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DOE OSTI2017

Ab initio calculation of the potential bubble nucleus Si 34

Background: The possibility that an unconventional depletion (referred to as a “bubble”) happens in the middle of the charge density distribution of certain nuclei due to a purely quantum mechanical effect has attracted theoretical and experimental attention in recent years. Based on a mean-field rationale, a correlation between the occurrence of such a semibubble and an anomalously weak splitting between low angular-momentum spin-orbit partners has been further conjectured. Energy density functional and valence-space shell model calculations have been performed to identify and characterize the best candidates, among which Si 34 appears as a particularly interesting case. While the experimental determination of the charge density distribution of the unstable Si 34 is currently out of reach, ($d, p$) experiments on this nucleus have been performed recently to test the correlation between the presence of a bubble and an anomalously weak 1/2 – –3/2 – splitting in the spectrum of Si 35 as compared to S 37 . Purpose: We study the potential bubble structure of Si 34 on the basis of the state-of-the-art ab initio self-consistent Green's function many-body method. Methods: We perform the first ab initio calculations of Si 34 and S 36 . In addition to binding energies, the first observables of interest are the charge density distribution and the charge root-mean-square radius for which experimental data exist in S 36 . The next observable of interest is the low-lying spectroscopy of Si 35 and S 37 obtained from ($d, p$) experiments along with the spectroscopy of Al 33 and P 35 obtained from knock-out experiments. The interpretation in terms of the evolution of the underlying shell structure is also provided. The study is repeated using several chiral effective field theory Hamiltonians as a way to test the robustness of the results with respect to input internucleon interactions. The convergence of the results with respect to the truncation of the many-body expansion, i.e., with respect to the many-body correlations included in the calculation, is studied in detail. We eventually compare our predictions to state-of-the-art multireference energy density functional and shell model calculations. Results: The prediction regarding the (non)existence of the bubble structure in Si 34 varies significantly with the nuclear Hamiltonian used. Yet, demanding that the experimental charge density distribution and the root-mean-square radius of S 36 be well reproduced, along with Si 34 and S 36 binding energies, only leaves the NNLO sat Hamiltonian as a serious candidate to perform this prediction. In this context, a bubble structure, whose fingerprint should be visible in an electron scattering experiment of Si 34 , is predicted. Furthermore, a clear correlation is established between the occurrence of the bubble structure and the weakening of the 1/2 – –3/2 – splitting in the spectrum of Si 35 as compared to S 37 . Conclusions: The occurrence of a bubble structure in the charge distribution of Si 34 is convincingly established on the basis of state-of-the-art ab initio calculations. This prediction will have to be reexamined in the future when improved chiral nuclear Hamiltonians are constructed. On the experimental side, present results act as a strong motivation to measure the charge density distribution of Si 34 in future electron scattering experiments on unstable nuclei. In the meantime, it is of interest to perform one-neutron removal on Si 34 and S 36 in order to further test our theoretical spectral strength distributions over a wide energy range.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2024

Kleinian black holes

We prove there is a unique vacuum solution in split-signature spacetimes with Kleinian S O ( 2 , 1 ) spherical symmetry. We extend our analysis to accommodate a positive or negative cosmological constant and we prove the Kleinian spherically symmetric solutions to Einstein’s equation are locally isomorphic to the split-signature analogs of Schwarzschild–(anti)-de Sitter or Nariai spacetimes. Our analysis provides a Kleinian extension of Birkhoff’s theorem to metrics with split signature. Axisymmetric vacuum solutions are also considered, including (2,2) signature formulations of the Kerr and Taub-Newman-Unti-Tamburino metrics. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Photon topology

The topology of photons in vacuum is interesting because there are no photons with k = 0, creating a hole in momentum space. We show that while the set of all photons forms a trivial vector bundle $γ$ over this momentum space, the R and L photons form topologically nontrivial subbundles $γ±$ with first Chern numbers ∓2. In contrast, $γ$ has no linearly polarized subbundles, and there is no Chern number associated with linear polarizations. It is a known difficulty that the standard version of Wigner’s little group method produces singular representations of the Poincaré group for massless particles. By considering representations of the Poincaré group on vector bundles we obtain a version of Wigner’s little group method for massless particles which avoids these singularities. Here we show that any massless bundle representation of the Poincaré group can be canonically decomposed into irreducible bundle representations labeled by helicity, which in turn can be associated to smooth irreducible Hilbert space representations. This proves that the R and L photons are globally well defined as particles and that the photon wave function can be uniquely split into R and L components. This formalism offers a method of quantizing the electromagnetic field without invoking discontinuous polarization vectors as in the traditional scheme. We also demonstrate that the spin-Chern number of photons is not a purely topological quantity. Lastly, there has been an extended debate on whether photon angular momentum can be split into spin and orbital parts. Our work explains the precise issues that prevent this splitting. Photons do not admit a spin operator; instead, the angular momentum associated with photons’ internal degree of freedom is described by a helicity-induced subalgebra corresponding to the translational symmetry of $γ$.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2016

