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DOE OSTI2021

Beam Envelope Stability in an Advanced Linear Induction Accelerator

A new linear induction accelerator (LIA) is under development for multipulse flash radiography. Because it has substantially more cells than present LIAs, higher magnetic focusing fields are needed to suppress beam breakup (BBU). It is, therefore, more susceptible to the parametric beam envelope instability (PEI), which has an instability threshold that has usually been typified by the vacuum phase advance per cell exceeding some large fraction of π . Here we derive a threshold criterion for PEI that depends not only on the magnetic field, but also on the beam space charge and emittance. A tune designed to suppress BBU in Scorpius is shown to be stable to the PEI according to this criterion, and also by the lack of emittance growth in particle-in-cell (PIC) code simulations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2023

Scalar dark matter vortex stabilization with black holes

Galaxies and their dark-matter halos are commonly presupposed to spin. But it is an open question how this spin manifests in halos and soliton cores made of scalar dark matter (SDM, including fuzzy/wave/ultralight-axion dark matter). One way spin could manifest in a necessarily irrotational SDM velocity field is with a vortex. But recent results have cast doubt on this scenario, finding that vortices are generally unstable except with substantial repulsive self-interaction. Here, in this paper, we introduce an alternative route to stability: in both (non-relativistic) analytic calculations and simulations, a black hole or other central mass at least as massive as a soliton can stabilize a vortex within it. This conclusion may also apply to AU-scale halos bound to the sun and stellar-mass-scale Bose stars.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2024

Low-Level Liquid-Bearing Clouds Contribute to Seasonal Lower Atmosphere Stability and Surface Energy Forcing over a High-Mountain Watershed Environment

Measurements of atmospheric structure and surface energy budgets distributed along a high-altitude moun tain watershed environment near Crested Butte, Colorado, from two separate, but coordinated, field campaigns, Surface Atmosphere Integrated field Laboratory (SAIL) and Study of Precipitation, the Lower Atmosphere, and Surface for Hydrometeorology (SPLASH), are analyzed. This study identifies similarities and differences in how clouds influence the radiative budget over one snow-free summer season (2022) and two snow-covered seasons (2021/22; 2022/23) for this alpine location. A relationship between lower-tropospheric stability stratification and longwave radiative flux from the presence or absence of clouds is identified. When low clouds persisted, often with signatures of supercooled liquid in win ter, the lower troposphere experienced weaker stability, while radiatively clear skies that are less likely to be influenced by liquid droplets were associated with appreciably stronger lower-tropospheric stratification. Corresponding surface turbu lent heat fluxes partitioned differently based upon the cloud–stability stratification regime derived from early morning radiosounding profiles. Combined with the differences in the radiative budget largely resulting from dramatic seasonal dif ferences in surface albedo, the lower atmosphere stratification, surface energy budget, and near-surface thermodynamics are shown to be modified by the effective longwave radiative forcing of clouds. The diurnal evolution of thermodynamics and surface energy components varied depending on the early morning stratification state. Thus, the importance of quies cent versus synoptically active large-scale meteorology is hypothesized as a critical forcing for cloud properties and associ ated surface energy budget variations. The physical relationships between clouds, radiation, and stratification can provide a useful suite of metrics for process understanding and to evaluate numerical models in such an undersampled, highly com plex terrain environment.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1986

Impact of turbulence modeling on numerical accuracy and efficiency of compressible flow simulations

Discussed is the numerical implementation of turbulence models used in viscous compressible flow simulations and their performance described with respect to numerical accuracy, efficiency and stability. The basic approach utilizes the Reynolds-averaged compressible Navier-Stokes equations in which the Reynolds stresses and heat fluxes are mathematically modeled by suitable turbulence models. The turbulence models investigated include zero-, one-, and two-equation eddy viscosity models. The flow fields investigated include theoretical and supersonic flows about two-dimensional and axisymmetric bodies. Discussions concerning the numerical implementation of models include differencing procedures and boundary conditions used to assume numerical stability and accuracy. Numerical performance is also evaluated by comparing computations with experimental results.

Coakley, Thomas J.↗

DOE OSTI2023

Measuring qubit stability in a gate-based NISQ hardware processor

Some of the most problematic issues that limit the implementation of applications on Noisy Intermediate Scale Quantum (NISQ) machines are the adverse impacts of both incoherent and coherent errors. We conducted an in-depth study of coherent errors on a quantum hardware platform using a transverse field Ising model Hamiltonian as a sample user application. We report here on the results from these computations using several error mitigation protocols that profile these errors and provide an indication of the hardware qubit stability. Through a detailed set of measurements we identify inter-day and intra-day qubit calibration drift and the impacts of quantum circuit placement on groups of qubits in different physical locations on the processor. This paper also discusses how these measurements can provide a better understanding of these types of errors and how they may improve efforts to validate the accuracy of quantum computations.

