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DOE OSTI2020

Dark matter clusters and time correlations in direct detection experiments

Assuming that dark matter (DM) efficiently clusters on various scales we analyse the possible impact on direct DM searches. For certain sizes and densities of DM clusters, mutual detector-cluster encounters may occur only once a year or every several years leading to the apparent failure of individual experiments searching for DM to discover it. If, however, encounters with Earth size and up to 10 4 times bigger clusters occur about once a year, then finding time correlations between events in different underground detectors can lead to DM discovery.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2022

Dark Grand Unification in the axiverse: decaying axion dark matter and spontaneous baryogenesis

The quantum chromodynamics axion with a decay constant near the Grand Unification (GUT) scale has an ultralight mass near a neV. We show, however, that axion-like particles with masses near the keV–PeV range with GUT-scale decay constants are also well motivated in that they naturally arise from axiverse theories with dark c gauge groups. We demonstrate that the correct dark matter abundance may be achieved by the heavy axions in these models through the misalignment mechanism in combination with a period of early matter domination from the long-lived dark glueballs of the same gauge group. Heavy axion dark matter may decay to two photons, yielding mono-energetic electromagnetic signatures that may be detectable by current or next-generation space-based telescopes. We project the sensitivity of next-generation telescopes including Athena, AMEGO, and e-ASTROGAM to such decaying axion dark matter. If the dark sector contains multiple confining gauge groups, then the observed primordial baryon asymmetry may also be achieved in this scenario through spontaneous baryogenesis. We present explicit orbifold constructions where the dark gauge groups unify with the SM at the GUT scale and axions emerge as the fifth components of dark gauge fields with bulk Chern-Simons terms.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Nature of the spin resonance mode in CeCoIn 5

Spin-fluctuation-mediated unconventional superconductivity can emerge at the border of magnetism, featuring a superconducting order parameter that changes sign in momentum space. Detection of such a sign-change is experimentally challenging, since most probes are not phase-sensitive. The observation of a spin resonance mode (SRM) from inelastic neutron scattering is often seen as strong phase-sensitive evidence for a sign-changing superconducting order parameter, by assuming the SRM is a spin-excitonic bound state. Here we show that for the heavy fermion superconductor CeCoIn 5 , its SRM defies expectations for a spin-excitonic bound state, and is not a manifestation of sign-changing superconductivity. Instead, the SRM in CeCoIn 5 likely arises from a reduction of damping to a magnon-like mode in the superconducting state, due to its proximity to magnetic quantum criticality. Our findings emphasize the need for more stringent tests of whether SRMs are spin-excitonic, when using their presence to evidence sign-changing superconductivity.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS2003

Laboratory Characterization and Modeling of a Near-Infrared Enhanced Photomultiplier Tube

The photon-starved channel for optical communications from deep space requires the development of detector technology that can achieve photon-counting sensitivities with high bandwidth. In this article, a near-infrared enhanced photomultiplier tube (PMT) with a quantum e.ciency of 0.08 at a 1.06- m wavelength is characterized in the laboratory. A Polya distribution model is used to compute the probability distribution function of the emitted secondary photoelectrons from the PMT. The model is compared with measured pulse-height distributions with reasonable agreement. The model accounts for realistic device parameters, such as the individual dynode stage gains and a shape parameter that is representative of the spatial uniformity of response across the photocathode and dynodes. Bit-error rate (BER) measurements also are presented for 4- and 8-pulse-position modulation (PPM) modulation schemes with data rates of 20 to 30 Mb/s. A BER of 10-2 is obtained for a mean of 8 detected photons.

