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At least 1,531 records · Page 85

van der Waals-corrected density functional study of electric field noise heating in ion traps caused by electrode surface adsorbates

Abstract In order to realize the full potential of ion trap quantum computers, an improved understanding is required of the motional heating that trapped ions experience. Experimental studies of the temperature-, frequency-, and ion–electrode distance-dependence of the electric field noise responsible for motional heating, as well as the noise before and after ion bombardment cleaning of trap electrodes, suggest that fluctuations of adsorbate dipoles are a likely source of so-called ‘anomalous heating,’ or motional heating of the trapped ions at a rate much higher than the Johnson noise limit. Previous computational studies have investigated how the fluctuation of model adsorbate dipoles affects anomalous heating. However, the way in which specific adsorbates affect the electric field noise has not yet been examined, and an electric dipole model employed in previous studies is only accurate for a small subset of possible adsorbates. Here, we analyze the behavior of both in-plane and out-of-plane vibrational modes of twenty-one adsorbate–electrode combinations within the independent fluctuating dipole model, utilizing accurate first principles computational methods to determine the surface-induced dipole moments. We find the chemical specificity of the adsorbate can change the electric field noise by seven orders of magnitude and specifically that soft in-plane modes of weakly-adsorbed hydrocarbons produce the greatest noise and ion heating. We discuss the dynamics captured by the fluctuating dipole model, namely the adsorbate-dependent turn-on temperature and electric field noise magnitude, and also discuss the model’s failure to reproduce the measured 1/ ω noise frequency scaling with a single adsorbate species. We suggest future research directions for improved, quantitatively predictive models based on extensions of the present framework to multiple interacting adsorbates.

74 ATOMIC AND MOLECULAR PHYSICS↗

Engineering the radiative dynamics of thermalized excitons with metal interfaces

As a platform for optoelectronic devices based on exciton dynamics, monolayer transition metal dichalcogenides (TMDCs) are often placed near metal interfaces or inside planar cavities. While the radiative properties of point dipoles at metal interfaces has been studied extensively, those of excitons, which are delocalized and exhibit a temperature-dependent momentum distribution, lack a thorough treatment. Here, we analyze the emission properties of excitons in TMDCs near planar metal interfaces and explore their dependence on exciton center-of-mass momentum, transition dipole orientation, and temperature. Defining a characteristic energy scale k B T c = ($\hbar k$) 2 /2m (k being the radiative wavevector and m the exciton mass), we find that at temperatures T $\gg$ T c and low densities where the momentum distribution can be characterized by Maxwell-Boltzmann statistics, the modified emission rates (normalized to free space) behave similarly to point dipoles. This similarity in behavior arises due to the broad nature of wavevector components making up the exciton and point dipole emission. On the other hand, the narrow momentum distribution of excitons for T < T c can result in significantly different emission behavior as compared to point dipoles. These differences can be further amplified by considering excitons with a Bose Einstein distribution at high phase space densities, such as in a condensate phase. We find suppression or enhancement of emission relative to the point dipole case by several orders of magnitude. These insights can help optimize the performance of optoelectronic devices that incorporate 2D semiconductors near metal electrodes and can inform future studies of exciton radiative dynamics at low temperatures. Additionally, these studies show that nanoscale optical cavities are a viable pathway to generating long-lifetime exciton states in TMDCs.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Competing interactions in semiconductor quantum dots

In this study, we introduce an integrability-based method enabling the study of semiconductor quantum dot models incorporating both the full hyperfine interaction as well as a mean-field treatment of dipole-dipole interactions in the nuclear spin bath. By performing free induction decay and spin echo simulations we characterize the combined effect of both types of interactions on the decoherence of the electron spin, for external fields ranging from low to high values. We show that for spin echo simulations the hyperfine interaction is the dominant source of decoherence at short times for low fields, and competes with the dipole-dipole interactions at longer times. On the contrary, at high fields the main source of decay is due to the dipole-dipole interactions. In the latter regime an asymmetry in the echo is observed. Furthermore, the non-decaying fraction previously observed for zero field free induction decay simulations in quantum dots with only hyperfine interactions, is destroyed for longer times by the mean-field treatment of the dipolar interactions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Nuclear multipole responses from chiral effective field theory interactions

