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NASA NTRS1994

Plant Responses to Increased UV-B Radiation: A Research Project

Ozone decrease implies more ultraviolet-B (UV-B) radiation reaching the surface of the Earth. Increased UV-B radiation triggers responses by living organisms. Despite the large potential impacts on vegetation, little is known about UV-B effects on terrestrial ecosystems. Long-term ecological studies are needed to quantify the effects of increased UV radiation on terrestrial ecosystems, asses the risks, and produce reliable data for prediction. Screening pigments are part of one of the protective mechanism in plants. Higher concentrations of screening pigments in leaves may be interpreted as a response to increased UV radiation. If the screening effect is not sufficient, important molecules will be disturbed by incoming radiation. Thus, genetics, photosynthesis, growth, plant and leaf shape and size, and pollen grains may be affected. This will have an impact on ecosystem dynamics, structure and productivity. It is necessary to monitor selected terrestrial ecosystems to permit detection and interpretation of changes attributable to global climate change and depleted ozone shield. The objectives of this project are: (1) To identify and measure indicators of the effects of increased solar UV-B radiation on terrestrial plants; (2) to select indicators with the greatest responses to UV-B exposure; (3) to test, adapt or create ecosystem models that use the information gathered by this project for prediction and to enhance our understanding of the effects of increased UV-B radiation on terrestrial ecosystems. As a first step to achieve these objectives we propose a three-year study of forest and steppe vegetation on the North slope of the Brooks Range (within the Arctic circle, in Alaska), in the Saguaro National Monument (near Tucson, Arizona) and in the forests and steppes of Patagonia (Argentina). We selected (1) vegetation north of the Polar Circle because at 70N there is 8% risk of plant damage due to increased UV-B radiation; (2) the foothills of Catalina Mountains because there is anecdotal evidence of plant damage on the saguaros that has been linked to increased UV radiation, and (3) the forests of Nothofagus spp. and the steppe of Patagonia where the risk of plant damage at 35S is 5% and increases to as much as 15% at 55S due to increased UV-B radiation. Measurements of UV-B radiation impinging on the surface at 55S largely exceed the predicted UV-B radiation values at 50 latitude and 0% ozone depletion. Preliminary HPLC analyses of UV-B absorbing compounds in Nothofagus antartica, N. pumilio, N. betuloides and Rumex sp. in natural conditions show species-specific patterns. The spectrum of N. antartica grown at 38S differs significantly from that of N. antartica in natural conditions in Ushuaia (55S). These results suggest that the selected main area (Patagonia) is appropriate for assessing the problem and its magnitude and that Nothofagus is appropriate for our study.

DAntoni, H. L.↗

DOE OSTI2022

Indices of extremes: geographic patterns of change in extremes and associated vegetation impacts under climate intervention

Extreme weather events have been demonstrated to be increasing in frequency and intensity across the globe and are anticipated to increase further with projected changes in climate. Solar climate intervention strategies, specifically stratospheric aerosol injection (SAI), have the potential to minimize some of the impacts of a changing climate while more robust reductions in greenhouse gas emissions take effect. However, to date little attention has been paid to the possible responses of extreme weather and climate events under climate intervention scenarios. We present an analysis of 16 extreme surface temperature and precipitation indices, as well as associated vegetation responses, applied to the Geoengineering Large Ensemble (GLENS). GLENS is an ensemble of simulations performed with the Community Earth System Model (CESM1) wherein SAI is simulated to offset the warming produced by a high-emission scenario throughout the 21st century, maintaining surface temperatures at 2020 levels. GLENS is generally successful at maintaining global mean temperature near 2020 levels; however, it does not completely offset some of the projected warming in northern latitudes. Some regions are also projected to cool substantially in comparison to the present day, with the greatest decreases in daytime temperatures. The differential warming–cooling also translates to fewer very hot days but more very hot nights during the summer and fewer very cold days or nights compared to the current day. Extreme precipitation patterns, for the most part, are projected to reduce in intensity in areas that are wet in the current climate and increase in intensity in dry areas. We also find that the distribution of daily precipitation becomes more consistent with more days with light rain and fewer very intense events than currently occur. In many regions there is a reduction in the persistence of long dry and wet spells compared to present day. However, asymmetry in the night and day temperatures, together with changes in cloud cover and vegetative responses, could exacerbate drying in regions that are already sensitive to drought. Overall, our results suggest that while SAI may ameliorate some of the extreme weather hazards produced by global warming, it would also present some significant differences in the distribution of climate extremes compared to the present day.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2020

