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At least 1,495 records · Page 83

A compact dication source for Ba 2+ tagging and heavy metal ion sensor development

Here, we present a tunable metal ion beam that delivers controllable ion currents in the picoamp range for testing of dry-phase ion sensors. Ion beams are formed by sequential atomic evaporation and single or multiple electron impact ionization, followed by acceleration into a sensing region. Controllability of the ionic charge state is achieved through tuning of electrode potentials that influence the retention time in the ionization region. Barium, lead, and cadmium samples have been used to test the system, with ion currents identified and quantified using a quadrupole mass analyzer. Realization of a clean Ba 2+ ion beam within a bench-top system represents an important technical advance toward the development and characterization of barium tagging systems for neutrinoless double beta decay searches in xenon gas. This system also provides a testbed for investigation of novel ion sensing methodologies for environmental assay applications, with dication beams of Pb 2+ and Cd 2+ also demonstrated for this purpose.

47 OTHER INSTRUMENTATION↗

Properties of a constricted-tube air-flow levitator

The properties of a constricted-tube gas flow levitator first developed by Berge et al. (1981) have been investigated experimentally in order to predict its behavior in a gravity-free environment and at elevated temperatures. The levitator consists of a constricted (quartz) tube fed at one end by a source of heated air or gas. A spherical sample is positioned by the air stream on the downstream side of the constriction, where it can be melted and resolidified without touching the tube. It is shown experimentally that the kinematic viscosity is the important fluid parameter for operation in thermal equilibrium at high temperatures. If air is heated from room temperature to 1200 C, the kinematic viscosity increases by a factor of 14. To maintain a given value of the Reynolds number, the flow rate would have to be increased by the same factor for a specific geometry of tube and sample. Thus, to maintain stable equilibrium, the flow rate should be increased as the air or other gas is heated. The other stability problem discussed is associated with changes in the shape of a cylindrical sample as it melts.

Rush, J. E.↗

Apollo 16 core 60013/14 as a product of path 1 and path 2 regolith evolution processes

We have made a petrographic study of 12 samples along the 62 cm profile of Apollo 16 core 60013/14 taken at Station 10 near the lunar module. The basic core description and maturity variations have been discussed earlier. This core is important because it enables a stratigraphic comparison with nearby cores 60001-7 and 60009/10. These cores form a triangle with sides 35-40 m. FMR data show a maturity-match between 60009/10 and 60013/14. Unfortunately, segments of the core 60001-7 are too disturbed for any cm scale comparison. We present new data on the grain size distribution and the modal petrography for six samples from six levels of 60013 using the same approach and rationale used for 60014. We have combined the new data with our previous data on 60014 to plot the variations of grain size distributions and grain type abundances, in the 500-1000 m and 90-150 micrometers size fractions, with depth. Agglutinate abundances match the I sub s/FeO profile and both show a significant break at a depth of about 45 cm, with lower maturity material below that point. Grain size distributions show that for all analyzed samples, the mean grain size is below 90 micrometers. The two lowest samples are somewhat more coarse-grained than the rest of the core. The break at about 45 cm is the most prominent feature of the core and was described during the initial dissection as a pronounced change in color from dark to light. It now seems clear that this break is primarily one of maturity rather than of bulk chemical composition.

Basu, A.↗

Point-of-use filtration units as drinking water distribution system sentinels

Abstract Municipal drinking water distribution systems (DWDSs) and associated premise plumbing (PP) systems are vulnerable to proliferation of opportunistic pathogens, even when chemical disinfection residuals are present, thus presenting a public health risk. Monitoring the structure of microbial communities of drinking water is challenging because of limited continuous access to faucets, pipes, and storage tanks. We propose a scalable household sampling method, which uses spent activated carbon and reverse osmosis (RO) membrane point-of-use (POU) filters to evaluate mid- to long-term occurrence of microorganisms in PP systems that are relevant to consumer exposure. As a proof of concept, POU filter microbiomes were collected from four different locations and analyzed with 16S rRNA gene amplicon sequencing. The analyses revealed distinct microbial communities, with occasional detection of potential pathogens. The findings highlight the importance of local, and if possible, continuous monitoring within and across distribution systems. The continuous operation of POU filters offers an advantage in capturing species that may be missed by instantaneous sampling methods. We suggest that water utilities, public institutions, and regulatory agencies take advantage of end-of-life POU filters for microbial monitoring. This approach can be easily implemented to ensure drinking water safety, especially from microbes of emerging concerns; e.g., pathogenic Legionella and Mycobacterium species.

