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DOE OSTI2020

An Observational Comparison of Level of Neutral Buoyancy and Level of Maximum Detrainment in Tropical Deep Convective Clouds

Tropical deep convective clouds are important drivers of large-scale atmospheric circulation representing the main vertical transport pathway through the depth of the troposphere for heat, momentum, water, and chemical species. The strength and depth of this transport are impacted by the convective updraft size and intensity that are driven by buoyancy, dynamical forcing, and mixing of environmental air, i.e., entrainment. In this paper, we identify tropical deep convective systems with well-defined forward anvils using Atmospheric Radiation Measurement (ARM) ground-based profiling radars, at three ARM fixed-sites in the Tropical Western Pacific (TWP; i.e., Manus, Nauru, Darwin) and three ARM Mobile Facility deployments in Niamey, Niger; Gan Island, Maldives; and Manacapuru, Brazil. We use the difference between the level of neutral buoyancy (LNB) and the level of maximum detrainment (LMD) as a proxy for the effective bulk convective entrainment (εproxy). The LNB, the theoretical height that a parcel raised above the level of free convection would reach with no mixing, is calculated based on pre-convection radiosonde measurements using parcel theory. The LMD is the height of the maximum reflectivity observed in forward anvil clouds by profiling radars. Deep convective systems over the TWP show higher LNBs that extend to 16.3 km on average and larger εproxy (median LNB minus LMD up to 6.5 km) compared to their continental counterparts in the Amazon and West Africa. Oceanic conditions show larger convective available potential energy (CAPE) coupled with higher moisture at low levels which favors larger εproxy. In contrast, continental cases initiate and develop under high convective inhibition, steeper environmental lapse rate, and high wind shear conditions, which show smaller offset between LNB and LMD. Deep convective cases that promote significant cold pools at the surface experience less εproxy. Using a Random Forest regression algorithm, CAPE is associated with the highest feature importance score for predicting convective εproxy, followed by low-level relative humidity. For continental cases, the low-level wind shear also indicates higher importance.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1985

The impact of polar stratospheric clouds on the heating rates of the winter polar stratosphere

The perturbation affecting IR radiative heating rates of the lower stratosphere that are prompted by the occurrence of polar stratospheric clouds (PSCs) during the Arctic and Antarctic winter are presently calculated by means of a multispectral radiative transfer code that allows for scattering, absorption, and thermal emission by particles and gases. Attention is given to perturbations arising from both the particulate opacity of the PSCs and the decrease of H2O vapor accompanying their formation. For plausible values of model parameters, the former, direct effect is always one of increased radiative cooling, while the indirect effect is always one of decreased cooling.

Pollack, J. B.↗

NASA NTRS1990

Analysis of radiation parameters derived from the multisatellite Earth Radiation Budget Experiment

To quantify the diurnal radiative heating and cooling cycles of the earth and the atmosphere, data from instruments on the Earth Radiation Budget Satellite (ERBS) spacecraft and NOAA-9 satellites obtained from February 1985 through January 1986 were used to investigate longwave (LW) and shortwave (SW) flux as well as albedo for each month of the year. Seasonal variations of radiative parameters and their diurnal cycles are examined for the deserts, vegetated land, and oceans over the globe. The results show significant seasonal variations in both the outgoing LW and the absorbed SW flux, and a pronounced difference was found between oceanic and continental surfaces. Over much of the globe, LW warming is balanced by SW cooling, and clouds have a net cooling effect on the earth. Many areas of the earth were found to exhibit significant diurnal variations in both the LW flux and albedo.

Gibson, G. G.↗

NASA NTRS1993

Plasma irregularities caused by cycloid bunching of the CRRES G-2 barium release

The Combined Release and Radiation Effects Satellite (CRRES) spacecraft carried a number of barium thermite canisters for release into the upper atmosphere. The barium release labeled G-2 showed evidence of curved irregularities not aligned with the ambient magnetic field B. The newly discovered curved structures can be explained by a process called cycloid bunching. Cycloid bunching occurs when plasma is created by photoionization of a neutral cloud injected at high velocity perpendicular to B. If the injection velocity is much larger than the expansion speed of the cloud, the ion trail will form a cycloid that has irregularities spaced by the product of the perpendicular injection speed and the ion gyroperiod, Images of the solar-illuminated barium ions are compared with the results of a three-dimensional kinetic simulation. Cycloid bunching is shown to be responsible for the rapid generation of both curved and field-aligned irregularities in the CRRES G-2 experiment.

