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At least 1,567 records · Page 87

Atmospheric Data-Driven Visualization of Air Quality Variation in Megacities

The growth and spread of human settlements and increasing urban density are important processes in global change. Urbanization has accelerated with population growth, and more densely populated urban areas have major effects on the local and regional environments. Air quality in megacities has been a concern for decades. Data for anthropogenic emissions, pollutants, and particulate matter can inform research on the interactions between urban landscapes and the atmosphere, assist policy makers in developing sustainable, healthy environments, and inform the general public. To better assist researchers, students, the public, and policymakers in understanding the annual and seasonal variation of aerosol and gas intensity in megacities, the Science Outreach Team at NASA Langley Research Center’s Atmospheric Science Data Center (ASDC) Distributed Active Archive Center (DAAC) demonstrate data products at the ASDC that can be used to visualize these parameters. The presentation uses data from the ASDC-supported NASA missions Measurements Of Pollution In The Troposphere (MOPITT), Cloud-Aerosol and Infrared Pathfinder Satellite Observation (CALIPSO), Tropospheric Emission Spectrometer (TES), and Multi-angle Imaging Spectro Radiometer (MISR)

Air Quality↗

Mesoscale Convective Systems Tracking Method Intercomparison (MCSMIP): Application to DYAMOND Global km‐Scale Simulations

Abstract Global kilometer‐scale models represent the future of Earth system modeling, enabling explicit simulation of organized convective storms and their associated extreme weather. Here, we comprehensively evaluate tropical mesoscale convective system (MCS) characteristics in the DYAMOND (DYnamics of the atmospheric general circulation modeled on non‐hydrostatic domains) simulations for both summer and winter phases. Using 10 different feature trackers applied to simulations and satellite observations, we assess MCS frequency, precipitation, and other key characteristics. Substantial differences (a factor of 2–3) arise among trackers in observed MCS frequency and their precipitation contribution, but model‐observation differences in MCS statistics are more consistent across trackers. DYAMOND models are generally skillful in simulating tropical mean MCS frequency, with multi‐model mean biases ranging from −2%–8% over land and −8%–8% over ocean (summer vs. winter). However, most DYAMOND models underestimate MCS precipitation amount (23%) and their contribution to total precipitation (17%). Biases in precipitation contributions are generally smaller over land (13%) than over ocean (21%), with moderate inter‐model variability. While models better simulate MCS diurnal cycles and cloud shield characteristics, they overestimate MCS precipitation intensity and underestimate stratiform rain contributions (up to a factor of 2), particularly over land, albeit observational uncertainties exist. Additionally, models exhibit a wide range of precipitable water in the tropics compared to reanalysis and satellite observations, with many models showing exaggerated sensitivity of MCS precipitation intensity to precipitable water. The MCS metrics developed here provide process‐oriented diagnostics to guide future model development.

54 ENVIRONMENTAL SCIENCES↗

PERSIANN Dynamic Infrared–Rain Rate Model (PDIR) for High-Resolution, Real-Time Satellite Precipitation Estimation

Precipitation measurements with high spatiotemporal resolution are a vital input for hydrometeorological and water resources studies; decision-making in disaster management; and weather, climate, and hydrological forecasting. Moreover, real-time precipitation estimation with high precision is pivotal for the monitoring and managing of catastrophic hydroclimate disasters such as flash floods, which frequently transpire after extreme rainfall. While algorithms that exclusively use satellite infrared data as input are attractive owing to their rich spatiotemporal resolution and near-instantaneous availability, their sole reliance on cloud-top brightness temperature (T b ) readings causes underestimates in wet regions and overestimates in dry regions—this is especially evident over the western contiguous United States (CONUS). We introduce an algorithm, the Precipitation Estimations from Remotely Sensed Information Using Artificial Neural Networks (PERSIANN) Dynamic Infrared–Rain rate model (PDIR), which utilizes climatological data to construct a dynamic (i.e., laterally shifting) T b –rain rate relationship that has several notable advantages over other quantitative precipitation-estimation algorithms and noteworthy skill over the western CONUS. Validation of PDIR over the western CONUS shows a promising degree of skill, notably at the annual scale, where it performs well in comparison to other satellite-based products. Analysis of two extreme landfalling atmospheric rivers show that solely IR-based PDIR performs reasonably well compared to other IR- and PMW-based satellite rainfall products, marking its potential to be effective in real-time monitoring of extreme storms. This research suggests that IR-based algorithms that contain the spatiotemporal richness and near-instantaneous availability needed for rapid natural hazards response may soon contain the skill needed for hydrologic and water resource applications.

