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At least 1,549 records · Page 86

Characterizing the modulation transfer function for X-ray radiography in high energy density experiments

Here, the Modulation Transfer Function ( MTF ) is an established means for characterizing imaging performance of X-ray radiography systems. We report on experiments using high energy, laser-driven X-ray radiography systems that assess performance using MTF values measured with the knife-edge projection method. The broadband, hard X-ray systems under study use line-projection imaging produced by narrowing the laser-generated X-ray source with a slit. We find that good contrast resolution can be achieved (the MTF = 0.5 at 75 μm wavelength) and that this performance is reproduced on different laser facilities. We also find that the MTF is sensitive both to the thickness of the line-projection slit and to the backing material thickness under the knife-edge. Both these sensitivities are due to a common mechanism, namely induced changes in the spectrally-averaged spatial widths of the X-ray source. The same line-projection system is also used on experimental campaigns measuring Rayleigh-Taylor instability growth by dynamically imaging sinusoidal, high Z micro-targets with wavelengths of 100 μm or less. By applying the measured MTF values to correct the ripple target contrast measurements, we can predict ripple growth to approximately 10% accuracy.

47 OTHER INSTRUMENTATION↗

The CWS Experiments – An Experimental Study of the Effects of Chlorine on Thermal Neutron Absorption

The Chlorine Worth Study (CWS) experiments consist of layers of Zero Power Physics Reactor plates moderated by high density polyethylene, polyvinyl chloride, and chlorinated polyvinyl chloride with the goal to produce a thermal critical experiment. A thick high density polyethylene reflector surrounds the experiments. Aluminum fuel trays and frames were used to conduct the intrinsic heat generation of the plutonium plates away from the core and out to the top plate and the platen, both acting as heat sinks. The goal of the CWS experiments was to provide benchmark critical experiments that were sensitive to chlorine and matched the sensitivity of criticality safety applications for aqueous chloride operations at PF-4 at Los Alamos National Laboratory. The specific aqueous chloride PF-4 applications were solutions of 30 g/L plutonium, 300 g/L plutonium, and 600 g/L plutonium. The CWS experiments were designed using prototype methods developed by the ARCHIMEDES and EUCLID projects at Los Alamos National Laboratory. The CWS experiments were performed in December of 2021 at the National Criticality Experiments Research Center at the Nevada Nuclear Security Site on the Planet critical assembly. It is intended that the CWS experiments will be evaluated and submitted to the ICSBEP in the future as criticality safety benchmarks.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

First test of BNL electron beam ion source with high current density electron beam

A new electron gun with electrostatic compression has been installed at the Electron Beam Ion Source (EBIS) Test Stand at BNL. This is a collaborative effort by BNL and CERN teams with a common goal to study an EBIS with electron beam current up to 10 A, current density up to 10,000 A/cm{sup 2} and energy more than 50 keV. Intensive and pure beams of heavy highly charged ions with mass-to-charge ratio < 4.5 are requested by many heavy ion research facilities including NASA Space Radiation Laboratory (NSRL) at BNL and HIE-ISOLDE at CERN. With a multiampere electron gun, the EBIS should be capable of delivering highly charged ions for both RHIC facility applications at BNL and for ISOLDE experiments at CERN. Details of the electron gun simulations and design, and the Test EBIS electrostatic and magnetostatic structures with the new electron gun are presented. The experimental results of the electron beam transmission are given.

43 PARTICLE ACCELERATORS↗

Comparison of SiC MOSFET‐based and GaN HEMT‐based high‐efficiency high‐power‐density 7.2 kW EV battery chargers

As two exemplary candidates of wide‐bandgap devices, SiC MOSFETs and GaN HEMTs are regarded as successors of Si devices in medium‐to‐high‐voltage (>1200 V) and low‐voltage (<650 V) domains, respectively, thanks to their excellent switching performance and thermal capability. With the introduction of 650 V SiC MOSFETs and GaN HEMTs, the two technologies are in direct competition in <650 V domains, such as Level 2 battery chargers for electric vehicles (EVs). This study applies 650 V SiC and GaN to two 240 VAC/7.2 kW EV battery chargers, respectively, aiming to provide a head‐to‐head comparison of these two devices in terms of overall efficiency, power density, thermal performance, and cost. The charger essentially is an indirect matrix converter with a dual‐active‐bridge stage handling the power factor correction and power delivery simultaneously. These two chargers utilise the same control strategy, varying the phase‐shift and switching frequency to cover the wide input range (80–260 VAC) and wide output range (200 V–450 VDC). Experimental results indicated that at the same efficiency level, the GaN charger is smaller, more efficient and cheaper, while the SiC charger has a better thermal performance.

