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At least 1,567 records · Page 87

Dynamic Control of Sodium Cold Trap Purification Temperature Using LSTM System Identification

This study investigates the dynamic regulation of the sodium cold trap purification temperature at Argonne National Laboratory’s liquid sodium test facility, employing long short-term memory (LSTM) system identification techniques. The investigation introduces an innovative hybrid approach by integrating model predictive control (MPC) based on first principles dynamic models with a multi-step time–frequency LSTM model in predicting the temperature profiles of a sodium cold trap purification system. The long short-term memory–model predictive controller (LSTM-MPC) model employs a sliding window scheme to gather training samples for multi-step prediction, leveraging historical data to construct predictive models that capture the non-linearities of the complex system dynamics without explicitly modeling the underlying physical processes. The performance of the LSTM-MPC and MPC were evaluated through simulation experiments, where both models were assessed on their capacity to maintain the cold trap temperature within predefined set-points while minimizing deviations and overshoots. Results obtained show how the data-driven LSTM-MPC model demonstrates stability and adaptability. In contrast, the traditional MPC model exhibits irregularities, particularly evident as overshoots around set-point limits, which can potentially compromise its effectiveness over long prediction time intervals. The findings obtained offer valuable insights into integrating data-driven techniques for enhancing real-time monitoring systems.

LSTM-MPC↗

Structure of Offshore Low-Level Jet Turbulence and Implications to Mesoscale-to-Microscale Coupling

This paper explores realistic nonstationary atmospheric boundary layer (ABL) turbulence arising from nonstationarity at the mesoscale, particularly within offshore low-level jets with implications to offshore wind farms, using high-fidelity multiscale large-eddy simulations (LES). To this end, we analyzed the single-point turbulence statistical structure of a North-Atlantic offshore LLJ event simulated using high-resolution LES (AMR-Wind). The nonstationary LLJ is simulated using a mesoscale-to-microscale coupled (MMC) simulation procedure involving data assimilation of mesoscale velocity and temperature data from the Weather Research and Forecasting (WRF) model. Unlike the assimilation of mesoscale velocity data into the LES, the direct assimilation of temperature profiles had a strong impact on turbulence stratification, thereby causing erroneous predictions of turbulence both above and within the jet layer. Various approaches to mitigate this effect have resulted in multiple (four) variants of this MMC strategy. Outcomes from this work clearly show that the turbulence within the low-level jet is a strong function of the MMC approach as the turbulence structure within the low-level jet is dependent on the flux of residual turbulence from outside the jet, which in turn depends on the temperature forcing history. Additionally, the turbulence predicted by all these different methods (as well as the observation data) show similar deviations from equilibrium as evidenced by comparisons with idealized atmospheric turbulence structure obtained using the same numerical method. In general, we observe that the predicted LLJ turbulence tends to differ from canonical ABL turbulence with comparable shear. Particularly, the combination of shear and turbulence observed in such nonstationary low-level turbulence cannot be matched using equilibrium settings and therefore, represents a critical use-case for both testing and leveraging meso–micro coupling strategies.

17 WIND ENERGY↗

Lidar measurements of polar stratospheric clouds during the 1989 airborne Arctic stratospheric expedition

The Airborne Arctic Stratospheric Expedition (AASE) was conducted during January to February 1989 from the Sola Air Station, Norway. As part of this expedition, the NASA Langley Research Center's multiwavelength airborne lidar system was flown on the NASA Ames Research Center's DC-8 aircraft to measure ozone (O3) and aerosol profiles in the region of the polar vortex. The lidar system simultaneously transmitted laser beams at 1064, 603, 311, and 301.5 nm to measure atmospheric scattering, polarization and O3 profiles. Long range flights were made between Stavanger, Norway, and the North Pole, and between 40 deg W and 20 deg E meridians. Eleven flights were made, each flight lasting an average of 10 hours covering about 8000 km. Atmospheric scattering ratios, aerosol polarizations, and aerosol scattering ratio wavelength dependences were derived from the lidar measurements to altitudes above 27 km. The details of the aerosol scattering properties of lidar observations in the IR, VIS, and UV regions are presented along with correlations with the national meteorological Center's temperature profiles.

