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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,567 records · Page 87
All sourcesNASA NTRSDOE OSTI
DOE OSTI2015

Correlation of anisotropy and directional conduction in β-Li{sub 3}PS{sub 4} fast Li{sup +} conductor

This letter reports the correlation of anisotropy and directional conduction in the fast Li{sup +} conductor β-Li{sub 3}PS{sub 4}, one of the low-symmetry crystalline electrolyte candidates. The material has both high conductivity and good stability that serves well for the large-scale energy storage applications of all-solid-state lithium ion batteries. The anisotropic physical properties, demonstrated here by the thermal expansion coefficients, are crucial for compatibility in the solid-state system and battery performance. Neutron and X-ray powder diffraction measurements were done to determine the crystal structure and thermal stability. The crystallographic b-axis was revealed as a fast expansion direction, while negligible thermal expansion was observed along the a-axis around the battery operating temperatures. The anisotropic behavior has its structural origin from the Li{sup +} conduction channels with incomplete Li occupancy and a flexible connection of LiS{sub 4} and PS{sub 4} tetrahedra within the framework. This indicates a strong correlation in the direction of the ionic transport in the low-symmetry Li{sup +} conductor.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2012

Optimizing moderation of He-3 neutron detectors for shielded fission sources

Abstract: The response of 3-He neutron detectors is highly dependent on the amount of moderator incorporated into the detector system. If there is too little moderation, neutrons will not react with the 3-He. If there is too much moderation, neutrons will not reach the 3-He. In applications for portal or border monitors where 3He detectors are used to interdict illicit Importation of plutonium, the fission source is always shielded to some extent. Since the energy distribution of neutrons emitted from the source depends on the amount and type of shielding present, the optimum placement of moderating material around 3-He tubes is a function of shielding. In this paper, we use Monte Carlo techniques to model the response of 3-He tubes placed in polyethylene boxes for moderation. To model the shielded fission neutron source, we use a 252-Cf source placed in the center of spheres of water of varying radius. Detector efficiency as a function of box geometry and shielding are explored. We find that increasing the amount of moderator behind and to the sides of the detector generally improves the detector response, but that benefits are limited if the thickness of the polyethylene moderator is greater than about 5-7 cm. The thickness of the moderator in front of the 3He tubes, however, is very important. For bare sources, about 5-6 cm of moderator is optimum, but as the shielding increases, the optimum thickness of this moderator decreases to 0-1 cm. A two-tube box with a moderator thickness of 5 cm in front of the first tube and a thickness of 1 cm in front of the second tube is proposed to improve the detector's sensitivity to lower-energy neutrons.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Bimodal Long-lasting Components in Short Gamma-Ray Bursts: Promising Electromagnetic Counterparts to Neutron Star Binary Mergers

Long-lasting emission of short gamma-ray bursts (GRBs) is crucial to reveal the physical origin of the central engine as well as to detect electromagnetic (EM) counterparts to gravitational waves (GWs) from neutron star binary mergers. We investigate 65 X-ray light curves of short GRBs, which is six times more than previous studies, by combining both Swift /BAT and XRT data. The light curves are found to consist of two distinct components at >5 σ with bimodal distributions of luminosity and duration, i.e., extended (with a timescale of ≲10{sup 3} s) and plateau emission (with a timescale of ≳10{sup 3} s), which are likely the central engine activities, but not afterglows. The extended emission has an isotropic energy comparable to the prompt emission, while the plateau emission has ∼0.01–1 times this energy. Half (50%) of our sample has both components, while the other half is consistent with having both components. This leads us to conjecture that almost all short GRBs have both the extended and plateau emission. The long-lasting emission can be explained by the jets from black holes with fallback ejecta, and could power macronovae (or kilonovae) like GRB 130603B and GRB 160821B. Based on the observed properties, we quantify the detectability of EM counterparts to GWs, including the plateau emission scattered to the off-axis angle, with CALET /HXM, INTEGRAL /SPI-ACS, Fermi /GBM, MAXI /GSC, Swift /BAT, XRT, the future ISS-Lobster /WFI, Einstein Probe /WXT, and eROSITA .