Taylor, Allan↗

Effects of fuel thickness on thermal and mechanical performance of U10-Mo monolithic fuel plates

Monolithic fuels are being considered for conversion of high performance research and test reactors. These plate-type fuels are comprised of a low enrichment, high density U-Mo alloy fuels within an aluminum cladding. Although the plates have demonstrated satisfactory performance; still, use of a high density fuel in a foil form retains technical challenges that could affect the overall performance. To understand performance of this new design during fabrication and irradiation, the plates have been evaluated for various geometrical and operational variables. As a part of these set of parametric sensitivity studies, effects of foil thickness on performance were studied. Because high performance research reactors will utilize different fuel thicknesses, it is necessary to evaluate possible effects for a range of thicknesses that are being considered for various designs. Based on the preliminary design specifications, the fuel thicknesses were varied between the limiting cases. The bounding fuel thicknesses were 0.203 mm as minimum that is projected for ATR, and 0.635 mm as maximum that is projected for MITR. To study possible effects, a behavioral model was developed for a selected plate from RERTR-12 experiments and the plate was simulated with as run irradiation history. The simulations were repeated for a range of fuel thicknesses, while keeping the cladding thickness and the operational parameters the same. The results have indicated that the plates with thicker fuels would have higher temperatures, deformations and shutdown stresses. To investigate the effects of fuel thickness exclusively, operational parameters were scaled. In particular, a second set of simulations with prorated volumetric heat generation rates were performed. The results indicated that the fabrication stresses in the fuel foil decrease with an increasing fuel thickness. On contrary, irradiation stresses of the fuel at shutdown are higher for the plates with thicker fuels. Greater peak deformations occurred in plates with thicker fuels.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Examining the creep strengthening nanoprecipitation in novel highly reinforced heat resistant steels

Here we studied the creep strengthening nanoprecipitation in novel heat resistant steels strengthened by a high density of stable nanoprecipitates. The results show that the high number density of MX nanoprecipitates within the martensitic laths in these steels comes from the great amount of MX former elements present in their chemical compositions and the high dislocation density generated by the martensitic transformation that takes place during cooling after austenitization. These dislocations act as nucleation sites for these nanoprecipitates during the tempering applied after the austenitization and quenching. Atom probe tomography measurements show that these nanoprecipitates are rich in Nb, V, Cr and N for the HDSN1 and HDSN2 steels and V, Cr and N for the HDSN3 steel. The distribution of the nanoprecipitates within the martensitic laths suggests that the creep strengthening produced by the Nb, V, Cr and N nanoprecipitates in the HDSN1 and HDSN2 steels is more effective at pinning dislocations at high temperature than that obtained in the HDSN3 steel by the V, Cr and N nanoprecipitates. However, the high amount of W in the HDSN3 steel enhances the solid solution strengthening at high temperatures, resulting in a similar high temperature strength for all HDSN steels.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Solution-Processed, High-Speed, and High-Quantum-Efficiency Quantum Dot Infrared Photodetectors

For over a decade, much effort has been focused on passivation of the high density of localized electronic trap states in colloidal semiconductor quantum dots (QDs), which lead to reduced performance in solar cell, light-emitting diode, laser, and photoconductor applications. However, here we take advantage of the naturally occurring high density of trap states to demonstrate solution-processed high-speed PbSe quantum dot near-infrared photodetectors. Carrier transport dynamics studies reveal multiple trapping and release transport dynamics in band tail states. A sandwich microstrip transmission line photodetector utilizing these QD films was fabricated to achieve high performance by allowing carriers to be swept to the electrodes before they fall into the band tail states. As a result, this device demonstrates external quantum efficiency, responsivity, and response time (full width at half-maximum) of 54%, 0.36 A/W, and 74 ps, respectively.