Yeter-Aydeniz, Kübra↗

DOE OSTI2021

Migration of inclusions in a matrix due to a spatially varying interface energy

An interfacial energy can be a function of a bulk field such as temperature or electric field. Here we find that in a system with a gradient in temperature or electric potential, the resulting variation in interfacial energy can induce a particle to migrate by either surface or bulk diffusion. For a circular particle under a constant unidirectional gradient in the bulk field, the field dependence of the interfacial energy induces a circular particle to move as a circle at a constant velocity along the direction from higher to lower interfacial energy. A linear stability analysis of this steady state migration suggests that perturbations will damp out as time evolves, and thus under these conditions a migrating circular particle is morphologically stable. Other spatial distributions of interface energy can lead to the distortion of an initially circular shaped particle during migration. A phase field model is developed that captures these distortions and verifies the theoretical results mentioned above.

36 MATERIALS SCIENCE↗

DOE OSTI2023

Resonant interactions involving local vibrational modes in crystals

When an impurity with a light mass is inserted into a crystal, it can undergo a high-frequency oscillation referred to as a local vibrational mode (LVM). A Fermi resonance may occur between the LVM and lower-frequency modes of the defect. The LVM may also interact with phonons or the electromagnetic field. Understanding these interactions can help model and control diffusion, defect reactions, and thermal conductivity. LVMs have been probed in semiconductors using pressure and alloying as experimental parameters, resulting in anticrossing between localized and extended vibrational modes. Furthermore, these types of vibrational interactions could play an important role in the stability and thermal properties of organic–inorganic hybrid semiconductors. The coupling between an LVM and electromagnetic wave yields an “LVM polariton,” an excitation that has significant vibrational and electric-field amplitudes.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

NASA NTRS1975

A theoretical evaluation of rigid baffles in suppression of combustion instability

An analytical technique for the prediction of the effects of rigid baffles on the stability of liquid propellant combustors is presented. This analysis employs both two and three dimensional combustor models characterized by concentrated combustion sources at the chamber injector and a constant Mach number nozzle. An eigenfunction-matching method is used to solve the linearized partial differential equations describing the unsteady flow field for both models. Boundary layer corrections to this unsteady flow are used in a mechanical energy dissipation model to evaluate viscous and turbulence effects within the flow. An integral stability relationship is then employed to predict the decay rate of the oscillations. Results of this analysis agree qualitatively with experimental observations and show that sufficient dissipation exists to indicate that the proper mechanism of baffle damping is a fluid dynamic loss.

Combustion instability↗

DOE OSTI2022

Multiplicative Shot-Noise: A New Route to Stability of Plastic Networks

Fluctuations of synaptic weights, among many other physical, biological, and ecological quantities, are driven by coincident events of two “parent” processes. Here we propose a multiplicative shot-noise model that can capture the behaviors of a broad range of such natural phenomena, and analytically derive an approximation that accurately predicts its statistics. We apply our results to study the effects of a multiplicative synaptic plasticity rule that was recently extracted from measurements in physiological conditions. Using mean-field theory analysis and network simulations, we investigate how this rule shapes the connectivity and dynamics of recurrent spiking neural networks. The multiplicative plasticity rule is shown to support efficient learning of input stimuli, and it gives a stable, unimodal synaptic-weight distribution with a large fraction of strong synapses. The strong synapses remain stable over long times but do not “run away.” Our results suggest that the multiplicative shot-noise offers a new route to understand the tradeoff between flexibility and stability in neural circuits and other dynamic networks.

59 BASIC BIOLOGICAL SCIENCES↗

DOE OSTI2024

Work Function Tuning of a Weak Adhesion Homojunction for Stable Perovskite Solar Cells

Perovskite solar cells (PSCs) have demonstrated a comparable efficiency to Si-based cells. However, the buried interface with weak adhesion remains a critical issue since the ion migration enhanced by the built-in electric field at this interface might lead to instability. We report here that adjusting the energy-level alignment at the weak adhesion homojunction interface can mitigate ion migration and thereby enhance the stability and photovoltaic performance of PSCs. Functional molecules with self-assembled monolayer characteristics were introduced to the surface of the SnO2 layer using silane derivatives, which tuned the work function of the homojunction depending on the functional groups in the molecules and thereby significantly reduced the built-in electric field. The PSC exhibited a power conversion efficiency (PCE) of 25.3%. The maximum power point (MPP) tracking under continuous illumination confirmed that the device retained more than 97% of its initial PCE, even after 1,000 h.

homojunction↗

DOE OSTI2021

Electrothermoplasmonic Trapping and Dynamic Manipulation of Single Colloidal Nanodiamond