Automated Parton-Shower Variations in Pythia 8

In the era of precision physics measurements at the LHC, efficient and exhaustive estimations of theoretical uncertainties play an increasingly crucial role. In the context of Monte Carlo (MC) event generators, the estimation of such uncertainties traditionally requires independent MC runs for each variation, for a linear increase in total run time. In this work, we report on an automated evaluation of the dominant (renormalization-scale and nonsingular) perturbative uncertainties in the pythia 8 event generator, with only a modest computational overhead. Each generated event is accompanied by a vector of alternative weights (one for each uncertainty variation), with each set separately preserving the total cross section. Explicit scale-compensating terms can be included, reflecting known coefficients of higher-order splitting terms and reducing the effect of the variations. The formalism also allows for the enhancement of rare partonic splittings, such as g→bb¯ and q→qγ, to obtain weighted samples enriched in these splittings while preserving the correct physical Sudakov factors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2023

Measurement of Suppression of Large-Radius Jets and Its Dependence on Substructure in Pb+Pb Collisions at $\sqrt{s_{NN}}$ = 5.02 TeV with the ATLAS Detector

This letter presents a measurement of the nuclear modification factor of large-radius jets in $\sqrt{s_{NN}}$ = 5.02 TeV Pb + Pb collisions by the ATLAS experiment. The measurement is performed using 1.72 nb –1 and 257 pb –1 of Pb + Pb and pp data, respectively. The large-radius jets are reconstructed with the anti-k t algorithm using a radius parameter of R = 1.0, by reclustering anti-k t R = 0.2 jets, and are measured over the transverse momentum (p T ) kinematic range of 158 < p T <1000 GeV and absolute pseudorapidity |y| < 2.0. The large-radius jet constituents are further reclustered using the k t algorithm in order to obtain the splitting parameters, $\sqrt{d_{12}}$ and Δ⁢R 12 , which characterize the transverse momentum scale and angular separation for the hardest splitting in the jet, respectively. The nuclear modification factor, R AA , obtained by comparing the Pb + Pb jet yields to those in pp collisions, is measured as a function of jet transverse momentum (p T ) and $\sqrt{d_{12}}$ or Δ⁢R 12 . A significant difference in the quenching of large-radius jets having single subjet and those with more complex substructure is observed. Systematic comparison of jet suppression in terms of R AA for different jet definitions is also provided. Presented results support the hypothesis that jets with hard internal splittings lose more energy through quenching and provide a new perspective for understanding the role of jet structure in jet suppression.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

Asymmetric equilibrium core structures of pyramidal-II < c + a > dislocations in ten hexagonal-close-packed metals

The structures of pyramidal-II < c + a > dislocations, one of the most important defects in structural hexagonal-close-packed (HCP) metals, have not been fully characterized for many of the HCP metals in use today. Here, we employ ab initio informed phase-field dislocation dynamics to determine the minimum energy structure of pyramidal {1¯1¯22} < 11¯23 > dislocations in ten HCP metals, including Be, Co, Mg, Re, Ti, Zn, Cd, Hf, Y, and Zr. As input for the simulations, we calculate, using first-principles density functional theory, the {1¯1¯22} generalized stacking fault energy (GSFE) curves for all ten metals. From these calculations, it is found that magnetism in Co is necessary for achieving a local minimum in the GSFE curve. We observe in simulations that edge and screw character dislocations split into two partials separated by a low-energy intrinsic stacking fault. The splitting distance is shown to scale inversely with the local minimum energy normalized by the product of its shear modulus and Burgers vector. Interestingly, some HCP metals exhibit an asymmetric structure, with either unequal partial Burgers vectors or widths, in contrast to the symmetric configuration expected from linear elastic dislocation theory. We explain these structures by properties of the local maxima in their GSFE curves. Metals with larger degrees of elastic anisotropy result in dislocations with larger splitting distances than would be expected under the commonly used assumption of elastic isotropy. Furthermore, these findings on the sizes and asymmetry in the structures of pyramidal-II < c + a > dislocations are fundamental to understanding how these dislocations glide and interact or react with other defects when these metals are mechanically strained.