Biswas, A.↗

NASA NTRS2010

Active Galaxy Unification in the Era of X-Ray Polarimetry

Active galactic nuclei (AGNs), Seyfert galaxies, and quasars are powered by luminous accretion and often accompanied by winds that are powerful enough to affect the AGN mass budget, and whose observational appearance bears an imprint of processes that are happening within the central parsec around the black hole (BH). One example of such a wind is the partially ionized gas responsible for X-ray and UV absorption (warm absorbers). Here, we show that such gas will have a distinct signature when viewed in polarized X-rays. Observations of such polarization can test models for the geometry of the flow and the gas responsible for launching and collimating it. We present calculations that show that the polarization depends on the hydrodynamics of the flow, the quantum mechanics of resonance-line scattering, and the transfer of polarized X-ray light in the highly ionized moving gas. The results emphasize the three-dimensional nature of the wind for modeling spectra. We show that the polarization in the 0.1-10 keV energy range is dominated by the effects of resonance lines. We predict a 5%-25% X-ray polarization signature of type-2 objects in this energy range. These results are generalized to flows that originate from a cold torus-like structure, located approximately 1 pc from the BH, which wraps the BH and is ultimately responsible for the apparent dichotomy between type 1 and type 2 AGNs. Such signals will be detectable by future dedicated X-ray polarimetry space missions, such as the NASA Gravity and Extreme Magnetism Small Explorer SMEX, "GEMS" Swank et al. (2008).

Dorodnitsyn, A.↗

DOE OSTI2023

Deconstructing magnetization noise: Degeneracies, phases, and mobile fractionalized excitations in tetris artificial spin ice

Direct detection of spontaneous spin fluctuations, or “magnetization noise,” is emerging as a powerful means of revealing and studying magnetic excitations in both natural and artificial frustrated magnets. Depending on the lattice and nature of the frustration, these excitations can often be described as fractionalized quasiparticles possessing an effective magnetic charge. Here, by combining ultrasensitive optical detection of thermodynamic magnetization noise with Monte Carlo simulations, we reveal emergent regimes of magnetic excitations in artificial “tetris ice.” A marked increase of the intrinsic noise at certain applied magnetic fields heralds the spontaneous proliferation of fractionalized excitations, which can diffuse independently, without cost in energy, along specific quasi-1D spin chains in the tetris ice lattice.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2024

Unveiling Sea Quark Dynamics: Measuring Sivers Asymmetry with Polarized Target at SpinQuest

SpinQuest is a cutting-edge, high-luminosity Drell-Yan experiment utilizing polarized hy- drogen and deuterium targets to measure the Sivers asymmetry for the light sea quarks in the nucleon. Detecting a nonzero Sivers asymmetry would provide clear evidence for nonzero or- bital angular momentum of sea quarks. The Sivers asymmetry presents itself as an azimuthal asymmetry in the production of virtual photons via the Drell-Yan process, and SpinQuest will be able to measure this asymmetry using the existing SeaQuest dimuon spectrometer. In addi- tion to making measurements sensitive to the sea quark Sivers function, we will also measure the azimuthal asymmetry in the production of J/ψ particles, which is sensitive to the gluon Sivers function. Additionally, observing a sign change in the Sivers asymmetry between this measurement and future measurements at the Electron-Ion Collider would be a test of a funda- mental prediction of Quantum Chromodynamics. In this poster we will review the physics and technology underpinning the experiment.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Quantum computation solves a half-century-old enigma: Elusive vibrational states of magnesium dimer found

The high-lying vibrational states of the magnesium dimer (Mg 2 ), which has been recognized as an important system in studies of ultracold and collisional phenomena, have eluded experimental characterization for half a century. Until now, only the first 14 vibrational states of Mg 2 have been experimentally resolved, although it has been suggested that the ground-state potential may support five additional levels. Here, we present highly accurate ab initio potential energy curves based on state-of-the-art coupled-cluster and full configuration interaction computations for the ground and excited electronic states involved in the experimental investigations of Mg 2 . Our ground-state potential unambiguously confirms the existence of 19 vibrational levels, with ~1 cm -1 root mean square deviation between the calculated rovibrational term values and the available experimental and experimentally derived data. Our computations reproduce the latest laser-induced fluorescence spectrum and provide guidance for the experimental detection of the previously unresolved vibrational levels.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2021

The Global Magneto-ionic Medium Survey: A Faraday Depth Survey of the Northern Sky Covering 1280–1750 MHz