We probe nuclear multipole resonances in the framework of the random-phase approximation by using the interaction obtained from the chiral effective field theory. The three-nucleon force is included in a form of the in-medium two-nucleon interaction, which was derived from the chiral three-nucleon force. The isoscalar monopole, isoscalar dipole, isovector dipole, and isoscalar quadrupole resonances of the closed-shell 56,68,78 Ni have been investigated. The calculations reasonably reproduce the experimental multipole resonances of 56,68 Ni, and well describe the pygmy dipole resonance and dipole polarizability measured in 68 Ni. The multipole resonances of 78 Ni, including pygmy dipole resonance and dipole polarizability, are predicted. The detailed effects of the tensor force and three-body force are analyzed by dissecting the chiral interaction. In this work, we find that in general the tensor force effect on electric giant resonances is not as significant as the effect from the three-body force, although the tensor force provides more than half of the binding energy. The effect from three-body force is strong in light nuclei. Particularly, three-body force is crucial for the formation of the pygmy resonance in calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Progress on HL-LHC Nb 3 Sn Magnets

The high-luminosity Large Hadron Collider (HL-LHC) project aims at allowing to increase the collisions in the LHC by a factor of ten in the decade 2025-2035. One essential element is the superconducting magnet around the interaction region points, where the large aperture magnets will be installed to allow to further reduce the beam size in the interaction point. The core of this upgrade is the Nb 3 Sn triplet, made up of 150-mm aperture quadrupoles in the range of 7-8 m. The project is being shared between the European Organization for Nuclear Research and the US Accelerator Upgrade Program, based on the same design, and on the two strand technologies. The project is ending the short model phase, and entering the prototype construction. We will report on the main results of the short model program, including the quench performance and field quality. A second important element is the 11 T dipole that replaces a standard dipole making space for additional collimators. The magnet is also ending the model development and entering the prototype phase. A critical point in the design of this magnet is the large current density, allowing increase of the field from 8 to 11 T with the same coil cross section as in the LHC dipoles. This is also the first two-in-one Nb 3 Sn magnet developed so far. We will report the main results on the test and the critical aspects.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Advanced Design for the WIQ Magnet With Steering Corrector Function

The Facility for Rare Isotopes Beams (FRIB) delivers heavy-ion primary beams at energies of up to 300 MeV/u at 10 kW of beam power to generate rare isotope beams for experiments and will eventually operate at beam power of 400 kW. The preseprator of the Advanced Rare Isotope Separator (ARIS) is equipped with six warm-iron quadrupole (WIQ) singlets and two dipoles integrated right after the production target. They have a compact structure and operate in a high radiation vacuum environment within a hot cell having remote handling capabilities for installation and maintenance. Due to asymmetry with respect to the quadrupole poles, nested sextupole excitations in WIQs induce vertical dipoles that offset the centroid trajectory; Magnet misalignments also result in trajectory offsets. Such offsets degrade separator performance but can be minimized by changing the current distribution on sextupole and octupole coils. In this work, we show how modifications to the WIQ coil design can allow superimposed dipole fields to be included to the octupole and sextupole windings, as well as addition of dipole components by splitting coil currents over groups with separator power supplies. Adjusting the group currents can cancel the sextupole-induced vertical dipole component which can be as high as 0.012 Tm. Octupole coil changes may superimpose a horizontal dipole integrated strength as high as 0.0332 Tm. Unwanted higher harmonics induced as a side effect of the new design are kept to a minimum such that separator performance is preserved as much as possible.

Accelerator magnets↗

Technical Reports - FY16 Q1 - October-December 2015

Recent experiments have demonstrated that the frequency dependence of motional heating rates in ion traps can vary dramatically with temperature.1-6 More specifically, it has been shown that, at temperatures below roughly 70 K, heating rates are substantially lower than those observed at temperatures above 70 K.1,2 These observations, combined with experiments that show that ion bombardment may also reduce heating rates,4,5 suggest that one potential source of heating may be the presence of unwanted adatoms on trap surfaces. Based upon this evidence, this past quarter, we have used our previously detailed microscopic model of anomalous heating to study which adatoms may be responsible for the observed temperature-dependent scaling of motional heating rates with frequency. We have also examined the validity of one of the key assumptions in our model - that surface adatom dipoles can be accurately obtained from a variational ansatz - by using more direct DFT calculations of the dipole moments. Our current results suggest that the adatoms potentially responsible for the observed motional heating rates should bind weakly to the electrode surface and likely have a mass that exceeds that of Ne. Preliminary DFT calculations suggest that an analytical adatom dipole model,9 previously used in the ion trap noise literature7 to obtain the dipole as a function of adatom-surface distance, may be insufficiently accurate. Therefore, we are working toward obtaining a tabulation of the distance-dependent dipole for several adsorbates using first principles calculations for more accurate input to the heating model. The accurate calculation of the adatom dipole is important because its fluctuation is what couples to and heats the trapped ion qubit. Future work will focus on calculating the frequency spectra of a variety of hydrocarbons, which should have the binding characteristics identified below as necessary for reproducing experimental results. Upcoming efforts will moreover be directed toward deriving an improved microscopic model of heating which will enable direct comparisons of heating rates with measured ion-surface distances and will more accurately account for experimental parameters such as the trapping frequency, ion-electrode distance, and RF power applied to the electrodes.

