Aqua Status and 2020 Senior Review (A very brief overview)
A brief overview presentation by the Aqua Deputy Project Scientist during the virtual MODIS-VIIRS Atmosphere Discipline Science Team Meeting.
Aqua↗
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Results for “Atmospheric Science”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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SAGE III/ISS Rapid Data Analysis Through Dashboarding with Jupyter Notebooks
Spaceborne remote sensing observations of Earth’s atmosphere produce significant quantities of data over the life of each mission. In the case of the Stratospheric Aerosol and Gas Experiment III on the International Space Station (SAGE III/ISS) nearly four years of vertical profiles of atmospheric ozone, water vapor, and nitrogen dioxide concentrations as well as aerosol extinction coefficients have been released. The dichotomy of the desire for both long-term trends in the atmospheric state alongside the assessment of short-term impacts of major disruptive events such as volcanic eruptions and pyrocumulus injections requires agile tools to handle these cases in near real-time as new data are produced. The analysis landscape is further complicated by the desire to compare results between the numerous contemporary observations available for a given dataset. The SAGE III/ISS team has developed a suite of tools leveraging modern web-based frameworks allowing members to interact with a dashboard-style interface to load the data record, assess new profiles as they are generated and in ensemble, compare between species, and additionally add in measurements observed by other platforms as necessary. Leveraging a commonly packaged data format of NetCDF alongside the Python Jupyter Notebook framework, the data can be served to interested parties from an analysis server while still runnable on personal systems if required. This presentation illustrates the ecosystem developed by the SAGE III/ISS team, the applicability to measurements made by any limb-observing platform, and the benefit to transforming routine analyses into readily accessible dynamic plots. Frameworks currently exist at larger scales with projects such as GIOVANNI, and this illustration seeks to show that similar frameworks are accessible and possible within the local research environment while simultaneously unloading human processing cycles for more specialized analysis tasks.
Dashboarding↗
The Climates of Earth's Next Supercontinent: Effects of Tectonics, Rotation Rate, and Insolation
We explore two possible Earth climate scenarios, 200 and 250 million years into the future, using projections of the evolution of plate tectonics, solar luminosity, and rotation rate. In one scenario, a supercontinent forms at low latitudes, whereas in the other it forms at high northern latitudes with an Antarctic subcontinent remaining at the south pole. The climates between these two end points are quite stark, with differences in mean surface temperatures approaching several degrees. The main factor in these differences is related to the topographic height of the high latitude supercontinents where higher elevations promote snowfall and subsequent higher planetary albedos. These results demonstrate the need to consider multiple boundary conditions when simulating Earth-like exoplanetary climates.
insolation↗
Airborne and Ground-Based Measurements of Aerosol Optical Depth of Freshly Emitted Anthropogenic Plumes in the Athabasca Oil Sands Region
In this work we report the airborne aerosol optical depth (AOD) from measurements within freshly emitted anthropogenic plumes arising from mining and processing operations in the Athabasca Oil Sands Region (AOSR) in the context of ground-based AERONET climatological daily averaged AODs at Fort McMurray (Alberta, Canada). During two flights on 9 and 18 June 2018, the NASA airborne 4STAR (Spectrometers for Sky-Scanning, Sun-Tracking Atmospheric Research) Sun photometer registered high fine-mode (FM, <1 µm) in-plume AODs of up to 0.4 and 0.9, respectively, in the vicinity of the plume source (<20 km). Particle composition shows that the plumes were associated with elevated concentrations of sulfates and ammonium. These high AODs significantly exceed climatological averages for June and were not captured by the nearby AERONET instrument (mean daily AODs of 0.10±0.01 and 0.07±0.02, maximum AOD of 0.12) due possibly to horizontal inhomogeneity of the plumes, plume dilution and winds which in certain cases were carrying the plume away from the ground-based instrument. The average 4STAR out-of-plume (background) AODs deviated only marginally from AERONET daily averaged values. While 4STAR AOD peaks were generally well correlated in time with peaks in the in situ-measured particle concentrations, we show that differences in particle size are the dominant factor in determining the 4STAR-derived AOD. During the two flights of 24 June and 5 July 2018 when plumes likely travelled distances of 60 km or more, the average 4STAR FM AOD increased by 0.01–0.02 over ∼50 km of downwind particle evolution, which was supported by the increases in layer AODs calculated from the in situ extinction measurements. Based on these observations as well as the increases in organic mass, we attribute the observed AOD increase, at least in part, to secondary organic aerosol formation. The in-plume and out-of-plume AODs for this second pair of flights, in contrast to clear differences in in situ optical and other measurements, were practically indistinguishable and compared favourably to AERONET within 0.01–0.02 AOD. This means that AERONET was generally successful in capturing the background AODs, but missed some of the spatially constrained high-AOD plumes with sources as close as 30–50 km, which is important to note since the AERONET measurements are generally thought to be representative of the regional AOD loading. The fact that industrial plumes can be associated with significantly higher AODs in the vicinity of the emission sources than previously reported from AERONET can potentially have an effect on estimating the AOSR radiative impact.
