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At least 1,513 records · Page 84
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Progress on Light-Element Standard Cross Sections at Los Alamos [Slides]

Presenters identified the following statuses of the light-element standards: Extension of N-N scattering analysis to 200 MeV will likely come in time for ENDF/B VIII.1 and new data are to be added even in the energy range up to 100 MeV; for n- 3 He, a more recent 4 He R-matrix analysis from which updated n+ 3 He cross sections could be obtained for ENDF/B VIII.1; for n- 6 Li, more work is required to get a reasonable fit to all data up to E n = 8 MeV. Of particular concern are the t+ 4 He scattering data at E t > 14 MeV. For n- 10 B, new work on the 11 B system has not yet been started and there is much new data to add for n+ 10 B reactions, and maybe also for &#945 + 7 Li reactions. The proliferation of excited-state channels will limit the upper neutron energy of the analysis to a few MeV. For n- 12 C, new elastic and inelastic scattering data from Vanhoy support the results of the present analysis. More work is needed to extend the fit successfully above 6.5 MeV.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

AMPX Status 2024 [Slides]

This presentation focus on AMPX development for 2024 it also touches on ENDF/B-VIII.1. The slides touches on Thermal Neutron Scattering Library, AMPX Development Highlights, and Transport libraries for SCALE 7.0.0.

ENDF/B-VIII.1↗
DOE OSTI2020

Superfluidity in Disordered Neutron Stars Crusts

Nonequilibrium conditions imposed by neutrino cooling through the liquid-solid transition lead to disorder in the solid crust of neutron stars. Disorder reduces the superfluid fraction, $\rho_s/\rho$, at densities above that of neutron drip, $\rho_d \approx 4\times 10^{11}\,g/cm^3$. For an amorphous solid crust the suppression of $\rho_s$ is small, except in the highest density regions of the crust. In contrast to the strong reduction in neutron conduction predicted for coherent Bragg scattering in a crystalline crust, the disordered solid crust supports sufficient neutron superfluid density to account for pulsar glitches.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Designing observables for measurements with deep learning

Many analyses in particle and nuclear physics use simulations to infer fundamental, effective, or phenomenological parameters of the underlying physics models. When the inference is performed with unfolded cross sections, the observables are designed using physics intuition and heuristics. We propose to design targeted observables with machine learning. Unfolded, differential cross sections in a neural network output contain the most information about parameters of interest and can be well-measured by construction. The networks are trained using a custom loss function that rewards outputs that are sensitive to the parameter(s) of interest while simultaneously penalizing outputs that are different between particle-level and detector-level (to minimize detector distortions). We demonstrate this idea in simulation using two physics models for inclusive measurements in deep inelastic scattering. We find that the new approach is more sensitive than classical observables at distinguishing the two models and also has a reduced unfolding uncertainty due to the reduced detector distortions.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

Volume 4: Detection Systems and Ultra-Cold Neutrons

As part of the Sustaining and Enhancing Nuclear Science (SENSe) initiative at Oak Ridge National Laboratory (ORNL), the prospect of adding new detection systems to support High Flux Isotope Reactor (HFIR) operations and to advance scientific research has prompted many ideas and discussions regarding potential features, configurations, locations, and applications. A working group of ORNL staff members was organized to further develop the concepts and recommending one or more configurations to best support future HFIR operations and scientific capacities and to provide order-of-magnitude cost estimates and timing. The areas of investigation included fast access detection systems, non-scattering beamline instruments, shielded detection instruments, and an ultracold neutron source. In each case, the focus was to develop world leading capabilities that would be unmatched by any other facility.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
NASA NTRS1993

