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Investigating the impacts of Saharan dust on tropical deep convection using spectral bin microphysics

Abstract. To better understand the impacts of dust aerosols on deep convective cloud (DCC) systems reported by previous observational studies, a case study in the tropical eastern Atlantic was investigated using the Weather Research and Forecasting (WRF) model coupled with a spectral bin microphysics (SBM) model. A detailed set of ice nucleation parameterizations linking ice formation with aerosol particles has been implemented in the SBM. Increasing ice nuclei (IN) concentration in the dust cases results in the formation of more numerous small ice particles in the heterogeneous nucleation regime (between −5 and −38 °C) compared to the background ( Clean ) case. Convective updrafts are invigorated by increased latent heat release due to depositional growth and riming of these more numerous particles, which results in increased overshooting and higher convective core top heights. Competition between the more numerous particles for available water vapor during diffusional growth and available smaller crystals and/or drops during collection reduces particle growth rates and shifts precipitation formation to higher altitudes in the heterogeneous nucleation regime. A greater number of large snow particles form in the dust cases, which are transported from the core into the stratiform regime and sediment out quickly. Together with reduced homogeneous ice formation, the stratiform and/or anvil cloud occurrence shifts frequency to warmer temperatures and reduces anvil cloud extents. Total surface precipitation accumulation is reduced proportionally as IN concentration is increased; though the stratiform precipitation accumulation is increased due to greater snow formation and growth, it does not counteract the reduced convective accumulation due to less efficient graupel formation. Radar reflectivity values are increased in the dust cases at temperatures below 0 °C in both the convective and stratiform regimes due to more large snow particles, and reduced in the convective core near the surface due to melt of small ice or graupel particles, consistent with case study observations.

54 ENVIRONMENTAL SCIENCES↗

Aerosol Impacts on Mesoscale Convective Systems Forming Under Different Vertical Wind Shear Conditions

Following our previous study of wind shear effect on mesoscale convective system (MCS) organization under a clean atmospheric condition using the Weather Research and Forecasting model coupled with Spectral-Bin Microphysics, we conduct sensitivity simulations by increasing cloud condensation nuclei (CCN) concentration and investigate aerosol impacts on MCSs forming under different wind shear conditions. We find that, aerosols induce stronger updrafts and downdrafts in all MCSs. The stronger updrafts and enlarged convective core area contribute to larger vertical mass fluxes and enhance precipitation, indicating convective invigoration. Increased updraft speed below 8-km altitude mainly results from enhanced condensational heating, and increased water loading effect is not large enough to overcome the increase in thermal buoyancy. Interestingly, above 8-km altitude we see reduced updraft speed by the increased aerosols due to reduced vertical pressure perturbation gradient force, and weakened depositional growth due to competition of water vapor by enhanced condensation. The accumulated rainfall and mean rain rate are increased, with an increased occurrence frequency of heavy rain. The increase of rain rate is seen in both convective and stratiform regions, with a more significant increase in convective rain rate. In general, we see a higher frequency of deep convective cloud in the polluted condition because of invigorated convection, and more stratiform/anvil clouds, but a lower frequency of shallow warm clouds. The unanimously invigorated MCSs by aerosols under various wind shear conditions revealed by this study has an important implication in weather and climate at warm and humid regions that are influenced by pollution.

54 ENVIRONMENTAL SCIENCES↗

Climatology of the Vertical Profiles of Polarimetric Radar Variables and Retrieved Microphysical Parameters in Continental/Tropical MCSs and Landfalling Hurricanes

