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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Selective Detection in Impulsive Low-Frequency Raman Imaging Using Shaped Probe Pulses

Impulsive stimulated Raman scattering (ISRS) using a single short femtosecond pump pulse to excite molecular vibrations offers an elegant pump-probe approach to perform vibrational imaging below 200 cm –1 . One shortcoming of ISRS is its inability to offer vibrational selectivity as all the vibrational bonds whose frequencies lie within the short pump-pulse bandwidth are excited. To date, several coherent control techniques have been explored to address this issue and selectively excite a specific molecular vibration by shaping the pump pulse. There has not been any systematic work that reports an analogous shaping of the probe pulse to implement preferential detection. In this work, we focus on vibrational imaging and report vibrational selective detection by shaping the probe pulse in time. Here, we demonstrate numerically and experimentally two pulse-shaping strategies with one functioning as a vibrational notch filter and the other functioning as a vibrational low-pass filter. This enables fast (25 μs/pixel) and selective hyperspectral imaging in the low-frequency regime (< 200 cm –1 ).

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS2003

Energy Scales in X-Ray Microcalorimeters

Microcalorimeter pulse shape characteristics, such as pulse height, decay time and rise time, are dependent on the detector temperature and bias as well as the photon energy and flux. We examine the nature of the temperature dependency by illuminating the ASTRO-E2 X-ray Spectrometer (XRS) microcalorimeter array with X-rays generated by electron impact on a range of foil targets. The resulting pulses are collected for a range of detector temperatures. We observe and model the temperature dependence of the pulse shape characteristics by fitting the data with non-linear pulse models. Our aim is to determine a robust method for correcting the energy scale obtained in ground calibration for slight differences in the operating conditions while in orbit.

Tillotson, W. A.↗
DOE OSTI2024

Determining Key Factors for the Open-Loop Control of Molecular Fragmentation Using Shaped Strong Fields

Pulse shaping has long been employed for tailoring femtosecond laser pulses to study and control the fragmentation of polyatomic molecules. In many cases, a physical explanation connecting the properties of the field to the observed control is difficult to ascertain. We utilized 80 bit binary spectral phase functions to parametrize and map the search space, gaining insight into which pulse parameters most impact the ion yield and fragmentation pattern for the relatively large triethylamine [N(C 2 H 5 ) 3 ] molecule. Pulse structures used to control the m/z 86 branching ratio beyond a simple intensity dependence are identified and compared to pump–probe results. All of these findings are explained in terms of control via a dissociative Rydberg state in the neutral molecule. This methodology may be used to discover new control mechanisms and shed light onto which pulse parameters most influence the interaction between strong field lasers and matter.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1993

Every Good Virtue You Ever Wanted in a Q-switched Solid-state Laser and More: Monolithic, Diode-pumped, Self-q-switched, Highly Reproducible, Diffraction-limited Nd:yag Laser

The applications of Q-switched lasers are well known, for example, laser radar, laser remote sensing, satellite orbit determination, Moon orbit and 'moon quake' determination, satellite laser communication, and many nonlinear optics applications. Most of the applications require additional properties of the Q-switched lasers, such as single-axial and/or single-transverse mode, high repetition rate, stable pulse shape and pulse width, or ultra compact and rugged oscillators. Furthermore, space based and airborne lasers for lidar and laser communication applications require efficient, compact, lightweight, long-lived, and stable-pulsed laser sources. Diode-pumped solid-state lasers (DPSSL) have recently shown the potential for satisfying all of these requirements. We will report on the operating characteristics of a diode-pumped, monolithic, self-Q-switched Cr,Nd:YAG laser where the chromium ions act as a saturable absorber for the laser emission at 1064 nm. The pulse duration is 3.5 ns and the output is highly polarized with an extinction ratio of 700:1. It is further shown that the output is single-longitudinal-mode with transform-limited spectral line width without pulse-to-pulse mode competition. Consequently, the pulse-to-pulse intensity fluctuation is less than the instrument resolution of 0.25 percent. This self-stabilization mechanism is because the lasing mode bleaches the distributed absorber and establishes a gain-loss grating similar to that used in the distributed feedback semiconductor lasers. A repetition rate above 5 KHz has also been demonstrated. For higher power, this laser can be used for injection seeding an amplifier (or amplifier chain) or injection locking of a power oscillator pumped by diode lasers. We will discuss some research directions on the master oscillator for higher output energy per pulse as well as how to scale the output power of the diode-pumped amplifier(s) to multi-kilowatt average power.

