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At least 1,531 records · Page 85

Development of MCNP Training Modules for Safeguards Practitioners [Abstract]

The Monte-Carlo N-Particle (MCNP) software developed at LANL is the most widely used neutron transport code in the world. It is an essential tool for a variety of applications including detector development and design, nuclear fuel burnup simulation, criticality safety, and nondestructive assay system optimization. For this reason, it is indispensable within the safeguards and materials control & accountability (MC&A) communities. Multiple MCNP training courses have been created and taught over the last several decades by the MCNP development team at LANL, however there are no existing courses that cover specialized topics considered fundamental to NDA and safeguards models. To fill this gap, the MCNP team and Safeguards Science and Technology group at LANL have co-created a set of training modules customized to meet the specialized needs of the safeguards and MC&A communities. The basic modules cover concepts such as NDA system optimization, He-specific and other capture tallies, and tools for improved theoretical understanding. An advanced module was also created to cover topics including variance reduction for active interrogation simulations, use of the LANL MCNPTools post-processor, PTRAC (particle tracking) and list-mode data simulations, and fuel burnup simulations. The training modules teach to the latest and most state-of-the-art MCNP features and tools released by the development team at LANL and are intended to be taught jointly by the developers and safeguards experts. Ultimately, we hope that creation of these modules will serve to capture and convey the safeguards modeling and MCNP expertise at LANL, and that we will be able to share the modules more broadly with the MC&A and safeguards communities.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The Pixel Anomaly Detection Tool : a user-friendly GUI for classifying detector frames using machine-learning approaches

Data collection at X-ray free electron lasers has particular experimental challenges, such as continuous sample delivery or the use of novel ultrafast high-dynamic-range gain-switching X-ray detectors. This can result in a multitude of data artefacts, which can be detrimental to accurately determining structure-factor amplitudes for serial crystallography or single-particle imaging experiments. Here, a new data-classification tool is reported that offers a variety of machine-learning algorithms to sort data trained either on manual data sorting by the user or by profile fitting the intensity distribution on the detector based on the experiment. This is integrated into an easy-to-use graphical user interface, specifically designed to support the detectors, file formats and software available at most X-ray free electron laser facilities. The highly modular design makes the tool easily expandable to comply with other X-ray sources and detectors, and the supervised learning approach enables even the novice user to sort data containing unwanted artefacts or perform routine data-analysis tasks such as hit finding during an experiment, without needing to write code.

47 OTHER INSTRUMENTATION↗

Automated electrophoresis apparatus

Computer-controlled electro-optical system tracks particles in essentially real-time, analyzes data, and presents video and hard copy results. System presents significant increase in sampling rate and improved analysis of particle motion.

Baker, L. R.↗

Emissions of Black Carbon, Organic, and Inorganic Aerosols From Biomass Burning in North America and Asia in 2008

Reliable assessment of the impact of aerosols emitted from boreal forest fires on the Arctic climate necessitates improved understanding of emissions and the microphysical properties of carbonaceous (black carbon (BC) and organic aerosols (OA)) and inorganic aerosols. The size distributions of BC were measured by an SP2 based on the laser-induced incandescence technique on board the DC-8 aircraft during the NASA ARCTAS campaign. Aircraft sampling was made in fresh plumes strongly impacted by wildfires in North America (Canada and California) in summer 2008 and in those transported from Asia (Siberia in Russia and Kazakhstan) in spring 2008. We extracted biomass burning plumes using particle and tracer (CO, CH3CN, and CH2Cl2) data. OA constituted the dominant fraction of aerosols mass in the submicron range. The large majority of the emitted particles did not contain BC. We related the combustion phase of the fire as represented by the modified combustion efficiency (MCE) to the emission ratios between BC and other species. In particular, we derived the average emission ratios of BC/CO = 2.3 +/- 2.2 and 8.5 +/- 5.4 ng/cu m/ppbv for BB in North America and Asia, respectively. The difference in the BC/CO emission ratios is likely due to the difference in MCE. The count median diameters and geometric standard deviations of the lognormal size distribution of BC in the BB plumes were 136-141 nm and 1.32-1.36, respectively, and depended little on MCE. These BC particles were thickly coated, with shell/core ratios of 1.3-1.6. These parameters can be used directly for improving model estimates of the impact of BB in the Arctic.