AERONET↗
Machine-Learning Reveals Climate Forcing From Aerosols is Dominated by Increased Cloud Cover
Aerosol-cloud interactions have a potentially large impact on climate, but are poorly quantified and thus contribute a significant and long-standing uncertainty in climate projections. The impacts derived from climate models are poorly constrained by observations, because retrieving robust large-scale signals of aerosol-cloud interactions are frequently hampered by the considerable noise associated with meteorological co-variability. The Iceland-Holuhraun effusive eruption in 2014 resulted in a massive aerosol plume in an otherwise near-pristine environment and thus provided an ideal natural experiment to quantify cloud responses to aerosol perturbations. Here we disentangle significant signals from the noise of meteorological co-variability using a satellite-based machine-learning approach. Our analysis shows that aerosols from the eruption increased cloud cover by approximately 10%, and this appears to be the leading cause of climate forcing, rather than cloud brightening as previously thought. We find that volcanic aerosols do brighten clouds by reducing droplet size, but this has a significantly smaller radiative impact than changes in cloud fraction. These results add substantial observational constraints on the cooling impact of aerosols. Such constraints are critical for improving climate models, which still inadequately represent the complex macro-physical and micro-physical impacts of aerosol-cloud interactions.
Aerosols↗
Perturbations in Stratospheric Aerosol Evolution Due to the Water-Rich Plume of the 2022 Hunga-Tonga Eruption
The January 2022 Hunga Tonga-Hunga Ha'apai (HTHH) volcanic eruption injected a relatively small amount of SO2, but significantly more water into the stratosphere than previously seen in the modern satellite record. Here we show that the large amount of water resulted in large perturbations to stratospheric aerosol evolution. Our Community Earth System Model simulation reproduces the enhanced water vapor observed by the Microwave Limb Sounder at pressure levels between 10 and 50 hPa for three months. Compared with a simulation without a water injection, this additional source of water vapor increases OH, which halves the SO2 lifetime. Subsequent coagulation creates larger sulfate particles that double the stratospheric aerosol optical depth. A seasonal forecast of volcanic plume transport in the southern hemisphere indicates this eruption will greatly enhance the aerosol surface area and water vapor near the polar vortex until at least October 2022, suggesting that there will continue to be an impact of the HTHH eruption on the climate system.
Atmospheric science↗
Analysis and Impact of the Hunga Tonga-Hunga Ha’apai Stratospheric Water Vapor Plume
On Jan. 15, 2022, the Hunga Tonga-Hunga Ha’apai eruption injected SO2 and H2O into the 31 middle stratosphere. The eruption produced a persistent mid-stratospheric sulfate aerosol and H2O layer mostly confined to Southern Hemisphere (SH) tropics (Eq. to 30°S). These layers are still present in the tropics 5 ½ months after the eruption. The SH tropical confinement is simulated using a trajectory model. Measurements following the eruption show that the H2O layer is slowly rising while the aerosol layer is descending. The H2O layer’s upward movement is consistent with the residual vertical velocity. Gravitationally settling explains the descent of the aerosol layer. A -4K temperature anomaly coincident with the H2O enhancement is observed and is caused by thermal adjustment to the additional H2O IR cooling. A simple model of volcanic water injection at the time of the eruption simulates the observed vertical distribution H2O.
Atmospheric science↗
Tracking the 2022 Hunga Tonga-Hunga Ha'Apai Aerosol Cloud in the Upper and Middle Stratosphere Using Space-Based Observations
On 15 January 2022, the submarine Hunga Tonga volcanic eruption lofted materials high into the upper stratosphere, reaching a record-breaking altitude of ~58 km, unprecedented in the satellite observations era. Within two weeks, the bulk of the injected material circulated the globe between 20 – 30 km altitude, as observed by satellite instruments. We estimate that the stratospheric aerosol optical depth (sAOD) is the largest since the Pinatubo eruption and is at least twice as great as the sAOD after the 2015 Calbubo eruption despite the similar SO 2 injection from that eruption. We use space-based observations to monitor the Hunga-Tonga volcanic plume evolution and transport at different altitudes as it circulates the globe. While the main aerosol layer remains trapped in the tropical pipe, small parts have already made it to both the northern and southern hemisphere poles by April, which is almost certain to influence this year's ozone hole.