Ismail, Syed↗

The challenge in making models of fast CMEs

It has been a challenge to explain theoretically how fast CMEs (exceeding {approx} 1,000km/s) occur. Our numerical models suggest that it is not easy to release enough magnetic energy impulsively from an active region. We have been studying CME models that are constrained by observed magnetic fields, with realistic coronal plasma density and temperature profiles, as derived from thermodynamic models of the corona. We find that to get fast CMEs, the important parameters are the magnetic energy density, the magnetic field drop-off index, and the Alfven speed profile in active regions. We describe how we energize active regions, and how we subsequently initiate CMEs via flux cancellation. We contrast CMEs from idealized zero-beta models with more sophisticated models based on thermodynamic solutions.

79 ASTRONOMY AND ASTROPHYSICS↗

Characterization of Energy Savings and Thermal Comfort Improvements Derived from Using Interior Storm Windows

This field study of a single historic home in Seattle, WA documents the performance of Indow ® Windows’s interior storm window inserts. Energy use and the temperature profile of the house were monitored before and after the installation of the window inserts and changes in the two recorded metrics were examined. Using the defined analysis approach, it was determined that the interior storm windows produced a 22% reduction of the HVAC energy bill and had an undetermined effect on the thermal comfort in the house. Although there was no measurable changes in the thermal comfort of the house, the occupant noted the house to be “warmer in the winter and cooler in the summer” and that the “temperatures are more even (throughout the house).” The interior storm windows were found to be not cost effective, largely due to the retrofits completed on its heating system. However, if the economic analysis was conducted based on the old heating system, a 72% efficient oil fired furnace, the Indow Windows proved to be economical and had a simple payback period of 9.0 years.

high performance housing↗

Visualization of the freeze/thaw characteristics of a copper/water heat pipe - Effects of non-condensible gas

The freeze/thaw characteristics of a copper/water heat pipe of rectangular cross section were investigated experimentally to determine the effect of variations in the amount of non-condensible gases (NCG) present. The transient internal temperature profiles in both the liquid and vapor channels are presented along with contours of the frozen fluid configuration obtained through visual observation. Several interesting phenomena were observed including total blockage of the vapor channel by a solid plug, evaporator dryout during restart, and freezing blowby. In addition, the restart characteristics are shown to be strongly dependent upon the shutdown procedure used prior to freezing, indicating that accurate prediction of the startup or restart characteristics requires a complete thermal history. Finally, the experimental results indicate that the freeze/thaw characteristics of room temperature heat pipes may be significantly different from those occurring in higher temperature, liquid metal heat pipes due to differences in the vapor pressures in the frozen condition.

Ochterbeck, J. M.↗

Experimental and Numerical Characterization of High Heat Fluxes During Transient Blackbody Calibrations

High heat fluxes are encountered in numerous applications, such as hypersonic vehicles in flight, fires, and engines, Calibration of heat flux gages may be performed in a dual cavity cylindrical blackbody resulting in a transient calibration environment. To characterize the transient heat fluxes. experiments were performed on a dual cavity cylindrical blackbody at nominal temperatures varying from 800 C to 1900 C in increments of 100 C. Based on experiments, the optimum heat flux sensor insertion location as measured from the center partition was determined. The pre-insertion steady state axial temperature profile is compared experimentally, numerically, and analytically. The effect of convection in the blackbody cavity during the insertion is calculated and found to be less than 2 per cent. Also, an empirical correlation for predicting the emissivity of the blackbody is included. Detailed transient thermal models have been developed to simulate the heat flux calibration process at two extreme fluxes. The high (1MW/sq m) and relatively low (70 kw/sq m) fluxes are reported in this article. The transient models show the effect of inserting a heat flux gage at room temperature on the thermal equilibrium of the blackbody at 1800 C and 800 C nominal temperatures, respectively. Also, heat flux sensor outputs are derived from computed sensor temperature distributions and compared to experimental results.

