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Mechanistic insights into selective oxidation and corrosion of multi-principal element alloys from high resolution and in situ microscopy
Multiple principal elements alloys (MPEAs) have drawn significant recent interest from the metallurgical research community. These novel alloys have the potential to replace traditional alloys with a range of tailored mechanical properties, corrosion resistance, and radiation tolerance enabled by complex compositions. The broad alloy design space of MPEAs presents a great opportunity to discover new forms of oxidation and corrosion resistance in extreme environments that break away from conventional corrosion resistant alloy design criteria. However, understanding the oxidation and corrosion response of MPEAs can be a challenging task due the complex composition, structural, and chemical state changes occurring in the corrosion product and at its interface with the base alloy. This perspective discusses the utility of high resolution and in situ microscopy techniques for revealing unique aspects of MPEA oxidation behavior at the near-atomic level. Challenges of studying these alloys and several open questions are presented.
Multi-layered polymerized high internal phase emulsions with controllable porosity and strong interf
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Wave energy resources assessment for the multi-modal sea state of Hawaii
This paper describes development and validation of a 32-year wave hindcast for Hawaii as part of the wave energy resources assessment for the Exclusive Economic Zones of the US and affiliated territories. The nested model system comprises structured WAVEWATCH III models for the entire globe and the Central North Pacific as well as an unstructured SWAN model around the Hawaiian Islands with wind forcing from the Global Forecast System Reanalysis and its regional downscaling. The development effort follows the standards introduced by the International Electrotechnical Commission (IEC). The hindcast dataset was firstly validated with buoy measurements in terms of the six IEC wave energy resources parameters including the omnidirectional wave power ????, significant wave height ????????0, energy period ????????, spectral width ????0, direction of maximum directionally resolved wave power ?????????? ????????, and directionality coefficient ????. The comparison shows good overall agreement but with greater uncertainties for the spectral parameters ????0, ???????????????????? , and ???? formulated for narrow band spectra. The multimodal sea state in Hawaii always includes a mix of short-period wind seas, long-period swells from the North and South Pacific as well as waves with moderate periods from multiple sources. We partition the hindcast spectra based on the respective period ranges and directions and validate the partitioned spectral energy and parameters with measured values for implementation in wave energy resources assessment. The partitioned wave parameters from the hindcast allow separate seasonal descriptions of wind seas, north and south swells, and moderate-period waves for in-depth understanding of the wave climate and resources in Hawaii.
Multi-decade high-resolution regional hindcasts for wave energy resource characterization in U.S. coastal waters
Long-term, high-resolution, regional wave hindcast datasets were generated using unstructured-grid Simulating WAves Nearshore (SWAN) models for the U.S. coastal waters to support nearshore wave energy development in the U.S. including those bordering U.S. territorial islands. The model domains resolved the entire U.S. exclusive economic zones, with a spatial resolution of approximately 200 m nearshore. The regional SWAN models were driven by the global WAVEWATCH III® model outputs and run for a 42-year period from 1979 to 2020. Extensive model validations were performed using buoy observations and altimeter data. Regional resource characterization was performed based on hindcast data points at 2 km from shore and along the 100 m isobath. Aggregations of wave resource parameters were produced, and spatial and seasonal variations were analyzed for all the regions. Wave resource metrics recommended by international standards, including a 3-hour time series of six resource parameters, hourly frequency- and directionally resolved wave spectra at selected “virtual buoy” locations, and average-annual values of omni-directional wave power, significant wave height, and energy period are publicly disseminated through an Amazon Web Service and a Marine Energy Atlas web application tool to facilitate wave energy research and a wide range of coastal ocean applications.
Multi-source information fusion to assess control room operator performance
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Microscopy-based Multi-technique, Multi-scale Characterization of Polymer Electrolyte Membrane Devices
This paper will cover recent developments of both fuel cell and electrolyzer catalysts and catalyst layers, and the vital role of each technique in obtaining a comprehensive picture of how to improve constituent interactions within the device.
