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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Examining the EMC effect using the ${F}_{2}^{n}$ neutron structure function

The persistently mysterious deviations from unity of the ratio of nuclear target structure functions to those of deuterium as measured in deep inelastic scattering (often termed the “EMC effect”) have become the canonical observable for studies of nuclear medium modifications to free nucleon structure in the valence regime. The structure function of the free proton is well known from numerous experiments spanning decades. The free neutron structure function, however, has remained difficult to access. Recently it has been extracted in a systematic study of the global data within a parton distribution function extraction framework and is available from the CTEQ–Jefferson Lab (CJ) Collaboration. Here, we leverage the latter to introduce a new method to study the EMC effect in nuclei by reexamining existing data in light of the the magnitude of the medium modifications to the free neutron and proton structure functions independently. From the extraction of the free neutron from world data, it is possible to examine the nuclear effects in deuterium and their contribution to our interpretation of the EMC effect. In this study, we observe that the ratio of the deuteron to the sum of the free neutron and proton structure functions has some x B and Q 2 dependencies that impact the magnitude of the EMC effect as typically observed. Specifically, different EMC slopes are obtained when data from different x B and Q 2 values are utilized. Furthermore, while a linear correlation persists between the EMC and short range correlation effects, the slope is modified when deuteron nuclear effects are removed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Using neutron star observations to determine crust thicknesses, moments of inertia, and tidal deformabilities

Here, we perform a systematic assessment of models for the equation of state (EOS) of dense matter in the context of recent neutron star mass and radius measurements to obtain a broad picture of the structure of neutron stars. We demonstrate that currently available neutron star mass and radius measurements provide strong constraints on moments of inertia, tidal deformabilities, and crust thicknesses. Moreover, a measurement of the moment of inertia of PSR J0737-3039A with a 10% error, without any other information from observations, will constrain the EOS over a range of densities to within 50% 60%. We find tidal deformabilities between 0.6 and 6 1036 g cm 2 s 2 (to 95% confidence) for M = 1.4 M ⊙ , and any measurement which constrains this range will provide an important constraint on dense matter. The crustal fraction of the moment of inertia can be as large as 10% for M = 1.4 M ⊙ permitting crusts to have a large enough moment of inertia reservoir to explain glitches in the Vela pulsar even with a large amount of superfluid entrainment. Finally, due to the uncertainty in the equation of state, there is at least a 40% variation in the thickness of the crust for a fixed mass and radius, which implies that future simulations of the cooling of a neutron star crust which has been heated by accretion will need to take this variation into account.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2011

QCD trace anomaly

In this brief report we compare the predictions of a recent next-to-next-to-leading order hard-thermal-loop perturbation theory (HTLpt) calculation of the QCD trace anomaly to available lattice data. We focus on the trace anomaly scaled by T{sup 2} in two cases: N{sub f}=0 and N{sub f}=3. When using the canonical value of {mu}=2{pi}T for the renormalization scale, we find that for Yang-Mills theory (N{sub f}=0) agreement between HTLpt and lattice data for the T{sup 2}-scaled trace anomaly begins at temperatures on the order of 8T{sub c}, while treating the subtracted piece as an interaction term when including quarks (N{sub f}=3) agreement begins already at temperatures above 2T{sub c}. In both cases we find that at very high temperatures the T{sup 2}-scaled trace anomaly increases with temperature in accordance with the predictions of HTLpt.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2011

Rapid Cooling of the Neutron Star in Cassiopeia A Triggered by Neutron Superfluidity in Dense Matter

We propose that the observed cooling of the neutron star in Cassiopeia A is due to enhanced neutrino emission from the recent onset of the breaking and formation of neutron Cooper pairs in the {sup 3}P{sub 2} channel. We find that the critical temperature for this superfluid transition is {approx_equal}0.5x10{sup 9} K. The observed rapidity of the cooling implies that protons were already in a superconducting state with a larger critical temperature. This is the first direct evidence that superfluidity and superconductivity occur at supranuclear densities within neutron stars. Our prediction that this cooling will continue for several decades at the present rate can be tested by continuous monitoring of this neutron star.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Whole-genome relationships among Francisella bacteria of diverse origins define new species and provide specific regions for detection