The Galactic interstellar medium hosts a significant magnetic field, which can be probed through the synchrotron emission produced from its interaction with relativistic electrons. Linearly polarized synchrotron emission is generated throughout the Galaxy and, at longer wavelengths, modified along nearly every path by Faraday rotation in the intervening magneto-ionic medium. Full characterization of the polarized emission requires wideband observations with many frequency channels. We have surveyed polarized radio emission from the Northern sky over the range 1280–1750 MHz, with channel width 236.8 kHz, using the John A. Galt Telescope (diameter 25.6 m) at the Dominion Radio Astrophysical Observatory, as part of the Global Magneto-Ionic Medium Survey. The survey covered 72% of the sky, decl. −30° to +87° at all R.A. The intensity scale was absolutely calibrated, based on the flux density and spectral index of Cygnus A. Polarization angle was calibrated using the extended polarized emission of the Fan Region. Data are presented as brightness temperatures with angular resolution 40′. Sensitivity in Stokes Q and U is 45 mK rms in a 1.18 MHz band. We have applied rotation measure synthesis to the data to obtain a Faraday depth cube of resolution 150 rad m{sup −2} and sensitivity 3 mK rms of polarized intensity. Features in Faraday depth up to a width of 110 rad m{sup −2} are represented. The maximum detectable Faraday depth is ±2 × 10{sup 4} rad m{sup −2}. The survey data are available at the Canadian Astronomy Data Centre.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2025

Listening for new physics with quantum acoustics

We present a novel application of a qubit-coupled phonon detector to search for new physics, e.g., ultralight dark matter (DM) and high-frequency gravitational waves. The detector, motivated by recent advances in quantum acoustics, is composed of superconducting transmon qubits coupled to high-overtone bulk acoustic resonators (ℎ⁡BARs) and operates in the GHz−10 GHz frequency range. New physics can excite 𝒪⁡(10 μ⁢eV) phonons within the ℎ⁡BAR, which are then converted to qubit excitations via a transducer. We detail the design, operation, backgrounds, and expected sensitivity of a prototype detector, as well as a next-generation detector optimized for new physics signals. We find that a future detector can complement current haloscope experiments in the search for both dark photon DM and high-frequency gravitational waves. Lastly, we comment on such a detector’s ability to operate as a 𝒪⁡(10 μ⁢eV) athermal phonon sensor for sub-GeV DM detection.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2022

Electronic and magnetic properties of the topological semimetal SmMg 2 Bi 2

Dirac semimetals show nontrivial physical properties and can host exotic quantum states like Weyl semimetals and topological insulators under suitable external conditions. Here, by combining angle-resolved photoemission spectroscopy measurements (ARPES) and first-principle calculations, we demonstrate that the Zintl-phase compound SmMg 2 Bi 2 is in close proximity to a topological Dirac semimetallic state. ARPES results show a Dirac-like band crossing at the zone center near the Fermi level (E F ), which is further confirmed by first-principle calculations. Theoretical studies also reveal that SmMg 2 Bi 2 belongs to a Z 2 topological class and hosts spin-polarized states around the E F . Zintl's theory predicts that the valence state of Sm in this material should be Sm 2+ , however, we detect many Sm-4f multiplet states (flat-bands) whose energy positions and relative intensities suggest the presence of both dominant Sm 2+ and minor Sm 3+ . The small concentration (2.5%) of Sm 3+ in the bulk of a crystal is inferred to arise from Sm vacancies in the crystal. It is also evident that these flat bands and other dispersive states are strongly hybridized when they cross each other. Due to the presence of Sm 3+ ions, the temperature dependence of the magnetic susceptibility χ (T) shows a Curie-Weiss-like contribution in the low-temperature region, in addition to the Van Vleck-like behavior expected for the Sm 2+ ions. The present study will help to better understand the electronic structure, magnetism, and transport properties of related materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2020

Evolution of Radicals from the Photolysis of High Ionic Strength Alkaline Nitrite Solutions

