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At least 1,513 records · Page 84

Enlarged Nonclosure of Surface Energy Balance With Increasing Atmospheric Instabilities Linked to Changes in Coherent Structures

The nonclosure of surface energy balance remains an outstanding problem in eddy covariance (EC) measurements of land-surface fluxes of heat, water vapor, and CO 2 . Our data collected from an EC tower over a semiarid sagebrush ecosystem indicate that under unstable atmospheric conditions, the nonclosure becomes increased with increasing instability, consistent with many other studies. It is demonstrated that the increased nonclosure is not caused by the inadequate sampling of large-scale turbulent motions using a 30-min averaging interval, though the scales of turbulent motions dominating sensible and latent heat fluxes become enlarged with increasing instability. Quadrant analysis is then used to reveal that the flux contributions from ejections remain nearly constant with increasing instability, whereas the flux contributions from sweeps are reduced and their time fractions increase. Our results imply that the increased nonclosure of surface energy balance is associated with changes in turbulent structures including their dominant time scales and flux contributions of ejections and sweeps as the atmospheric instability increases, which require further studies using vertically distributed observations and/or large eddy simulations.

54 ENVIRONMENTAL SCIENCES↗

Coherent multidimensional photoelectron spectroscopy of ultrafast quasiparticle dressing by light

Abstract Depending on the applied strength, electromagnetic fields in electronic materials can induce dipole transitions between eigenstates or distort the Coulomb potentials that define them. Between the two regimes, they can also modify the electronic properties in more subtle ways when electron motion becomes governed by time and space-periodic potentials. The optical field introduces new virtual bands through Floquet engineering that under resonant conditions interacts strongly with the preexisting bands. Under such conditions the virtual bands can become real, and real ones become virtual as the optical fields and electronic band dispersions entangle the electronic response. We reveal optical dressing of electronic bands in a metal by exciting four-photon photoemission from the Cu(111) surface involving a three-photon resonant transition from the Shockley surface band to the first image potential band. Attosecond resolved interferometric scanning between identical pump–probe pulses and its Fourier analysis reveal how the optical field modifies the electronic properties of a solid through combined action of dipole excitation and field dressing.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