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NASA NTRS2022

Quantifying Energy Release in Solar Flares and Solar Eruptive Events

Solar flares and the often associated solar eruptive events serve as an outstanding laboratory to study the magnetic reconnection and the associated energy release and conversion processes under plasma conditions difficult to reproduce in the laboratory, and with considerable spatiotemporal details not possible elsewhere in the universe. In the past decade, thanks to advances in multiwavelength imaging spectroscopy, as well as developments in theories and numerical modeling, significant progress has been made in improving our understanding of solar flare/eruption energy release. In particular, broadband imaging spectroscopy at microwave wavelengths offered by the Expanded Owens Valley Solar Array (EOVSA) has enabled the revolutionary capability of measuring the time-evolving coronal magnetic fields at or near the flare reconnection region. However, owing to EOVSA’s limited dynamic range, imaging fidelity, and angular resolution, such measurements can only be done in a region around the brightest source(s) where the signal-to-noise is sufficiently large. In this white paper, after a brief introduction to the outstanding questions and challenges pertinent to magnetic energy release in solar flares and eruptions, we will demonstrate how a next-generation radio facility with many (∼100–200) antenna elements can bring the next revolution by enabling high dynamic range, high fidelity broadband imaging spectropolarimetry along with a sub-second time resolution and arcsecond level angular resolution. We recommend to prioritize the implementation of such a ground-based instrument within this decade. We also call for facilitating multi-wavelength, multi-messenger observations and advanced numerical modeling in order to achieve a comprehensive understanding of the “system science” of solar flares and eruptions.

Bin Chen↗
NASA NTRS2024

Key Perseverance Sampling Locations for the Ancient Martian Crust and Implications for Mars Science

Since Feb 2021, the Perseverance rover has collected samples in the Jezero crater. The plan baselined at the 2018 landing site selection, subsequently further developed by the Mars-2020 team, and presented to the Decadal Survey included the exploration and sampling of the Jezero crater rim and the Nili Planum area, a rock record that is important to preserving the science return of the endeavor. Specifically, the science team identified the following prioritized science objectives aligned with community objectives that are not covered by the current sample cache: 1) Investigate the habitable environments with potential biosignatures from a more ancient time interval and from a diverse set of geological environments (incl. exposed subsurface) than the Jezero crater sedimentary deposits (Fig. 2). (2) Determine radioisotopic ages for well-defined craterretaining surfaces and/or the Isidis basin impact event. (3) Characterize ancient aqueous environments to study climate, environmental transitions, and habitability on ancient Mars. (4) Investigate planetary accretion, crustal evolution, and dynamo activity through analysis and sampling of igneous lithologies. (5) Study the geology of basin-forming impacts. In addition, for the Jezero rim and any Jezero ejecta: (6) Analyze Jezero impactites for potentially habitable hydrothermal environments and radioisotopic dating of the Jezero crater formation. From 2018 to now, we used a combination of High Resolution Imaging Experiment (HiRISE) and Compact Reconnaissance Imaging Spectrometer for Mars (CRISM) data to further characterize Jezero rim and Nili Planum, culminating in our prioritized sample location recommendations: (1) Monument Valley and (2) Northwest Jezero rim.

Mars sample return↗
DOE OSTI2020

Measurement of engine-oil fuel dilution using laser induced florescence spectroscopy

An optical diagnostic, based on laser-induced fluorescence (LIF), has been developed for on-engine measurements of real-time fuel dilution of engine oil, or fuel in oil (FiO). Fuel dilution of oil is believed to be one of the underlying mechanisms that promotes low speed pre-ignition (LSPI) during high-load engine operations. While standard (e.g., ASTM D3524-90) methods are not capable of transient measurements, the LIF technique resolves transient dilution on the minutes time scale, making it possible to study the relation between FiO and LSPI. The measurement is based on adding a dye (ca. 500 ppm) to the fuel and monitoring for its presence in the oil via LIF. The instrument contains a 532-nm laser diode, and a spectrometer to resolve the LIF spectra. A fiber-optic assembly links the instrument to the engine measurement location; the probe is in a Y-configuration with the six fibers around one on a common probe end that connects to the engine; the Y-assembly legs are connected to the instrument; the two legs are the six fibers for transporting the laser light, and the single fiber for the fluorescence. We have expanded on our previous work (Parks et al, SAE paper 2007-01-4108, 2007), by demonstrating the diagnostic technique with to measure transient oil dilution on a 2.0-liter GM ECOTEC LNF single cylinder SI engine. The proposed LIF diagnostic will be critical in studying oil-dilution correlation with LSPI events.

