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At least 1,531 records · Page 85
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Burning conditions and transportation pathways determine biomass-burning aerosol properties in the Ascension Island marine boundary layer

Abstract. African biomass-burning aerosol (BBA) in the southeast Atlantic Ocean (SEA) marine boundary layer (MBL) is an important contributor to Earth's radiation budget, yet its representation remains poorly constrained in regional and global climate models. Data from the Layered Atlantic Smoke Interactions with Clouds (LASIC) field campaign on Ascension Island (7.95° S, 14.36° W) provide insight into how burning conditions, fuel type, transport pathways, and atmospheric processing affect the chemical, microphysical, and optical properties of BBA between June and September 2017. A total of 10 individual plume events characterize the seasonal evolution of the BBA properties. Early-season inefficient fires, determined by low refractory black carbon to above-background carbon monoxide mixing ratios (rBC : ΔCO), led to enhanced concentrations of organic- and sulfate-rich aerosols. Mid-season efficient fires, determined by higher rBC : ΔCO values, led to rBC-enriched BBA. A mix of efficient and inefficient fires later in the season resulted in conflicting BBA properties. Prolonged transport (∼ 10 d) through the MBL and lower free troposphere (FT) facilitated chemical and aqueous-phase processing, which led to a reduction in organic aerosol mass concentrations. This resulted in lower organic aerosol (OA) to rBC (OA : rBC) mass ratios (2–5) in the MBL compared to higher values (5–15) in the nearby FT. These atmospheric and cloud oxidation processes yield more light-absorbing BBA and explain the notably low single-scattering albedo at 530 nm (SSA530) values (< 0.80) observed in the MBL. This study establishes a robust correlation between SSA530 and OA : rBC across the MBL and FT, underscoring the dependency of optical properties on chemical composition.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1991

Plasma waves at Venus

Many significant wave phenomena have been discovered at Venus with the plasma wave instrument on the Pioneer Venus Orbiter. It has been shown that whistler-mode waves in the magnetosheath of the planet may be an important source of energy for the topside ionosphere. Plasma waves are also associated with thickening of the ionopause current layer. Current-generated waves in plasma clouds may also provide anomalous resistance resulting in electron acceleration, possibly producing aurora. Ion-acoustic waves are observed in the bow shock, and appear to be a feature of the magnetotail boundary. Lastly, plasma waves have been cited as evidence for lightning on Venus.

Strangeway, R. J.↗
NASA NTRS1999

Climatic Implications of the Observed Temperature Dependence of the Liquid Water Path of Low Clouds in the Southern Great Plains

Satellite observations of low-level clouds have challenged the assumption that adiabatic liquid water content combined with constant physical thickness will lead to a negative cloud optics feedback in a decadal climate change. We explore the reasons for the satellite results using four years of surface remote sensing data from the Atmospheric Radiation Measurement Program Cloud and Radiation Testbed site in the Southern Great Plains of the United States. We find that low cloud liquid water path is approximately invariant with temperature in winter but decreases strongly with temperature in summer, consistent with the satellite inferences at this latitude. This behavior occurs because liquid water content shows no detectable temperature dependence while cloud physical thickness decreases with warming. Thinning of clouds with warming is observed on seasonal, synoptic, and diurnal time scales; it is most obvious in the warm sectors of baroclinic waves. Although cloud top is observed to slightly descend with warming, the primary cause of thinning is the ascent of cloud base due to the reduction in surface relative humidity and the concomitant increase in the lifting condensation level of surface air. Low cloud liquid water path is not observed to be a continuous function of temperature. Rather, the behavior we observe is best explained as a transition in the frequency of occurrence of different boundary layer types: At cold temperatures, a mixture of stratified and convective boundary layers is observed, leading to a broad distribution of liquid water path values, while at warm temperatures, only convective boundary layers with small liquid water paths, some of them decoupled, are observed. Our results, combined with the earlier satellite inferences, imply that the commonly quoted 1.50 C lower limit for the equilibrium global climate sensitivity to a doubling of CO2, which is based on models with near-adiabatic liquid water behavior and constant physical thickness, should be revised upward.