Impacts of Wildfire Aerosols on Global Energy Budget and Climate: The Role of Climate Feedbacks

Aerosols emitted from wildfires could significantly affect global climate through perturbing global radiation balance. In this study, the Community Earth System Model with prescribed daily fire aerosol emissions is used to investigate fire aerosols’ impacts on global climate with emphasis on the role of climate feedbacks. The total global fire aerosol radiative effect (RE) is estimated to be -0.78 ± 0.29 W m -2 , which is mostly from shortwave RE due to aerosol–cloud interactions (REaci; -0.70 ± 0.20 W m -2 ). The associated global annual-mean surface air temperature (SAT) change ΔT is -0.64 ± 0.16 K with the largest reduction in the Arctic regions where the shortwave REaci is strong. Associated with the cooling, the Arctic sea ice is increased, which acts to reamplify the Arctic cooling through a positive ice-albedo feedback. The fast response (irrelevant to ΔT) tends to decrease surface latent heat flux into atmosphere in the tropics to balance strong atmospheric fire black carbon absorption, which reduces the precipitation in the tropical land regions (southern Africa and South America). The climate feedback processes (associated with ΔT) lead to a significant surface latent heat flux reduction over global ocean areas, which could explain most (~80%) of the global precipitation reduction. The precipitation significantly decreases in deep tropical regions (5°N) but increases in the Southern Hemisphere tropical ocean, which is associated with the southward shift of the intertropical convergence zone and the weakening of Southern Hemisphere Hadley cell. Such changes could partly compensate the interhemispheric temperature asymmetry induced by boreal forest fire aerosol indirect effects, through intensifying the cross-equator atmospheric heat transport.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1988

X-ray fluorescence surface contaminant analyzer: A feasibility study

The bonding of liner material to the inner metal surfaces of solid rocket booster cases is adversely affected by minute amounts of impurities on the metal surface. Suitable non-destructive methods currently used for detecting these surface contaminants do not provide the means of identifying their elemental composition. The feasibility of using isotopic source excited energy dispersive X-ray fluorescence as a possible technique for elemental analysis of such contaminants is investigated. A survey is made of the elemental compositions of both D-6ac steel, a common construction material for the booster cases, and Conoco HD-2 grease, a common surface contamination. Source and detector choices that maximize signal to noise ratio in a Recessed Source Geometry are made. A Monte Carlo simulation is then made of the optimized device incorporating the latest available X-ray constants at the energy of the chosen source to determine the device's response to a D-6ac steel surface contained with Conoco HD-2 grease.

Eldridge, Hudson B.↗

NASA NTRSDate not supplied

Mineralogy and Spectroscopy of Mount Etna Lava Flows as an Analogue to Venus

Reports of geologically recent volcanism at Venus [1–3] raise the question of whether Venus is actively resurfacing. Observing the venusian surface is difficult due to the planet’s thick, relatively opaque atmosphere, but emission from the surface is detectable via a few atmospheric windows in the near-infrared (NIR) around 1 μm [4]. Spectroscopy of rocks at these wavelengths varies due to its primary composition and the presence of secondary weathering products [2, 5, 6]. If degree of alteration can be tied to the spectroscopic response, then the weathering of the venusian surface can reveal its age and extent of recent volcanism [2, 7]. Mount Etna on Earth is a potential analogue to Venus that can aid our understanding. The composite volcano is currently active and exhibits a progression of dated lava flows with a range of textures (‘a‘¯a versus p¯ahoehoe flows) and degrees of alteration [8]. While not a perfect analogue due to differing weathering environments, Mount Etna represents a natural age progression of altered basaltic rock [8] that can provide a useful comparison to volcanic structures on Venus. Here we will determine if spectroscopy can determine the alteration state of these flows as a proxy for their age. Future missions to Venus such as VERITAS, En- Vision, and DAVINCI will observe the surface in NIR emissivity. Kirchhoff’s Law holds that e = 1−r, where e is the emissivity and r is the reflectance. NIR emissivity can be reliably calculated from reflectance measurements of rocks [9], so laboratory reflectance spectroscopy is useful to rapidly test potential Venus analogue materials.

