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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,531 records · Page 85
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

Surface Proton Hopping and Fast-Kinetics Pathway of Water Oxidation on Co 3 O 4 (001) Surface

A mechanism of water splitting on cobalt oxide surface is proposed, with atomistic thermodynamic and kinetic details. The density-functional theory studies suggest that the oxidation process could proceed with several nonelectrochemical (spontaneous) intermediate steps, following the initial electrochemical hydroxyl-to-oxo conversion. More specifically, the single oxo sites Co IV =O can hop (via surface proton/electron hopping) to form oxo pair Co IV (=O)-O-Co IV =O, which will undergo nucleophilic attack by a water molecule and form the hydroperoxide CoIII -OOH. Encounter with another oxo would generate a superoxo Co III -OO, followed by the O 2 release. Finally the addition and deprotonation of a fresh water molecule will restart the catalytic cycle by forming the hydroxyl Co III -OH at this active site. Our theoretical investigations indicate that all nonelectrochemical reactions are kinetically fast and thermodynamically downhill. This hypothesis is supported by recent in situ spectroscopic observations of surface superoxo that is stabilized by hydrogen bonding to adjacent hydroxyl group as an intermediate on fast-kinetics Co catalytic site.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Single-Phase Spinel NiCo 2 O 4 as Highly Active and Stable Electrocatalysts for Urea Oxidation Reaction in Urea Electrolysis

Exploring and designing a stable and active catalyst for the urea electro-oxidation reaction (UOR, CO(NH 2 ) 2 + 6OH – → CO 2 + N 2 + 5H 2 O + 6e – ) is crucial for the long-term sustainability of ecological systems and clean energy production. We found that spinel NiCo 2 O 4 is a stable and active electrocatalyst for UOR at a relatively low anodic potential without triggering the competing oxygen evolution reaction (OER). A urea electrolysis cell (CO(NH 2 )2 + H 2 O → CO 2 + N 2 + 2H 2 ) utilizing a spinel NiCo 2 O 4 anode and a commercial Pt cathode was further characterized through galvanostatic polarization tests, demonstrating excellent structural stability at various current densities. Post-mortem analysis of long-term urea electrolysis measurements suggested that NiCo 2 O 4 electrocatalysts maintained a stable spinel structure. However, redistribution of Ni 3+ to Ni 2+ valence on the catalyst surface was observed, in contrast to the intact Co valence, indicating that (i) Ni sites are active toward urea adsorption and sequential electro-oxidation; (ii) while urea oxidation proceeds primarily through the direct electro-oxidation mechanism, chemical reactions between the Ni 3+ site and urea occur during long-term electrochemical UOR operation. Density functional theory (DFT) simulations were used to calculate the adsorption energies of urea molecules on NiO, Co 3 O 4 , and NiCo 2 O 4 , revealing the importance of regulating the configuration of adsorbed urea molecules on the NiCo 2 O 4 surface.

36 MATERIALS SCIENCE↗
DOE OSTI2019

The Shape and Density Evolution of Snow Aggregates

Abstract Snow aggregates evolve into a variety of observed shapes and densities. Despite this diversity, models and observational studies employ fractal or Euclidean geometric measures that are assumed universal for all aggregates. This work therefore seeks to improve understanding and representation of snow aggregate geometry and its evolution by characterizing distributions of both observed and Monte Carlo–generated aggregates. Two separate datasets of best-fit ellipsoid estimates derived from Multi-Angle Snowflake Camera (MASC) observations suggest the use of a bivariate beta distribution model for capturing aggregate shapes. Product moments of this model capture shape effects to within 4% of observations. This mathematical model is used along with Monte Carlo simulated aggregates to study how combinations of monomer properties affect aggregate shape evolution. Plate aggregates of any aspect ratio produce a consistent ellipsoid shape evolution whereas thin column aggregates evolve to become more spherical. Thin column aggregates yield fractal dimensions much less than the often-assumed value of 2.0. Ellipsoid densities and fractal analogs of density (lacunarity) are much more variable depending on combinations of monomer size and shape. Simple mathematical scaling relationships can explain the persistent triaxial ellipsoid shapes that appear in both observed and modeled aggregates. Overall, both simulations and observations prove aggregates are rarely oblate. Therefore, the use of the proposed bivariate ellipsoid distribution in models will allow for similar-sized aggregates to exhibit a realistic dispersion of masses and fall speeds.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRSDate not supplied