Most existing cloud models tend to overestimate the size of cloud ice particles and underestimate their concentration. This emphasizes the need to provide a reliable observational reference to optimize cloud model performance, particularly in areas of high concentration of ice at high altitudes. The dual-polarization radars give the community a unique opportunity to quantify cloud ice with a good accuracy using polarimetric radar retrievals. Here, in this study, we utilize the network of operational WSR-88D radars to build a climatology of the vertical profiles of radar variables, such as radar reflectivity Z, differential reflectivity Z DR , and specific differential phase K DP as well as the radar-retrieved vertical profiles of ice water content (IWC) above the melting layer and liquid water content below it, mean volume diameter D m , and total number concentration N t of ice and liquid particles. Such climatology was created for continental/marine mesoscale convective systems (MCSs) and tropical cyclones including hurricanes. The dataset includes 13 continental MCSs, 10 marine MCSs, and 11 tropical cyclones. Separate statistics of the “background” vertical profiles and the ones associated with high IWC aloft have been obtained in the course of this study. It is shown that continental MCSs exhibit larger size of ice in lower concentration aloft compared to the marine MCSs and especially tropical cyclones/hurricanes. A combination of high KDP and low Z aloft signifies lower D m , higher N t , and often substantial IWC.

54 ENVIRONMENTAL SCIENCES↗

Diurnal Cycle of Convection in the East Pacific ITCZ during EPIC-2001

During the last three weeks of September 2001, the EPIC-2001 intensive field campaign focused on studies of deep convection in the ITCZ over the Mexican warm pool region (10N, 95W) of the East Pacific. This study focuses on the pronounced observed diurnal cycle of environmental and convective parameters within the experiment domain. Data from three primary sources are examined: the R/V Ronald H. Brown C-band weather radar, 4-hourly soundings from the Brown and the Global Atmospherics, Inc. National Lightning Detection Network (long range product). Satellite data from TRMM, GOES and OV-1 are also used. The domain boundary layer shows a robust daily evolution of moist enthalpy (as reflect by equivalent potential temperature, theta-e, or wet bulb potential temperature, theta-w), with contributions from changes in both dry and moist entropy. Peak theta-w is found after local nightfall; the average diurnal range of theta-w is approximately 1 deg C. A composite diurnal cycle of convective properties was derived from the C-band volume scans, sampled continuously through the experiment at 10 minute updates. Products derived from the volumetric data include a surface PPI, 15 and 30 dBZ echo top height, vertically integrated liquid, and 6 km (mixed phase region) reflectivity CAPPIs. For almost all products, the parameter means showed virtually no diurnal cycle. However, for the upper-level products, the parameter spectra showed a clear peak in the occurrence of deep/vigorous convection (the "tail end of the distribution") between 7-9 UTC (1-3 AM local), while overall frequency of occurrence peaked later, from 12-15 UTC (6-9 AM local). This represents a daily "outbreak" of isolated deep cells a couple of hours after sunset and subsequent growth, organization and decay through the nighttime hours. The coherence of the diurnal cycle of the convective spectrum is impressive given the wide variety of convective organization observed during the experiment, and given the modulation by passage of 3-5 day easterly waves. While earlier satellite OLR composites suggested an offshore coastal migration of storms into the domain at night, examination of the 150 km and 300 km range radar products showed little evidence of such organization; almost all convection developed "in-place" within the analysis domain. Consistent with the diurnal thermodynamic and microphysical evolution, a clear cycle in cloud-to-ground (CG) lightning occurrence was observed. The local CG diurnal cycle is significantly stronger than the satellite-derived tropical ocean diurnal cycle of total (IC+CG) lightning. Flash rates of 3-4 fl/min were often visually observed after nightfall; these are fairly 'healthy' flash rates for tropical ocean storms, and the domain was qualitatively noted to be unusually lightning-productive by the R/V Brown crew (also consistent with satellite-based climatologies).

Boccippio, Dennis J.↗

TPSAS-NF1676L-18612-DND

Can a space-based elastic backscatter lidar and coincident infrared radiometer recognize the varied microphysical properties observed by aircraft-based cloud probes in cirrus clouds? If so, then the global and continuous coverage provided by the satellite instruments can extend the knowledge about cirrus cloud properties gained from intensive aircraft field campaigns. The recent Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) aircraft field mission that occurred during August and September, 2013 is an ideal data set to use to test whether this is possible. During SEAC4RS there was extensive sampling of cirrus clouds occurring in widely varied conditions, including the North American Monsoon, forest fires, midlatitude frontal convection and tropical convection. Aircraft cloud probe sampling (2D-S, FCDP or FSSP, CPI) was performed from three airplanes, often coordinated with remote sensing by an aircraft-based elastic backscatter lidar (CPL). During the mission the CALIPSO satellite also observed these clouds from space with a similar elastic backscatter lidar (CALIOP) and an infrared radiometer (IIR). There are several cases where the airplanes sampled directly along the satellite track, but also many overpasses of the region and these features that were not coincident with the aircraft-based sampling. This presentation seeks to address the question of whether relationships between the cloud particle size distribution measurements and habits observed by the SPEC cloud probes and CPL aircraft lidar parameters can be up-scaled to classify the CALIPSO satellite observations from this region and time period. The lidar can also provide cloud top information and evidence of whether there was irreversible transport of ice and aerosols into the UT/LS.

