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At least 1,549 records · Page 86
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Flat-band-induced itinerant ferromagnetism in RbCo 2 Se 2

ACo 2 Se 2 (A=K,Rb,Cs) is a homologue of the iron-based superconductor, AFe 2 Se 2 . From a comprehensive study of RbCo 2 Se 2 via measurements of magnetization, transport, neutron diffraction, angle-resolved photoemission spectroscopy, and first-principle calculations, we identify a ferromagnetic order accompanied by an orbital-dependent spin-splitting of the electronic dispersions. However, we identify the ordered moment to be dominated by a d x 2 –y 2 flatband near the Fermi level, which exhibits the largest spin splitting across the ferromagnetic transition, suggesting an itinerant origin of the ferromagnetism. In the broader context of the iron-based superconductors, we find this d x 2 –y 2 flatband to be a common feature in the band structures of both iron chalcogenides and iron pnictides, accessible via heavy electron doping.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Nonlinear electromagnetic formulation for particle-in-cell simulation of lower hybrid waves in toroidal geometry

An electromagnetic particle simulation model has been formulated and verified for nonlinear processes of lower hybrid (LH) waves in fusion plasmas. Electron dynamics are described by the drift kinetic equation using either kinetic momentum or canonical momentum. Ion dynamics are treated as the fluid system or by the Vlasov equation. Compressible magnetic perturbation is retained to simulate both the fast and slow LH waves. Numerical properties are greatly improved by using the electron continuity equation to enforce the consistency between electrostatic potential and vector potential, and by using the importance sampling scheme. The simulation model has been implemented in the gyrokinetic toroidal code (GTC), and verified for the dispersion relation and nonlinear particle trapping of the electromagnetic LH waves.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2018

Magnetic excitations of the Cu 2 + quantum spin chain in Sr 3 CuPtO 6

Here, we report the magnetic excitation spectrum as measured by inelastic neutron scattering for a polycrystalline sample of Sr 3 CuPtO 6 . Modeling the data by the 2+4 spinon contributions to the dynamical susceptibility within the chains, and with interchain coupling treated in the random phase approximation, accounts for the major features of the powder-averaged structure factor. The magnetic excitations broaden considerably as temperature is raised, persisting up to above 100 K and displaying a broad transition as previously seen in the susceptibility data. No spin gap is observed in the dispersive spin excitations at low momentum transfer, which is consistent with the gapless spinon continuum expected from the coordinate Bethe ansatz. However, the temperature dependence of the excitation spectrum gives evidence of some very weak interchain coupling.

1-dimensional spin chains↗
DOE OSTI2022

Whistler waves generated by nongyrotropic and gyrotropic electron beams during asymmetric guide field reconnection

Using a two-dimensional particle-in-cell simulation of asymmetric reconnection with a guide field whose strength is 0.3 times the reconnecting magnetic field, we study electron distribution functions and wave intensities in the diffusion region, focusing on the electron diffusion region (EDR). Wave activities with frequencies below the electron cyclotron frequency are observed, and these are whistler waves propagating almost anti-parallel to the magnetic field. The waves are concentrated near the magnetospheric separatrix away from the X line, but the wave activity also spreads through the EDR near the X line. The reconnection outflows are asymmetric in the outflow direction in the magnetospheric side, and the wave intensity is stronger in the side of the faster electron outflow. We study the whistler waves using the fast Fourier transform, analyses of electron velocity distribution functions, and the dispersion solver calculation. Along the magnetospheric separatrix in the stronger outflow side, highly anisotropic electron beams exist with super-Alfvénic drift speeds. The dispersion analysis shows that there are two modes: a temperature anisotropy mode and a beam mode. Outside the EDR, the whistler wave intensity is highest near the separatrix, but the wave intensity decreases if we move away from the separatrix toward the magnetic neutral line because of the increase in the electron population near zero parallel velocity. In the EDR, in the velocity plane perpendicular to the magnetic field, ring/crescent electron distribution functions are observed. Near the X-line, the wave power is enhanced where nongyrotropic electrons contribute to increase the perpendicular temperature anisotropy.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS2022

Whistler Waves Generated by Nongyrotropic and Gyrotropic Electron Beams During Asymmetric Guide Field Reconnection