Gabriel L. Eggers↗

NASA NTRS1988

Experimental simulations of oxidizing conditions and organic decomposition on the surface of Mars

One important scientific objective of a Mars Rover Sample Return mission would be to look for traces of living and extinct life on Mars. An instrument to search for organic carbon may be the simplest instrument that could screen samples which are interesting from a biological point of view. An experimental program is described which would help to understand the nature of the oxidizing soil on Mars and the mechanism responsible for organic degradation on the Martian surface. This is approached by lab simulations of the actual conditions that occur on Mars, particularly the oxidant production by atmospheric photochemistry, and the combined effects of UV light and oxidants in decomposing organic compounds. The results will be used to formulate models of the photochemistry of the atmospheric, the atmosphere-soil interaction, and the diffusion of reactive compounds into the soils. This information will provide insights and constraints on the design of a sampling strategy to search for organic compounds on Mars.

Stoker, C. R.↗

NASA NTRS1992

Application of self-preservation in the diurnal evolution of the surface energy budget to determine daily evaporation

Evaporation from natural land surfaces often exhibits a strong variation during the course of a day, mostly in response to the daily variation of radiative energy input at the surface. This makes it difficult to derive the total daily evaporation, when only one or a few instantaneous estimates of evaporation are available. It is often possible to resolve this difficulty by assuming self-preservation in the diurnal evolution of the surface energy budget. Thus if the relative partition of total incoming energy flux among the different components remains the same, the ratio of latent heat flux and any other flux component can be taken as constant through the day. This concept of constant flux ratios is tested by means of data obtained during the First ISLSCP Field Experiment; the instantaneous evaporation values were calculated by means of the atmospheric boundary layer bulk similarity approach with radiosonde profiles and radiative surface temperatures. Good results were obtained for evaporative flux ratios with available energy flux, with net radiation, and with incoming shortwave radiation.

Brutsaert, Wilfried↗

NASA NTRS2011

Active-Controlled Fluid Film Based on Wave-Bearing Technology

It has been known since 1967 that the steady-state and dynamic performance, including the stability of a wave bearing, are highly dependent on the wave amplitude. A wave-bearing profile can be readily obtained by elastically distorting the stationary bearing sleeve surface. The force that distorts the elastic sleeve surface could be an applied force or pressure. The magnitude and response of the distorting force would be defined by the relation between the bearing surface stiffness and the bearing pressure, or load, in a feedback loop controller. Using such devices as piezoelectric or other electromechanical elements, one could step control or fully control the bearing. The selection between these systems depends on the manner in which the distortion forces are applied, the running speed, and the reaction time of the feedback loop. With these techniques, both liquid- (oil-) or gas- (air-) lubricated wave bearings could be controlled. This report gives some examples of the dependency of the bearing's performance on the wave amplitude. The analysis also was proven experimentally.

Dimofte, Florin↗

NASA NTRS1996

Validation of the ASTER Thermal Infrared Surface Radiance Data Product

The Advanced Spaceborne Thermal Emission and reflection Radiometer (ASTER) is a 14 channel high spatial resolution instrument selected for flight on the EOS AM-1 platform...To provide an objective assessment of the validity of the atmospheric correction, in situ measurements of water surfaces under a variety of atmospheric conditions will be used to estimate the surface leaving radiance at the scale of an ASTER pixel... These measurements and the spectral emissivity of the water will be combined with the relative system spectral response to provide and estimater of thermal infrared surface leaving radiance for each ASTER thermal channel. An example of this approach using a multichannel thermal aircraft scanner as a stand in for ASTER will be described.