Melody Avery↗

Cirrus clouds. I - A cirrus cloud model. II - Numerical experiments on the formation and maintenance of cirrus

A simplified cirrus cloud model is presented which may be used to investigate the role of various physical processes in the life cycle of a cirrus cloud. The model is a two-dimensional, time-dependent, Eulerian numerical model where the focus is on cloud-scale processes. Parametrizations are developed to account for phase changes of water, radiative processes, and the effects of microphysical structure on the vertical flux of ice water. The results of a simulation of a thin cirrostratus cloud are given. The results of numerical experiments performed with the model are described in order to demonstrate the important role of cloud-scale processes in determining the cloud properties maintained in response to larger scale forcing. The effects of microphysical composition and radiative processes are considered, as well as their interaction with thermodynamic and dynamic processes within the cloud. It is shown that cirrus clouds operate in an entirely different manner than liquid phase stratiform clouds.

Starr, D. OC.↗

Aerosol-Cloud Interactions From Aviation Soot Emissions

Current models estimate global aviation contributes approximately 5% to the total anthropogenic climate forcing, with aerosol-cloud interactions having the greatest effect. However, radiative forcing estimates from aviation aerosol-cloud interactions remain undetermined. There is an expected significant increase in aircraft emissions with aviation demand expected to rise by over 4% per year. Soot may play an important role in the ice nucleation of aircraft-induced cirrus formation due to a high emission rate, but the ice nucleating properties are poorly constrained. Understanding the microphysical processes leading to atmospheric ice crystal formation is crucial for the reliable parameterization of aerosol-cloud interactions in climate models due to their impact on precipitation and cloud radiative properties. Ice nucleation of aircraft-emitted soot is potentially affected by particle morphology with condensation of supercooled water occurring in pores followed by ice nucleation. However, soot has heterogeneous properties and undergoes atmospheric aging and oxidation that could change surface properties and contribute to complex ice nucleation processes. Further, this review synthesizes current knowledge of ice nucleation catalyzed by aviation in the cirrus regime and its effects on global radiative forcing. Further research is required to determine the ice nucleation and microphysical processes of cirrus cloud formation from aviation emissions in both controlled laboratory and field investigations to inform models for more accurate climate predictions and to provide efficient mitigation strategies.

54 ENVIRONMENTAL SCIENCES↗

Self-Supervised Cloud Classification

Abstract Low-level marine clouds play a pivotal role in Earth’s weather and climate through their interactions with radiation, heat and moisture transport, and the hydrological cycle. These interactions depend on a range of dynamical and microphysical processes that result in a broad diversity of cloud types and spatial structures, and a comprehensive understanding of cloud morphology is critical for continued improvement of our atmospheric modeling and prediction capabilities moving forward. Deep learning has recently accelerated our ability to study clouds using satellite remote sensing, and machine learning classifiers have enabled detailed studies of cloud morphology. A major limitation of deep learning approaches to this problem, however, is the large number of hand-labeled samples that are required for training. This work applies a recently developed self-supervised learning scheme to train a deep convolutional neural network (CNN) to map marine cloud imagery to vector embeddings that capture information about mesoscale cloud morphology and can be used for satellite image classification. The model is evaluated against existing cloud classification datasets and several use cases are demonstrated, including training cloud classifiers with very few labeled samples, interrogation of the CNN’s learned internal feature representations, cross-instrument application, and resilience against sensor calibration drift and changing scene brightness. The self-supervised approach learns meaningful internal representations of cloud structures and achieves comparable classification accuracy to supervised deep learning methods without the expense of creating large hand-annotated training datasets. Significance Statement Marine clouds heavily influence Earth’s weather and climate, and improved understanding of marine clouds is required to improve our atmospheric modeling capabilities and physical understanding of the atmosphere. Recently, deep learning has emerged as a powerful research tool that can be used to identify and study specific marine cloud types in the vast number of images collected by Earth-observing satellites. While powerful, these approaches require hand-labeling of training data, which is prohibitively time intensive. This study evaluates a recently developed self-supervised deep learning method that does not require human-labeled training data for processing images of clouds. We show that the trained algorithm performs competitively with algorithms trained on hand-labeled data for image classification tasks. We also discuss potential downstream uses and demonstrate some exciting features of the approach including application to multiple satellite instruments, resilience against changing image brightness, and its learned internal representations of cloud types. The self-supervised technique removes one of the major hurdles for applying deep learning to very large atmospheric datasets.

