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At least 1,477 records · Page 82

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DOE OSTI2022

Strong Coulomb coupling influences ion and neutral temperatures in atmospheric pressure plasmas

Molecular dynamics simulations are used to model ion and neutral temperature evolution in partially-ionized atmospheric pressure plasma at different ionization fractions. Results show that ion–ion interactions are strongly coupled at ionization fractions as low as 10 –5 and that the temperature evolution is influenced by effects associated with the strong coupling. Specifically, disorder-induced heating is found to rapidly heat ions on a timescale of the ion plasma period (~10 s ps) after an ionization pulse. This is followed by the collisional relaxation of ions and neutrals, which cools ions and heats neutrals on a longer (~ns) timescale. Slight heating then occurs over a much longer (~100 s ns) timescale due to ion-neutral three-body recombination. An analytic model of the temperature evolution is developed that agrees with the simulation results. Finally, a conclusion is that strong coupling effects are important in atmospheric pressure plasmas.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS2000

An Overview of Unsteady Pressure Measurements in the Transonic Dynamics Tunnel

The NASA Langley Transonic Dynamics Tunnel has served as a unique national facility for aeroelastic testing for over forty years. A significant portion of this testing has been to measure unsteady pressures on models undergoing flutter, forced oscillations, or buffet. These tests have ranged from early launch vehicle buffet to flutter of a generic high-speed transport. This paper will highlight some of the test techniques, model design approaches, and the many unsteady pressure tests conducted in the TDT. The objectives and results of the data acquired during these tests will be summarized for each case and a brief discussion of ongoing research involving unsteady pressure measurements and new TDT capabilities will be presented.

Schuster, David M.↗

DOE OSTI2024

Quantum stabilization and flat hydrogen-based bands of nitrogen-doped lutetium hydride

We explore the electronic and structural properties of Lu-H-N structures with specific N,H ordering due to their remarkably narrow hydrogen-based bands at the Fermi level. Although exhibits a classical instability persisting up to 17 GPa, it is anharmonically stable near ambient pressure when accounting for quantum nuclear effects. The presence of flat bands near is understood to arise from destructive quantum interference between and surrounding orbitals, with certain types of defects leaving the flat bands unaffected. The results suggest that if this system is superconducting, there is an optimal pressure near ambient where the superconducting is maximized by anharmonically stabilized low-frequency and nonadiabatically coupled high-frequency hydrogen modes. Despite the metastability of this structure, its dynamical stability when modeled beyond a classical harmonic approach suggests the narrow bands near do not cause structural distortions in certain Lu-H-N stoichiometries.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2020

In situ X-ray diffraction of silicate liquids and glasses under dynamic and static compression to megabar pressures

Properties of liquid silicates under high-pressure and high-temperature conditions are critical for modeling the dynamics and solidification mechanisms of the magma ocean in the early Earth, as well as for constraining entrainment of melts in the mantle and in the present-day core–mantle boundary. In this paper, we present in situ structural measurements by X-ray diffraction of selected amorphous silicates compressed statically in diamond anvil cells (up to 157 GPa at room temperature) or dynamically by laser-generated shock compression (up to 130 GPa and 6,000 K along the MgSiO 3 glass Hugoniot). The X-ray diffraction patterns of silicate glasses and liquids reveal similar characteristics over a wide pressure and temperature range. Beyond the increase in Si coordination observed at 20 GPa, we find no evidence for major structural changes occurring in the silicate melts studied up to pressures and temperatures exceeding Earth’s core mantle boundary conditions. This result is supported by molecular dynamics calculations. Our findings reinforce the widely used assumption that the silicate glasses studies are appropriate structural analogs for understanding the atomic arrangement of silicate liquids at these high pressures.

58 GEOSCIENCES↗

DOE OSTI2021

Anharmonic theory of superconductivity in the high-pressure materials

Electron-phonon superconductors at high pressures have displayed the highest values of critical superconducting temperature Tc on record, now rapidly approaching room temperature. Despite the importance of high-P superconductivity in the quest for room-temperature superconductors, a mechanistic understanding of the effect of pressure and its complex interplay with phonon anharmonicity and superconductivity is missing, as numerical simulations can bring only system-specific details, clouding out key players controlling the physics. In this work, we develop a minimal model of electron-phonon superconductivity under an applied pressure which takes into account the anharmonic decoherence of the optical phonons. We find that T c behaves nonmonotonically as a function of the ratio Γ/ω 0 , where Γ is the optical phonon damping and ω 0 is the optical phonon energy at zero pressure and momentum. Optimal pairing occurs for a critical ratio Γ/ω 0 when the phonons are on the verge of decoherence (“diffusonlike” limit). Our framework gives insights into recent experimental observations of T c as a function of pressure in the complex BCS material TlInTe 2 .