A search for energetic ion directivity in large solar flares

One of the key observational questions for solar flare physics is: What is the number, the energy spectrum, and the angular distribution of flare accelerated ions? The standard method for deriving ion spectral shape employs the ratio of influences observed on the 4-7 MeV band to the narrow neutron capture line at 2.223 MeV. The 4-7 MeV band is dominated by the principal nuclear de-excitation lines from C-12 and O-16 which are generated in the low chromosphere by the direct excitation or spallation of nuclei by energetic ions. In contrast, the narrow 2.223 MeV line is produced by the capture of thermal neutrons on protons in the photosphere. These capture neutrons are generated by energetic ion interactions and thermalized by scattering in the solar atmosphere. In a series of papers, Ramaty, Lingenfelter, and their collaborators have calculated the expected ratio of fluence in the 4-7 MeV band to the 2.223 MeV line for a wide range of energetic ion spectral shapes (see, e.g. Hua and Lingenfelter 1987). Another technique for deriving ion spectral shapes and angular distributions uses the relative strength of the Compton tail associated with the 2.223 MeV neutron capture line (Vestrand 1988, 1990). This technique can independently constrain both the angular and the energy distribution of the energetic parent ions. The combination of this tail/line strength diagnostic with the line/(4-7) MeV fluence ratio can allow one to constrain both properties of the energetic ion distributions. The primary objective of our Solar Maximum Mission (SMM) guest investigator program was to study measurements of neutron capture line emission and prompt nuclear de-excitation for large flares detected by the Solar Maximum Mission/ Gamma-Ray Spectrometer (SMM/GRS) and to use these established line diagnostics to study the properties of flare accelerated ions.

Vestrand, W. Thomas↗
DOE OSTI2022

Updates and Validation for the n+ 63,65 Cu Cross Sections [Abstract]

The neutron induced total, elastic, and capture cross sections of 63,65 Cu isotopes were selected for evaluation in the resolved and unresolved resonance energy ranges by the National Criticality Safety Program to resolve discrepancies related to benchmark performance. This is especially evident for the series of ZEUS benchmarks in which copper is used as a reflector. Because copper is also used as structural material in both fission and fusion reactors, the need to address benchmark discrepancies linked to nuclear data deficiencies is a task of primary importance. The aim of this work is to describe the steps of evaluation work towards a consistent improvement of the benchmark performance. The R-matrix analysis with the SAMMY code focused on the 63 Cu(n,γ) reaction channel between 100-300 keV coupled to unresolved resonance region parameters up to 650 keV to fit average cross section data from a recent experiment. Due to the high sensitivity of many benchmarks to elastic scattering angular distribution data, especially for the 65 Cu isotope, the impact of these data was tested by generating Legendre coefficients from both resonance parameters and the Hauser-Feshbach model. Guided by the findings of Shaw et al., the performance of the current evaluation for 65 Cu was compared to that of ENDF/B-VII.1 and ENDF/B-VIII.0 by testing the reactivity coefficients corresponding to the validation suite of experimental criticality benchmarks for thermal, intermediate, and fast systems taken from the International Criticality Safety Benchmark Experiments Project Handbook. The benchmark performance is especially sensitive to 63 Cu(n,γ) and 65 Cu elastic scattering for neutron energies in the 100–500 keV region, whereas 100 keV is the upper limit of the resolved resonance region in the ENDF/B-VIII.0 evaluations for 63,65 Cu. The results highlight the need to handle the transition from the resolved resonance region to the high energy region carefully.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2022

From classical to quantum dynamics of atomic and ionic species interacting with graphene and its analogue

Graphene and its analogues offer a broad range of application opportunities for (opto)-electronics, sensing, catalysis, phase separation, energy conversion and storage, etc. Engineering graphene properties often relies on its controllable functionalization, defect formation and patterning, and reactive gas etching. In this chapter, we survey the dynamics of graphene using classical and quantum-classical dynamics methods. We discuss the reactivity, scattering, and transmission of atomic and ionic species including Ar cluster ion, H/D, and H+/D+ on graphene flakes of various sizes, focusing on the atomic-scale motion and energy dissipation pathways involved in forming and breaking covalent bonding. Discussions on the nuclear quantum effects of light species, the effects of isotopic substitution, and the methodologies for such modeling are also included.