Abdelmessih, Amanie N.↗

TEMPERATURE CONSTRAINT OF THE MISTASTIN LAKE IMPACT STRUCTURE IMPACT MELT ROCKS

Impact melt is a product of hypervelocity cratering events formed by the instantaneous melting of near-surface target rocks. The temperatures of impact melt upon formation are believed to be superheated, vastly exceeding the liquidus temperature of igneous rocks formed via endogenic processes. However, quantitative understanding of the formation and duration of superheated temperatures remains incomplete. To date, only one datum on the hottest post-shock temperature (>2370 °C) has been derived by Timms et al. (2017) [1]. These authors studied the microstructures and crystallographic orientations preserved within a rim of vermicular ZrO2 of a zircon grain entrained within impact glass at the Mistastin Lake impact structure, Canada. Diagnostic crystallographic orientation indicated the presence of cubic zirconia, requiring a minimum temperature for the impact melt of >2370°C from the dissociation of zircon to cubic zirconia and liquid SiO2. With only one temperature datum, it cannot be stated whether the temperature of the impact melt sheet was homogenous across the entire structure or if the thermal history of the melt varied with spatial distribution. In this study, we present a preliminary investigation of 70 zircon grains, 22 of which exhibit rims of vermicular ZrO2 dissociation textures, similar to those studied by Timms et al. (2017). To acquire a more accurate temperature profile representative of impact melt, zircon crystals were collected from different types of impact melt bearing units, including additional samples of the impact glass studied by Timms et al. (2017). Of the 22 zircon grains with dissociation textures, at least 4 grains in the impact glass show diagnostic evidence of pre-existing cubic zirconia, and 1 grain from a glass-bearing breccia exhibits granular zircon textures, possible evidence of a transition from high-P to high-T conditions. These results show the heterogeneous post-shock temperature distribution of superheated impact melt within the Mistastin impact structure. [1] Timms, N.E., Erickson, T.M., Zanetti, M.R., Pearce, M.A., Cayron, C., Cavosie, A.J., Reddy, S.M., Wittmann, A. and Carpenter, P.K., 2017. Cubic zirconia in> 2370° C impact melt records Earth's hottest crust. Earth and Planetary Science Letters, 477, pp.52-58.

rock↗

Using Bayesian analysis and Gaussian processes to infer electron temperature and density profiles on the Mega-Ampere Spherical Tokamak experiment

A unified, Bayesian inference of midplane electron temperature and density profiles using both Thomson scattering (TS) and interferometric data is presented. Beyond the Bayesian nature of the analysis, novel features of the inference are the use of a Gaussian process prior to infer a mollification length-scale of inferred profiles and the use of Gauss-Laguerre quadratures to directly calculate the depolarisation term associated with the TS forward model. Results are presented from an application of the method to data from the high resolution TS system on the Mega-Ampere Spherical Tokamak, along with a comparison to profiles coming from the standard analysis carried out on that system.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Integrated Data Analysis to Improve Te and Zeff Measurement on NSTX-U

The multi-energy soft x-ray (ME-SXR) camera is a new concept for a fusion plasma diagnostic based on a pixelated detector with adjustable photon cutoff thresholds. It is a single, compact, solid-state detector which combines spatial and spectral sensitivity and can be configured remotely at run time, making it ideal for a fusion environment. The detector can be configured for application to a wide range of physics problems including impurity transport, electron temperature profiles, and non-thermal effects. The detector has been installed on the Madison Symmetric Torus (MST) as part of a collaboration between Princeton Plasma Physics Laboratory and the University of Wisconsin–Madison to develop the technology and analysis techniques. A full diagnostic forward model of the ME-SXR diagnostic has been developed to enable analysis of the raw photon count data. This model incorporates the atomic physics underlying the plasma emission, diagnostic geometry, and detector response characteristics. Employing this model, a Bayesian analysis approach is used to extract electron temperature from the raw data. This analysis approach uses all available information, clearly quantifies prior information, and handles uncertainties transparently. The ME-SXR camera is being used to study the 3D (helical, stellarator-like) state that forms in the MST device. This helical core structure has improved energy confinement. The transition to the helical state is accompanied by a rise in electron temperature in the central part of the helical structure, but then this enhancement fluctuates. The characteristics of this fluctuation are being compared to a magneto-hydrodynamics model.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Nonaxisymmetric evolution in protostellar disks