Neupane, Sneha↗
DOE OSTI2020

Quantifying the impact of climate change on erosion - 20397

The New York State Energy Research and Development Authority (NYSERDA) is the owner of the Western New York Nuclear Service Center (WNYNSC), a 1,351-ha (3,338-ac) site located approximately 48 km (30 mi) south of Buffalo, New York. In 1962, Nuclear Fuel Services, Inc. (NFS) entered into Agreements with the Atomic Energy Commission and New York State to construct the first commercial reprocessing plant of nuclear fuel in the United States. NFS, a private company, built and operated the spent fuel reprocessing plant and waste disposal facilities, processing 640 Mg (metric tons, or 705 short tons) of spent nuclear fuel from 1966 to 1972 under an Atomic Energy Commission license. Nuclear fuel reprocessing operations ended in 1972 and never reopened, leaving behind radioactive and chemical wastes. Erosion can play an important role in the fate and transport of waste at sites where disposal of long-lived waste is anticipated. The statistical characterization of key processes related to erosion is essential to the understanding of site stability through time. One of the key processes governing erosion is extreme precipitation and it is critical that trends in the distribution of extreme precipitation events through time be represented. The evidence of climate change is increasingly well documented and projected impacts on extreme precipitation events should be incorporated in performance assessment studies when relevant. Not evaluating future climate states in a performance assessment is contradictory to good modeling practice. Specifically, excluding climate change limits development of modeling information that could aid in effective decision making. The current climate literature provides both observational evidence and climate model projections of climate trends and/or climate change in the late 20. and early 21. centuries for North America and the northeast United States. In this work, this information was used to assess the impacts of potential changes in climate on erosion processes. The goal was to understand how projections of future climate relate to the performance of the WNYNSC through time. In the first stage of this work multi-temporal historical aerial images were analyzed in conjunction with orthophotography and Lidar data to develop probability distributions for variables representing important erosion processes. The information from these analyses was then used in conjunction with simulated data from the West Valley Erosion Working Group (EWG). Analysis of EWG simulations provides estimates for the change in erosion rates through time that is driven by changes in climate. The time-varying rates of erosion change were applied to the historical aerial imagery data in order to inform time-varying rates of erosion that are driven by changes in climate. Ultimately, this process resulted in the identification of locations for features like gully heads using both the Lidar dataset and projection of the estimated location from the historical aerial photo under consideration back to the Lidar dataset. The distance between the estimate of the location from the historical image and that of the Lidar dataset was the estimated distance the feature has moved. This distance was then divided by the number of years between the Lidar dataset and the year of the historical aerial image of interest to get a rate of movement through time. This was done for several dozen points on each historical aerial image. The analyses from the EWG were used to characterize the relative impact of climate change on the erosion rates. This relative impact was quantified by comparing the LEM based estimates of erosion that were derived using historical climate data with LEM based estimates of erosion that were derived using projections of future climate. The relative increase in the erosion rates was then applied to the historical estimates of erosion derived from the analysis of the historical aerial imagery. This approach was used since the LEM-based estimated of the historical erosion rates from the past century have a bias towards underestimating erosion. This underestimation is hypothesized to be a consequence of an inability of the LEMs to account for the impacts of land-use change (i.e. deforestation) which had been shown to significantly increase erosion in similar Northern hardwood forest ecosystems. In summary, gully head retreat rate and gully widening rate were characterized using statistical probability distributions from the historical aerial image analysis. Simulated data from the EWG was used to estimate the climatically-driven changes in erosion rates through time. The changes through time from the EWG were applied to the gully head retreat rate and gully widening rate characterized using the historical aerial image analysis. This information can be used to inform PPA models to project future risks from a given site. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2025

Rare Lepton Decays and Differentiable Hadronization Models - From Signatures of New Physics to Data-driven Event Generation

