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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Electron-hole asymmetry in the phase diagram of carrier-tuned CsV3Sb5

In this work, we study the effect of electron doping on the kagome superconductor CsV 3 Sb 5 . Single crystals and powders of CsV 3 Sb 5− x Te x are synthesized and characterized via magnetic susceptibility, nuclear quadrupole resonance, and x-ray diffraction measurements, where we observe a slight suppression of the charge density wave transition temperature and superconducting temperature with the introduction of electron dopants. In contrast to hole doping, both transitions survive relatively unperturbed up to the solubility limit of Te within the lattice. A comparison is presented between the electronic phase diagrams of electron- and hole-tuned CsV 3 Sb 5 .

36 MATERIALS SCIENCE↗
DOE OSTI2026

Optics and Systems Design of the Ring-to-Second Target Transport Beam-Line for the SNS Second Target Station

The Second Target Station (STS) project at the Spallation Neutron Source (SNS) is being developed to provide world-leading cold neutron brightness for next-generation neutron scattering experiments. The STS Accelerator Systems (AS) scope includes the design and implementation of the Ring-to-Second Target (RTST) proton beam transport line, which extracts 1.3 GeV proton beam pulses from the existing Ring-to-Beam Transport (RTBT) system and delivers them to the STS target. The RTST design emphasizes operational reliability [high reliability], low activation [minimum activation of components and the tunnel], maintainability, and compatibility with existing SNS infrastructure through extensive reuse of proven RTBT systems and components. The beamline includes a new extraction region, a transport lattice consisting of dipole, quadrupole, and corrector magnets, beam instrumentation systems, vacuum systems, personnel protection systems, and radiation shielding systems. Beam optics and particle tracking studies were performed using PyORBIT to validate extraction trajectories, beam transport, and target beam spot requirements [60–90 cm² beam spot area]. This paper presents the optics design philosophy, extraction system architecture, transport lattice design, instrumentation strategy, vacuum system approach, and radiation protection integration for the RTST beamline. Particle tracking simulations indicate successful beam transport without beam loss under nominal operating conditions. The RTST is designed to transport 1.3 GeV proton beam pulses at repetition rates up to 15 Hz, delivering nominal beam power of 700 kW to the Second Target Station.

Baron, Alex [ORNL]↗
DOE OSTI2026

High-Resolution Laser Spectroscopy on the Hyperfine Structure of 255Fm (𝑍=100)

We report on high-resolution laser spectroscopy of 255Fm (𝑇1/2=20 h), one of the heaviest nuclides available from reactor breeding. The hyperfine structures in two different atomic ground-state transitions at 398.4 nm and 398.2 nm were probed by in-source laser spectroscopy at the RISIKO mass separator in Mainz, using the perpendicularly illuminated laser ion source and trap (PI-LIST) high-resolution ion source. Experimental results were combined with hyperfine fields from various atomic ab initio calculations, in particular using multiconfiguration Dirac-Hartree-Fock theory, as implemented in grasp18. In this manner, the nuclear magnetic dipole and electric quadrupole moments were derived to be 𝜇=−0.75⁢(5) 𝜇N and 𝑄s=+5.84⁢(13) eb, respectively. The magnetic moment indicates occupation of the 𝜈⁢7/2⁢[613] Nilsson orbital, while the large quadrupole moment confirms strong, stable prolate deformation consistent with systematics in the heavy actinides. Comparisons with available expectation values from nuclear theory show good agreement, providing a stringent benchmark for the used theoretical models. These results revise earlier data and establish 255Fm as a reference isotope for future high-resolution studies.

Ezold, Julie [ORNL] (ORCID:0000000250550022)↗
DOE OSTI2023

Exploring the Focusing Mechanism of the NuMI Horn Magnets

Neutrinos at the Main Injector (NuMI) is a project at Fermilab that provides an intense beam of neutrinos used by a number of experiments. NuMI creates a beam of pions that decay into neutrinos, muons, and other particles. Muons are registered by the muon monitors. Magnetic horns are the key elements of the NuMI beam line. This paper uses the muon beam profile observed at the muon monitors to study the NuMI horn focusing mechanism. It is found that the horn magnet generates dipole and quadrupole fields to focus pions. This suggests that the optics of the horn magnet are predominantly linear. Our study shows that the muon beam profile accurately detects the horn current within 0.05%.