36 MATERIALS SCIENCE↗

A Saturated Genetic Linkage Map of Autotetraploid Alfalfa ( Medicago sativa L.) Developed Using Genotyping-by-Sequencing Is Highly Syntenous with the Medicago truncatula Genome

A genetic linkage map is a valuable tool for quantitative trait locus mapping, map-based gene cloning, comparative mapping, and whole-genome assembly. Alfalfa, one of the most important forage crops in the world, is autotetraploid, allogamous, and highly heterozygous, characteristics that have impeded the construction of a high-density linkage map using traditional genetic marker systems. Using genotyping-by-sequencing (GBS), we constructed low-cost, reasonably high-density linkage maps for both maternal and paternal parental genomes of an autotetraploid alfalfa F 1 population. The resulting maps contain 3591 single-nucleotide polymorphism markers on 64 linkage groups across both parents, with an average density of one marker per 1.5 and 1.0 cM for the maternal and paternal haplotype maps, respectively. Chromosome assignments were made based on homology of markers to the M. truncatula genome. Four linkage groups representing the four haplotypes of each alfalfa chromosome were assigned to each of the eight Medicago chromosomes in both the maternal and paternal parents. The alfalfa linkage groups were highly syntenous with M. truncatula, and clearly identified the known translocation between Chromosomes 4 and 8. In addition, a small inversion on Chromosome 1 was identified between M. truncatula and M. sativa. GBS enabled us to develop a saturated linkage map for alfalfa that greatly improved genome coverage relative to previous maps and that will facilitate investigation of genome structure. GBS could be used in breeding populations to accelerate molecular breeding in alfalfa.

59 BASIC BIOLOGICAL SCIENCES↗

The Early History of the Quark-Gluon Plasma

We present the historical antecedents to the field of relativistic heavy ion physics, beginning with early attempts to model the strong interaction and ending with the endorsement of a relativistic heavy ion collider in the 1983 U.S. Long-Range Plan for Nuclear Science. Particular attention is paid to two major themes: 1) A program to study high density states of nuclear matter emerging from the 1974 Bear Mountain conference and 2) Efforts to understand the predictions of QCD for matter at high densities and/or temperatures.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The relativistic inverse stellar structure problem

The observable macroscopic properties of relativistic stars (whose equations of state are known) can be predicted by solving the stellar structure equations that follow from Einstein’s equation. For neutron stars, however, our knowledge of the equation of state is poor, so the direct stellar structure problem can not be solved without modeling the highest density part of the equation of state in some way. This talk will describe recent work on developing a model independent approach to determining the high-density neutron-star equation of state by solving an inverse stellar structure problem. This method uses the fact that Einstein’s equation provides a deterministic relationship between the equation of state and the macroscopic observables of the stars which are composed of that material. This talk illustrates how this method will be able to determine the high-density part of the neutron-star equation of state with few percent accuracy when high quality measurements of the masses and radii of just two or three neutron stars become available. This talk will also show that this method can be used with measurements of other macroscopic observables, like the masses and tidal deformabilities, which can (in principle) be measured by gravitational wave observations of binary neutron-star mergers.

79 ASTRONOMY AND ASTROPHYSICS↗

Reversible Iron Oxyfluoride (FeOF)–Graphene Composites as Sustainable Cathodes for High Energy Density Lithium Batteries

Two large barriers are impeding the wide implementation of electric vehicles, namely driving-range and cost, primarily due to the low specific energy and high cost of mono-valence cathodes used in lithium-ion batteries. Iron is the ideal element for cathode materials considering its abundance, low cost and toxicity. However, the poor reversibility of (de)lithiation and low electronic conductivity prevent iron-based high specific energy multi-valence conversion cathodes from practical applications. In this work, a sustainable FeOF nanocomposite is developed with extraordinary performance. The specific capacity and energy reach 621 mAh g –1 and 1124 Wh kg –1 with more than 100 cycles, which triples the specific capacity, and doubles the specific energy of current mono-valence intercalation LiCoO 2 . This is the result of an effective approach, combing the nanostructured FeOF with graphene, realized by making the (de)lithiation reversible by immobilizing FeOF nanoparticles and the discharge products over the graphene surface and providing the interparticle electric conduction. Importantly, it demonstrates that introducing small amount of graphene can create new materials with desired properties, opening a new avenue for altering the (de)lithiation process. Finally, such extraordinary performance represents a significant breakthrough in developing sustainable conversion materials, eventually overcoming the driving range and cost barriers.