Life-Cycle Emissions and Human Health Implications of Multi-Input, Multi-Output Biorefineries
To meaningfully broaden the supply of fuels for the transportation sector, biofuel production must be scaled up and this requires a wider array of biomass feedstocks, including agricultural residues and organic waste. Rather than pursuing conversion of lignocellulosic biomass to fuels and anaerobic digestion of wastes as separate pathways, there are economic and environmental advantages associated with integrating these processes in a single facility. However, existing research rarely goes beyond carbon footprints in quantifying the effects of such a shift in bioenergy production. In addition to CO2, CH4, and N2O, this study explores the life-cycle air pollution (NH3, volatile organic compounds, NOx, SO2, and PM2.5), marine eutrophication, acidification, and local external cost implications of biorefineries capable of taking in crop residues, food waste, and manure to produce liquid fuel, electricity, and/or other options such as renewable natural gas (RNG), hydrogen, bioplastics, and protein-rich livestock feed. Relative to a single-input, single-output baseline, biorefineries integrated with organic waste codigestion to coproduce electricity or RNG can reduce life-cycle CO2-equivalent emissions by 84-149%, and the monetized external impacts across all scenarios range from $1.07/gallon to -$0.75/gallon ethanol.
Characterizing the Mechanisms of Ca and Mg Carbonate Ion-Pair Formation with Multi-Level Molecular Dynamics/Quantum Mechanics Simulations
The carbonate minerals of Ca and Mg are abundant throughout the lithosphere and have recently garnered significant research interest as possible long-term carbon sinks in the sequestration of atmospheric carbon dioxide. Nonetheless, an understanding of the atomic-level processes comprising their mineralization remains limited. Furthermore, we characterize and contrast the mechanisms of contact ion-pair formation in aqueous Ca and Mg carbonate systems, which represents the most fundamental step leading to the formation of their mineral solids. Utilizing multilevel embedded correlated wavefunction-based ab initio molecular dynamics/quantum mechanics simulations, we characterize not only the dynamics of these processes but also factors arising from the electronic structure of the involved species, revealing further details of the fundamentally different mechanisms for the interconversion between the contact ion-pairs and solvent-shared ion-pairs of Ca versus Mg carbonate.
Chemical and Conformational Control of the Spectroscopic Properties of Multi-Layer and Multi-Defect Carbon Dots
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Engineering Organization of DNA Nano-Chambers through Dimensionally Controlled and Multi-Sequence Encoded Differentiated Bonds
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Identification of beneficial and detrimental bacteria impacting sorghum responses to drought using multi-scale and multi-system microbiome comparisons
Abstract Drought is a major abiotic stress limiting agricultural productivity. Previous field-level experiments have demonstrated that drought decreases microbiome diversity in the root and rhizosphere. How these changes ultimately affect plant health remains elusive. Toward this end, we combined reductionist, transitional and ecological approaches, applied to the staple cereal crop sorghum to identify key root-associated microbes that robustly affect drought-stressed plant phenotypes. Fifty-three Arabidopsis-associated bacteria were applied to sorghum seeds and their effect on root growth was monitored. Two Arthrobacter strains caused root growth inhibition (RGI) in Arabidopsis and sorghum. In the context of synthetic communities, Variovorax strains were able to protect plants from Arthrobacter-caused RGI. As a transitional system, high-throughput phenotyping was used to test the synthetic communities. During drought stress, plants colonized by Arthrobacter had reduced growth and leaf water content. Plants colonized by both Arthrobacter and Variovorax performed as well or better than control plants. In parallel, we performed a field trial wherein sorghum was evaluated across drought conditions. By incorporating data on soil properties into the microbiome analysis, we accounted for experimental noise with a novel method and were able to observe the negative correlation between the abundance of Arthrobacter and plant growth. Having validated this approach, we cross-referenced datasets from the high-throughput phenotyping and field experiments and report a list of bacteria with high confidence that positively associated with plant growth under drought stress. In conclusion, a three-tiered experimental system successfully spanned the lab-to-field gap and identified beneficial and deleterious bacterial strains for sorghum under drought.
Correction: Identification of beneficial and detrimental bacteria impacting sorghum responses to drought using multi-scale and multi-system microbiome comparisons
Correction to: The ISME Journal, published online 6 May 2022 In this article the author name Kira M. Veley was incorrectly written as Kira W. Veley. The original article has been corrected.
Multi-scale chemo-mechanical evolution during crystallization of mixed conducting SrTi[subscript 0.6
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