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At least 1,495 records · Page 83
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DOE OSTI2025

Southern Ocean Aerosols Field Campaign Report

Atmospheric processes over the Southern Ocean have a profound influence on regional and global climate. This is a part of the world where global climate models perform particularly poorly, with models persistently overpredicting the amount of sunlight reaching the Earth's surface (Regayre et al. 2020). A major challenge when trying to improve the representation of atmospheric processes in this part of the globe is the scarcity of observations capable of constraining our understanding. During 2024/25 a U.S. Department of Energy Atmospheric Radiation Measurement (ARM) User Facility field campaign (CAPE-k) deployed a suite of instrumentation at the kennaook/Cape Grim atmospheric monitoring station in Tasmania, Australia to provide detailed cloud-aerosol observations in this region in order to address the greatest source of uncertainty in climate models – atmospheric aerosols and how they influence cloud formation (Carslaw et al. 2013). In support of the ARM observations, an Australian Research Council (ARC)-funded project “Southern Ocean aerosols: sources, sinks and impact on cloud properties,” led by the Queensland University of Technology, complemented the ARM measurements with a suite of chemical measurements at the kennaook/Cape Grim site in northwestern Tasmania to provide more information on the processes controlling aerosol formation and growth. The deployment of the University of York LIF-SO2 instrument (Temple et al. 2025) in the ARM mobile facility container was part of this chemistry-focused deployment. Increased observational efforts are critical for understanding sources and sinks of Southern Ocean aerosols, in particular the role of marine micro-organisms (phytoplankton, algae) on aerosols formation, their properties and growth, cloud droplet formation, and the conversion of cloud droplets to ice crystals and precipitation. The observational focus of the ARC-funded project is aerosol chemical composition and their gaseous precursors. The remote nature of the Southern Ocean poses a significant analytical challenge when studying gaseous precursors, as low concentrations are often below the limits of detection of commercial instrumentation. Historically this has meant that observations have had to be time-averaged over days to weeks to achieve the limits of detection required. Although useful when considering overall average levels of aerosol precursors, this time-averaging obscures temporal variability that can provide insight into the controlling processes. Over recent years advances in analytical techniques have made high-time-resolution measurements of key gas-phase aerosol precursors achievable with sufficiently low limits of detection.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Deciphering Atmospheric Ice Nucleation using Molecular-Scale Microscopy

Atmospheric ice affects Earth's radiative properties and initiates most precipitation. Growing ice typically requires a particle, often airborne mineral dust, e.g., to catalyze freezing of supercooled cloud droplets. How chemistry, structure and morphology determine the ice-nucleating ability of minerals remains elusive. Not surprisingly, poor understanding of a erosol-cloud interactions is a major source of uncertainty in climate models. In this project, we combine d optical microscopy with atomic force microscopy to explore the mechanisms of initial ice formation on alkali feldspar, a mineral proposed to dominate ice nucleation in Earth's atmosphere. When cold air becomes supersaturated with respect to water, we discovered that supercooled liquid water condenses at steps without having to overcome a nucleation barrier, and subsequently freezes quickly. Our results imply that steps, common even on macroscopically flat feldspar surfaces, can accelerate water condensation followed by freezing, thus promoting glaciation and dehydration of mixed - phase clouds. Motivated by the fact that current climate simulations do not properly account for feldspar's extreme efficiency to nucleate ice, we modified DOE's climate model, the Energy Exascale Earth System Model (E3SM), to increase the activation of ice nucleation on feldspar dust. This included adding a new aerosol tracer into the model and updating the ice nucleation parameterization, based on Classical Nucleation Theory, for multiple mineral dust tracers. Although t he se modifications have little impact on global averages , predictions of regional averages can be strongly affected .