This dissertation is partitioned into two parts: phenomenological studies focused on rare lepton decays as probes of heavy and light new physics, and the development of differentiable, data-driven hadronization models. Part I develops the phenomenology of new physics signatures stemming from rare charged lepton flavor violating decays probed by experiments at the intensity frontier. These include interactions mediated by both high-scale effective operators and light new physics, manifesting in multi-lepton final states ($\mu \to 5e$), elastic nuclear transitions ($\mu \to e$ conversion), baryon-number-violating muon capture, and time-dependent signals from ultralight dark matter ($\mu \to e \phi, \tau \to \ell \phi$). Part II develops two distinct strategies for advancing differentiable and data-driven hadronization models. One involves comprehensive reweighting frameworks for hadronization that enable efficient uncertainty estimation, facilitate parameter tuning, and interface naturally with differentiable programming paradigms. The other introduces machine-learning-based methods for extracting microscopic fragmentation dynamics directly from macroscopic observables through the deformation of existing models -- effectively providing solutions to the inverse problem of hadronization. Altogether, these studies advance the interpretability, flexibility, and precision of theoretical predictions for both high-intensity and high-energy experiments.

Menzo, Tony [Cincinnati U.] (ORCID:000000022013457↗
NASA NTRS2005

Correlation Between Low Frequency Auroral Kilometric Radiation (AKR) and Auroral Structures

Auroral Kilometric Radiation (AKR) is a radio wave emission that has long been associated with auroral activity. AKR is normally observed in the frequency range from -60 - 600 kHz. Low frequency AKR (or LF-AKR) events are characterized as a rapid extension of AKR related emissions to 30 kHz or lower in frequency for typically much less than 10 minutes. LF-AKR emissions predominantly occur within a frequency range of 20 kHz - 30 kHz, but there are LF-AKR related emissions that reach to a frequency of 5 kHz. This study correlates all instances of LF-AKR events during the first four years of observations from the IMAGE spacecraft's Radio Plasma Imager (WI) instrument with auroral observations from the wideband imaging camera (WIC) onboard IMAGE. The correlation between LF-AKR occurrence and WIC auroral observations shows that in the 295 confirmed cases of LF-AKR emissions, bifurcation of the aurora is seen in 74% of the cases. The bifurcation is seen in the dusk and midnight sectors of the auroral oval, where AKR is believed to be generated. The polarization of these LF-AKR emissions has yet to be identified. Although LF-AKR may not be the only phenomena correlated with bifurcated auroral structures, bifurcation will occur in most instances when LF-AKR is observed. The LF-AKR emissions may be an indicator of specific auroral processes sometimes occurring during storm-time conditions in which field-aligned density cavities extend a distance of perhaps 5-6 RE tailward from the Earth for a period of 10 minutes or less.

Paxamickas, Katherine A.↗
NASA NTRS2001

Monthly Variability in Upper Ocean Biogeochemistry due to Mesoscale Eddy Activity in the Sargasso Sea

A comparison of monthly biogeochemical measurements made from 1993 to 1995, combined with hydrography and satellite altimetry, was used to observe the impacts of nine eddy events on primary productivity and particle flux in the Sargasso Sea. Measurements of primary production, thorium-234 flux, nitrate+nitrite, and photosynthetic pigments made at the US JGOFS Bermuda Atlantic Time-series Study (BATS) site were used. During the three years of this study, four out of six high thorium-234 flux events over 1000 dpm/sq m/d occurred during the passage of an eddy. Primary production nearly as high as the spring bloom maximum was observed in two modewater eddies (May 1993 and July 1995). The 1994 spring bloom at BATS was suppressed by the passage of an anticyclone. Distinct phytoplankton community shifts were observed in mode-water eddies, which had an increased percentage diatoms and dinoflagelletes, and in cyclones, which had an increased percentage cyanobacteria (excluding Prochlorococcus). The difference in the observations of mode-water eddies and cyclones may result from the age of the eddy, which was very important to the biological response. In general, eddies that were one to two months old elicited a large biological response; eddies that were three months old may show a biological response and were accompanied by high thorium flux measurements, eddies that were four months old or older did not show a biological response or high thorium flux. Our conceptual model depicting the importance of temporal changes during eddy upwelling and decay fit the observations well in all 7 upwelling eddies. Additional information is needed to determine the importance of deeper mixed layers and winter mixing to the magnitude of the eddy impacts. Also, sampling generally captured only the beginning, end, and /or edge of an eddy due to the monthly to semi-monthly frequency of the measurements made at BATS. Lagrangian studies, higher resolution time-series, and/or more spatial coverage is needed to provide additional information for improved C and N budgets in the Sargasso Sea and to complete our understanding of the temporal changes that occur in an eddy.

