAGE O3 and NO2 columnar density distributions. Strong longitudinal gradients are shown with the low values within and wherever the vortex exists. This characteristic is maintained during and after the circumpolar vortex is disturbed, even after breakdown, indicating an isolation of the material within the vortex.

Wang, P.-H.↗
NASA NTRS1985

Latitudinal variation of spectral optical thickness and columnar size distribution of the El Chichon stratospheric aerosol layer

Measurements are presented for the spectral optical thickness of El Chichon's stratospheric aerosol layer, obtained during an airborne latitudinal survey in April and May of 1983. Columnar aerosol size distributions of the stratosphere are derived by inverting the aerosol optical thickness measurements as a function of wavelength and from spectral aerosol depth measurements obtained during an airborne survey in October and November 1982. Spectral optical thickness data and the derived size distributions from both airborne missions show latitidunal regions with similar characteristics. Airborne solar radiometer measurements are shown to be useful in studies of the latitudinal variations of optical and related particle size characteristics of the stratospheric aerosol layer.

Spinhirne, J. D.↗
NASA NTRS1986

Observations of stratospheric aerosols associated with the El Chichon eruption

Lidar observations of aerosols were carried out at Aberystwyth between Nov. 1982 and Dec. 1985 using a frequency doubled and frequency tripled Nd/Yag laser and a receiver incorporating a 1 m diameter in a Newtonian telescope configuration. In analyses of the experimental data attention is paid to the magnitude of the coefficient relating extinction and backscatter, the choice being related to the possible presence of aerosols in the upper troposphere and the atmospheric densities employed in the normalisation procedure. The aerosol loading showed marked day to day changes in early months and an overall decay was apparent only after April 1983, this decay being consistent with an e sup -1 time of about 7 months. The general decay was accompanied by a lowering of the layer but layers of aerosols were shown intermittently at heights above the main layer in winter months. The height variations of photon counts corrected for range, or of aerosol backscatter ratio, showed clear signatures of the tropopause. A strong correlation was found between the heights of the tropopause identified from the lidar measurements and from radiosonde-borne temperature measurements. A notable feature of the observations is the appearance of very sharp height gradients of backscatter ratio which seem to be produced by differential advection.

Thomas, L.↗
NASA NTRS1986

Dispersion characteristics of volcanically injected aerosol as seen by SAGE I, SAM II, and SAGE II

General features of the dispersion of aerosols injected into the atmosphere by volcanic eruptions are described on the bases of data from the SAGE I, SAGE II and SAM II satellites. All three satellites carried sensors which measured the vertical profile of aerosol extinction at 1 micron wavelength. The discussion covers the eruptions of seven volcanoes over the period 1979-82. The events occurred at low latitudes and in the Northern Hemisphere. Aerosols from Northern Hemisphere eruptions stayed in the Northern Hemisphere, while aerosols from low latitude events spread to both hemispheres. Dispersion was fastest in the winter hemisphere. Sample details are discussed from tracking the dispersion of the aerosol from the eruption of El Chichon by SAGE II sensors.

Kent, G. S.↗
NASA NTRS1986

A global-scale model of aerosol backscatter at CO2 wavelengths for satellite-based lidar sensors

The status of a global-scale model of background aerosol backscatter cross-sections at CO2 wavelengths is described. The model needs, strategy, concept, parameters, and capabilities are addressed, and the data base is discussed, concluding data selection, CO2 backscatter measurements, aerosol optical measurements, aerosol microphysical measurements, water vapor measurements, and data analysis. Strong evidence is reported for a 'universal' background tropospheric aerosol population. Typical background backscatter values at CO2 wavelengths appear to be about 3 x 10 to the -11th to 8 x 10 to the -11th/m/sr. Background signatures are evident in most aerosol data sets which have global-scale coverage in space or time.

Bowdle, David A.↗
NASA NTRS1986

Antarctic springtime measurements of ozone, nitrogen dioxide, and aerosol extinction by SAM II, SAGE, and SAGE II

Simultaneous vertical profiles of O3, NO2, and aerosol extinction obtained with the Stratospheric Aerosol Measurement II, Stratospheric Aerosol and Gas Experiment (SAGE), and SAGE II satellite instruments across the southern polar vortex show that significant differences exist at all altitudes. Both gaseous species display lower concentrations within the vortex over measurement altitudes ranging from the tropopause to 60 km and 20 to 40 km for O3 and NO2, respectively. Aerosol extinction above 15-18 km and total aerosol stratospheric column are also lower inside the vortex than outside. Total column amounts of O3 and NO2 are found to be strongly coupled to spatial location within the vortex, with minimum total values located around the vortex center. Vertical profiles selected to emphasize the observed difference across the circumpolar vortex are presented for October 13, 1981, and October 13, 1985, near 70 and 68 deg S latitude, respectively.