Thurmer, Konrad↗
DOE OSTI2024

Soil Moisture‐Cloud‐Precipitation Feedback in the Lower Atmosphere From Functional Decomposition of Satellite Observations

Abstract The feedback of topsoil moisture (SM) content on convective clouds and precipitation is not well understood and represented in the current generation of weather and climate models. Here, we use functional decomposition of satellite‐derived SM and cloud vertical profiles (CVP) to quantify the relationship between SM and the vertical distribution of cloud water in the central US. High‐dimensional model representation is used to disentangle the contributions of SM and other land‐surface and atmospheric variables to the CVP. Results show that the sign and strength of the SM‐cloud‐precipitation feedback varies with cloud height and time lag and displays a large spatial variability. Positive anomalies in antecedent 7‐hr SM and land‐surface temperature enhance cloud reflectivity up to 4 dBZ in the lower atmosphere about 1–3 km above the surface. Our approach presents new insights into the SM‐cloud‐precipitation feedback and aids in the diagnosis of land‐atmosphere interactions simulated by weather and climate models.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Accounting for adaptation and intensity in projecting heat wave-related mortality

Highlights: • We propose novel models for intensity of and adaptation to heat waves in projections of heat wave- mortality. • The modeling used a large national dataset and the projections used a rich set of climate models and scenarios. • Future heat wave-related mortality would be substantially overestimated, if adaptation were ignored. • The time trend of future heat wave-related mortality will vary substantially across climate regions. How adaptation and intensity of heat waves affect heat wave-related mortality is unclear, making health projections difficult.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2010

Trend Analysis and Detection of Changes in the Stratospheric Circulation

Increases in the circulation of the stratosphere appear to be a robust result of climate change in chemistry-climate models over decadal time scales. To date observations have yet to show a significant change in this circulation. It is important for the design of future observational missions to identify suitable atmospheric constituents and to determine the accuracy and length of record needed to identify a significant trend that can be attributed to circulation change. First, we determine what atmospheric variables can be used as proxies for stratospheric circulation changes. A few examples are changes in tropical lower stratospheric ozone, phase lag of the water vapor tape recorder, CO2, and SF6. Then, using both the Goddard Earth Observing System Chemistry-Climate Model (GEOS CCM) and observations from satellites and balloon soundings, we calculate the number of years needed to detect a significant trend, taking into account observational uncertainty. Model simulations will be evaluated to see how well they represent observed variability. In addition, the impacts of autocorrelation among the output or data and gaps in the observational record will be discussed.

Oman, Luke↗
DOE OSTI2018

Attribution of Anthropogenic Influence on Atmospheric Patterns Conducive to Recent Most Severe Haze Over Eastern China

Severe haze pollution in eastern China has caused substantial health impacts and economic loss. Conducive atmospheric conditions are important to affect occurrence of severe haze events, and circulation changes induced by future global climate warming are projected to increase the frequency of such events. However, a potential contribution of an anthropogenic influence to recent most severe haze (December 2015 and January 2013) over eastern China remains unclear. Here we show that the anthropogenic influence, which is estimated by using large ensemble runs with a climate model forced with and without anthropogenic forcings, has already increased the probability of the atmospheric patterns conducive to severe haze by at least 45% in January 2013 and 27% in December 2015, respectively. We further confirm that simulated atmospheric circulation pattern changes induced by anthropogenic influence are driven mainly by increased greenhouse gas emissions. Our results suggest that more strict reductions in pollutant emissions are needed under future anthropogenic warming.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1991

Is CO2 capable to keeping early Mars warm?

One of the goals of NASA's Exobiology Research Program is to determine whether life exists today on Mars (unlikely) or whether it might have existed there at some time in the past (more likely). Speculation about extinct life is driven by the observation of channels on the Martian surface, thought to indicate the past presence of liquid water and, hence, the existence of a warmer climate. Current thinking suggests that such a climate could have been maintained if early Mars had a dense CO2 atmosphere with a surface pressure of 1 to 5 bars. One of the phenomena that Martian climate modelers have not looked at very carefully is the process of CO2 condensation. Reexamination of some of my own calculations indicates that condensation should occur at high altitudes in some high-CO2, Martian atmospheres, particularly those in which the solar constant is set to its initial main sequence value (about 70 percent of present. CO2 condensation should affect the surface temperature in two ways: (1) if it occurs in the convective lower atmosphere, condensation will reduce the magnitude of the greenhouse effect by decreasing the lapse rate; and (2) condensation at any altitude will produce clouds, which can either warm or cool the climate depending on their altitude and optical depth. Preliminary calculations with a 1-D, radiative-convective climate model indicate that the lapse rate change is substantial for low solar luminosity models. Other aspects of this study are discussed.