54 ENVIRONMENTAL SCIENCES↗

The Boreal Summer Madden–Julian Oscillation and Moist Convective Morphology over the Maritime Continent

Abstract While the boreal summer Madden–Julian oscillation (MJO) is commonly defined as a planetary-scale disturbance, the convective elements that constitute its cloud dipole exhibit pronounced variability in their morphology. We therefore investigate the relationship between the intraseasonal cloud anomaly of the MJO and the convective elements that populate its interior by simulating a boreal summer MJO event over the Maritime Continent using a cloud-resolving model. A progressive relationship between convective cell morphology and the MJO within the convectively enhanced region of the MJO was identified and characterized as follows: anomalously long-lasting cells in the initial phases, followed by an increased number of cells in the intermediate phases, progressing into more expansive cells in the terminal phases. A progressive relationship does not seem to exist within the convectively suppressed region of the MJO within the simulated domain, however. Within the convectively enhanced region of the MJO, the progressive relationship is partially explained by the evolution of bulk atmospheric characteristics, such as instability and wind shear. Positive midlevel moisture anomalies coincide with anomalously long-lasting convective cells, which is hypothesized to further cascade into an increase in convective cell volume, although variability in the number of convective cells seems to be related to an unidentified variable. This intraseasonal relationship between convective cell morphology and the boreal summer MJO within the Maritime Continent may have broader implications for the large-scale structure and evolution of the MJO, related to both convective moistening and cloud-radiative feedbacks.

54 ENVIRONMENTAL SCIENCES↗

Monitoring Atmospheric CO2 From Space: Challenge & Approach

Atmospheric CO2 is the key radiative forcing for the Earth's climate and may contribute a major part of the Earth's warming during the past 150 years. Advanced knowledge on the CO2 distributions and changes can lead considerable model improvements in predictions of the Earth's future climate. Large uncertainties in the predictions have been found for decades owing to limited CO2 observations. To obtain precise measurements of atmospheric CO2, certain challenges have to be overcome. For an example, global annual means of the CO2 are rather stable, but, have a very small increasing trend that is significant for multi-decadal long-term climate. At short time scales (a second to a few hours), regional and subcontinental gradients in the CO2 concentration are very small and only in an order of a few parts per million (ppm) compared to the mean atmospheric CO2 concentration of about 400 ppm, which requires atmospheric CO2 space monitoring systems with extremely high accuracy and precision (about 0.5 ppm or 0.125%) in spatiotemporal scales around 75 km and 10-s. It also requires a decadal-scale system stability. Furthermore, rapid changes in high latitude environments such as melting ice, snow and frozen soil, persistent thin cirrus clouds in Amazon and other tropical areas, and harsh weather conditions over Southern Ocean all increase difficulties in satellite atmospheric CO2 observations. Space lidar approaches using Integrated Path Differential Absorption (IPDA) technique are considered to be capable of obtaining precise CO2 measurements and, thus, have been proposed by various studies including the 2007 Decadal Survey (DS) of the U.S. National Research Council. This study considers to use the Intensity-Modulated Continuous-Wave (IM-CW) lidar to monitor global atmospheric CO2 distribution and variability from space. Development and demonstration of space lidar for atmospheric CO2 measurements have been made through joint adventure of NASA Langley Research Center and Exelis, Inc. As prototype space IPDA lidars, airborne laser absorption lidar systems operating in 1.57 CO2 absorption band have been developed and tested through lab, ground-based range, and flight campaigns. Very encouraging results have been obtained. The signal-to-noise ratio (SNR) for clear sky IPDA measurements of CO2 differential absorption optical depth (DAOD) for a 10-s integration over vegetated areas with about 10 km range was found to be as high as 1300, resulting in an error 0.077% or equivalent CO2 mixing ratio (XCO2) column precision of ~0.3 ppm. Precise range measurements using the IM-CW lidar approach were also achieved, and the uncertainties have been shown to be at sub meter level. Based on the airborne lidar development, space lidar and atmospheric CO2 observations are simulated. It shows that with the IM-CW approach, accurate atmospheric CO2 measurements can be achieved from space, and a space mission such as that proposed by the DS will meet science goals of atmospheric CO2 monitoring.