54 ENVIRONMENTAL SCIENCES↗

Application of the CloudSat and NEXRAD Radars Toward Improvements in High Resolution Operational Forecasts

As computational power increases, operational forecast models are performing simulations with higher spatial resolution allowing for the transition from sub-grid scale cloud parameterizations to an explicit forecast of cloud characteristics and precipitation through the use of single- or multi-moment bulk water microphysics schemes. investments in space-borne and terrestrial remote sensing have developed the NASA CloudSat Cloud Profiling Radar and the NOAA National Weather Service NEXRAD system, each providing observations related to the bulk properties of clouds and precipitation through measurements of reflectivity. CloudSat and NEXRAD system radars observed light to moderate snowfall in association with a cold-season, midlatitude cyclone traversing the Central United States in February 2007. These systems are responsible for widespread cloud cover and various types of precipitation, are of economic consequence, and pose a challenge to operational forecasters. This event is simulated with the Weather Research and Forecast (WRF) Model, utilizing the NASA Goddard Cumulus Ensemble microphysics scheme. Comparisons are made between WRF-simulated and observed reflectivity available from the CloudSat and NEXRAD systems. The application of CloudSat reflectivity is made possible through the QuickBeam radiative transfer model, with cautious application applied in light of single scattering characteristics and spherical target assumptions. Significant differences are noted within modeled and observed cloud profiles, based upon simulated reflectivity, and modifications to the single-moment scheme are tested through a supplemental WRF forecast that incorporates a temperature dependent snow crystal size distribution.

Molthan, A. L.↗

Parameterizing deep convection using the assumed probability density function method

Due to their coarse horizontal resolution, present-day climate models must parameterize deep convection. This paper presents single-column simulations of deep convection using a probability density function (PDF) parameterization. The PDF parameterization predicts the PDF of subgrid variability of turbulence, clouds, and hydrometeors. That variability is interfaced to a prognostic microphysics scheme using a Monte Carlo sampling method.The PDF parameterization is used to simulate tropical deep convection, the transition from shallow to deep convection over land, and mid-latitude deep convection.These parameterized single-column simulations are compared with 3-D reference simulations. The agreement is satisfactory except when the convective forcing is weak. The same PDF parameterization is also used to simulate shallow cumulus and stratocumulus layers. The PDF method is sufficiently general to adequately simulate these five deep, shallow, and stratiform cloud cases with a single equation set. This raises hopes that it may be possible in the future, with further refinements at coarse time step and grid spacing, to parameterize all cloud types in a large-scale model in a unified way.