Kasting, J. F.↗
DOE OSTI2016

Fate of the Atlantic Meridional Overturning Circulation: Strong decline under continued warming and Greenland melting

The most recent Intergovernmental Panel on Climate Change assessment report concludes thatthe Atlantic Meridional Overturning Circulation (AMOC) could weaken substantially but is very unlikely tocollapse in the 21st century. However, the assessment largely neglected Greenland Ice Sheet (GrIS)mass loss, lacked a comprehensive uncertainty analysis, and was limited to the 21st century. Here in acommunity effort, improved estimates of GrIS mass loss are included in multicentennial projections usingeight state-of-the-science climate models, and an AMOC emulator is used to provide a probabilisticuncertainty assessment. We find that GrIS melting affects AMOC projections, even though it is of secondaryimportance. By years 2090–2100, the AMOC weakens by 18% [3%, 34%; 90% probability] in an intermediategreenhouse-gas mitigation scenario and by 37% [15%, 65%] under continued high emissions. Afterward, itstabilizes in the former but continues to decline in the latter to 74% [+4%, 100%] by 2290–2300, with a 44%likelihood of an AMOC collapse. This result suggests that an AMOC collapse can be avoided by CO2mitigation.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2018

Projecting future climate change impacts on heat-related mortality in large urban areas in China

Highlights: • The study projects future heat-related mortality risk in 51 major cities in China. • The projections are based on high resolution climate and population projections. • Future heat mortality risk is likely to be considerable under all emission scenarios. • Climate mitigation and heat risk management are needed to reduce such risk. Global climate change is anticipated to raise overall temperatures and has the potential to increase future mortality attributable to heat. Urban areas are particularly vulnerable to heat because of high concentrations of susceptible people. As the world's largest developing country, China has experienced noticeable changes in climate, partially evidenced by frequent occurrence of extreme heat in urban areas, which could expose millions of residents to summer heat stress that may result in increased health risk, including mortality. While there is a growing literature on future impacts of extreme temperatures on public health, projecting changes in future health outcomes associated with climate warming remains challenging and underexplored, particularly in developing countries. This is an exploratory study aimed at projecting future heat-related mortality risk in major urban areas in China. We focus on the 51 largest Chinese cities that include about one third of the total population in China, and project the potential changes in heat-related mortality based on 19 different global-scale climate models and three Representative Concentration Pathways (RCPs). City-specific risk estimates for high temperature and all-cause mortality were used to estimate annual heat-related mortality over two future twenty-year time periods. We estimated that for the 20-year period in Mid-21st century (2041–2060) relative to 1970–2000, incidence of excess heat-related mortality in the 51 cities to be approximately 37,800 (95% CI: 31,300–43,500), 31,700 (95% CI: 26,200–36,600) and 25,800 (95% CI: 21,300–29,800) deaths per year under RCP8.5, RCP4.5 and RCP2.6, respectively. Slowing climate change through the most stringent emission control scenario RCP2.6, relative to RCP8.5, was estimated to avoid 12,900 (95% CI: 10,800–14,800) deaths per year in the 51 cities in the 2050s, and 35,100 (95% CI: 29,200–40,100) deaths per year in the 2070s. The highest mortality risk is primarily in cities located in the North, East and Central regions of China. Population adaptation to heat is likely to reduce excess heat mortality, but the extent of adaptation is still unclear. Future heat mortality risk attributable to exposure to elevated warm season temperature is likely to be considerable in China's urban centers, with substantial geographic variations. Climate mitigation and heat risk management are needed to reduce such risk and produce substantial public health benefits.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2020