36 MATERIALS SCIENCE↗

DOE OSTI2025

Quasiaperiodic grain boundary phases of Σ⁢5 tilt grain boundaries in refractory metals

We report ground-state structures and phase transitions in Σ⁢5⁢[001] tilt grain boundaries (GBs) in body-centered-cubic (bcc) refractory metals Nb, Ta, Mo, and W. Σ⁢5 tilt GBs have been extensively investigated over the past several decades, with their ground-state structure—composed of kite-shaped structural units—previously thought to be well understood. By performing a rigorous GB structure search that optimizes the number of atoms in the boundary core, we predict different quasiaperiodic “split kite” phases analogous to those previously found in GBs in face-centered-cubic metals. Furthermore, our results suggest that complex aperiodic phases of GBs appear to be a general phenomenon, as validated through density functional theory calculations. Moreover, the atoms in the split kite phase demonstrate distinct collective diffusion dynamics. Phase-contrast image simulations of split kites show better agreement with experimental observations, offering an alternative explanation for previous microscopy results and motivating future atomically resolved imaging of the GB structure.

Body-centered cubic↗

DOE OSTI2026

Extreme confinement of hydrogen gas within fullerenelike nanoporous carbon

Nanoporous carbons and carbon nanostructures can store hydrogen at cryogenic temperatures but lack the volumetric and gravimetric capacity to be industrially significant. Recent inelastic neutron scattering experiments suggest a highly dense phase of hydrogen at temperatures well above the melting point of solid hydrogen. However, it remains unclear how pore geometry and intermolecular interactions enable these dense phases to exist, with dispersion (van der Waals) or electrostatic/induction suggested to be the key effects in slit and curved pores but their relative contributions have yet to be quantified. In this paper, we perform benchmark electronic structure calculations allowing the interactions between planar and curved aromatic molecules with hydrogen to be accurately determined. Dispersion was found to dominate over electrostatic and inductive effects with some many-body charge transfer (Dobson type-A) effects needed to capture the most highly curved structures. Density functional methods that include type-A many-body effects were found to accurately describe the intermolecular interactions at a fraction of the cost of coupled-cluster simulations and these approaches were used to calculate the energies inside large carbon bowl and slit pores. The interaction energies inside the bowl pores were found to depend on the orientation of the hydrogen molecule. This rotational barrier, modeled as a quantum hindered rotor, could reproduce the peak splitting observed in inelastic neutron scattering experiments, with weak splitting arising from bowl-like fullerene pores and strong splitting from highly confining nanotubelike pores. Increasing the fraction of such curved pores in nanoporous carbons may therefore offer a pathway to enhance their hydrogen-storage capacity. Moreover, the preferential adsorption of ortho hydrogen on nanotubelike pores could enable the storage of high-density hydrogen without the need to remove heat produced during the ortho-para hydrogen conversion.

36 MATERIALS SCIENCE↗

DOE OSTI2026

Feature Engineering and Ensemble Methods for Imbalanced ICS Intrusion Detection: Pipeline Audit and Constrained Evaluation

Industries are becoming increasingly connected and are more vulnerable to cyberattacks due to the widened attack surface. Industrial Control Systems (ICS) are among the most critical sectors that malicious actors can target, as such attacks can cause significant operational disruption and physical damage. It is imperative to detect such attacks as early as possible. This paper evaluates constraint-conditioned optimistic performance estimates for traditional ML models in ICS intrusion detection (i.e., estimates obtained under contiguous, non-shuffled temporal evaluation without test-set alteration, but with pre-split feature engineering that may introduce temporal leakage, due to dataset constraints). Our findings are threefold. First, we quantify how iterative feature engineering affects tree-based ensemble performance and examine how pipeline decisions (split strategy, sampling scope, and cleaning policy) can inflate or reduce reported IDS results under constraint-bound evaluation. Second, we compare intrinsic class-imbalance handling across ensemble models. Third, under our current pipeline constraints (including pre-split feature engineering), CatBoost achieves the best performance on Water Storage Tank (accuracy: 0.9831, class-1 F1: 0.9682), while Light- GBM achieves the best performance on Gas Pipeline (accuracy: 0.9618, class-1 F1: 0.9086).