Using a two-dimensional particle-in-cell simulation of asymmetric reconnection with a guide field whose strength is 0.3 times the reconnecting magnetic field, we study electron distribution functions and wave intensities in the diffusion region, focusing on the electron diffusion region (EDR). Wave activities with frequencies below the electron cyclotron frequency are observed, and these are whistler waves propagating almost anti-parallel to the magnetic field. The waves are concentrated near the magnetospheric separatrix away from the X line, but the wave activity also spreads through the EDR near the X line. The reconnection outflows are asymmetric in the outflow direction in the magnetospheric side, and the wave intensity is stronger in the side of the faster electron outflow. We study the whistler waves using the fast Fourier transform, analyses of electron velocity distribution functions, and the dispersion solver calculation. Along the magnetospheric separatrix in the stronger outflow side, highly anisotropic electron beams exist with super-Alfvénic drift speeds. The dispersion analysis shows that there are two modes: a temperature anisotropy mode and a beam mode. Outside the EDR, the whistler wave intensity is highest near the separatrix, but the wave intensity decreases if we move away from the separatrix toward the magnetic neutral line because of the increase in the electron population near zero parallel velocity. In the EDR, in the velocity plane perpendicular to the magnetic field, ring/crescent electron distribution functions are observed. Near the X-line, the wave power is enhanced where nongyrotropic electrons contribute to increase the perpendicular temperature anisotropy.

magnetic reconnection↗
DOE OSTI2023

Control of ternary alloy composition during remote epitaxy on graphene

Understanding the sticking coefficient σ, i.e., the probability of an adatom sticking to a surface, is essential for controlling the stoichiometry during epitaxial film growth. However, σ on monolayer graphene-covered surfaces and its impact on remote epitaxy are not understood. Here, using molecular-beam epitaxial growth of the magnetic shape memory alloy Ni 2 MnGa, we show that the sticking coefficients for metals on graphene-covered MgO (001) are less than one and are temperature and element dependent, as revealed by ion backscattering spectrometry and energy-dispersive x-ray spectroscopy. This lies in stark contrast with most transition metals sticking on semiconductor and oxide substrates, for which σ is near unity at typical growth temperatures (T < 800°C). By initiating growth below 400°C, where the sticking coefficients are closer to unity and wetting on the graphene surface is improved, we demonstrate the epitaxy of Ni 2 MnGa films with controlled stoichiometry that can be exfoliated to produce freestanding membranes. Straining these membranes tunes the magnetic coercive field. Finally, our results provide a route to synthesize membranes with complex stoichiometries whose properties can be manipulated via strain.

36 MATERIALS SCIENCE↗
DOE OSTI2012

RESOLVED MAGNETIC FIELD MAPPING OF A MOLECULAR CLOUD USING GPIPS

We present the first resolved map of plane-of-sky magnetic field strength for a quiescent molecular cloud. GRSMC 45.60+0.30 subtends 40 Multiplication-Sign 10 pc at a distance of 1.88 kpc, masses 16,000 M{sub Sun }, and exhibits no star formation. Near-infrared background starlight polarizations were obtained for the Galactic Plane Infrared Polarization Survey using the 1.8 m Perkins telescope and the Mimir instrument. The cloud area of 0.78 deg{sup 2} contains 2684 significant starlight polarizations for Two Micron All Sky Survey matched stars brighter than 12.5 mag in the H band. Polarizations are generally aligned with the cloud's major axis, showing an average position angle dispersion of 15 {+-} 2 Degree-Sign and polarization of 1.8 {+-} 0.6%. The polarizations were combined with Galactic Ring Survey {sup 13}CO spectroscopy and the Chandrasekhar-Fermi method to estimate plane-of-sky magnetic field strengths, with an angular resolution of 100 arcsec. The average plane-of-sky magnetic field strength across the cloud is 5.40 {+-} 0.04 {mu}G. The magnetic field strength map exhibits seven enhancements or 'magnetic cores'. These cores show an average magnetic field strength of 8.3 {+-} 0.9 {mu}G, radius of 1.2 {+-} 0.2 pc, intercore spacing of 5.7 {+-} 0.9 pc, and exclusively subcritical mass-to-flux ratios, implying their magnetic fields continue to suppress star formation. The magnetic field strength shows a power-law dependence on gas volume density, with slope 0.75 {+-} 0.02 for n{sub H{sub 2}} {>=}10 cm{sup -3}. This power-law index is identical to those in studies at higher densities, but disagrees with predictions for the densities probed here.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

Sol–gel method as a way of carbonyl iron powder surface modification for interaction improvement