Pre-Tropical Cyclone Squall Lines and the Connection to the Diurnal Cycle during Hurricane Laura (2020)

Previous studies on the tropical cyclone (TC) diurnal cycle have shown in observations and modeling the presence of outward propagating squall lines. These squall lines were observed in several TCs during the 2020 Atlantic hurricane season. Of these squall lines, one observed in Hurricane Laura made landfall over 14 hours prior to the hurricane’s eye. This squall was responsible for numerous tornado warnings, which disrupted preparations and evacuations ahead of the storm’s landfall. This study seeks to characterize these squall lines and their environmental and thermodynamic characteristics, determine whether they behave more like midlatitude squall lines or tropical cyclone rain bands, and assess the performance of the convection-allowing High Resolution Rapid Refresh model in forecasting them over the ocean and over land. By using a combination of operational radar data, a network of surface weather observations from land and sea, satellite data, and HRRR model output, this case will undergo an extensive evaluation based on criteria from past literature in order to better understand these features as a whole and in relation to the diurnal cycle.

Vivian L Brasfield↗
NASA NTRSDate not supplied

Pre-Tropical Cyclone Squall Lines and the Connection to the Diurnal Cycle in Hurricane Laura (2020)

Previous studies on the tropical cyclone (TC) diurnal cycle have shown in observations and modeling the presence of outward propagating squall lines. These squall lines were observed in several TCs during the 2020 Atlantic hurricane season. Of these squall lines, one observed in Hurricane Laura made landfall over 13 hours prior to the hurricane’s eye. This squall was responsible for numerous tornado warnings, which disrupted preparations and evacuations ahead of the storm’s landfall. This study seeks to characterize these squall lines and their environmental and thermodynamic characteristics, determine whether they behave more like midlatitude squall lines or tropical cyclone rain bands, and assess the performance of the convection-allowing High Resolution Rapid Refresh model in forecasting them over the ocean and over land. By using a combination of operational radar data, a network of surface weather observations from land and sea, satellite data, and HRRR model output, this case will undergo an extensive evaluation based on criteria from past literature in order to better understand these features as a whole and in relation to the diurnal cycle.

Vivian L Brasfield↗
NASA NTRSDate not supplied

Observational Analysis of Atlantic Basin Tropical Cyclone Squall Lines and Relationship to the Diurnal Cycle

Previous studies on the tropical cyclone (TC) diurnal cycle have shown in observations and modeling the presence of outward propagating squall lines. These squall lines were observed in several TCs during recent Atlantic hurricane seasons. Of these squall lines, one observed in Hurricane Laura made landfall over 14 hours prior to the hurricane’s eye. This squall was responsible for 40 tornado warnings, which disrupted preparations and evacuations ahead of the storm’s landfall. This study seeks to characterize these squall lines and their environmental and thermodynamic characteristics, determine whether they behave more like midlatitude squall lines or tropical cyclone rain bands, and assess the performance of the convection-allowing High Resolution Rapid Refresh model in forecasting them over the ocean and over land. By using a combination of operational radar data, a network of surface weather observations from land and sea, satellite data, and HRRR model output, this case will undergo an extensive evaluation based on criteria from past literature in order to better understand these features as a whole and in relation to the diurnal cycle.

