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NASA NTRS2013

Recent Progress in DIB Research: Survey of PAHS and DIBS

The spectra of several neutral and ionized PAHs isolated in the gas phase at low temperature have been measured in the laboratory under experimental conditions that mimic interstellar conditions and are compared with an extensive set of astronomical spectra of reddened, early type stars [1, 2]. The comparisons of astronomical and laboratory data provide upper limits for the abundances of specific neutral PAH molecules and ions along specific lines-of-sight. Something that is not attainable from infrared observations alone. We present the characteristics of the laboratory facility (COSmIC) that was developed for this study and discuss the findings resulting from the comparison of these unique laboratory data with high resolution, high S/N ratio astronomical observations. COSmIC combines a supersonic free jet expansion with discharge plasma and high-sensitivity cavity ringdown spectroscopy and provides experimental conditions that closely mimic the interstellar conditions. The column densities of the individual neutral PAH molecules and ions probed in these surveys are derived from the comparison of these unique laboratory data with high resolution, high S/N ratio astronomical observations. The comparisons of astronomical and laboratory data lead to clear and unambiguous conclusions regarding the expected abundances for PAHs of various sizes and charge states in the interstellar environments probed in the surveys. Band profile comparisons between laboratory and astronomical spectra lead to information regarding the molecular structures and characteristics associated with the DIB carriers in the corresponding lines-of-sight. These quantitative surveys of neutral and ionized PAHs in the optical range open the way for unambiguous quantitative searches of PAHs and complex organics in a variety of interstellar and circumstellar environments.

Salama, Farid↗
NASA NTRS2019

Millimeter/Submillimeter Spectroscopic Detection of Desorbed Ices: A New Technique in Laboratory Astrochemistry

A new laboratory technique has been developed that utilizes gas-phase, direct-absorption millimeter and submillimeter spectroscopy to detect and identify desorbed species from interstellar and cometary ice analogs. Rotational spectroscopy is a powerful structure-specific technique for detecting isomers and other species possessing the same mass that are indistinguishable with mass spectrometry. Furthermore, the resultant laboratory spectra are directly comparable to observational data from far-infrared and millimeter telescopes. Here we present the proof-of-concept measurements of the detection of thermally desorbed H2O, D2O, and CH3OH originating in a solid film created at low temperature (~12 K). The surface binding energy of H2O is reported and compared to results from traditional techniques, including mass spectrometry and quartz-crystal microbalance measurements of mass loss. Lastly, we demonstrate that this technique is capable of deriving thermodynamic values including the sublimation enthalpy and entropy of H2O.

Katarina M. Yocum↗
DOE OSTI2021

Gas-phase synthesis of corannulene – a molecular building block of fullerenes

Fullerenes (C 60 , C 70 ) detected in planetary nebulae and carbonaceous chondrites have been implicated to play a key role in the astrochemical evolution of the interstellar medium. However, the formation mechanism of even their simplest molecular building block—the corannulene molecule (C 20 H 10 )—has remained elusive. Here we demonstrate via a combined molecular beams and ab initio investigation that corannulene can be synthesized in the gas phase through the reactions of 7-fluoranthenyl (C 16 H 9 ˙) and benzo[ghi]fluoranthen-5-yl (C 18 H 9 ˙) radicals with acetylene (C 2 H 2 ) mimicking conditions in carbon-rich circumstellar envelopes. This reaction sequence reveals a reaction class in which a polycyclic aromatic hydrocarbon (PAH) radical undergoes ring expansion while simultaneously forming an out-of-plane carbon backbone central to 3D nanostructures such as buckybowls and buckyballs. In conclusion, these fundamental reaction mechanisms are critical in facilitating an intimate understanding of the origin and evolution of the molecular universe and, in particular, of carbon in our galaxy.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1981

Interstellar hot plasma contributions to the diffuse ultraviolet background

The intensity of the diffuse background emission in the far ultraviolet from hot coronal gas present in the plane and halo of the galaxy is calculated. The main emission lines expected are those of C III, IV, N III, IV and Si III, IV at 1909, 1549, 1749, 1487, 1207 and 1398 A respectively. Unless the gas is unusually clumped or has extremely depleted abundances, this source is not of sufficient intensity to influence current broadband measurements of the diffuse continuous ultraviolet background. However, future observations at higher sensitivity and resolution might have to take this effect into account.