36 MATERIALS SCIENCE↗

Measurement of the Energy Spread for CeC Project

The Coherent Electron Cooling requires small energy spread and uniformity of energy along the bunch. The diagnostics line is utilized for the measurement of the electron beam parameters. The beamline layout is shown in Fig. 1. Three quadrupoles after the linac are used to match beam into the common section. The main dipole is used to deflect beam towards common section. If it is switched off the beam goes to the diagnostics line. The beam optics in the diagnostics line is controlled by four quadrupoles. The deflecting cavity sweeping beam in the vertical direction follows the quadrupoles. Sector dipole is used for energy parameters measurement. It has deflection angle of 30 degrees. With diagnostics dipole switched off the beam propagated to the insertable slits system for emittance measurement. There are four profile monitors in the line, The first profile monitor (ACC YAG) is after the main dipole. The second profile monitor (YAG3) is in front of the diagnostics dipole after the deflecting cavity. YAG1 profile monitor is placed after the slits, and YAG2 profile monitor is placed after the diagnostics dipole. There is a solenoid between the deflecting cavity and YAG3. It is used for the beam energy measurement.

43 PARTICLE ACCELERATORS↗

Time domain-induced polarization geophysical data collected in the Rifle Floodplain, Colorado, USA

The IP data set was collected using a time domain-induced polarization (TDIP) method along 65 profiles of various lengths over the floodplain. Surface time domain?induced polarization (TDIP) data was collected to create the 3?D images of the complex electrical resistivity, in terms of magnitude and phase, which are associated with mineral precipitation and other lithological properties. The TDIP data was then used to estimate the spatial distribution of naturally reduced zones, which are known to be biogeochemical hotspots in floodplains having increased uranium and other redox-sensitive metal concentrations as well as high carbon contents. In the TDIP method, the transient decay of voltage is measured after current shut-off, typically in the form of an integral of decay curves over a predefined time window (so-called integral chargeability). TDIP measurements at the site were collected using the Syscal Iris Pro Switch equipment with a square-wave current injection, 50% duty cycle, and a pulse length of 2 s. The integral chargeability measurements were carried out using 20 windows during voltage decay between 240 and 1840 ms after current shut-off. Tomographic measurements were collected by deploying stainless steel electrodes with an electrode separation of 1.8 m and using a dipole-dipole ‘‘skip-2’’ and ‘‘skip-3’’ measuring protocol (i.e., for a dipoles length of 5.4 and 7.2 m, respectively). The sequence of dipole-dipole measurements was carefully arranged to (1) minimize unwanted electromagnetic coupling effects in the data, avoiding potential measurements with electrodes located inside the current dipole, (2) prevent voltage measurements using electrodes, which might be polarized due to previous current injection, and (3) increase the signal-to-noise ratio for an intended exploration depth of 8 m, i.e., the bottom of the aquifer. All measurements were collected as normal and reciprocal pairs for estimation of the data error. The IP measurements were collected with symmetric arrays (i.e., the measuring equipment placed at the center of the electrode array) with a maximum of 36 electrodes, considering that longer profiles revealed a significant increase in the normal-reciprocal misfit for the measurements of the decay curve, probably due to greater impact of electromagnetic coupling on the data. The TDIP data sets were inverted in a twodimensional domain along each transect using CRTomo, which is a smoothness-constraint inversion code based on a finite element algorithm. The resistivity and phase shift values at each pixel were then assigned at the corresponding point within the 3-D floodplain domain (the black rectangle Figure 1b) and used in the 3-D estimation. The TDIP inversion results provided the distribution of the complex resistivity, expressed in terms of its magnitude and phase-shift. The analysis of the normal-reciprocal misfit was used to estimate the relative error. We removed the measurement with smallest voltage difference (<2 mV), representing about 2% variations in the data. For the inversion of TDIP measurements, chargeability values were linearly converted to frequency domain phase values (at the fundamental frequency of 0.125 Hz), by assuming a constant-phase response. This approach has been demonstrated to provide consistent results in previous studies