43 PARTICLE ACCELERATORS↗
DOE OSTI2021

Magnetic Field Measurements of First Pre-series Full -Length 4.2 m Quadrupole MQXFA03 Using PCB Rotating Coils for the Hi Hi-Lumi LHC Project

The U.S. Hi-Lumi LHC Accelerator Upgrade Project (AUP) and CERN have joined efforts to develop high field quad-rupoles for the Hi-Lumi LHC upgrade. The US national laborato-ries in the AUP project will deliver 10 magnets and each cryostat has two 4.2 m high gradient quadrupoles in it. These magnets are made of Nb3Sn conductors, with large aperture (150 mm) and in-tegrated gradient of 556.9 T. This paper reports on magnetic measurements performed during the vertical test at Brookhaven National Laboratory (BNL) in 2019-2020. A warm measurement Z-Scan (+/- 15 A) with 42 Z-positions before cool-down was per-formed at BNL. The results were directly compared to field data measured at LBNL during magnet assembly. Measured harmonics and magnetic center offsets (ΔX and ΔY) have provided timely and informative diagnostics on the magnet structure’s shape at both warm and cold temperatures. A new centering fixture was de-signed and added to better center the warm bore tube which con-tains the rotating coil probe. After the quench training to 16.47 kA was achieved, a complete set of cold measurements (Z-Scan at 16.47 kA and I-Scan from 960 A to 16.47 kA and back to 960 A) was made. Periodic axial variation of allowed and nonallowed harmonics was observed which is related to the coil radial and/or mid-plane variations along the magnet axis. Overall, the average harmonics in the straight section are within the required field boundaries.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Left-right canted-cosine-theta magnets

Disclosed herein are superconducting gantry magnets that include multiple quadrupole winding sections placed in sequence on a curve such that the effective current direction is reversed between sections. This produces alternating quadrupole field regions along the length of the bend whose individual integral strengths can be tuned by the location of the current polarity transitions. A simple transition scheme to reverse the current between sections can be implemented to allow for the use of one continuous winding and power supply. Dipole windings can be included in the superconducting gantry magnets so that the magnets produce superposed dipole and alternating quadrupole fields. The disclosed design for the windings and transition scheme to reverse current polarity can be implemented for higher order multipoles as well.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

Charge radii and electromagnetic moments of 214−218 Bi : Exploring the “southern” border of the 𝑍 > 82 octupole-deformation region

The changes in the mean-squared charge radii relative to 209 Bi 126 (𝛿⁢⟨𝑟 2 ⟩ 𝑁,126 ) and the magnetic dipole and electric quadrupole moments in 214−218 Bi have been measured using the in-source resonance-ionization spectroscopy technique at ISOLDE (CERN). Magnetic moments of odd-odd bismuth nuclei have been analyzed by the additivity relation. Previous tentative spin-parity and configuration assignments based on the 𝛽-decay feeding patterns have been supported. A normal odd-even staggering in charge radii of bismuth isotopes with 𝑁>126 has been observed. The new data for the 𝛿⁡⟨𝑟 2 ⟩ of bismuth isotopes allow a study of the isotonic dependencies in the charge radii, revealing jumps in 𝛿⁢⟨𝑟 2 ⟩ 132,126 and 𝛿⁢⟨𝑟 2 ⟩ 134,126 at 𝑍 = 84. This pattern could be explained by a sudden onset of octupole deformation at 𝑁 = 132 and 134 when going from polonium (𝑍 = 84) to astatine (𝑍 = 85).

fundamental symmetries↗
DOE OSTI2020

Test Results of Fast Decaying Current-Induced AC Losses in SHMS Superconducting Magnets at Jefferson Lab

The 11 GeV Super High Momentum Spectrometer (SHMS) of Hall C, part of the recent 12 GeV accelerator Upgrade at Jefferson Lab, was successfully commissioned in 2017. Fast current discharges of the SHMS Q2, Q3 quadrupoles and dipole superconducting magnets experienced some level of operational difficulty, during commissioning and normal operation. Measurements and analyses demonstrate that the fast current discharge leads to substantial AC losses in the conductor and subsequently triggers a quench-back effect. The details of the measurements and analyses have been reported previously. This paper focuses on the test results of the magnets using a reduced value of the protection dump resistor for each magnet to lower the current decay rate. Finally, the test results confirmed that the reduced dump resistances eliminated the quench-back effect for the SHMS Q2, Q3 and Dipole magnets, thus improving their cryogenic operability.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Achromat Design for Multi-Pulse Test Line

This note describes the design of a 90° achromatic bend on DARHT Axis 2 to support multi-pulse target studies. The achromatic bend consists of two 45° dipole magnets with a focusing quadrupole centered between the dipoles. The optical design of the achromat is described followed by a discussion of the sensitivity to space charge and variations in the beam energy. The preliminary design of the magnets is then described with a description of the electro-mechanical parameters.