Low-power trapping of nanoscale objects can be achieved by using the enhanced fields near plasmonic nanoantennas. Unfortunately, in this approach the trap site is limited to the position of the plasmonic hotspots and continuous dynamic manipulation is not feasible. In this work, we report a low-frequency electrothermoplasmonic tweezer (LFET) that provides low-power, high-stability and continuous dynamic manipulation of a single nanodiamond. LFET harnesses the combined action of the laser illumination of a plasmonic nanopillar antenna array and low-frequency alternating current (ac) electric field to establish an electrohydrodynamic potential capable of the stable trapping and dynamic manipulation of single nanodiamonds. We experimentally demonstrate the fast transport, trapping, and dynamic manipulation of a single nanodiamond using a low-frequency ac field below 5 kHz and low-laser power of 1 mW. This nanotweezer platform for nanodiamond manipulation holds promise for the scalable assembly of single photon sources for quantum information processing and low noise quantum sensors.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

DOE OSTI2020

Theoretical analysis of energetic-ion-driven resistive interchange mode stabilization strategies using a Landau closure model

The aim of the present study is to perform a theoretical analysis of different strategies to stabilize energetic-ion-driven resistive interchange mode (EIC) in Large Helical Device (LHD) plasma. In this work, we use a reduced MHD for the thermal plasma coupled with a gyrofluid model for the energetic particles (EP) species. The hellically trapped EP component is introduced through a modification of the drift frequency to include their precessional drift. The stabilization trends of the 1/1 EIC observed experimentally with respect to the thermal plasma density and temperature are reproduced by the simulations, showing a reasonable agreement with the data. The LHD operation scenarios with stable 1/1 EIC are identified, leading to the stabilization of the 1/1 EIC if the thermal plasma density and temperature are above a given threshold. Additionally, the 1/1 EIC are also stabilized if the rotational transform is modified in a way that the 1/1 rational surface is located further away than 0.9 times the normalized radius, or the magnetic shear in the plasma periphery is enhanced. Also, LHD discharges with large magnetic fields show a higher EIC destabilization threshold with respect to the thermal plasma density. If the perpendicular NBI deposition region is moved further inward than 0.875 times the normalized radius the 1/1 EIC are also stabilized. Furthermore, increasing the perpendicular NBI voltage such that the EP energy is higher than 30 keV stabilizes the 1/1 EIC. Moreover, deuterium plasmas show a higher stability threshold for the 1/1 EIC than hydrogen plasmas. The experimental data shows a larger time interval between EIC events as the power of the tangential NBI is increased providing that the perpendicular NBI power is at least 13 MW. This implies a stabilizing effect of the tangential NBI.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS1990

Kinetic instability associated with spherical shell distribution of cometary pickup ions

The stability of ion shell distribution is an interesting and important issue in view of the fact that it is stable under perturbations propagating parallel to the ambient magnetic field, despite large amount of free energy it contains. It was found, however, that if the shell distribution of ions has a sufficient amount of drift speed with respect to the solar wind hydromagnetic waves, it can become unstable. The obliquely propagating hydromagnetic instability associated with the ion shell distribution was recently discovered. This letter presents the unified stability analysis of the ion shell distribution, under what condition the drift-induced instability of the type first discussed by Gary and Sinha (1989), and the oblique hydromagnetic instability discussed by Wu and Yoon (1990) are excited, and how the two types of instabilities are related.

Yoon, Peter H.↗

NASA NTRS1990

Slosh wave excitation and stability of spacecraft fluid systems

The instability of liquid and gas interface can be induced by the pressure of longitudinal and lateral accelerations, vehicle vibration, and rotational fields of spacecraft in a microgravity environment. Characteristics of slosh waves excited by the restoring force field of gravity jitters have been investigated. Results show that lower frequency gravity jitters excite slosh waves with higher ratio of maximum amplitude to wave length than that of the slosh waves generated by the higher frequency gravity jitters.

Hung, R. J.↗

NASA NTRS1992

Investigation of the aerothermodynamics of hypervelocity reacting flows in the ram accelerator

New diagnostic techniques for measuring the high pressure flow fields associated with high velocity ram accelerator propulsive modes was experimentally investigated. Individual propulsive modes are distinguished by their operating Mach number range and the manner in which the combustion process is initiated and stabilized. Operation of the thermally choked ram accelerator mode begins by injecting the projectile into the accelerator tube at a prescribed entrance velocity by means of a conventional light gas gun. A specially designed obturator, which is used to seal the bore of the gun, plays a key role in the ignition of the propellant gases in the subsonic combustion mode of the ram accelerator. Once ignited, the combustion process travels with the projectile and releases enough heat to thermally choke the flow within several tube diameters behind it, thereby stabilizing a high pressure zone on the rear of the projectile. When the accelerating projectile approaches the Chapman-Jouguet detonation speed of the propellant mixture, the combustion region is observed to move up onto the afterbody of the projectile as the pressure field evolves to a distinctively different form that implies the presence of supersonic combustion processes. Eventually, a high enough Mach number is reached that the ram effect is sufficient to cause the combustion process to occur entirely on the body. Propulsive cycles utilizing on-body heat release can be established either by continuously accelerating the projectile in a single propellant mixture from low initial in-tube Mach numbers (M less than 4) or by injecting the projectile at a speed above the propellant's Chapman-Jouguet detonation speed. The results of experimental and theoretical explorations of ram accelerator gas dynamic phenomena and the effectiveness of the new diagnostic techniques are presented in this report.