We present a two-dimensional, multigridded hydrodynamical simulation of the collapse of an axisymmetric, rotating, 1 solar mass protostellar cloud, which forms a resolved, hydrotastic disk. The code includes the effects of physical viscosity, radiative transfer and radiative acceleration but not magnetic fields. We examine how the disk is affected by the inclusion of turbulent viscosity by comparing a viscous simulation with an inviscid model evolved from the same initial conditions, and we derive a disk evolutionary timescale on the order of 300,000 years if alpha = 0.01. Effects arising from non-axisymmetric gravitational instabilities in the protostellar disk are followed with a three-dimensional SPH code, starting from the two-dimensional structure. We find that the disk is prone to a series of spiral instabilities with primary azimulthal mode number m = 1 and m = 2. The torques induced by these nonaxisymmetric structures elicit material transport of angular momentum and mass through the disk, readjusting the surface density profile toward more stable configurations. We present a series of analyses which characterize both the development and the likely source of the instabilities. We speculate that an evolving disk which maintains a minimum Toomre Q-value approximately 1.4 will have a total evolutionary span of several times 10(exp 5) years, comparable to, but somewhat shorter than the evolutionary timescale resulting from viscous turbulence alone. We compare the evolution resulting from nonaxisymmetric instabilities with solutions of a one-dimensional viscous diffusion equation applied to the initial surface density and temperature profile. We find that an effective alpha-value of 0.03 is a good fit to the results of the simulation. However, the effective alpha will depend on the minimum Q in the disk at the time the instability is activated. We argue that the major fraction of the transport characterized by the value of alpha is due to the action of gravitational torques, and does not arise from inherent viscosity within the smoothed particle hydrodynamics method.

Laughlin, Gregory↗

Relationships among top‐of‐atmosphere radiation and atmospheric state variables in observations and CESM

Abstract A detailed examination is made in both observations and the Community Earth System Model (CESM) of relationships among top‐of‐atmosphere radiation, water vapor, temperatures, and precipitation for 2000–2014 to assess the origins of radiative perturbations and climate feedbacks empirically. The 30‐member large ensemble coupled runs are analyzed along with one run with specified sea surface temperatures for 1994 to 2005 (to avoid volcanic eruptions). The vertical structure of the CESM temperature profile tends to be top heavy in the model, with too much deep convection and not enough lower stratospheric cooling as part of the response to tropospheric heating. There is too much absorbed solar radiation (ASR) over the Southern Oceans and not enough in the tropics, and El Niño–Southern Oscillation (ENSO) is too large in amplitude in this version of the model. However, the covariability of monthly mean anomalies produces remarkably good replication of most of the observed relationships. There is a lot more high‐frequency variability in radiative fluxes than in temperature, highlighting the role of clouds and transient weather systems in the radiation statistics. Over the Warm Pool in the tropical western Pacific and Indian Oceans, where nonlocal effects from the Walker circulation driven by the ENSO events are important, several related biases emerge: in response to high SST anomalies there is more precipitation, water vapor, and cloud and less ASR and outgoing longwave radiation in the model than observed. Different model global mean trends are evident, however, possibly hinting at too much positive cloud feedback in the model.

Trenberth, Kevin E.↗

Data & Code from Phoenix CPPP Phase 2 Analysis

This data and code package supports the analysis presented in “Beyond Surface Cooling: Comprehensive Field Assessment of Reflective Pavement Thermal Performance in Phoenix, Arizona” and provides fully reproducible workflows for evaluating the thermal performance of cool pavement treatments in a hot urban environment. The dataset integrates multi-modal field measurements collected across residential and nonresidential settings, including mobile air temperature traverses, stationary air temperature monitoring, residential mean radiant temperature (MRT) measurements, subsurface temperature profiles, and controlled testbed observations. The data package contains raw and processed datasets in comma-separated value (CSV) format, accompanying metadata files describing site characteristics and measurement protocols, and R scripts (.R files) used for data cleaning, time synchronization, spatial and temporal matching, quality control filtering, statistical comparison, and figure generation. All analyses were conducted using R (version ≥ 4.2.0) with commonly available packages (e.g., tidyverse, lubridate, data.table, ggplot2). No proprietary software is required to reproduce results. Field campaigns were designed to quantify the effects of high-reflectance pavement coatings on surface temperature, near-surface air temperature, subsurface heat propagation, and radiative heat exposure. Temporal alignment procedures include standardized timestamp conversion and nearest-neighbor matching of high-frequency sensor measurements to stop-based metadata within defined tolerance windows to ensure comparability across instruments. The workflows generate summary statistics, treatment–control contrasts, depth-dependent thermal gradients, and time-series visualizations used in the associated publication. By integrating mobile, stationary, radiative, and subsurface measurements within a unified and transparent processing framework, this package enables comprehensive evaluation of cool pavement performance across multiple thermal exposure pathways and supports reuse in future urban heat mitigation and climate resilience studies.