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Constraints on the Muon Fraction and Density Profile in Neutron Stars

Muons in neutron stars (NSs) play especially important roles in addressing several interesting new physics questions associated with detecting as well as understanding interactions and astrophysical effects of muonphilic dark matter particles. The key model inputs for studying the latter are the total muon mass M μ , the muon mass fraction M μ /M NS over the NS mass M NS , and the muon radial density profile ρ μ (r) in NSs of varying masses. We investigate these quantities within a minimum model for the core of NSs consisting of neutrons, protons, electrons, and muons using an explicitly isospin-dependent parametric equation of state (EOS) constrained by available nuclear laboratory experiments and the latest astrophysical observations of NS masses, radii, and tidal deformabilities. Here, we found that the absolutely maximum muon mass M μ and its mass fraction M μ /M NS in the most massive NSs allowed by causality are about 0.025 M ⊙ and 1.1%, respectively. For the most massive NS of mass 2.14 M ⊙ observed so far, they reduce to about 0.020 M ⊙ and 0.9%, respectively. We also study respective effects of individual parameters describing the EOS of high-density neutron-rich nucleonic matter on the muon contents in NSs with varying masses. We found that the most important but uncertain nuclear physics ingredient for determining the muon contents in NSs is the high-density nuclear symmetry energy.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Polychromatic diffraction contrast tomography

This tutorial review introduces the use of polychromatic radiation for 3D grain mapping using X-ray diffraction contrast tomography. The objective is to produce a 3D map of the grain shapes and orientations within a bulk, millimeter-sized polycrystalline sample. The use of polychromatic radiation enables the standard synchrotron X-ray technique to be applied in a wider range of contexts: 1) Using laboratory X-ray sources allows a much wider application of the diffraction contrast tomography technique. 2) Neutron sources allow large samples, or samples containing high Z elements to be studied. 3) Applied to synchrotron sources, smaller samples may be treated, or faster measurements may be possible. Challenges and particularities in the data acquisition and processing, and the limitations of the different variants, are discussed. - Highlights: • We present a tutorial review of polychromatic diffraction contrast tomography techniques. • The use of polychromatic radiation allows the standard synchrotron DCT technique to be extended to a range of other sources. • The characteristics and limitations of all variants of the techniques are derived, discussed and compared. • Examples using laboratory X-ray and cold neutron radiation are presented. • Suggestions for the future development of these techniques are presented.

36 MATERIALS SCIENCE↗
DOE OSTI2016

The Need for Precise and Well-documented Experimental Data on Prompt Fission Neutron Spectra from Neutron-induced Fission of {sup 239}Pu

The spectrum of neutrons emitted promptly after {sup 239}Pu(n,f)—a so-called prompt fission neutron spectrum (PFNS)—is a quantity of high interest, for instance, for reactor physics and global security. However, there are only few experimental data sets available that are suitable for evaluations. In addition, some of those data sets differ by more than their 1-σ uncertainty boundaries. We present the results of MCNP studies indicating that these differences are partly caused by underestimated multiple scattering contributions, over-corrected background, and inconsistent deconvolution methods. A detailed uncertainty quantification for suitable experimental data was undertaken including these effects, and test-evaluations were performed with the improved uncertainty information. The test-evaluations illustrate that the inadequately estimated effects and detailed uncertainty quantification have an impact on the evaluated PFNS and associated uncertainties as well as the neutron multiplicity of selected critical assemblies. A summary of data and documentation needs to improve the quality of the experimental database is provided based on the results of simulations and test-evaluations. Given the possibly substantial distortion of the PFNS by multiple scattering and background effects, special care should be taken to reduce these effects in future measurements, e.g., by measuring the {sup 239}Pu PFNS as a ratio to either the {sup 235}U or {sup 252}Cf PFNS.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Dirac Magnons, Nodal Lines, and Nodal Plane in Elemental Gadolinium