DelGenio, Anthony D.↗
NASA NTRS1999

Climatic Implications of the Observed Temperature Dependence of the Liquid Water Path of Low Clouds in the Southern Great Plains

Satellite observations of low-level clouds have challenged the assumption that adiabatic liquid water content combined with constant physical thickness will lead to a negative cloud optics feedback in a decadal climate change. We explore the reasons for the satellite results using four years of surface remote sensing data from the Atmospheric Radiation Measurement Program Cloud and Radiation Testbed site in the Southern Great Plains of the United States. We find that low cloud liquid water path is approximately invariant with temperature in winter but decreases strongly with temperature in summer, consistent with the satellite inferences at this latitude. This behavior occurs because liquid water content shows no detectable temperature dependence while cloud physical thickness decreases with warming. Thinning of clouds with warming is observed on seasonal, synoptic, and diurnal time scales; it is most obvious in the warm sectors of baroclinic waves. Although cloud top is observed to slightly descend with warming, the primary cause of thinning, is the ascent of cloud base due to the reduction in surface relative humidity and the concomitant increase in the lifting condensation level of surface air. Low cloud liquid water path is not observed to be a continuous function of temperature. Rather, the behavior we observe is best explained as a transition in the frequency of occurrence of different boundary layer types. At cold temperatures, a mixture of stratified and convective boundary layers is observed, leading to a broad distribution of liquid water path values, while at warm temperatures, only convective boundary layers with small liquid water paths, some of them decoupled, are observed. Our results, combined with the earlier satellite inferences, imply that the commonly quoted 1.5C lower limit for the equilibrium global climate sensitivity to a doubling of CO2 which is based on models with near-adiabatic liquid water behavior and constant physical thickness, should be revised upward.

DelGenio, Anthony↗
NASA NTRS2004

Examination of Surface Roughness on Light Scattering by Long Ice Columns by Use of a Two-Dimensional Finite-Difference Time-Domain Algorithm

Natural particles such as ice crystals in cirrus clouds generally are not pristine but have additional micro-roughness on their surfaces. A two-dimensional finite-difference time-domain (FDTD) program with a perfectly matched layer absorbing boundary condition is developed to calculate the effect of surface roughness on light scattering by long ice columns. When we use a spatial cell size of 1/120 incident wavelength for ice circular cylinders with size parameters of 6 and 24 at wavelengths of 0.55 and 10.8 mum, respectively, the errors in the FDTD results in the extinction, scattering, and absorption efficiencies are smaller than similar to 0.5%. The errors in the FDTD results in the asymmetry factor are smaller than similar to 0.05%. The errors in the FDTD results in the phase-matrix elements are smaller than similar to 5%. By adding a pseudorandom change as great as 10% of the radius of a cylinder, we calculate the scattering properties of randomly oriented rough-surfaced ice columns. We conclude that, although the effect of small surface roughness on light scattering is negligible, the scattering phase-matrix elements change significantly for particles with large surface roughness. The roughness on the particle surface can make the conventional phase function smooth. The most significant effect of the surface roughness is the decay of polarization of the scattered light.