Bernhardt, P. A.↗

NASA NTRS1994

Ion Chemistry in Atmospheric and Astrophysical Plasmas

There are many differences and also remarkable similarities between the ion chemistry and physics of planetary ionospheres and the ion chemistry and physics of astronomical environments beyond the solar system. In the early Universe, an expanded cooling gas of hydrogen and helium was embedded in the cosmic background radiation field and ionized by it. As the Universe cooled by adiabatic expansion, recombination occurred and molecular formation was driven by catalytic reactions involving the relict electrons and protons. Similar chemical processes are effective in the ionized zones of gaseous and planetary nebulae and in stellar winds where the ionization is due to radiation from the central stars, in the envelopes of supernovae where the ionization is initiated by the deposition of gamma-rays, in dissociative shocks where the ionization arises from electron impacts in a hot gas and in quasar broad-line region clouds where the quasar is responsible for the ionization. At high altitudes in the atmospheres of the Jovian planets, the main constituents are hydrogen and helium and the ion chemistry and physics is determined by the same processes, the source of the ionization being solar ultraviolet radiation and cosmic rays. After the collapse of the first distinct astronomical entities to emerge from the uniform flow, heavy elements were created by nuclear burning in the cores of the collapsed objects and distributed throughout the Universe by winds and explosions. The chemistry and physics became more complicated. Over 90 distinct molecular species have been identified in interstellar clouds where they are ionized globally by cosmic ray impacts and locally by radiation and shocks associated with star formation and evolution. Complex molecules have also been found in circumstellar shells of evolved stars. At intermediate and low altitudes in the Jovian atmospheres, the ion chemistry is complicated by the increasing abundance of heavy elements such as carbon, and an extensive array of complex molecules has been predicted. Reactions involving heavy elements dominate the structure of the ionspheres of the terrestrial planets and the satellites Titan and Triton.

Dalgarno, A.↗

NASA NTRS1994

How well was total ozone abundance inferred with Mariner 9?

Ozone is a key to understanding atmospheric chemistry on Mars. Over 20 photochemical models of the martian atmosphere have been published, and O3 is often used as a benchmark for these models. O3 abundance has been inferred from instrumentation on several spacecraft, with the most complete coverage provided by Mariner 9. The Mariner 9 UV spectrometer scanned from 2100 to 3500 Angstroms with a spectral resolution of 15 Angstroms and an effective field-of-view of approximately 300 sq km. The only atmospheric absorption in the 2000 to 3000 A wavelength region was previously assumed to come from the Hartley band system of ozone, which has an opacity of order unity at winter polar latitudes. Therefore, the amount of ozone was inferred by fitting this absorption feature with laboratory data of ozone absorption. Mars O3 shows strong seasonal and latitudinal variation, with column abundances ranging from 0.2 micron-atm at equatorial latitudes to 60 micron-atm over northern winter polar latitudes (1 micron-atm is a column abundance of 2.689 x 10 exp 15 molecules cm(exp -2)). However, the O3 abundance is never great enough to significantly affect atmospheric temperatures or surface temperatures and frost amounts. Some of the previously-inferred O3 abundances are shown. A radiative transfer computer model is used to re-examine the Mariner 9 UV spectra. Assuming a constant mixing ratio for O3 and no chemical or radiative interaction between O3 and clouds/dust, it is shown that when typical amounts of dust and cloud are present that significant underestimation of O3 abundance occurs. A factor of 3 times as much O3 is needed to generate the same spectrum the spacecraft would measure for a cloudy, dusty atmosphere as for a clear atmosphere. If the scattering properties of martian clouds and dust were well known, then their appearance would not be a problem, as a model would be capable of retrieving the O3 abundance. However, these properties are not well known, which raises doubts about the effectiveness of the UV reflectance spectroscopy technique for measuring O3 abundance on Mars.