Kondo, Y.↗

Simulation of Dust-Laden Flow in the DLR L2K Facility

An integrated CFD-particle trajectory code called US3D-DUST is used to simulate the dusty flow environments performed in the German Aerospace Center (DLR) L2K arcjet facility. The particle trajectory code uses a Lagrangian approach, where the particle trajectories through the shock layer can be computed using a set of coupled ordinary differential equations. The L2K experiments measured mass loss to flat-face shaped samples of the Norcoat-Liège thermal protection system material. The US3D-DUST simulations were able to reproduce particle velocity and stagnation point heating rate data. When applied to the L2K dusty flow conditions, the US3D-DUST predictions of mass loss due to particle impacts and surface recession rates over-predicted the experimental values. It is recommended to perform additional dusty flow tests in the L2Kto provide and improve the surface damage model for Norcoat-Liège.

Thermal protection systems↗

ENDF/B-VIII.1: Updated Nuclear Reaction Data Library for Science and Applications

The ENDF/B-VIII.1 library is the newest recommended evaluated nuclear data file by the Cross Section Evaluation Working Group (CSEWG) for use in nuclear science and technology applications, and incorporates advances made in the six years since the release of ENDF/B-VIII.0. Among key advances made are that the 239 Pu file was reevaluated by a joint international effort and that updated 16,18 O, 19 F, 28–30 Si, 50–54 Cr, 55 Mn, 54,56,57 Fe, 63,65 Cu, 139 La, 233,235,238 U, and 240,241 Pu neutron nuclear data from the IAEA coordinated INDEN collaboration were adopted. Over 60 neutron dosimetry cross sections were adopted from the IAEA's IRDFF-II library. In addition, the new library includes significant changes for 3 He, 6 Li, 9 Be, 51 V, 88 Sr, 103 Rh, 140,142 Ce, Dy, 181 Ta, Pt, 206–208 Pb, and 234,236 U neutron data, and new nuclear data for the photonuclear, charged-particle and atomic sublibraries. Numerous thermal neutron scattering kernels were reevaluated or provided for the very first time. On the covariance side, work was undertaken to introduce better uncertainty quantification standards and testing for nuclear data covariances. The significant effort to reevaluate important nuclides has reduced bias in the simulations of many integral experiments with particular progress noted for fluorine, copper, and stainless steel containing benchmarks. Data issues hindered the successful deployment of the previous ENDF/B-VIII.0 for commercial nuclear power applications in high burnup situations. These issues were addressed by improving the 238 U and 239,240,241 Pu evaluated data in the resonance region. The new library performance as a function of burnup is similar to the reference ENDF/B-VII.1 library.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Dark sector searches with the CMS experiment

Astrophysical observations provide compelling evidence for gravitationally interacting dark matter in the universe that cannot be explained by the standard model of particle physics. The extraordinary amount of data from the CERN LHC presents a unique opportunity to shed light on the nature of dark matter at unprecedented collision energies. This Report comprehensively reviews the most recent searches with the CMS experiment for particles and interactions belonging to a dark sector and for dark-sector mediators. Models with invisible massive particles are probed by searches for signatures of missing transverse momentum recoiling against visible standard model particles. Searches for mediators are also conducted via fully visible final states. The results of these searches are compared with those obtained from direct-detection experiments. Searches for alternative scenarios predicting more complex dark sectors with multiple new particles and new forces are also presented. Many of these models include long-lived particles, which could manifest themselves with striking unconventional signatures with relatively small amounts of background. Searches for such particles are discussed and their impact on dark-sector scenarios is evaluated. Many results and interpretations have been newly obtained for this Report.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Exhaust plume impingement of chemically reacting gas-particle flows

A series of computer codes has been developed to predict gas-particle flows and resulting impingement forces, moments and heating rates to surfaces immersed in the flow. The gas-particle flow solution is coupled via heat transfer and drag between the phases with chemical effects included in the gas phase. The flow solution and impingement calculations are discussed. Analytical results are compared with test data obtained to evaluate gas-particle effects on the Space Shuttle thermal protection system during the staging maneuver.

