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At least 145 records · Page 8

Development of a two photon/laser induced fluorescence technique for the detection of atmospheric OH radicals

The development of a new mid-IR laser source was the primary goal. Backward propagating stimulated D2 Raman frequency down conversion of a commercially available 1.06 micron Nd:YAG laser was shown to generate an efficient source of 1.56 micron radiation with near diffraction limited beam quality. The efficient generation of a 2.9 micron laser source was also achieved using backward propagating CH4 Raman frequency down conversion of the 1.56 micron pump. Slightly higher efficiencies were obtained for frequency down conversion of the 1.06 micron Nd:YAG using the H2 Raman shift yielding a near diffraction limited source in the 200 mJ range at 1.9 micron. Similar conversion efficiencies are anticipated as a result of extending the wavelength coverage of recently available Ti:sapphire pulse laser to not only cover the 740 to 860 nm fundamental wavelength range but also the .95 to 1.15 and 1.06 to 1.33 micron range using D2 and H2, respectively. The anticipated sensitivity of a TP-LIF OH sensor using this mid-IR source would give signal limited detection of 1.4 x 10(exp 5) OH/cu cm under boundary layer conditions and 5.5 x 10(exp 4) OH/cu cm under free troposphere sampling conditions for a five minute signal integration period. This level of performance coupled with the techniques non-perturbing nature and freedom from both interferences and background would allow reliable tropospheric OH measurement to be obtained under virtually any ambient condition of current interest, including interstitial and sampling.

Bradshaw, John↗

Infrared Pulse-laser Long-path Absorption Measurement of Carbon Dioxide Using a Raman-shifted Dye Laser

A pulsed laser source is effective in infrared laser long-path absorption measurements when the optical path length is very long or the reflection from a hard target is utilized, because higher signal-to-noise ratio is obtained in the detection of weak return signals. We have investigated the performance of a pulse-laser long-path absorption system using a hydrogen Raman shifter and a tunable dye laser pumped by a Nd:YAG laser, which generates second Stokes radiation in the 2-micron region.

Minato, Atsushi↗

Filtered Rayleigh scattering measurements in supersonic/hypersonic facilities

Preliminary measurements are presented of flow field properties in Mach 3 and Mach 5 flows using filtered Rayleigh scattering. Filter properties have been characterized by high resolution spectroscopy in order to optimize the selection of laser frequency and filter operating conditions, as well as for the development of an accurate filter modeling program. An optimized filter is used the background suppression feature of this technique to image the boundary layer structure in a Mach 3 high Reynolds number facility and the shock structure in a Mach 5 overexpanded jet. This had been achieved using a visible laser source. By frequency scanning the laser, time-averaged velocity measurements in the Mach 3 and Mach 5 flows are made. Data acquisition at 10 torr and below indicates that this approach can be extrapolated for use in hypersonic flow facilities and is applicable as an in-flight optical air data device for hypersonic vehicles.

Miles, Richard B.↗

Two-Photon/Laser-Induced Fluorescence (TP/LIF) sensor

The Two-Photon/Laser-Induced Fluorescence (TP/LIF) technique is based on the stepwise excitation of the OH transitions, X(exp 2)II, v(exp '') = 0 yields X(exp 2)II, v(exp '') = 1 (lambda = 2.9 microns) and X(exp 2)II v(exp '') = 1 yields A(exp2)Sigma, v' = 0 (lambda = 345 nm) with background free fluorescence monitoring of the A(exp 2)Sigma, v' = 0 yields X(exp 2)II, v(exp '') = 0 transition near 309 nm. This technique has awaited the advent of a suitable mid-infrared (2.9 microns) laser source. Turnable mid-IR lasers now exist that are capable of meeting the specifications required of a high sensitivity TP/LIF OH sensor.