Hertzberg, A.↗

DOE OSTI2022

A two-directional vibrational probe reveals different electric field orientations in solution and an enzyme active site

We report the catalytic power of an electric field depends on its magnitude and orientation with respect to the reactive chemical species. Understanding and designing new catalysts for electrostatic catalysis thus requires methods to measure the electric field orientation and magnitude at the molecular scale. We demonstrate that electric field orientations can be extracted using a two-directional vibrational probe by exploiting the vibrational Stark effect of both the C=O and C–D stretches of a deuterated aldehyde. Combining spectroscopy with molecular dynamics and electronic structure partitioning methods, we demonstrate that, despite distinct polarities, solvents act similarly in their preference for electrostatically stabilizing large bond dipoles at the expense of destabilizing small ones. In contrast, we find that for an active-site aldehyde inhibitor of liver alcohol dehydrogenase, the electric field orientation deviates markedly from that found in solvents, which provides direct evidence for the fundamental difference between the electrostatic environment of solvents and that of a preorganized enzyme active site.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2023

Characterization of the Fast-Neutron Irradiator and the Fast-Flux Tube Irradiation Fixtures at the Pennsylvania State Breazeale Reactor

Accurate knowledge of the neutron spectrum at a nuclear research reactor is a prerequisite for planning irradiation experiments, as well as for evaluating irradiation exposure results. The neutron-flux spectrum in the fast-neutron irradiator (FNI) and the fast-flux tube (FFT) irradiation fixtures at the Pennsylvania State Breazeale Reactor (PSBR) were characterized using the multi-foil neutron activation method. These irradiation fixtures make use of graded shielding to produce unique neutron fields. Multiple foil sets were irradiated in the fixtures with different exposure times and reactor powers to understand the stability over a wide range of operating conditions. Measured results were evaluated against a MCNP6 simulation to produce a measurement-informed neutron flux-energy spectrum for each fixture using STAYSL_PNNL. Simulated estimates of the FNI fixture, a newer fixture (~25 years old), demonstrated excellent agreement with measured results; the FFT did not. Thermal neutron measurements from the FFT suggest there is additional thermal leakage not captured in the simulation model. In conclusion, possible explanations for the discrepancy include burn-out or degradation (i.e., micro-cracking, gaps, etc.) in the boral and cadmium liners over the lifetime of the fixture (~40 years old).

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

DOE OSTI2022

Radiolytic evaluation of select sulfur chlorides (S 2 Cl 2 and SOCl 2 ) for advanced low temperature chlorination of zirconium-based used nuclear fuel cladding

New sulfur chloride compounds—sulfur monochloride (S 2 Cl 2 ) and thionyl chloride (SOCl 2 )—have been proposed as alternative chlorinating agents for the chemical decladding of zirconium-based used nuclear fuel cladding materials. However, the radiation stability of these compounds has not been thoroughly evaluated, despite envisioned process conditions involving intense, multi-component radiation fields. Knowledge of the radiation chemistry of these sulfur chlorides is essential for the development and optimization of alternative chlorination technologies. To this end, we present preliminary findings on the gamma radiolysis of neat S 2 Cl 2 and SOCl 2 at ambient temperature up to ~ 34 MGy. In this study, Raman spectroscopy and density functional theory calculations were used to identify the Raman-active degradation products from S 2 Cl 2 and SOCl 2 radiolysis. Both sulfur chloride compounds exhibited significant radiation resistance, with respect to changes in the Raman signatures of the parent compounds and the ingrowth of Raman-active degradation products. For S 2 Cl 2 , molecular chlorine (Cl 2 ) was directly identified as the predominant degradation product, which was completely consumed at higher absorbed doses (> 9 MGy). Similarly, the main degradation product from SOCl 2 radiolysis was also Cl 2 , although in this system it continued to grow in with dose over the entire dose range. Further, an “S=O” containing degradation product(s) was also identified as a compliment to Cl 2 . Overall, the perceived radiation resistance of these sulfur chloride compounds makes them suitable for inclusion in a used nuclear fuel chemical decladding process, especially as radiolytically formed Cl 2 can be used to reform the parent compounds, thereby increasing the longevity of the solvents used.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