AIR TEMPERATURE↗

Hot streaks and phantom cooling in a turbine rotor passage. II - Combined effects and analytical modelling

Experimental documentation and analytical correlations demonstrating the effects of hot streak accumulation and phantom cooling on turbine rotor airfoil surface temperature are presented. Results are shown which quantify the impact of a nonuniform temperature profile at the entrance of a turbine due to combustor-generated hot and cold streaks, and cooling air discharged from the trailing edge of the upstream stator. Experimental results are shown for a range of controlling variables to identify where streak accumulation and phantom cooling were most likely to be strongest. These variables include streak-to-free stream density ratio, streak injection location, and coolant-to-free stream density and velocity ratios. Experimental results are shown for the combined effects of hot streak and stator coolant on the adiabatic recovery temperature of the rotor.

Roback, Richard J.↗

Endoluminal ultrasound applicators for MR-guided thermal ablation of pancreatic tumors: Preliminary design and evaluation in a porcine pancreas model

Purpose: Endoluminal ultrasound may serve as a minimally invasive option for delivering thermal ablation to pancreatic tumors adjacent to the stomach or duodenum. The objective of this study was to explore the basic feasibility of this treatment strategy through the design, characterization, and evaluation of proof-of-concept endoluminal ultrasound applicators capable of placement in the gastrointestinal (GI) lumen for volumetric pancreas ablation under MR guidance. Methods: Two variants of the endoluminal applicator, each containing a distinct array of two independently powered transducers (10 × 10 mm 3.2 MHz planar; or 8 × 10 × 20 mm radius of curvature 3.3 MHz curvilinear geometries) at the distal end of a meter long flexible catheter assembly, were designed and fabricated. Transducers and circulatory water flow for acoustic coupling and luminal cooling were contained by a low-profile polyester balloon covering the transducer assembly fixture. Each applicator incorporated miniature spiral MR coils and mechanical features (guiding tips and hinges) to facilitate tracking and insertion through the GI tract under MRI guidance. Acoustic characterization of each device was performed using radiation force balance and hydrophone measurements. Device delivery into the upper GI tract, adjacent to the pancreas, and heating characteristics for treatment of pancreatic tissue were evaluated in MR-guided ex vivo and in vivo porcine experiments. MR guidance was utilized for anatomical target identification, tracking/positioning of the applicator, and MR temperature imaging (MRTI) for PRF-based multislice thermometry, implemented in the real-time RTHawk software environment. Results: Force balance and hydrophone measurements indicated efficiencies of 48.8% and 47.8% and −3 dB intensity beam-widths of 3.2 and 1.2 mm for the planar and curvilinear transducers, respectively. Ex vivo studies on whole-porcine carcasses revealed capabilities of producing ablative temperature rise (ΔT > 15 °C) contours in pancreatic tissue 4–40 mm long and 4–28 mm wide for the planar transducer applicator (1–13 min sonication duration, ∼4 W/cm{sup 2} applied acoustic intensity). Curvilinear transducers produced more selective heating, with a narrower ΔT > 15 °C contour length and width of up to 1–24 mm and 2–7 mm, respectively (1–7 min sonication duration, ∼4 W/cm{sup 2} applied acoustic intensity). Active tracking of the miniature spiral coils was achieved using a Hadamard encoding tracking sequence, enabling real-time determination of each coil’s coordinates and automated prescription of imaging planes for thermometry. In vivo MRTI-guided heating trials in three pigs demonstrated capability of ∼20 °C temperature elevation in pancreatic tissue at 2 cm depths from the applicator, with 5–7 W/cm{sup 2} applied intensity and 6–16 min sonication duration. Dimensions of thermal lesions in the pancreas ranged from 12 to 28 mm, 3 to 10 mm, and 5 to 10 mm in length, width, and depth, respectively, as verified through histological analysis of tissue sections. Multiple-baseline reconstruction and respiratory-gated acquisition were demonstrated to be effective strategies in suppressing motion artifacts for clear evolution of temperature profiles during MRTI in the in vivo studies. Conclusions: This study demonstrates the technical feasibility of generating volumetric ablation in pancreatic tissue using endoluminal ultrasound applicators positioned in the stomach lumen. MR guidance facilitates target identification, device tracking/positioning, and treatment monitoring through real-time multislice PRF-based thermometry.