Mccormick, M. P.↗
NASA NTRS1987

Concepts for collection of aerosols in Titan's atmosphere

This paper considers design of instruments for collection of aerosols during entry in Titan's atmosphere. Major constraints on designs are small sample collection time, low aerosol column density, and the need to collect 1-10 micrograms of aerosol for gas chromatographic analysis. Thus, it is important to maximize aerosol collection through collector design, which includes consideration of various types of collectors, and maximizing the collection efficiency of a given type of collector. Sampling systems discussed include inertial impactors, filters, electrostatic devices, and multistage instruments. Aerosol sampling is reviewed in the context of high-altitude (200-70 km) and low-altitude (60-30 km) regions of Titan's atmosphere.

Oberbeck, Verne R.↗
NASA NTRS1988

Forty-eight-inch lidar aerosol measurements taken at the Langley Research Center, May 1974 to December 1987

A ground based lidar system located at NASA Langley Research Center in Hampton, Va., was used to obtain high resolution vertical profiles of the stratospheric and upper tropospheric aerosol since 1974. More than 200 measurements obtained at a wavelength of 0.6943 microns during 1974 to 1987 are summarized. Plots of peak backscatter mixing ratio and integrated backscatter vs time are presented for the entire measurement sequence. The plots highlight the influence of several major volcanic eruptions on the long term stratospheric aerosol layer. In particular, the eruptions of El Chichon in late Mar. to early Apr. 1982, produced a massive aerosol layer. Aerosol enhancement from El Chichon reached Hampton, Va. by May 1982, with a scattering ratio of approx. 50 detected on Jul. 1, 1982. In addition, scattering ratio profiles for June 1982 to December 1987, along with tables containing numerical values of the backscatter ratio and backscattering function versus altitude, are included to further describe the upper tropospheric and stratospheric aerosol layer. A 14 year summary is presented, in a ready to use format, of lidar observations at a fixed midlatitude location to be used for further study.

Fuller, W. H., Jr.↗
NASA NTRS1987

Effects of El Chichon on stratospheric aerosols late 1982 to early 1984

Stratospheric aerosols collected over the western U.S. from late 1982 to early 1984 show the strong effects of El Chichon's eruption. Although mineral particles disappeared during this period, large acid droplets were still common. Because these have never been seen in prevolcanic, background-level collections, they apparently result from increased droplet growth made possible by the unusual abundance of sulfate. Aerosol size distributions show a wide variety of multimodal curves due to mixing of air masses containing aerosols of various ages or histories. Toward the end of the study time there are fewer large aerosols because of gravitational settling and poleward transport. The result is a steady reduction in sulfate, as most aerosol mass is concentrated in a small number of large droplets. Even the later sulfate levels are, however, five times typical prevolcanic background contents. Thus the influence of El Chichon on high-altitude was still considerable 22 months after eruption.

Snetsinger, K. G.↗
NASA NTRS1988

Regional aerosol chemistry of the Amazon Basin during the dry season

The distribution and chemical composition of the atmospheric aerosol over the Amazon Basin forest were determined during the 1985 July-August dry season, using data on the aerosol chemical constituent concentration collected during the NASA Global Tropospheric Experiment Amazon Boundary Layer Experiment 2A mission. The results of the analyses suggest that there is a remarkable compositional and spatial homogeneity of the atmospheric aerosol on an extensive regional scale. Particulate organic carbon is the dominant component of the atmospheric aerosol, exhibiting an average concentration of about 740 nmol/cu m in the mixed layer and about 220 nmol/cu m in free tropospheric air. Oxalate and SO4(2-) exhibited the greatest enrichment in the mixed layer, while Cl(-) showed essentially no enrichment. The aerosol in the Amazonian atmosphere is essentially acid-base neutral, primarily as a result of incorporation of NH(+), which is presumably derived from NH3 released by the forest ecosystem.

Talbot, R. W.↗
NASA NTRS1989

Lidar sensing of aerosols and clouds in the troposphere and stratosphere

Advances in the development and application of lidar as a tool for the remote sensing of atmospheric aerosols and clouds are reviewed. The lidar sensing technique is described, and various approaches for solving the lidar equation to retrieve aerosol properties are summarized. Examples are presented of lidar applications to aerosol and cloud sensing in both the troposphere and stratosphere. These include environmental monitoring, atmospheric-boundary-layer studies, retrieval of aerosol optical and physical properties, sensing of clouds, and investigation of volcanic effects in the stratosphere. Comments are offered regarding the future outlook for aerosol and cloud sensing by both ground-based and spaceborne lidars.