Lindner, Bernhard Lee↗

DOE OSTI2025

Multiscale ACI Satellite Database

The SATELLITE_EAGLES_PNNL NetCDF dataset contains a suite of satellite- and reanalysis-derived atmospheric and surface parameters on a regular latitude–longitude grid. The dataset includes core geophysical fields such as land fraction, aerosol optical depth at multiple wavelengths (465, 550, 667, and 865 nm), sea surface temperature, estimated inversion strength, and various thermodynamic and dynamic quantities (e.g., relative humidity, vertical velocity, boundary-layer height, and surface fluxes) from both MERRA and ERA reanalysis products, provided as daily-mean and instantaneous values. A major component of the dataset consists of MODIS-retrieved cloud microphysical properties, including cloud droplet number concentration, cloud effective radius, optical thickness, and liquid water path, provided for three compositing regimes (“All,” “Q06,” and “G18”). Corresponding cloud-top parameters—temperature, height, and pressure—along with total and domain-mean cloud fraction fields are also included. The file further integrates additional satellite data from AMSR-E (for cloud water, rain water, and surface precipitation retrievals) and CERES (for top-of-atmosphere radiative fluxes, cloud fractions, and albedo). This dataset is designed to evaluate aerosol–cloud interactions in warm clouds, emphasizing the use of MODIS for deriving cloud droplet number concentration and liquid water path statistics. The complementary satellite and reanalysis fields are co-located and time-matched to the same instantaneous MODIS observations, enabling consistent comparisons between cloud properties, aerosol loading, and large-scale meteorological conditions. The dataset is recently featured in Christensen et al. (2025), Machine Learning Reveals Strong Grid-Scale Dependence in the Satellite Nd–LWP Relationship, EGUsphere [preprint], https://doi.org/10.5194/egusphere-2025-3850, 2025.

Christensen, Matthew [Pacific Northwest National L↗

DOE OSTI2025

Multiscale ACI Satellite Database

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1993

Remote sensing cloud properties from high spectral resolution infrared observations

A technique for estimating cloud radiative properties (spectral emissivity and reflectivity) in the IR is developed based on observations at a spectral resolution of approximately 0.5/cm. The algorithm uses spectral radiance observations and theoretical calculations of the IR spectra for clear and cloudy conditions along with lidar-determined cloud-base and cloud-top pressure. An advantage of the high spectral resolution observations is that the absorption effects of atmospheric gases are minimized by analyzing between gaseous absorption lines. The technique is applicable to both ground-based and aircraft-based platforms and derives the effective particle size and associated cloud water content required to satisfy, theoretically, the observed cloud IR spectra. The algorithm is tested using theoretical simulations and applied to observations made with the University of Wisconsin's ground-based and NASA ER-2 aircraft High-Resolution Infrared Spectrometer instruments.

Smith, William L.↗

NASA NTRS2003

Vertically Resolved Aerosol Optical Properties over the ARM SGP Site

In order to meet one of its goals - to relate observations of radiative fluxes and radiances to the atmospheric composition - the Department of Energy's Atmospheric Radiation Measurement (ARM) program has pursued measurements and modeling activities that attempt to determine how aerosols impact atmospheric radiative transfer, both directly and indirectly. However, significant discrepancies between aerosol properties measured in situ or remotely remain. To this end, the ARM program will conduct an Aerosol Intensive Operational Period (IOP) in May 2003 at the ARM Southern Great Plains (SGP) site in north central Oklahoma. The IOP involves airborne measurements from two airplanes over the heavily instrumented SGP site. We will give an overview of early airborne results obtained aboard Center for Interdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS) Twin Otter aircraft. The aircraft will carry instrumentation to perform in-situ measurements of aerosol absorption, scattering, extinction and particle size including such novel techniques as the photoacoustic and cavity ring-down methods. Aerosol optical depth and extinction will be measured with the NASA Ames Airborne Tracking 14-channel sunphotometer. Furthermore up- and downwelling solar (broadband and spectral) and infrared radiation will be measured using three different instruments. The up-looking radiation instruments will be mounted on a newly developed stabilized platform, which will keep the instruments level up to aircraft pitch and roll angles of 10 degrees. Additional effort will be directed toward measurement of cloud condensation nucleus concentration as a function of supersaturation and relating CCN concentration to aerosol composition and size distribution. This relation is central to description of the aerosol indirect effect.

