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DOE OSTI2023

Model predictive control of mixing controlled compression ignition operation for low reactivity fuels

Using gasoline or other low reactivity fuels with a pilot injection or port fuel injection in a compression ignition engine has shown great potential in reducing NOx emissions while keeping high thermal efficiency compared to diesel. However, excessive combustion noise is caused by a high maximum pressure rise rate in the cylinder due to the higher fractions of premixed charge of the low-reactivity fuel. This noise can result in structural damage to engine components and as such, combustion noise limits the range of the operating parameters and makes the control of such engines challenging. In this study, a simulation environment was built up in MATLAB/Simulink leveraging a physics-based zero-dimension combustion model to capture the in-cylinder pressure time traces as well as metrics relevant to thermal efficiency and combustion noise. Here, in order to also facilitate the control of emissions, machine learning models were investigated to capture NOx emissions. A kernel-based extreme learning machine (K-ELM) performed best and had a coefficient of correlation (R-squared) of 0.998. The combustion and NOx emission models are valid for not only conventional gasoline fuel but also oxygenated alternative fuel blends at three different pilot injection strategies. In order to track key combustion metrics while keeping noise and emissions within constraints, a model predictive control (MPC) was applied for a compression ignition engine operating with a range of potential fuels and fuel injection strategies. The MPC is validated under different scenarios, including a load step change, fuel type change, and injection strategy change, with proportional–integral (PI) control as the baseline. The simulation results show that MPC reduces about 26% of ringing intensity in the transient process and 17% at the steady state for E30. Generally, MPC can optimize the overall performance through modifying the main injection timing, pilot fuel mass, and exhaust gas recirculation (EGR) fraction.

42 ENGINEERING↗

DOE OSTI2024

Measurement of the CKM angle $\gamma $ in the ${{{B} ^0} \rightarrow {D} {{K} ^{*0}}}$ channel using self-conjugate ${D} \rightarrow {{K} ^0_{\textrm{S}}} h^+ h^-$ decays

A model-independent study of $C\!P$ violation in ${{B} ^0} \rightarrow {D} {{K} ^{*0}}$ decays is presented using data corresponding to an integrated luminosity of 9 fb -1 collected by the LHCb experiment at centre-of-mass energies of $\sqrt{s}=7, \, 8$ and 13 TeV. The CKM angle $\gamma$ is determined by examining the distributions of signal decays in phase-space bins of the self-conjugate ${D} \rightarrow {{K} ^0_{\textrm{S}}} h^+ h^-$ decays, where $h = \pi , K$. Observables related to $C\!P$ violation are measured and the angle $\gamma$ is determined to be $\gamma =(49^{+ 22}_{-19})^\circ$. Measurements of the amplitude ratio and strong-phase difference between the favoured and suppressed ${B} ^0$ decays are also presented.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Multiplicity dependence of $\pi$, K, and p production in pp collisions at $\sqrt{s}$ = 13 TeV

This paper presents the measurements of π ± , K ± , p and $\bar{p}$ transverse momentum (p T ) spectra as a function of charged-particle multiplicity density in proton–proton (pp) collisions at $\sqrt{s}$ = 13TeV with the ALICE detector at the LHC. Such study allows us to isolate the center-of-mass energy dependence of light-flavour particle production. The measurements reported here cover a p T range from 0.1 to 20 GeV / c and are done in the rapidity interval | y| < 0.5. The p T -differential particle ratios exhibit an evolution with multiplicity, similar to that observed in pp collisions at $\sqrt{s}$ = 7 TeV, which is qualitatively described by some of the hydrodynamical and pQCD-inspired models discussed in this paper. Furthermore, the p T -integrated hadron-to-pion yield ratios measured in pp collisions at two different center-of-mass energies are consistent when compared at similar multiplicities. This also extends to strange and multi-strange hadrons, suggesting that, at LHC energies, particle hadrochemistry scales with particle multiplicity the same way under different collision energies and colliding systems.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS2016

The 2 Pi Charged Particles Analyzer: All-Sky Camera Concept and Development for Space Missions

Increasing the temporal resolution and instant coverage of velocity space of space plasma measurements is one of the key issues for experimentalists. Today, the top-hat plasma analyzer appears to be the favorite solution due to its relative simplicity and the possibility to extend its application by adding a mass-analysis section and an electrostatic angular scanner. Similarly, great success has been achieved in MMS mission using such multiple top-hat analyzers to achieve unprecedented temporal resolution. An instantaneous angular coverage of charged particles measurements is an alternative approach to pursuing the goal of high time resolution. This was done with 4-D Fast Omnidirectional Nonscanning Energy Mass Analyzer and, to a lesser extent, by DYMIO instruments for Mars-96 and with the Fast Imaging Plasma Spectrometer instrument for MErcury Surface, Space ENvironment, GEochemistry, and Ranging mission. In this paper we describe, along with precursors, a plasma analyzer with a 2 electrostatic mirror that was developed originally for the Phobos-Soil mission with a follow-up in the frame of the BepiColombo mission and is under development for future Russian missions. Different versions of instrument are discussed along with their advantages and drawbacks.