In this report we investigate the magnetic excitations of elemental gadolinium (Gd) using inelastic neutron scattering, showing that Gd is a Dirac magnon material with nodal lines at K and nodal planes at half integer ℓ. We find an anisotropic intensity winding around the K-point Dirac magnon cone, which is interpreted to indicate Berry phase physics. Using linear spin wave theory calculations, we show the nodal lines have nontrivial Berry phases, and topological surface modes. We also discuss the origin of the nodal plane in terms of a screw-axis symmetry, and introduce a topological invariant characterizing its presence and effect on the scattering intensity. Together, these results indicate a highly nontrivial topology, which is generic to hexagonal close packed ferromagnets. We discuss potential implications for other such systems.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Impact of the equation of state on f - and p - mode oscillations of neutron stars

We investigate the impact of the neutron-star matter equation of state on the f- and p1-mode oscillations of neutron stars obtained within the Cowling approximation and linearized general relativity. The f- and p 1 -mode oscillation frequencies, and their damping times are calculated using representative sets of Skyrme Hartree-Fock and relativistic mean-field models, all of which reproduce nuclear systematics and support 2M ⊙ neutron stars. Our study shows strong correlations between the frequencies of f- and p 1 -modes and their damping times with the pressure of β-equilibrated matter at densities equal to or slightly higher than the nuclear saturation density ρ 0 . Such correlations are found to be almost independent of the composition of the stars. The frequency of the p 1 -mode of 1.4M ⊙ star is strongly correlated with the slope of the symmetry energy L 0 and β-equilibrated pressure at density ρ 0 . Compared to GR calculations, the error in the Cowling approximation for the f-mode is about 30% for neutron stars of low mass, whereas it decreases with increasing mass. Here, the accuracy of the p 1 -mode is better than 15% for neutron stars of maximum mass, and improves for lower masses and higher number of radial nodes. I.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

Core Combination Method of Approximation (CCMA) for Neutron Fluence Calculation

Neutron fluence, or accumulative neutron fluence rate, is a key parameter of the neutron irradiation resistance of materials (Wagner, Bergner et al. 2016). So we must try to obtain it during irradiation experiments. Neutron fluence is defined as the time integral of neutron fluence rate. To get the quantity, or to do this integral, we need to know how neutron fluence rate varied with time. The integral might not be difficult when we conduct a material irradiation experiment, because we can put certain kind of neutron detectors in the location of species, to measure neutron fluence rate (Tanaka, Endo et al. 2011). At this circumstance, the reactor power is usually maintained to be constant (Ferroukhi, Hollard et al. 2009; Dupre, Vasiliev et al. 2015). So the neutron fluence is equal to the product of neutron fluence rate and irradiation time. However, it's not the same case when we want to get the neutron fluence of structure materials used in the SPRR- 300 (Swimming Pool Research Reactor -300). This reactor is a light-water-moderated, enriched-uranium-fueled research reactor developed by China. Structural materials, such as graphite, are of great value for research (Asamoah, Gyampo et al. 2012). Graphite was used as reflector in reactor. It is a waste of material and a waste of money to dismantle it simply. However, to reuse post-irradiation graphite assemblies faces some challenges, such as neutron fluence calculation, radiation protection, etc. The former will be discussed in this paper, whereas the latter will remain to be studied for the following time. The problem is how to acquire neutron fluence distribution in structure materials, since specific measurement of neutron fluence rate were not conducted intentionally during historical reactor operation. So we need to figure it out by a method of calculation. Considering a large number of reactor refueling, we propose an approximate method, Core Combination Method of Approximation (CCMA), to calculate accumulative neutron fluence rate of key structure materials during a long period of irradiation time.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2025

Applications of quantum materials in nuclear physics experiments (Final Report)

The goals of this project are to search for hypothesized spin-hall effects of neutrons and variants of neutron-electron hybrid spin hall effects in quantum materials with strong spin-orbit-coupling (SOC) – such as: • Deflection of neutrons dependent on spin (polarization) states (a); • Electrical current induced electron spin polarization or (dynamically polarized) nuclear spin polarization (as suggested in PI’s prior work) may affect polarization states of transmitted or reflected neutron beam • Spin polarized neutrons transfer some spin angular momenta to electrons, which get converted to electronic charge voltage via electronic inverse spin Hall effect (b), which if realized, offers an electrical method to detect neutron spins.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2012