42 ENGINEERING↗
DOE OSTI2020

Hyperfine and quadrupole interactions for Dy isotopes in DyPc 2 molecules

Nuclear spin levels play a vital role in understanding magnetization dynamics and implementation and control of quantum bits in lanthanide-based single-molecule magnets. We investigate the hyperfine and nuclear quadrupole interactions for 161 Dy and 163 Dy nuclei in anionic DyPc 2 (Pc=phthalocyanine) single-molecule magnets, using multiconfigurational ab initio methods (beyond density-functional theory) including spin–orbit interaction. The two isotopes of Dy are chosen because the others have zero nuclear spin. Both isotopes have the nuclear spin I =5/2, although the magnitude and sign of the nuclear magnetic moment differ from each other. The large energy gap between the electronic ground and first-excited Kramers doublets, allows us to map the microscopic hyperfine and quadrupole interaction Hamiltonian onto an effective Hamiltonian with an electronic pseudo-spin that corresponds to the ground Kramers doublet. Our ab initio calculations illustrate that the coupling between the nuclear spin and electronic orbital angular momentum contributes the most to the hyperfine interaction and that both the hyperfine and nuclear quadrupole interactions for 161 Dy and 163 Dy nuclei are much smaller than those for the 159 Tb nucleus in TbPc 2 single-molecule magnets. The calculated separations of the electronic-nuclear levels are comparable to experimental data reported for 163 DyPc 2 . We demonstrate that hyperfine interaction for the Dy Kramers ion leads to tunnel splitting (or quantum tunneling of magnetization) at zero field. This effect does not occur for TbPc 2 single-molecule magnets. The magnetic field values of the avoided level crossings for 161 DyPc 2 and 163 DyPc 2 are found to be noticeably different, which can be observed from the experiment.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Competing Electronic Ground States in the Heavy-Fermion Superconductor CeRh 2 As 2

CeRh 2 ⁢As 2 is rare among superconductors, in that the magnetic field tunes it between two distinct superconducting phases. Combined with a lack of local inversion symmetry and an upper critical field exceeding the Pauli paramagnetic limit, this excitingly suggests triplet multicomponent superconductivity. Preceding the superconducting onset, 𝑓-electron correlations cause long-range order, attributed both to local antiferromagnetism and itinerant (quadrupole) density waves. A magnetic field provides a significant perturbation of the 𝑓 electrons and may reveal the nature of the many-body correlations. Therefore, we report comprehensive magnetization and magnetotransport studies on microstructured devices in fields of up to 73 T. Applied along the 𝑐 axis, the field causes a low-temperature change of majority (hole) carrier density at 𝜇 0⁢ 𝐻 ≈ 2⁢4 T. By contrast, in-plane fields produce a cascade of phase transitions; the field-induced in-plane conductivity anisotropy and lack of accompanying magnetic features, plus the closed-dome nature of the overall phase boundary is consistent with a hierarchy of field-induced density-wave states.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Ferrimagnetism in EuFe 4 As 12 revealed by 153 Eu NMR and 75 As NQR measurements

Filled skutterudite compound EuFe 4 As 12 shows the highest magnetic ordering temperature of T C =154K among Eu-based skutterudite compounds, but its magnetic ground state has not been determined yet. In this study, we performed 153 Eu nuclear magnetic resonance (NMR) and 75 As nuclear quadrupole resonance (NQR) measurements on EuFe 4 As 12 to reveal its magnetic ground state as well as the physical properties from a microscopic point of view. From the temperature and magnetic field dependence of 153 Eu NMR spectrum in the magnetically ordered state, we found that the Eu ions are in Eu 2+ state with a nearly 7 μB corresponding to S=7/2 spins. Combined with the magnetization measurements, which show the reduced saturation moments of 4.5 μB/f.u., we determined the ground magnetic structure in EuFe 4 As 12 to be ferrimagnetic where the Eu 2+ 4f and the Fe 3d ordered moments are ferromagnetically aligned in each sublattice but the moments between the sublattices are antiferromagnetically aligned. We also found the local distortion at the Eu site from the cubic symmetry in the magnetically ordered state. The relationship between the rattling motion of Eu atoms and the local symmetry of the Eu ions is discussed. From the 75 As NQR nuclear spin-lattice relaxation time measurements as well as 153 Eu NMR measurements, we found that the 4f electrons of the Eu ions are well described by the local moment picture in both the magnetic and paramagnetic metallic states.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Calorimetric measurement of nuclear spin-lattice relaxation rate in metals