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2021

Microsecond Carrier Lifetimes in Polycrystalline CdSeTe Heterostructures and in CdSeTe Thin Film Solar Cells

We report significant advances in understanding and reducing nonradiative Shockley-Read-Hall recombination in polycrystalline CdSe x Te 1-x , leading to microsecond charge carrier lifetimes. In undoped Al 2 O 3 -passivated heterostructures we find external radiative efficiency 0.2%, quasi-Fermi level splitting 950 mV, mobility 100 cm 2 /(Vs), and diffusion length 14 µm. In solar cells measured lifetimes can exceed 1 µs. We interpret this data to indicate MgZnO/CdSeTe interface recombination velocity <; 100 cm/s. Based on our results, it appears CdTe PV technology has potentially overcome longstanding “recombination lifetime” limitation and in the near future will transition to improving other aspects of device design.

41 EE - Solar Energy Technologies Office (EE-4S)↗

DOE OSTI2017

An optically passive method that rate doubles 2-GHz timing fiducials

Solid-state optical comb-pulse generators provide a convenient and accurate method to include timing fiducials in a streak camera image for time base correction. Commercially available vertical-cavity surface-emitting lasers (VCSEL’s) emitting in the visible currently in use can be modulated up to 2 GHz. An optically passive method is presented to interleave a time-delayed path of the 2-GHz comb with itself, producing a 4-GHz comb. This technique can be applied to VCSEL’s with higher modulation rates. A fiber-delivered, randomly polarized 2 GHz VCSEL comb is polarization split into s polarization and p polarization paths. One path is time delayed relative to the other by twice the 2-GHz rate with 1-ps accuracy; the two paths then recombine at the fiber-coupled output. High throughput (≥90%) is achieved by carefully using polarization beam-splitting cubes, a total internal reflection beam-path–steering prism, and antireflection coatings. The glass path-length delay block and turning prism are optically contacted together. The beam polarizer cubes that split and recombine the paths are precision aligned and permanently cemented into place. We expect the palm-sized, inline fiber-coupled, comb-rate–doubling device to maintain its internal alignment indefinitely.

optical comb-pulse generators, timing fiducials, s↗

DOE OSTI2015

SU-E-T-433: Field-In-Field Irradiation for Breast Cancer with VERO-4DRT System: A Feasibility Study

Purpose: The Vero-4DRT system is a dedicated system for high precision radiation therapy. However, the field size is limited at 15 cm x 15 cm and shapes by using multi-leaf collimator (MLC) without X-Jaw and Y-Jaw. Therefore VERO-4DRT system is not available to simple wedged irradiation for breast cancer. In this study, we suppose FIF with ring and/or tilt/pan angles whole breast irradiation (FIFWBI). The purpose of this study is to verify the feasibility of FIFWBI with VERO-4DRT system. Methods: As fundamental evaluation, we performed commissioning test with phantom. The absorbed dose evaluation at several reference points and dose distribution including split area were performed. We planned 10 demonstrative shapes in phantom for measuring these contents with i-plan workstation (BrainLAB). As clinical evaluation, the dose distribution and dose indexes were evaluated with actual patient data. Five patients with breast cancer were designed FIFWBI radiotherapy plan with split fields. Then, the dose distribution and dose indexes (including Dmax, Dmin, D95, D5 and Homogeneity index) were evaluated in these plans. Results: As the results of fundamental evaluation, all absorbed dose errors between calculated and measured doses were within 2%. The gamma passing rates with 2 mm/3% criteria in all cases were 96±2%. As the results of clinical evaluation, the values of Dmax, D95, D50, D5, and Homogeneity Index were 41.7±0.90 Gy, 49.4±0.34 Gy, 52.26±0.24 Gy, and 1.39±0.03, respectively. For Japanese breast cancer patients, this technique was feasible. However, the large split region was happened in FIFWBI in case of patient with large breast. Conclusion: We evaluated the FIFWBI technique with VERO-4DRT system. This technique is feasible for Japanese patients, but the patient with large breast should be disagreed with this technique.