Clouds Damp the Impacts of Polar Sea Ice Loss

The amount of solar energy absorbed by the Earth is believed to strongly depend on clouds, due to their ability to scatter and reflect part of solar energy back to space. Here, we investigate this relationship using satellite data and 32 climate models, showing that this relationship holds everywhere except over polar seas, where an increased reflection by clouds corresponds to an increase in absorbed solar radiation at the surface. We resolve this paradox by quantifying a strong correlation between clouds and sea-ice extent. An increase in absorbed solar radiation, when sea ice retreats, leads to an increase in cloud cover/thickness and associated reflection to space. This interplay between clouds and sea ice reduces by half the increase of net radiation at the surface that follows the sea-ice retreat, therefore damping the impact of polar sea ice loss. We further highlight how this process is mis-represented in some climate models.

Ramdane Alkama↗
NASA NTRS2000

Earth Rotation and Coupling to Changes in Atmospheric Angular Momentum

The research supported under the contract dealt primarily with: (a) the mechanisms responsible for the exchange of angular momentum between the solid Earth and atmosphere; (b) the quality of the data sets used to estimate atmospheric angular momentum; and (c) the ability of these data and of global climate models to detect low-frequency signals in the momentum and, hence, circulation of the atmosphere. Three scientific papers reporting on the results of this research were produced during the course of the contract. These papers identified the particular torques responsible for the peak in atmospheric angular momentum and length-of-day during the 1982-93 El Nino event, and, more generally, the relative roles of torques over land and ocean in explaining the broad spectrum of variability in the length-of-day. In addition, a tendency for interannual variability in atmospheric angular momentum to increase during the last several decades of the 20th century was found in both observations and a global climate model experiment.

Rosen, Richard D.↗
DOE OSTI2023

An Ensemble of Neural Networks for Moist Physics Processes, Its Generalizability and Stable Integration

Abstract With the recent advances in data science, machine learning has been increasingly applied to convection and cloud parameterizations in global climate models (GCMs). This study extends the work of Han et al. (2020, https://doi.org/10.1029/2020MS002076 ) and uses an ensemble of 32‐layer deep convolutional residual neural networks, referred to as ResCu‐en, to emulate convection and cloud processes simulated by a superparameterized GCM, SPCAM. ResCu‐en predicts GCM grid‐scale temperature and moisture tendencies, and cloud liquid and ice water contents from moist physics processes. The surface rainfall is derived from the column‐integrated moisture tendency. The prediction uncertainty inherent in deep learning algorithms in emulating the moist physics is reduced by ensemble averaging. Results in 1‐year independent offline validation show that ResCu‐en has high prediction accuracy for all output variables, both in the current climate and in a warmer climate with +4K sea surface temperature. The analysis of different neural net configurations shows that the success to generalize in a warmer climate is attributed to convective memory and the 1‐dimensional convolution layers incorporated into ResCu‐en. We further implement a member of ResCu‐en into CAM5 with real world geography and run the neural‐network‐enabled CAM5 (NCAM) for 5 years without encountering any numerical integration instability. The simulation generally captures the global distribution of the mean precipitation, with a better simulation of precipitation intensity and diurnal cycle. However, there are large biases in temperature and moisture in high latitudes. These results highlight the importance of convective memory and demonstrate the potential for machine learning to enhance climate modeling.

