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NASA NTRS1984

Mineralogic and petrologic studies of meteorites and lunar samples

During a 13 year period beginning in 1971, the Extraterrestrial Petrology Group examined lunar soils from all 6 Apollo missions and those returned by the Soviet Luna 16, Luna 20, and Luna 24 missions. In addition, the properties and apparent origin of the carbonaceous chondrites were examined. Chondrules, calcium-aluminum-rich inclusions (CAI) and the fine grained matrix materials that accompany chondrules and CAI's in primitive meteorites were investigated. The effects of planetary hydrothermal alteration of matrix materials in the C1 chondrite was also investigated. Full length papers and extended abstracts published during the grant are listed chronologically.

Wood, J. A.↗

NASA NTRS1983

Isotopically anomalous nitrogen in primitive meteorites

The extreme enrichement in N-14 (up to 48 percent) found in acid-resistant residues of the Allende and Murchison meteorites cannot be attained by normal solar system processes and must therefore be due to stellar nucleosynthesis. Consequently the xenon component enriched in the heavy isotopes associated with the light nitrogen very probably was made by stellar nucleosynthesis rather than by fission of an extinct superheavy element.

Lewis, R. S.↗

NASA NTRS1983

Barium isotopes in Allende meteorite - Evidence against an extinct superheavy element

Carbon and chromite fractions from the Allende meteorite that contain isotopically anomalous xenon-131 to xenon-136 (carbonaceous chondrite fission or CCF xenon) at up to 5 x 10 to the 11th atoms per gram show no detectable isotopic anomalies in barium-130 to barium-138. This rules out the possibility that the CCF xenon was formed by in situ fission of an extinct superheavy element. Apparently the CCF xenon and its carbonaceous carrier are relics from stellar nucleosynthesis.

Lewis, R. S.↗

NASA NTRS1983

The origin of SNC meteorites - An alternative to Mars

The possibility that certain very young meteorites originated as impact melts on a large asteroid or asteroids is investigated. Calculations of the thermal evolution of impact melt show that the solidification time should be long enough to produce igneous or quasi-cumulate textures within rocks if the crater is large enough and if the initial clast concentration is low, at least in some portion of the melt sheet. The number of collisions within the asteroid belt which would produce craters of the requisite size is calculated. Using an estimate of the current size distribution of asteroids, it is found that over 3000 such collisions should have occurred during the lifetime of the solar system. Excavation and ejection of the solidified melt by a subsequent impact would be dynamically easy because of the low escape velocities of even the largest asteroids but improbable because of the depth that must be sampled. A second, sufficiently large impact is rare, so only the products of one such double event have been obtained up to now.

Vickery, A. M.↗

NASA NTRS1983

Nickel-iron spherules in tektites - Non-meteoritic in origin

The concentrations of several diagnostic trace elements were determined in two comparatively large NiFe spherules extracted from tektites. The purpose of the study was to obtain some clues about the chemistry of the projectile that is presumed responsible for the formation of these tektites. However, the trace element pattern is distinctly terrestrial implying that the spherules are the result of in-situ reduction of the host rock and are not meteoritic in origin.

Ganapathy, R.↗

NASA NTRS1983

The composition of asteroid 2 Pallas and its relation to primitive meteorites

High resolution spectroscopic observations of asteroid 2 Pallas from 1.7-3.5 microns are reported. These data are combined with previous measurements from 0.4-1.7 microns to interpret Pallas' surface mineralogy. Evidence is found for low-Fe(2+) hydrated silicates, opaque components, and low Fe(2+) anhydrous silicates. This assemblage is very similar to carbonaceous chondrite matrix material such as is found in type CI and CM meteorites, but it has been subjected to substantial aqueous alteration and there is a major extraneous anhydrous silicate component. This composition is compared to that of asteroid 1 Ceres. Although there are substantial differences in their broad band spectral reflectances it appears that both asteroids are genetically related to know carbonaceous chondrites.

Larson, H. P.↗

NASA NTRS1984

'Fluffy' Type A Ca-, Al-rich inclusions in the Allende meteorite

Inclusions called 'fluffy' Type A's or FTA's in the Allende meteorite are examined as possible candidates for relict vapor-solid condensate grains, remaining from the original solar nebula. Type A inclusions are characterized by abundant melilite and absence of primary anorthite and titaniferous pyroxene. Fluffy Type A's were probably loosely bound clumps of crystals drifting in the solar nebula, analogous to dustballs or snowflakes. Polished thin sections of all samples were studied optically and with a JEOL JSM-35 scanning electron microscope. It is reasonably clear that neither whole FTA's nor constituent nodules of the coarser grained ones were ever molten. Despite solid-state recrystallization which has affected these inclusions to varying degrees, the coarser grained material remaining in many of them is probably a relic of vapor-solid condensation in the solar nebula.