ASTER↗

NASA NTRSDate not supplied

Lapse-Rate Feeback: The Key to Reconciling TOA and Surface Attributions of Surface Warming

The impact of climate feedbacks on surface warming is conventionally evaluated using a decomposition of the top-of-atmosphere (TOA) energy budget. Alternatively, the climate feedback analysis can also be carried out using the surface energy budget. However, the two perspectives do not provide the same interpretation of process contributions to surface warming, particularly when executing a spatial analysis. The TOA energy budget is equal to the sum of the surface and atmospheric energy budgets. Using the CMIP5 RCP 8.5 model projections, we show that the major discrepancies between the surface and TOA climate feedback attributions of surface warming are due to non-negligible changes in the atmospheric energy budget that differ from their counterparts at the surface. Individual radiative and non-radiative processes cause vertically non-uniform energy flux perturbations, in response to an external forcing, that naturally lead to a vertically non-uniform temperature change. The TOA lapse-rate feedback is the manifestation of these multiple processes that produce a vertically non-uniform warming response such that it accounts for the asymmetry between the changes in the atmospheric and surface energy budgets. Using the climate feedback-response analysis method, we can decompose the lapse-rate feedback into contributions by individual processes. The negative lapse-rate feedback in the tropics is due to greater moist convection and condensational heating along with ocean heat storage. On the other hand, the positive lapse-rate feedback in polar regions is primarily due to the surface albedo and water vapor feedbacks. Combining the process contributions that are hidden within the lapse-rate feedback with their respective direct impacts on the TOA energy budget allows for a very consistent picture of process contributions to surface warming and its inter-model spread as that given by the surface energy budget approach. With the modified approach, both perspectives indicate water vapor feedback is the largest contributor in the tropics, while surface albedo feedback is the greatest contributor in polar regions. Dynamics and ocean heat storage are the main suppressors of surface warming, except over Antarctica. Both perspectives show there is large inter-model uncertainty in the contributions of water vapor, clouds, albedo, and dynamics plus ocean heat storage.

Sergio A Sejas↗

NASA NTRS1988

Experimental study of thin-walled composite beams

Thin-walled rectangular section composite beams are built out of graphite-epoxy prepreg tape using an autoclave molding technique. Cantilevered beams are tested under static loads using a specially-built apparatus and bending slope and elastic twist at a station are measured using a laser system. Measured bending slope and bending-induced twist distributions are correlated with predicted results obtained using a simple beam analysis as well as a refined finite element analysis. Natural vibration characteristics at different rotational speeds are determined experimentally by testing beams in a specially built 10 ft diameter vacuum chamber. The rotor is excited by piezo-electric crystals and response is determined from strain gages mounted on the surface. For composite beams with bending-twisting couplings (symmetric layup), effects of section warping and transverse shear on structural response are found to be substantial. These results were substantiated by the analyses.

Chandra, Ramesh↗

NASA NTRS2022

Development of an Effective Finite-rate Oxidation Model for NuSil-coated Charred Carbon Preform Ablators