42 ENGINEERING↗

Semi-analytical covariance matrices for two-point correlation function for DESI 2024 data

We present an optimized way of producing the fast semi-analytical covariance matrices for the Legendre moments of the two-point correlation function, taking into account survey geometry and mimicking the non-Gaussian effects. We validate the approach on simulated (mock) catalogs for different galaxy types, representative of the Dark Energy Spectroscopic Instrument (DESI) Data Release 1, used in 2024 analyses. We find only a few percent differences between the mock sample covariance matrix and our results, which can be expected given the approximate nature of the mocks, although we do identify discrepancies between the shot-noise properties of the DESI fiber assignment algorithm and the faster approximation (emulator) used in the mocks. Importantly, we find a close agreement (≤ 8% relative differences) in the projected errorbars for distance scale parameters for the baryon acoustic oscillation measurements. This confirms our method as an attractive alternative to simulation-based covariance matrices, especially for non-standard models or galaxy sample selections, making it particularly relevant to the broad current and future analyses of DESI data.

79 ASTRONOMY AND ASTROPHYSICS↗

Machine-to-machine variability of roughness and corrosion in additively manufactured 316L stainless steel

Numerous studies on the corrosion response of metal AM have been conducted. Nonetheless, the specimens being tested are commonly ground or polished to remove the outer as-built surface. If metal AM is truly going to be employed as a transformative technology that can produce complex shapes that do not require traditional machining, then the material needs to be evaluated in the as-built state. The reality is that AM alloys have shown significant inconsistencies regarding as-built surface texture, topology, and residual stress. One metric that has shown significant unpredictability in the literature is the susceptibility to localized corrosion of typically passive alloys, such as stainless steel (SS). There are a large number of studies that have attempted to understand the corrosion response of metal AM materials, but these studies are typically performed on materials that have been printed on a single machine and often mechanically polished to a smooth finish. This study compares the corrosion response of as-built AM, laser-beam powder bed fusion (LB-PBF), 316L SS parts that have been fabricated on five different machines. The majority of this work focused on understanding the susceptibility to localized corrosion of AM metals with respect to machine-dependent variables, namely surface roughness, and build angle. Surface roughness data was collected using scanning white light triangulation, laser scanning confocal microscopy, and coherence scanning interferometry. The results show that there is significant variability (p two-tail < 0.05) in the susceptibility to local corrosion initiation of LB-PBF 316L SS samples built on different machines. Surface oxides were probed with electron dispersive spectroscopy and revealed that variations in local corrosion susceptibility likely arise from differences in the stability of the passive film caused by chemical segregation, unique microstructure, and tortuous roughness features at the as-built surfaces. The variability of roughness and corrosion properties from test samples printed on different machines was corroborated by property measurements performed at five different testing sites, proving reproducibility of the data. Most importantly, this study shows that if the as-built surface layer is removed through grinding or electropolishing the machine-to-machine variation observed in the corrosion susceptibility is reduced.

36 MATERIALS SCIENCE↗

A Benchmark to Test Generalization Capabilities of Deep Learning Methods to Classify Severe Convective Storms in a Changing Climate

Abstract This is a test case study assessing the ability of deep learning methods to generalize to a future climate (end of 21st century) when trained to classify thunderstorms in model output representative of the present‐day climate. A convolutional neural network (CNN) was trained to classify strongly rotating thunderstorms from a current climate created using the Weather Research and Forecasting model at high‐resolution, then evaluated against thunderstorms from a future climate and found to perform with skill and comparatively in both climates. Despite training with labels derived from a threshold value of a severe thunderstorm diagnostic (updraft helicity), which was not used as an input attribute, the CNN learned physical characteristics of organized convection and environments that are not captured by the diagnostic heuristic. Physical features were not prescribed but rather learned from the data, such as the importance of dry air at mid‐levels for intense thunderstorm development when low‐level moisture is present (i.e., convective available potential energy). Explanation techniques also revealed that thunderstorms classified as strongly rotating are associated with learned rotation signatures. Results show that the creation of synthetic data with ground truth is a viable alternative to human‐labeled data and that a CNN is able to generalize a target using learned features that would be difficult to encode due to spatial complexity. Most importantly, results from this study show that deep learning is capable of generalizing to future climate extremes and can exhibit out‐of‐sample robustness with hyperparameter tuning in certain applications.