36 MATERIALS SCIENCE↗

DOE OSTI2020

Cesium Removal and Hydraulic Performance Comparisons of CST Ion Exchange Media Batches in Support of the Tank Closure Cesium Removal Project - 20522

Three batches of Crystalline Silicotitanate (CST) ion exchange media have been evaluated for cesium removal efficiency from a Savannah River Site (SRS) High Level Waste (HLW) supernate simulant in support of the Tank Closure Cesium Removal (TCCR) Project, which involves at-tank column waste treatment. Results will be utilized to select the CST media batch to be added to the next TCCR unit columns. Two of the CST media samples were recent production batches and the third was an archived batch studied extensively at SRS nearly two decades ago. The archived CST batch had a significantly smaller average particle diameter than more recent batches. Small-scale (∼23 mL), side-by-side column tests were conducted at 35 deg. C with each of the CST batches using the same simulant at flow rates near 1.2 mL/min (3.0-3.4 CST bed volumes/hr). The cesium ion exchange column performance results were lower than expected for all three CST batches, but the data indicated that 30% more simulant volume and 40% more equivalent CST bed volumes of solution can be processed with the older CST batch prior to reaching the 50% cesium breakthrough point than can be processed with the newer CST batches. Hydraulic evaluations of the CST columns were also conducted in simulant at 24 deg. C to determine the impact of the different particle size distributions and associated bed porosities on frictional pressure drop under dynamic flow conditions. Higher differential pressure drops were observed with the archived CST batch relative to recent production batches, due to the smaller particle size distribution and the packing characteristics of the archived batch. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

NASA NTRS1978

Some load limits and self-lubricating properties of plain spherical bearings with molded graphite fiber reinforced polyimide liners to 320 C

Plain spherical bearings with molded liners of self-lubricating graphite fiber-polyimide composite were developed and their dynamic load capacities were determined. Liners were prepared by transfer molding a prepolymer resin-fiber mix into the space between the ball and outer race, the completing polymerization under heat and pressure. Bearing dynamic load capacities were in excess of 140 MPa (20,000 psi) from room temperature to 260 C and about 70 MPa (10,000 psi) at 320 C. Friction coefficients were about 0.20 at room temperatures and light loads and tended to decrease with increasing temperatures and loads to about 0.15. Thermal expansion of the liner at uniform bearing temperatures of 200 C or higher produced a bearing preload which could be alleviated by providing an initial internal diametral clearance of 0.05 to 0.10 mm.

Sliney, H. E.↗

NASA NTRS1985

The role of a pressure-dependent rheology in the dynamics of mantle circulation

A thermomechanical model for upper mantle convection was constructed such that the thickness and the structure of the lithosphere are determined self consistently by the heat transported by convection. In this study of the interaction between the lithosphere and upper mantle, strongly temperature and pressure dependent rheologies for both Newtonian and non-Newtonian creep mechanisms are employed. For a strictly temperature dependent rheology an insignificant amount of heat, less than 12.5 mW/sq m, can be transported convectively for an interior viscosity, 0(10 sup 21 Pas), compatible with post glacial rebound. On the other hand, for similar values of the interior viscosity, steady heat fluxes between 20 and 40 mW/sq m are produced by introducing pressure dependence into the rheology. For the temperature and pressure dependent flow law the horizontally averaged interior temperature displays very little variation with the amount of heat evacuated, once all of the rheological parameters are fixed. This finding may have important ramifications for parameterized convection.

Yuen, D. A.↗

NASA NTRS2006

A Summary of the Experimental Results for a Generic Tractor-Trailer in the Ames Research Center 7- by 10-Foot and 12-Foot Wind Tunnels

Experimental measurements of a generic tractor-trailer were obtained in two wind tunnels at Ames Research Center. After a preliminary study at atmospheric conditions in the 7- by 10-Foot Wind Tunnel, additional testing was conducted at Reynolds numbers corresponding to full-scale highway speeds in the 12-Foot Pressure Wind Tunnel. To facilitate computational modeling, the 1:8-scale geometry, designated the Generic Conventional Model, included a simplified underbody and omitted many small-scale details. The measurements included overall and component forces and moments, static and dynamic surface pressures, and three-component particle image velocimetry. This summary report highlights the effects of numerous drag reduction concepts and provides details of the model installation in both wind tunnels. To provide a basis for comparison, the wind-averaged drag coefficient was tabulated for all configurations tested. Relative to the baseline configuration representative of a modern class-8 tractor-trailer, the most effective concepts were the trailer base flaps and trailer belly box providing a drag-coefficient reduction of 0.0855 and 0.0494, respectively. Trailer side skirts were less effective yielding a drag reduction of 0.0260. The database of this experimental effort is publicly available for further analysis.