Lin, Bing↗

Megadrought: A Series of Unfortunate La Niña Events?

Megadroughts are multidecadal periods of aridity more persistent than most droughts during the instrumental period. Paleoclimate evidence suggests that megadroughts occur in many parts of the world, including North America, Central America, western Europe, eastern Asia, and northern Africa. It remains unclear to what extent such megadroughts require external forcing or whether they can arise from internal climate variability alone. A novel statistical–dynamical approach is used to evaluate the possibility that such events arise solely as a function of interannual tropical sea surface temperature (SST) variations. A statistical emulator of tropical SST variations is constructed by using an empirical moving-blocks bootstrap approach that randomly samples multiyear sequences of the observational SST record. This approach preserves the power spectrum, seasonal cycle, and spatial pattern of El Niño-Southern Oscillation (ENSO) but removes longer timescale fluctuations embedded in the observational record. These resampled SST anomalies are then used to force an atmospheric model (the Community Atmosphere Model Version 5). As megadroughts emerge in this run, they should, therefore, be solely a consequence of La Niña sequences combined with internal atmospheric variability and persistence driven by soil moisture storage and other land-surface processes. We indeed find that megadroughts in this simulation have an amplitude-duration rate that is generally indistinguishable from the rate documented in paleoclimate records of the western United States. Our findings support the idea that megadroughts may occur randomly when the unforced climate system evolves freely over a sufficiently long period of time, implying that an unforced unusual but statistically plausible series of La Niña events may be sufficient to generate megadrought.

54 ENVIRONMENTAL SCIENCES↗

The Doppler Wind Temperature Sensor (DWTS) Flight Evaluation and Experiments (TES-16, 17)

The Doppler Wind and Temperature Sounder instrument (DWTS), developed by Global Atmospheric Technologies and Sciences (GATS), is a simple but powerful tool that has the potential to become a new window through which to study the dynamics of the upper atmosphere. Based around a defense-grade infrared camera peering through a static gas cell used as a scanning spectral filter, the DWTS instrument infers wind velocities and kinetic temperatures through the stratosphere and lower thermosphere. The DWTS achieves this scanning by measuring the induced Doppler shift and Doppler broadening of emissions as they pass through the DWTS field of view (Gordley, et al., 2011). The DWTS holds promise in improving accuracy in weather determination , and the core technology can be adapted to study other planetary atmospheres. In partnership with GATS, NOAA, and other collaborators, NASA Ames and the Nano Orbital Workshop group have been working to evaluate the DWTS instrument on orbit and optimize it as a flexible nanosatellite payload. The first mission selected for DWTS evaluation is preparing for flight in early 2024, which will be followed by a more capable science mission in 2025, with both missions being part of the TES-n/NOW heritage flight series. The first rapid technology demonstration flight, TES-16/DWTS-A, will demonstrate a single DWTS instrument in an approximately 2U payload volume with the imaging aperture perpendicular to the flight velocity vector. With an estimated power consumption of 50 watts, supplied via a custom NOW-designed DC-DC converter, the instrument will maintain the imaging sensor plane at 80K during instrument evaluation periods using an integrated pulse-tube cryocooler. Data from DWTS will be captured and processed via a NOW-designed custom data interface unit before being transmitted via S-band radio back to select ground stations, with instrument command and control operated via L-band global-coverage radio. The subsequent TES-17/DWTS-B mission will be a dedicated science mission to obtain full altitude coverage from 20 to 200 km during both day and night, all from a single small-satellite equipped with three DWTS instruments, each hosting a different gas cell chemistry. The intention of this flight series, and one of NASA’s interests in this instrument, is to advance a Martian atmospheric instrument (Colaprete, Gordley, et al) which, if successful, would greatly further understanding of Martian atmospheric behavior. The proposed paper will review the flight series in detail, including challenges facing the TES-16 flight tests and the projected challenges and application to Mars study. Additional detail regarding the possible applications of a Cognitive Communication technique in current flight development by NOW collaborators at the NASA Glenn Research Center will also be discussed, including the implications of using an automated User Initiated Service (UIS) protocol to maximize the data collected per orbit.