Vaisberg, O.↗

DOE OSTI2025

Aerosol Microphysics and Chemical Measurements at Mt. Soledad and Scripps Pier during the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) from February 2023 to February 2024 UCSD Library Collection

This dataset includes guest instrument measurements and other PI products for aerosol microphysics and chemical measurements collected at Mt. Soledad and Scripps Pier during the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) from February 2023 to February 2024. The measurements include the following instruments at Mt. Soledad: High-Resolution Time-of-Flight Aerosol Mass Spectrometer (HR-ToF-AMS, Aerodyne), Scanning Electrical Mobility Spectrometer (SEMS, Brechtel Manufacturing Inc.), Aerodynamic Particle Sizer (APS, Droplet Measurements Technologies), Single Particle Soot Photometer (SP2, Drople Measurements Technologies), Meteorological Station (WXT520, Vaisala), Ozone (Teco), and trace gas proxies (Teledyne). In addition, the analyses of particle filters collected at Mt. Soledad for three dry-diameter size cuts (<1 micron, <0.5 micron, <0.18 micron) and at Scripps Pier for one dry-diameter size cut (<1 micron) by Fourier Transform Infrared (FTIR) and X-ray Fluorescence (XRF) are reported. A differential mobility analyzer operated as a scanning mobility particle sizer (SMPS, TSI Inc.), a printed particle optical spectrometer (POPS, Grimm), and a continuous flow diffusion cloud condensation nuclei (CCN, DMT) counter provide the mobility aerosol size distribution (30-360 nm), optical size distribution (150 - 6000 nm), size-resolved CCN distribution (30-360 nm) at 0.2, 0.4, 0.6, 0.8, and 1.0% supersaturation. Measurements are reported for both sampling from an isokinetic aerosol inlet and from a Counterflow Virtual Impactor (CVI, Brechtel Manufacturing Inc.). The data are available at the following link: https://library.ucsd.edu/dc/collection/bb0898306q

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1974

Formation of O3/+/ by the reaction of metastable O2/+/ ions with O2

The high resolution of the photoionization mass spectrophotometer was utilized to resolve some doubts about the participating species in the reaction of metastable oxygen molecular ions with oxygen molecules to yield ozone ions and oxygen radicals. It is found from inspection of the appearance potential of the ozone ion that an a4 Pi-excited state is responsible for the formation of ozone near the appearance potential of these lines.

Ajello, J. M.↗

NASA NTRS1993

Report of the Meteoroid and Debris Special Investigation Group

The LDEF Meteoroid and Debris Special Investigation Group (hereafter M&D SIG) was formed to maximize the data harvest from LDEF by permitting the characterization of the meteoroid and space debris impact record of the entire satellite. Thus, our work is complementary to that of the various M&D PI's, all of whom are members of the SIG. This presentation will summarize recent results and discussions concerning five critical SIG goals: (1) classification of impactors based upon composition of residues, (2) small impact (microimpact) features, (3) impact cratering and penetration data to derive projectile sizes and masses, (4) particulate flux estimates in low-Earth orbit, and (5) the LDEF Meteoroid and Debris database.

Zolensky, Michael E.↗

DOE OSTI2023

Search for $D^{*}(2007)^{0} \rightarrow \mu ^{+} \mu ^{-}$ in $B^{-}\rightarrow \pi ^{-} \mu ^{+} \mu ^{-}$ decays

The very rare D* (2007) 0 → μ + μ – decay is searched for by analysing B – → μ + μ – decays. The analysis uses a sample of beauty mesons produced in proton–proton collisions collected with the LHCb detector between 2011 and 2018, corresponding to an integrated luminosity of 9 fb –1 . The signal signature corresponds to simultaneous peaks in the μ + μ – and π – μ + μ – invariant masses. No evidence for an excess of events over background is observed and an upper limit is set on the branching fraction of the decay at B (D* (2007) 0 → μ + μ – ) < 2.6 x 10 –8 at 90% confidence level. This is the first limit on the branching fraction of D* (2007) 0 → μ + μ – decays and the most stringent limit on D* (2007) 0 decays to leptonic final states. The analysis is the first search for a rare charm-meson decay exploiting production via beauty decays.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2020