Jakobsen, P.↗
NASA NTRS1982

A heuristic criterion for instability to fragmentation in rotating, interstellar clouds

A heuristic criterion, based on linear perturbation analysis, is applied to the initial growth of density perturbations in isothermal or adiabatic gas clouds, with initially uniform density and uniform rotation. The heuristic criterion is shown to be consistent with the available results from numerical calculations of cloud collapse. The criterion predicts that perturbations varying as cos(m-phi) will be most likely to grow when m is small, unless the cloud is nearly pressureless.

Boss, A. P.↗
NASA NTRS1982

A Heuristic Criterion for Instability to Fragmentation in Rotating, Interstellar Clouds

A heuristic criterion, based on linear perturbation analysis, is applied to the initial growth of density perturbations in isothermal or adiabatic gas clouds, with initially uniform density and uniform rotation. The heuristic criterion is shown to be consistent with the available results from numerical calculations of cloud collapse. The criterion predicts that perturbations varying as cos (m(phi)) will be most likely to grow when )pi is small, unless the cloud is nearly pressureless.

Boss, Alan Paul↗
NASA NTRS1996

Revised Depletions and New Constraints on Interstellar Dust Composition

We have reviewed the literature on composition of young stars, both hot and cool, as well as older solar-type stars. We find that all these classes of stars have lower abundances of the heavy elements (specifically C, N, O, Mg, Si, and Fe) than the sun. Therefore studies of interstellar depletions in which the solar composition is used as the reference standard are probably in error, tending to overestimate the total quantities of these elements, hence the depletions. We have revised the depletion estimates, using stellar abundances as the reference standard and making use of recent IS gas-phase abundance measurements. As a result of our revised depletions, we can place new and stringent constraints on several published models for the interstellar dust.

Snow, Theodore P.↗
DOE OSTI2014

C{sup +} in the interstellar medium: Collisional excitation by H{sub 2} revisited

C{sup +} is a critical constituent of many regions of the interstellar medium, as it can be a major reservoir of carbon and, under a wide range of conditions, the dominant gas coolant. Emission from its 158 μm fine structure line is used to trace the structure of photon-dominated regions in the Milky Way and is often employed as a measure of the star formation rate in external galaxies. Under most conditions, the emission from the single [C II] line is proportional to the collisional excitation rate coefficient. We here used improved calculations of the deexcitation rate of [C II] by collisions with H{sub 2} to calculate more accurate expressions for interstellar C{sup +} fine structure emission, its critical density, and its cooling rate. The collision rates in the new quantum calculation are ∼25% larger than those previously available, and narrow the difference between rates for excitation by atomic and molecular hydrogen. This results in [C II] excitation being quasi-independent of the molecular fraction and thus dependent only on the total hydrogen particle density. A convenient expression for the cooling rate at temperatures between 20 K and 400 K, assuming an LTE H{sub 2} ortho to para ratio is Λ=(11.5+4.0 e{sup −100} {sup K/T{sup k{sup i{sup n}}}}) e{sup −91.25} {sup K/T{sup k{sup i{sup n}}}} n(C{sup +}) n(H{sub 2})×10{sup −24} erg cm{sup −3} s{sup −1}. The present work should allow more accurate and convenient analysis of the [C II] line emission and its cooling.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

The effect of selective desorption mechanisms during interstellar ice formation

Major components of ices on interstellar grains in molecular clouds—water and carbon oxides—occur at various optical depths. This implies that selective desorption mechanisms are at work. An astrochemical model of a contracting low-mass molecular cloud core is presented. Ice was treated as consisting of the surface and three subsurface layers (i.e., sublayers). Photodesorption, reactive desorption, and indirect reactive desorption were investigated. The latter manifests itself through desorption from H+H reaction on grains. Desorption of shallow subsurface species was also included. Modeling results suggest the existence of a “photon-dominated ice” during the early phases of core contraction. Subsurface ice is chemically processed by interstellar photons, which produces complex organic molecules (COMs). Desorption from the subsurface layer results in high COM gas-phase abundances at A{sub V} = 2.4–10 mag. This may contribute toward an explanation for COM observations in dark cores. It was found that photodesorption mostly governs the onset of ice accumulation onto grains. Reaction-specific reactive desorption is efficient for small molecules that form via highly exothermic atom-addition reactions. Higher reactive desorption efficiency results in lower gas-phase abundances of COMs. Indirect reactive desorption allows for closely reproducing the observed H{sub 2}O:CO:CO{sub 2} ratio toward a number of background stars. Presumably, this can be done by any mechanism whose efficiency fits with the sequence CO⩾CO{sub 2}≫H{sub 2}O. After the freeze-out has ended, the three sublayers represent chemically distinct parts of the mantle. The likely A{sub V} threshold for the appearance of CO ice is 8–10.5 mag. The lower value is supported by observations.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1990