nanosatellite↗

Titan Flagship Mission 3-Degree-of-Freedom Simulation Analysis

A NASA flagship mission to Titan, the largest moon of Saturn and the only moon in the solar system with a significant atmosphere, has been designed that uses three separate spacecraft, each requiring significant interaction with the atmosphere. The first vehicle is a Titan lander for lower-atmosphere and surface science. The second is an aerial vehicle for aerial science at approximately 10 km altitude with an expected lifetime of one year. This spacecraft will use the natural winds of Titan to cover a large area over its lifetime. The third vehicle is a Titan orbiter that will interact with the atmosphere in two respects. The first atmospheric interaction is the orbital insertion maneuver that will be accomplished using aerocapture, during which time the hyperbolic approach of 6.5 km/s will be reduced to 1.6 km/s over 41 minutes with an exit periapsis altitude of 130 km. The second atmospheric interaction occurs after a propulsive maneuver has raised the periapsis after aerocapture to 1170 km, where the atmosphere will be sampled over several months. This is the first phase of aerosampling that covers southern latitudes. After a 3.3-year circular science phase at an altitude of 1700 km, a second phase of additional aerosampling is performed sampling northern latitudes. The atmospheric trajectory analysis for these three spacecraft will be discussed throughout this paper.

Prince, Jill L.↗

The Correlation of Mesoscale Humidity Anomalies With Mesoscale Organization of Marine Stratocumulus From Observations Over the ARM Eastern North Atlantic Site

The structure of mesoscale cellular organization in marine cloud-topped boundary layers is found to be well characterized by using a novel compositing approach based on mesoscale variations in the column water vapor path (WVP). The approach is applied to ground-based observations from the Atmospheric Radiation Measurement (ARM) Eastern North Atlantic site. Based on a set of satellite and ground-based observational criteria, 381 hr of closed-cell and 227 hr of open-cell cases were selected from late 2015 to early 2018. Strong correlations are found between mesoscale-filtered cloud properties and WVP for both closed-cell and open-cell regimes. In the moist atmospheric columns, the clouds are thicker with higher tops and lower bases, and stronger precipitation compared to that in the dry columns. Overall, cloud properties of open and closed cells covary similarly with mesoscale moisture perturbations, except that the correlation of liquid water path with WVP is much weaker for open cells. The relations of subcloud properties with WVP are also examined. In the moist columns, surface equivalent potential temperature and relative humidity are higher than in the dry columns. A marginally negative correlation between mesoscale-filtered subcloud turbulence eddy dissipation rate and WVP is found for closed cells. These results are consistent with the conceptual model of closed cellular mesoscale circulations of Zhou and Bretherton (2019).

54 ENVIRONMENTAL SCIENCES↗

Coastal Sea Level Observations Record the Twentieth-Century Enhancement of Decadal Climate Variability

Changes in the amplitude of decadal climate variability over the twentieth century have been noted, with most evidence derived from tropical Pacific sea surface temperature records. However, the length, spatial coverage, and stability of most instrumental records are insufficient to robustly identify such nonstationarity, or resolve its global spatial structure. Here, it is found that the long-term, stable, observing platform provided by tide gauges reveals a dramatic increase in the amplitude and spatial coherence of decadal (11–14-yr period) coastal sea level (ζ) variability between 1960 and 2000. During this epoch, western North American ζ was approximately out of phase with ζ in Sydney, Australia, and led northeastern U.S. ζ by approximately 1–2 years. The amplitude and timing of changes in decadal ζ variability in these regions are consistent with changes in atmospheric variability. Specifically, central equatorial Pacific wind stress and Labrador Sea heat flux are highly coherent and exhibit contemporaneous, order-of-magnitude increases in decadal power. These statistical relationships have a mechanistic underpinning: Along the western North American coastline, equatorial winds are known to drive rapidly propagating ζ signals along equatorial and coastal waveguides, while a 1–2-yr lag between Labrador Sea heat fluxes and northeastern United States ζ is consistent with a remotely forced, buoyancy-driven, mechanism. Tide gauges thus provide strong independent support for an increase in interbasin coherence on decadal time scales over the second half of the twentieth century, with implications for both the interpretation and prediction of climate and sea level variability.