Vivian Brasfield↗
DOE OSTI2019

Surface Solar Irradiance in Continental Shallow Cumulus Fields: Observations and Large-Eddy Simulation

This study examines shallow cumulus cloud fields and their surface shortwave radiative effects using large-eddy simulation (LES) along with observations across multiple days at the Atmospheric Radiation Measurement Southern Great Plains atmospheric observatory. Pronounced differences are found between probability density functions (PDFs) of downwelling surface solar irradiance derived from observations and LES one-dimensional (1D) online radiation calculations. The shape of the observed PDF is bimodal, which is only reproduced by offline three-dimensional (3D) radiative transfer calculations, demonstrating PDF bimodality as a 3D radiative signature of continental shallow cumuli. Local differences between 3D and 1D radiative transfer calculations of downwelling surface solar irradiance are, on average, larger than 150 W m -2 on one afternoon. The differences are substantially reduced when spatially averaged over the LES domain and temporally averaged over the diurnal cycle, but systematic 3D biases ranging from 2 to 8 W m -2 persist across different days. Covariations between the domain-averaged surface irradiance, framed as a surface cloud radiative effect, and the simulated cloud fraction are found to follow a consistent diurnal relationship, often exhibiting hysteresis. In contrast, observations show highly variable behavior. By subsampling the LES domain, it is shown that this is due to the limited sampling density of inherently 3D observations. These findings help to define observational requirements for detecting such relationships, provide valuable insight for evaluating weather and climate models against surface observations as they push to ever higher resolutions, and have important implications for future assessments of solar renewable energy potential.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2015

The structure and dark halo core properties of dwarf spheroidal galaxies

The structure and dark matter halo core properties of dwarf spheroidal galaxies (dSphs) are investigated. A double-isothermal (DIS) model of an isothermal, non-self-gravitating stellar system embedded in an isothermal dark halo core provides an excellent fit to the various observed stellar surface density distributions. The stellar core scale length a{sub *} is sensitive to the central dark matter density ρ{sub 0,d}. The maximum stellar radius traces the dark halo core radius r{sub c,d}. The concentration c{sub *} of the stellar system, determined by a King profile fit, depends on the ratio of the stellar-to-dark-matter velocity dispersion σ{sub ∗}/σ{sub d}. Simple empirical relationships are derived that allow us to calculate the dark halo core parameters ρ{sub 0,d}, r{sub c,d}, and σ{sub d} given the observable stellar quantities σ{sub *}, a{sub *}, and c{sub *}. The DIS model is applied to the Milky Way’s dSphs. All dSphs closely follow the same universal dark halo scaling relations ρ{sub 0,d}×r{sub c,d}=75{sub −45}{sup +85} M{sub ⊙} pc{sup −2} that characterize the cores of more massive galaxies over a large range in masses. The dark halo core mass is a strong function of core radius, M{sub c,d}∼r{sub c,d}{sup 2}. Inside a fixed radius of ∼400 pc the total dark matter mass is, however, roughly constant with M{sub d}=2.6±1.4×10{sup 7} M{sub ⊙}, although outliers are expected. The dark halo core densities of the Galaxy’s dSphs are very high, with ρ{sub 0,d} ≈ 0.2 M{sub ⊙} pc{sup −3}. dSphs should therefore be tidally undisturbed. Evidence for tidal effects might then provide a serious challenge for the CDM scenario.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2016

Investigation of the relationships between DCS cloud properties, lifecycle, and precipitation with meteorological regimes and aerosol sources at the ARM SGP Site

In this proposed research, we will investigate how different meteorological regimes and aerosol sources affect DCS properties, diurnal and life cycles, and precipitation using multiple observational platforms (surface, satellite, and aircraft) and NARR reanalysis at the ARM SGP site. The Feng et al. (2011, 2012) DCS results will serve as a starting point for this proposed research, and help us to address some fundamental issues of DCSs, such as convective initiation, rain rate, areal extent (including stratiform and convective regions), and longevity. Convective properties will be stratified by meteorological regime (synoptic/mesoscale patterns) identified by reanalysis. Aerosol information obtained from the ARM SGP site will also be stratified by meteorological regimes to understand their effects on convection. Finally, the aircraft in-situ measurements and various radar observations and retrievals during the MC3E campaign will provide a “cloud-truth” dataset and are an invaluable data source for verifying the findings and investigating the proposed hypotheses in Objective 1.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRSDate not supplied