Measurements of $\pi^-$ production in $^7$Be+$^9$Be collisions at beam momenta from 19$A$ to 150$A$GeV/$c$ in the NA61/SHINE experiment at the CERN SPS

The NA61/SHINE collaboration studies at the CERN Super Proton Synchrotron (SPS) the onset of deconfinement in hadronic matter by the measurement of particle production in collisions of nuclei with various sizes at a set of energies covering the SPS energy range. This paper presents results on inclusive double-differential spectra and mean multiplicities of $\pi^{-}$ mesons produced in the 5% most central $^7$Be + $^9$Be collisions at beam momenta of 19$A$, 30$A$, 40$A$, 75$A$ and 150$A$ GeV/$c$ obtained by the so-called $h^-$ method which does not require any particle identification. The shape of the transverse mass spectra differs from the shapes measured in central Pb + Pb collisions and inelastic p + p interactions. The normalized width of the rapidity distribution decreases with increasing collision energy and is in between the results for inelastic nucleon-nucleon and central Pb + Pb collisions. The mean multiplicity of pions per wounded nucleon in central $^7$Be + $^9$Be collisions is close to that in central Pb + Pb collisions up to 75$A$GeV/$c$. However, at the top SPS energy the result is close to the one for inelastic nucleon-nucleon interactions. The results are discussed in the context of predictions for the onset of deconfinement at the CERN SPS collision energies.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS2009

Saturn's Magnetosphere and Properties of Upstream Flow at Titan: Preliminary Results

Using Cassini Plasma Spectrometer (CAPS) Ion Mass Spectrometer (IMS) measurements, we present the ion fluid properties and its ion composition of the upstream flow for Titan's interaction with Saturn's magnetosphere. A 3D ion moments algorithm is used which is essentially model independent with only requirement is that ion flow is within the CAPS IMS 2(pi) steradian field-of-view (FOV) and that the ion 'velocity distribution function (VDF) be gyrotropic. These results cover the period from TA flyby (2004 day 300) to T22 flyby (2006 363). Cassini's in situ measurements of Saturn's magnetic field show it is stretched out into a magnetodisc configuration for Saturn Local Times (SLT) centered about midnight local time. Under those circumstances the field is confined near the equatorial plane with Titan either above or below the magnetosphere current sheet. Similar to Jupiter's outer magnetosphere where a magnetodisc configuration applies, one expects the heavy ions within Saturn's outer magnetosphere to be confined within a few degrees of the current sheet while at higher magnetic latitudes protons should dominate. We show that when Cassini is between dusk-midnight-dawn local time and spacecraft is not within the current sheet that light ions (H, 142) tend to dominate the ion composition for the upstream flow. If true, one may expect the interaction between Saturn's magnetosphere, locally devoid of heavy ions and Titan's upper atmosphere and exosphere to be significantly different from that for Voyager 1, TA and TB when heavy ions were present in the upstream flow. We also present observational evidence for Saturn's magnetosphere interaction with Titan's extended H and H2 corona which can extend approx. 1 Rs from Titan.

Sittler, E. C., Jr.↗

NASA NTRS1986

The Pegasus drive - A multi-megawatt nuclear electric propulsion system

Pegasus, a power generating system for use in space, is multimegawatt power system that would enable missions of almost any conceivable duration and scope. The Pegassus Drive is the coupling of this nuclear electric power system with a 6 MWe MPD thruster. The power system has a maximum power output of 8.5 MWe. The MPD thruster requires 6 MWe to provide spacecraft propulsion and 1.5 MWe are available for mission-specific tasks and experiments. The balance of power generated is used to operate the power system. The size and mass limitations of the STS are of prime consideration in the design of this system to allow the collapsed system to be placed in lower earth orbit by two Shuttle missions. The main system (19,120 kg) employing a shadow shield would require one launch and the balance of the four-pi shield (27,830 kg) would occupy the second launch. Development of this power system could be completed by the mid 1990's and the system available near the turn of the century.