Bradshaw, John D.↗

Real-Time Thermographic-Phosphor-Based Temperature Measurements of Thermal Barrier Coating Surfaces Subjected to a High-Velocity Combustor Burner Environment

Surface temperature measurements were conducted on metallic specimens coated with an yttria-stabilized zirconia (YSZ) thermal barrier coating (TBC) with a YAG:Dy phosphor layer that were subjected to an aggressive high-velocity combustor burner environment. Luminescence-based surface temperature measurements of the same TBC system have previously been demonstrated for specimens subjected to static furnace or laser heating. Surface temperatures were determined from the decay time of the luminescence signal of the YAG:Dy phosphor layer that was excited by a pulsed laser source. However, the furnace and laser heating provides a much more benign environment than that which exists in a turbine engine, where there are additional challenges of a highly radiant background and high velocity gases. As the next step in validating the suitability of luminescence-based temperature measurements for turbine engine environments, new testing was performed where heating was provided by a high-velocity combustor burner rig at Williams International. Real-time surface temperature measurements during burner rig heating were obtained from the decay of the luminescence from the YAG:Dy surface layer. The robustness of several temperature probe designs in the sonic velocity, high radiance flame environment was evaluated. In addition, analysis was performed to show whether the luminescence decay could be satisfactorily extracted from the high radiance background.

Eldridge, Jeffrey I.↗

Experiments with Lasers and Frequency Doublers

Solid state laser sources, such as diode-pumped Nd:YAG lasers, have given us CW laser light of high power with unprecedented stability and low noise performance. In these lasers most of the technical sources of noise can be eliminated allowing them to be operated close to the theoretical noise limit set by the quantum properties of light. The next step of reducing the noise below the standard limit is known as squeezing. We present experimental progress in generating reliably squeezed light using the process of frequency doubling. We emphasize the long term stability that makes this a truly practical source of squeezed light. Our experimental results match noise spectra calculated with our recently developed models of coupled systems which include the noise generated inside the laser and its interaction with the frequency doubler. We conclude with some observations on evaluating quadrature squeezed states of light.

Bachor, H.-A.↗

FAST-GREENS: A High Efficiency Free Electron Laser Driven by Superconducting RF Accelerator

In this paper we’ll describe the FAST-GREENS experimental program where a 4 m-long strongly tapered helical undulator with a seeded prebuncher is used in the high gain TESSA regime to convert a significant fraction (up to 10 %) of energy from the 240 MeV electron beam from the FAST linac to coherent 515 nm radiation. We’ll also discuss the longer term plans for the setup where by embedding the undulator in an optical cavity matched with the high repetition rate from the superconducting accelerator (3,9 MHz), a very high average power laser source can be obtained. Eventually, the laser pulses can be redirected onto the relativistic electrons to generate by inverse compton scattering a very high flux of circularly polarized gamma rays for polarized positron production.

43 PARTICLE ACCELERATORS↗

Development of an airborne laser bathymeter

An airborne laser depth sounding system was built and taken through a complete series of field tests. Two green laser sources were tried: a pulsed neon laser at 540 nm and a frequency-doubled Nd:YAG transmitter at 532 nm. To obtain a depth resolution of better than 20 cm, the pulses had a duration of 5 to 7 nanoseconds and could be fired up to at rates of 50 pulses per second. In the receiver, the signal was detected by a photomultiplier tube connected to a 28 cm diameter Cassegrainian telescope that was aimed vertically downward. Oscilloscopic traces of the signal reflected from the sea surface and the ocean floor could either be recorded by a movie camera on 35 mm film or digitized into 500 discrete channels of information and stored on magnetic tape, from which depth information could be extracted. An aerial color movie camera recorded the geographic footprint while a boat crew of oceanographers measured depth and other relevant water parameters. About two hundred hours of flight time on the NASA C-54 airplane in the area of Chincoteague, Virginia, the Chesapeake Bay, and in Key West, Florida, have yielded information on the actual operating conditions of such a system and helped to optimize the design. One can predict the maximum depth attainable in a mission by measuring the effective attenuation coefficient in flight. This quantity is four times smaller than the usual narrow beam attenuation coefficient. Several square miles of a varied underwater landscape were also mapped.