Sun, W.↗
NASA NTRS2005

Variability and Extremes of Precipitation in the Global Climate as Determined by the 25-Year GEWEX/GPCP Data Set

The Global Precipitation Climatology Project (GPCP) 25-year precipitation data set is used to evaluate the variability and extremes on global and regional scales. The variability of precipitation year-to-year is evaluated in relation to the overall lack of a significant global trend and to climate events such as ENSO and volcanic eruptions. The validity of conclusions and limitations of the data set are checked by comparison with independent data sets (e.g., TRMM). The GPCP data set necessarily has a heterogeneous time series of input data sources, so part of the assessment described above is to test the initial results for potential influence by major data boundaries in the record. Regional trends, or inter-decadal changes, are also analyzed to determine validity and correlation with other long-term data sets related to the hydrological cycle (e.g., clouds and ocean surface fluxes). Statistics of extremes (both wet and dry) are analyzed at the monthly time scale for the 25 years. A preliminary result of increasing frequency of extreme monthly values will be a focus to determine validity. Daily values for an eight-year are also examined for variation in extremes and compared to the longer monthly-based study.

Adler, R. F.↗
DOE OSTI2019

Cloud Influence on ERA5 and AMPS Surface Downwelling Longwave Radiation Biases in West Antarctica

The surface downwelling longwave radiation component (LW?) is crucial for the determination of the surface energy budget and has significant implications for the resilience of ice surfaces in the polar regions. Accurate model evaluation of this radiation component requires knowledge about the phase, vertical distribution, and associated temperature of water in the atmosphere, all of which control the LW? signal measured at the surface. In this study, we examine the LW? model errors found in the Antarctic Mesoscale Prediction System (AMPS) operational forecast model and the ERA5 reanalysis model relative to observations from the AWARE campaign at McMurdo Station and the West Antarctic Ice Sheet (WAIS) Divide. The errors are calculated separately for observed clear sky conditions, ice cloud occurrences, and liquid-bearing cloud layer (LBCL) occurrences. The analysis results show a tendency (in both models at each site) to underestimate the LW? during clear sky conditions, high error variability (standard deviations > 20 W/m2) during any type of cloud occurrence, and negative LW? biases when LBCLs are observed (bias magnitudes > 15 W/m2 in tenuous LBCL cases; > 43 W/m2 in optically thick/opaque LBCLs instances). We suggest that a generally dry and liquid water-deficient atmosphere responsible for the identified LW? biases in both models is the result of excessive ice formation and growth, which could stem from model initial and lateral boundary conditions, microphysics scheme, aerosol representation, and/or limited vertical resolution.

Silber, Israel↗
NASA NTRS2003

Boundary Conditions of the Heliosphere

As described in the Revised Task Statement for this grant (submitted following the award at a reduced budget), my role in these investigations is to focus on the theoretical calculations relevant to the ionization state and dust content of the Local Cloud that surrounds the Solar System. An important motivation for our investigations is to aid in the interpretation of pick-up ion (PUI) and anomalous cosmic ray (ACR) observations which depends on knowledge of the flux of neutral atoms of various elements into the heliosphere. This flux depends on the ionization and elemental abundances of the gas of the Local Cloud. We have made substantial progress in our program to understand the ionization of the Local Cloud. Our steady state photoionization models are remarkably successful in accounting for the ionization observed both by line of sight (column density) observations towards nearby stars and in situ measurements. By lifting some of the simplifying assumptions in our earlier modeling we hope to make further progress in this understanding. In future work on this project we will continue our exploration of photoionization models, focusing on making sense of the differences between the LIC and the BC. In addition we will explore the effects of altered abundances in the hot gas on the ionization and thermal balance in the LIC.

Frisch, Priscilla C.↗
NASA NTRS1979

Arctic Sea ice decay simulated for a CO2-induced temperature rise

A large scale numerical time-dependent model of sea ice that takes into account the heat fluxes in and out of the ice, the seasonal occurrence of snow, and ice motions was used in an experiment to determine the response of the Arctic Ocean ice pack to a warming of the atmosphere. The degree of warming specified is that expected for a doubling of atmospheric carbon dioxide with its associated greenhouse effect, a condition that could occur before the middle of the next century. The results of three 5-year simulations with a warmer atmosphere and varied boundary conditions were: (1) that in the face of a 5 K surface atmospheric temperature increase the ice pack disappeared completely in August and September but reformed in the central Arctic Ocean in mid fall; (2) that the simulations were moderately dependence on assumptions concerning cloud cover; and (3) that even when atmospheric temperature increases of 6-9 K were combined with an order-of-magnitude increase in the upward heat flux from the ocean, the ice still appeared in winter. It should be noted that a year-round ice-free Arctic Ocean has apparently not existed for a million years or more.