Coomes, E. P.↗

NASA NTRS2016

Campaign 9 of the K2 Mission: Observational Parameters, Scientific Drivers, and Community Involvement for a Simultaneous Space- and Ground-based Microlensing Survey

K2ʼs Campaign 9 (K2C9) will conduct a approximately 3.7 sq. deg survey toward the Galactic bulge from 2016 April 22 through July 2 that will leverage the spatial separation between K2 and the Earth to facilitate measurement of the microlens parallax Pi(sub E) for approximately greater than 170 microlensing events. These will include several that are planetary in nature as well as many short-timescale microlensing events, which are potentially indicative of free-floating planets (FFPs). These satellite parallax measurements will in turn allow for the direct measurement of the masses of and distances to the lensing systems. In this article we provide an overview of the K2C9 space- and ground-based microlensing survey. Specifically, we detail the demographic questions that can be addressed by this program, including the frequency of FFPs and the Galactic distribution of exoplanets, the observational parameters of K2C9, and the array of resources dedicated to concurrent observations. Finally, we outline the avenues through which the larger community can become involved, and generally encourage participation in K2C9, which constitutes an important pathfinding mission and community exercise in anticipation of WFIRST.

K2s Campaign 9 (K2C9)↗

DOE OSTI2020

Isotope effects in molecular structures and electronic properties of liquid water via deep potential molecular dynamics based on the SCAN functional

Here, Feynman path-integral deep potential molecular dynamics (PI-DPMD) calculations have been employed to study both light (H 2 O) and heavy water (D 2 O) within the isothermalisobaric ensemble. In particular, the deep neural network is trained based on ab initio data obtained from the strongly constrained and appropriately normed (SCAN) exchange-correlation functional. Because of the lighter mass of hydrogen than deuteron, the properties of light water are more influenced by nuclear quantum effect than those of heavy water. Clear isotope effects are observed and analyzed in terms of hydrogen-bond structure and electronic properties of water that are closely associated with experimental observables. The molecular structures of both liquid H 2 O and D 2 O agree well with the data extracted from scattering experiments. The delicate isotope effects on radial distribution functions and angular distribution functions are well reproduced as well. Our approach demonstrates that deep neural network combined with SCAN functional based ab initio molecular dynamics provides an accurate theoretical tool for modeling water and its isotope effects.

36 MATERIALS SCIENCE↗

NASA NTRS1984

Studies of the chemistry of vibrationally and electronically excited species in planetary upper atmospheres

The vibrational distribution of O2(+) in the atmospheres of Venus and Mars was investigated to compare with analogous values in the Earth's atmosphere. The dipole moment of the Z(2) Pi sub u - X(2) Pi sub g transition of O2(+) is calculated as a function of internuclear distance. The band absorption oscillator strengths and band transition probabilities of the second negative system are derived. The vibrational distribution of O2(+) in the ionosphere of Venus is calculated for a model based on data from the Pioneer Venus neutral mass spectrometer.

Fox, J. L.↗

NASA NTRS1985

The phi-meson and Chiral-mass-meson production in heavy-ion collisions as potential probes of quark-gluon-plasma and Chiral symmetry transitions

Possibilities of observing abundances of phi mesons and narrow hadronic pairs, as results of QGP and Chiral transitions, are considered for nucleus-nucleus interactions. Kinematical requirements in forming close pairs are satisfied in K+K decays of S(975) and delta (980) mesons with small phi, and phi (91020) mesons with large PT, and in pi-pi decays of familiar resonance mesons only in a partially restored chiral symmetry. Gluon-gluon dominance in QGP can enhance phi meson production. High hadronization rates of primordial resonance mesons which form narrow hadronic pairs are not implausible. Past cosmic ray evidences of anomalous phi production and narrow pair abundances are considered.

Takahashi, Y.↗

DOE OSTI2024

Measurement of absolute branching fractions of $$ {\textrm{D}}_{\textrm{s}}^{+} $$ hadronic decays

Abstract Usinge + e − collision data collected at the BESIII detector at center-of-mass energies between 4.128 and 4.226 GeV, corresponding to an integrated luminosity of 7.33 fb −1 , we determine the absolute branching fractions of fifteen hadronic$$ {D}_s^{+} $$ D s + decays with a double-tag technique. In particular, we make precise measurements of the branching fractions$$ \mathcal{B}\left({D}_s^{+}\to {K}^{+}{K}^{-}{\pi}^{+}\right)=\left(5.49\pm 0.04\pm 0.07\right)\% $$ B D s + → K + K − π + = 5.49 ± 0.04 ± 0.07 % ,$$ \mathcal{B}\left({D}_s^{+}\to {K}_S^0{K}^{+}\right)=\left(1.50\pm 0.01\pm 0.01\right)\% $$ B D s + → K S 0 K + = 1.50 ± 0.01 ± 0.01 % and$$ \mathcal{B}\left({D}_s^{+}\to {K}^{+}{K}^{-}{\pi}^{+}{\pi}^0\right)=\left(5.50\pm 0.05\pm 0.11\right)\% $$ B D s + → K + K − π + π 0 = 5.50 ± 0.05 ± 0.11 % , where the first uncertainties are statistical and the second ones are systematic. TheCPasymmetries in these decays are also measured and all are found to be compatible with zero.