This article presents a method for modification of carbonyl iron particles’ surface (CIP), (d{sub 50}=4–9 µm) by silica coatings obtained using the sol–gel method. Reaction parameters were determined to obtain dry magnetic powder with homogeneous silica coatings without further processing and without any by-product in the solid or liquid phase. This approach is new among the commonly used methods of silica coating of iron particles. No attempt has been made to cover a carbonyl iron surface by silica in a waste-free method, up to date. In the current work two different silica core/shell structures were made by the sol–gel process, based on different silica precursors: tetraethoxy-silane (TEOS) and tetramethoxy-silane (TMOS). The dependence between the synthesis procedure and thickness of silica shell covering carbonyl iron particles has been described. Surface morphology of the modified magnetic particles and the coating thickness were characterized with the use of scanning electron microscopy (SEM) and transmission electron microscopy (TEM). Determination of the physicochemical structure of the obtained materials was performed by the energy-dispersive X-ray spectroscope (EDS), and the infrared technique (IR). The surface composition was analyzed using X-ray photoelectron spectroscopy (XPS). Additionally, distribution of particle size was measured using light microscopy. The new, efficient process of covering micro-size CIP with a nanometric silica layer was shown. Results of a performed analysis confirm the effectiveness of the presented method. - Highlights: • Proper covering CIP by sol–gel silica layer avoids agglomeration. • A new solid waste-free method of CIP coating is proposed. • Examination of the properties of modified CIP in depends on washing process. • Coatings on CIP particles doesn’t change the magnetic properties of particles.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2011

ELECTROMAGNETIC THERMAL INSTABILITY WITH MOMENTUM AND ENERGY EXCHANGE BETWEEN ELECTRONS AND IONS IN GALAXY CLUSTERS

Thermal instability in an electron-ion magnetized plasma, which is relevant in the intragalactic medium of galaxy clusters, solar corona, and other two-component plasma objects, is investigated. We apply the multicomponent plasma approach where the dynamics of all species are considered separately through electric field perturbations. General expressions for the dynamical variables obtained in this paper can be applied over a wide range of astrophysical and laboratory plasmas also containing neutrals and dust grains. We assume that background temperatures of electrons and ions are different and include the energy exchange in thermal equations for electrons and ions along with the collisional momentum exchange in equations of motion. We take into account the dependence of collision frequency on density and temperature perturbations. The cooling-heating functions are taken for both electrons and ions. A condensation mode of thermal instability has been studied in the fast sound speed limit. We derive a new dispersion relation including different electron and ion cooling-heating functions and other effects mentioned above and find its simple solutions for growth rates in limiting cases. We show that the perturbations have an electromagnetic nature and demonstrate the crucial role of the electric field perturbation along the background magnetic field in the fast sound speed limit. We find that at the conditions under consideration, condensation must occur along the magnetic field while the transverse scale sizes can be both larger and smaller than the longitudinal ones. The results obtained can be useful for interpretating observations of dense cold regions in astrophysical objects.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Pseudogap in elemental plutonium

Electronic correlations associated with incipient magnetism have long been recognized as an important factor in stabilizing the largest atomic volume δ phase of plutonium, although their strength compared to those in the rare earths and neighboring actinides in the periodic table has largely remained a mystery. We show here using calorimetry measurements, together with prior detailed measurements of the phonon dispersion, that the 5f electrons of the δ phase reside in a pseudogapped state, accompanied by reductions in various physical properties below a characteristic temperature T* ≈ 100 K. The small characteristic energy scale of the pseudogapped state implies that the 5f electrons in plutonium are much closer to the threshold for localization and magnetic order than has been suggested by state-of-the-art electronic structure theory, revealing plutonium to be arguably the most strongly correlated of the elements.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2012

Multidimensional Nature of Molecular Organic Conductors Revealed by Angular Magnetoresistance Oscillations

Angle-dependent magnetoresistance experiments on organic conductors exhibit a wide range of angular oscillations associated with the dimensionality and symmetry of the crystal structure and electron energy dispersion. In particular, characteristics associated with 1, 2, and 3-dimensional electronic motion are separately revealed when a sample is rotated through different crystal planes in a magnetic field. Originally discovered in the TMTSF-based conductors, these effects are particularly pronounced in the related system (DMET){sub 2}I{sub 3}. Here, experimental and computational results for magnetoresistance oscillations in this material, over a wide range of magnetic field orientations, are presented in such a manner as to uniquely highlight this multidimensional behavior. The calculations employ the Boltzmann transport equation that incorporates the system's triclinic crystal structure, which allows for accurate estimates of the transfer integrals along the crystallographic axes, verifying the 1D, 2D and 3D nature of (DMET){sub 2}I{sub 3}, as well as crossovers between dimensions in the electronic behavior.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Low-Energy Ion Scattering Intensities from Supported Nanoparticles: The Spherical Cap Model