Heat flux↗
DOE OSTI2024

Quantifying the impacts of marine aerosols over the southeast Atlantic Ocean using a chemical transport model: implications for aerosol–cloud interactions

The southeast Atlantic region, characterized by persistent stratocumulus clouds, has one of the highest uncertainties in aerosol radiative forcing and significant variability across climate models. In this study, we analyze the seasonally varying role of marine aerosol sources and identify key uncertainties in aerosol composition at cloud-relevant altitudes over the southeast Atlantic using the GEOS-Chem chemical transport model. We evaluate simulated aerosol optical depth (AOD) and speciated aerosol concentrations against those collected from ground observations and aircraft campaigns such as LASIC, ORACLES, and CLARIFY, conducted during 2017. The model consistently underestimates AOD relative to AERONET, particularly at remote locations like Ascension Island. However, when compared with aerosol mass concentrations from aircraft campaigns during the biomass burning period, it performs adequately at cloud-relevant altitudes, with a normalized mean bias (NMB) between -3.5 % (CLARIFY) and -7.5 % (ORACLES). At these altitudes, in the model, organic aerosols (63 %) dominate during the biomass burning period, while sulfate (41 %) prevails during austral summer, when dimethylsulfide (DMS) emissions peak in the model. Our findings indicate that marine sulfate can account for up to 69 % of total sulfate during the high-DMS period. Sensitivity analyses indicate that refining DMS emissions and oxidation chemistry may increase sulfate aerosol produced from marine sources, highlighting that there remains large uncertainty as to the role of DMS emissions in the marine boundary layer. Additionally, we find marine primary organic aerosol emissions may substantially increase total organic aerosol concentrations, particularly during austral summer. This study underscores the imperative need to refine marine emissions and their chemical transformations, as aerosols from marine sources are a major component of total aerosols at cloud-relevant altitudes and may impact uncertainties in aerosol radiative forcing over the southeast Atlantic.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Atmospheric Boundary Layer Classification With Doppler Lidar

We present a method using Doppler lidar data for identifying the main sources of turbulent mixing within the atmospheric boundary layer. The method identifies the presence of turbulence and then assigns a turbulent source by combining several lidar quantities: attenuated backscatter coefficient, vertical velocity skewness, dissipation rate of turbulent kinetic energy, and vector wind shear. Both buoyancy-driven and shear-driven situations are identified, and the method operates in both clear-sky and cloud-topped conditions, with some reservations in precipitation. To capture the full seasonal cycle, the classification method was applied to more than 1 year of data from two sites, Hyytiälä, Finland, and Jülich, Germany. Analysis showed seasonal variation in the diurnal cycle at both sites; a clear diurnal cycle was observed in spring, summer, and autumn seasons, but due to their respective latitudes, a weaker cycle in winter at Jülich, and almost non-existent at Hyytiälä. Additionally, there are significant contributions from sources other than convective mixing, with cloud-driven mixing being observed even within the first 500 m above ground. Also evident is the considerable amount of nocturnal mixing within the lowest 500 m at both sites, especially during the winter. The presence of a low-level jet was often detected when sources of nocturnal mixing were diagnosed as wind shear. The classification scheme and the climatology extracted from the classification provide insight into the processes responsible for mixing within the atmospheric boundary layer, how variable in space and time these can be, and how they vary with location.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Formation and evolution of protostellar accretion discs – I. Angular-momentum budget, gravitational self-regulation, and numerical convergence