Francisella tularensis is a highly virulent zoonotic pathogen that causes tularemia and, because of weaponization efforts in past world wars, is considered a tier 1 biothreat agent. Detection and surveillance of F. tularensis may be confounded by the presence of uncharacterized, closely related organisms. Through DNA-based diagnostics and environmental surveys, novel clinical and environmental Francisella isolates have been obtained in recent years. Here we present 7 new Francisella genomes and a comparison of their characteristics to each other and to 24 publicly available genomes as well as a comparative analysis of 16S rRNA and sdhA genes from over 90 Francisella strains. Delineation of new species in bacteria is challenging, especially when isolates having very close genomic characteristics exhibit different physiological features—for example, when some are virulent pathogens in humans and animals while others are nonpathogenic or are opportunistic pathogens. Species resolution within Francisella varies with analyses of single genes, multiple gene or protein sets, or whole-genome comparisons of nucleic acid and amino acid sequences. Analyses focusing on single genes (16S rRNA, sdhA ), multiple gene sets (virulence genes, lipopolysaccharide [LPS] biosynthesis genes, pathogenicity island), and whole-genome comparisons (nucleotide and protein) gave congruent results, but with different levels of discrimination confidence. We designate four new species within the genus; Francisella opportunistica sp. nov. (MA06-7296), Francisella salina sp. nov. (TX07-7308), Francisella uliginis sp. nov. (TX07-7310), and Francisella frigiditurris sp. nov. (CA97-1460). Lastly, this study provides a robust comparative framework to discern species and virulence features of newly detected Francisella bacteria.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2021

The tundra phenology database: more than two decades of tundra phenology responses to climate change

Observations of changes in phenology have provided some of the strongest signals of the effects of climate change on terrestrial ecosystems. The International Tundra Experiment (ITEX), initiated in the early 1990s, established a common protocol to measure plant phenology in tundra study areas across the globe. Today, this valuable collection of phenology measurements depicts the responses of plants at the colder extremes of our planet to experimental and ambient changes in temperature over the past decades. The database contains 150 434 phenology observations of 278 plant species taken at 28 study areas for periods of 1–26 years. Here we describe the full data set to increase the visibility and use of these data in global analyses and to invite phenology data contributions from underrepresented tundra locations. Portions of this tundra phenology database have been used in three recent syntheses, some data sets are expanded, others are from entirely new study areas, and the entirety of these data are now available at the Polar Data Catalogue (https://doi.org/10.21963/13215).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Formal Approach For Resilient Reachability based on End-System Route Agility

The deterministic nature of existing routing protocols has resulted into an ossified Internet with static and predictable network routes. This gives persistent attackers (e.g. eavesdroppers and DDoS attackers) plenty of time to study the network and identify the vulnerable links (critical) to plan a devastating and stealthy attack. Recently, route mutation approaches have been proposed to address such issues. However, these approaches incur significantly high overhead and depend upon the availability of disjoint routes in the network, which inherently limit their use for mission critical services. To cope with these issues, we extend the current routing architecture to consider end-hosts as routing elements, and present a formal method based agile defense mechanism to increase resiliency of the existing cyber infrastructure. The major contributions of this paper include: (1) formalization of efficient and resilient End to End (E2E) reachability problem as a constraint satisfaction problem, which identifies the potential end-hosts to reach a destination while satisfying resilience and QoS constraints, (2) design and implementation of a novel decentralized End Point Route Mutation (EPRM) protocol, and (3) design and implementation of planning algorithm to minimize the overlap between multiple flows, for the sake of maximizing the agility in the system. Our implementation and evaluation validates the correctness, effectiveness and scalability of the proposed approach.