Smith, S. D.↗

Characterization of Individual Aerosol Particles Associated with Clouds (CRYSTAL-FACE)

The aim of our research was to obtain data on the chemical and physical properties of individual aerosol particles from near the bottoms and tops of the deep convective systems that lead to the generation of tropical cirrus clouds and to provide insights into the particles that serve as CCN or IN. We used analytical transmission electron microscopy (ATEM), including energy-dispersive X-ray spectrometry (EDS) and electron energy-loss spectroscopy (EELS), and field-emission electron microscopy (FESEM) to compare the compositions, concentrations, size distributions, shapes, surface coatings, and degrees of aggregation of individual particles from cloud bases and the anvils near the tropopause. Aggregates of sea salt and mineral dust, ammonium sulfate, and soot particles are abundant in in-cloud samples. Cirrus samples contain many H2SO4 droplets, but acidic sulfate particles are rare at the cloud bases. H2SO4 probably formed at higher altitudes through oxidation of SO2 in cloud droplets. The relatively high extent of ammoniation in the upper troposphere in-cloud samples appears to have resulted from vertical transport by strong convection. The morphology of H2SO4 droplets indicates that they had been at least yartiy ammoniated at the time of collection. They are internally mixed with organic materials, metal sulfates, and solid particles of various compositions. Ammoniation and internal mixing of result in freezing at higher temperature than in pure H2SO4 aerosols. K- and S-bearing organic particles and Si-Al-rich particles are common throughout. Sea salt and mineral dust were incorporated into the convective systems from the cloud bases and worked as ice nuclei while being vertically transported. The nonsulfate particles originated from the lower troposphere and were transported to the upper troposphere and lower stratosphere.

Buseck, Peter R.↗

Physicochemical and Molecular Insights into the Boundary Layer and Free Troposphere Aerosol Interactions over the Southern Great Plains

Ambient aerosols’ vertical profiles are critical for evaluating the role of aerosols in atmospheric chemistry and radiative transfer, but limited data on these profiles hinders our ability to fully assess their impact on the Earth's radiative balance. Here, in this study, we investigated the size-, time-, and altitude resolved composition of individual particles and bulk molecular composition of particle samples collected by an uncrewed aerial system–ArcticShark over the Southern Great Plains. Single particle microanalysis shows that, the free tropospheric (FT) samples are dominated (56-66%) by carbonaceous sulfate particles, while boundary layer (BL) samples are dominated (57-74%) by carbonaceous particles. Back trajectory simulations suggest that FT particles are likely influenced by long-range transport and have undergone aqueous-phase processing. Conversely, in-situ size distribution data shows evidence of particle growth in the upper BL and just below the FT. This observation may indicate vertical transport of particles from an elevated aerosol layer in the FT, possibly linked to a new particle formation event. This observation is further supported by high resolution molecular composition data, which reveals particle volatility increasing with increasing size, which aligns with the growth event. This study aids in fundamental understanding of the compositional and molecular specificity of vertically resolved organic aerosols to provide insights into particle size evolution for future atmospheric models.

ArcticShark↗

Airborne auroral data and satellite data analysis

The photometric data taken during the 1969 CV990 expedition were analyzed. It was found that the so-called soft auroral zone extends right through the night side auroral zone. The soft precipitation is a permanent feature of the night side auroral zone and probably signifies the position of the plasma sheet. The harder auroras which include the conventional visible auroras occur less frequently. The intensity and mean energy of auroral electrons is correlated suggesting that the fluctuation in auroral intensity comes primarily from the variability of the acceleration mechanism rather than the variations in the particle population densities. During the 1969 CV990 expedition, coordinated data was taken with the particle experiments on OV1-18 and ATS-5 satellites. The satellite data was reduced to facilitate coordinated investigations with the airborne experimenters. The airborne photometric lambda 5200 NI data were analyzed and the effective life time was found to be 4.5 minutes.