The quasiparticle density of states in correlated and quantum-critical metals directly probes the effect of electronic correlations on the Fermi surface. Measurements of the nuclear spin-lattice relaxation rate provide one such experimental probe of quasiparticle mass through the electronic density of states. By far the most common way of accessing the spin-lattice relaxation rate is via nuclear magnetic resonance and nuclear quadrupole resonance experiments, which require resonant excitation of nuclear spin transitions. Here we report nonresonant access to spin-lattice relaxation dynamics in AC-calorimetric measurements. The nuclear spin-lattice relaxation rate is inferred in our measurements from its effect on the frequency dispersion of the thermal response of the calorimeter-sample assembly. Further, we use fast, lithographically defined nanocalorimeters to access the nuclear spin-lattice relaxation times in metallic indium from 0.3 to 7 K and in magnetic fields up to 35 T.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2026

Status of 22 GeV CEBAF Upgrade Using FFA Arcs

Jefferson Lab is exploring an upgrade to extend CEBAF’s energy to ~22 GeV within the existing tunnel by incorporating Fixed-Field Alternating-Gradient (FFA) arcs. In this scheme, the two lowest-energy electromagnetic arcs are removed, the remaining arcs are reassigned to lower energies, and a new pair of high-energy FFA arcs enables six additional recirculations using the existing SRF linacs. The non-scaling FFA lattice employs Halbach-derived permanent magnets with provisions for dipole, quadrupole, and higher-order components, offering large momentum acceptance and reduced operating cost. Implementing this concept requires updated linac optics, modifications to the remaining arcs, and a redesigned electromagnetic switchyard. Ongoing beam-dynamics studies address synchrotron-radiation–induced energy loss and emittance growth, along with strategies for their mitigation.

Ogur, S. [Thomas Jefferson National Accelerator Fa↗
DOE OSTI2025

Electromagnetic moments of 215,217 Bi: Probing shell evolution beyond N = 126

The nuclear properties of bismuth isotopes (Z = 83) , with just one valence proton above the closed spherical shell at (Z = 82) , are expected to be governed by a single unpaired proton. However, already in semimagic 209 Bi (Z = 83, N = 126) , , the magnetic moment (μ) strongly deviates from the single-particle Schmidt value. A near linear decrease in μ with the increase of N after the N = 126 magic number was observed up to N = 130 . In order to test whether this trend is kept at N > 130 and to reveal the underlying mechanisms, an investigation of 215,217 Bi (N = 132, 134) has been undertaken. The magnetic dipole and electric quadrupole moments of the I π = 9/2 - nuclear ground states in these isotopes have been measured for the first time using the in-source resonance-ionization spectroscopy technique at ISOLDE (CERN). It has been shown that the linearly decreasing trend of μ( 209,211,213 Bi g ) is broken in 215,217 Bi with a nearly constant value of μ observed. Experimental data have been compared to calculations in the framework of the configuration-interaction shell model with the monopole-based universal V MU +LS interaction. The peculiarities in the behavior of μ(Bi, 9/2 - ) with increasing neutron number are explained as being due to the shell evolution, change of the neutron orbitals occupancies and strong configuration mixing beyond N = 130 . Also, the difference in the μ trends for bismuth (Z = 83) and astatine (Z = 85) isotopes with N > 126 are reproduced by the shell-model calculations. It is shown that monopole interaction plays noticeable role in the description of the peculiarities of the μ behaviour. Additionally, the extension of the application of the V MU interaction to the μ isotopic trends for heavy nuclei is important for further study of the capabilities of this promising version of the shell-model calculations.