Recently, a detailed effective finite-rate surface chemistry model was developed for the oxidation of FiberForm [1] using the molecular beam experimental data of Poovathingal et al., [2]. FiberForm is the major building block of the thermal protection system (TPS) material Phenolic Impregnated Carbon Ablator (PICA), commonly used by NASA. The surface chemistry model consists of detailed surface reaction mechanisms such as adsorption, desorption, and several types of Langmuir-Hinshelwood (LH) reactions to characterize the oxygen-carbon interactions at the surface. This model provides excellent agreement with the experimental data for oxidation product compositions and corresponding translational energy distributions. Further, an effective oxidation model was constructed that captures the equivalent interaction of oxygen inside the microstructure (including multiple surface collisions) via a modified reactivity for a smooth wall boundary condition. This enables the use of this model directly into Computational Fluid Dynamics (CFD) codes and Material Response (MR) codes to accurately simulate the gas–surface interactions within FiberForm without using the detailed micro-structure. However, this effective model is valid only for the virgin FiberForm. As the TPS material undergoes ablation, the preform carbon burns and turns into char. In addition, PICA is also coated with a protective silicon coating called NuSil for the purpose of mitigating the spread of phenolic dust, and limit contamination during clean room operations. Fig. 1 shows a X-ray microtomography image of a charred NuSil-coated PICA. The NuSil layer introduces species containing silicon into the product mixture. Further, the reactivity of the carbon within the char layer is different from the virgin FiberForm as shown in Fig. 2. Recently a new set of molecular beam experiments were performed on this NuSil-coated TPS material [3] with the same type of oxygen beam used in the previous experiments. Using the latest experimental data, the previously developed effective model will be extended to account for the charred carbon as well as the NuSil coating. Finally, this new effective model with three phases – preform carbon, char, and NuSil; will be compared and validated against the experimental product compositions.

K Swaminathan Gopalan↗

NASA NTRS1973

Some effects of surface anomalies in a global general circulation model.

The Mintz-Arakawa two-level general circulation model has been used in a series of experiments to compute the response of the atmosphere to certain persistent sea-surface temperature anomalies and to changes in the position of the continental Northern Hemisphere snow line over periods up to 90 days. Results are shown in terms of differences between anomaly and control histories are revealed by global, 30-day mean sea-level pressure maps, and time series of three regional indices of synoptic activity. The experiments show significant interhemispheric effects after about 1 month, phase shifts of 1 to 2 weeks in major cyclone developments, stronger reactions to sea-temperature anomalies in winter than in summer, and marked influence of the snow line on the winter monsoonal pressure difference between the continents and the North Atlantic Ocean.

Spar, J.↗

DOE OSTI2019

Enrichment and Distribution of Pb 2+ Ions in Zwitterionic Poly(cysteine methacrylate) Brushes at the Solid–Liquid Interface

Cysteine-based polyzwitterionic brushes have been prepared via a two-step route. First, poly(allyl methacrylate) (PAMA) brushes have been grown from the surface of silicon substrates using surface-initiated atom transfer radical polymerization. The obtained PAMA brushes with free pendant vinyl groups were further modified via radical thiol-ene addition reaction to attach L-cysteine moieties. Surface zeta potential investigations on pH-responsiveness of these poly(cysteine methacrylate) (PCysMA) brushes confirm their zwitterionic character at intermediate pH range, while at pH values either below pH 3.50 or above pH 8.59, they exhibit polyelectrolyte character. Under acid (pH < 3.50) or base (pH > 8.59) conditions, they possess either cationic or anionic character, respectively. In the zwitterionic region, these PCysMA brushes show positive surface $\zeta$ potential in the presence of Pb(CH 3 COO) 2 solutions of various concentrations. The results are in line with microscopic investigations using anomalous X-ray reflectivity (AXRR) carried out along the absorption edge of Pb 2+ ions. When the photon energies were varied around the absorption L3 edge of lead (13037 eV), the Pb 2+ concentration normal to the silicon substrates, as a function of depth inside PCysMA brushes, could be revealed at the nanoscale. Both zeta potential and AXRR measurements confirm the enrichment of Pb 2+ ions inside PCysMA brushes, indicating the potential of PCysMA to be used as a water purification material.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2022

Importance of the Antarctic Slope Current in the Southern Ocean Response to Ice Sheet Melt and Wind Stress Change