Sweeney, Erin N.↗
NASA NTRS2001

Monthly Variability in Upper Ocean Biogeochemistry Due to Mesoscale Eddy Activity in the Sargasso Sea

A comparison of monthly biogeochemical measurements made from 1993 to 1995, combined with hydrography and satellite altimetry, was used to observe the impacts of nine eddy events on primary productivity and particle flux in the Sargasso Sea. Measurements of primary production, thorium-234 flux, nitrate+nitrite, and photosynthetic pigments made at the US JGOFS Bermuda Atlantic Time-Series Study (BATS) site were used. During the three years of this study, four out of six high thorium-234 flux events over 1000 dpm/sq m/d occurred during the passage of an eddy. Primary production nearly as high as the spring bloom maximum was observed in two mode-water eddies (May 1993 and July 1995). The 1994 spring bloom at BATS was suppressed by the passage of an anticyclone. Distinct phytoplankton community shifts were observed in mode-water eddies, which had an increased percentage diatoms and dinoflagelletes, and in cyclones, which had an increased percentage cyanobacteria (excluding Prochlorococcus). The difference in the observations of mode-water eddies and cyclones may result from the age of the eddy, which was very important to the biological response. In general, eddies that were one to two months old elicited a large biological response; eddies that were three months old may show a biological response and were accompanied by high thorium flux measurements; eddies that were four months old or older did not show a biological response or high thorium flux. Our conceptual model depicting the importance of temporal changes during eddy upwelling and decay fit the observations well in all seven upwelling eddies. Additional information is needed to determine the importance of deeper mixed layers and winter mixing to the magnitude of the eddy impacts. Also, sampling generally captured only the beginning, end, and/or edge of an eddy due to the monthly to semi-monthly frequency of the measurements made at BATS. Lagrangian studies, higher resolution time-series, and/or more spatial coverage is needed to provide additional information for improved C and N budgets in the Sargasso Sea and to complete our understanding of the temporal changes that occur in an eddy.

Sweeney, Erin N.↗
NASA NTRS1999

A LIS Validation Study at the KSC-ER using LDAR and Field Mill Data

The chance of having the TRMM satellite pass over east central Florida when there is lightning over the NASA Kennedy Space Center (KSC) and USAF Eastern Range (ER) is small; however, such a condition did occur on September 21, 1998 (Day 264). Starting at about 20:40 GMT, the Lightning Imaging Sensor (LIS) reported 5 flashes during a 90 second interval that the KSC-ER was within the sensor field of view. Ground-based instrumentation, the Lightning Detection and Ranging (LDAR) system and a network of electric field mills (FM), detected 6 flashes in the same interval. In this paper, we will compare the times and locations of the optical pulses that were detected by LIS with the times and locations of RF sources (LDAR) and the charges that were deposited by the flash (FM network). We will show that LIS responded to all flashes that the LDAR and FM network detected; however, two discharges that were separated by less than 1 second in time and by about 10 km in space were grouped as one flash by the LIS data processing algorithm. In spite of the fact that all flashes occurred near the edge of the LIS field of view, the locations of the LIS events were consistent with both the LDAR and FM locations (the latter are usually within 1-2 kilometers of each other and often are co-located). Two of the 5 flashes reported by LIS were shifted north by about 8 km from the corresponding LDAR and FM locations. The LIS flash times tended to be after the first LDAR pulse was detected and before the last, and the integrated light signal (per LIS event) was surprisingly constant over the 5 flashes that were detected by LIS. In the future, we plan to study more correlated events and will try to determine whether and how the LIS light signal is related to the charge transfer in the flash and/or the number and spatial extent of RF sources.

Koshak, William J.↗
NASA NTRS2023

How Have Hydrological Extremes Changed Over the Past 20 Years?

