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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Unifying femtosecond and picosecond single-pulse magnetic switching in Gd-Fe-Co

Many questions are still open regarding the physical mechanisms behind the magnetic switching in Gd-Fe-Co alloys by single optical pulses. Phenomenological models suggest a femtosecond scale exchange relaxation between sublattice magnetization as the driving mechanism for switching. The recent observation of thermally induced switching in Gd-Fe-Co by using both several picosecond optical laser pulse as well as electric current pulses has questioned this previous understanding. This has raised the question of whether or not the same switching mechanics are acting at the femtosecond and picosecond scales. In this work, we aim at filling this gap in the understanding of the switching mechanisms behind thermal single-pulse switching. To that end, we have studied experimentally thermal single-pulse switching in Gd-Fe-Co alloys, for a wide range of system parameters, such as composition, laser power, and pulse duration. We provide a quantitative description of the switching dynamics using atomistic spin dynamics methods with excellent agreement between the model and our experiments across a wide range of parameters and timescales, ranging from femtoseconds to picoseconds. Furthermore, we find distinct element-specific damping parameters as a key ingredient for switching with long picosecond pulses and argue that switching with pulse durations as long as 15 ps is possible due to a low damping constant of Gd. Our findings can be easily extended to speed up dynamics in other contexts where ferrimagnetic Gd-Fe-Co alloys have been already demonstrated to show fast and energy-efficient processes, e.g., domain-wall motion in a track and spin-orbit torque switching in spintronics devices.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Ultrafast electron dynamics in platinum and gold thin films driven by optical and terahertz fields

Here, we investigate the ultrafast electron dynamics triggered by terahertz and optical pulses in thin platinum and gold films by probing their transient optical reflectivity. The response of the platinum film to an intense terahertz pulse is similar to the optically induced one and can be described by a two-temperature model with a 20% larger electron–phonon coupling for the terahertz-driven dynamics compared to the optically induced one, ascribed to an additional nonthermal electron–phonon coupling contribution. Surprisingly, gold films exhibit a much smaller terahertz pulse-induced reflectivity change and with a sign opposite to the optical case. Additionally we explain this remarkable observation with field emission of electrons due to Fowler–Nordheim tunneling, enabled in samples with thicknesses below the structural percolation threshold, where nanostructuring promotes near-field enhancement. Our results provide a fundamental insight into the ultrafast processes relevant to modern electro- and magneto-optical applications.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS1998

Coupled Opto-Electronic Oscillators

These experiments demonstrate that COEOs are promising compact sources for generating low jitter optical pulses and low phase noise RF/millimeter wave signals.

opto-electronic oscillator (COEO) ring laser mode-↗
DOE OSTI2021

Broadband sum-frequency generation of spectrally incoherent pulses

We study and demonstrate the nonlinear frequency conversion of broadband optical pulses from 1053 nm to 351 nm using sum-frequency generation with a narrowband pulse at 526.5 nm. The combination of angular dispersion and noncollinearity cancels out the wave-vector mismatch and its frequency derivative, yielding an order-of-magnitude increase in spectral acceptance compared to conventional tripling. This scheme can support the nonlinear frequency conversion of broadband spectrally incoherent nanosecond pulses generated by high-energy lasers and optical parametric amplifiers to mitigate laser−plasma instabilities occurring during interaction with a target. The experimental results obtained with KDP crystals are in excellent agreement with modeling, demonstrating the generation of spectrally incoherent pulses with a bandwidth larger than 10 THz at 351 nm.

47 OTHER INSTRUMENTATION↗
NASA NTRS1981

X-ray spectra of the Crab pulsar and Nebula

The X-ray spectra of the Crab pulsar and Crab Nebula are analyzed. Observations were made with OSO 8 on March 17-18, 1978, with all spacecraft telemetry assigned to one detector during seven dwell mode experiments. A resolution of 1.25 ms was obtained for pulse-height-analyzed counts in 64 channels. Progressive hardening and subsequent softening of the spectrum across the pulse was found. The fraction of the pulsed flux, exhibiting a spectral variability of about 0.14 was concentrated solely in the region between the two peaks. A model is suggested in which the pulsed X-ray emission from the Crab pulsar consists of two components: one is physically related to the double-peaked gamma-ray pulse and possibly to radio and optical pulses, but has no spectral dependence on the pulse phase, while the other exhibits spectral variability with the pulse phase but is confined to the interpeak emission seen with X-ray energies.