60 APPLIED LIFE SCIENCES↗

Parametric Modeling and Economic Analysis of a 2MW th 3-Stream sCO 2 Heat Exchanger

Here, this paper presents the design and cost optimization of a novel 2MW th 3-stream sCO2 plate-fin heat exchanger. This heat exchanger design is unique in that it uses reduced metal oxide particle-to-sCO2 heat exchanger for cost-effective energy storage applications. The design uses low velocity, laminar air as the re-oxidizing reactant to transfer the heat of the re-oxidizing reaction to a sCO2 power loop. The design of the heat exchanger is based on a 2-D, 3-fluid plate/fin heat transfer model. The model parameterizes the size, shape, and number of passages of the heat exchanger to calculate the temperature profile, pressure drop, and fluid velocities of all three fluids. Global heat exchanger parameters such as the effectiveness and total heat transferred to the sCO2 are then calculated for overall performance. Due to the value and increased use of sCO2 heat exchangers in power cycles, a cost model of the system based on the unique high temperature/high pressure operating conditions was created using quotes from reference projects and market analysis. These quoted air-to-sCO2 heat exchangers are then processed using multiple weighting factors pertinent to heat exchanger design, including heat exchanger type, maximum temperature, differential pressures, fluids, duty, and more. These factors are then used in an exponential function in order to generate a parameterized cost curve. The design and cost of the heat exchanger are then optimized using the SMPSO genetic algorithm in Python. The optimization objectives for the system are to maximize the overall system effectiveness, including an air recuperator for preheating, and to minimize unit costs. Additional constraints are added to the system for the sCO2 and air pressure drops, air velocity to reduce particle entrainment, and the length and volume of the heat exchanger.

Cost Model↗

RP-1 and JP-8 Thermal Stability Experiments

This work experimentally investigates the effect of fuel composition changes on jet and rocket fuel thermal stability. A High Reynolds Number Thermal Stability test device evaluated JP-8 and RP-1 fuels. The experiment consisted of an electrically heated, stainless steel capillary tube with a controlled fuel outlet temperature. An optical pyrometer monitored the increasing external temperature profiles of the capillary tube as deposits build inside during each test. Multiple runs of each fuel composition provided results on measurement repeatability. Testing a t two different facilities provided data on measurement reproducibility. The technique is able to distinguish between thermally stable and unstable compositions of JP-8 and intermediate blends made by combining each composition. The technique is also able to distinguish among standard RP-1 rocket fuels and those having reduced sulfur levels. Carbon burn off analysis of residue in the capillary tubes on the RP-1 fuels correlates with the external temperature results.

Brown, Sarah P.↗

Validation of IASI Satellite Ammonia Observations at the Pixel Scale Using In Situ Vertical Profiles

Satellite ammonia (NH 3 ) observations provide unprecedented insights into NH3 emissions, spatiotemporal variabilities and trends, but validation with in situ measurements remains lacking. Here, total columns from the Infrared Atmospheric Sounding Interferometer (IASI) were intercompared to boundary layer NH 3 profiles derived from aircraft- and surface-based measurements primarily in Colorado, USA, in the summer of 2014. IASI-NH 3 version 3 near real-time data set compared well to in situ derived columns (windows ±15 km around centroid, ±1 h around overpass time) with a correlation of 0.58, a slope of 0.78 ± 0.14 and an intercept of 2.1 × 10 15 ±1.5 × 10 15 molecules cm −2 . Agreement degrades at larger spatiotemporal windows, consistent with the short atmospheric lifetime of NH 3 . We also examined IASI version 3R data, which relies on temperature retrievals from the ERA Reanalysis, and a third product generated using aircraft-measured temperature profiles. The overall agreement improves slightly for both cases, and neither is biased within their combined measurement errors. Thus, spatiotemporal averaging of IASI over large windows can be used to reduce retrieval noise. Nonetheless, sampling artifacts of airborne NH 3 instruments result in significant uncertainties of the in situ-derived columns. For example, large validation differences exist between ascent and descent profiles, and the assumptions of the free tropospheric NH 3 profiles used above the aircraft ceiling significantly impact the validation. Because short-lived species like NH 3 largely reside within the boundary layer with complex vertical structures, more comprehensive validation is needed across a wide range of environments. More accurate and widespread in situ NH 3 data sets are therefore required for improved validations of satellite products.

Ammonia↗