Mende, S. B.↗

Machine Learning-Based Extreme Data Reduction for Prompt Supernova Pointing at DUNE

One of the goals of the Deep Underground Neutrino Experiment (DUNE) is to use the massive underground liquid argon time projection chamber (LArTPC) detectors at its far site for multimessenger astronomy (MMA), in the detection of neutrinos from core-collapse supernovae (SNe). Its current baseline trigger strategy detects activity in the detector that is consistent with supernova (SN) neutrinos and saves the raw data for further offline analysis but provides no prompt pointing information crucial for optical follow-ups by other observatories. This approach is based on the assumption that prompt pointing determination using raw data is computationally prohibitive. In this article, we demonstrate a proof-of-concept based on applying extreme data reduction on the buffered SN data in the DUNE data acquisition (DAQ) system’s front-end computers using a machine learning (ML) workflow. This reduces the data by ~5 orders of magnitude, allowing a full track reconstruction to be carried out quickly on a single server. The total time to perform the ML-based data reduction and the full track reconstruction is less than the time to transfer the SN data back to Fermilab or a high-performance computing (HPC) center. This shows that prompt processing of raw SN data is possible and, in fact, trivial once the data have been reduced to reject radiological backgrounds, paving the way to a high-quality SN pointing trigger that is based on fully reconstructed data instead of trigger primitives (TPs).

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Effects of the August 1972 solar particle events on stratospheric ozone

High-energy proton data obtained by polar-orbiting satellite and several balloon flights are used to derive the spatial extent and ionization profiles of regions irradiated by the intense solar particle events (SPE) of August 1972. Backscattered ultraviolet ozone sensors on the Nimbus 4 satellite identified and tracked the polar ozone cavity created by particle ionization during the intense, ten-hour period of August 4, which persisted and rotated as a semirigid mass in an east-to-west direction during 53 days of continuous tracking. Time-dependent chemistry calculations have been performed to show the cause, magnitude, and temporal features of the ozone reduction. Attempts to verify the predicted temperature changes have been unsuccessful due to limitations in the temperature measurement techniques used.

Reagan, J. B.↗

Extinction coefficient (1 micrometer) properties of high-altitude clouds from solar occultation measurements (1985-1990): Evidence of volcanic aerosol effect

The properties of the 1-micrometer volume extinction coefficient of two geographically different high-altitude cloud systems have been examined for the posteruption period (1985-1990) of the April 1982 El Chichon volcanic event with emphasis on the effect of volcanic aerosols on clouds. These two high-altitude cloud systems are the tropical clouds in the tropopause region observed by the Stratospheric Aerosol and Gas Experiment (SAGE) 2 and the polar stratospheric clouds (PSCs) sighted by the Stratospheric Aerosol Measurement (SAM) 2. The results indicate that volcanic aerosols alter the frequency distributions of these high-altitude clouds in such a manner that the occurrence of clouds having high extinction coefficients (6 x 10(exp -3) - 2 x 10(exp -2)/km) is suppressed, while that of clouds having low extinction coefficients (2 x 10(exp -3) - 6 x 10(exp -2)/km) is enhanced. This influence of the volcanic aerosols appears to be opposite to the increase in the extinction coefficient of optically thick clouds observed by the Earth Radiation Budget Experiment (ERBE) during the initial posteruption period of the June 1991 Pinatubo eruption. A plausible explanation of this difference, based on the Mie theory, is presented. As a consequence of the Mie theory, the effective radius of most, if not all, of the high-altitude clouds, measured by the SAGE series of satellite instruments must be less than about 0.8 micrometers. This mean cloud particle size implied by the satellite extinction-coefficient data at a single wavelength (1 micrometer) is further substantiated by the particle size analysis based on cloud extinction coefficient at two wavelengths (0.525 and 1.02 micrometers) obtained by the SAGE 2 observations. Most of the radiation measured by ERBE is reflected by cloud systems comprised of particles having effective radii much greater than 1 micrometer. A reduction in the effective radius of these clouds due to volcanic aerosols is expected to increase their extinction-coefficient values, opposite the effect observed by SAGE 2 and SAM 2. This work further illustrates the capability of the solar occultation satellite sensor to provide particulate extinction-coefficient measurements important to the study of the aerosol-cloud interactions. It is important to examine the variations of the extinction coefficient of these two high-altitude cloud systems for the posteruption years of the Pinatubo volcanic event for further evidence of the impact of volcanic aerosols on high-altitude clouds.