Macpherson, G. J.↗

NASA NTRS1983

The Ne-21 production rate in stony meteorites estimated from Be-10 and other radionuclides

The Be-10 contents of 28 stony meteorites with known Ne-21 contents range from 0.97 to 23 dpm/kg and give an average Ne-21 production rate (P sub 21) of (0.28 + or - 0.02) x 10 to the -8th cu cm STP/g-My for shielding conditions corresponding to Ne-22/Ne-21 = 1.114 in an H-chondrite. This P sub 21 (Be) agrees with others' P sub 21 based on Na-22, Kr-81, and Mn-53, but not an Al-26. Temporal variations in the cosmic ray flux do not explain the disagreement satisfactorily; major errors in the radionuclide half-lives are not indicated. The discrepancy seems rooted in the data selection and the difficulties of making accurate corrections for shielding, chemical composition and other sources of variability.

Moniot, R. K.↗

NASA NTRS1982

Anomalies within the system - Rochechouart target rock meteorite

Contaminated impact crater formations are pertinent to the study of meteoritic contamination at the Cretaceous-Tertiary boundary and other Ir-enriched layers. Target mixing considerations and volumetric estimates of Rochechouart breccias are presently combined with the geochemistry of both major and siderophile trace elements, to evaluate how the chemistry of the preserved target rock-projectile mixture evolved since deposition. Over 99 percent of the mass of extraterrestrial Ir and Os in preserved formations at Rochechouart is located in suevite-like breccias and impact melts. Hydrothermal alteration and/or weathering are the most likely processes to explain both major and trace element redistribution in Rochechouart formations.

Lambert, P.↗

NASA NTRS1984

Petrogenesis of the SNC (shergottites, nakhlites, chassignites) meteorites - Implications for their origin from a large dynamic planet, possibly Mars

Comprehensive chemical data are presented on the shergottites Shergotty, Zagami, Allan Hills (ALHA) 77005, and the new member Elephant Moraine (EETA) 79001 using results of sequential instrumental and radiochemical neutron activation analysis. The close relationship of the Antarctic shergotites indicates that ALHA 77005 is a residual source produced by incongruent melting of a source similar in bulk composition to EETA 79001A and that EETA 79001B and the interstitial phases in EETA 79001A are the melts produced by such melting episodes. The large ion lithophile LIL) trace element abundanced of the shergottites require variable but extensive degrees of nomodal melting of isotopically constrained parent sources. The SNG sources are consistent with their derivation by extensive fractionation of a primitive magma initially produced from a source having chondritic refractory LIL trace element abundances. Petrogenetic and age relationships among SNC meteorites suggest a single complex-provenance on a dynamic planet not unlike earth, probably Mars.

Smith, M. R.↗

NASA NTRS1982

Reflectance spectroscopy of diogenite meteorite types from Antarctica and their relationship to asteroids

Measurements of the spectral reflectance (0.4-2.5 microns) of three diogenite meteorites found in Antarctica are examined. Comparisons are made with previous measurements of diogenites in order to correlate the mineralogy and petrography with the spectral characteristics that can also be measured on solar system objects of unknown composition. Even though the Antarctic diogenites have the same spectral characteristics as other diogenites, there are measurable differences between all diogenite spectra. Bands caused by spin-forbidden transitions of Fe(2+) ions in pyroxene, which are identified for the first time in reflectance spectra of powdered samples, are revealed in an analysis of the spectra into sums of Gaussian components. It is shown from these laboratory measurements that spectral reflectance measurements of asteroids and other solar system objects made with the visible CVF (circular variable filter) spectrometer used for laboratory measurements can provide useful information on their surface composition.

Mcfadden, L. A.↗

NASA NTRS1984

Proposed structures for poorly characterized phases in C2M carbonaceous chondrite meteorites

A recent investigation of C2M carbonaceous chondrite meteorite matrices using electron microscopy and High-Resolution Transmission Electron Microscopy (HRTEM) has provided data on the structure and chemistry of Poorly Characterized Phases (PCP). It is suggested that a dominant matrix variety (10 A PCP) has a structure equivalent to iron-rich tochinilite (6Fe0.9S5/Fe, Mg//OHO2/), which consists of coherently intrastratified mackinawite and brucite sheets. In addition, it is proposed that 17 A PCP is a commensurate intergrowth of serpentine and tochinilite layers. Various forms of PCP observed in carbonaceous chondrites appear to be intergrowths of tochinilite, serpentine, and tochinilite-serpentine minerals.