Atmospheric science↗
Monitoring the 2022 Hunga Tonga-Hunga Ha'apai Aerosol Cloud Using Space-Based Observations
- We will analyze the volcanic plume progression, spread and properties using space-based observations - OMPS LP, SAGE III/ISS, CALIPSO, TROPOMI - OMPS LP and SAGE III/ISS are limb instruments that measure the aerosol vertical profiles globally, while CALIPSO is a LIDAR that measures the backscatter and depolarization ratio of the aerosol profiles. -TROPOMI is a UV instrument that measures SO2 and absorbing aerosol total column - Volcanic plume in the upper stratosphere - The main plume in middle stratosphere - Volcanic aerosol transport to SH/NH - Volcanic aerosol optical properties
Atmospheric Science↗
Monitoring the 2022 Hunga Tonga-Hunga Ha'apai Aerosol Cloud Using Space-Based Observations
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Atmospheric Science↗
Near Space Demonstration of A Compact LWIR Spectro-Polarimeter for Ice Cloud Measurements
In the summer of 2021, an InfraRed Channeled Spectro-Polarimeter (IRCSP) was demonstrated in the near space environment aboard a NASA Columbia Scientific Ballooning Facility high-altitude balloon out of Fort Sumner, NM. The compact IRCSP is sensitive to linearly polarized long-wave infrared (LWIR) light between 7-12 micron and targets cloud micro-physical properties. Post landing the instrument was retrieved with no damage to the optical payload and collected over 150 minutes of flight data at altitudes above 30 km. The results collected both demonstrate the application of uncooled microbolometers in the low pressure environment and represent the first know field evidence of a polarized signal from clouds in the LWIR. During deployment, the IRCSP reported brightness temperatures between 250-285K with uncertainty of < 1.5K. In addition, multiple intervals of statistically significant polarization with degrees of linear polarization (DoLP) between 1−20% were detected. These results support the hypothesis that the LWIR polarimetry has the potential to add new sensitivity to existing remote sensing platforms.
remote sensing↗
The Cross Equatorial Transport of the Hunga Tonga-Hunga Ha’apai Eruption Plume
On 15 January 2022, the Hunga Tonga-Hunga Ha'apai (HT) eruption injected SO 2 and water into the middle stratosphere. Shortly after the eruption, the water vapor anomaly moved northward toward and across the equator. This northward movement appears to be due to equatorial Rossby waves forced by the excessive infrared water vapor cooling. Following the early eruption stage, persistent mid-stratospheric water vapor and aerosol layers were mostly confined to Southern Hemisphere tropics (Eq. to 30°S). However, during the spring of 2022, the westerly phase of the tropical quasi-biennial oscillation (QBO) descended through the tropics. The HT water vapor and aerosol anomalies were observed to again move across the equator coincident with the shift in the Brewer-Dobson circulation and the descent of the QBO shear zone.
Atmospheric Science↗
Virus Infection of Phytoplankton Increases Average Molar Mass and Reduces Hygroscopicity of Aerosolized Organic Matter
Viral infection of phytoplankton is a pervasive mechanism of cell death and bloom termination, which leads to the production of dissolved and colloidal organic matter that can be aerosolized into the atmosphere. Earth-observing satellites can track the growth and death of phytoplankton blooms on weekly time scales but the impact of viral infection on the cloud forming potential of associated aerosols is largely unknown. Here, we determine the influence of viral-derived organic matter, purified viruses, and marine hydrogels on the cloud condensation nuclei activity of their aerosolized solutions, compared to organic exudates from healthy phytoplankton. Dissolved organic material derived from exponentially growing and infected cells of well-characterized eukaryotic phytoplankton host-virus systems, including viruses from diatoms, coccolithophores and chlorophytes, was concentrated, desalted, and nebulized to form aerosol particles composed of primarily of organic matter. Aerosols from infected phytoplankton cultures resulted in an increase in critical activation diameter and average molar mass in three out of five combinations evaluated, along with a decrease in organic kappa (hygroscopicity) compared to healthy cultures and seawater controls. The infected samples also displayed evidence of increased surface tension depression at realistic cloud water vapor supersaturations. Amending the samples with xanthan gum to simulate marine hydrogels increased variability in organic kappa and surface tension in aerosols with high organic to salt ratios. Our findings suggest that the pulses of increased dissolved organic matter associated with viral infection in surface waters may increase the molar mass of dissolved organic compounds relative to surface waters occupied by healthy phytoplankton or low phytoplankton biomass.