The Land Surface in Earth System Reanalysis

Current global atmospheric reanalysis products such as ERA-5, MERRA-2, and JRA-55 provide estimates of land surface states and fluxes, including soil moisture, soil temperature, snow mass, latent and sensible heat fluxes, and runoff. These land surface estimates are based on land surface process models and, depending on the reanalysis product, on precipitation observations or the assimilation of land surface observations of soil moisture and snow conditions from satellites and in situ networks. The land models used in the current global atmospheric reanalysis systems are generally focused on water and energy balance processes, with prescribed static land cover and prescribed climatological vegetation conditions. That is, current global atmospheric reanalysis products do not reflect changes in land use or land cover, nor do they provide dynamic estimates of the land carbon cycle. These and other gaps, including the omission of anthropogenic processes such as irrigation in the land model, need to be addressed in the development of the next generation Earth system reanalysis systems. This presentation provides an overview of the state-of-the-art and future developments of land surface estimates in global reanalysis systems.

Rolf Reichle↗
NASA NTRS2019

Integrating Remote Sensing Observations with NASA's GEOS-5 Modeling Framework in Support of Retrospective Analyses and Seasonal Prediction of Biosphere-Atmosphere CO2 Flux

The absorption of nearly half of all anthropogenic carbon dioxide (CO2) emissions by terrestrial and marine ecosystems has played a critical role in mitigating climate change. However, a persistent lack of understanding of these uptake processes impedes attribution, and thereby introduces large uncertainties into projections of the trajectory of carbon and climate in coming decades. A better understanding and quantification of the seasonal and interannual variability of carbon flux between the atmosphere and ocean and terrestrial biospheres is critically needed to improve predictions from Earth system models. We propose to bring together a diverse suite of remote sensing observations, mechanistic models, and NASA's Goddard Earth Observing System, version 5 (GEOS-5) model to address two objective 1) quantify the processes controlling the temporal variability of biosphere-atmosphere CO2 flux on seasonal and interannual timescales from 1989 to 2018 and 2) evaluating the predictability of the components of carbon flux on seasonal timescales. Because GEOS-5 has been developed to incorporate a variety of Earth system observations and includes a complete and physically consistent depiction of the atmosphere, land, and ocean carbon cycles, it represents a unique and ideal synthesis framework for this effort. By expanding the realism of processes that could be included in GEOS-5 seasonal forecasts, this effort supports NASA's goals toward an integrated Earth system modeling and prediction framework.We propose to integrate a number of observations into the GEOS-5 modeling system to refine retrospective estimates of both terrestrial and marine carbon flux and to test hypotheses regarding the effects of climate drivers on terrestrial carbon flux. This will include assimilating several satellite ocean color products in the NASA Ocean Biogeochemistry Model (NOBM) to improve the representation of ocean biology. We will also utilize remote sensing datasets to increase the temporal resolution of global land-use change estimates and fire emissions to better constrain the temporal variability of the terrestrial carbon cycle. This information will be incorporated into two NASA terrestrial biosphere models Catchment-CN, a dynamic vegetation model that is integrated within GEOS-5 and the Ecosystem Demography (ED) model, a core modeling resource supporting the Global Ecosystem Dynamics Investigation (GEDI) mission to map biomass. Fluxes will be evaluated through 1) comparison to top-down flux estimates inferred from surface CO2 observations and 2) comparison against available aircraft and satellite observations.By combining predictions of net ecosystem exchange and air-sea CO2 flux from land and ocean models with statistical predictions of land use change, fire, and fossil fuel emissions, we propose to create the first dynamical CO2 forecast on seasonal timescales. Because of the experimental nature of this endeavor, an important project objective will be to evaluate the limits to the predictability of different carbon cycle processes over lead times of 1-12 months using different satellite and surface data streams.