Schmid, B.↗

NASA NTRS2008

Quasi-Optical Transmission Line for 94-GHz Radar

A quasi-optical transmission line (QOTL) has been developed as a low-loss transmission line for a spaceborne cloudobserving radar instrument that operates at a nominal frequency of 94 GHz. This QOTL could also readily be redesigned for use in terrestrial millimeter-wave radar systems and millimeter-wave imaging systems. In the absence of this or another lowloss transmission line, it would be necessary to use a waveguide transmission line in the original radar application. Unfortunately, transmission losses increase and power-handling capacities of waveguides generally decrease with frequency, such that at 94 GHz, the limitation on transmitting power and the combined transmission and reception losses (greater than 5 dB) in a waveguide transmission line previously considered for the original application would be unacceptable. The QOTL functions as a very-lowloss, three-port circulator. The QOTL includes a shaped input mirror that can be rotated to accept 94-GHz transmitter power from either of two high-power amplifiers. Inside the QOTL, the transmitter power takes the form of a linearly polarized beam radiated from a feed horn. This beam propagates through a system of mirrors, each of which refocuses the beam to minimize diffraction losses. A magnetically biased ferrite disc is placed at one of the foci to utilize the Faraday effect to rotate the polarization of the beam by 45 degrees. The beam is then transmitted via an antenna system. The radar return (scatter from clouds, and/or reflections from other objects) is collected by the same antenna and propagates through the Faraday rotator in the reverse of the direction of propagation of the transmitted beam. In the Faraday rotator, the polarization of the received signal is rotated a further 45 degrees, so that upon emerging from the Faraday rotator, the received beam is polarized at 90 with respect to the transmitted beam. The transmitted and received signals are then separated by a wire-grid polarizer.

Perez, Raul M.↗

NASA NTRS2015

The Coupled Mars Dust and Water Cycles: Understanding How Clouds Affect the Vertical Distribution and Meridional Transport of Dust and Water.

The dust and water cycles are crucial to the current Martian climate, and they are coupled through cloud formation. Dust strongly impacts the thermal structure of the atmosphere and thus greatly affects atmospheric circulation, while clouds provide radiative forcing and control the hemispheric exchange of water through the modification of the vertical distributions of water and dust. Recent improvements in the quality and sophistication of both observations and climate models allow for a more comprehensive understanding of how the interaction between the dust and water cycles (through cloud formation) affects the dust and water cycles individually. We focus here on the effects of clouds on the vertical distribution of dust and water, and how those vertical distributions control the net meridional transport of water. For this study, we utilize observations of temperature, dust and water ice from the Mars Climate Sounder (MCS) on the Mars Reconnaissance Orbiter (MRO) combined with the NASA ARC Mars Global Climate Model (MGCM). We demonstrate that the magnitude and nature of the net meridional transport of water between the northern and southern hemispheres during NH summer is sensitive to the vertical structure of the simulated aphelion cloud belt. We further examine how clouds influence the atmospheric thermal structure and thus the vertical structure of the cloud belt. Our goal is to identify and understand the importance of radiative/dynamic feedbacks due to the physical processes involved with cloud formation and evolution on the current climate of Mars.

Martian climate↗

NASA NTRS2017

Radiative Impacts of Further Arctic Sea Ice Melt: Using past Observations to Inform Future Climate Impacts