Pravdo, S. H.↗
NASA NTRS1981

X-ray spectra of the Crab pulsar and nebula

The spectrum of the Crab pulsar was measued from 2 to 50 keV as a function of pulse phase and a progressive hardening and subsequent softening of the spectrum across the pulse was found. The fraction of the pulsed flux which exhibits spectral variability is 0.14 and is concentrated solely in the region between the two peaks. A model is suggested in which the pulsed X-ray emission from the Crab pulsar consists of two components: one which has no spectral dependence with pulse phase and which is physically related to the double peaked gama ray pulse and, perhaps, the radio and optical pulses; and another component which exhibits spectral variability with pulse phase is confined to and comprises the interpeak emission, and which is only seen at X-ray energies. These results and studies of the binary X-ray pulsar Hercules X-1 suggest a phenomonological similarity. If the spectrally varying component in the Crab pulsar arises from a hot, magnetized plasma near the neutron star surface then higher energy spectral observations of this phase region might reveal spectral features which can be used to determine the surface field strength.

Pravdo, S. H.↗
DOE OSTI2020

An ultrafast laser pulse picker technique for high-average-current high-brightness photoinjectors

Beam diagnostics in high brightness photoinjectors requires that optical pulses from a high-power drive laser be picked up with an ultrahigh pulse contrast ratio and without temporal profile distortion. In high-average-current high-brightness photoinjectors, high-power drive lasers are routinely operated at GHz-level pulse repetition rate and it is challenging to achieve pulse picking without any pulse distortion. Here, we report on a new ultrafast pulse picker technique for beam diagnostics in high-average-current high-brightness photoinjectors. By efficiently combining an ultrafast low-power electro-optic modulator, high-power fiber laser amplifiers, a high-power Pockels Cell, and a frequency doubling module, we have successfully demonstrated optical bunch (30 pulses per bunch) pickup from a 704 MHz high-power drive laser and achieved a 10 6 :1 pulse contrast ratio and nearly zero pulse distortion. The performance of this pulse picking technique has been verified through beam characterization and electron cooling in the low energy RHIC electron cooling accelerator at Brookhaven National Laboratory.

43 PARTICLE ACCELERATORS↗
DOE OSTI2021

Analysis of pump-to-signal noise transfer in two-stage ultra-broadband optical parametric chirped-pulse amplification

In optical parametric chirped-pulse amplification (OPCPA), pump temporal intensity modulation is transferred to the chirped-signal spectrum via instantaneous parametric gain and results in contrast degradation of the recompressed signal. We investigate, for the first time to our knowledge, the pump-to-signal noise transfer in a two-stage ultra-broadband OPCPA pumped by a single laser and show the dependence of pump-induced signal noise, characterized both before and after pulse compression, on the difference in pump-seed delay in the two stages. We demonstrate an up-to-15-dB reduction of the pump-induced contrast degradation via pump-seed delay optimization. Experiments and simulations show that, even when parametric amplifiers are operated in saturation, the pump-seed delay can be used to minimize the pump-induced contrast degradation that is attributed largely to the noises from the unsaturated edges of the pulse and that of the beam.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Excitation of optically trapped single particles using femtosecond pulses

Excitation from optically trapped particles is examined through laser-induced breakdown spectroscopy following interactions with mJ-level fs pulses. Optical emissions from sub-ng ablation of precisely positioned cupric oxide microparticles are used as a method to spatially resolve laser–particle interactions resulting in excitation. External focusing lenses are often used to change the dynamics of nonlinear self-focusing of fs pulses to form laser filaments or, alternatively, to form very intense air plasmas. Given the significant implications external focusing has on laser propagation and plasma conditions, single-particle emissions are studied with focusing lenses ranging from 50 to 300 mm. It is shown that, while single particles are less excited at longer focal lengths due to limited energy transfer through laser–particle interactions, the cooler plasma results in a lower thermal background to reveal resolved single-shot emission peaks. Furthermore, by developing an understanding in the fundamental interaction that occurs between single particles and fs pulses and filaments, practical improvements can be made for atmospheric remote sensing of low-concentration aerosols.

42 ENGINEERING↗
NASA NTRS1981

Ultrashort pulse generation in semiconductor lasers

Techniques to generate picosecond optical pulses from semiconductor lasers are reviewed. Experimental methods and results of theoretical analysis of active modelocking are presented. It is shown that modelocking will achieve the shortest pulses; but the use of a cumbersome external cavity will probably limit its practical use. Short pulses produced by direct modulation such as gain switching are considerably broader than those obtained by passive modelocking. However, no external cavity is needed; and the simplicity of this method makes it important to be explored further. Recent experimental results are discussed where picosecond pulses from a buried heterostructure laser diode with ultrashort current pulses obtained from a comb generator are generated. Also, 28 ps pulses were obtained at 2.5 GHz repetition frequency, using the gain switching method. An analytical analysis based on the rate equations shows qualitative agreement with our experimental results.