Storms, Bruce L.↗

NASA NTRS1992

Oligomeric baroeffect and gas aggregation states

The baroeffect is analyzed to include a gas that aggregates into higher-order polymers or oligomers. The resulting pressure change is found to vary independently of the molecular weight of the gas components and to depend only on the aggregation or oligomeric order of the gas. With increasing aggregation, diffusive slip velocities are found to increase. The calculations are extended to include general counterdiffusion of two distinct aggregation states (k-, j-mer) for the gas, and the pressure change is derived as a function that is independent of both molecular weight and the absolute aggregation. The only parameter that determines the baroeffect is the ratio of aggregated states, beta = k/j. For gases that reversibly aggregate, possible oscillatory behavior and complex dynamics for pressure are discussed. Gas aggregation may play a role for low-temperature crystal-growth conditions in which vapor concentrations of one (or more) species are high.

Noever, David A.↗

NASA NTRSDate not supplied

Aeroacoustic Analysis using Dynamic Mode Decomposition of Unsteady Pressure-Sensitive Paint Measurements

In this paper, we present a new method for the diagnosis and analysis of aeroacoustic phenomena. Taking advantage of the well-known property that the measurements of the Unsteady Pressure-Sensitive Paint (uPSP) have much higher spatial resolution compared to those of the conventional pressure transducers, the method is based on the visualization and analysis of the outputs of the Dynamic Mode Decomposition (DMD) of the uPSP measurements. The uPSP measurements were collected with four Phantom high-speed cameras in the Ascent Transient Aerodynamics Test (ATAT) of the Space Launch System (SLS) Block 1 cargo vehicle in the 11-by-11-foot transonic test section of the Unitary Plan Wind Tunnel (UPWT) at NASA Ames Research Center in September 2019. The method presented in this paper is demonstrated by investigating an interesting phenomenon observed in the SLS ATAT – the vortex shedding tone generated by the forward attachment of the Solid Rocket Booster (SRB). As examples, the DMD outputs of the uPSP measurements in a subsonic test in the SLS ATAT are presented. It is shown the information retrieved from the DMD outputs of the uPSP measurements can be effectively used in the identification and diagnosis of the aeroacoustic phenomena. The work described in this paper is a part of NASA’s development of a new state-of-the-art uPSP capability in production wind tunnels. Funding was provided by the NASA Aerosciences Evaluation and Test Capabilities Portfolio Office.

acoustics↗

NASA NTRSDate not supplied

Aeroacoustic Analysis using Dynamic Mode Decomposition of Unsteady Pressure-Sensitive Paint Measurements

acoustics↗

NASA NTRS1976

Experimental dynamic stiffness and damping of externally pressurized gas-lubricated journal bearings

A rigid vertical shaft was operated with known amounts of unbalance at speeds to 30,000 rpm and gas supply pressure ratios to 4.8. From measured amplitude and phase angle data, dynamic stiffness and damping coefficients of the bearings were determined. The measured stiffness was proportional to the supply pressure, while damping was little affected by supply pressure. Damping dropped rapidly as the fractional frequency whirl threshold was approached. A small-eccentricity analysis overpredicted the stiffness by 20 to 70 percent. Predicted damping was lower than measured at low speeds but higher at high speeds.