Chen, Y. C.↗
NASA NTRS1975

Spectral characteristics of digital phase-modulated signals

The power spectral density of two-level digital phase modulated signals is determined using various polar pulse shaping functions, the only restriction being that the pulses are independent and do not overlap. Rectangular pulses and pulses having finite rise and decay times are considered. It is shown that a substantial improvement in terms of minimizing spectral occupancy on a power basis over a given frequency band can be achieved by using linear and raised cosine pulse shaping functions. Further, the rate of decrease of the power spectral density is given for the asymptotic limit as f goes to infinity. The use of these and possibly other well chosen pulse shaping functions can then provide an additional aid to overall efficient spectrum utilization and management.

Mcgregor, D. N.↗
DOE OSTI2025

A monolithic antineutrino detector for non-intrusive reactor monitoring

Recent advances in organic detection media have found applications in reactor antineutrino physics. One example is the Precision Oscillation and Spectrum Experiment (PROSPECT), which leveraged pulse-shape sensitivity to enable a successful surface deployment at the High Flux Isotope Reactor (HFIR), achieving a signal to background of 4:1. PROSPECT utilized almost 4 tonnes of 6 Li-doped pulse-shape sensitive liquid scintillator in a two-dimensional segmented array. It used a combination of pulse-shape sensitivity and position sensitivity via segmentation to reduce the most prominent form of correlated background for surface detectors — cosmogenic fast neutrons. These new liquids may enable detector designs that bring additional tools for reducing backgrounds while reducing engineering complexity. In this paper, we present an investigation into a detector design that exploits properties of these liquids by maximizing spectral and pulse-shape sensitivity via highly efficient photon detection. The detector utilizes photomultiplier tubes (PMTs) placed at the top and bottom of a right cylinder, with highly reflective white walls. This design sacrifices some position sensitivity for maximal photon efficiency. In conclusion, the design choice has consequences for the identification of the background and antineutrino sensitivity, which we examine.

Pulse shape↗
NASA NTRS2022

X-Ray Burst and Persistent Emission Properties of the Magnetar SGR 1830-0645 in Outburst

We report on NICER X-ray monitoring of the magnetar SGR 1830−0645 covering 223 days following its 2020 October outburst, as well as Chandra and radio observations. We present the most accurate spin ephemerides of the source so far: ν = 0.096008680(2) Hz, $\dot{\n𝜈}=-6.2(1) x (10)^(-14) Hz/s, and significant second and third frequency derivative terms indicative of nonnegligible timing noise. The phase-averaged 0.8–7 keV spectrum is well fit with a double-blackbody (BB) model throughout the campaign. The BB temperatures remain constant at 0.46 and 1.2 keV. The areas and flux of each component decreased by a factor of 6, initially through a steep decay trend lasting about 46 days, followed by a shallow long-term one. The pulse shape in the same energy range is initially complex, exhibiting three distinct peaks, yet with clear continuous evolution throughout the outburst toward a simpler, single-pulse shape. The rms pulsed fraction is high and increases from about 40% to 50%. We find no dependence of pulse shape or fraction on energy. These results suggest that multiple hot spots, possibly possessing temperature gradients, emerged at outburst onset and shrank as the outburst decayed. We detect 84 faint bursts with NICER, having a strong preference for occurring close to the surface emission pulse maximum—the first time this phenomenon is detected in such a large burst sample. This likely implies a very low altitude for the burst emission region and a triggering mechanism connected to the surface active zone. Finally, our radio observations at several epochs and multiple frequencies reveal no evidence of pulsed or burst-like radio emission.

George Younes↗
DOE OSTI2020

Robust control of the minima of high-order harmonics by fine-tuning the alignment of CO 2 molecules for shaping attosecond pulses and probing molecular alignment

In a recent paper, we reported that the position and depth of the minima in the harmonic spectra of CO 2 molecules can be dramatically manipulated by a slight change of the degree of alignment, thus providing a convenient method of shaping attosecond pulses which could lead to the splitting of a typical single attosecond burst into two. Here, we demonstrate that harmonic minima can also be dramatically controlled by changing the pump-probe angles to shape attosecond pulses. In the meanwhile, since the pump-probe angle-dependent harmonic spectra are very sensitive to the degree of alignment, harmonic spectra can also be used to calibrate the alignment distribution of molecules. In this work we identify such robust control of harmonic generation is due to the optical property of CO 2 and the coherent harmonic emission from the oriented molecules. The photoionization transition dipoles (PITDs) of CO 2 exhibit deep minima that change rapidly with molecular orientations accompanied by large phase changes of π in PITDs, thus leading to strong interference when the dipoles are added up coherently.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS1978