Auyeung, J.↗
NASA NTRS1972

Synchronization using pulsed edge tracking in optical PPM communication system

A pulse position modulated (PPM) optical communication system using narrow pulses of light for data transmission requires accurate time synchronization between transmitter and receiver. The presence of signal energy in the form of optical pulses suggests the use of a pulse edge tracking method of maintaining the necessary timing. The edge tracking operation in a binary PPM system is examined, taking into account the quantum nature of the optical transmissions. Consideration is given first to pure synchronization using a periodic pulsed intensity, then extended to the case where position modulation is present and auxiliary bit decisioning is needed to aid the tracking operation. Performance analysis is made in terms of timing error and its associated statistics. Timing error variances are shown as a function of system signal to noise ratio.

Gagliardi, R.↗
NASA NTRS1989

Does Supernova 1987A contain a rapidly vibrating neutron star?

If the recently reported 0.5 ms-period pulsed optical signal from the direction of Supernova 1987A originated in a young neutron star, its interpretation as a rotational period has difficulties. The surface magnetic field would have to be much lower than expected, and the high rotation rate may rule out preferred nuclear equations of state. It is pointed out here that a remnant radial vibration of a neutron star, excited in the supernova event, may survive for several years with about the observed (gravitationally redshifted) period. Heavy ions at the low-density stellar surface, periodically shocked by the vibration, may efficiently produce narrow pulses of optical cyclotron radiation in a surface field of about a trillion gauss.

Wang, Q.↗
NASA NTRS1989

Does SN 1987A contain a rapidly vibrating neutron star

If the recently reported 0.5 ms-period pulsed optical signal from the direction of Supernova 1987A originated in a young neutron star, its interpretation as a rotational period has difficulties. The surface magnetic field would have to be much lower than expected, and the high rotation rate may rule out preferred nuclear equations of state. It is pointed out here that a remnant radial vibration of a neutron star, excited in the supernova event, may survive for several years with about the observed (gravitationally redshifted) period. Heavy ions at the low-density stellar surface, periodically shocked by the vibration, may efficiently produce narrow pulses of optical cyclotron radiation in a surface field of about a trillion gauss.

Wang, Q.↗
DOE OSTI2022

Ultrafast nonlinear absorption of TMDC quantum dots

Here, we study theoretically absorption properties of MoS 2 quantum dots placed in an ultrashort and strong optical pulse with the duration of a few femtoseconds and the amplitude up to 1.5 V/Å. While the monolayer of MoS 2 has a bandgap of ≈ 1.8 eV, the quantum dots of MoS 2 have in-gap edge states, which open additional absorption channels. The absorbance of the system strongly depends on the amplitude of the pulse. At small amplitude, less than 0.5 V/Å, the absorbance varies by more than 20% with the frequency of the pulse. The system shows saturable absorption if the frequency of the pulse is larger than the bulk bandgap and reverse saturable absorption if the frequency of the pulse is in the bandgap. At large amplitudes, > 0.5 V/Å, of the pulse, the ultrafast absorbance of a quantum dot has a weak dependence on the pulse frequency. If the frequency of the pulse is less than the corresponding bulk bandgap, the absorbance has a nonmonotonic dependence on the pulse amplitude with the maximum at ≈ 0.5 V/Å. We also present the results for QDs of different TMDC materials, which show that at large field amplitude, > 0.5 V/Å, the absorbance is universal and has weak dependence on the type of TMDC.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Optical parametric amplification of spectrally incoherent pulses

The optical parametric amplification of spectrally incoherent signals is analyzed and simulated using a set of normalized equations describing phase-matched three-wave nonlinear mixing. Varying the amplifier’s properties and the seeding conditions reveals different amplification regimes. In particular, the relative temporal walk-off of the signal, idler, and pump has a strong impact on the temporal and spectral properties of the amplified signal. The amplification efficiency for spectrally incoherent signals is not significantly lower than that of a coherent monochromatic signal, provided that the phase-matching bandwidth is sufficient. Here, the results obtained with the normalized set of equations are in good agreement with simulations based on the full description of the crystals’ dispersion for high-gain LBO and BBO preamplifiers and a low-gain DKDP power amplifier.

47 OTHER INSTRUMENTATION↗
DOE OSTI2020

Subnanosecond phase transition dynamics in laser-shocked iron

Iron is one of the most studied chemical elements due to its sociotechnological and planetary importance; hence, understanding its structural transition dynamics is of vital interest. By combining a short pulse optical laser and an ultrashort free electron laser pulse, we have observed the subnanosecond structural dynamics of iron from high-quality x-ray diffraction data measured at 50-ps intervals up to 2500 ps. We unequivocally identify a three-wave structure during the initial compression and a two-wave structure during the decaying shock, involving all of the known structural types of iron (α-, γ-, and ε-phase). In the final stage, negative lattice pressures are generated by the propagation of rarefaction waves, leading to the formation of expanded phases and the recovery of γ-phase. Our observations demonstrate the unique capability of measuring the atomistic evolution during the entire lattice compression and release processes at unprecedented time and strain rate.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