Rauf, Usman↗
DOE OSTI2017

Status of the Development of Superconducting Undulators for Storage Rings and Free Electron Lasers at the Advanced Photon Source

Development of superconducting undulator (SCU) technology continues at the Advanced Photon Source (APS). The experience of building and successful operating the first short-length, 16-mm period length superconducting undulator SCU0 paved the way for a 1-m long, 18-mm period device— SCU18-1— which has been in operation since May 2015. The APS SCU team has also built and tested a 1.5-m long, 21-mm period length undulator as a part of the LCLS SCU R&D program, aimed at demonstration of SCU technology availability for free electron lasers. This undulator successfully achieved all the requirements including a phase error of 5° RMS. Our team has recently completed one more 1-m long, 18-mm period length undulator— SCU18-2— that is replacing the SCU0. We are also working on a helical SCU for the APS. The status of these projects will be presented.

Ivanyushenkov, Y.↗
DOE OSTI2017

Scoping study to expedite development of a field deployable and portable instrument for UF6 enrichment assay

The primary objective of the present study is to identity the most promising, viable technologies that are likely to culminate in an expedited development of the next-generation, field-deployable instrument for providing rapid, accurate, and precise enrichment assay of uranium hexafluoride (UF6). UF6 is typically involved, and is arguably the most important uranium compound, in uranium enrichment processes. As the first line of defense against proliferation, accurate analytical techniques to determine the uranium isotopic distribution in UF6 are critical for materials verification, accounting, and safeguards at enrichment plants. As nuclear fuel cycle technology becomes more prevalent around the world, international nuclear safeguards and interest in UF6 enrichment assay has been growing. At present, laboratory-based mass spectrometry (MS), which offers the highest attainable analytical accuracy and precision, is the technique of choice for the analysis of stable and long-lived isotopes. Currently, the International Atomic Energy Agency (IAEA) monitors the production of enriched UF6 at declared facilities by collecting a small amount (between 1 to 10 g) of gaseous UF6 into a sample bottle, which is then shipped under chain of custody to a central laboratory (IAEA’s Nuclear Materials Analysis Laboratory) for high-precision isotopic assay by MS. The logistics are cumbersome and new shipping regulations are making it more difficult to transport UF6. Furthermore, the analysis is costly, and results are not available for some time after sample collection. Hence, the IAEA is challenged to develop effective safeguards approaches at enrichment plants. In-field isotopic analysis of UF6 has the potential to substantially reduce the time, logistics and expense of sample handling. However, current laboratory-based MS techniques require too much infrastructure and operator expertise for field deployment and operation. As outlined in the IAEA Department of Safeguards Long-Term R&D Plan, 2012–2023, one of the IAEA long-term R&D needs is to “develop tools and techniques to enable timely, potentially real-time, detection of HEU (Highly Enriched Uranium) production in LEU (Lowly Enriched Uranium) enrichment facilities” (Milestone 5.2). Because it is common that the next generation of analytical instruments is driven by technologies that are either currently available or just now emerging, one reasonable and practical approach to project the next generation of chemical instrumentation is to track the recent trends and to extrapolate them. This study adopted a similar approach, and an extensive literature review on existing and emerging technologies for UF6 enrichment assay was performed. The competitive advantages and current limitations of different analytical techniques for in-field UF6 enrichment assay were then compared, and the main gaps between needs and capabilities for their field use were examined. Subsequently, based on these results, technologies for the next-generation field-deployable instrument for UF6 enrichment assay were recommended. The study was organized in a way that a suite of assessment metric was first identified. Criteria used in this evaluation are presented in Section 1 of this report, and the most important ones are described briefly in the next few paragraphs. Because one driving force for in-field UF6 enrichment assay is related to the demanding transportation regulation for gaseous UF6, Section 2 contains a review of solid sorbents that convert and immobilized gaseous UF6 to a solid state, which is regarded as more transportation friendly and is less regulated. Furthermore, candidate solid sorbents, which show promise in mating with existing and emerging assay technologies, also factor into technology recommendations. Extensive literature reviews on existing and emerging technologies for UF6 enrichment assay, covering their scientific principles, instrument options, and current limitations are detailed in Sections 3 and 4, respectively. In Section 5, the technological gaps as well as start-of-the-art and commercial off-the-shelf components that can be adopted to expedite the development of a fieldable or portable UF6 enrichment-assay instrument are identified and discussed. Finally, based on the results of the review, requirements and recommendations for developing the next-generation field-deployable instrument for UF6 enrichment assay are presented in Section 6.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Modeling efficient and equitable distribution of COVID-19 vaccines