Storer, R. L.↗

Climate Impacts of Ice Nucleation

Several different ice nucleation parameterizations in two different General Circulation Models (GCMs) are used to understand the effects of ice nucleation on the mean climate state, and the Aerosol Indirect Effects (AIE) of cirrus clouds on climate. Simulations have a range of ice microphysical states that are consistent with the spread of observations, but many simulations have higher present-day ice crystal number concentrations than in-situ observations. These different states result from different parameterizations of ice cloud nucleation processes, and feature different balances of homogeneous and heterogeneous nucleation. Black carbon aerosols have a small (0.06 Wm(exp-2) and not statistically significant AIE when included as ice nuclei, for nucleation efficiencies within the range of laboratory measurements. Indirect effects of anthropogenic aerosols on cirrus clouds occur as a consequence of increasing anthropogenic sulfur emissions with different mechanisms important in different models. In one model this is due to increases in homogeneous nucleation fraction, and in the other due to increases in heterogeneous nucleation with coated dust. The magnitude of the effect is the same however. The resulting ice AIE does not seem strongly dependent on the balance between homogeneous and heterogeneous ice nucleation. Regional effects can reach several Wm2. Indirect effects are slightly larger for those states with less homogeneous nucleation and lower ice number concentration in the base state. The total ice AIE is estimated at 0.27 +/- 0.10 Wm(exp-2) (1 sigma uncertainty). This represents a 20% offset of the simulated total shortwave AIE for ice and liquid clouds of 1.6 Wm(sup-2).

Gettelman, Andrew↗

Application of Radon Transform to Multi-Angle Measurements Made by the Research Scanning Polarimeter: A New Approach to Cloud Tomography. Part I: Theory and Tests on Simulated Data.

The Research Scanning Polarimeter (RSP) is an airborne along-track scanner measuring the polarized and total reflectances in 9 spectral channels. The RSP was a prototype for the Aerosol Polarimetry Sensor (APS) launched on-board the NASA Glory satellite. Currently the retrieval algorithms developed for the RSP are being adopted for the measurements of the space-borne polarimeters on the upcoming NASA’s Plankton, Aerosol, Cloud Ocean Ecosystem (PACE)satellite mission. The RSP’s uniquely high angular resolution coupled with the high frequency of measurements allows for characterization of liquid water cloud droplet sizes using the polarized rainbow structure. It also provides geometric constraints on the cumulus cloud’s 2D cross section yielding the cloud’s geometric shape estimates. In this study we further build on the latter technique to develop a new tomographic approach to retrieval of cloud internal structure from remote sensing measurements. While tomography in the strict definition is a technique based on active measurements yielding a tomogram (directional optical thickness as a function of angle and offset of the view ray), we developed a “semi-tomographic” approach in which tomogram of the cloud is estimated from passive observations instead of being measured directly. This tomogram is then converted into 2D spatial distribution of the extinction coefficient using inverse Radon transform (filtered back projection) which is the standard tomographic procedure used e.g., in medical CT scans. This algorithm is computationally inexpensive compared to techniques relying on highly-multi-dimensional least-square fitting; it does not require iterative 3D RT simulations. The resulting extinction distribution is defined up to an unknown constant factor, so we discuss the ways to calibrate it using additional independent measurements. In the next step we use the profile of the droplet size distribution parameters from the cloud’s side (derived by fitting the polarized rainbows) to convert the 2D extinction distribution into that of the droplet number concentration. We illustrate and validate the proposed technique using 3D-RT-simulatedRSP observations of a LES-generated Cu cloud. Quantitative comparisons between the retrieved and the original optical and microphysical parameters are presented.

clouds↗

Updraft Dynamics and Microphysics: On the Added Value of The Cumulus Thermal Reference Frame in Simulations of Aerosol–Deep Convection Interactions

One fundamental question about atmospheric moist convection processes that remains debated is whether, or under which conditions, a relevant variability in background aerosol concentrations may have a significant dynamical impact on convective clouds and their associated precipitation. Furthermore, current climate models must parameterize both the microphysical and the cumulus convection processes, but this is usually implemented separately, whereas in nature there is a strong coupling between them. As a first step to improve our understanding of these two problems, we investigate how aerosol concentrations modify key properties of updrafts in eight large-eddy-permitting regional simulations of a case study of scattered convection over Houston, Texas, in which convection is explicitly simulated and microphysical processes are parameterized. Dynamical and liquid-phase microphysical responses are investigated using the following two different reference frames: static cloudy updraft grid cells versus tracked cumulus thermals. In both frameworks, we observe the expected microphysical responses to higher aerosol concentrations, such as higher cloud number concentrations and lower rain number concentrations. In terms of the dynamical responses, both frameworks indicate weak impacts of varying aerosol concentrations relative to the noise between simulations over the observationally derived range of aerosol variability for this case study. On the other hand, results suggest that thermals are more selective than cloudy updraft grid cells in terms of sampling the most active convective air masses. For instance, vertical velocity from thermals is significantly higher at upper levels than when sampled from cloudy updraft grid points, and several microphysical variables have higher average values in the cumulus thermal framework than in the cloudy updraft framework. In addition, the thermal analysis is seen to add rich quantitative information about the rates and covariability of microphysical processes spatially and throughout tracked thermal lifecycles, which can serve as a stronger foundation for improving subgrid-scale parameterizations.