Meteorology & Atmospheric Sciences↗
NASA NTRS2019

Water Vapour Adjustments and Responses Differ Between Climate Drivers

Water vapour in the atmosphere is the source of a major climate feedback mechanism and potential increases in the availability of water vapour could have important consequences for mean and extreme precipitation. Future precipitation changes further depend on how the hydrological cycle responds to different drivers of climate change, such as greenhouse gases and aerosols. Currently, neither the total anthropogenic influence on the hydrological cycle nor that from individual drivers is constrained sufficiently to make solid projections. We investigate how integrated water vapour (IWV) responds to different drivers of climate change. Results from 11 global climate models have been used, based on simulations where CO2, methane, solar irradiance, black carbon (BC), and sulfate have been perturbed separately. While the global-mean IWV is usually assumed to increase by 7% per kelvin of surface temperature change, we find that the feedback response of IWV differs somewhat between drivers. Fast responses, which include the initial radiative effect and rapid adjustments to an external forcing, amplify these differences. The resulting net changes in IWV range from 6.4±0.9%K(exp -1) for sulfate to 9.8±2%K(exp -1) for BC. We further calculate the relationship between global changes in IWV and precipitation, which can be characterized by quantifying changes in atmospheric water vapour lifetime. Global climate models simulate a substantial increase in the lifetime, from 8.2±0.5 to 9.9±0.7d between 1986-2005 and 2081-2100 under a high-emission scenario, and we discuss to what extent the water vapour lifetime provides additional information compared to analysis of IWV and precipitation separately. We conclude that water vapour lifetime changes are an important indicator of changes in precipitation patterns and that BC is particularly efficient in prolonging the mean time, and therefore likely the distance, between evaporation and precipitation.

Hodnebrog, Øivind↗
DOE OSTI2019

Cloud, Aerosol and Boundary Layer Structure across the Northeast Pacific Stratocumulus-Cumulus Transition as observed during CSET

During the Cloud System Evolution in the Trades (CSET) field study, 14 research flights of the National Science Foundation G-V sampled the stratocumulus-cumulus transition between Northern California and Hawaii and its synoptic variability. The G-V made vertically resolved measurements of turbulence, cloud microphysics, aerosol characteristics, and trace gases. It also carried dropsondes and a vertically pointing W-band radar and lidar. This paper summarizes these observations with the goals of fostering novel comparisons with theory, models and reanalyses, and satellite-derived products. A longitude-height binning and compositing strategy mitigates limitations of sparse sampling and spatiotemporal variability. Typically, a 1-km-deep decoupled stratocumulus-capped boundary layer near California evolved into 2-km-deep precipitating cumulus clusters surrounded by patches of thin stratus that dissipated toward Hawaii. Low cloud cover was correlated with estimated inversion strength more than with cloud droplet number, even though the thickest clouds were generally precipitating and ultraclean layers indicative of aerosol-cloud-precipitation interaction were common west of 140 degrees W. Accumulation-mode aerosol concentration correlated well with collocated cloud droplet number concentration and was typically largest near the surface. Aitken mode aerosol concentration was typically larger in the free troposphere. Wildfire smoke produced spikes of aerosol and trace gases on some flights. CSET data are compared with space-time collocated output from MERRA-2 reanalysis and from the CAM6 climate model run with winds and temperature nudged toward this reanalysis. The reanalysis compares better with the observed relative humidity than does nudged CAM6. Both vertically diffuse the stratocumulus cloud layer versus observations. MERRA-2 slightly underestimates in situ carbon monoxide measurements and underestimates ozone depletion within the boundary layer.

Bretherton, Christopher S.↗
NASA NTRS2011

The Response of Tropical Tropospheric Ozone to ENSO

We have successfully reproduced the Ozone ENSO Index (OEI) in the Goddard Earth Observing System (GEOS) chemistry-climate model (CCM) forced by observed sea surface temperatures over a 25-year period. The vertical ozone response to ENSO is consistent with changes in the Walker circulation. We derive the sensitivity of simulated ozone to ENSO variations using linear regression analysis. The western Pacific and Indian Ocean region shows similar positive ozone sensitivities from the surface to the upper troposphere, in response to positive anomalies in the Nino 3.4 Index. The eastern and central Pacific region shows negative sensitivities with the largest sensitivity in the upper troposphere. This vertical response compares well with that derived from SHADOZ ozonesondes in each region. The OEI reveals a response of tropospheric ozone to circulation change that is nearly independent of changes in emissions and thus it is potentially useful in chemistry-climate model evaluation.