Producing and distributing COVID-19 vaccine during the pandemic is a major logistical challenge requiring careful planning and efficient execution. This report presents information on logistical, policy and technical issues relevant to rapidly fielding a COVID-19 vaccination program. For this study we (a) conducted literature review and subject matter expert elicitation to understand current vaccine manufacturing and distribution capabilities and vaccine allocation strategies, (b) designed a baseline vaccine distribution strategy and modeling strategy to provide insight into the potential for targeted distribution of limited initial vaccine supplies, and (c) developed parametric interfaces to enable vaccine distribution scenarios to be analyzed in depth with Sandias Adaptive Recovery Model that will allow us evaluate the additional sub- populations and alternative distribution scenarios from a public health benefit and associated economic disruption Principal issues, challenges, and complexities that complicate COVID-19 vaccine delivery identified in our literature and subject matter expert investigation include these items: The United States has not mounted an urgent nationwide vaccination campaign in recent history. The existing global manufacturing and distribution infrastructure are not able to produce enough vaccine for the population immediately. Vaccines, once available will be scarce resources. Prioritization for vaccine allocation will be built on existing distribution networks. Vaccine distribution may not have a universal impact on disease transmission and morbidity because of scarcity, priority population demographics, and underlying disease transmission rates. Considerations for designing a vaccine distribution strategy are discussed. A baseline distribution strategy is designed and tested using the Adaptive Recovery Model, which couples a deterministic compartmental epidemiological model and a stochastic network model. We show the impact of this vaccine distribution strategy on hospitalizations, mortality, and contact tracing requirements. This model can be used to quantitatively evaluate alternative distribution scenarios, guiding policy decisions as vaccine candidates are narrowed down.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2025

Stockpile Stewardship and Nuclear Testing: A Technical Assessment

Since 1992, the United States has retained confidence in its nuclear weapon stockpile without performing any tests that produce nuclear yield. Instead, it has invested in a stockpile stewardship program (SSP) based on the same approach that was validated through fifty years of experience during the nuclear testing era. As the test moratorium continues and new information becomes available, it is both necessary and appropriate to periodically revisit the question of whether or not nuclear testing should resume. In a recent article by Dr. Mark Schneider, he asserts that the United States should return to nuclear testing to address the issues that negatively affect our country’s nuclear deterrent. A serious, technically informed evaluation of the most significant of the issues Dr. Schneider has raised is provided in this paper. The conclusion of this evaluation is that the strategy of a well-funded SSP coupled with rigorous assessments to identify if there is a specific need for a nuclear test is sound and cost-effective approach. Any decision otherwise needs to take into careful consideration all the classified SSP successes and data pertaining to the particular issues in question.