Wang, Pi-Huan↗

Homogenous Surface Nucleation of Solid Polar Stratospheric Cloud Particles

A general surface nucleation rate theory is presented for the homogeneous freezing of crystalline germs on the surfaces of aqueous particles. While nucleation rates in a standard classical homogeneous freezing rate theory scale with volume, the rates in a surface-based theory scale with surface area. The theory is used to convert volume-based information on laboratory freezing rates (in units of cu cm, seconds) of nitric acid trihydrate (NAT) and nitric acid dihydrate (NAD) aerosols into surface-based values (in units of sq cm, seconds). We show that a surface-based model is capable of reproducing measured nucleation rates of NAT and NAD aerosols from concentrated aqueous HNO3 solutions in the temperature range of 165 to 205 K. Laboratory measured nucleation rates are used to derive free energies for NAT and NAD germ formation in the stratosphere. NAD germ free energies range from about 23 to 26 kcal mole, allowing for fast and efficient homogeneous NAD particle production in the stratosphere. However, NAT germ formation energies are large (greater than 26 kcal mole) enough to prevent efficient NAT particle production in the stratosphere. We show that the atmospheric NAD particle production rates based on the surface rate theory are roughly 2 orders of magnitude larger than those obtained from a standard volume-based rate theory. Atmospheric volume and surface production of NAD particles will nearly cease in the stratosphere when denitrification in the air exceeds 40 and 78%, respectively. We show that a surface-based (volume-based) homogeneous freezing rate theory gives particle production rates, which are (not) consistent with both laboratory and atmospheric data on the nucleation of solid polar stratospheric cloud particles.

Tabazadeh, A.↗

Venus cloud models

Remote observations of Venus are reviewed. The strongest inferences of cloud properties can be drawn from polarization data which provide information about cloud particles near 68 km. Particle properties are not as well determined at higher and lower levels. If the clouds are generated photochemically from reduced sulfur species, the supply of O2 may be an important constraint on cloud production. Vapor-pressure data reviewed, and it is shown that deep clouds cannot be H2SO4-H2O aerosols unless the mixing ratios of both H2SO4 and H2O approach 0.001 below 50 km.

Wofsy, S. C.↗

Observation and modeling of energetic particles at synchronous orbit on July 29, 1977

In the 12 hours immediately after a worldwide storm sudden commencement at 0027 UT on July 29, there was a series of at least four magnetospheric substorms, the last and largest of which exhibited an expansion phase onset at approximately 1200 UT. Data from six spacecraft in three general local time groupings (0300, 0700, and 1300 LT) are examined, and vector magnetic field data and energetic electron and ion data from approximately 15 keV to more than 2MeV are employed. Four primary types of studies are carried out: (1) timing and morphology of energetic particle injections; (2) variation of particle phase space densities, using local magnetic field and particle flux data; (3) measurement of boundary motions, using high-energy ion gradient anisotropies; and (4) adiabatic modeling, which included injection, large-scale convection, corotation, and gradient drifts. For the 1200 UT substorms, it is concluded that there was a substantial flux dropout in a broad sector near local midnight because of a large-scale boundary motion, followed by a recovery to a predropout configuration.

Baker, D. N.↗