A scaling law of radial gas distribution in disk galaxies

Based on the idea that local conditions within a galactic disk largely determine the region's evolution time scale, researchers built a theoretical model to take into account molecular cloud and star formations in the disk evolution process. Despite some variations that may be caused by spiral arms and central bulge masses, they found that many late-type galaxies show consistency with the model in their radial atomic and molecular gas profiles. In particular, researchers propose that a scaling law be used to generalize the gas distribution characteristics. This scaling law may be useful in helping to understand the observed gas contents in many galaxies. Their model assumes an exponential mass distribution with disk radius. Most of the mass are in atomic gas state at the beginning of the evolution. Molecular clouds form through a modified Schmidt Law which takes into account gravitational instabilities in a possible three-phase structure of diffuse interstellar medium (McKee and Ostriker, 1977; Balbus and Cowie, 1985); whereas star formation proceeds presumably unaffected by the environmental conditions outside of molecular clouds (Young, 1987). In such a model both atomic and molecular gas profiles in a typical galactic disk (as a result of the evolution) can be fitted simultaneously by adjusting the efficiency constants. Galaxies of different sizes and masses, on the other hand, can be compared with the model by simply scaling their characteristic length scales and shifting their radial ranges to match the assumed disk total mass profile sigma tot(r).

Wang, Zhong↗
NASA NTRS1991

Sublimation and reformation of icy grains in the primitive solar nebula

The quantity of water ice that sublimates during the free fall of grains into the solar nebula from a surrounding interstellar cloud varies from over 90 percent of the grain mass as 30 AU from the nebular center to less than 10 percent at more than 100 AU. Virtually all the water that is sublimated ultimately recondenses, since the cold nebular gas lying beyond 10 AU is unable to hold more than a small portion as vapor. The return of most of the gas to solid phase near the nebular ambient temperature, of about 50 K, may result in at least two grain populations consisting, in one case, of unaltered interstellar grains which did not undergo sublimation, and in the other of water ice which cocondensed with more volatile gases at nebular ambient temperatures to yield volatile-rich amorphous phases.

Lunine, Jonathan I.↗
DOE OSTI2016

STAR FORMATION SUPPRESSION DUE TO JET FEEDBACK IN RADIO GALAXIES WITH SHOCKED WARM MOLECULAR GAS

We present Herschel observations of 22 radio galaxies, selected for the presence of shocked, warm molecular hydrogen emission. We measured and modeled spectral energy distributions in 33 bands from the ultraviolet to the far-infrared to investigate the impact of jet feedback on star formation activity. These galaxies are massive, early-type galaxies with normal gas-to-dust ratios, covering a range of optical and infrared colors. We find that the star formation rate (SFR) is suppressed by a factor of ∼3–6, depending on how molecular gas mass is estimated. We suggest that this suppression is due to the shocks driven by the radio jets injecting turbulence into the interstellar medium (ISM), which also powers the luminous warm H{sub 2} line emission. Approximately 25% of the sample shows suppression by more than a factor of 10. However, the degree of SFR suppression does not correlate with indicators of jet feedback including jet power, diffuse X-ray emission, or intensity of warm molecular H{sub 2} emission, suggesting that while injected turbulence likely impacts star formation, the process is not purely parameterized by the amount of mechanical energy dissipated into the ISM. Radio galaxies with shocked warm molecular gas cover a wide range in SFR–stellar mass space, indicating that these galaxies are in a variety of evolutionary states, from actively star-forming and gas-rich to quiescent and gas-poor. SFR suppression appears to have the largest impact on the evolution of galaxies that are moderately gas-rich.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