45 MILITARY TECHNOLOGY, WEAPONRY, AND NATIONAL DEF↗
DOE OSTI2010

Indispensable Roles of Plastids in Arabidopsis thaliana Embryogenesis

The plastid is an organelle vital to all photosynthetic and some non-photosynthetic eukaryotes. In the model plant Arabidopsis thaliana, a number of nuclear genes encoding plastid proteins have been found to be necessary for embryo development. However, the exact roles of plastids in this process remain largely unknown. Here we use publicly available datasets to obtain insights into the relevance of plastid activities to A. thaliana embryogenesis. By searching the SeedGenes database (http://www.seedgenes.org) and recent literature, we found that, of the 339 non-redundant genes required for proper embryo formation, 108 genes likely encode plastid-targeted proteins. Nineteen of these genes are necessary for development of preglobular embryos and/or their conversion to globular embryos, of which 13 genes encode proteins involved in non-photosynthetic metabolism. By contrast, among 38 genes which are dispensable for globular embryo formation but necessary for further development, only one codes for a protein involved in metabolism. Products of 21 of the 38 genes play roles in plastid gene expression and maintenance. Examination of RNA profiles of embryos at distinct growth stages obtained in laser-capture microdissection coupled with DNA microarray experiments revealed that most of the identified genes are expressed throughout embryo morphogenesis and maturation. These findings suggest that metabolic activities are required at preglobular and throughout all stages of embryo development, whereas plastid gene expression becomes necessary during and/or after the globular stage to sustain various activities of the organelle including photosynthetic electron transport.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2021

Estimation of the Ambient Wind Field From Wind Turbine Measurements Using Gaussian Process Regression

In the search for a lower levelized cost of wind energy, one approach is to increase the accuracy of wind turbine measurements such as wind speed and wind direction. The sensors available on wind turbines are susceptible to local turbulence and measurement bias, which can result in suboptimal turbine performance. As an alternative, recent research has considered using the sensor measurements in a coordinated manner. With such a cooperative approach, the local wind conditions can be estimated more accurately and reliably without the need for additional measurement equipment. In this paper, a novel wind field estimation approach is presented that estimates the local wind conditions based on turbine measurements using Gaussian processes. We show that the estimation framework is able to improve the accuracy of the wind direction estimate both in an offline and online manner, as well as identify possible biases in the sensors and reduce unnecessary wind turbine yaw activity.

49 EE - Wind and Water Power Program - Wind (EE-4W↗
DOE OSTI2012

Catabolism and Deactivation of the Lipid-Derived Hormone Jasmonoyl-Isoleucine

The oxylipin hormone jasmonate controls myriad processes involved in plant growth, development, and immune function. The discovery of jasmonoyl-L-isoleucine (JA-Ile) as the major bioactive form of the hormone highlights the need to understand biochemical and cell biological processes underlying JA-Ile homeostasis. Among the major metabolic control points governing the accumulation of JA-Ile in plant tissues are the availability of jasmonic acid, the immediate precursor of JA-Ile, and oxidative enzymes involved in catabolism and deactivation of the hormone. Recent studies indicate that JA-Ile turnover is mediated by a ω-oxidation pathway involving members of the CYP94 family of cytochromes P450. This discovery opens new opportunities to genetically manipulate JA-Ile levels for enhanced resistance to environmental stress, and further highlights ω-oxidation as a conserved pathway for catabolism of lipid-derived signals in plants and animals. Functional characterization of the full complement of CYP94 P450s promises to reveal new pathways for jasmonate metabolism and provide insight into the evolution of oxylipin signaling in land plants.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Global Carbon Budget 2024