54 ENVIRONMENTAL SCIENCES↗

A Better Method to Calculate Fuel Burnup in Pebble Bed Reactors Using Machine Learning

Burnup measurement is an important step in material control and accountancy (MC&A) at nuclear reactors, and may be done by examining gamma spectra of fuel samples. Traditional approaches rely on known correlations to specific photopeaks (e.g. 137 Cs) and operate via a standard linear regression method. However, the quality of these regression methods is limited even in the best case, and is significantly poorer at short fuel cool-down times, due to the elevated radiation background by short life-time isotopes, and self-shielding effect of the fuel. For practical operation of pebble bed reactors (PBRs), quick measurements (in minutes) and short cooling times (in hours) are required from a safety and security perspective. We investigated the efficacy and performance of machine learning (ML) methods to predict the burnup of the pebble fuel from full gamma spectra (rather than specific discrete photopeaks) and found a full-spectrum ML approach to far outperform baseline regression predictions in all measurement and cooling conditions - including in operational-like measurement conditions. We also performed model and data ablation experiments to determine the relative performance impact of our ML methods' capacity to model data nonlinearities and the inherent additional information in full spectra. Applying our ML methods, we found a number of surprising results, including improved accuracy at shorter fuel cooling times (the opposite of the norm), remarkable robustness to spectrum compression (via rebinning), and competitive burnup predictions even when using background signal only (i.e. explicitly omitting known isotope photopeaks).

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Interplay between magnetism and superconductivity in UTe 2

Time-reversal symmetry breaking (TRSB) in UTe 2 was inferred from observations of a spontaneous Kerr response in the superconducting state after cooling in zero magnetic field, while a finite c-axis magnetic field training was further used to determine the nature of the nonunitary composite order parameter of this material. Here, we present an extensive study of the magnetic-field-trained Kerr effect, which unveils a unique critical state of pinned “ferromagnetic vortices.” We show that a remanent Kerr signal appears following the removal of a training magnetic field, which reflects the response to the TRSB order parameter and the external magnetic field through the paramagnetic susceptibility. Furthermore, this unambiguously demonstrates the importance of the magnetic fluctuations and their intimate relation to the composite order parameter. Focusing the beam on the center of the sample, we are able to accurately determine the maximum field that is screened by the critical state and the respective critical current. Measurements in the presence of magnetic field show the tendency of the superconductor to produce shielding currents that oppose the increase in vortex-induced magnetization due to the diverging paramagnetic susceptibility.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Optimal Twirling Depth for Classical Shadows in the Presence of Noise

The classical shadows protocol is an efficient strategy for estimating properties of an unknown state p using a small number of state copies and measurements. In its original form, it involves twirling the state with unitaries from some ensemble and measuring the twirled state in a fixed basis. It was recently shown that for computing local properties, optimal sample complexity (copies of the state required) is remarkably achieved for unitaries drawn from shallow depth circuits composed of local entangling gates, as opposed to purely local (zero depth) or global twirling (infinite depth) ensembles. Here, we consider the sample complexity as a function of the depth of the circuit, in the presence of noise. We find that this noise has important implications for determining the optimal twirling ensemble. Under fairly general conditions, we (i) show that any single-site noise can be accounted for using a depolarizing noise channel with an appropriate damping parameter f, (ii) compute thresholds f th at which optimal twirling reduces to local twirling for Pauli operators, (iii) nth order Renyi entropies (n ≥2), and (iv) provide a meaningful upper bound t max on the optimal circuit depth for any finite noise strength f, which applies to observables and entanglement entropy measurements. In conclusion, these thresholds strongly constrain the search for optimal strategies to implement shadow tomography and are easily tailored to the experimental system at hand.

97 MATHEMATICS AND COMPUTING↗

Bottomonium suppression in pNRQCD and open quantum system approach

By employing the potential non-relativistic quantum chromodynamics (pNRQCD) effective field theory within an open quantum system framework, we derive a Lindblad equation governing the evolution of the heavy-quarkonium reduced density matrix, accurate to next-to-leading order (NLO) in the ratio of the state's binding energy to the medium's temperature [1]. The derived NLO Lindblad equation provides a more reliable description of heavy-quarkonium evolution in the quark-gluon plasma at low temperatures compared to the leading-order truncation. For phenomenological applications, we numerically solve this equation using the quantum trajectories algorithm. By averaging over Monte Carlo-sampled quantum jumps, we obtain solutions without truncation in the angular momentum quantum number of the considered states. Our analysis highlights the importance of quantum jumps in the nonequilibrium evolution of bottomonium states within the quark-gluon plasma [2]. Additionally, we demonstrate that the quantum regeneration of singlet states from octet configurations is essential to explain experimental observations of bottomonium suppression. The heavy-quarkonium transport coefficients used in our study align with recent lattice QCD determinations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Skylab experiments on semiconductors and alkali halides

The space processing experiments performed during the Skylab missions included one on single crystal growth of germanium selenide and telluride, one on pure and doped germanium crystals, two on pure and doped indium antimonide, one on gallium-indium-antimony systems, and one on a sodium chloride-sodium fluoride eutectic. In each experiment, three ampoules of sample were processed in the multipurpose electric furnace within the Skylab Materials Processing Facility. All were successful in varying degrees and gave important information about crystal growth removed from the effects of earth surface gravity.