Abstract We use two coupled climate models, GFDL‐CM4 and GFDL‐ESM4, to investigate the physical response of the Southern Ocean to changes in surface wind stress, Antarctic meltwater, and the combined forcing of the two in a pre‐industrial control simulation. The meltwater cools the ocean surface in all regions except the Weddell Sea, where the wind stress warms the near‐surface layer. The limited sensitivity of the Weddell Sea surface layer to the meltwater is due to the spatial distribution of the meltwater fluxes, regional bathymetry, and large‐scale circulation patterns. The meltwater forcing dominates the Antarctic shelf response and the models yield strikingly different responses along West Antarctica. The disagreement is attributable to the mean‐state representation and meltwater‐driven acceleration of the Antarctic Slope Current (ASC). In CM4, the meltwater is efficiently trapped on the shelf by a well resolved, strong, and accelerating ASC which isolates the West Antarctic shelf from warm offshore waters, leading to strong subsurface cooling. In ESM4, a weaker and diffuse ASC allows more meltwater to escape to the open ocean, the West Antarctic shelf does not become isolated, and instead strong subsurface warming occurs. The CM4 results suggest a possible negative feedback mechanism that acts to limit future melting, while the ESM4 results suggest a possible positive feedback mechanism that acts to accelerate melt. Our results demonstrate the strong influence the ASC has on governing changes along the shelf, highlighting the importance of coupling interactive ice sheet models to ocean models that can resolve these dynamical processes.

Beadling, R. L.↗

NASA NTRS1985

Front and back polysilicon-contacted silicon solar cells

The first use of a (silicon)/ (heavily doped polysilicon)/ (metal) structure to replace the conventional high-low junction (or back-surface-field, BSF) structure of silicon solar cells is reported. Compared with BSF and back-ohmic-contact control samples, the polysilicon-back solar cells show improvements in red spectral response and open-circuit voltage. Measurement reveals that a decrease in effective surface recombination velocity S is responsible for this improvement. Decreased S results for n-type (Si:As) polysilicon, consistent with past findings for bipolar transistors, and for p-type (Si:B) polysilicon, reported here for the first time. Though the present polysilicon-back solar cells are far from optimal, the results suggest a new class of designs for high efficiency silicon solar cells. Detailed technical reasons are advanced to support this view.

Lindholm, F. A.↗

DOE OSTI2024

Roles of the atmosphere and ocean in the projected north atlantic warming hole

There exists a warming deficit in sea surface temperatures (SST) over the subpolar North Atlantic in response to quadrupled CO 2 , referred to as the projected North Atlantic warming hole (WH). This study employs a partial coupling technique to accurately verify the relative roles of oceanic and atmospheric processes in the formation of the projected WH within an atmosphere-ocean coupled framework. By decomposing the SST anomalies in the subpolar North Atlantic into two components: those induced by atmospheric processes (i.e., the atmosphere-forced component) and those driven by changes in ocean circulation (i.e., the ocean-driven component), we find that the projected WH is primarily driven by changes in ocean circulation, with almost no contribution from atmospheric processes. Specifically, the slowdown of the Atlantic Meridional Overturning Circulation (AMOC) results in a cooling of SST in the WH region due to reduced northward ocean heat transport into this region. This study further quantifies the influence of a positive coupled feedback through surface heat flux (SHF) on the AMOC response under greenhouse gas forcing within this self-consistent framework. It is found that the AMOC slowdown leads to a negative SST anomaly in the subpolar North Atlantic and subsequently a positive ocean-driven SHF anomaly, which in turn further weakens the AMOC. In conclusion, this positive feedback through the SHF contributes about 50% to the total AMOC slowdown in response to quadrupled CO 2 .

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1980

Simulation of charging response of SCATHA (P78-2) satellite

A model of the satellite charging at high altitudes (SCATHA P78-2) satellite was used to simulate the charging response of SCATHA at geosynchronous orbit. The model includes a description of the geometry, currents to exposed surface materials, and electrical connections on the spacecraft. The charging response of the vehicle to that predicted by the NASCAP model for the Day 87, 1979 eclipse charging event, in which the spacecraft charged to several kilovolts negative during a magnetospheric substorm are compared. Double Maxwellian representations of the plasma environment reproduce the charging response observed experimentally.

Schnuelle, G. W.↗