Supported nanoparticles are of great importance to many technologies like fuel processing and chemical synthesis using catalysts and electrocatalysts, energy storage and generation using fuel cells and batteries, electrochemistry, magnetic information storage, and more. Low-energy ion scattering spectroscopy (LEIS) with noble gas ions like He+ is a powerful tool for the characterization of nanoparticles dispersed across flat support surfaces due to its ability to probe the elemental composition in the topmost atomic layer of a surface, providing quantitative information regarding the size and number density of nanoparticles. In this work, we present a derivation of the LEIS intensities expected from nanoparticles and the support material as a function of the average particle size, their number per unit area, and their contact angle with the support when modeled as spherical caps of the nanoparticle material dispersed over the surface of a flat support. The model assumes that the ion intensities are determined only by the physical blocking of linear ion trajectories and independent of the tilt angle of the local surface relative to the incident and scattered ion directions, an assumption we support by quantitative modeling of published data which tested tilt-angle effects. The model is a generalization to arbitrary contact angles of the hemispherical cap model, which assumes 90° contact angle and has been widely used to model spectroscopic signals in LEIS (and also in Auger and photoelectron spectroscopies) during nanoparticle growth. Here, this new model quantitatively reveals how LEIS signals are sensitive not only to the diameter and number density of the nanoparticle but also to their contact angle (or height/diameter ratio). With the use of additional data (e.g., from microscopy or adsorption microcalorimetry), the model presented here will enable more accurate determination of the average size, shape, and number density of supported nanoparticles based on LEIS intensity measurements.

99 GENERAL AND MISCELLANEOUS↗
DOE OSTI2017

A FODO racetrack ring for nuSTORM: design and optimization

Here, the goal of nuSTORM is to provide well-defined neutrino beams for precise measurements of neutrino cross-sections and oscillations. The nuSTORM decay ring is a compact racetrack storage ring with a circumference of ~ 480 m that incorporates large aperture (60 cm diameter) magnets. There are many challenges in the design. In order to incorporate the Orbit Combination section (OCS), used for injecting the pion beam into the ring, a dispersion suppressor is needed adjacent to the OCS . Concurrently, in order to maximize the number of useful muon decays, strong bending dipoles are needed in the arcs to minimize the arc length. These dipoles create strong chromatic effects, which need to be corrected by nonlinear sextupole elements in the ring. In this paper, a FODO racetrack ring design and its optimization using sextupolar fields via both a Genetic Algorithm (GA) and a Simulated Annealing (SA) algorithm will be discussed.

43 PARTICLE ACCELERATORS↗
DOE OSTI2014

INTERACTION BETWEEN TWO CORONAL MASS EJECTIONS IN THE 2013 MAY 22 LARGE SOLAR ENERGETIC PARTICLE EVENT

We investigate the eruption and interaction of two coronal mass ejections (CMEs) during the large 2013 May 22 solar energetic particle event using multiple spacecraft observations. Two CMEs, having similar propagation directions, were found to erupt from two nearby active regions (ARs), AR11748 and AR11745, at ∼08:48 UT and ∼13:25 UT, respectively. The second CME was faster than the first CME. Using the graduated cylindrical shell model, we reconstructed the propagation of these two CMEs and found that the leading edge of the second CME caught up with the trailing edge of the first CME at a height of ∼6 solar radii. After about two hours, the leading edges of the two CMEs merged at a height of ∼20 solar radii. Type II solar radio bursts showed strong enhancement during this two hour period. Using the velocity dispersion method, we obtained the solar particle release (SPR) time and the path length for energetic electrons. Further assuming that energetic protons propagated along the same interplanetary magnetic field, we also obtained the SPR time for energetic protons, which were close to that of electrons. These release times agreed with the time when the second CME caught up with the trailing edge of the first CME, indicating that the CME-CME interaction (and shock-CME interaction) plays an important role in the process of particle acceleration in this event.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Spin and charge excitations in the correlated multiband metal Ca 3 Ru 2 O 7