A search for optical pulsations from GX 1+4 at H-alpha

H-alpha observations of the binary-star candidate for the slowly pulsating hard X-ray source GX 1+4 are reported which were undertaken to search for pulsations in the H-alpha flux that are synchronous with the X-ray period of about 2 min. No significant periodic variation of the candidate star was detected in the frequency band searched. Three-sigma upper limits of 1.7% (sinusoidal pulse shape) and 0.7% (X-ray pulse shape) are set for the pulsed fraction of the H-alpha flux. It is noted that because of possible diffusion from a cloud that is optically thick to Balmer radiation, the observed lack of pulsations in the H-alpha flux need not compromise the identification of GX 1+4 with the candidate star.

Krzeminski, W.↗
NASA NTRS2020

Position-Sensitive Magnetic Calorimeters for Lynx

We describe the performance of position-sensitive metallic magnetic calorimeter X-ray detectors for potential future astrophysics missions, such as Lynx. The motivation behind this is to achieve a large focal plane area by increasing the number of pixels compared to the number of readout channels (called hydra). The detector consists of a 5×5 array of gold absorbers thermally coupled to a paramagnetic sensor. Since each absorber has a different thermal link to the sensor, it generates a different pulse shape and enables discrimination of pixel position. Recently, we have been successfully able to discriminate 25 averaged pulse shapes by means of rise-time and pulse height. The measured pulse shapes and distribution agree well with the modeling results. The estimated energy resolutions based on the pulse height and noise data we measured are 2.8–3.7 eV for MnKα X-ray photons at 50 mK.

Magnetic calorimeters↗
NASA NTRS1999

35-Day Evolution of the Her X-1 Pulse Profile: Evidence for a Resolved Inner Disk Occultation of the Neutron Star

Ginga and RXTE observations have allowed an unprecedented view of the recurrent systematic pulse shape changes associated with the 35-day cycle of Her X-1, a phenomena currently unique among the known accretion-powered pulsars. We present observations of the pulse shape evolution. An explanation for the pulse evolution in terms of a freely precessing neutron star is reviewed and shown to have several major difficulties in explaining the observed pulse evolution pattern. Instead, we propose a phenomenlogical model for the pulse evolution based upon an occultation of the pulse emitting region by the tilted, inner edge of a precessing accretion disk. The systematic and repeating pulse shape changes require a resolved occultation of the pulse emission region. The observed pulse profile motivates the need for a pulsar beam consisting of a composite coaxial pencil and fan beam but the observed evolution pattern requires the fan beam to be focused around the neutron star and beamed in the antipodal direction. The spectral hardness of the pencil beam component suggests an origin at the magnetic polar cap, with the relatively softer fan beam emission produced by backscattering from within the accretion column, qualitatively consistent with several theoretical models for X-ray emission from the accretion column of an accreting neutron star.

Scott, D. Matthew↗
NASA NTRS2000

The 35 Day Evolution of the Hercules X-1 Pulse Profile: Evidence for a Resolved Inner Disk Occultation of the Neutron Star

Ginga and Rossi X-Ray Timing Explorer observations have allowed an unprecedented view of the recurrent systematic pulse shape changes associated with the 35 day cycle of Hercules X-1, a phenomenon currently unique among the known accretion-powered pulsars. We present observations of the pulse shape evolution. An explanation for the pulse evolution in terms of a freely precessing neutron star is reviewed and shown to have several major difficulties in explaining the observed pulse evolution pattern. Instead, we propose a phenomenological model for the pulse evolution based on an occultation of the pulse-emitting region by the tilted, inner edge of a precessing accretion disk. The systematic and repeating pulse shape changes require a resolved occultation of the pulse emission region. The observed pulse profile motivates the need for a pulsar beam consisting of a composite coaxial pencil and fan beam, but the observed evolution pattern requires the fan beam to be focused around the neutron star and beamed in the antipodal direction. The spectral hardness of the pencil beam component suggests an origin at the magnetic polar cap, with the relatively softer fan beam emission produced by backscattering from within the accretion column, qualitatively consistent with several theoretical models for X-ray emission from the accretion column of an accreting neutron star.