Kim, H., H.↗

Plasma lasers (a strong source of coherent radiation in astrophysics)

The generation of electromagnetic radiation from the free energy available in electron streams is discussed. The fundamental principles involved in a particular class of coherent plasma radiation sources, i.e., plasma lasers, are reviewed, focusing on three wave coupling, nonlinear parametric instabilities, and negative energy waves. The simplest case of plasma lasers, that of an unmagnetized plasma containing a finite level of density fluctuations and electrons streaming with respect to the ions, is dealt with. A much more complicated application of plasma lasers to the case of auroral kilometric radiation is then examined. The concept of free electron lasers, including the role of relativistic scattering, is elucidated. Important problems involving the escape of the excited radiation from its generation region, effects due to plasma shielding and nonlinear limits, are brought out.

Papadopoulos, K.↗

Laser induced spark ignition of methane-oxygen mixtures

Results from an experimental study of laser induced spark ignition of methane-oxygen mixtures are presented. The experiments were conducted at atmospheric pressure and 296 K under laminar pre-mixed and turbulent-incompletely mixed conditions. A pulsed, frequency doubled Nd:YAG laser was used as the ignition source. Laser sparks with energies of 10 mJ and 40 mJ were used, as well as a conventional electrode spark with an effective energy of 6 mJ. Measurements were made of the flame kernel radius as a function of time using pulsed laser shadowgraphy. The initial size of the spark ignited flame kernel was found to correlate reasonably well with breakdown energy as predicted by the Taylor spherical blast wave model. The subsequent growth rate of the flame kernel was found to increase with time from a value less than to a value greater than the adiabatic, unstretched laminar growth rate. This behavior was attributed to the combined effects of flame stretch and an apparent wrinkling of the flame surface due to the extremely rapid acceleration of the flame. The very large laminar flame speed of methane-oxygen mixtures appears to be the dominant factor affecting the growth rate of spark ignited flame kernels, with the mode of ignition having a small effect. The effect of incomplete fuel-oxidizer mixing was found to have a significant effect on the growth rate, one which was greater than could simply be accounted for by the effect of local variations in the equivalence ratio on the local flame speed.

Santavicca, D. A.↗

Studying AC-LGAD strip sensors from laser and testbeam measurements

Here, this paper presents the setup assembled to characterize and measure the spatial and timing resolutions of AC-coupled Low Gain Avalanche Diodes (AC-LGADs), using a 1060 nm laser source to deposit initial charges with a defined calibration methodology. The results were compared to those obtained with a 120 GeV proton beam. Despite the differences in the charge deposition mechanism between the laser and proton beam, the spatial and temporal resolutions were found to be compatible between the two sources after calibration. With 4D tracking detectors expected to play a vital role in upcoming collider experiments, we foresee this work as a way to evaluate the performance of semiconductor sensors that can augment testbeam measurements and accelerate R&D efforts. Additionally, simulation studies using Silvaco TCAD and Weightfield2 were carried out to understand the various contributing factors to the total time resolution in AC-LGAD sensors, measured using the laser source.

FOS: Physical sciences↗

High-Resolution Laser Spectroscopy on the Hyperfine Structure of 255Fm (𝑍=100)

We report on high-resolution laser spectroscopy of 255Fm (𝑇1/2=20 h), one of the heaviest nuclides available from reactor breeding. The hyperfine structures in two different atomic ground-state transitions at 398.4 nm and 398.2 nm were probed by in-source laser spectroscopy at the RISIKO mass separator in Mainz, using the perpendicularly illuminated laser ion source and trap (PI-LIST) high-resolution ion source. Experimental results were combined with hyperfine fields from various atomic ab initio calculations, in particular using multiconfiguration Dirac-Hartree-Fock theory, as implemented in grasp18. In this manner, the nuclear magnetic dipole and electric quadrupole moments were derived to be 𝜇=−0.75⁢(5) 𝜇N and 𝑄s=+5.84⁢(13) eb, respectively. The magnetic moment indicates occupation of the 𝜈⁢7/2⁢[613] Nilsson orbital, while the large quadrupole moment confirms strong, stable prolate deformation consistent with systematics in the heavy actinides. Comparisons with available expectation values from nuclear theory show good agreement, providing a stringent benchmark for the used theoretical models. These results revise earlier data and establish 255Fm as a reference isotope for future high-resolution studies.