25 ENERGY STORAGE↗

An interface facet driven Rayleigh instability in high-aspect-ratio bimetallic nanolayered composites

One limitation hindering the structural and electrical applications of nanostructured metals is the loss of their nanostructure and strength under elevated temperatures. Nanostructured metals often have grain structures that contain a high density of triple junctions, where thermally induced instabilities commonly initiate. Prior work has resulted in fabrication of nanolayered two-phase composites that possess high-aspect ratio grains, a scarcity of triple junctions, and a thermally stable microstructure. In this work, transmission electron microscopy is used to investigate how these composites could eventually breakdown during heating. We reveal an unconventional thermal instability mechanism in this class of materials, which operates without the assistance of triple junctions. The mechanism can be rationalized by that thermally induced pinch off occurs as the result of bimetal interface faceting and can trigger a classic Rayleigh instability.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Injection of auxiliary electrons for increasing the plasma density in highly charged and high intensity ion sources

Different electron guns based on cold- or hot-cathode technologies have been developed since 2009 at INFN for operating within ECR plasma chambers as sources of auxiliary electrons, with the aim of boosting the source performances by means of a higher plasma lifetime and density. Their application to microwave discharge ion sources, where plasma is not confined, has required an improvement of the gun design, in order to “screen” the cathode from the plasma particles. Experimental tests carried out on a plasma reactor show a boost of the plasma density, ranging from 10% to 90% when the electron guns are used, as explained by plasma diffusion models.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Comparison of the Microstructure and Flux Pinning Properties of Polycrystalline YBa{sub 2}Cu{sub 3}O{sub 7-d} Containing Zn{sub 0.95}Mn{sub 0.05}O or Al{sub 2}O{sub 3} Nanoparticles

Here we compare the microstructure and flux pinning properties of polycrystalline YBa{sub 2}Cu{sub 3}O{sub 7-d} (Y-123 or YBCO) containing either Al{sub 2}O{sub 3} or Zn{sub 0.95}Mn{sub 0.05}O nanoparticles. Samples were prepared using a standard solid-state reaction process, and nanoparticles were added up to a concentration of 0.1 wt%. The crystal structure, microstructure, electrical and magnetic properties were analyzed using X-ray diffraction, scanning electron microscopy and transmission electron microscopy (TEM), and electrical resistivity and DC magnetization measurements, respectively. TEM observations showed that the addition of Zn{sub 0.95}Mn{sub 0.05}O resulted in a high density of fine twins and a variety of interacting microstructures, while Al{sub 2}O{sub 3} addition resulted in a high density of Al-rich nanoscale inhomogeneities embedded in the Y-123 matrix. Flux pinning forces were determined, and predominant pinning mechanisms in the prepared samples were proposed. We evaluated the superconducting properties of YBCO considering the effects of adding insulating or magnetic nanoparticles.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Large dielectric constant, high acceptor density, and deep electron traps in perovskite solar cell material CsGeI 3

Here we report that many metal halides that contain cations with the ns 2 electronic configuration have recently been discovered as high-performance optoelectronic materials. In particular, solar cells based on lead halide perovskites have shown great promise as evidenced by the rapid increase of the power conversion efficiency. In this paper, we show density functional theory calculations of electronic structure and dielectric and defect properties of CsGeI 3 (a lead-free halide perovskite material). The potential of CsGeI 3 as a solar cell material is assessed based on its intrinsic properties. We find anomalously large Born effective charges and a large static dielectric constant dominated by lattice polarization, which should reduce carrier scattering, trapping, and recombination by screening charged defects and impurities. Defect calculations show that CsGeI 3 is a p-type semiconductor and its hole density can be modified by varying the chemical potentials of the constituent elements. Despite the reduction of long-range Coulomb attraction by strong screening, the iodine vacancy in CsGeI3 is found to be a deep electron trap due to the short-range potential, i.e., strong Ge–Ge covalent bonding, which should limit electron transport efficiency in p-type CsGeI 3 . This is in contrast to the shallow iodine vacancies found in several Pb and Sn halide perovskites (e.g., CH 3 NH 3 PbI 3 , CH 3 NH 3 SnI 3 , and CsSnI 3 ). The low-hole-density CsGeI 3 may be a useful solar absorber material but the presence of the low-energy deep iodine vacancy may significantly reduce the open circuit voltage of the solar cell. Still, on the other hand, CsGeI 3 may be used as an efficient hole transport material in solar cells due to its small hole effective mass, the absence of low-energy deep hole traps, and the favorable band offset with solar absorber materials such as dye molecules and CH 3 NH 3 PbI 3 .

36 MATERIALS SCIENCE↗