Physics↗

DOE OSTI2024

Developing Platinum-Group-Metal-Free Catalysts for Oxygen Reduction Reaction in Acid: Beyond the Single Metal Site

This project is to develop M (x) -N-C catalysts with dense multiple metal center (MMC) sites to meet the DOE 2025 activity target of 0.044 mA/cm 2 at 0.9 V IR-free ., as well as other goals such as durability. We have made important contributions to both catalyst development and fundamental understandings of the active sites in M-N-C catalysts in this project. We successfully made M (x) -N-C catalysts with some multiple metal center (MMC) sites by combining ionothermal carbonization with chemical vapor deposition (CVD). These catalysts, however, are not as active as the most active single-atom Fe-N-C catalysts made by the similar CVD process, owing likely to the low site density and the presence of inorganic Fe species such as iron carbides and nanoparticles. The most significant accomplishments we achieved in this project are: (1) we unraveled the formation pathway of Fe-N 4 sites during pyrolysis step-by-step and identified the trans-metalation mechanism, in collaboration with Deborah Myers and her colleagues at Argonne National Laboratory (ANL); (2) inspired by this finding, we pioneered the CVD synthesis of M-N-C catalysts (M = Mn, Fe, and Co), in which the Fe-N-C catalyst by CVD demonstrated an ORR activity of 33 mA/cm 2 at 0.9 V in H 2 -O 2 proton exchange membrane fuel cells (PEMFCs), very close to the ultimate goal of 35 mA/cm 2 of our project. This catalyst is the first Fe-N-C catalyst that contains only D1 sites without the D2 sites; whereas D1 and D2 sites have been always identified by Mossbauer in previous Fe-N-C catalysts. This finding helps to understand what the D1 and D2 sites are and their roles in catalyzing the ORR. (3) by improving the mass transport of the carbon matrix prior to the CVD process, the revised Fe-N-C catalyst made by CVD delivered a maximum power density of 0.53 W/cm 2 in H 2 -air PEMFCs. The improvement strategy was partly inspired by the computational modeling work by Adam Weber from LBNL, the Co-PI of this project, by developing, coding, and exercising a continuum level model of transport phenomena within a PGM-free catalyst layer. The model demonstrated that local resistances combined with limited site density of the PGM-free catalyst can result in limiting currents and poor polarization performance. The model also gave design guidance for impact of ECSA and overall catalyst-layer thickness. However, both Fe-N-C and Co-N-C catalysts developed by CVD showed poor durability in PEMFCS, in comparison with the traditional M-N-C catalysts synthesized via regular pyrolysis process. Consequently, we did not achieve the proposed durability targets. Despite so, we believe the FeNC-CVD catalysts with the poor durability and D1 sites only provides an excellent platform to understand the degradation mechanism of Fe-N-C in PEMFCs, the most important challenge in the development of M-N-C catalysts.

08 HYDROGEN↗

NASA NTRS1993

Continued investigation of LDEF's structural frame and thermal blankets by the Meteoroid and Debris Special Investigation Group

This report focuses on the data acquired by detailed examination of LDEF intercostals, 68 of which are now in possession of the Meteoroid and Debris Special Investigation Group (M&D SIG) at JSC. In addition, limited data will be presented for several small sections from the A0178 thermal control blankets that were examined/counted prior to being shipped to Principal Investigators (PI's) for scientific study. The data presented here are limited to measurements of crater and penetration-hole diameters and their frequency of occurrence which permits, yet also constrains, more model-dependent, interpretative efforts. Such efforts will focus on the conversion of crater and penetration-hole sizes to projectile diameters (and masses), on absolute particle fluxes, and on the distribution of particle-encounter velocities. These are all complex issues that presently cannot be pursued without making various assumptions which relate, in part, to crater-scaling relationships, and to assumed trajectories of natural and man-made particle populations in LEO that control the initial impact conditions.

See, Thomas H.↗