Atmospheric science↗
Fundamental Science Achievable with a Single Atmospheric Probe
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Kathleen E. Mandt↗
Observations Suggest That North African Dust Absorbs Less Solar Radiation Than Models Estimate
Desert dust accounts for a large fraction of shortwave radiation absorbed by aerosols, which adds to the climate warming produced by greenhouse gases. However, it remains uncertain exactly how much shortwave radiation dust absorbs. Here, we leverage in-situ measurements of dust single-scattering albedo to constrain absorption at mid-visible wavelength by North African dust, which accounts for approximately half of the global dust. We find that climate and chemical transport models overestimate North African dust absorption aerosol optical depth (AAOD) by up to a factor of two. This occurs primarily because models overestimate the dust imaginary refractive index, the effect of which is partially masked by an underestimation of large dust particles. Similar factors might contribute to an overestimation of AAOD retrieved by the Aerosol Robotic Network, which is commonly used to evaluate climate and chemical transport models. The overestimation of dust absorption by models could lead to substantial biases in simulated dust impacts on the Earth system, including warm biases in dust radiative effects.
Atmospheric science↗
Validation of OMPS LP Ozone Profile Retrievals Using Solar Occultation Satellite Measurements
The OMPS Limb Profiler (OMPS LP) satellite instrument, launched in October 2011, performs limb measurements of scattered solar radiation in the ultraviolet and visible wavelengths, which allow for the retrieval of ozone profiles from the top of clouds up to 55km. In this study we utilize ozone retrievals from two solar occultation satellite instruments, SAGE III/ISS and ACE-FTS, to validate OMPS LP profile measurements processed with the new NASA GSFC version 2.6 retrieval algorithm. OMPS LP started operational observations in April 2012, whereas ACE-FTS observations started in February 2004, therefore, there are currently 12 years of data overlap to exploit for validation. SAGE III/ISS observations started in June 2017, which provides 7 years of data overlap with OMPS LP. The OMPS LP is a solar scattering instrument that makes observations in the sunlit portion of the Earth, whilst ACE-FTS and SAGE III/ISS are solar occultation instruments that measure ozone only at sunrise and sunset. To account for these differences in measurement times we use the Goddard Diurnal Ozone Climatology (GDOC). Diurnal adjustments using this climatology have been shown to help reduce biases above 30 km. Our analysis shows that biases between OMPS LP v2.6, ACE-FTS, and SAGE III/ISS are <10% between 18 and 45 km, and increase above and below these altitudes, which are comparable to the previous version of OMPS LP ozone retrievals (v2.5). The vertical patterns of the differences are similar across different latitudes and seasons, with larger seasonal variations observed in the Northern Hemisphere.
Atmospheric Science↗
Comparisons of ozone profile retrievals from the OMPS Limb Profiler and ACE-FTS
The OMPS Limb Profiler (OMPS LP) was launched in October 2011, and has more than 10 years of overlap with ACE-FTS. Therefore, ACE-FTS offers an excellent opportunity to obtain independent ozone profile data with which to validate OMPS LP ozone retrievals. In this study we utilize ACE-FTS ozone retrievals to evaluate 10 years of OMPS LP profile measurements processed with the new NASA GSFC version 2.6 retrieval algorithm. The OMPS LP is a solar scattering instrument that makes observations in the sunlit portion of the Earth, whilst ACE-FTS is a solar occultation instrument that measures ozone only at sunrise and sunset. To account for these differences in measurement times we use the Goddard Diurnal Ozone Climatology (GDOC). Diurnal adjustments using this climatology have been shown to help reduce biases above 30 km. Our analysis shows that biases between OMPS LP v2.6 and ACE-FTS v5.2 are <10% between 18 and 45 km, and increase above and below these altitudes. The vertical patterns of the differences are similar across different latitudes and seasons, with larger seasonal variations observed in the Northern Hemisphere. We also analyze ozone time series from the two instruments.
Atmospheric Science, Stratospheric Ozone↗