Garashchuk, Sofiya V.↗
DOE OSTI2022

The Gamow shell model with realistic interactions: a theoretical framework for ab initio nuclear structure at drip-lines

Abstract Ab initio approaches are among the most advanced models to solve the nuclear many-body problem. In particular, the no-core–shell model and many-body perturbation theory have been recently extended to the Gamow shell model framework, where the harmonic oscillator basis is replaced by a basis bearing bound, resonance and scattering states, i.e. the Berggren basis. As continuum coupling is included at basis level and as configuration mixing takes care of inter-nucleon correlations, halo and resonance nuclei can be properly described with the Gamow shell model. The development of the no-core Gamow shell model and the introduction of the Q ¯ ˆ -box method in the Gamow shell model, as well as their first ab initio applications, will be reviewed in this paper. Peculiarities compared to models using harmonic oscillator bases will be shortly described. The current power and limitations of ab initio Gamow shell model will also be discussed, as well as its potential for future applications.

Physics↗
DOE OSTI2021

Theory of ultrafast photoinduced low-to-high spin crossover in divalent iron systems

Here a theory is developed for the ultrafast low-to-high spin transition in divalent iron. Following the photoinduced metal-to-ligand charge transfer (MLCT), the 1 A 1 MLCT state decays on a sub-100-fs timescale into the 5 T 2 MLCT using a 3 T 1 MLCT state as intermediary. Damping of nuclear motion is crucial in obtaining a full singlet-to-quintet transition mediated by the spin-orbit interaction. Destructive interference suppresses transitions to metal-centered (MC) states. The relaxation to the MC 5 T 2 is a result of Coulomb scattering with the surroundings.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Neutrino-nucleus CC 0 π cross-section tuning in GENIE v3

This article summarizes the state of the art of v μ and $\bar{v}_μ$ CC0π cross-section measurements on carbon and argon and discusses the relevant nuclear models, parametrizations and uncertainties in GENIE v3. The CC0π event topology is common in experiments at a few-GeV energy range. Although its main contribution comes from quasi-elastic interactions, this topology is still not well understood. The GENIE global analysis framework is exploited to analyze CC0π datasets from MiniBooNE, T2K and MINERvA. A partial tune for each experiment is performed, providing a common base for the discussion of tensions between datasets. The results offer an improved description of nuclear CC0π datasets as well as data-driven uncertainties for each experiment. This work is a step towards a GENIE global tune that improves our understanding of neutrino interactions on nuclei. It follows from earlier GENIE work on the analysis of neutrino scattering datasets on hydrogen and deuterium.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Characterization of the Sulfur Saturated Versions of the High-Chromium Matrix Glasses

In this report, the Savannah River National Laboratory provides chemical analysis of a series of sulfur saturated melt versions of simulated nuclear waste glasses, and chemical analysis of the wash solutions resulting from the preparation of these glasses. The glasses were selected and fabricated by the Pacific Northwest National Laboratory as part of a broader study of the influence of glass composition on chemical durability, sulfur retention, and other properties. The resulting data will be used in the development of improved property/composition models to support operation of the Hanford Tank Waste Treatment and Immobilization Plant. Some degree of scatter among the Al₂O₃, B₂O₃, CaO, K₂O, Na₂O, and SiO₂ measurements was noted for the study glasses. The measured concentrations of B₂O₃, chlorine, and fluorine were below the targeted values for most of the study glasses, likely because of volatility during the multiple melting steps. The measured concentrations of Cr₂O₃ and K₂O were generally low relative to the targeted values. These components were identified in the wash solutions, indicating partitioning to the excess sulfate phase that was washed from the glasses prior to analyses. As expected, the measured concentrations of SO₃ in the glasses were higher than targeted due to the use of the sulfur saturation method in fabricating these glasses. Minor scatter among the triplicate measurements of some of the analytes of the wash solutions was noted. The wash solutions contained mainly sulfur and sodium, with moderate concentrations of chromium and potassium. Revision 1 of this report corrects the omission of Al₂O₃ values from Table A-4 in Appendix A.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2020

Building Interfaces with Echo Using R

The following report details the functionality that was developed to directly query the MongoDB and read in echo records from within R, and the ability to create a cinema database directly from echo records. Both of these efforts used the data collected under the MINOS project for development. The nuclear facility under consideration is the High-Flux Isotope Reactor (HFIR) and co-located Radiochemical Engineering Development Center (REDC) at Oak Ridge National Laboratory in Oak Ridge, TN. HFIR is an 85 MW research reactor and is used primarily for production of a medical radioisotopes, material irradiation experiments, neutron activation, and neutron scattering. Targets for the reactor are fabricated and processed and dissolved at REDC, in addition to other glove-box and hot-cell type activities. An overhead view of the facility is provided. The rest of the report is organized as follows: Section 2 describes how to query the MongoDB and load in echo records from within R, with background information on the database type, MongoDB, and the file format of echo records, hdf5, as well as lessons learned during the development phase. Section 3 details the functionality and usage of creating a cinema database directly from echo records within R. A series of appendixes display all the R code (Section 5), some example scripts where the code is used (Section 6), and useful links for further exploration (Section 7).