Scott, D. Matthew↗
NASA NTRS1978

A comparative study of optimum and suboptimum direct-detection laser ranging receivers

A summary of previously proposed receiver strategies for direct-detection laser ranging receivers is presented. Computer simulations are used to compare performance of candidate implementation strategies in the 1- to 100-photoelectron region. Under the condition of no background radiation, the maximum-likelihood and minimum mean-square error estimators were found to give the same performance for both bell-shaped and rectangular optical-pulse shapes. For signal energies greater than 100 photoelectrons, the root-mean-square range error is shown to decrease as Q to the -1/2 power for bell-shaped pulses and Q to the -1 power for rectangular pulses, where Q represents the average pulse energy. Of several receiver implementations presented, the matched-filter peak detector was found to be preferable. A similar configuration, using a constant-fraction discriminator, exhibited a signal-level dependent time bias.

Abshire, J. B.↗
NASA NTRS1976

Pulse analysis of acoustic emission signals

A method for the signature analysis of pulses in the frequency domain and the time domain is presented. Fourier spectrum, Fourier transfer function, shock spectrum and shock spectrum ratio are examined in the frequency domain analysis, and pulse shape deconvolution is developed for use in the time domain analysis. To demonstrate the relative sensitivity of each of the methods to small changes in the pulse shape, signatures of computer modeled systems with analytical pulses are presented. Optimization techniques are developed and used to indicate the best design parameters values for deconvolution of the pulse shape. Several experiments are presented that test the pulse signature analysis methods on different acoustic emission sources. These include acoustic emissions associated with: (1) crack propagation, (2) ball dropping on a plate, (3) spark discharge and (4) defective and good ball bearings.

Houghton, J. R.↗
NASA NTRS1977

Pulse analysis of acoustic emission signals

A method for the signature analysis of pulses in the frequency domain and the time domain is presented. Fourier spectrum, Fourier transfer function, shock spectrum and shock spectrum ratio were examined in the frequency domain analysis, and pulse shape deconvolution was developed for use in the time domain analysis. Comparisons of the relative performance of each analysis technique are made for the characterization of acoustic emission pulses recorded by a measuring system. To demonstrate the relative sensitivity of each of the methods to small changes in the pulse shape, signatures of computer modeled systems with analytical pulses are presented. Optimization techniques are developed and used to indicate the best design parameters values for deconvolution of the pulse shape. Several experiments are presented that test the pulse signature analysis methods on different acoustic emission sources. These include acoustic emissions associated with: (1) crack propagation, (2) ball dropping on a plate, (3) spark discharge and (4) defective and good ball bearings. Deconvolution of the first few micro-seconds of the pulse train are shown to be the region in which the significant signatures of the acoustic emission event are to be found.

Houghton, J. R.↗
NASA NTRS1977

Pulse analysis of acoustic emission signals

A method for the signature analysis of pulses in the frequency domain and the time domain is presented. Fourier spectrum, Fourier transfer function, shock spectrum and shock spectrum ratio were examined in the frequency domain analysis and pulse shape deconvolution was developed for use in the time domain analysis. Comparisons of the relative performance of each analysis technique are made for the characterization of acoustic emission pulses recorded by a measuring system. To demonstrate the relative sensitivity of each of the methods to small changes in the pulse shape, signatures of computer modeled systems with analytical pulses are presented. Optimization techniques are developed and used to indicate the best design parameter values for deconvolution of the pulse shape. Several experiments are presented that test the pulse signature analysis methods on different acoustic emission sources. These include acoustic emission associated with (a) crack propagation, (b) ball dropping on a plate, (c) spark discharge, and (d) defective and good ball bearings. Deconvolution of the first few micro-seconds of the pulse train is shown to be the region in which the significant signatures of the acoustic emission event are to be found.

Houghton, J. R.↗
DOE OSTI2023

Spectral shaping of an ultrafast ytterbium fiber laser via a passive intracavity optical filter: a simple and reliable route to sub-45 fs pulses

We investigate the use of passive intracavity optical filters for controlling the laser output spectrum of a polarization-mode-locked, ultrafast ytterbium fiber laser. The overall lasing bandwidth is increased or extended by strategic choice of the filter cutoff frequency. Overall laser performance, including pulse compression and intensity noise, is investigated for both shortpass and longpass filters with a range of cutoff frequencies. The intracavity filter not only shapes the output spectra, but also provides a route for overall broader bandwidths and shorter pulses in ytterbium fiber lasers. These results demonstrate that spectral shaping with a passive filter is a useful tool to routinely achieve sub-45 fs pulse durations in ytterbium fiber lasers.

Cooper, Nicholas D.↗