THE HERSCHEL REFERENCE SURVEY: DUST IN EARLY-TYPE GALAXIES AND ACROSS THE HUBBLE SEQUENCE

We present Herschel observations of 62 early-type galaxies (ETGs), including 39 galaxies morphologically classified as S0+S0a and 23 galaxies classified as ellipticals using SPIRE at 250, 350, and 500 {mu}m as part of the volume-limited Herschel Reference Survey (HRS). We detect dust emission in 24% of the ellipticals and 62% of the S0s. The mean temperature of the dust is (T{sub d} ) = 23.9 {+-} 0.8 K, warmer than that found for late-type galaxies in the Virgo Cluster. The mean dust mass for the entire detected early-type sample is logM{sub d} = 6.1 {+-} 0.1 M{sub Sun} with a mean dust-to-stellar-mass ratio of log(M{sub d} /M{sub *}) = -4.3 {+-} 0.1. Including the non-detections, these parameters are logM{sub d} = 5.6 {+-} 0.1 and log(M{sub d} /M{sub *}) = -5.1 {+-} 0.1, respectively. The average dust-to-stellar-mass ratio for the early-type sample is fifty times lower, with larger dispersion, than the spiral galaxies observed as part of the HRS, and there is an order-of-magnitude decline in M{sub d} /M{sub *} between the S0s and ellipticals. We use UV and optical photometry to show that virtually all the galaxies lie close to the red sequence yet the large number of detections of cool dust, the gas-to-dust ratios, and the ratios of far-infrared to radio emission all suggest that many ETGs contain a cool interstellar medium similar to that in late-type galaxies. We show that the sizes of the dust sources in S0s are much smaller than those in early-type spirals and the decrease in the dust-to-stellar-mass ratio from early-type spirals to S0s cannot simply be explained by an increase in the bulge-to-disk ratio. These results suggest that the disks in S0s contain much less dust (and presumably gas) than the disks of early-type spirals and this cannot be explained simply by current environmental effects, such as ram-pressure stripping. The wide range in the dust-to-stellar-mass ratio for ETGs and the lack of a correlation between dust mass and optical luminosity suggest that much of the dust in the ETGs detected by Herschel has been acquired as the result of interactions, although we show these are unlikely to have had a major effect on the stellar masses of the ETGs. The Herschel observations tentatively suggest that in the most massive systems, the mass of interstellar medium is unconnected to the evolution of the stellar populations in these galaxies.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

DEMOGRAPHICS AND PHYSICAL PROPERTIES OF GAS OUTFLOWS/INFLOWS AT 0.4 < z < 1.4

We present Keck/LRIS spectra of over 200 galaxies with well-determined redshifts between 0.4 and 1.4. We combine new measurements of near-ultraviolet, low-ionization absorption lines with previously measured masses, luminosities, colors, and star formation rates to describe the demographics and properties of galactic flows. Among star-forming galaxies with blue colors, we find a net blueshift of the Fe II absorption greater than 200 km s{sup -1} (100 km s{sup -1}) toward 2.5% (20%) of the galaxies. The fraction of blueshifted spectra does not vary significantly with stellar mass, color, or luminosity but does decline at specific star formation rates less than roughly 0.8 Gyr{sup -1}. The insensitivity of the blueshifted fraction to galaxy properties requires collimated outflows at these redshifts, while the decline in outflow fraction with increasing blueshift might reflect the angular dependence of the outflow velocity. The low detection rate of infalling gas, 3%-6% of the spectra, suggests an origin in (enriched) streams favorably aligned with our sightline. We find that four of these nine infalling streams have projected velocities commensurate with the kinematics of an extended disk or satellite galaxy. The strength of the Mg II absorption increases with stellar mass, B-band luminosity, and U - B color, trends arising from a combination of more interstellar absorption at the systemic velocity and less emission filling in more massive galaxies. Our results provide a new quantitative understanding of gas flows between galaxies and the circumgalactic medium over a critical period in galaxy evolution.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2006

Laboratory Spectroscopy of Large Carbon Molecules and Ions in Support of Space Missions. A New Generation of Laboratory & Space Studies

Polycyclic Aromatic Hydrocarbons (PAHs) are an important and ubiquitous component of carbon-bearing materials in space. A long-standing and major challenge for laboratory astrophysics has been to measure the spectra of large carbon molecules in laboratory environments that mimic (in a realistic way) the physical conditions that are associated with the interstellar emission and absorption regions [1]. This objective has been identified as one of the critical Laboratory Astrophysics objectives to optimize the data return from space missions [2]. An extensive laboratory program has been developed to assess the properties of PAHs in such environments and to describe how they influence the radiation and energy balance in space. We present and discuss the gas-phase electronic absorption spectra of neutral and ionized PAHs measured in the UV-Visible-NIR range in astrophysically relevant environments and discuss the implications for astrophysics [1]. The harsh physical conditions of the interstellar medium characterized by a low temperature, an absence of collisions and strong VUV radiation fields - have been simulated in the laboratory by associating a pulsed cavity ringdown spectrometer (CRDS) with a supersonic slit jet seeded with PAHs and an ionizing, penning-type, electronic discharge. We have measured for the {\it first time} the spectra of a series of neutral [3,4] and ionized [5,6] interstellar PAHs analogs in the laboratory. An effort has also been attempted to quantify the mechanisms of ion and carbon nanoparticles production in the free jet expansion and to model our simulation of the diffuse interstellar medium in the laboratory [7]. These experiments provide {\it unique} information on the spectra of free, large carbon-containing molecules and ions in the gas phase. We are now, for the first time, in the position to directly compare laboratory spectral data on free, cold, PAH ions and carbon nano-sized carbon particles with astronomical observations in the UV-NIR range (interstellar UV extinction, DIBs in the NUV-NIR range). This new phase offers tremendous opportunities for the data analysis of current and upcoming space missions geared toward the detection of large aromatic systems Le., the "new frontier space missions" (Spitzer, HST, COS, JWST, SOFIA,...).