We use Ru $L_3$-edge resonant inelastic x-ray scattering to study the full range of excitations in Ca 3 Ru 2 O 7 from meV-scale magnetic dynamics through to the eV-scale interband transitions. This bilayer 4d-electron correlated metal expresses a rich phase diagram, displaying long-range magnetic order below 56 K followed by a concomitant structural, magnetic, and electronic transition at 48 K. In the low-temperature phase, we observe a magnetic excitation with a bandwidth of ~30 meV and a gap of ~8 meV at the zone center, in excellent agreement with inelastic neutron scattering data. The dispersion can be modeled using a Heisenberg Hamiltonian for a bilayer S = 1 system with single-ion anisotropy terms. At a higher energy loss, dd-type excitations show heavy damping in the presence of itinerant electrons, giving rise to a fluorescencelike signal appearing between the $t_{2g}$ and $e_g$ bands. At the same time, we observe a resonance originating from localized $t_{2g}$ excitations, in analogy to the structurally related Mott insulator Ca 2 RuO 4 . But whereas Ca 2 RuO 4 shows sharp separate spin-orbit excitations and Hund’s-rule driven spin-state transitions, here we identify only a single broad asymmetric feature. These results indicate that local intraionic interactions underlie the correlated physics in Ca 3 Ru 2 O 7 , even as the excitations become strongly mixed in the presence of itinerant electrons.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2011

Field Dynamics of Coherent Synchrotron Radiation Using a Direct Numerical Solution of Maxwell's Equations

We present and discuss the properties of the coherent electromagnetic fields of a very short, ultrarelativistic bunch in a rectangular vacuum chamber inside a bending magnet. The analysis is based on the results of a direct numerical solution of Maxwell's equations together with Newton's equations. We use a new dispersion-free time-domain algorithm which employs a more efficient use of finite element mesh techniques and, hence, produces self-consistent and stable solutions for very short bunches. We investigate the fine structure of the coherent synchrotron radiation fields. We also discuss coherent edge radiation. We present a clear picture of the field using the electric field lines constructed from the numerical solutions. This method should be useful in the study of existing and future concepts of particle accelerators and ultrafast coherent light sources, where high peak currents and very short bunches are envisioned.

43 PARTICLE ACCELERATORS↗
NASA NTRS1985

Electromagnetic ion beam instabilities - Hot beams at interplanetary shocks

This paper considers Vlasov instabilities driven by a very hot ion beam streaming parallel to a magnetic field. The linear theory of electromagnetic instabilities driven by such a beam in a homogeneous, collisionless, nonrelativistic plasma is used. Numerical solutions of the full linear dispersion equation for bi-Maxwellian distribution functions are presented. If the thermal speed of the beam is greater than its drift speed, the two dominant modes are the right-hand and left-hand resonant ion beam instabilities. The parametric dependencies of the threshold drift speeds and growth rates for both modes are presented. In particular, the thresholds are shown to be sensitive functions of the beam temperature anisotropies. Arguments are presented that these two modes are driven by the suprathermal ion component at interplanetary shocks, and that the growth of these modes is sufficient to account for the amplitudes of MHD-like waves observed at such shocks.

Gary, S. P.↗
NASA NTRS1994

Kinematics of the ion tail of comet P/Swift-Tuttle

We have obtained long-slit high resolution spectra of the H2O(+) 6199 A complex in the near tail of comet P/Swift-Tuttle. The observations were made using the Hamilton echelle spectrometer fed by the Lick Observatory 0.6 m coude auxiliary telescope. For most of our observations, the spectral slit was aligned along the Sun-tail axis and the cometary nucleus was placed at one end of the slit, giving us spectra having the spatial and spectral resolution needed to measure the radial velocity and velocity dispersion continuously down the cometary tail out to a distance of 4X10(exp 5) km. The radial velocities confirm the earlier more restricted observations by Rauer & Jockers (1993) and by Wyckoff & Lindholm (1994) showing that the tail motions are indeed bulk flows in the antisolar direction. Out to 3X10(exp 5) km in the tail typical bulk flows are at a speed of approximately 30 km/s. The velocity dispersion, (sigma(sub r)), of the H2O(+) lines follows a pattern that is quite systematic; sigma(sub r) is smallest near the cometary nucleus, and steadily increases down the tail. The highest velocity dispersions are found ahead of the nucleus and off the tail axis. These velocity dispersions are equivalent to ion temperatures ranging from 10(exp 5) to 10(exp 6) K. We note a clear anticorrelation between the H2O(+) line intensities (related to the ion density) and the bulk flow and dispersion velocities; direct mass loading of the solar wind by the observed water ions may be responsible. We discuss several approximate equipartition methods used to infer local magnetic fields induced by the interaction of the cometary ions with the solar wind particle/field stream. Typical fields derived are near 50 nT. The measured tailward accelerations are consistent with this order of magnitude B field.

Spinrad, Hyron↗