Ezold, Julie [ORNL] (ORCID:0000000250550022)↗

Semiconductor Laser Low Frequency Noise Characterization

This work summarizes the efforts in identifying the fundamental noise limit in semiconductor optical sources (lasers) to determine the source of 1/F noise and it's associated behavior. In addition, the study also addresses the effects of this 1/F noise on RF phased arrays. The study showed that the 1/F noise in semiconductor lasers has an ultimate physical limit based upon similar factors to fundamental noise generated in other semiconductor and solid state devices. The study also showed that both additive and multiplicative noise can be a significant detriment to the performance of RF phased arrays especially in regard to very low sidelobe performance and ultimate beam steering accuracy. The final result is that a noise power related term must be included in a complete analysis of the noise spectrum of any semiconductor device including semiconductor lasers.

SEMICONDUCTOR LASERS↗

Gain Stability of Hamamatsu R5912-MOD Photo-Multipliers at Low Temperature

The Photon Detection System is a crucial component of the ICARUS detector in the Short Baseline Neutrino (SBN) Program at Fermi National Accelerator Laboratory (FNAL). It consists of 360 Photo Multiplier Tubes (PMTs) 8” Hamamatsu R5912-MOD and, since June 2020, it has been operated at the liquid Argon cryogenic temperature. During these years, the PMTs have shown gain losses as an aging effect. Using a climatic chamber at the INFN Sezione di Catania, we confirmed a stable gain for a single PMT 8” Hamamatsu 5912-MOD when operated at room temperature, and a persistent gain loss at temperatures around -70°C, although far from the liquid Argon one. No gain recovery was obtained bringing the PMT back to room temperature. We suspect that dynode deterioration due to temperature gradient plays a significant role in this phenomenon. During our test, the PMT was illuminated by a 520 nm laser source and operated in current mode. The laser beam was split into two optical fibers, the first one transmitting light through Neutral Density filters and then diffusing it over the surface of the PMT photocathode. The other optical fiber was used for an independent reference measurement of the injected light via a bolometric photodetector. In this presentation, the main technical characteristics of the measurement system are shown together with preliminary results which need further investigation to elucidate the underlying mechanisms driving the gain loss and to propose new mitigation strategies.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Simple technique for sequential Q-switching of molecular lasers.

A simple technique for sequentially Q-switching molecular lasers is discussed in which an optical scanner is used as an optical folding element in a laser cavity consisting of a stationary diffraction grating and partially reflecting mirror. Sequential Q-switching of a conventional CO2 laser is demonstrated in which over sixty-two transitions between 9.2 and 10.8 microns are observed. Rapid repetition rates (200 Hz) and narrow laser pulses (less than 5 microsec) allow conventional signal processing techniques to be used with this multiwavelength laser source which is a versatile tool for laser propagation studies, absorption spectroscopy, and gain measurements. Results of a preliminary experiment demonstrating the utility of measuring selective absorption of CO2 laser wavelengths by C2H4 are shown.