Simulation of Photon energy Spectra Using MISC, SOURCES, MCNP and GADRAS

The detector response functions included in the Gamma Detector Response and Analysis Software (GADRAS) are a valuable resource for simulating radioactive source emission spectra. Application of these response functions to the results of three-dimensional transport calculations is a useful modeling capability. Using a 26.2 kg shell of depleted uranium (DU) as a simple test problem, this work illustrates a method for manipulating current tally results from MCNP into the GAM file format necessary for a practical link to GADRAS detector response functions. MISC (MCNP Intrinsic Source Constructor) and SOURCES 4C were used to develop photon and neutron source terms for subsequent MCNP transport, and the resultant spectrum is shown to be in good agreement with that from GADRAS. A 1 kg DU sphere was also modeled with the method described here and showed similarly encouraging results.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2017

Design Parameter Space for a High Pressure Optimized Dense Plasma Focus Operating with Deuterium

The potential of the Dense Plasma Focus (DPF) for industrial applications in many fields is well recognized, although yet to be realized in practice. Particularly attractive is the possibility of its use as inexpensive industrial source of nuclear reactions for diverse high value applications such as fast pulsed neutron radiography of hydrogenous materials, non-intrusive neutron interrogation of concealed organic contraband and rapid production of short lived radioisotopes for medical diagnostics and therapy. Recently, it has been suggested that it may be possible to operate the DPF efficiently in a High-Pressure-Optimized (HPO) mode. This paper explores the design parameter space for such HPO-DPF based on the revised Resistive Gratton-Vargas (RGV) model with a view to identify a practicable set of system parameters and their scaling. The current waveform predicted by the revised RGV model for the chosen set of parameters is fitted to the Lee model to estimate the likely neutron yield.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2018

Exotic atoms at extremely high magnetic fields: the case of neutron star atmosphere

The presence of exotic states of matter in neutron stars (NSs) is currently an open issue in physics. The appearance of muons, kaons, hyperons, and other exotic particles in the inner regions of the NS, favoured by energetic considerations, is considered to be an effective mechanism to soften the equation of state (EoS). In the so-called two-families scenario, the softening of the EoS allows for NSs characterized by very small radii, which become unstable and convert into a quark stars (QSs). In the process of conversion of a NS into a QS material can be ablated by neutrinos from the surface of the star. Not only neutron-rich nuclei, but also more exotic material, such as hypernuclei or deconfined quarks, could be ejected into the atmosphere. In the NS atmosphere, atoms like H, He, and C should exist, and attempts to model the NS thermal emission taking into account their presence, with spectra modified by the extreme magnetic fields, have been done. However, exotic atoms, like muonic hydrogen (p μ - ) or the so-called Sigmium (Σ + e - ), could also be present during the conversion process or in its immediate aftermath. At present, analytical expressions of the wave functions and eigenvalues for these atoms have been calculated only for H. In this work, we extend the existing solutions and parametrizations to the exotic atoms (p μ - ) and (Σ + e - ), making some predictions on possible transitions. Their detection in the spectra of NS would provide experimental evidence for the existence of hyperons in the interior of these stars.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