54 ENVIRONMENTAL SCIENCES↗

Dynamically Downscaled (WRF) 1km, Hourly Meteorological Conditions 1987-2020. East/Taylor Watersheds

This dataset contains meteorological output from the Weather Research and Forecasting (WRF) version 3.8.1. This dataset has been created to 1) investigate hydrometeorological processes impacting the East River and water-delivery to the Critical Zone, and 2) provide meteorological forcing data for distributed Earth-science modeling applications in the East River watershed. Variables have a 1 kilometer spatial resolution and hourly temporal resolution and encompass a rectangular region encompassing the East and Taylor River watersheds, Colorado, near the town of Crested Butte. WRF was forced using Climate Forecast System Reanalysis (CFSR) lateral boundary conditions. Each .zip file contains one "water year" of data (October 1 -- September 30; i.e. water year 2017 starts October 1, 2016 and ends September 30, 2017). Each zip folder contains 12 netcdf (.nc) files containing one month of hourly data each and are approximately 250mb. Model timestamps are in UTC time.The files contain the following data variables:EAST_MASK: binary mask of the watershed regionTAYLOR_MASK: binary mask of the watershed regionGLW downwelling longwave radiation (w/m2)HR_PRCP: Hourly Precipitation Rate (mm/hr). Includes all hydrometeors (solid+liquid). HFX NoahMP LSM total grid-cell modelled sensible heat flux (w/m2) [positive towards atmosphere]LH NoahMP LSM total grid-cell modelled latent heat flux (w/m2) [positive towards atmosphere; can be converted to ET]PSFC Surface Barometric Pressure (hPa)Q2 Two-meter specific humidity (kg/kg)SWDOWN Downwelling shortwave solar radiation (w/m2)SWNORM Terrain-normal downwelling shortwave radiation (w/m2)T2 Two-meter air temperature (deg K)U10 10-m U-component of wind velocity (m/s)V10 10m V-component of wind velocity (m/s)XLAT Latitude of grid-center point XLONG Longitude of grid-center point XTIME Model timestamp, **in UTC**

54 ENVIRONMENTAL SCIENCES↗

The Atlantic Jet Response to Stratospheric Events: A Regime Perspective

The tropospheric response to Sudden Stratospheric Warmings (SSWs) is associated with an equatorward shift in the midlatitude jet and associated storm tracks, while Strong Polar Vortex (SPV) events elicit a contrasting response. Recent analyses of the North Atlantic jet using probability density functions of a jet latitude index have identified three preferred jet latitudes, raising the question of whether the tropospheric response to SSWs and SPVs results from a change in relative frequencies of these preferred jet regimes rather than a systematic jet shift. We explore this question using atmospheric reanalysis data from 1979 to 2018 (26 SSWs and 33 SPVs), and a 202-years integration of the Whole Atmosphere Community Climate Model (92 SSWs and 68 SPVs). Following SSWs, the northern jet regime becomes less common and the central and southern regimes become more common. These changes occur almost immediately following “split” vortex events, but are more delayed following “displacement” events. In contrast, the northern regime becomes more frequent and the southern regime less frequent following SPV events. Following SSWs, composites of 500-hPa geopotential heights, surface air temperatures, and precipitation most closely resemble composites of the southern jet regime, and are generally opposite in sign to the composites of the northern jet regime. These comparisons are reversed following SPVs. Thus, one possible interpretation is that the two southernmost regimes appear to be favored following SSWs, while the southernmost regime becomes less common following SPVs.