54 ENVIRONMENTAL SCIENCES↗

Theoretical and observational analysis of spacecraft fields

In order to investigate the nondipolar contributions of spacecraft magnetic fields a simple magnetic field model is proposed. This model consists of randomly oriented dipoles in a given volume. Two sets of formulas are presented which give the rms-multipole field components, for isotropic orientations of the dipoles at given positions and for isotropic orientations of the dipoles distributed uniformly throughout a cube or sphere. The statistical results for an 8 cu m cube together with individual examples computed numerically show the following features: Beyond about 2 to 3 m distance from the center of the cube, the field is dominated by an equivalent dipole. The magnitude of the magnetic moment of the dipolar part is approximated by an expression for equal magnetic moments or generally by the Pythagorean sum of the dipole moments. The radial component is generally greater than either of the transverse components for the dipole portion as well as for the nondipolar field contributions.

Neubauer, F. M.↗

Theoretical and observational analysis of spacecraft fields

In order to investigate the dipolar and nondipolar contributions of spacecraft magnetic fields, a simple magnetic field model is proposed. This model consists of a number N of randomly oriented dipoles of strength M sub k in a given volume. Two sets of formulas are presented that give the rms multipole field components, first, for isotropic orientations of the dipoles at given positions and second, for isotropic orientations of the dipoles distributed uniformly throughout a cube or sphere. The statistical results for a cube (8 cu m in size) together with individual examples computed numerically show the following features. Beyond about 2- to 3-m distance from the center of the cube the field is dominated by an equivalent dipole. The magnitude of the magnetic moment of the dipolar part is approximated by N to the 1/2 power times M for equal magnetic moments or generally by the Pythagorean sum of the dipole moments. The radial component tend to be greater than either of the transverse components for the dipole portion as well as for the nondipolar field contributions.

Neubauer, F. M.↗

The moon's permanent magnetic field - A cratered-shell model

The possibility is considered that the properties of the larger-scale lunar magnetic field may depend in a rather straightforward manner on the geometrical properties of the distribution of larger craters. The relevant effects of cratering are analyzed in the framework of a model of a spherically symmetric shell magnetized to some specific intensity by a concentric dipolar magnetic field. The remanent dipole moment of the model is determined by calculating the dipole moment of the material removed to form craters and them computing the remanent dipole moment for three mutually orthogonal orientations of the magnetizing dipole. The resulting absolute values for the remanent dipole moment are found to be comparable to the upper limit of 10 to the -19th power G-cu cm estimated from Apollo subsatellite measurements. It is concluded that for a crust with an empirically reasonable mean magnetization, the craters can account for a dipole moment as great as that indicated by the estimated upper limit.

Weiss, H.↗

Formation of iron metal and grain coagulation in the solar nebula

The interstellar grain population in the giant molecular cloud from which the sun formed contained little or no iron metal. However, thermal processing of individual interstellar silicates in the solar nebula is likely to result in the formation of a population of very small iron metal grains. If such grains are exposed to even transient magnetic fields, each will become a tiny dipole magnet capable of interacting with other such dipoles over spatial scale orders of magnitude larger than the radii of individual grains. Such interactions will greatly increase the coagulation cross-section for this grain population. Furthermore, the magnetic attraction between two iron dipoles will significantly increase both the collisional sticking coefficient and the strength of the interparticle binding energy for iron aggregates. Formation of iron metal may therefore be a key step in the aggregation of planetesimals in a protoplanetary nebula. Such aggregates may have already been observed in protoplanetary systems. The enhancement in the effective interaction distance between two magnetic dipoles is directly proportional to the strength of the magnetic dipoles and inversely proportional to the relative velocity. It is less sensitive to the reduced mass of the interacting particles (alpha M(exp -1/2)) and almost insensitive to the initial number density of magnetic dipoles (alpha n(sub o)(exp 1/6)). We are in the process of measuring the degree of coagulation in our condensation flow apparatus as a function of applied magnetic field and correlating these results by means of magnetic remanance acquisition measurements on our iron grains with the strength of the magnetic field to which the grains are exposed. Results of our magnetic remanance acquisition measurements and the magnetic-induced coagulation study will be presented as well as an estimate of the importance of such processes near the nebular midplane.