The Arctic region has seen dramatic changes over the past several decades, from polar amplification of global temperature rise to ecosystem changes to the decline of the sea ice. While there has been much speculation as to when the world will see an ice-free Arctic, the radiative impacts of an eventual disappearance of the Arctic sea ice are likely to be significant regardless of the timing. Using CERES radiation and microwave satellite sea ice data, Pistone et al (2014) estimated the radiative forcing due to albedo changes associated with the Arctic sea ice retreat over the 30 years of the satellite data record. In this study, we found that the Arctic Ocean saw a decrease in all-sky albedo of 4% (from 52% to 48%), for an estimated increase in solar heating of 6.4 W/m(exp 2) between 1979 and 2011, or 0.21 W/m(exp 2) when averaged over the globe. This value is substantial--approximately 25% as large as the forcing due to the change in CO2 during the same period. Here we update and expand upon this previous work and use the CERES broadband shortwave observations to explore the radiative impacts of a transition to completely ice-free Arctic Ocean. We estimate the annually-averaged Arctic Ocean planetary albedo under ice-free and cloud-free conditions to be 14% over the region, or approximately 25% lower in absolute terms than the Arctic Ocean cloud-free albedo in 1979. However, the question of all-sky conditions (i.e. including the effects of clouds) introduces a new level of complexity. We explore several cloud scenarios and the resultant impact on albedo. In each of these cases, the estimated forcing is not uniformly distributed throughout the year. We describe the relative contributions of ice loss by month as well as the spatial distributions of the resulting changes in absorbed solar energy. The seasonal timing and location—in addition to magnitude—of the altered solar absorption may have significant implications for atmospheric and ocean dynamics in the Arctic and at lower latitudes; this observationally-based estimate of the large-scale characteristics of an ice-free Arctic thus provides a valuable tool to complement and validate model-based assessments of future climate.

Pistone, K.↗

NASA NTRS2018

NASA's Black Marble Nighttime Lights Product Suite

NASA's Black Marble nighttime lights product suite (VNP46) is available at 500 meters resolution since January 2012 with data from the Visible Infrared Imaging Radiometer Suite (VIIRS) Day/Night Band (DNB) onboard the Suomi National Polar-orbiting Platform (SNPP). The retrieval algorithm, developed and implemented for routine global processing at NASA's Land Science Investigator-led Processing System (SIPS), utilizes all high-quality, cloud-free, atmospheric-, terrain-, vegetation-, snow-, lunar-, and stray light-corrected radiances to estimate daily nighttime lights (NTL) and other intrinsic surface optical properties. Key algorithm enhancements include: (1) lunar irradiance modeling to resolve non-linear changes in phase and libration; (2) vector radiative transfer and lunar bidirectional surface anisotropic reflectance modeling to correct for atmospheric and BRDF (Bidirectional Reflectance Distribution Function) effects; (3) geometric-optical and canopy radiative transfer modeling to account for seasonal variations in NTL; and (4) temporal gap-filling to reduce persistent data gaps. Extensive benchmark tests at representative spatial and temporal scales were conducted on the VNP46 time series record to characterize the uncertainties stemming from upstream data sources. Initial validation results are presented together with example case studies illustrating the scientific utility of the products. This includes an evaluation of temporal patterns of NTL dynamics associated with urbanization, socioeconomic variability, cultural characteristics, and displaced populations affected by conflict. Current and planned activities under the Group on Earth Observations (GEO) Human Planet Initiative are aimed at evaluating the products at different geographic locations and time periods representing the full range of retrieval conditions.

Suomi-NPP↗

NASA NTRS2017

Accounting for the Effects of Surface BRDF on Satellite Cloud and Trace-Gas Retrievals: A New Approach Based on Geometry-Dependent Lambertian-Equivalent Reflectivity Applied to OMI Algorithms

Most satellite nadir ultraviolet and visible cloud, aerosol, and trace-gas algorithms make use of climatological surface reflectivity databases. For example, cloud and NO2 retrievals for the Ozone Monitoring Instrument (OMI) use monthly gridded surface reflectivity climatologies that do not depend upon the observation geometry. In reality, reflection of incoming direct and diffuse solar light from land or ocean surfaces is sensitive to the sun-sensor geometry. This dependence is described by the bidirectional reflectance distribution function (BRDF). To account for the BRDF, we propose to use a new concept of geometry-dependent Lambertian equivalent reflectivity (LER). Implementation within the existing OMI cloud and NO2 retrieval infrastructure requires changes only to the input surface reflectivity database. The geometry-dependent LER is calculated using a vector radiative transfer model with high spatial resolution BRDF information from the Moderate Resolution Imaging Spectroradiometer (MODIS) over land and the Cox-Munk slope distribution over ocean with a contribution from water-leaving radiance. We compare the geometry-dependent and climatological LERs for two wavelengths, 354 and 466 nm, that are used in OMI cloud algorithms to derive cloud fractions. A detailed comparison of the cloud fractions and pressures derived with climatological and geometry-dependent LERs is carried out. Geometry-dependent LER and corresponding retrieved cloud products are then used as inputs to our OMI NO2 algorithm. We find that replacing the climatological OMI-based LERs with geometry-dependent LERs can increase NO2 vertical columns by up to 50% in highly polluted areas; the differences include both BRDF effects and biases between the MODIS and OMI-based surface reflectance data sets. Only minor changes to NO2 columns (within 5 %) are found over unpolluted and overcast areas.