54 ENVIRONMENTAL SCIENCES↗

Climate Dynamics Preceding Summer Forest Fires in California and the Extreme Case of 2018

Recent record-breaking wildfire seasons in California prompt an investigation into the climate patterns that typically precede anomalous summer burned forest area. Using burned-area data from the U.S. Forest Service’s Monitoring Trends in Burn Severity (MTBS) product and climate data from the fifth major global reanalysis produced by the European Centre for Medium-Range Weather Forecasts (ERA5) over 1984–2018, relationships between the interannual variability of antecedent climate anomalies and July California burned area are spatially and temporally characterized. Lag correlations show that antecedent high vapor pressure deficit (VPD), high temperatures, frequent extreme high temperature days, low precipitation, high subsidence, high geopotential height, low soil moisture, and low snowpack and snowmelt anomalies all correlate significantly with July California burned area as far back as the January before the fire season. Seasonal regression maps indicate that a global midlatitude atmospheric wave train in late winter is associated with anomalous July California burned area. July 2018, a year with especially high burned area, was to some extent consistent with the general patterns revealed by the regressions: low winter precipitation and high spring VPD preceded the extreme burned area. However, geopotential height anomaly patterns were distinct from those in the regressions. Extreme July heat likely contributed to the extent of the fires ignited that month, even though extreme July temperatures do not historically significantly correlate with July burned area. While the 2018 antecedent climate conditions were typical of a high-burned-area year, they were not extreme, demonstrating the likely limits of statistical prediction of extreme fire seasons and the need for individual case studies of extreme years.

54 ENVIRONMENTAL SCIENCES↗

Atmospheric Rivers Impacting Northern California Exhibit a Quasi-Decadal Frequency

Periods of water surplus and deficit in Northern California follow a pronounced quasi-decadal cycle. This cycle is largely driven by the frequency of atmospheric rivers (ARs), affecting the region’s wet and dry periods. Our analyses demonstrate that the quasi-decadal cycle of AR frequency relies on moisture transport associated with the position and intensity of the Aleutian Low. In observations, the Aleutian Low is shown to covary with tropical Pacific sea surface temperature anomalies. A modeling experiment, which incorporates ocean observations from the equatorial Pacific into the fully coupled climate model, provides support that the quasi-decadal cycle of the Aleutian Low is forced by the tropical Pacific. Subsequently, the tropical Pacific modulates the wet season moisture transport toward California on decadal time scales, affecting AR frequency. These results provide metrics for improving interannual-to-decadal prediction of AR activity, which drives hydrological cycles in Northern California.

54 ENVIRONMENTAL SCIENCES↗

Decadal predictability of North Atlantic blocking and the NAO

Can multi-annual variations in the frequency of North Atlantic atmospheric blocking and mid-latitude circulation regimes be skilfully predicted? Recent advances in seasonal forecasting have shown that mid-latitude climate variability does exhibit significant predictability. However, atmospheric predictability has generally been found to be quite limited on multi-annual timescales. New decadal prediction experiments from NCAR are found to exhibit remarkable skill in reproducing the observed multi-annual variations of wintertime blocking frequency over the North Atlantic and of the North Atlantic Oscillation (NAO) itself. This is partly due to the large ensemble size that allows the predictable component of the atmospheric variability to emerge from the background chaotic component. The predictable atmospheric anomalies represent a forced response to oceanic low-frequency variability that strongly resembles the Atlantic Multi-decadal Variability (AMV), correctly reproduced in the decadal hindcasts thanks to realistic ocean initialization and ocean dynamics. The occurrence of blocking in certain areas of the Euro-Atlantic domain determines the concurrent circulation regime and the phase of known teleconnections, such as the NAO, consequently affecting the stormtrack and the frequency and intensity of extreme weather events. Therefore, skilfully predicting the decadal fluctuations of blocking frequency and the NAO may be used in statistical predictions of near-term climate anomalies, and it provides a strong indication that impactful climate anomalies may also be predictable with improved dynamical models.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Aerosol Direct Radiative Effects at the ARM SGP and TWP Sites: Clear Skies