Ott, Lesley↗
DOE OSTI2014

Femtosecond time-resolved photoemission electron microscopy for spatiotemporal imaging of photogenerated carrier dynamics in semiconductors

We constructed an instrument for time-resolved photoemission electron microscopy (TR-PEEM) utilizing femtosecond (fs) laser pulses to visualize the dynamics of photogenerated electrons in semiconductors on ultrasmall and ultrafast scales. The spatial distribution of the excited electrons and their relaxation and/or recombination processes were imaged by the proposed TR-PEEM method with a spatial resolution about 100 nm and an ultrafast temporal resolution defined by the cross-correlation of the fs laser pulses (240 fs). A direct observation of the dynamical behavior of electrons on higher resistivity samples, such as semiconductors, by TR-PEEM has still been facing difficulties because of space and/or sample charging effects originating from the high photon flux of the ultrashort pulsed laser utilized for the photoemission process. Here, a regenerative amplified fs laser with a widely tunable repetition rate has been utilized, and with careful optimization of laser parameters, such as fluence and repetition rate, and consideration for carrier lifetimes, the electron dynamics in semiconductors were visualized. For demonstrating our newly developed TR-PEEM method, the photogenerated carrier lifetimes around a nanoscale defect on a GaAs surface were observed. The obtained lifetimes were on a sub-picosecond time scale, which is much shorter than the lifetimes of carriers observed in the non-defective surrounding regions. Our findings are consistent with the fact that structural defects induce mid-gap states in the forbidden band, and that the electrons captured in these states promptly relax into the ground state.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Strong-coupling anisotropic s-wave superconductivity in the type-II Weyl semimetal TaIrTe 4

TaIrTe 4 is a recently discovered type-II Weyl semimetal, hosting only four Weyl points. In this work, we study the cleaved TaIrTe 4 crystal using scanning tunneling microscopy/spectroscopy and find that it also hosts a superconducting state with a transition temperature of 3.9 K. From Dynes function fitting, the superconducting phase is consistent with anisotropic s-wave pairing, with a superconducting gap of 1.31 meV. This value leads to a value of 2Δ max /k B T C = 7.81 , much larger than the 3.53 predicted by Bardeen-Cooper-Schrieffer theory for weak-coupling superconductors. The critical field is found to be 0.7 T based on the analysis of tunneling conductance as a function of magnetic field. Two types of nonmagnetic defects on the TaIrTe 4 surface are observed, neither of which induce bound states inside the superconducting gap, further supporting conventional s-wave superconductivity in the TaIrTe 4 system.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS2021

Temperature Fluctuations and Boundary Layer Turbulence as seen by Mars Exploration Rovers Miniature Thermal Emission Spectrometer

The Mini-TES spectrometer carried by Spirit and Opportunity is a unique instrument that enabled vertical temperature profiles to be retrieved at high frequency (every 2 s, or “ICK”). Observations obtained from this instrument provide information on boundary layer activity. As an extension of previous work, we have retrieved ICK-by-ICK vertical temperature profiles to characterize turbulent behavior at each rover site for up to two Mars Years. We have also retrieved ICK-by-ICK near-surface (1.1 m) atmospheric temperatures and surface temperatures from dedicated atmospheric observations as well as geologic observations that extend the coverage of near-surface observations. The extension and increased frequency of retrievals as well as the additional observations provide a more complete view of the vertical and temporal variation of temperature fluctuations within the PBL. Temperature fluctuations are assessed using detrended temperature time-series data. The results show fluctuations can be as large as 10 K at the surface and 8 K aloft with timescales on the order of minutes. We have calculated the peak-to-peak amplitudes of temperature fluctuations and the corresponding timescales over which they occur. Spirit and Opportunity temperature fluctuation amplitudes decrease in magnitude vertically, where higher atmospheric levels show smaller fluctuations in amplitudes than at the surface. The magnitude of temperature fluctuations changes with the difference in surface and air temperature. This difference varies little as a function of season at both rover sites. Fluctuations are observed to quickly decrease in the late afternoon reaching a minimum near 17:00 LTST followed by moderately increased activity near sunset caused by forced convection. There is no significant change in the observed convective activity as a function of dust optical depth during regional dust storms. The few large temperature fluctuations that are concurrent with dust events are likely the result of large-scale systems.