Here, we investigate the formation and early evolution of a protostellar disc from a magnetized prestellar core using non-ideal magnetohydrodynamic (MHD) simulations including ambipolar diffusion and Ohmic dissipation. The dynamical contraction of the prestellar core ultimately leads to the formation of a first hydrostatic core, after ambipolar diffusion decouples the magnetic field from the predominantly neutral gas. The hydrostatic core accumulates angular momentum from the infalling material, evolving into a rotationally supported torus; this ‘first hydrostatic torus’ then forms an accreting protostar and a rotationally supported disc. The disc spreads out by gravitational instability, reaching ~30 au in diameter at ~3 kyr after protostar formation. The total mass and angular momentum of the protostar–disc system are determined mainly by accretion of gas from an infalling pseudo-disc, which has low specific angular momentum because of magnetic braking; their removal from the protostar–disc system by outflow and disc magnetic braking are negligible, in part because the magnetic field is poorly coupled there. The redistribution of angular momentum within the protostar–disc system is facilitated mainly by gravitational instability; this allows formation of relatively large discs even when the specific angular momentum of infalling material is low. We argue that such discs should remain marginally unstable as they grow (with Toomre Q ~ 1–2), an idea that is broadly consistent with recent observational estimates for Class 0/I discs. We discuss the numerical convergence of our results, and show that properly treating the inner boundary condition is crucial for achieving convergence at an acceptable computational cost.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1982

Planetary-scale waves in the Venus atmosphere

Observed wave-like cloud features on Venus, which at times form a Y-like structure which encircles the planet, were modelled numerically. Linearized primitive equations for a shallow, hydrostatic atmosphere are defined, along with upper boundary layer conditions for the 4-6 day periods detected in the atmospheric response to forcing. The basic state of the Venus atmosphere was considered to display variations in static stability and the mean zonal wind as a function of altitude. Forcing was introduced over a wide range of frequencies in order to produce the target oscillation modes. Combination of a midlatitude Rossby wave and an equatorial Kelvin wave was found to yield the observed Y-shape, which could be preserved with nonlinear coupling.

Covey, C.↗
NASA NTRS1989

Mesoscale acid deposition modeling studies

The work performed in support of the EPA/DOE MADS (Mesoscale Acid Deposition) Project included the development of meteorological data bases for the initialization of chemistry models, the testing and implementation of new planetary boundary layer parameterization schemes in the MASS model, the simulation of transport and precipitation for MADS case studies employing the MASS model, and the use of the TASS model in the simulation of cloud statistics and the complex transport of conservative tracers within simulated cumuloform clouds. The work performed in support of the NASA/FAA Wind Shear Program included the use of the TASS model in the simulation of the dynamical processes within convective cloud systems, the analyses of the sensitivity of microburst intensity and general characteristics as a function of the atmospheric environment within which they are formed, comparisons of TASS model microburst simulation results to observed data sets, and the generation of simulated wind shear data bases for use by the aviation meteorological community in the evaluation of flight hazards caused by microbursts.

Kaplan, Michael L.↗
NASA NTRS1990

Feedback Processes and Climate Response

The response of the climate system to an external perturbation--e.g., a change in solar irradiance or a change in atmospheric opacity due to an increase in CO2--depends rather strongly on feedback processes in the system, which either amplify or dampen the effects of the initial perturbation. A simple representation of the climate system is used to compare several important feedbacks, based upon general circulation model (GCM) simulations by various investigators. The models are in general agreement with respect to water vapor feedback, but in wide disagreement with respect to cloud feedback. Because of the arguments raised by Lindzen (1990)--that the processes which determine water vapor mixing ratio in the upper atmosphere are quite different from those which operate in the planetary boundary layer, and that upper tropospheric water vapor might actually decrease even when the boundary layer is getting warmer and more moist--researchers undertook a study to determine the sensitivity of climate to changes in water vapor at various levels in the troposphere. The result is that climate is just as sensitive to percentage changes in upper tropospheric water vapor, where the mixing ratio is very small, as it is to percentage changes in the boundary layer, which contains the bulk of total column water vapor.