Severe floods and droughts, including their back-to-back occurrences (weather whiplash), have been increasing in frequency and severity around the world. Improved understanding of systematic changes in hydrological extremes is essential for preparation and adaptation. In this study, we identified and quantified extreme wet and dry events globally by applying a clustering algorithm to terrestrial water storage (TWS) data from the Gravity Recovery and Climate Experiment (GRACE) and GRACE Follow-On (FO). The most intense events, ranked using an intensity metric, often reflect impacts of large-scale oceanic oscillations such as El Niño–Southern Oscillation and consequences of climate change. The severity of both wet and dry events, represented by standardized TWS anomalies, increased significantly in most cases, likely associated with intensification of wet and dry weather regimes in a warmer world, and consequently, exhibited strongest correlation with global temperature. In the Dry climate, the number of wet events decreased while the number of dry events increased significantly, suggesting a drying trend that may be attributed to climate variability and possible increases in irrigation and reliance on groundwater. In the Continental climate where temperature has risen faster than global average, dry events increased significantly. Characteristics of extreme events often showed strong correlations with global temperature, especially when averaged over all climates. These results suggest changes in hydrological extremes and underscore the importance of quantifying total water storage changes when studying hydrological extremes. Extending the GRACE/FO record, which spans 2002 to the present, is essential to continuously tracking changes in TWS and hydrological extremes.

Bailing Li↗
NASA NTRS1974

Geomagnetic background events observed by Uhuru

Problems due to sporadic background events observed by Uhuru (Small Astronomy Satellite - A) do not compromise the study of discrete X-ray sources. Nevertheless, direct particle effects and auroral type X-ray events in the atmosphere may occasionally occur. Therefore, even on the geomagnetic equator, an experiment must be prepared to recognize and eliminate such events when the ultimate level of sensitivity is desired. The test equipment contained in the satellite and the orbital mechanics of Small Astronomy Satellite - A are described. The sporadic events which were observed by the satellite are analyzed.

Schwartz, D. A.↗
NASA NTRS1992

Nonadiabatic processes in the Earth's magnetotail

The challenge of the assumption of an adiabatic equation of state for the plasma sheet made in several studies of quiet time convection and expansive phase activity is addressed. The observed plasma pressures at distances of approximately 10 RE are less than that predicted by adiabatic convection by over an order of magnitude. Studies of the local plasma properties for individual events as well as an ensemble of all quiet time plasma sheet samples during two years of ISEE coverage show that the polytropic index is below 5/3, and on occasion may be less than unity. During substorm activity the main effect of the plasma sheet is an increase in plasma temperature. This is seen both in statistical and case studies of individual substorms. The nature of the heating process is nonadiabatic, as evidenced by the anticorrelation between changes in plasma density and temperature. These recent observations of nonadiabatic behavior emphasize thermodynamic processes in the magnetosphere, an area which has been largely ignored.

Huang, C. Y.↗
NASA NTRS1988

A regional perspective on the palynofloral response to K-T boundary event(s) with emphasis on variations imposed by the effects of sedimentary facies and latitude

Palynological studies deal with fossil reproductive bodies that were produced by fully functioning plants, whereas most faunal studies are based on death assemblages. Therefore, changes in pollen and spore assemblages cannot be used directly as evidence of catastrophic mass killings but only to indicate changes in ecological conditions. The impact of the Cretaceous-Tertiary boundary event on terrestrial plant communities is illustrated by the degree, rate and selectivity of change. As in most classical palynological studies, the degree of change is expressed in terms of relative abundance and changes in species diversity. It is recognized that sampling interval and continuity of the rock record within individual sections can affect the percieved rate of change. Even taking these factors into account, a gradual change in relative abundance and multiple levels of apparent extinctions, associated with the interval bounding the K-T boundary, can be demonstrated. Climatic change, which locally exceeds the tolerance of individual species, and the possible loss of a group of pollinating agents are examined as possible explanations for the selectivity of apparent extinctions and/or locally truncated occurrences. The aspects of change are demonstrated with data from four different K-T boundary localities in Western Canada between paleolatitudes 60 and 75 deg north. Together, the four localities discussed allow changes imposed by latitude and differences in the depositional environment be isolated from the boundary event itself which is reflected by the truncated ranges of several species throughout the region of study. What must be recognized is that variations in the response of vegetation to the K-T boundary event(s) occurred throughout the Western Interior basin.