Abstract. Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere in a changing climate is critical to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe and synthesize datasets and methodologies to quantify the five major components of the global carbon budget and their uncertainties. Fossil CO2 emissions (EFOS) are based on energy statistics and cement production data, while emissions from land-use change (ELUC) are based on land-use and land-use change data and bookkeeping models. Atmospheric CO2 concentration is measured directly, and its growth rate (GATM) is computed from the annual changes in concentration. The global net uptake of CO2 by the ocean (SOCEAN, called the ocean sink) is estimated with global ocean biogeochemistry models and observation-based fCO2 products (fCO2 is the fugacity of CO2). The global net uptake of CO2 by the land (SLAND, called the land sink) is estimated with dynamic global vegetation models. Additional lines of evidence on land and ocean sinks are provided by atmospheric inversions, atmospheric oxygen measurements, and Earth system models. The sum of all sources and sinks results in the carbon budget imbalance (BIM), a measure of imperfect data and incomplete understanding of the contemporary carbon cycle. All uncertainties are reported as ±1σ. For the year 2023, EFOS increased by 1.3 % relative to 2022, with fossil emissions at 10.1 ± 0.5 GtC yr−1 (10.3 ± 0.5 GtC yr−1 when the cement carbonation sink is not included), and ELUC was 1.0 ± 0.7 GtC yr−1, for a total anthropogenic CO2 emission (including the cement carbonation sink) of 11.1 ± 0.9 GtC yr−1 (40.6 ± 3.2 GtCO2 yr−1). Also, for 2023, GATM was 5.9 ± 0.2 GtC yr−1 (2.79 ± 0.1 ppm yr−1; ppm denotes parts per million), SOCEAN was 2.9 ± 0.4 GtC yr−1, and SLAND was 2.3 ± 1.0 GtC yr−1, with a near-zero BIM (−0.02 GtC yr−1). The global atmospheric CO2 concentration averaged over 2023 reached 419.31 ± 0.1 ppm. Preliminary data for 2024 suggest an increase in EFOS relative to 2023 of +0.8 % (−0.2 % to 1.7 %) globally and an atmospheric CO2 concentration increase by 2.87 ppm, reaching 422.45 ppm, 52 % above the pre-industrial level (around 278 ppm in 1750). Overall, the mean of and trend in the components of the global carbon budget are consistently estimated over the period 1959–2023, with a near-zero overall budget imbalance, although discrepancies of up to around 1 GtC yr−1 persist for the representation of annual to semi-decadal variability in CO2 fluxes. Comparison of estimates from multiple approaches and observations shows the following: (1) a persistent large uncertainty in the estimate of land-use change emissions, (2) low agreement between the different methods on the magnitude of the land CO2 flux in the northern extra-tropics, and (3) a discrepancy between the different methods on the mean ocean sink. This living-data update documents changes in methods and datasets applied to this most recent global carbon budget as well as evolving community understanding of the global carbon cycle. The data presented in this work are available at https://doi.org/10.18160/GCP-2024 (Friedlingstein et al., 2024).

Friedlingstein, Pierre (ORCID:0000000333094739)↗
DOE OSTI2026

Global Carbon Budget 2025

Accurate assessment of anthropogenic carbon dioxide (CO 2 ) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere in a changing climate is critical to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe and synthesise datasets and methodologies to quantify the five major components of the global carbon budget and their uncertainties. Fossil CO 2 emissions (E FOS ) are based on energy and cement production data. Emissions from land-use change (E LUC ) are estimated by bookkeeping models based on land-use data. The global atmospheric CO 2 growth rate (G ATM ) is computed from changes in concentration measured at surface stations. The global net uptake of CO 2 by the ocean (S OCEAN ) is estimated with global ocean biogeochemistry models and observation-based fCO 2 -products. The global net uptake of CO 2 by the land (S LAND ) is estimated with dynamic global vegetation models. Additional lines of evidence are provided by atmospheric inversions, atmospheric oxygen measurements, ocean interior observation-based estimates, and Earth System Models. This year, we introduced corrections on the E LUC , S OCEAN and S LAND estimates. The sum of all sources and sinks results in the carbon budget imbalance (B IM ), a measure of imperfect data and incomplete understanding of the contemporary carbon cycle. All uncertainties are reported as ± 1σ. For the year 2024, E FOS increased by 1.1 % relative to 2023, with fossil emissions at 10.3 ± 0.5 GtC yr −1 (including the cement carbonation sink, 0.2 GtC yr −1 ), E LUC was 1.3 ± 0.7 GtC yr −1 , for total anthropogenic CO 2 emissions of 11.6 ± 0.9 GtC yr −1 (42.4 ± 3.2 GtCO2 yr −1 ). Also, for 2024, G ATM was 7.9 ± 0.2 GtC yr−1 (3.73 ± 0.1 ppm yr −1 ), 2.2 GtC above the 2023 growth rate. SOCEAN was 3.4 ± 0.4 GtC yr −1 and S LAND was 1.9 ± 1.1 GtC yr −1 , leaving a large negative B IM (−1.7 GtC yr −1 ), suggesting that the total sink or G ATM is strongly overestimated in 2024. The global atmospheric CO 2 concentration averaged over 2024 reached 422.8 ± 0.1 ppm. Preliminary data for 2025 suggest an increase in E FOS relative to 2024 of +1.0 % (0.2 % to 1.7 %) globally, and atmospheric CO 2 concentration increasing by 2.1 ppm reaching 425.6 ppm, 53 % above the pre-industrial level (around 278 ppm in 1750). Overall, the mean and trend in the components of the global carbon budget are consistently estimated over the period 1959–2024, with a near-zero overall budget imbalance, although discrepancies of up to around 1 GtC yr −1 persist for the representation of annual to decadal variability in CO 2 fluxes. Comparison of estimates from multiple approaches and observations shows: (1) a persistent large uncertainty in the estimate of land-use change emissions, (2) a low agreement between the different methods on the magnitude of the land CO 2 flux in the northern extra-tropics, and (3) a discrepancy between the different methods on the mean ocean sink. This living data update documents changes in methods and datasets applied to this most-recent global carbon budget as well as evolving community understanding of the global carbon cycle. The data presented in this work are available at https://doi.org/10.18160/GCP-2025 (Friedlingstein et al., 2025c).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2011