Fleming, D. P.↗

NASA NTRS1976

Dynamic stiffness and damping of externally pressurized gas lubricated journal bearings

A rigid vertical shaft was operated with known amounts of unbalance at speeds up to 30,000 rpm and gas supply pressure ratios to 4.8. From measured amplitude and phase angle data, dynamic stiffness and damping coefficients of the bearings were determined. The measured stiffness was proportional to the supply pressure, while damping was little affected by supply pressure. Damping dropped rapidly as the fractional frequency whirl threshold was approached. A small eccentricity analysis overpredicted the stiffness by 4 to 55 percent. Predicted damping was close to measured at low speeds but higher at high speeds

Fleming, D. P.↗

DOE OSTI2021

Controlling the Morphology of Dynamic Thia-Michael Networks to Target Pressure-Sensitive and Hot Melt Adhesives

A series of multistage (pressure-sensitive/hot melt) adhesives utilizing dynamic thia-Michael bonding motifs are reported. The benzalcyanoacetate Michael acceptors used in this work undergo bond exchange under ambient conditions without external catalysis, facilitating pressure-sensitive adhesion. A key feature of this system is the dynamic reaction-induced phase separation that lends reinforcement to the otherwise weakly bonded materials, enabling weak, repeatable pressure-sensitive adhesion under ambient conditions and strong adhesion when processed as a hot melt adhesive. Furthermore, by using different pairs of benzalcyanoacetate cross-linking units, the phase separation characteristics of the adhesives can be directly manipulated, allowing for a tailored adhesive response.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2026

3D probabilistic fracture mechanics / computational fluid dynamics simulation of a reactor pressure vessel under transient conditions

Reactor pressure vessels (RPVs) are safety-critical light-water-reactor components that, under irradiation, experience long-term material degradation in the form of embrittlement. This can increase their susceptibility to fracture under thermal-shock conditions, which could occur during off-normal transients such as loss-of-coolant accidents (LOCAs). During a LOCA, the most severe conditions for the RPV occur when emergency core cooling water is injected through the cold legs into the water-and-steam-filled RPV. The rapid cooling of the downcomer and internal RPV surface causes decreased temperature and elevated thermally driven tensile stresses in the RPV wall. This, combined with long-term material embrittlement, may cause fracture initiation at pre-existing flaws, challenging the integrity of the RPV. Assessing RPV integrity during transients with a large spatial variation in the coolant temperature requires a modeling approach that considers the effects of spatially varying coolant temperature on the fracture probability of a population of flaws distributed throughout the RPV, accounting for spatially varying embrittlement. Here, the present study addresses this need by demonstrating first-of-its-kind coupling of a high-fidelity 3D computational fluid dynamics code with 3D probabilistic fracture mechanics This was accomplished using representative models of a pressurized-water reactor subjected to small- and medium-break LOCA conditions, both of which can result in large spatial temperature variations. While the observed impact of accounting for 3D effects was minimal under the small-break LOCA this study indicates a significant increase in the probability of fracture initiation under the medium-break LOCA when 3D effects are considered, relative to a spatially uniform cooling scenario.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

DOE OSTI2023

Dynamic modeling and simulation of pressure swing adsorption processes using toPSAil

Pressure swing adsorption (PSA) has attracted significant recent interest for chemical process intensification due to its potential for high energy efficiency and amenability to small, modular designs. However, the lack of simulation tools that are readily available, transparent, and trusted, has been identified as a serious impediment to widespread adoption of PSA, as well as to further research on PSA modeling, numerical solution, optimization, and control. This paper presents a complete framework for dynamic modeling and simulation of PSA processes and its implementation in an open-source simulator called toPSAil. Further, the presentation is tutorial and includes many modeling and implementation details often overlooked in existing literature. Novel methods are presented for handling flow reversals and implementing various pressure–flow relationships, along with controlled boundary conditions. Finally, the code contains several innovations designed to improve efficiency and reduce the extensive trial-and-error tuning often required to produce a working PSA cycle.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NASA NTRS1994

Dynamic Leg Exercise Improves Tolerance to Lower Body Negative Pressure

These results clearly demonstrate that dynamic leg exercise against the footward force produced by LBNP substantially improves tolerance to LBNP, and that even cyclic ankle flexion without load bearing also increases tolerance. This exercise-induced increase of tolerance was actually an underestimate, because subjects who completed the tolerance test while exercising could have continued for longer periods. Exercise probably increases LBNP tolerance by multiple mechanisms. Tolerance was increased in part by skeletal muscle pumping venous blood from the legs. Rosenhamer and Linnarsson and Rosenhamer also deduced this for subjects cycling during centrifugation, although no measurements of leg volume were made in those studies: they found that male subjects cycling at 98 W could endure 3 Gz centrifugation longer than when they remained relaxed during centrifugation. Skeletal muscle pumping helps maintain cardiac filling pressure by opposing gravity-, centrifugation-, or LBNP-induced accumulation of blood and extravascular fluid in the legs.

Watenpaugh, D. E.↗