Dipole magnetic moments↗
DOE OSTI2022

Laser spectroscopy for the study of exotic nuclei

Investigation into the properties and structure of unstable nuclei far from stability is a key avenue of research in modern nuclear physics. These efforts are motivated by the continual observation of unexpected structure phenomena in nuclei with unusual proton-to-neutron ratios. In recent decades, laser spectroscopy techniques have made significant contributions in our understanding of exotic nuclei in different mass regions encompassing almost the entire nuclear chart. This is achieved through determining multiple fundamental properties of nuclear ground and isomeric states, such as nuclear spins, magnetic dipole and electric quadrupole moments and charge radii, via the measurement of hyperfine structures and isotope shifts in the atomic or ionic spectra of the nuclei of interest. These properties offer prominent tests of recently developed state-of-the-art nuclear theory and help to stimulate new developments in improving the many-body methods and nucleon–nucleon interactions at the core of these models. With the aim of exploring more exotic short-lived nuclei located ever closer to the proton and neutron driplines, laser spectroscopy techniques, with their continuous technological developments towards higher resolution and higher sensitivity, are extensively employed at current- and next-generation radioactive ion beam facilities worldwide. Ongoing efforts in parallel promise to improve the availability of these even more exotic species at next-generation facilities. Very recently, an innovative application of laser spectroscopy on molecules containing short-lived nuclei has been demonstrated offering additional opportunities for several fields of research, e.g. fundamental symmetry studies and astrophysics. Here, in this review, the basic nuclear properties measurable with laser spectroscopy will be introduced. How these observables are associated with nuclear structure and nucleon–nucleon interactions will be discussed. Following this, a general overview of different laser spectroscopy methods will be given with particular emphasis on technical advancements reported in recent years. The main focus of this article is to review the numerous highlights that have resulted from studying exotic nuclei in different mass regions with laser spectroscopy techniques since the last edition in this series. Finally, the challenges facing the field in addition to future opportunities will be discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Intrinsic operators for the translationally-invariant many-body problem

Abstract The need to enforce fermionic antisymmetry in the nuclear many-body problem commonly requires use of single-particle coordinates, defined relative to some fixed origin. To obtain physical operators which nonetheless act on the nuclear many-body system in a Galilean-invariant fashion, thereby avoiding spurious center-of-mass contributions to observables, it is necessary to express these operators with respect to the translational intrinsic frame. Several commonly-encountered operators in nuclear many-body calculations, including the magnetic dipole and electric quadrupole operators (in the impulse approximation) and generators of U(3) and Sp ( 3 , R ) symmetry groups, are bilinear in the coordinates and momenta of the nucleons and, when expressed in intrinsic form, become two-body operators. To work with such operators in a second-quantized many-body calculation, it is necessary to relate three distinct forms: the defining intrinsic-frame expression, an explicitly two-body expression in terms of two-particle relative coordinates, and a decomposition into one-body and separable two-body parts. We establish the relations between these forms, for general (non-scalar and non-isoscalar) operators bilinear in coordinates and momenta.

Physics↗
DOE OSTI2022

Experimental study of the Si 30 ( He 3 , d ) P 31 reaction and thermonuclear reaction rate of Si 30 ( p , γ ) P 31

Background: Abundance anomalies in some globular clusters, such as the enhancement of potassium and the depletion of magnesium, can be explained in terms of an earlier generation of stars polluting the presently observed ones. It was shown that the potential range of temperatures and densities of the polluting sites depends on the strength of a few critical reaction rates. The 30 Si(p,γ) 31 P reaction has been identified as one of these important reactions. Purpose: The key ingredient for evaluating the thermonuclear 30 Si(p,γ) 31 P reaction rate is the strength of the resonances which, at low energy, are proportional to their proton width. Therefore, the goal of this work is to determine the proton widths of unbound 31 P states. Method: States in 31 P were studied at the Maier-Leibnitz-Laboratorium using the one-proton 30 Si( 3 He,d) 31 P transfer reaction. Deuterons were detected with the high resolution one quadrupole three dipoles (Q3D) magnetic spectrometer. Angular distribution and spectroscopic factors were extracted for 27 states, and proton widths and resonance strengths were calculated for the unbound states. Results: Several 31 P unbound states have been observed for the first time in a one-proton transfer reaction. Above 20 MK, the 30 Si(p,γ) 31 P reaction rate is now entirely estimated from the observed properties of 31 P states. The reaction rate uncertainty from all resonances other than the E$^{c.m.}_{r}$ = 149 keV resonance has been reduced down to less than a factor of 2 above that temperature. The unknown spin and parity of the E$^{c.m.}_{r}$ = 149 keV resonance dominates the uncertainty in the rate in the relevant temperature range. Conclusion: Here, the remaining source of uncertainty on the 30 Si(p,γ) 31 P reaction rate comes from the unknown spin and parity of the E$^{c.m.}_{r}$ = 149 keV resonance which can change the reaction rate by a factor of 10 in the temperature range of interest.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