Reactive nitrogen species (RNS), along with reactive oxygen species (ROS), are significant products from radiolysis in solution. While much research has been focused on biological systems, these species are also important products in the autoradiolysis that occurs in nuclear waste. In this work, we determine the correlation between solution constituents, particularly nitrite, and radical products in highly alkaline solutions relevant to liquid waste. Because these radicals tend to be very short-lived, we employ spin trapping in conjunction with electron paramagnetic resonance (EPR) to detect them and quantify their production. Most spin traps do not function in these conditions (>1 M NaOH); however, nitroalkanes such as nitromethane will act as spin traps in their aci form, which is dominant at high pH. To restrict the products to those originating from nitrite, we use 280–480 nm UV light to generate radicals, avoiding products from the photolysis of water. Under these circumstances, nitric oxide, nitrite radicals, and hydroxyl radicals are detected, and the trends with the concentration of the constituents of the solutions are tracked. These include nitrite, nitrate, hydroxide, and carbonate. We find that, while the equilibrium shifts with increasing pH from hydroxyl radicals to the more slowly reacting oxide radicals, the production of nitrite radicals does not decrease.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

Manipulating chiral spin transport with ferroelectric polarization

A magnon is a collective excitation of the spin structure in a magnetic insulator and can transmit spin angular momentum with negligible dissipation. This quantum of a spin wave has always been manipulated through magnetic dipoles (that is, by breaking time-reversal symmetry). Here we report the experimental observation of chiral spin transport in multiferroic BiFeO 3 and its control by reversing the ferroelectric polarization (that is, by breaking spatial inversion symmetry). The ferroelectrically controlled magnons show up to 18% modulation at room temperature. The spin torque that the magnons in BiFeO 3 carry can be used to efficiently switch the magnetization of adjacent magnets, with a spin-torque efficiency comparable to the spin Hall effect in heavy metals. Utilizing such controllable magnon generation and transmission in BiFeO 3 , an all-oxide, energy-scalable logic is demonstrated composed of spin-orbit injection, detection and magnetoelectric control. In conclusion, our observations open a new chapter of multiferroic magnons and pave another path towards low-dissipation nanoelectronics.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Toward a machine-guided approach to energetic material discovery

In this article, we trained a machine learning (ML) model to connect microstructural details of an energetic material formulation to its performance for the purpose of guiding the discovery of new explosive formulations. Our hypothesis was that the algorithm would robustly learn the training data and produce an accurate surrogate model. Specifically, the algorithm learned the relationship between details of the void size distribution (VSD), initiating shock pressure, and the energetic material performance. We used realistic constraints on the VSD and a range of cases were ingested by a physically informed reactive flow model working within a hydrodynamic solver running on high-performance computing resources. The ML algorithm produced a surrogate model that accurately predicted known test points around the parameter space. In addition to the utility of the model and the process used for its development, we noted interesting comparisons between what we, the authors—subject matter experts, would heuristically conclude from the training data and the surrogate model predictions. We detected nuanced details that were missed by the surrogate model; however, these details are not important to an energetic material formulator. We concluded that the algorithm did indeed robustly learn the training data and produce an accurate surrogate model. We further concluded that the surrogate model is a powerful tool to guide the formulator in the absence of subject matter experts and limited-access computing resources.

42 ENGINEERING↗

DOE OSTI2025

New physics search at the CEPC: a general perspective

A next generation, high-intensity electron-positron collider “Higgs factory”, such as the Circular Electron-Positron Collider (CEPC), is among the highest priority for the global high energy collider physics community. The CEPC can provide unprecedented opportunities for making fundamental discoveries and providing decisive insights in the quest for a “New Standard Model (SM)” of nature’s fundamental interactions. The CEPC could: 1) Identify the origin of matter, especially the mechanism related to the first-order phase transition in the early Universe, which could produce a detectable gravitational wave signal. 2) Discover dark matter, particularly dark matter particles with a mass between one tenth and 100 times the proton mass. 3) Observe an array of new physics smoking guns, with sensitivities orders of magnitude better than those of existing facilities. The SM of Particle Physics is a triumph of the past half a century, as it predicts and interprets almost all the phenomena observed in experiments from the highest energies with colliders to low energy “tabletop” studies. On the other hand, deep mysteries exist concerning the most fundamental interactions of matter and the space-time fabric of the Universe, including the nature of dark matter, the origin of “visible” matter, the vast hierarchy of elementary particle masses, the quantum nature of gravity, and the mechanism of inflation. These mysteries challenge us to look for “new physics” beyond the SM and General Relativity. Indeed, physicists believe that the SM is simply a low-energy effective theory that reflects aspects of the more profound theory that answers the aforementioned mysteries. Uncovering this “New SM”, the profound theory who supports the SM is the primary mission for particle physics in the post-Higgs boson era.