60 APPLIED LIFE SCIENCES↗

DOE OSTI2016

A region-based segmentation method for ultrasound images in HIFU therapy

Purpose: Precisely and efficiently locating a tumor with less manual intervention in ultrasound-guided high-intensity focused ultrasound (HIFU) therapy is one of the keys to guaranteeing the therapeutic result and improving the efficiency of the treatment. The segmentation of ultrasound images has always been difficult due to the influences of speckle, acoustic shadows, and signal attenuation as well as the variety of tumor appearance. The quality of HIFU guidance images is even poorer than that of conventional diagnostic ultrasound images because the ultrasonic probe used for HIFU guidance usually obtains images without making contact with the patient’s body. Therefore, the segmentation becomes more difficult. To solve the segmentation problem of ultrasound guidance image in the treatment planning procedure for HIFU therapy, a novel region-based segmentation method for uterine fibroids in HIFU guidance images is proposed. Methods: Tumor partitioning in HIFU guidance image without manual intervention is achieved by a region-based split-and-merge framework. A new iterative multiple region growing algorithm is proposed to first split the image into homogenous regions (superpixels). The features extracted within these homogenous regions will be more stable than those extracted within the conventional neighborhood of a pixel. The split regions are then merged by a superpixel-based adaptive spectral clustering algorithm. To ensure the superpixels that belong to the same tumor can be clustered together in the merging process, a particular construction strategy for the similarity matrix is adopted for the spectral clustering, and the similarity matrix is constructed by taking advantage of a combination of specifically selected first-order and second-order texture features computed from the gray levels and the gray level co-occurrence matrixes, respectively. The tumor region is picked out automatically from the background regions by an algorithm according to a priori information about the tumor position, shape, and size. Additionally, an appropriate cluster number for spectral clustering can be determined by the same algorithm, thus the automatic segmentation of the tumor region is achieved. Results: To evaluate the performance of the proposed method, 50 uterine fibroid ultrasound images from different patients receiving HIFU therapy were segmented, and the obtained tumor contours were compared with those delineated by an experienced radiologist. For area-based evaluation results, the mean values of the true positive ratio, the false positive ratio, and the similarity were 94.42%, 4.71%, and 90.21%, respectively, and the corresponding standard deviations were 2.54%, 3.12%, and 3.50%, respectively. For distance-based evaluation results, the mean values of the normalized Hausdorff distance and the normalized mean absolute distance were 4.93% and 0.90%, respectively, and the corresponding standard deviations were 2.22% and 0.34%, respectively. The running time of the segmentation process was 12.9 s for a 318 × 333 (pixels) image. Conclusions: Experiments show that the proposed method can segment the tumor region accurately and efficiently with less manual intervention, which provides for the possibility of automatic segmentation and real-time guidance in HIFU therapy.

60 APPLIED LIFE SCIENCES↗

DOE OSTI2019

Response to comment on “Giant electromechanical coupling of relaxor ferroelectrics controlled by polar nanoregion vibrations”

Gehring et al . argue that a splitting observed by us in the transverse acoustic (TA) phonon in the relaxor ferroelectric Pb[(Mg 1/3 Nb 2/3 ) 1- x Ti x ]O 3 with x = 0.30 (PMN-30PT) is caused by a combination of inelastic-elastic multiple scattering processes called ghostons. Their argument is motivated by differences observed between their measurements made on a triple-axis spectrometer and our measurements on a time-of-flight spectrometer. We show that the differences can be explained by differences in the instrument resolution functions. We demonstrate that the multiple scattering conditions proposed by Gehring et al . do not work for our scattering geometry. We also demonstrate that, when a ghoston is present, it is too weak to detect and therefore cannot explain the splitting. Finally, this phonon splitting is just one part of the argument, and the overall conclusion of the original paper is supported by other results.

36 MATERIALS SCIENCE↗

DOE OSTI2015

Phase transitions and photoinduced transformations at high pressure in the molecular donor-acceptor fullerene complex (Cd(dedtc){sub 2}){sub 2} · C{sub 60}