Lundquist, C. A.↗

Spectrophotometry of faint cluster galaxies and the Hubble diagram - An approach to cosmology

New spectrophotometric data are presented for large-redshift galaxies in clusters. A new approach to aperture corrections and the analysis of the Hubble diagram is outlined, including the explicit incorporation of evolutionary effects. The importance of selection effects on the usual methods of analysis are in principle overcome in the analysis, although the heterogeneity of the sample still makes conclusions about cosmology slightly suspect. Formal values of the deceleration parameter are derived under several sets of assumptions, yielding results between +0.33 and -1.27 with formal standard deviations of order 0.7.

Gunn, J. E.↗

Research study on IPS digital controller design

The performance is investigated of the simplified continuous-data model of the Instrument Pointing System (IPS). Although the ultimate objective is to study the digital model of the system, knowledge on the performance of the continuous-data model is important in the sense that the characteristics of the digital system should approach those of the continuous-data system as the sampling period approaches zero.

Kuo, B. C.↗

Shock compression and adiabatic release of a titaniferous mare basalt

A report is presented regarding the dynamic properties of a rock indigenous to the mare basins of the moon. The reported data were obtained in a study of sample 70215, a very titanium-rich basalt (58% pyroxene, 18% ilmenite, 15% plagioclase, 6% olivine, and 3% quartz by weight). This rock is probably representative of a class of the earliest mare-filling extrusive rocks which are exposed on the present lunar surface. Two series of experiments were performed. One set of experiments involved the measuring of Hugoniot and release adiabats to 15.7 GPa with a propellant gun apparatus. In the second set of experiments, a light-gas gun was employed to yield Hugoniot data at about 120 GPa and release states at about 90 GPa. Lunar basalt 70215 appears to be among the densest rocks in the present lunar sample collection, having a crystal density of 3.38 g/cu cm and a porosity of about 1.3%. The results of the experiments have important implications for both the degree of shock metamorphism expected for impact processes and the extent of ejecta transport on mare surfaces with high-titanium basalt composition.

Ahrens, T. J.↗

Improved optics for an ultracentrifuge

Ultracentrifuge is important tool in study of polymers, biomolecules, and cell structures. In typical ultracentrifuge rotor supports pair of optically matched vials; one contains sample mixed in solvent, and other is reference that contains only solvent. Doubleslit optical system, transverse to rotor, creates interference pattern on photographic plate each time vials pass through optics. Medium in sample vial displaces interference maximums such that shift gives measurement of density distribution along length of sample.

Miller, C. G.↗

Luminosity correlations in quasars

Simulations are conducted with and without flux thresholds in an investigation of quasar luminosity correlations by means of a Monte Carlo analysis, for various model distributions of quasars in X-rays and optical luminosity. For the case where the X-ray photons are primary, an anticorrelation between X-ray-to-optical luminosity ratio and optical luminosity arises as a natural consequence which resembles observations. The low optical luminosities of X-ray selected quasars can be understood as a consequence of the same effect, and similar conclusions may hold if the X-ray and optical luminosities are determined independently by a third parameter, although they do not hold if the optical photons are primary. The importance of such considerations is demonstrated through a reanalysis of the published X-ray-to-optical flux ratios for the 3CR sample.

Chanan, G. A.↗

Non-equilibrium freezing of water-ice in sandy basaltic regoliths and implications for fluidized debris flows on Mars

Many geomorphic features on Mars were attributed to Earth-analogous, cold-climate processes involving movement of water or ice lubricated debris. Clearly, knowledge of the behavior of water in regolith materials under Martian conditions is essential to understanding the postulated geomorphic processes. Experiments were performed with sand-sized samples of natural basaltic regoliths in order to further elucidate how water/regolith interactions depend upon grain size and mineralogy. The data reveal important contrasts with data for clay-mineral substrates and suggest that the microphysics of water/mineral interactions might affect Martian geomorphic processes in ways that are not fully appreciated. Sand and silt sized fractions of two soils from the summit of Mauna Kea were used as Mars-analogous regolith materials. Temperatures were measured for water/ice phase transitions as wet slurries of individual soil fractions which were cooled or heated at controlled rates under a carbon dioxide atmosphere. Freezing and melting of ice was studied as a function of water/soil mass ratio, soil particle size, and thermal-cycle rate. Comparison tests were done under the same conditions with U.S. Geological Survey standard rock powders.

Gooding, J. L.↗