The clear-sky aerosol direct radiative effect (DRE) was estimated at the Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) and Tropical Western Pacific (TWP) sites. The NASA Langley Fu-Liou radiation model was used with observed inputs including aerosol vertical extinction profile from the Raman lidar; spectral aerosol optical depth (AOD), single-scattering albedo and asymmetry factor from Aerosol Robotic Network; temperature and water vapor profiles from radiosondes; and surface shortwave (SW) spectral albedo from radiometers. A radiative closure experiment was conducted for clear-sky conditions. The mean differences of modeled and observed surface downwelling SW total fluxes were 1 W m-2 at SGP and 2 W m -2 at TWP, which are within observational uncertainty. At SGP, the estimated annual mean clear-sky aerosol DRE is -3.00 W m -2 at the top of atmosphere (TOA) and -6.85 W m -2 at the surface. The strongest aerosol DRE of -4.81 (-10.77) W m -2 at the TOA (surface) are in the summer when AODs are largest. The weakest aerosol DRE of -.28 (-2.77) W m -2 at the TOA (surface) are in November–January when AODs and single-scattering albedos are lowest. At TWP, the annual mean clear-sky DRE is -2.82 W m-2 at the TOA and -10.34 W m -2 at the surface. The strongest aerosol DRE of -5.95 (-22.20) W m -2 at the TOA (surface) are in November (October) due to the biomass burning season’s peak. The weakest aerosol DRE of -0.96 (-4.16) W m -2 at the TOA (surface) are in March (April) when AODs are smallest.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Atmospheric Correction at AERONET Locations: A New Science and Validation Data Set

This paper describes an AERONET-based Surface Reflectance Validation Network (ASRVN) and its dataset of spectral surface bidirectional reflectance and albedo based on MODIS TERRA and AQUA data. The ASRVN is an operational data collection and processing system. It receives 50x50 square kilometer subsets of MODIS L1B data from MODAPS and AERONET aerosol and water vapor information. Then it performs an accurate atmospheric correction for about 100 AERONET sites based on accurate radiative transfer theory with high quality control of the input data. The ASRVN processing software consists of L1B data gridding algorithm, a new cloud mask algorithm based on a time series analysis, and an atmospheric correction algorithm. The atmospheric correction is achieved by fitting the MODIS top of atmosphere measurements, accumulated for 16-day interval, with theoretical reflectance parameterized in terms of coefficients of the LSRT BRF model. The ASRVN takes several steps to ensure high quality of results: 1) cloud mask algorithm filters opaque clouds; 2) an aerosol filter has been developed to filter residual semi-transparent and sub-pixel clouds, as well as cases with high inhomogeneity of aerosols in the processing area; 3) imposing requirement of consistency of the new solution with previously retrieved BRF and albedo; 4) rapid adjustment of the 16-day retrieval to the surface changes using the last day of measurements; and 5) development of seasonal back-up spectral BRF database to increase data coverage. The ASRVN provides a gapless or near-gapless coverage for the processing area. The gaps, caused by clouds, are filled most naturally with the latest solution for a given pixels. The ASRVN products include three parameters of LSRT model (k(sup L), k(sup G), k(sup V)), surface albedo, NBRF (a normalized BRF computed for a standard viewing geometry, VZA=0 deg., SZA=45 deg.), and IBRF (instantaneous, or one angle, BRF value derived from the last day of MODIS measurement for specific viewing geometry) for MODIS 500m bands 1-7. The results are produced daily at resolution of 1 km in gridded format. We also provide cloud mask, quality flag and a browse bitmap image. The new dataset can be used for a wide range of applications including validation analysis and science research.

Wang, Yujie↗

Effects of the large-scale circulation on temperature and water vapor distributions in the Π Chamber

Abstract. Microphysical processes are important for the development of clouds and thus Earth's climate. For example, turbulent fluctuations in the water vapor mixing ratio, r, and temperature, T, cause fluctuations in the saturation ratio, S. Because S is the driving factor in the condensational growth of droplets, fluctuations may broaden the cloud droplet size distribution due to individual droplets experiencing different growth rates. The small-scale turbulent fluctuations in the atmosphere that are relevant to cloud droplets are difficult to quantify through field measurements. We investigate these processes in the laboratory using Michigan Tech's Π Chamber. The Π Chamber utilizes Rayleigh–Bénard convection (RBC) to create the turbulent conditions inherent in clouds. In RBC it is common for a large-scale circulation (LSC) to form. As a consequence of the LSC, the temperature field of the chamber is not spatially uniform. In this paper, we characterize the LSC in the Π Chamber and show how it affects the shape of the distributions of r, T, and S. The LSC was found to follow a single roll with an updraft and downdraft along opposing walls of the chamber. Near the updraft (downdraft), the distributions of T and r were positively (negatively) skewed. At each measuring position, S consistently had a negatively skewed distribution, with the downdraft being the most negative.

54 ENVIRONMENTAL SCIENCES↗