The Raman spectra of crystals of C{sub 60} fullerene-cadmium diethyldithiocarbamate molecular donor-acceptor complexes (Cd(dedtc){sub 2}){sub 2} · C{sub 60} were measured at pressures of up to 17 GPa, and the crystal lattice parameters of these complexes were determined at pressures of up to 6 GPa. An increase in pressure up to ∼2 GPa leads to changes in the Raman spectra, which are manifested by splitting of the intramolecular H{sub g}(1)-H{sub g}(8) phonon modes and by softening of the A{sub g}(2) mode of the C{sub 60} molecule. A further increase in pressure up to 17 GPa does not induce significant new changes to the Raman spectra, while a decrease is accompanied by the reverse transformation at a pressure of about 2 GPa. The pressure dependence of the lattice parameters also exhibits a reversible feature at 2 GPa related to a jumplike decrease in compressibility. All these data are indicative of a phase transition in the vicinity of 2 GPa related to the formation of covalent bonds between C{sub 60} molecules and, probably, the appearance of C{sub 120} dimers in fullerene layers. It was also found that, in the pressure interval from 2 to 6.3 GPa, the Raman spectra of complexes exhibit photoinduced transformations under prolonged exposure to laser radiation with a wavelength of λ = 532 nm and power density up to 5000 W/cm{sup 2}. These changes are manifested by splitting and softening of the A{sub g}(2) mode and resemble analogous changes accompanying the photopolymerization of C{sub 60} fullerene. The intensity of new bands exhibits exponential growth with increasing exposure time. The photopolymer yield depends on both the laser radiation power and external pressure. The A{sub g}(2) mode splitting under irradiation can be related to the formation of photo-oligomers with various numbers of intermolecular covalent bonds per C{sub 60} molecule.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2015

Anisotropic spin–orbit stark effect in cubic semiconductors without an inversion center

The effect of external electric and magnetic fields on shallow donor levels in a semiconductor of the T{sub d} crystallographic class is analyzed. Application of an electric field eliminates the symmetry of the donor potential with respect to space inversion; as a result, corrections from the momentum-odd spin–orbit Dresselhaus term appear in the donor levels. In a strong electric field, such corrections determine the anisotropy of spin splitting of the donor levels relative to the directions of the external fields in the crystallographic coordinate system. Analytic expressions are derived for the spin splitting anisotropy for various relations between the magnitudes of the magnetic and electric fields. The results of this study can be used to determine the Dresselhaus spin–orbit interaction constant by a new method (in experiments on spin splitting of donor levels)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2017

Investigation of a nonequilibrium polariton condensate in cylindrical micropillars in a strong magnetic field

We analyze the photoluminescence of a nonequilibrium polariton condensate in cylindrical micropillars etched on the surface of a high-Q GaAs microcavity in a wide range of detunings in a magnetic field up to 12 T for various levels of nonresonant laser pumping by nanosecond pulses. With such a method of excitation, a considerable effect of the interaction of the reservoir of photoexcited excitons with the condensate on the Zeeman splitting of the polariton condensate levels can be expected, which can lead to a decrease in its value and even to sign reversal. However, the measurements of photoluminescence in a wide range of optical excitation densities show that Zeeman splitting weakly depends on the optical pumping (its variation does not exceed 15% of the splitting in a field of 12 T). The estimation of the exciton density in the reservoir based on these data gives a value lower than 10{sup 8} cm{sup –2}. In addition, a noticeable decrease (by a factor of about 1.8) in the polariton condensation threshold in a magnetic field is detected.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2018

Investigation of a Polariton Condensate in Micropillars in a High Magnetic Field

The photoluminescence of a nonequilibrium polariton condensate in cylindrical and rectangular micropillars etched on the surface of a high-Q GaAs microcavity is investigated in magnetic fields of up to 12 T. The measurements are carried out under different levels of nonresonant optical pumping with nanosecond laser pulses for a wide range of cavity detuning. As far as nonresonant excitation produces a high density of excitons in a reservoir, it should be expected that the exciton–polariton interaction, which depends on the pump level, has a considerable effect on the Zeeman splitting and polarization of the condensate. However, measurements of the Zeeman splitting and polarization in high magnetic fields demonstrate that only minor changes take place up to the highest available pump levels. This means that, in the case under study, the effect of exciton–polariton interaction on the polariton system is insignificant. At the same time, the data obtained provide an estimate for the exciton density in the reservoir. In contrast to cylindrical micropillars, the photoluminescence of the condensate in rectangular micropillars consists of two perpendicularly linearly polarized lines which retain a high degree of linear polarization even in a field as high as 12 T. The Zeeman splitting in this case is nearly independent of the pump power. The degrees of both circular and linear polarization change with pump power, but these changes are noticeably smaller than the ones predicted theoretically. This indicates that the system of polaritons in micropillars deviates considerably from thermodynamic equilibrium.

36 MATERIALS SCIENCE↗