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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Anomalous dispersion in coupled surface plasmons and excitons

We studied dispersion in Rhodamine laser dyes in the Kretschmann geometry and found (i) multi-branch “staircase” dispersion curves in singly doped and double doped PMMA polymer, (ii) emergence of the new dispersion “fork” branch, (iii) unparallel dispersion and coupling in the mixture of two different dyes, and (iv) effect of high dye concentration on strong coupling without metal.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Tunable Work Functions in Plasmonic Metals

We have studied the effect of BITh molecules on the work functions of Ag and Au, with and without quartz lamp illumination. Silver and gold films coated with BITh molecules were fabricated and studied in reflection and Kelvin Probe experiments. The deposition of BITh films on Ag and Au reduced their work functions (in agreement with our recent study, wherein a similar reduction was caused by the deposition of a PMMA polymer). Illumination of the BITh-coated samples with a quartz lamp caused reductions in work functions by several tens of meV, which (almost) returned to their original values when the light was turned off. The characteristic time of this process (~15 min) was much shorter than that of photopolymerization (~180 min), suggesting that these two phenomena are nearly independent of each other. The effects of the Au substrates were qualitatively similar to those of the Ag substrates. Our findings pave the way to fundamental studies and applications of light–matter interactions.

BITh↗
NASA NTRS1966

Interaction of plasmons.

Nonlinear interaction between plasma oscillation normal modes in hydrodynamic approximation

WAVE INTERACTION↗
NASA NTRS1969

Surface plasmons in thin films.

Dispersion relations for surface plasma oscillations in normal metals for single and multiple films taking into account retardation effects, noting dielectric function

Economou, E. N.↗
NASA NTRS1974

Holography utilizing surface plasmon resonances

A holographic recording medium with a substrate which has a diffraction grating composed of a number of spaced line ridges on the surface is discussed. The first layer consists of a metal with a plasma wavelength shorter than that of the selected light source. A second layer, or coating, on top of the first layer consists of a thin film of photosensitive emulsion. A diagram of the device is provided. The principles of operation are explained.

Cowan, J. J.↗