Arking, Albert↗
NASA NTRS2002

Cloud Physics Lidar Optical Measurements During the SAFARI-2000 Field Campaign

In this presentation, we will show new optical data processing results from the Cloud Physics War during SAFARI-2000. Retrieved products include aerosol and cloud layer location and identification, layer optical depths, vertical extinction profiles, and extinction-to-backscatter (S) ratios for 532 and 1064 nm. The retrievals will focus on the persistent and smoky planetary boundary layer and occasional elevated aerosol layers found in southern Africa during August and September 2000.

Hlavka, Dennis L.↗
NASA NTRS2011

A Summary of the Flux-Rope CDAW events

In this paper, I summarize some of the results obtained during previous CDAW on the events selected for analysis. The events were selected based on the following criteria: 1. The events must be well observed in the interplanetary medium as shock-driving interplanetary coronal mass ejections (ICMEs), 2. The ICMEs should have corresponding CMEs near the Sun, observed in white-light coronal images, and 3. The heliographic coordinates of the solar sources must be within 15 degrees from the Sun Center. In all, 24 magnetic cloud (MC) events and 35 non-MC evens were analyzed. Of the 35 non-MC events selected for analysis, it was possible to fit flux ropes to 31/35 events if different boundaries and multiple flux ropes are used. The four events without flux rope structure seem to be poor events (short duration, poor magnetic and plasma signatures). Coronal flux rope fitting suggests (at least for a subset) that non-MC events become non-central during propagation. It was also found that MCs have high charge states; half of the non-MC events also have high charge states. The direction parameter of CMEs seems to be high for MCs. All these results are consistent with the idea that alll CMEs may be flux ropes.

Gopalswamy, Natchimuthuk↗
NASA NTRSDate not supplied

Convective Transport and Evolution of Clouds and aerosols in the Asian Summer Monsoon Region

The existence of a persistent layer in the lowermost stratosphere in the Asian Monsoon region is well-known and has been observed by satellites and also in situ by balloon-borne sensors. This aerosol layer has been observed to persist every year by both SAGE sensors and by CALIOP, between the tropopause and the lower boundary of the Junge stratospheric sulfate layer. But how does this layer form and why? Apparently, aerosols are lofted by convection form the Indian and Asian continents, into the upper troposphere/lower stratosphere (UT/LS) area in the middle of a persistent anticyclone associate with the Asian summer monsoon. But some mysteries remain. The top of this aerosol layer is well above the altitude of maximum convective outflow, so why is the top of the aerosol layer so high? Are the aerosols coming from China or from India? And finally, is there an observable impact of these aerosol on thin cirrus distributions in the UT/LS? We explore the interesting difference in altitude between the ATAL layer and the convective cloud top height, using observations from CALIOP and from SAGE. In the process of doing this we examine the accuracy of both CALIOP and SAGE cloud/aerosol discrimination, and the impact of various averaging lengths. We compare the apparent "observational tropopause" with observations from COSMIC, CALIOP (clouds), and with modeled interpolation from MERRA-2. We also compare CALIOP and CloudSat daytime cloud top heights for convective clouds with the vertical aerosol distribution, and evaluate convection in this region as represented by MERRA-2. Finally, and maybe most importantly we compare convective cloud top heights and temperatures with diurnal variability during the most recent years by using observations from the geostationary Himawari satellite. How representative are the twice-daily A-Train observations, when compared to the natural diurnal variability of convection? The goal is to establish the origins of these UT/LS aerosols, whether these aerosol distributions can be completely explained by convective transport, and to evaluate convective lofting of aerosol by models. Ultimately, the convective lofting of aerosols as modeled is needed to explain the Asian Monsoon aerosol distributions. The observations contribute much-needed information to enhance the model accuracy.

clouds↗