Reagan, John A.↗
NASA NTRS1990

SAM II and lidar aerosol profile comparisons during AASE

The NASA Langley Research Center aerosol lidar system was one of several instruments that flew aboard a DC-8 during the Airborne Arctic Stratospheric Expedition. Several of the Stratospheric Aerosol Measurement II (SAM II) altitude profiles of aerosol extinction were close enough in time and space to allow for intercomparison with the lidar measurements of aerosol backscatter. Comparisons between three SAM II 1.0 micron aerosol extinction profiles and analogous profiles inferred from nearly simultaneous airborne lidar measurements are discussed. The other two comparisons show the first near-simultaneous SAM II/lidar measurements of a polar stratospheric cloud (PSC). The comparison made well within the edge of a relatively homogeneous PSC layer was also good, especially using an extinction-to-backscatter model derived from in situ PSC particle size measurements.

Osborn, M. T.↗
NASA NTRS1990

Amazon Basin ozone and aerosol - Wet season observations

The ozone and aerosol number density data obtained from aircraft flights over the Amazon Basin (AB) during April and May of 1987 are summarized with particular attention given to the general characteristics of ozone and aerosol for wet season (WS), compared to dry season (DS), meteorology. It is concluded that the AB provides favorable conditions for the production of hydroxyl radical and subsequent chemical and photochemical reactions which generate or consume key atmospheric trace species. It is determined that a negative ozone gradient exists within the mixed layer (ML). WSML ozone is about 7 ppbv lower than that of DS. The net sink characteristics of the WSML are seen throughout the troposphere of the AB in that the ozone at 3-4 km altitude is typically 15-25 ppbv as compared to DS values of 30-35 ppbv. In terms of aerosol source characteristics of the AB, ML aerosols are 5-10 times higher than observed in the troposphere with ML values of 100-200 aerosols/cu cm. An analysis of aerosol size distribution data is presented.

Gregory, Gerald L.↗
NASA NTRS1990

Stratospheric ion and aerosol chemistry and possible links with cirrus cloud microphysics - A critical assessment

Aspects of stratospheric ion chemistry and physics are assessed as they relate to aerosol formation and the transport of aerosols to upper tropospheric regions to create conditions favorable for cirrus cloud formation. It is found that ion-induced nucleation and other known phase transitions involving ions and sulfuric acid vapor are probably not efficient processes for stratospheric aerosol formation, and cannot compete with condensation of sulfuric acid on preexisting particles of volcanic or meteoritic origin which are larger than about 0.15 micron in radius. Thus, galactic cosmic rays cannot have a significant impact on stratospheric aerosol population. Changes in the stratospheric aerosol burden due to volcanos are up to two orders of magnitude larger than changes in ion densities. Thus, volcanic activity may modulate the radiative properties of cirrus clouds.

Mohnen, Volker A.↗
NASA NTRS1984

The numerical simulation of the evolution of a Saharan dust outbreak by using a general prognostic aerosol model

A three-dimensional model is developed that explicitly predicts the evolution of the spatial distributions of aerosols utilizing a time-dependent, initial value prognostic aerosol model based on aerosol physicochemical processes, a knowledge of aerosol sinks and sources, and the predicted motions of the atmosphere. These models serve a useful purpose in determining standardized aerosol spectra for utilization in radiative transfer calculations. The first numerical prediction of a Saharan dust outbreak evolution is described. It is shown that the results are in qualitative agreement with measurements despite the fact that in this preliminary simulation the generation of the dust depended upon several empirically based assumptions. IR satellite photographs taken during GATE are being examined in an attempt to determine the sources of the dust.

Westphal, Douglas L.↗
NASA NTRS1991

Role of heterogeneous conversion of N2O5 on sulphate aerosols in global ozone losses

The reaction rate of N2O5 on sulphate aerosols is included in a model to predict global ozone loss and the column abundances of atmospheric gases. Because the reaction of N2O5 and the aerosols can take place in the stratospheric sulphate aerosol layer, it is included in the 2D model so that the results can be compared to abundances derived from satellite data and ground-based measurements. The N2O5/sulphate reaction is the only heterogeneous reaction in the model, in which aerosol loading is assumed to be constant and only diurnal values are examined. The decadal ozone trends resulting from calculations based on the model are found to be closer to the observed values. An important conclusion is that measurements of OH, ClO, HNO3, NO, and NO2 in the region of about 14-25 km are needed to examine significant changes in their abundances resulting from the inclusion of the N2O5/sulphate aerosol reaction.

Rodriguez, Jose M.↗
NASA NTRS1991

Condensational growth and trace species scavenging in stratospheric sulfuric acid/water aerosol droplets

Stratospheric aerosols play a significant role in the environment. The composition of aerosols is believed to be a liquid solution of sulfuric acid and water with numerous trace species. Of these trace species, ozone in particular was recognized as being very important in its role of shielding the environment from harmful ultraviolet radiation. Also among the trace species are HCl and ClONO2, the so called chlorine reservoir species and various oxides of nitrogen. The quantity of stratospheric aerosol and its particle size distribution determines, to a large degree, the chemistry present in the stratosphere. Aerosols experience 3 types of growth: nucleation, condensation, and coagulation. The application of condensation investigations to the specific problem of stratospheric aerosols is discussed.

Tompson, Robert V., Jr.↗