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2020

Ab initio study of ${(\nu_\ell,\ell^-)}$ and ${(\overline{\nu}_\ell,\ell^+)}$ inclusive scattering in $^{12}\hbox{C}$: confronting the MiniBooNE and $\hbox{T2K CCQE}$ data

We carry out an ab initio calculation of the neutrino flux-folded inclusive cross sections, measured on $^{12}$C by the MiniBooNE and T2K collaborations in the charged-current quasielastic regime. The calculation is based on realistic two- and three-nucleon interactions, and on a realistic nuclear electroweak current with one-and two-nucleon terms that are constructed consistently with these interactions and reproduce low-energy electroweak transitions. Numerically exact quantum Monte Carlo methods are utilized to compute the nuclear weak response functions, by fully retaining many-body correlations in the initial and final states and interference effects between one- and two-body current contributions. We employ a nucleon axial form factor of the dipole form with $\Lambda_A = 1.0$ or $1.15$ GeV, the latter more in line with a very recent lattice QCD determination. The calculated cross sections are found to be in good agreement with the neutrino data of MiniBooNE and T2K, and antineutrino MiniBooNE data, yielding a consistent picture of nuclei and their electroweak properties across a wide regime of energy and momenta.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Holographic wavefront sensors

A brief historical review of the first designs of holographic wavefront sensors (WFS’s) and the concepts lying in their basis is presented. The main directions in the development of these sensors are highlighted and considered. One of these directions implies a two-stage transition from the use of several separate measuring channels with holograms filtering only one Zernike mode: first to the use of one channel with a multiplexed hologram filtering several first Zernike modes, and then to filtering the entire set of Zernike modes with the aid of one combined multiplexed hologram. Another line of research in this field (related to the first one) is the optimisation of the filter hologram structure in order to reduce cross-modulation interferences, increase multiplexing level, etc. One more line of research implements principles of dynamic holography by introducing spatial light modulators into the WFS composition. Hence, the advantages of time multiplexing of holograms can be used. The approach developed by G. Andersen’s team, aimed at adapting the holographic WFS design for operation as an element of adaptive optical system with a zonal corrector, as well as an approach implying development of hybrid holographic sensors, are considered separately. The results of the authors’ studies of holographic WFS’s with application of the methods of Fourier holography (i.e., holography of focused beams, in particular, using diffuse scatterers in a hologram recording channel) are also reported. (paper)

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Entanglement maximization in low-energy neutron-proton scattering

The entanglement properties of neutron-proton scattering are investigated using a measure that counts the number of entangled pairs produced by the action of a scattering operator on a given initial neutron-proton state. All phase shifts relevant for scattering at laboratory energies up to 350 MeV are used. Entanglement is found to depend strongly on the initial state. Entanglement is maximized in very low energy scattering if the initial spin state is | ↑ ↓ >, but not if the initial state is | ↑ ↑ > . At such energies the Hamiltonian obeys Wigner SU(4) symmetry, and an entanglement maximum is a sign of that symmetry. At higher energies the angular dependence of entanglement is strong and the entanglement is large for many scattering angles. Furthermore, the tensor force is shown to play a significant role in producing entanglement at laboratory kinetic energies greater than about 50 MeV.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

AMPX Developments in 2024 [Slides]

The priority for AMPX development for FY2024 has been to support processing the ENDF/B-VIII.1 library. This includes the development to support Thermal Neutron Scattering Library, GNDS-2.1 support and AMPX maintenance, and transport libraries for SCALE 7.0.0.

Nuclear Criticality Safety Program (NCSP)↗