Mars, atmosphere↗
NASA NTRS2013

ISSM: Ice Sheet System Model

In order to have the capability to use satellite data from its own missions to inform future sea-level rise projections, JPL needed a full-fledged ice-sheet/iceshelf flow model, capable of modeling the mass balance of Antarctica and Greenland into the near future. ISSM was developed with such a goal in mind, as a massively parallelized, multi-purpose finite-element framework dedicated to ice-sheet modeling. ISSM features unstructured meshes (Tria in 2D, and Penta in 3D) along with corresponding finite elements for both types of meshes. Each finite element can carry out diagnostic, prognostic, transient, thermal 3D, surface, and bed slope simulations. Anisotropic meshing enables adaptation of meshes to a certain metric, and the 2D Shelfy-Stream, 3D Blatter/Pattyn, and 3D Full-Stokes formulations capture the bulk of the ice-flow physics. These elements can be coupled together, based on the Arlequin method, so that on a large scale model such as Antarctica, each type of finite element is used in the most efficient manner. For each finite element referenced above, ISSM implements an adjoint. This adjoint can be used to carry out model inversions of unknown model parameters, typically ice rheology and basal drag at the ice/bedrock interface, using a metric such as the observed InSAR surface velocity. This data assimilation capability is crucial to allow spinning up of ice flow models using available satellite data. ISSM relies on the PETSc library for its vectors, matrices, and solvers. This allows ISSM to run efficiently on any parallel platform, whether shared or distrib- ISSM: Ice Sheet System Model NASA's Jet Propulsion Laboratory, Pasadena, California uted. It can run on the largest clusters, and is fully scalable. This allows ISSM to tackle models the size of continents. ISSM is embedded into MATLAB and Python, both open scientific platforms. This improves its outreach within the science community. It is entirely written in C/C++, which gives it flexibility in its design, and the power/speed that C/C++ allows. ISSM is svn (subversion) hosted, on a JPL repository, to facilitate its development and maintenance. ISSM can also model propagation of rifts using contact mechanics and mesh splitting, and can interface to the Dakota software. To carry out sensitivity analysis, mesh partitioning algorithms are available, based on the Scotch, Chaco, and Metis partitioners that ensure equal area mesh partitions can be done, which are then usable for sampling and local reliability methods.

Larour, Eric↗
NASA NTRS2003

Analysis of Surface and Bulk Behavior in Ni-Pd Alloys

The most salient features of the surface structure and bulk behavior of Ni-Pd alloys have been studied using the BFS method for alloys. Large-scale atomistic simulations were performed to investigate surface segregation profiles as a function of temperature, crystal face, and composition. Pd enrichment of the first layer was observed in (111) and (100) surfaces, and enrichment of the top two layers occurred for (110) surfaces. In all cases, the segregation profile shows alternate planes enriched and depleted in Pd. In addition, the phase structure of bulk Ni-Pd alloys as a function of temperature and composition was studied. A weak ordering tendency was observed at low temperatures, which helps explain the compositional oscillations in the segregation profiles. Finally, based on atom-by-atom static energy calculations, a comprehensive explanation for the observed surface and bulk features will be presented in terms of competing chemical and strain energy effects.