Benchmarking ENDF/B-VII.1, JENDL-4.0 and JEFF-3.1.1 with MCNP6

Recent releases of three major world nuclear reaction data libraries, ENDF/B-VII.1, JENDL-4.0, and JEFF-3.1.1, have been tested extensively using benchmark calculations. The calculations were performed with the latest release of the continuous energy Monte Carlo neutronics code MCNP, i.e. MCNP6. Three types of benchmarks were used, viz. criticality safety benchmarks, (fusion) shielding benchmarks, and reference systems for which the effective delayed neutron fraction is reported. For criticality safety, more than 2000 benchmarks from the International Handbook of Criticality Safety Benchmark Experiments were used. Benchmarks from all categories were used, ranging from low-enriched uranium, compound fuel, thermal spectrum ones (LEU-COMP-THERM), to mixed uranium-plutonium, metallic fuel, fast spectrum ones (MIX-MET-FAST). For fusion shielding many benchmarks were based on IAEA specifications for the Oktavian experiments (for Al, Co, Cr, Cu, LiF, Mn, Mo, Si, Ti, W, Zr), Fusion Neutronics Source in Japan (for Be, C, N, O, Fe, Pb), and Pulsed Sphere experiments at Lawrence Livermore National Laboratory (for {sup 6}Li, {sup 7}Li, Be, C, N, O, Mg, Al, Ti, Fe, Pb, D2O, H2O, concrete, polyethylene and teflon). The new functionality in MCNP6 to calculate the effective delayed neutron fraction was tested by comparison with more than thirty measurements in widely varying systems. Among these were measurements in the Tank Critical Assembly (TCA in Japan) and IPEN/MB-01 (Brazil), both with a thermal spectrum, two cores in Masurca (France) and three cores in the Fast Critical Assembly (FCA, Japan), all with fast spectra. The performance of the three libraries, in combination with MCNP6, is shown to be good. The results for the LEU-COMP-THERM category are on average very close to the benchmark value. Also for most other categories the results are satisfactory. Deviations from the benchmark values do occur in certain benchmark series, or in isolated cases within benchmark series. Such instances can often be related to nuclear data for specific non-fissile elements, such as C, Fe, or Gd. Indications are that the intermediate and mixed spectrum cases are less well described. The results for the shielding benchmarks are generally good, with very similar results for the three libraries in the majority of cases. Nevertheless there are, in certain cases, strong deviations between calculated and benchmark values, such as for Co and Mg. Also, the results show discrepancies at certain energies or angles for e.g. C, N, O, Mo, and W. The functionality of MCNP6 to calculate the effective delayed neutron fraction yields very good results for all three libraries.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Incommensurate Spiral Spin Order in CaMn 2 Bi 2 Observed via High-Pressure Neutron Diffraction

Here, high-pressure neutron diffraction is employed to investigate the magnetic behavior of CaMn 2 Bi 2 in extreme conditions. In contrast to antiferromagnetic ordering on Mn atoms reported at ambient pressure, our results reveal that at high pressure, incommensurate spiral spin order emerges due to the interplay between magnetism on the Mn atoms and strong spin–orbit coupling on the Bi atoms: sinusoidal spin order is observed at pressures as high as 7.4 GPa. First-principles calculations with a noncollinear spin orientation demonstrate band crossing behavior near the Fermi level as a result of strong hybridization between the d orbitals of Mn and the p orbitals of Bi atoms. Competing antiferromagnetic order is observed at different temperatures in the partially frustrated lattice. Theoretical models have been developed to investigate spin dynamics. This research provides a unique toolbox for conducting experimental and theoretical magnetic and spin dynamics studies of magnetic quantum materials via high-pressure neutron diffraction.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Collision Tracking in OpenMC: Methods and Applications in Neutron Noise, Neutron Imaging, Time-of-Flight, and Multiplicity Counting

We present the development and application of a collision tracking feature within the OpenMC Monte Carlo particle transport code, designed for diverse applications such as neutron spectroscopy, scatter camera system, neutron noise, and multiplicity counting simulations. This feature enables the tracking of individual particle collisions, with potential applications in nuclear nonproliferation, reactor physics, and nuclear security. Additionally, the feature holds potential for the calibration of neutron detectors, specifically in converting light output into energy deposited within the detectors. The implementation consists of a set of filters—such as reaction type, energy, cell, and material—that constrain the set of collisions that are tracked, extensions to the Python API to enable simple input specification, and support for writing either OpenMC’s native HDF5-based format or the Monte Carlo particle list format. This feature was added to the official OpenMC release in version 0.15.3. In this work, the feature will be applied to showcase scenarios such as time-of-flight simulations, scatter-camera imaging for neutron source localization, neutron-noise analysis to extract integral kinetic parameters such as the prompt decay constant α, and multiplicity counting to estimate the mass of special nuclear materials. Ultimately, this feature aims to expand the application scope of open-source Monte Carlo particle transport codes such as OpenMC.

Monte Carlo code↗