Oman, L. D.↗
NASA NTRS2021

3D Simulations of the Early Martian Hydrological Cycle Mediated by a H2-CO2 Greenhouse

For decades, the scientific community has been trying to reconcile abundant evidence for fluvialactivity on Noachian and early Hesperian Mars with the faint young Sun and reasonableconstraints on ancient atmospheric pressure and composition. Recently, the investigation of H2-CO2 collision-induced absorption has opened up a new avenue to warm Noachian Mars. We usethe ROCKE-3D global climate model to simulate plausible states of the ancient Martian climatewith this absorptive warming and reasonable constraints on surface paleopressure. We find that1.5-2 bar CO2-dominated atmospheres with ≥3% H2 can produce global mean surfacetemperatures above freezing, while also providing sufficient warming to avoid surfaceatmospheric CO2 condensation at 0°-45° obliquity. Simulations conducted with both moderntopography and a paleotopography, before Tharsis formed, highlight the importance of Tharsis asa cold trap for water on the planet. Additionally, we find that low obliquity (modern and 0°) ismore conducive to rainfall over valley network locations than high (45°) obliquity. PLAIN LANGUAGE SUMMARY Much evidence tells us that ancient Mars had liquid water on its surface. But reconciling thatwith the fainter young Sun and reasonable constraints on Mars' early atmosphere is challenging.We use a 3D global climate model with an atmosphere containing some amount of hydrogen (apossible greenhouse gas) to study Mars' early hydrological cycle and compare it to the geologicalevidence of surface liquid water billions of years ago. We find that hydrogen and carbon dioxidetogether in an atmosphere twice as thick as modern Earth can warm early Mars above thefreezing point of water and that a low axial tilt produces rainfall patterns that best match thegeologic evidence

Scott D Guzewich↗
DOE OSTI2018

Local radiative feedbacks over the Arctic based on observed short-term climate variations

We compare various radiative feedbacks in response to short-term climate variations estimated from reanalysis, satellite, and global climate model datasets using the combined Kernel-Gregory approach over the Arctic (60-90°N). Except for the shortwave cloud feedback, all feedbacks are positive over the Arctic. Lapse rate feedback is comparable with surface albedo feedback. Relative to the tropics (30°S-30°N), the temperature feedback (lapse rate feedback plus Planck feedback deviation from its global mean) is the largest contributor to Arctic amplification among all feedbacks, followed by surface albedo feedback. The choice of meteorological fields has a small impact on the cloud feedback estimate, but different top-of-the-atmosphere clear-sky fluxes datasets can result in a wide spread of estimated cloud feedbacks. The net cloud feedback over the Arctic is positive due to a larger positive in longwave than the negative shortwave feedback, but has the largest uncertainty. Relative to the tropics, the longwave cloud feedback largely contributes to the Arctic amplification.

Zhang, Rudong↗
DOE OSTI2019

Return period of extreme rainfall substantially decreases under 1.5 °C and 2.0 °C warming: a case study for Uttarakhand, India

In June 2013, Uttarakhand experienced a hydro-meteorological disaster due to a 4 d extreme precipitation event of return period more than 100 years, claiming thousands of lives and causing enormous damage to infrastructure. Using the weather@home climate modelling system and its Half a degree Additional warming, Prognosis and Projected Impacts simulations, this study investigates the change in the return period of similar events in a 1.5 °C and 2 °C warmer world, compared to current and pre-industrial levels. We find that the likelihood of such extreme precipitation events will significantly increase under both future scenarios. We also estimate the change in extreme river flow at the Ganges; finding a considerable increase in the risk of flood events. Our results also suggest that until now, anthropogenic aerosols may have effectively counterbalanced the otherwise increased meteorological flood risk due to greenhouse gas (GHG) induced warming. Disentangling the response due to GHGs and aerosols is required to analyses the changes in future rainfall in the South Asia monsoon region. More research with other climate models is also necessary to make sure these results are robust.

54 ENVIRONMENTAL SCIENCES↗