Mackinnon, I. D. R.↗

NASA NTRS1984

The microstructure of minerals in coarse-grained Ca-Al-rich inclusions from the Allende meteorite

Transmission electron microscopy (TEM) is used to investigate the microstructure and microchemistry of minerals in Ca-Al-rich, coarse-grained inclusions (CAI) from the meteorite. The spinels contain only low to moderate dislocation densities and are characterized by a ubiquitous, fine black spotty texture that is thought to originate from a slightly nonstoichiometric composition. Whereas the Ti-Al-pyroxenes are relatively devoid of features, they contain veins of secondary phases apparently deposited in unhealed cracks. Chromite is identified in the veins, indicating transport of oxidized iron during alteration. The melilites show the greatest variety of microstructures and are the most heavily altered phase in CAI. High dislocation densities are common and the crystals exhibit considerable internal strain, suggesting that they have not been annealed.

Barber, D. J.↗

NASA NTRS1984

Compositional trends and cooling rates of group IVB iron meteorites

It is found, on the basis of new neutron activation data for group IVB, that log-element - log-Ni trends are best understood in terms of core formation and fractional crytstallizaion. The limited compositional range found in gorup IVB is thought to reflect the fact that, owing to the low concentrations of S, P, and C and the high concentration of Ni, the k sub x (the solid/liquid partition ratio) values are closer to unity than are those in other magmatic groups. Mean volatile abundances in group IVB are significantly lower than those found in any group of chondritic meteorites, indicating that these low abundances are not entirely the result of nebular processes and that planetary outgassing was also involved.

Rasmussen, K. L.↗

NASA NTRS1984

Early solar system aqueous activity - Sr isotope evidence from the Orgueil CI meteorite

The Sr isotopic composition and Rb-87/Sr-86 ratio have been measured in carbonates and sulfate separated from the Orgueil meteorite in order to determine the time when liquid water may have acted on the parent body. Both of the studied phases probably precipitated from aqueous solution. The results show that carbonate deposition occurred contemporaneously with parent body formation or shortly after it, probably within 100 Myr. On the other hand, at least some of the calcium sulfate seems to have been formed recently.

Macdougall, J. D.↗

NASA NTRS1984

Carbon isotope composition of low molecular weight hydrocarbons and monocarboxylic acids from Murchison meteorite

Carbon isotopic compositions have been measured for individual hydrocarbons and monocarboxylic acids from the Murchison meteorite, a C2 carbonaceous chondrite which fell in Australia in 1969. With few exceptions, notably benzene, the volatile products are substantially isotopically heavier than their terrestrial counterparts, signifying their extraterrestrial origin. For both classes of compounds, the ratio of C-13 to C-12 decreases with increasing carbon number in a roughly parallel manner, and each carboxylic acid exhibits a higher isotopic ratio than the hydrocarbon containing the same number of carbon atoms. These trends are consistent with the kinetically controlled synthesis of higher homologues from lower ones. The results suggest the possibility that the production mechanisms for hydrocarbons and carboxylic acids may be similar, and impose constraints on the identity of the reactant species.

Yuen, G.↗

NASA NTRS1984

Titanium isotopic anomalies in meteorites

Studies of Ti isotopic compositions have shown that virtually every Ca-Al-rich Allende inclusion contains anomalous Ti. The present investigation is concerned with the results of a study of Ti isotopic compositions in meteorites. One objective of the study is to evaluate the possibility of a relation between oxygen and Ti anomalies, while another objective is to explore questions regarding the origin of the Ti anomalies. A summary of the major experimental findings of the study of Ti isotopic compositions is also presented. It is noted that an assessment of the implications of the Ti results favors a chemical memory type of model in which products from various nucleosynthetic sources survive in mineral grains. Isotopic heterogeneities are then preserved due to incomplete mixing and/or equilibriation with the bulk of solar system matter. Strong arguments are found to exist against a pure late supernova injection model.

Niemeyer, S.↗

NASA NTRS1984

The influence of gravitational body force in meteoritic chondrule and lunar glass formation

The effects of gravitational body force must be considered in the formation of extraterrestrial materials such as meteoritic chondrules and lunar glasses. Solidification experiments conducted in microgravity as well as g values greater than Earth's gravitational force have demonstrated that gravitational force can have profound and sometimes unexpected effects upon the way materials solidify and, therefore, upon their physical and mechanical properties. Solutal, thermal and sedimentation effects differ from those experienced on Earth. Because buoyancy forces are reduced, materials of different densities may remain in close proximity. The spherical morphology of chondrules and many lunar glasses may reflect the tendency for free floating liquids to form spherical droplets in a microgravity environment, a form which minimizes surface energy. Under these conditions, surface energy forces dominate gravity forces. The formation of two common chondrule textures, barred and radiating chondrules, can be explained using observations from glass science.

Budka, P. Z.↗