Lambert-equivalent reflectivity↗

NASA NTRSDate not supplied

Comparison of Observed Longwave, Shortwave Irradiance and Surface Temperature from “MOSAiC” to CERES Radiative Transfer Calculations and Inputs

As atmospheric temperatures rise due to increased anthropogenic forcing, the effect is expected to be larger over the arctic than midlatitude and tropics, known as polar amplification. A multi-national program, the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) was ran between Sept 2019 and Oct 2020. The project deployed scientific instruments on board the German research vessel Polarstern with the ship remaining across a year to observe all aspects of polar climate. The US DOE deployed the ARM AMF2 aboard the ship along with several off-ship sites for extended spatial observations. Of particular importance was the measurement of the energetics of the ice/ocean/atmosphere interactions through observations of surface irradiance and surface temperatures. NASA’s Clouds and the Earth’s Radiant Energy System (CERES) project produces the SYN1deg Edition 4 data product. This product provides high quality, hourly, globally gridded and temporally complete maps of top of atmosphere (TOA), in atmosphere, and surface irradiances. TOA fluxes are derived from CERES instruments and geostationary satellites. In addition, TOA, in atmosphere, and surface irradiances are computed using the Langley Fu and Liou radiative transfer model. The radiative transfer model is run hourly at 1 degree ~equal area spatial resolution. Meteorological profiles are provided by Global Modeling and Assimilation Office’s GEOS-541 reanalysis product. Cloud properties are derived solely from Terra and Aqua MODIS imagers northward of 60°. Here we compare SYN1deg hourly calculations of surface irradiance to observations from the AMF2 to validate the products estimates of surface irradiance in this challenging area. Along with the irradiance comparisons we take a close look at the surface temperature record in the GEOS-541 product and compare it over both time and space to several surface observations provided by MOSAiC. Along with the comparison to the re-analysis record we will compare these observed surface temperatures to those derived from the AIRS product, which is known to have some difficulty in extreme high latitude areas. The goals of this study are 1) understand computed surface downward irradiance and temperature error separated by surface type (e.g. sea ice or open water) and by season, and 2) error covariance in spatial and temporal space. We seek to use this information to extrapolate the error from the MOSAiC domain to a larger arctic region.

David A Rutan↗

NASA NTRS1980

Lunar and Planetary Science Conference, 11th, Houston, TX, March 17-21, 1980, Proceedings. Volume 2 - Meteorite and regolith studies

Topics discussed include studies of chondrites, mesosiderites, and achondrites; isotope modeling; Antarctic weathering; irradiation effects; lunar regolith studies; the Apollo 17 drill core; soils and agglutinates; and volatiles. Particular attention is given to the proportional retention of I and Xe-129 in preheated Allende, olivine clasts from mesosiderites and howardites as clues to the nature of achondritic parent bodies, a record of solar corpuscular radiation in minerals from lunar soils, the experimental shock metamorphism of lunar soil, and the clouding of pyroxene and plagioclase in eucrites.

Merrill, R. B.↗

NASA NTRS1983

A comparison of experimental and theoretical bidirectional reflectance functions

Bidirectional reflectance models developed by radiative transfer theory calculations are compared with empirical models from Nimbus 7 ERB measurements for two cloud altitudes (medium height cloud tops at 3 km and high cloud tops at 9 km). For solar zenith angles less than 60 deg, the models agree to within 10 percent. For larger zenith angles, however, the differences between the models increase rapidly. These differences are attributed to three-dimensional cloud effects and to smearing effects associated with averaging measurements over finite solar zenith angle ranges. It is thus demonstrated, that the theoretical models provide a good description of the radiance fields of clouds as seen by the satellite.

Stuhlmann, R.↗