Lucht, R. A.↗

Radiation sensitive area detection device and method

A radiation sensitive area detection device for use in conjunction with an X ray, ultraviolet or other radiation source is provided which comprises a phosphor containing film which releases a stored diffraction pattern image in response to incoming light or other electromagnetic wave. A light source such as a helium-neon laser, an optical fiber capable of directing light from the laser source onto the phosphor film and also capable of channelling the fluoresced light from the phosphor film to an integrating sphere which directs the light to a signal processing means including a light receiving means such as a photomultiplier tube. The signal processing means allows translation of the fluoresced light in order to detect the original pattern caused by the diffraction of the radiation by the original sample. The optical fiber is retained directly in front of the phosphor screen by a thin metal holder which moves up and down across the phosphor screen and which features a replaceable pinhole which allows easy adjustment of the resolution of the light projected onto the phosphor film. The device produces near real time images with high spatial resolution and without the distortion that accompanies prior art devices employing photomultiplier tubes. A method is also provided for carrying out radiation area detection using the device of the invention.

Carter, Daniel C.↗

Every Good Virtue You Ever Wanted in a Q-switched Solid-state Laser and More: Monolithic, Diode-pumped, Self-q-switched, Highly Reproducible, Diffraction-limited Nd:yag Laser

The applications of Q-switched lasers are well known, for example, laser radar, laser remote sensing, satellite orbit determination, Moon orbit and 'moon quake' determination, satellite laser communication, and many nonlinear optics applications. Most of the applications require additional properties of the Q-switched lasers, such as single-axial and/or single-transverse mode, high repetition rate, stable pulse shape and pulse width, or ultra compact and rugged oscillators. Furthermore, space based and airborne lasers for lidar and laser communication applications require efficient, compact, lightweight, long-lived, and stable-pulsed laser sources. Diode-pumped solid-state lasers (DPSSL) have recently shown the potential for satisfying all of these requirements. We will report on the operating characteristics of a diode-pumped, monolithic, self-Q-switched Cr,Nd:YAG laser where the chromium ions act as a saturable absorber for the laser emission at 1064 nm. The pulse duration is 3.5 ns and the output is highly polarized with an extinction ratio of 700:1. It is further shown that the output is single-longitudinal-mode with transform-limited spectral line width without pulse-to-pulse mode competition. Consequently, the pulse-to-pulse intensity fluctuation is less than the instrument resolution of 0.25 percent. This self-stabilization mechanism is because the lasing mode bleaches the distributed absorber and establishes a gain-loss grating similar to that used in the distributed feedback semiconductor lasers. A repetition rate above 5 KHz has also been demonstrated. For higher power, this laser can be used for injection seeding an amplifier (or amplifier chain) or injection locking of a power oscillator pumped by diode lasers. We will discuss some research directions on the master oscillator for higher output energy per pulse as well as how to scale the output power of the diode-pumped amplifier(s) to multi-kilowatt average power.

Chen, Y. C.↗

Approaching the Lower Temporal Limit of Laser‐Produced Plasma Sources for Table‐Top Soft X‐Ray NEXAFS Measurements

Abstract The increasing popularity of time‐resolved X‐ray absorption measurements for understanding dynamics in molecular and material systems has led to many advances in table‐top sources for pulsed X‐rays. We report on a table‐top laser‐produced plasma (LPP) source that can perform soft X‐ray (SXR), near‐edge X‐ray absorption fine structure (NEXAFS) measurements using a laser source with 23 ps pulse duration. The spectrometer's key specifications, such as brilliance, resolution, and stability, are characterized against the more commonly used longer‐pulse‐duration LPP sources. The 23 ps laser produced approximately an order of magnitude weaker SXR flux than the 8 ns laser for a higher power density due to the smaller total energy absorbed by the plasma. The increased repetition rate, as well as the use of a high line‐density X‐grating, and a self‐referencing scheme still allowed for NEXAFS measurements of Si 3 N 4 and TiO 2 thin films with 2.5 minute acquisition times, a resolving power of E/ΔE=424, and a signal‐to‐noise ratio of 100. It was observed that degradation of the gas jet nozzle led to long‐term instability of the source, which can be remediated using alternative nozzle designs. This work demonstrates the feasibility of achieving higher temporal resolution in future time‐resolved X‐ray absorption measurements using table‐top LPP sources.

Nimlos, Danika [Division of Chemistry and Chemical↗