Development of moving bed simulation model for carbon capture from fossil energy systems.

The capture and separation of carbon dioxide (CO2) has been identified as a high-priority topic to cope with global climate change. Fossil fuels currently supply the most of the world's energy needs, and their utilization is the major source of the anthropogenic CO2 emission [1]. Particularly, the existing coal-fired power plants annually emit about 2 billion tons of CO2 which is equivalent to two-thirds of the total emissions from U.S. power sector [2]. Therefore, it is critical to develop the cost-effective technologies to mitigate this problem. There are three options for capture for capturing CO2 from fossil energy system: post-combustion capture, pre-combustion capture, and oxy-combustion. Among them, post-combustion capture has the greatest near-term potential for reducing CO2 emission, because it can be applied to the existing coal-fired power plant with relative ease through a retrofit. The current commercially available solvent-based processes have advantages of fast kinetics and strong reactions, however only at a significant cost and efficiency penalty. Recently, various solid sorbents are being explored for one of promising CO2 capture technology, which are expected to reduce energy requirement and water usage with the approaches of fluidized or moving bed. However, solids are inherently more difficult to work with than liquids and no large scale system has yet been commercialized. In this study, we developed the rigorous 1-D PDE model for moving beds in Aspen Custom Modeler; the entire system consists of adsorbers, regenerators, and auxiliary equipment. The simulation result will be expected to compare with those of other post-combustion processes. We will deal with not only advantages of lower capital costs and power requirements but also problems associated with pressure drop and heat transfer.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗
DOE OSTI2013

ENRICHED STABLE ISOTOPE TARGET PREPARATION AT THE OAK RIDGE NATIONAL LABORATORY

Since the 1960s the Department of Energy (DOE) Isotope Program, through the Isotope Development Group at the Oak Ridge National Laboratory, has been developing and supplying, among other things, enriched stable isotope targets for nuclear research around the world. This group also maintains and distributes the DOE inventory of enriched stable isotopes. Chemical and pyrochemical techniques are used to prepare enriched stable isotopes from this inventory in the desired chemical form. Metallurgical, ceramic, or vacuum processing methods are then used to prepare the isotopes in a wide range of physical forms from thin films, foils, and coatings to large fabricated shapes to meet the needs of experimenters. Significant characterization capabilities are also available to assist in the preparation and evaluation of these custom materials. This work is part of the DOE Isotope Program, which recently transferred to the Office of Nuclear Physics, DOE Office of Science, resulting in a stronger emphasis on enabling R&D. This presentation will focus on the custom preparation of enriched stable isotope targets and other research materials.

accelerator targets↗