Sweet, A. R.↗
NASA NTRS2014

Geostationary Coastal and Air Pollution Events (GeoCAPE) Wide Angle Spectrometer (WAS)

The GeoCAPE Wide Angle Spectrometer (WAS) Study was a revisit of the COEDI Study from 2012. The customer primary goals were to keep mass, volume and cost to a minimum while meeting the science objectives and maximizing flight opportunities by fitting on the largest number of GEO accommodations possible. Riding on a commercial GEO satellite minimizes total mission costs. For this study, it is desired to increase the coverage rate,km2min, while maintaining ground sample size, 375m, and spectral resolution, 0.4-0.5nm native resolution. To be able to do this, the IFOV was significantly increased, hence the wide angle moniker. The field of view for COEDI was +0.6 degrees or (2048) 375m ground pixels. The WAS Threshold (the IDL study baseline design) is +2.4 degrees IDL study baseline design) is +2.4 degrees.

pointing and jitter↗
DOE OSTI2025

Subsurface heatwaves in lakes

Abstract Lake heatwaves (extreme hot water events) can substantially disrupt aquatic ecosystems. Although surface heatwaves are well studied, their vertical structures within lakes remain largely unexplored. Here we analyse the characteristics of subsurface lake heatwaves (extreme hot events occurring below the surface) using a spatiotemporal modelling framework. Our findings reveal that subsurface heatwaves are frequent, often longer lasting but less intense than surface events. Deep-water heatwaves (bottom heatwaves) have increased in frequency (7.2 days decade −1 ), duration (2.1 days decade −1 ) and intensity (0.2 °C days decade −1 ) over the past 40 years. Moreover, vertically compounding heatwaves, where extreme heat occurs simultaneously at the surface and bottom, have risen by 3.3 days decade −1 . By the end of the century, changes in heatwave patterns, particularly under high emissions, are projected to intensify. These findings highlight the need for subsurface monitoring to fully understand and predict the ecological impacts of lake heatwaves.

Environmental Sciences & Ecology↗
DOE OSTI2021

Simultaneously characterization of tumoral angiogenesis and vasculogenesis in stem cell-derived teratomas

Highlights: • CAM supports the growth and differentiation of embryonic stem cells into teratomas. • In teratomas, parenchymal Embryonic stem cell-derived endothelial cells form chimeric vessels with stromal endothelial cells. • CAM allows the simultaneously characterization of vasculogenesis and angiogenesis processes. Tumor neovascularization may occur via both angiogenic and vasculogenic events. In order to investigate the vessel formation during tumor growth, we developed a novel experimental model that takes into account the differentiative and tumorigenic properties of Embryonic Stem cells (ESCs). Leukemia Inhibitory Factor-deprived murine ESCs were grafted on the top of the chick embryo chorionallantoic membrane (CAM) in ovo. Cell grafts progressively grew, forming a vascularized mass within 10 days. At this stage, the grafts are formed by cells with differentiative features representative of all three germ layers, thus originating teratomas, a germinal cell tumor. In addition, ESC supports neovascular events by recruiting host capillaries from surrounding tissue that infiltrates the tumor mass. Moreover, immunofluorescence studies demonstrate that perfused active blood vessels within the tumor are of both avian and murine origin because of the simultaneous occurrence of angiogenic and vasculogenic events. In conclusion, the chick embryo ESC/CAM-derived teratoma model may represent a useful approach to investigate both vasculogenic and angiogenic events during tumor growth and for the study of natural and synthetic modulators of the two processes.

60 APPLIED LIFE SCIENCES↗
NASA NTRS2017

Quantifying Black Carbon Deposition Over the Greenland Ice Sheet from Forest Fires in Canada

Black carbon (BC) concentrations observed in 22 snowpits sampled in the northwest sector of the Greenland ice sheet in April 2014 have allowed us to identify a strong and widespread BC aerosol deposition event, which was dated to have accumulated in the pits from two snow storms between 27 July and 2 August 2013. This event comprises a significant portion (57 on average across all pits) of total BC deposition over 10 months (July 2013 to April 2014). Here we link this deposition event to forest fires burning in Canada during summer 2013 using modeling and remote sensing tools. Aerosols were detected by both the Cloud-Aerosol Lidar with Orthogonal Polarization (on board CALIPSO) and Moderate Resolution Imaging Spectroradiometer (Aqua) instruments during transport between Canada and Greenland. We use high-resolution regional chemical transport modeling (WRF-Chem) combined with high-resolution fire emissions (FINNv1.5) to study aerosol emissions, transport, and deposition during this event. The model captures the timing of the BC deposition event and shows that fires in Canada were the main source of deposited BC. However, the model underpredicts BC deposition compared to measurements at all sites by a factor of 2100. Underprediction of modeled BC deposition originates from uncertainties in fire emissions and model treatment of wet removal of aerosols. Improvements in model descriptions of precipitation scavenging and emissions from wildfires are needed to correctly predict deposition, which is critical for determining the climate impacts of aerosols that originate from fires.

albedo↗