Ai 艾, Xiaocong 小聪 [Zhengzhou University (China); e↗

DOE OSTI2024

The Origin Symphony: Probing Baryogenesis with Gravitational Waves

Affleck-Dine (AD) baryogenesis is compelling yet challenging to probe because of the high energy physics involved. We demonstrate that this mechanism can be realized generically with low-energy new physics without supersymmetry while producing detectable gravitational waves (GWs) sourced by parametric resonance of a light scalar field. In viable benchmark models, the scalar has a mass of ${\cal O}(0.1-10)$ GeV, yielding GWs with peak frequencies of ${\cal O}(10-100)$ Hz. This study further reveals a new complementarity between upcoming LIGO-frequency GW detectors and laboratory searches across multiple frontiers of particle physics.

Cosmology and Nongalactic Astrophysics (astro-ph.C↗

DOE OSTI2025

Precision measurement of lifetime and branching ratios of the 4⁢𝑓 13⁡ 5⁢𝑑⁢6⁢𝑠 1 ⁢[5/2] 5/2 state in Yb + ions

We report spectroscopic and time-resolved experimental observations to characterize the [Xe]⁢4⁢𝑓 13 ⁡( 2 𝐹$^𝑜_{5/2}$)⁢5⁢𝑑⁢6⁢𝑠⁡( 1 𝐷)⁢ 1 ⁢[5/2]$^𝑜_{5/2}$ state in 172 Yb + ions. We access this state from the metastable 4⁢𝑓 14 ⁡5⁢𝑑⁡( 2 𝐷 3/2,5/2 ) manifold and observe an unexpectedly long lifetime of 𝜏 = 37.9⁢(9) ⁢µ⁢s that allows visible Rabi oscillations and resolved-sideband spectroscopy. Using a combination of coherent population dynamics, high-fidelity detection and heralded state preparation, and optical pumping methods, we measure the branching ratios to the 2 𝐷 3/2 , 2 𝐷 5/2 , and 2 𝑆 1/2 states to be 0.359⁢(2), 0.639(2), and 0.0023⁢(16), respectively. The branching ratio to the 4⁢𝑓 13⁡ 6⁢𝑠 2 ⁡( 2 𝐹 7/2 ) is compatible with zero within our experimental resolution. We also report measurements of Landé 𝑔-factor of the 1 ⁢[5/2]$^𝑜_{5/2}$ state. Further, the branching ratio of the 2 𝐷 5/2 to 2 𝑆 1/2 decay in 172 Yb + was measured to be 0.188(3), improving its relative uncertainty by an order of magnitude. Our measurements provide experimental benchmarks for better understanding the atomic structure of Yb + ions, which still lacks accurate numerical descriptions, and the use of high-lying excited states for partial detection and qubit manipulation in the omg architecture.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2026

Quantum enabled precision measurements of the 229Th nuclear isomer transition (final report)

The existence of the nuclear isomer transition in thorium-229 was first inferred from keV lines in the gamma spectrum of uranium-233 decay more than 40 years ago. Over the years, the value of the transition energy has been refined with indirect measurements using nuclear physics techniques, and the current evidence points to transition energy in the laser-accessible vacuum ultra-violet region of the spectrum. At the start of this project, the two best measurements of the transition energy were 7.8±0.5 eV and 8.28±0.17 eV from high precision gamma ray spectroscopy and kinetic energy of internal conversion electrons, respectively. This project aimed to reduce the uncertainty in the transition energy to 10 meV using direct calorimetric measurements of the decay energy with superconducting nanowire single photon detectors (SNSPDs). Specifically, the method that was pursued was to generate thorium-229 in the excited isomer state by the alpha decay of uranium-233, embed the excited state thorium into an SNSPD, then detect the energy released when the isomer deexcites.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