Nuth, Joseph A., III↗

Warm core ring dynamics derived from satellite imagery

A reinterpretation of the life history of warm core ring 82-b is constructed from drifter trajectories, hydrographic profiles, and satellite-derived sea surface temperature fields. An analysis of the observations strongly suggests this ring is fundamentally a dipole structure for much of its existence. The dipole has unequal strength vortices, with the cyclone being the weaker component. Quantification of the dipole indicates the anticyclonic is oval shaped and rotates at approximately 7.7 deg per day, while the cyclone revolves around the anticyclone at about 14.5 deg per day, yielding an orbit period of approximately 25 days for the cyclone. The elusive part of the dipole explanation is in interpreting its surface signature as a function of time, as the cyclone appears to disappear when in proximity to the steep continental slope. Vortex modeling suggests that when the weaker cyclonic eddy is placed close to a boundary, the cyclone is drawn into a filament as it is advected through the gap between the anticyclone and the boundary. This means the cyclone is either in a filamentation state or undergoing the straining associated with filamentation approximately three fourths of this time, which is in complete agreement with the satellite imagery. In addition, the 82-B dipole configuration is sufficiently robust to survive continuous interaction with the continental slope and the onset of a Gulf Stream interaction. Although only warm core ring 82-B is analyzed in detail (and found to be a vortex pair), dipole configurations are found in the warm core ring 81-F time series as well.

Hooker, Stanford B.↗

Radiative and Nonradiative Transitions of the Rare-Earth Ions Tm(3+) and Ho(3+) in Y3AI5O12 and LiYF4

The optical spectra of rare earth ions in solids arise primarily from electric and magnetic dipole transitions between stark split multiplets of the 4f(sup N) electronic configuration. Electric dipole transitions are parity forbidden between levels of the 4f(sup N) configuration, while those of magnetic dipole origin are allowed. It is known from experiment, however, that the significant contributions to the intensities of most transitions are electric dipole in nature. Judd and Ofelt developed the theory of forced electric dipole transitions of rare-earth ions. This study is devoted to determining electric dipole transition probabilities and branching ratios for Tm(3+) and Ho(3+) ions in Yttrium Aluminum Garnet (YAG) and Yttrium Lithium Fluoride (YLF) using the theory of Judd and Ofelt. The radiative rates determined from the Judd-Ofelt analysis are used with measured lifetimes to find nonradiative rates of relaxation.

Walsh, Brian M.↗

Computer Modeling of Electrostatic Aggregation of Granular Materials in Planetary and Astrophysical Settings

Electrostatic forces strongly influence the behavior of granular materials in both dispersed (cloud) systems and semi-packed systems. These forces can cause aggregation or dispersion of particles and are important in a variety of astrophysical and planetary settings. There are also many industrial and commercial settings where granular matter and electrostatics become partners for both good and bad. This partnership is important for human exploration on Mars where dust adheres to suits, machines, and habitats. Long-range Coulombic (electrostatic) forces, as opposed to contact-induced dipoles and van der Waals attractions, are generally regarded as resulting from net charge. We have proposed that in addition to net charge interactions, randomly distributed charge carriers on grains will result in a dipole moment regardless of any net charge. If grains are unconfined, or fluidized, they will rotate so that the dipole always induces attraction between grains. Aggregates are readily formed, and Coulombic polarity resulting from the dipole produces end-to-end stacking of grains to form filamentary aggregates. This has been demonstrated in USML experiments on Space Shuttle where microgravity facilitated the unmasking of static forces. It has also been demonstrated in a computer model using grains with charge carriers of both sign. Model results very closely resembled micro-g results with actual sand grains. Further computer modeling of the aggregation process has been conducted to improve our understanding of the aggregation process, and to provide a predictive tool for microgravity experiments slated for Space Station. These experiments will attempt to prove the dipole concept as outlined above. We have considerably enhanced the original computer model: refinements to the algorithm have improved the fidelity of grain behavior during grain contact, special attention has been paid to simulation time steps to enable establishment of a meaningful, quantitative time axis, and calibration of rounding accuracies have been conducted to test cumulative numerical influences in the model. The model has been run for larger grain populations, variable initial cloud densities, and we have introduced random net charging to individual grains, as well as a net charge to the cloud as a whole. The model uses 3 positive and 3 negative charges randomly distributed on each grain, with up to 160 grains contained within various size "boxes" that define the initial number densities in the clouds. Each charge represents localized charged region on a grain, but does not necessarily imply single quantized charge carriers. The Coulomb equations are then allowed to interact for each monopole: dipoles and any higher order charge coupling is a natural product of these "free" interactions over which the modeler exerts no influence. The charges are placed on surfaces of grains at random locations. A series of runs was conducted for neutral grains that had a perfect balance of negative and positive char carriers. Runs were also conducted with grains having additional fractional charges ranging between 0 and 1. By adding fractional charges of one sign, the model created grain populations in which all grains had excess charges the same sign, giving the cloud an overall net charge. This simulates clouds subjected to ionizing radiation (e. protoplanetary debris disk around a protosun), or any other process of charge biasing in a grain population (e.g., volcanic plumes). In another run series, random fractional charges of either sign were added to the grains so th some grains had a slight net positive charge while others had a slight net negative charge. This simulates triboelectrically-charged grain populations in which acquisition of an electron by one surface is at the expense creating a hole elsewhere. This dual sign charging was applied in two ways: in one case the cloud remained neutral by ensuring that all grain excess charges added to zero; in the other case, the cloud was permitted slight net char by not imposing a charge-balance condition. Additional information is contained in the original.