Bozzolo, Guillermo↗
DOE OSTI2016

AN ORDERED MAGNETIC FIELD IN THE PROTOPLANETARY DISK OF AB Aur REVEALED BY MID-INFRARED POLARIMETRY

Magnetic fields ( B -fields) play a key role in the formation and evolution of protoplanetary disks, but their properties are poorly understood due to the lack of observational constraints. Using CanariCam at the 10.4 m Gran Telescopio Canarias, we have mapped out the mid-infrared polarization of the protoplanetary disk around the Herbig Ae star AB Aur. We detect ∼0.44% polarization at 10.3 μ m from AB Aur's inner disk ( r < 80 au), rising to ∼1.4% at larger radii. Our simulations imply that the mid-infrared polarization of the inner disk arises from dichroic emission of elongated particles aligned in a disk B -field. The field is well ordered on a spatial scale, commensurate with our resolution (∼50 au), and we infer a poloidal shape tilted from the rotational axis of the disk. The disk of AB Aur is optically thick at 10.3 μ m, so polarimetry at this wavelength is probing the B -field near the disk surface. Our observations therefore confirm that this layer, favored by some theoretical studies for developing magneto-rotational instability and its resultant viscosity, is indeed very likely to be magnetized. At radii beyond ∼80 au, the mid-infrared polarization results primarily from scattering by dust grains with sizes up to ∼1 μ m, a size indicating both grain growth and, probably, turbulent lofting of the particles from the disk mid-plane.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1999

Environmental Forcing of Super Typhoon Paka's (1997) Latent Heat Structure

The distribution and intensity of total (i.e., combined stratified and convective processes) rainrate/latent heat release (LHR) were derived for tropical cyclone Paka during the period 9-21 December, 1997 from the F-10, F-11, F-13, and F-14 Defense Meteorological Satellite Special Sensor Microwave/Imager and the Tropical Rain Measurement Mission Microwave Imager observations. These observations were frequent enough to capture three episodes of inner core convective bursts that preceded periods of rapid intensification and a convective rainband (CRB) cycle. During these periods of convective bursts, satellite sensors revealed that the rainrates/LHR: 1) increased within the inner eye wall region; 2) were mainly convectively generated (nearly a 65% contribution), 3) propagated inwards; 4) extended upwards within the middle and upper-troposphere, and 5) became electrically charged. These factors may have caused the eye wall region to become more buoyant within the middle and upper-troposphere, creating greater cyclonic angular momentum, and, thereby, warming the center and intensifying the system. Radiosonde measurements from Kwajalein Atoll and Guam, sea surface temperature observations, and the European Center for Medium Range Forecast analyses were used to examine the necessary and sufficient condition for initiating and maintaining these inner core convective bursts. For example, the necessary conditions such as the atmospheric thermodynamics (i.e., cold tropopause temperatures, moist troposphere, and warm SSTs [greater than 26 deg]) suggested that the atmosphere was ideal for Paka's maximum potential intensity (MPI) to approach super-typhoon strength. Further, Paka encountered weak vertical wind shear (less than 15 m/s ) before interacting with the westerlies on 21 December. The sufficient conditions, on the other hand, appeared to have some influence on Paka's convective burst, but the horizontal moisture flux convergence values in the outer core were weaker than some of the previously examined tropical cyclones. Also, the upper tropospheric outflow generation of eddy relative angular momentum flux convergence was 4D much less than that found during moderate tropical cyclone/trough interaction. These results indicated how important the external necessary condition and the internal forcing (i.e., CRB cycle) were in generating Paka's convective bursts as compared to the external sufficient forcing mechanisms found in higher latitude tropical cyclones. Later, as Paka began to interact with the westerlies, both the necessary (i.e., strong vertical shear and colder SSTs) and sufficient (i.e., dry air intrusion) external forcing mechanisms helped to decrease Paka's rainrate.

Rodgers, Edward B.↗