aerosols↗

Retrieving microphysical properties of concurrent pristine ice and snow using polarimetric radar observations

Abstract. Ice and mixed-phase clouds play a key role in our climate system because of their strong controls on global precipitation and radiation budget. Their microphysical properties have been characterized commonly by polarimetric radar measurements. However, there remains a lack of robust estimates of microphysical properties of concurrent pristine ice and aggregates because larger snow aggregates often dominate the radar signal and mask contributions of smaller pristine ice crystals. This paper presents a new method that separates the scattering signals of pristine ice embedded in snow aggregates in scanning polarimetric radar observations and retrieves their respective abundances and sizes for the first time. This method, dubbed ENCORE-ice, is built on an iterative stochastic ensemble retrieval framework. It provides the number concentration, ice water content, and effective mean diameter of pristine ice and snow aggregates with uncertainty estimates. Evaluations against synthetic observations show that the overall retrieval biases in the combined total microphysical properties are within 5 % and that the errors with respect to the truth are well within the retrieval uncertainty. The partitioning between pristine ice and snow aggregates also agrees well with the truth. Additional evaluations against in situ cloud probe measurements from a recent campaign for a stratiform cloud system are promising. Our median retrievals have a bias of 98 % in the total ice number concentration and 44 % in the total ice water content. This performance is generally better than the retrieval from empirical relationships. The ability to separate signals of different ice species and to provide their quantitative microphysical properties will open up many research opportunities, such as secondary ice production studies and model evaluations for ice microphysical processes.

54 ENVIRONMENTAL SCIENCES↗

Microphysics, Radiation and Surface Processes in the Goddard Cumulus Ensemble (GCE) Model

The response of cloud systems to their environment is an important link in a chain of processes responsible for monsoons, frontal depression, El Nino Southern Oscillation (ENSO) episodes and other climate variations (e.g., 30-60 day intra-seasonal oscillations). Numerical models of cloud properties provide essential insights into the interactions of clouds with each other, with their surroundings, and with land and ocean surfaces. Significant advances are currently being made in the modeling of rainfall and rain-related cloud processes, ranging in scales from the very small up to the simulation of an extensive population of raining cumulus clouds in a tropical- or midlatitude-storm environment. The Goddard Cumulus Ensemble (GCE) model is a multi-dimensional nonhydrostatic dynamic/microphysical cloud resolving model. It has been used to simulate many different mesoscale convective systems that occurred in various geographic locations. In this paper, recent GCE model improvements (microphysics, radiation and surface processes) will be described as well as their impact on the development of precipitation events from various geographic locations. The performance of these new physical processes will be examined by comparing the model results with observations. In addition, the explicit interactive processes between cloud, radiation and surface processes will be discussed.

Tao, Wei-Kuo↗

Dual-frequency (Ka-band and G-band) radar estimates of liquid water content profiles in shallow clouds