Marshall, J.↗

A Deeper Look at the Fundamentals of Heterodyne Detection Requirements

We generally accept the experimentally observed criteria for heterodyne detections that the two waves that are mixed must (i) be collinear, (ii) have matched wave fronts and (iii) cannot be orthogonally polarized. We have not found in the literature adequate physical explanations for these requirements. The purpose of this paper is to find deeper physical understanding of the coherent heterodyne detection processes that could lead to better coherent laser radar system designs1. We find that there are a number of unresolved paradoxes in classical and quantum optics regarding the definitions and understanding of the "interference" and "coherence" properties of light, which are attributed as essentially due to inherent properties of the EM waves. A deeper exploration indicates that it is the various quantum mechanical properties of the detecting material dipoles that make light detectable (visible, or measurable) to us. Accordingly, all the properties that we generally attribute to only light, are in reality manifestations of collective properties of dipole-light interactions. "Interference" and "coherence" can be better understood in terms of this mutual interaction, followed by energy absorption by the dipoles from EM wave fields, manifesting in some measurable transformation of the detecting dipoles. Light beams do not interfere by themselves. The superposition effects due to light beams become manifest through the response characteristics of the detecting dipoles. In this paper, we will show some preliminary expe rimental results that clearly demonstrate that the heterodyning wave fronts have quantitative degradation in signal generation as the angle between them deviates from perfect collinearity. Subsequently, we will propose a hypothesis for this behavior. We will present experimental data establishing that the so called incoherent light can be detected through heterodyne mixing as long as the pulse length contained in the "incoherent" light is longer than the response time of the detector. We will also present a correspondingly better interpretation of two distinguishable coherence properties, temporal coherence and spectral coherence. Our investigation provides a deeper insight into how to rela x various system requirements for heterodyne detection and accordingly develop systems that are simpler, more reliable and lower in cost. Also, we believe that engineering of detector architecture by appropriately modifying dipole behavior using emerging nanotechnology to optimize heterodyne efficiency will be advantageous.

Roychoudhuri, Chandrasekhar↗

Fluorescence from a quantum dot and metallic nanosphere hybrid system

We present energy absorption and interference in a quantum dot-metallic nanosphere system embedded on a dielectric substrate. A control field is applied to induce dipole moments in the nanosphere and the quantum dot, and a probe field is applied to monitor absorption. Dipole moments in the quantum dot or the metal nanosphere are induced, both by the external fields and by each other's dipole fields. Thus, in addition to direct polarization, the metal nanosphere and the quantum dot will sense one another via the dipole-dipole interaction. The density matrix method was used to show that the absorption spectrum can be split from one peak to two peaks by the control field, and this can also be done by placing the metal sphere close to the quantum dot. When the two are extremely close together, a self-interaction in the quantum dot produces an asymmetry in the absorption peaks. In addition, the fluorescence efficiency can be quenched by the addition of a metal nanosphere. This hybrid system could be used to create ultra-fast switching and sensing nanodevices.

77 NANOSCIENCE AND NANOTECHNOLOGY↗