Salama, Farid↗
NASA NTRS2001

Observations of O VI Emission from the Diffuse Interstellar Medium

We report the first Far Ultraviolet Spectroscopic Explorer (FUSE) measurements of diffuse O(VI) (lambda lambda 1032,1038) emission from the general diffuse interstellar medium outside of supernova remnants or superbubbles. We observed a 30 arcsec x 30 arcsec region of the sky centered at l = 315.0 deg and b = -41.3 deg. From the observed intensities (2930 +/- 290 (random) +/- 410 (systematic) and 1790 +/- 260 (random) +/- 250 (systematic) photons/sq cm/s/sr in the 1032 and 1038 angstrom emission lines, respectively), derived equations, and assumptions about the source location, we calculate the intrinsic intensity, electron density, thermal pressure, and emitting depth. The intensities are too large for the emission to originate solely in the Local Bubble. Thus, we conclude that the Galactic thick disk and lower halo also contribute. High velocity clouds are ruled out because there are none near the pointing direction. The calculated emitting depth is small, indicating that the O(VI)-bearing gas fills a small volume. The observations can also be used to estimate the cooling rate of the hot interstellar medium and constrain models. The data also yield the first intensity measurement of the C(II) 3s 2S(1/2) to 2p 2P(3/2) emission line at 1037 angstrom and place upper limits on the intensities of ultraviolet line emission from C(I), C(III), Si(II), S(III), S(IV), S(VI), and Fe(III).

Shelton, R. L.↗
NASA NTRS1985

On interstellar Fe X forbidden line absorption. III - The lambda 6367 feature

Echelle spectra of Zeta Oph and HD 190603 are reported which show a weak interstellar absorption feature near 6367 A. The feature had been previously detected only toward two members of the Cepheus OB2 association in an extensive search for interstellar Fe X forbidden line absorption (lambda 6375). On the basis of the resulting radial velocities, the two new detections exclude the preliminary identification of the lambda 6367 feature with high-velocity Fe X ions in the hot, X-ray-emitting gas and demonstrate that the feature arises instead in the ordinary diffuse clouds. This unidentified feature may be either a molecular transition or a very weak diffuse interstellar band.

Hobbs, L. M.↗
DOE OSTI2014

An XMM-Newton study of the mixed-morphology supernova remnant W28 (G6.4–0.1)

We have performed an XMM-Newton imaging and spectroscopic study of supernova remnant (SNR) W28, a prototype mixed-morphology or thermal composite SNR believed to be interacting with a molecular cloud. The observed hot X-ray emitting plasma is characterized by low metal abundances, showing no evidence of ejecta. The X-rays arising from the deformed northeastern shell consist of a thermal component with a temperature of ∼0.3 keV plus a hard component of either thermal (temperature ∼0.6 keV) or non-thermal (photon index = 0.9-2.4) origin. The X-ray emission in the SNR interior is blobby and the corresponding spectra are best described as the emission from a cold (∼0.4 keV) plasma in non-equilibrium ionization with an ionization timescale of ∼4.3 × 10{sup 11} cm{sup –3} s plus a hot (∼0.8 keV) gas in collisional ionization equilibrium. Applying the two-temperature model to the smaller central regions, we find non-uniform interstellar absorption, temperature, and density distribution, which indicates that the remnant is evolving in a non-uniform environment with denser material in the east and north. The cloudlet evaporation mechanism can essentially explain the properties of the X-ray emission in the center, and thermal conduction may also play a role for length scales comparable to the remnant radius. A recombining plasma model with an electron temperature of ∼0.6 keV is also feasible for describing the hot central gas with the recombination age of the gas estimated at ∼2.9 × 10{sup 4} yr.

79 ASTRONOMY AND ASTROPHYSICS↗