The profile of the liquid water content (LWC) in clouds provides fundamental information for understanding the internal structure of clouds, their radiative effects, propensity to precipitate, and degree of entrainment and mixing with the surrounding environment. In principle, differential absorption techniques based on coincident dual-frequency radar reflectivity observations have the potential to provide the LWC profile. Previous differential frequency radar reflectivity (DFR) efforts were challenged by the fact that the measurable differential attenuation for small quantities of LWC is usually comparable to the system measurement error. This typically renders the retrieval impractical, as the uncertainty can become many times greater than the retrieved value itself. Theoretically, this drawback can be mitigated following two interconnected approaches: (1) increasing the frequency separation between the dual-frequency radar system to measure greater differential attenuation and (2) increasing the radar operating frequency to reduce the instrument measurement random error. Our recently developed 239 GHz radar was deployed during the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) along with a variety of collocated remote sensing and in situ instruments. We have combined Ka-band (35 GHz) and G-band (239 GHz) observations to retrieve the LWC from more than 100 vertical profiles of shallow clouds with typical amounts of LWC smaller than 1 g m -3 . We theoretically and experimentally demonstrate that the Ka-band and G-band pair of frequencies offers at least a 65 % relative improvement in the LWC retrieval sensitivity compared to previous works reported in the literature using lower-frequency radars. This new technique provides a missing capability to determine the LWC in the challenging low liquid water path (LWP) range (< 200 g m -2 ) and suggests a way forward to characterize microphysical and dynamical processes more precisely in shallow clouds.

54 ENVIRONMENTAL SCIENCES↗

Understanding aerosol–cloud interactions using a single-column model for a cold-air outbreak case during the ACTIVATE campaign

Marine boundary layer clouds play a critical role in Earth's energy balance. Their microphysical and radiative properties are highly impacted by ambient aerosols and dynamic forcings. In this study, we evaluate the representation of these clouds and related aerosol–cloud interaction processes in the single-column version of the E3SM climate model (SCM) against field measurements collected during the NASA ACTIVATE campaign over the western North Atlantic, as well as intercompare results with high-resolution process level models. We show that E3SM SCM reproduces the macrophysical properties of post-frontal boundary layer clouds in a cold-air outbreak (CAO) case well. However, it generates fewer but larger cloud droplets compared to aircraft measurements. Further sensitivity tests show that the underestimation of both aerosol number concentration and vertical velocity variance contributes to this bias. Aerosol–cloud interactions are examined by perturbing prescribed aerosol properties in E3SM SCM with fixed dynamics. Higher aerosol number concentration or hygroscopicity leads to more numerous but smaller cloud droplets, resulting in a stronger cooling via shortwave cloud forcing. This apparent Twomey effect is consistent with prior climate model studies. The cloud liquid water path shows a weakly positive relation with cloud droplet number concentration due to precipitation suppression. This weak aerosol effect on cloud macrophysics may be attributed to the dominant impact of strong dynamical forcing associated with the CAO. Our findings indicate that the SCM framework is a key tool to bridge the gap between climate models, process level models, and field observations to facilitate process level understanding.

54 ENVIRONMENTAL SCIENCES↗

Updraft dynamics and microphysics: on the added value of the cumulus thermal reference frame in simulations of aerosol–deep convection interactions

One fundamental question about atmospheric moist convection processes that remains debated is whether, or under which conditions, a relevant variability in background aerosol concentrations may have a significant dynamical impact on convective clouds and their associated precipitation. Furthermore, current climate models must parameterize both the microphysical and the cumulus convection processes, but this is usually implemented separately, whereas in nature there is a strong coupling between them. As a first step to improve our understanding of these two problems, we investigate how aerosol concentrations modify key properties of updrafts in eight large-eddy-permitting regional simulations of a case study of scattered convection over Houston, Texas, in which convection is explicitly simulated and microphysical processes are parameterized. Dynamical and liquid-phase microphysical responses are investigated using the following two different reference frames: static cloudy updraft grid cells versus tracked cumulus thermals. In both frameworks, we observe the expected microphysical responses to higher aerosol concentrations, such as higher cloud number concentrations and lower rain number concentrations. In terms of the dynamical responses, both frameworks indicate weak impacts of varying aerosol concentrations relative to the noise between simulations over the observationally derived range of aerosol variability for this case study. On the other hand, results suggest that thermals are more selective than cloudy updraft grid cells in terms of sampling the most active convective air masses. For instance, vertical velocity from thermals is significantly higher at upper levels than when sampled from cloudy updraft grid points, and several microphysical variables have higher average values in the cumulus thermal framework than in the cloudy updraft framework. In addition, the thermal analysis is seen to add rich quantitative information about the rates and covariability of microphysical processes spatially and throughout tracked thermal lifecycles, which can serve as a stronger foundation for improving subgrid-scale parameterizations.

54 ENVIRONMENTAL SCIENCES↗